Micro-Scale Variability of Atmospheric Particle Concentration in the Urban Boundary Layer
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Micro-scale variability of atmospheric particle concentration in the urban boundary layer Kumulative Dissertation zur Erlangung des akademischen Grades doctor rerum naturalium Dr. rer. nat. im Fach Geographie eingereicht an der Mathematisch-Naturwissenschaftlichen Fakultät der Humboldt-Universität zu Berlin von M.Sc. Bastian Paas Präsidentin der Humboldt-Universität zu Berlin: Prof. Dr.-Ing. Dr. Sabine Kunst Dekan der Mathematisch-Naturwissenschaftlichen Fakultät: Prof. Dr. Elmar Kulke Gutachter: 1. Prof. Dr. Christoph Schneider 2. Prof. Dr. Wilfried Endlicher 3. Prof. Dr. Stefan Weber Tag der mündlichen Prüfung: 07.12.2017 III List of publications This thesis is presented in a cumulative form and is based on the following citation-indexed and peer-reviewed journal papers: I. Paas, B., Schmidt, T., Markova, S., Maras, I., Ziefle, M., & Schneider, C. (2016). Small-scale variability of particulate matter and perception of air quality in an inner-city recreational area in Aachen, Germany. Meteorologische Zeitschrift, 25(3), 305–317. https://doi.org/10.1127/metz/2016/0704 II. Paas, B. & Schneider, C. (2016). A comparison of model performance between ENVI-met and Austal2000 for particulate matter. Atmospheric Environment, 145, 392–404. https://doi.org/10.1016/j.atmosenv.2016.09.031 III. Paas, B., Stienen, J., Vorländer, M., & Schneider, C. (2017). Modeling of Urban Near-Road Atmospheric PM Concentrations Using an Artificial Neural Network Approach with Acoustic Data Input. Environments 2017, 4(2), 26. https://doi.org/10.3390/environments4020026 I: Distributed under the Creative Commons BY-NC 4.0 license. II: This paper is reprinted with permission of “Atmospheric Environment”, Elsevier Ltd. III: Distributed under the Creative Commons BY 4.0 license. IV The author made the following contributions to the journal papers on which this thesis is based: I. Responsible for the study design, the fieldwork (except for the survey), the modeling (except for the CAD pre-work) and numerical simulations, the data preparation, the data analysis, all figures, the literature review, and the writing (except for a few lines regarding the survey) II. Responsible for the study design, the fieldwork, the modeling and numerical simulations, the data preparation, the data analysis, all figures, the literature review, and the entire writing III. Responsible for the study design, the fieldwork (except for microphone calibrations), the model development and testing, the data preparation (except for acoustic raw data pre-processing), the data analysis, all figures, the literature review, and the entire writing V The author also contributed to the following full paper publications (conference proceedings or peer-reviewed journal papers) related to the thesis, which are, however, of minor relevance to the thesis itself: i. Stienen, J., Schmidt, T., Paas, B., Schneider, C., & Fels, J. (2014). Evaluation of combined stress factors on humans in urban areas. Proceedings of TECNIACUSTICA 2014, 45th Spanish Congress on Acoustics, 8th Iberian Congress on Acoustics, European Symposium on smart cities and environmental acoustics. Murcia, Spain. ii. Stienen, J., Schmidt, T., Paas, B., & Fels, J. (2015). Noise as a Stress Factor on Humans in Urban Environments in Summer and Winter. In Proceedings of the EuroNoise 2015. Maastricht, Netherlands, 2445-2450. iii. Schmidt, T., Maras, I., Paas, B., Stienen, J., & Ziefle, M. (2015). Psychophysical observations on human perceptions of climatological stress factors in an urban environment. Proceedings of the 19th Triennial Congress of the IEA. Melbourne, Australia, 1-8. iv. Maras, I., Schmidt, T., Paas, B., Ziefle, M., & Schneider, C. (2016). The impact of human-biometeorological factors on perceived thermal comfort in urban public places. Meteorologische Zeitschrift, 25(4), 407–420. https://doi.org/10.1127/metz/2016/0705 v. Daniels, B., Zaunbrecher, B., Paas, B., Ottermanns, R., Ziefle, M., & Roß-Nickoll, M. (2017). Assessment of urban green space structures and their quality from a multidimensional perspective. In a review for Science of the Total Environment1. 1Ms. Ref. No.: STOTEN-D-17-04181 VI Contents List of publications .................................................................................................... III Contents ...................................................................................................................... VI Abbreviations .......................................................................................................... VIII Figures ............................................................................................................................X Tables ........................................................................................................................ XIV Abstract ....................................................................................................................... XV Zusammenfassung ................................................................................................. XVI 1. Introduction ............................................................................................................ 1 1.1 Structure of the thesis ................................................................................................... 1 1.2 Perspective ....................................................................................................................... 3 1.3 Case study environments ............................................................................................. 6 1.4 Framework ....................................................................................................................... 8 1.5 Research questions ...................................................................................................... 10 1.6 Objectives & related approaches ............................................................................. 11 2. The field experiment analysis ........................................................................... 13 2.1 Context and motivation to carry out field experiments .................................... 13 2.2 Study design .................................................................................................................. 14 2.2.1 Areas under study ........................................................................................ 14 2.2.2 Particle concentration measurements .................................................... 16 2.2.3 Survey ............................................................................................................. 16 2.3 Micro-scale distribution of particles ....................................................................... 17 2.4 Perception of particle exposure ............................................................................... 18 3. Deterministic modeling of particle distribution in the urban ABL .......... 21 3.1 Context. .......................................................................................................................... 21 3.2 Analysis of model performance between ENVI-met and Austal2000 ............ 23 3.2.1 Motivation for the model performance assessment ............................ 23 3.2.2 Study design .................................................................................................. 24 3.2.3 Performance analysis .................................................................................. 27 3.3 Particle emissions out of resuspension sources ................................................... 32 VII 3.3.1 Motivation to quantify resuspension source emissions using Austal2000 ...................................................................................................... 32 3.3.2 Methods .......................................................................................................... 32 3.3.3 Main results ................................................................................................... 33 3.4 Influence of vegetation elements on ground-level aerosol concentrations .. 36 3.4.1 Motivation ...................................................................................................... 36 3.4.2 Methodical approach ................................................................................... 36 3.4.3 Main results ................................................................................................... 38 3.5 Summary ........................................................................................................................ 39 4. Prediction of particle concentrations using a newly developed statistical model ....................................................................................................................... 41 4.1 Context and motivation to develop an ANN model ........................................... 41 4.2 Concept .......................................................................................................................... 42 4.2.1 Areas of investigation ................................................................................. 42 4.2.2 ANN model development strategy .......................................................... 44 4.2.3 Performance measures ................................................................................ 46 4.3 Performance evaluation of the developed ANN models .................................... 47 5. Conclusions and outlook ...................................................................................