Charge States of Relativistic Heavy Ions in Matter

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Charge States of Relativistic Heavy Ions in Matter Nuclear Instruments and Methods in Physics Research B 142 (1998) 441±462 Charge states of relativistic heavy ions in matter C. Scheidenberger a,*, Th. Stohlker a, W.E. Meyerhof b, H. Geissel a, P.H. Mokler a, B. Blank c a Gesellschaft fur Schwerionenforschung, Planckstrasse 1, 64291 Darmstadt, Germany b Department of Physics, Stanford University, CA 94305, USA c Centre d'Etudes Nucleaires de Bordeaux, 33175 Gradignan, France Received 5 January 1998 Abstract Experimental and theoretical results on charge-exchange cross-sections and charge-state distributions of relativistic heavy ions penetrating through matter are presented. The data were taken at the Lawrence Berkeley Laboratory's BEVALAC accelerator and at the heavy-ion synchrotron SIS of GSI in Darmstadt in the energy range 80±1000 MeV/u. Beams from Xe to U impinging on solid and gaseous targets between Be and U were used. Theoretical models for the charge-state evolution inside matter for a given initial charge state are presented. For this purpose, computer codes have been developed, which are brie¯y described. Examples are given which show the successes and limitations of the models. Ó 1998 Elsevier Science B.V. All rights reserved. 1. Introduction For the design and operation of storage rings for heavy ions and colliders such as ESR (Darm- The advent of relativistic heavy-ion accelera- stadt), RHIC (Brookhaven) and LHC (Geneva), tors, as well as new applications with relativistic one has to know precisely the interaction cross- heavy-ion beams, require a detailed knowledge of sections with the residual gas and colliding beams atomic collision processes. For instance, accelera- in order to estimate beam lifetimes and loss rates. tors need ecient strippers which induce only Also, in the multiple-turn passage through these small emittance blow-up. High ionic charge states devices, the charge-state distribution of the beam allow for lower power consumption and/or smaller will evolve, with subsequent beam loss. machines, thus reducing their price and their oper- State selective atomic-collision experiments, ational costs. It is desirable to use as few stripper such as radiative transfer and excitation (RTE) stations as possible in order to minimize losses of measurements, require known initial charge states. beam intensity. For the interpretation of many nuclear-physics experiments, a knowledge of ionic charge-state dis- tributions is decisive, for instance for the determi- * Corresponding author. Tel.: +49-6159-71-2706; fax: +49- nation of the nuclear-charge yields of ®ssion 6159-71-2902; e-mail: [email protected]. products. 0168-583X/98/$19.00 Ó 1998 Elsevier Science B.V. All rights reserved. PII: S 0 1 6 8 - 5 8 3 X ( 9 8 ) 0 0 2 4 4 - 4 442 C. Scheidenberger et al. / Nucl. Instr. and Meth. in Phys. Res. B 142 (1998) 441±462 Indeed, the ®rst experimental results on ionic charge-state distributions for heavy ions were ob- tained with ®ssion fragments by Lassen [1]. Inter- esting eects, such as the gas±solid dierence in the mean charge state were discovered. However, due to the wide energy spread of ®ssion fragments, these experiments could not be very detailed. Moreover, the huge charge-changing cross-sections at low energies and the target preparation tech- niques at the time, did not allow for cross-section measurements under single-collision conditions. Pioneering theoretical work was done by Bohr [2] and Bohr and Lindhard [3]. The so-called Bohr criterion that projectile electrons are stripped o during the penetration of matter if their orbital ve- locity is smaller than the projectile velocity, was es- tablished and proven to be in good agreement with experimental ®ndings. Although this criterion is Fig. 1. Equilibrium charge-state spectra of U projectiles behind very useful and can be applied successfully even C foils: the left spectrum was measured at the UNILAC of GSI at relativistic velocities, it does not incorporate behind a 40-lg/cm2 thick target for an entrance energy of 1.4 MeV/u [8], the distribution depicted in the middle of the ®gure any target dependence. In later years, many semi- was obtained behind a 490 lg/cm2 target and an incident energy empirical parameterizations were developed, see of 11.5 MeV/u (courtesy of B. Franzke) [9], and the spectrum e.g. [4], to describe the energy and target depen- displayed on the right was measured at SIS behind a 400 mg/ dence of the mean charge and the width of cm2 target at an entrance energy of 940 MeV/u. charge-state distributions. Once the cross-sections are known, the charge- carbon at 1.4, 11.5 and 950 MeV/u. As depicted in state evolution for ions having any initial charge this comparison, at low energies the charge-state state can be obtained from the solution of rate spectrum is broad and bare ions cannot be pro- equations. For up to three charge states, they duced whereas at high enough energies the can be easily solved analytically [5]. Beyond this charge-state distribution receives contributions number of charge states, numerical approaches only from bare, H- and He-like ions in charge- are used frequently. A general analytical scheme state equilibrium. At still higher energy, the bare- for an arbitrary number of charge states has been ion fraction dominates. At low energies, carbon derived by Sigmund [6]. For heavy ions, many is the best stripper whereas at high energies carbon charge states typically contribute to the charge- is a poor stripper as compared to heavier target state distribution. Thus, in principle, one needs materials. The reason will be explained below. to know all the relevant cross-sections for excita- New experimental techniques have been devel- tion, decay, ionization and capture for all contrib- oped which give detailed insights into speci®c uting ground and excited states. One may charge-changing processes [10]. The observation overcome these diculties, by using 'eective' of photons emitted in radiative electron capture cross-sections for capture and loss, derived from (REC) is possible [11] and coincidence techniques the measured target-thickness dependence of [12] allow the measurement of dierential REC charge-state fractions [7]. For relativistic heavy cross-sections. Subshell resolved excitation cross- ions, the situation generally is simpli®ed compared sections also can be obtained [13,14]. A striking to low energies, since at charge-state equilibrium feature of atomic-collision experiments with even the heaviest ions carry only few electrons dur- relativistic heavy ions is that charge-changing ing their passage through matter. Fig. 1 compares cross-sections can be studied under single-collision equilibrium charge-state spectra of U projectiles in conditions in solids. Gas-jet targets at storage C. Scheidenberger et al. / Nucl. Instr. and Meth. in Phys. Res. B 142 (1998) 441±462 443 rings, such as at the ESR at GSI, open up unique available experimental data. For clarity, we restrict new experimental opportunities in this respect. the discussion to the simple cases of high-Z bare, The purpose of this paper is to summarize the- H- and He-like projectiles. One ®nds that the gen- oretical and experimental results on charge-chang- eral scaling laws of the charge-changing cross-sec- ing cross-sections, charge-state evolutions, and tions for these ions explain the overall features of equilibrium charge-state distributions. The data equilibrium charge-state distributions in the entire are derived from experiments carried out at the relativistic velocity domain, even quantitatively. BEVALAC (Berkeley) and at the heavy-ion synch- rotron SIS of GSI (Darmstadt) and associated fa- 2.1. Cross-sections for ionization and excitation cilities. Representative data, partly unpublished so far, are given for Xe, Au, and U projectiles im- As long as asymmetric collision systems are pinging with kinetic energies from 80 to 1000 considered (ZT ZP, where ZT and ZP denote the MeV/u on targets ranging from Be to U. For ex- nuclear charge of target and the projectile, respec- perimental details, the reader is referred to [15± tively), the ionization of H- and He-like high-Z 25]. Phase-state, directional, and ultra-relativistic projectile ions can be reasonably well described eects are beyond the scope of the present paper. within ®rst-order perturbation theory, such as Only charge states of relativistic projectiles are the semiclassical approximation (SCA) or the considered throughout this paper. Theoretical plane-wave Born approximation (PWBA). Here, models and their range of applicability are discus- the basic assumptions are that only an electronic sed. The models are implemented in two computer perturbation of the projectile atomic wave function codes developed for practical applications and able is caused by the target nuclear charge and that the to take into account, respectively, up to three and trajectory of projectile is not disturbed by the col- up to 28 electrons attached to the projectile. The lision. Within the non-relativistic PWBA, the K- results are compared with experimental data. shell ionization cross-section rion for a H-like pro- jectile follows the simple scaling law: v 2. Physical background rion: r0f : 1 vK 2 2 4 The modeling of charge-state distributions of In this equation, r0 4pa0ZT=ZP, a0 is the Bohr ion beams passing through matter requires the radius, and f v=vK is a slowly varying function knowledge of the basic interaction mechanisms be- of the projectile velocity v, which reaches a maxi- tween highly charged ions and neutral matter, i.e., mum near v vK, where vK denotes the velocity the processes of projectile excitation, deexcitation, of the active K-shell electron. Tabulated values and ionization, and of electron capture into empty of this function can be found in various publica- projectile states.
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