KFKI-1991-34/J, К
К. BÉREI L. VASÁROS
BIBLIOGRAPHY OF ASTATINE CHEMISTRY AND BIOMEDICAL APPLICATIONS
Hungarian Academy of Sciences CENTRAL RESEARCH INSTITUTE FOR PHYSICS
BUDAPEST KFKI-1991-34/J, К PREPRINT
BIBLIOGRAPHY OF ASTATINE CHEMISTRY AND BIOMEDICAL APPLICATIONS
K. BEREI, L. VASÁROS
Central Raaaarch Institute for Phytic* H-1626 Budapest 114, P.O.B. 49, Hungary
HU I88N 0369 6330 CONTENTS
1. Preface Э
2. General reviews 5
3. Discovery, natural occurrence 11
4. Nuclear data 17
5. Preparation, handling, radiation risk 42
6. Physico-chemical properties . 55
7. Astatine compounds and chemical reactions 78
A: Inorganic 78
B: Organic 110
8. Biological effects and applications 133
9. Author index 163 1. PREFACE
The necessity for a more or less complete bibliography on astatine chemistry and on the biological applications of its alpha emitting isotope 211At arose at the Astatine Workshop in Budapest in 1987. Prior to that, apart from numerous review articles and the Astatine volume of the Gmelin Handbook of Inorganic Chemistry, published in 1985, individual collections prepared by researchers on some special topics could be found as sources of the astatine literature. In preparing this work we took advantage of other lists including those of RJ. Grover and G.-J. Meyer kindly offered to us years ago, as well as of the bibliography for 1983-1989 published by K. Rdssler in the special Astatine issue of Radiochimica Acta (1989. 47. 163-168) together with our own earlier collections; in addition we utilized the sources cited in the Astatine volume of the Gmeiin Handbook or" Inorganic Chemistry as well as the data in Chemical Abstracts {CA.), Nuclear Science Abstracts (N.SA.), Comprehensive Dissertation Abstracts, Conference Papers Index. Excerpta Medica and the INIS Atomindex up to July 1991.
As its title shows the bibliography deals mainly with the chemistry and biomedical applications of astatine. In view of the fact that only radioactive isotopes of astatine are known and that those of them that are generally used in chemical and biological investigations or in medical studies (209At, 210At. 2,1At) can be obtained solely by nuclear methods, we considered the references on the nuclear properties of these isotopes (Ch. 4) to be of interest for specialists in the fields mentioned above as well.
To facilitate the use of this bibliography we tried to specify the original information to be found in the references relating to Chapters 2-8. Obviously some of the publications cited may be informative in more than one field: we. therefore, indicated this by the chapter numbers given at the end of each reference.
For reports, dissertations, conference papers and articles pubished in not too well known periodicals, often in less commonly used languages, we also attempted to give the source of an English translation or a summary. Unfortunately, not all such items could be found in the reference journals or data banks. On the other hand, some of the references cited in particular articles were not available to us in the original form, this means that some bibliographical data are incomplete. Even so, our view was that something is better than nothing and .-ven limited data might be of help to researchers in locating the original work.These Jeficiences may serve as a reason for continuing and completing the work on system&tization and possibly providing a short evaluation of different publications in this field.
3 In the course of collecting data we asked a number of colleagues to correct and complete our lists of their publications. In this respect we are pleased to express our sincere gratitude to Drs. EH. Appelman. P. Anderson, G.-J. Beyer. WD. Bloomer. G. A. Brinknan. I. Brown. LAI. Cobb. R. Dreyer. P.W. Durbin. JA. Grover, A. Harrison. KM. Lambrecht. Y. Legoux. G.-J. Meyer. Yu.V. Norseyev, F. Rösch. К. Rössler. G. Samson. N. Takahashi. G.WM Visser. M. R. Zalutsky for their help.
We should like to thank Ms Anna Szuja. and the staff of the litory at the Central Research Institute for Physics for the technical assistance in preparing this report.
Budapest. December 1991
Klara Berei and László Vasáros
4 2. GENERAL REVIEWS
ANDERS. E. Technetium and astatine chemistry. Anm. Rev. Nucl. ScL 1959. 9. 203-220. (Cb. 2)
APPELMAN. E. H. The radiochemistry of astatine. Report NAS-NS 3012 1960. 29 pp. CA. I960. 34. Na 19 191. (Cbs. 2. 5. 6.7/A)
APPELMAN. E. H. Chemical properties of astatine. PhJ). diss* University rf California. Berkeley. CA 1960. Report UCRL-9025 1960. 113 pp. С A. I960. 54, No. 16 998. (Cbs. 2. 5. 6, 7/A)
APPELMAN. E. H. Astatine. in The Encyclopedia of the Chemical Elements, edited by Hampel, С A., pp.33-35. New York: Reinhold, 1968. (Cbs. г. з, 4.6)
APPELMAN. Е. Н. "Astatine." in MTP (Med. Tech. Publ. Co.) Int. Rev. Sei»- Inorg. Chem* Ser. One, edited by Gutmann. V., Vol. 3. pp. 181-198. London: Butterworths, 1972. CA. 1972. 76. No. 120 925. (Cbs. 2. 5.6, 7/AB)
ATEN, A. H. W.V Jr. The chemistry of astatine. Adv. Inorg. Chem. and Radiochem. 1964. 6, 207-223. (Cbs, 2. 5. 7/AB)
BAGNALL, K.W. Astatine, francium and radon. in Chemistry of Rare Radioelements Polonium-Actinium, pp. 97-102. London: Butterworth. 1957. (Cb. 2)
5 BÉREI. К. The radioelement astatine and its prospects in nuclear medicine. (in German) Strahlenschutz-Kerntechnik. Suppl.l. edited by Giebeler, E .W., pp. 25-32. Darmstadt: GIT Verlag. 1988. (Cbs. 2. 7/AB. 8)
BEREI. K.. VÁSÁROS, L. Organic chemistry of astatine. Report KFKI-1981-Ю 1981. 73 pp. 1N1S Atomindcx 1981. 12. Na 609 373. (Chs. 2. 7/B, 8)
BEREI. K.. VÁSÁROS. L. Organic chemistry of astatine. in The Chemistry of Functional Groups. Suppi. D.. edited by Patai. S. and Rappoport. TL. pp. 405-440. New York: Wiley, 1983. (Cbs. 2, 7/B, 8)
BEYER. G.J.. DREYER. R.. HERRMANN. E. Radiochemistry of spallation products. (in German) Kernenergie 1981, 24, 388-393. CA. 1981, 95. No. 226 781. (Cbs. 2. 7/A)
BROWN. I. Astatine: its organonuclear chemistry and biomedical applications. in Adv. 1 nor^. Radiochem.. edited by Emeléus, H. J., Sharpé, A. G., Vol. 31, pp. 43-88. New York: Academic Press, 1987. (Chs. 2, 7/B, 8)
DOWNS, A. J., ADAMS, С J. The chemistry of chlorine, bromine, iodine and astatine, in Comprehensive inorganic Chemistry, edited by Bailar, J. C, Emeléus, H. J., Nyholm, R., . Trotman-Dickenson, A. F„ Vol. 2, pp. 1573-1594. Oxford: Pergamon, i973. С. A. 1975, 8.Я. No. 70 903. (Ch$. 2. 6, 7/AB)
DRANOVSKY, A. B. Polonium, actinium, protactinium, astatine and francium. (in Russian). in Osnoxy Mettallurgii, edited by Greiver, N. S., Sazhin, N. P., Strigín. I. A., Troickíj, А. В., pp. 169-171. Moscow: Metallurgia, 1968. СЛ. 1970. 72. No. 14 783. (Ch. 2)
DREYER, R., RÖSCH, F., BEYER. G.-J. Astatine. Study of an unstable, (in German) Wiss. Fort sehr. 1982. 32, 251-255. CA. 1982. 97. No. 151 718. (Cbs. 2. 3. 7/A)
6 DUVAL. С Astatine, (in French) CMm. Anal. 1963. 45. 557-559. CA. 1964. 6a No. 4751Г. (Ck 2) EMELÉUS. H. J. Transuranics and other newly discovered elements. Seil Progr. 1950. 38. 609-621. CA. 1951. 45. Na 403Г. (Chs. 2. 3)
GARNER. С S. Astatine. in Radioaamty Applied to Chemistry, edited by Wahl. A. C. Bonner. N. A., pp. 200-204. New York: Wiley. 1951. (Ch. 2) HAISSINSKY. M. The new chemical elements and the Periodica) System. (in French) Bull. Soc. Chim. 1949. 16. 668-678. (Chs. 2,3)
HAISSINSKY. M. Astatine. (in French) Chim. Mitt. 1960. 16. 659-666. (Chs. 2, 3)
HYDE. E. 1С The present status of elements 85 and 87. J. Phys. Chem. 1954. 58. 21-26. (Chi 2, 3)
HYDE. E. K. Astatine and francium. J. Chem. Educ. 1959, 36, 15-21. (Ch. 2) HYDE. E. K., PERLMAN, I.. SEABORG, 0. T. The isotopes of astatine. in The Nuclear Properties of the Heavy Elements, Vol. 2, pp. 1077-1094. Englewood Cliffs: Prentice-Hall. 1964. (Ом. 2.4)
KHALK1N, V. A.. HERRMANN, E. Inorganic chemistry of astatine, (in German) Isotopenpraxis 1975, 11, 333-340. СЛ. 1976, 84, No, 9632. <СЪ». 2, 3, 7/A)
7 KHALKIN. V. A.. HERRMANN. E.. NORSEYEV. Yu. V.. DREYER. I. Present state of astatine chemistry, (in Russian) Report JINR-R-6-W72S 1977. 42 pp. INIS Atomtod« 1978.9. Na 391 025. (Chs. 2. 5. 7/AB)
KHALKIN, V. A.. HERRMANN. E.. NORSEYEV. Yu. V.. DREYER. I. The present status of astatine chemistry, (in German) Chemiker-Ztg 1977. 101. 470481. CA. 1978. 88. Na 28 663. (du. 2, 5, 7/AB)
KLIVÉNYI. G. Т.. LAKATOS. В. Review on the 85th element: the astatine. (in Hungarian) Magy. Kern. Foly. 1954. 60. 136-141. CA. 1938. 52, Na 699S. (СЬ. 2}
KRAKKAY. T. V. Chemistry and nuclear properties of the missing elements. (in German) Fortschr. Chem. Forsch. 1958. 3, 738-821. СЛ. 1958. 52. No. 9829. (Cb. 2)
KUGLER, K. H., KELLER. C, Editors Astatine. Gmelin Handbook of Inorganic Chemistry, 8th Ed., 289 pp. Berlin: Springer. 1985. (Cb. 2)
KUZIN, V. I. Astatine, (in Russian) Khim. Zhizn. 1974, 6, 24-27. CA. 197S, 83. Nu. 2 052 016. (СЬ. 2)
LAVRUKHINA. А. К., POZDNYAKOV, A. A. in Analytical Chemistry of Technetium, Promethium, Astatine and Francium, pp. 227-260. Ann Arbor: Humphrey, 1970. CA. 1971. 75. No. 71 094. also in Russian: pp, 228-259, Moscow: Nauka, 1966. (Cb». 2.7/A)
8 MADDOCK. A. G. Astatine. in A Comprehensive Treatise of Inorganic and Theoretical Chemistry, edited by Mellor J. M., Vol. 8.. pp. 1064-1079. London: Longmans Green, 1956. also in Russian: Usp. Khim. 1960. 29. 1388-1406. MEYER. G.-J. On reactivity and selectivity of inorganic forms of radioelement astatine in replacement reactions with aromatic systems. (in German) Ph. D. disz, Kernforschungsanlage Jülich GmbH, Jülich (FRG) 1977. Report Jül-1418 1977, 108 pp. CA. 1978. 88. Na 71 113. (Cht. 2. 5. 7/AB) NEFEDOV. V. D.. NORSEYEV. Yu. V.. TOROPOVA. M. A.. KHALKIN. V. A. Astatine, (in Russian) Report J1NR-R-2895 1966, 33 pp. С А. 1967. 66. Na 70 899. (Cbs, 2. 5. 7/AB) NEFEDOV, V. D.. NORSEYEV, Yu. V.. TOROPOVA. M. A.. KHALKIN. V. A. Astatine. (in Russian) Usp. Khim. 1968, 37, 193-215. CA. 1968. 68. Na 100 679. (Cbs. 2. 3. 7/AB) QIAO, Ming-Lun Astatine and its chemical properties. (in Chinese) Huaxue Tongbao 1965, 48-52. N. & A. 1966, 20. No. 22 985. (Ch. 2) RÖSSLER, K. Preface of special edition on astatine. Radiochim. Acta 1989, 47, 163-168. (Ch. 2) RÖSSLER. K. Bibliography of astatine chemistry and biomedical application 1983-1989. Radiochim. Acta 1989, 47, 163-168. (Ch. 2) 9 SAMSON. 6. Astatine, the fifth halogen. (in Dutch) Chem. Weekbl. 1969. 65. 27-31. also in English: Report ANL-TRANS-859 1970. 11 pp. CA. 1970. 72. Na 17 315. (Chs. 2. 7/B) SAMSON. G. Organic compounds of astatine. Dr. Sei. diss* University of Amsterdam, Amsterdam 1971. 69 pp. (Chs. 2. 3. 7/B) SEDUET. J. Astatine (atomic number 85). in Treatise on Analytical Chemistry, Pari 1!.. Vol. 6 . edited by Kolthoff, I. M.. Eh/ing. P. J.. Sandell. Б. В.. pp. 487-501. New York: Wiley. 1964. «a». 2.7/A) SHISTKOVA. N. Astatine-211: examination of its possible uses. Report UJV 7962-0 1987. 17 pp. С А. 1988. 107. No. 143 093. (Chs. 2, 5. 7/B. 8) VJSSER. G. W. M. Some aspects of the organic, biological and inorganic chemistry of astatine. Ph. D. diss., University of Amsterdam, Amsterdam 1982. 119 pp. С A. 1984. 100. No. 60 773. (Ом. 2. 7/AB, 8) WANG. Quanji Astatine and its applications. (in Chinese) Huaxue Tongbao 1987. 5. 27-30. С A. 1988. 107. No. Í22 287. 10 3. DISCOVERY, NATURAL OCCURRENCE ALUSON. F. The magneto-optic method of analysis. У. Chem. Educ. 1933. 10. 71-78. (Ck. 3) ALUSON. F.. BISHOP. E. R.. SOMMER. A. L. Concentration, acids and lithium salts of element 85. J. An Chem. Soc. 1932, 54. 616-620. (On. 3, 7/A) ALUSON. F.. MURPHY. E. J., BÍSHOP. E R., SOMMER. A. L> Evidence of the detection of element 85 in сенат1 substances. Phys. Rev. 1931, 37, 1178-1180. (Ch. 3) ANDERSEN. E. B. Methods used for searching element 85. (in German) Kgl. Danske Videnskab. Selskab. Math.-fis. Medd. 1938. 16. 22 pp. 2 С A. 1939v 33, No. 474 . (Ch. 3) APPELMAN. E. H. Astatine. m The Encyclopedia of the Chemical Elements, edited by Hampel. С A., pp. 33-35. New York: Reinhold, 1968. (СЬ*. г, з, 4.6) ASIMOV. 1. The natural occurrence of short-lived isotopes. J. Chem. Educ. 1953, 30. 616-618. (Ch. 3) BARTON, G. W., GHIORSO, A., PERLMAN, I. Radioactivity of astatine isotopes, Phys. Rev. 1951, 82, 13-19. (Cte 3.4.3) BRIAND, J. P., CHEVALLIER, P., TUATI, A. Beta emission of francium-220, (in French) /. Phys. 1971, 32, 101-105. (Ch. 3) CORSON, D. R., MacKENZIE, K. R. Artificially produced alpha particle emitters. Phys. Rev. 1940, 57, 250. 11 CORSON. D. R.. MacKENZIE. K. R.. SEGRÉ. É Possible production of radioactive isotopes of element 85. Phys. Rev. 1940. 57, 459. (Cbs. 3. 5, 7/A, S) CORSON. D. R., MACKENZIE, К R.. SEGRÉ. E. Artificially radioactive element 85. Phys. Rev. 1940. 57. 1087. (du. 3.5) CORSON. D. R.. MacKENZIE. K. R., SEGRÉ. E. Artificially radioactive element 85. Phys. Rev. 1940. 58. 672-678. (Qu. 3. 7/A) CORSON. D. R.. MacKENZIE. K. R.. SEGRÉ. E Astatine: the element of atomic number 85. Nature 1947. 159. 24. (Cb.3) CRANE. E. J. Nomenclature, spelling and pronounciation. Chenu Eng. News 1951. 29. 2181-2182. (Cb.3) DE, Rajcndralal Twin elements in Travancore monazite. Separate, Dacca: Bani Press. 1937, 18 pp. C. A. 1937, 31, No. 61037. (Ch.3) EMELÉUS. H. J. Transuranics and other newly discovered elements. Sei. Progr. 1950, 38. 609-621. CA. 1951. 45. No. 403Г. (Cht. 2, 3) ENGLISH, A. C, CRANSHAW, T. E. DEMERS. P., HARVEY. J. A. H1NCKS, E. P., JELLEY. J. V., MAY, A. N. The (4n+l) radioactive series. Phys. Rev. 1947. 72, 253-254. (Cb%. 3,4) POOTE, P. D. Nitrogen and uranium. Mature 1924, 114, 789. (Cb.3) FRIEND, J.N. Examination of Dead Sea water for eka-cesium and eka-iodine. Nature 1926, 117,789-790. (Ch.3) OROVER, J. R. Rapid emanation of astatine and radon. in 155th Nat. Meet. Am. Chem. Soc., San Francisco, CA: 1-5 Apr. 1968. Abstr. 0-170. (Cb.3) 12 GROVER. J. R. LEBOWITZ. E. BAKER. Б. W. Prompt emanation of astatine and radon. Л Inatg. Mud. Chem. 1969. 3!. 3705-3720. (Chs. 3.7/A) HAGEMANN. F.. KATZIN. L. I.. STUDIER. M. H.. OHIORSO. A.. SEABORG. G. 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DRUCE, J. G. F. Eka-cesium and eka-iodine. Chem. News 1925, 131, 305. С A. 1926, 20. No. 8503. (Ch. 3) MEINKE. W. W., GHIORSO, A., SEABORG, G. T. Three additional collateral alpha decay chains. Phys. Rc\>. 1949, 75, 314-315. (Chs. 3, 4) MILLER. J. F.. HAMILTON, J. G., PURNAM, T. M., HAYMOND, H, R., ROSSI, G. B. Acceleration of stripped i2C and ,3C nuclei in the cyclotron. Phys. Rev. 1950, 80, 486. (Chs. 3, 5) MINDER, W. The beta radiation of RH A and the formation of the element with nuclear charge 85. (in German) Helv. Phys. Acta 1940, 13, 144-152. (Ch. 3) 15 SEGRE. E. The contribution of artificial radioactivity to the completion of the Periodic System. /. Appl. Phys. 1941. 12. 309-310. (Ch. 3) S1DGWICK. N. V. Element No. 85 (Astatine). in The Chemical Elements and Their Compounds. Vol. II. pp. 1260-1261. Oxford: Clarendon. 1950. TRIMBLE. R.F. What happened to alabamine, virginium and illinium? Chem. Educ. 1975. 52. 585. (Ch. 3) TURNER. L. A. Regularities among the heavy nuclei. Phys. Rev. 1940. 58. 181-182. (Chs. 3.4) YASHITA. S. Identification of new astatine isotopes using the gas-filled magnetic separator, SASSY. Report LBL-15 562 1984. 69 pp. С A. 198S. 101. No. 178 768. (Cb. 3) 16 4. NUCLEAR DATA ABDUMALIKOV. A. A.. ABDURAZAKOV. A. A., GROMOV. K. Ya.. KARAKHOZDAEV. A.. NORSEYEV. Yu. V.. TOSHEV, M. Conversion electron spectrum during astatine-209 decay, (in Russian) in Progr. Tezisy Dokl. Soveshch. Yad. Spektrosk. Stukt. At. Yadra. p. 161. Leningrad: Nauka. 1974. С. А. 1975. 82. No. 63 462. (Ch. 4) ABDUMALIKOV. A. A.. ^BDURAZAKOV. A. A., GROMOV. K. Ya.. KARAKHOZDAEV. A., NORSEYEV. Yu. V., TOSHEV. M. Spectra of conversion electrons during decay of astatine-208 and astatine-209. (in Russian) Nauchn. Tr. Tashk. Cos. Univ. 1974. 459. 8-13. C. A. 1976, 84, Nu. 9762. (Cb. 4) ADAM. I.. BONCi-OSMOLOVSKAYA. N. A.. VENOS. D.. et al. Angular correlations of gamma rays in the 2,,Rn decay, (in Russian) in 1N1S-SU-166 1989. pp. 127-128. 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III. 112, 125. 126, Appelman, EH. 5. 11. 19. 42, 55, 56. 78. 110, 127. 128. 135. 156 114 Berg, A. V. 19. 20 Appelqvisl, A. 28 Bvrger, A. 57 Arenas-Peris, U. E. 19 Bergstrom. I. 20. 21. 25, 34 Arnold, J. S. 143 Bernard, S. R. 136 Arvieu. R. 19 Bernért, T. 14 Asimov. I. 11 Bcrlschal. H. H. 57 Asling. С W. 134. 143. 145 Beyer. С J 6, 43. 44. 51. 80. 85. 108. 136. 143 Astner. O. 19, 21 Bhardwaj. M. K. 34 Alashroo, T, 72 Bhattacherrjec, S. K. 36 Alchcr. R. W. 78. 134. 136. 137. 145, 149 Bnulra. M. P. 74. 105 Aten. A. H. W.. Jr. 5. 42, 56, 78, 80, 104, 110, Bigner, D.D. 114, 144 161 124 Bimbót. R. 21. 25, Atkins. H. L. 134 Birkeliind, J. R. 45 Audi. O. 61 Bishop. E. R. 11.78 Axelrod-Hellcr. D 145 Bjornstad, T. 34, 103 Blanpied, O. S. 22 Baba. H. 105. 125 Blasse, C. 79 Babcnkov. M. I. 19 Blattmann, H. 134 Badalov. S. A. 20 Blokbin, M. A. 57 Bagnall. K. W 5 Biomqvist, J. 20. 21. 34 Bai, Xingping 31 Bloomer, W. D. 80, 119, 123, 133. 134. 136. 137. Bajkov. V. I. 56.79 148. 150. 153 163 Bobykin. 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С 73 Muminov, A. I. 22 Mani. R. S. ISO Murphy, E. J. 11 Manson, S. T. 61 Müller. H. 60 Marinov, A. 99 Miinzel. H. 33 Mark, H. 56. 58. 64 Myburg, J. A. 121, 152, 156 Markhol, M. 97 Marquicr, G. 23 Nagy. ü. Á. 100 Marsh. K. V. 48,97 Nakahara, H. 41 Marlin, M.J. 31,33 Nakai, K. 25 Martinov, A.A. 31 Narasimhan, P. T. 73 Maschuw, R. 27 Narula, A. S. 120, 132 Matsuoka, O. 70 Neergard, K. 32 Matsuyanagi, K. 32 Nefedov, V. D. 9, 50, 71. 93. 100, 101, 102. 116, Maxwell. R. D. 87. 145, 146 120, 121 May, A.N. 12.24 Ncirinckx, R. D. 50, 101. 121, 137, 152, 156 McLaughlin, R. 70 Nelson, G. С 71 Nelz, P. 142 168 NeskakiStA. 36 Pbadnis.S.G. 72 Nestor. С. W. Jr. 69 Piccardi. G. 72 Neumann. H. M. SO. 71. 101 Pickering, D. E. 153 Ncyens, G. 35 Pillái. К. M. R. 123. 153 Német. L. 43.57.79 Pitt. M. L. 29 Nguyen. Tat-To 29 Plalkov. A. I. 57 Nhan. Dang Due 44. 76. 82. 121. 122. 128. 129 Platl. J. R. 72 Nielsen. OB 24 Polelti, S. J. 24. 36 Niselyson. LA. 71. 101 Politzer, P. 73 Niton. O. 41 Poplavskii. I. 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A. 66. 91 Zollwcg, R. J. 77 172 The issues of the KFKI preprint/report series are classified as follows: A. Particle and Nuclear Physics B. General Relativity and Gravitation С Cosmic Rays and Space Research D. Fusion and Plasma Physics E. Solid Stale Physics F. Semiconductor and Bubble Memory Physics and Technology Q. Nuclear Reactor Physics and Technology H. Laboratory. Biomedical and Nuclear Reactor Electronics L Mechanical, Precision Mechanical and Nuclear Engineering J. Analytical and Physical Chemistry K. Health Physics L. Vibration Analysis. CAD. CAM M. Hardware and Software Development. Computer Applications. Programming N. Computer Design, CAMAC, Computer Controlled Measurements The complete series or issues discussing one or more of the subjects can be ordered; institutions are kindly requested to contact the KFKI Library, individuals the authors. Title and classification of the issues published this year: KFKI-1991-01/M A. Ambrozy. Experience during applying the ORACLE 4GL system (in Hungarian) KFKI-1991-02/M S. Dibuz Wagner: A knowledge base for protocols KFKM991-03/G Gy. Ézsöl et al Adaptation of RELAP5/M0D2 code: Analysis of IAEA SPE 3 (in Hungarian) KFKI-1991-04/G Gy. Ézsöl et al.: IAEA SPE 3. Valuation of measurement results (in Hungarian) KFKM991-06/G A Takács et al.: SM ABRE - as the dynamical model of the primary circuit for the code KARATE (in Hungarian) KFKM991-06/A J Balog et al Locality problem for the Liouville field KFKI-1991-07/E N. Éber et al.: Linear electromechanical effect In a polymeric ferroelectric liquid crystal KFKM991-08/C B. Lukács: Prices and sunspots KFKI-1891-06/E MV. Koztovsky et al.: A chfral side chain polymer with layered structure KFKM991-10/G P. Vértes: Calculation of transmission and other functlonals from evaluated data in ENDF format by means of personal computers KFKM991-11/E F Tóth: Non destructive testing methods (in Hungarian) KFKi-ieei-l2/H Vera Jánossy et al: Multichannel recordings and data analysis from spinal cord expiants and cell cultures KFKI-1991-13/G Z Szatmáry: User's manual of program RFIT Pari 1 General description KFKI-1991-14/G Z. Szatmáry: User's manual of program RFIT Part 2 Parameter estimation KFKI-1991-16/G 2 Szatmáry: User's manual of program RFIT Part 3. The data files KFKI-1891-16/G Z. Szatmáry. User's manual of program RFIT. Part 4. Statistical analysis. Task PLOT KFKM991-17/A T. Haugsetetal.: Is the breakup time a free parameter when describing heavy ion collisions? KFKI-1991-18/Q Margit Telbisz: SNARE A response matrix based few group nonlinear reactor code in hexagonal geometry KFKI-1991-19/B G. Paál et al.: Inflation and compactification from galaxy redshifts? KFKI-1991-20/6 L Pemeczky: ISP 27. Pre test calculations for BETHSY SB LOCA test with RELAP5/RMA code (in Hungarian) KFKI-1991 -21 /A VSh Gogohia et al Phenomenologlcal dynamics InQCD at large distances KFKI-1991 -22/C M.I Verigln et al.: The dependence of the Martian magnetopause and bow shock on solar wind ram pressure according to Phobos 2/T AUS Ion spectrometer measure ments KFKI-1991-23/A VSh Gogohia et al.: Dynamical chiral symmetry breaking and pion decay constant KFKI-1991 -24/A Gy Bencze el al.: Coulomb screening in low energy nuclear reactions KFKI-1991 -25/G E. Végh et al Compact simulators for WER 440 type nuclear power plants KFKI-1991 -26/B I Recz: Spacetime extensions I. KFKI-1991-27/K l Balásházy: Calculation of flow fields and aerosol particle trajectories in bifurcating tubes KFKI-1991-28/A T Csörgőét al (eds): Proceedings of the Workshop on Relatlvtstic Heavy Ion Physics at Present and Future Accelerators KFKI-1991 -29/B LB Szabados: Canonical pseudotensors, Sparling's form and Noether cur rents KFKI-1991 -30/B В Lukács et al.: About the possibility of a generalized metric KFKI-1991-31/L P Pellionisz et al.: Development of an expert system for acoustic emission testing: "AE DATA EXPERT" KFKM991-32/C B. Lukács el al. (eds ) Symmetry and topology in evolution KFKI-1991 -33/G I. Vidovszky et al.: Study of Gd lattices (Calculations and Intercomparison) KFKM991-34/J.K K. Bereietal: Bibliography of astatine chemistry and biomedical applications :H «е. 'í Iá i it", ff \á:á f" ' Síi'. tót- ilh- ^ U -' Kiadja a Központi Fizikai Kutató Intézet Felelős kiadó: Gadó János Szakmai lektor: Kiss István ü ! ! f4í, Nyelvi lektor: Példányszám: 254 ы ' Készült a PROSPERITÁS Kft. nyomdaüzemében \«\ Budapest, 1992. február hó