Atmos. Meas. Tech., 12, 5457–5473, 2019 https://doi.org/10.5194/amt-12-5457-2019 © Author(s) 2019. This work is distributed under the Creative Commons Attribution 4.0 License. Tracking down global NH3 point sources with wind-adjusted superresolution Lieven Clarisse1, Martin Van Damme1, Cathy Clerbaux2,1, and Pierre-François Coheur1 1Atmospheric Spectroscopy, Service de Chimie Quantique et Photophysique, Université libre de Bruxelles (ULB), Brussels, Belgium 2LATMOS/IPSL, Sorbonne Université, UVSQ, CNRS, Paris, France Correspondence: Lieven Clarisse (
[email protected]) Received: 13 March 2019 – Discussion started: 20 May 2019 Revised: 17 July 2019 – Accepted: 15 September 2019 – Published: 17 October 2019 Abstract. As a precursor of atmospheric aerosols, ammonia point-source catalog consisting of more than 500 localized (NH3) is one of the primary gaseous air pollutants. Given its and categorized point sources. Compared to our previous cat- short atmospheric lifetime, ambient NH3 concentrations are alog, the number of identified sources more than doubled. In dominated by local sources. In a recent study, Van Damme addition, we refined the classification of industries into five et al.(2018) have highlighted the importance of NH 3 point categories – fertilizer, coking, soda ash, geothermal and ex- sources, especially those associated with feedlots and indus- plosives industries – and introduced a new urban category trial ammonia production. Their emissions were shown to for isolated NH3 hotspots over cities. The latter mainly con- be largely underestimated in bottom-up emission inventories. sists of African megacities, as clear isolation of such urban The discovery was made possible thanks to the use of over- hotspots is almost never possible elsewhere due to the pres- sampling techniques applied to 9 years of global daily IASI ence of a diffuse background with higher concentrations.