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1 Trajectory Analysis of Saudi Arabian Dust Storms 2 3 Michael Notaro 4 Nelson Center for Climatic Research, University of Wisconsin-Madison 5 1225 West Dayton Street, Madison, Wisconsin 53706 6 * [email protected], 608-261-1503 7 8 Fahad Alkolibi, Eyad Fadda, Fawzieh Bakhrjy 9 King Saud University 10 11 Revised Research Article to the Journal of Geophysical Research-Atmospheres 12 13 Abstract

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15 Temporal and spatial characteristics of Saudi Arabian dust storms, with focus on

16 associated air parcel trajectories, are investigated using station and gridded weather

17 observations and remotely-sensed aerosol optical depth (AOD). For 13 focal stations, an

18 extensive pool of 84-hour backward trajectories is developed for dust storm days, and the

19 trajectories are grouped into 3-5 representative clusters based on the K-means technique

20 and Silhouette Coefficients.

21 Saudi Arabian dust storms are most prominent during February-June, with a mid-

22 winter peak along the southern coast of the Red Sea, spring peak across northern Saudi

23 Arabia around the An Nafud , and early summer peak in eastern around

24 the Ad Dahna Desert. Based on backward trajectories, the primary local dust source is the

25 Rub Al Khali Desert and the primary remote sources are the Saharan Desert, for western

26 Saudi Arabia, and Iraqi , for northern and eastern Saudi Arabia. During February-

27 April, the Mediterranean storm track is active, with passing cyclones and associated cold

28 fronts carrying Saharan dust to Saudi Arabian stations along the northern coast of the Red

29 Sea. Across Saudi Arabia, the highest AOD is achieved during dust storms that originate 2

30 from the Rub Al Khali and Iraqi Deserts. Most stations are dominated by local dust sources

31 (primarily Rub Al Khali), are characterized by three dominant trajectory paths, and achieve

32 AOD values exceeding 1. In contrast, for stations receiving predominantly remote dust

33 (particularly Saharan), 3-5 trajectory paths emerge and AOD values only reach

34 approximately 0.6 as dust is lost during transport.

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37 Key words: dust storms, Saudi Arabia, backward trajectories, aerosol optical depth, dust

38 sources, HYSPLIT

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52 3

53 1. Introduction

54

55 Global deserts supply roughly 5×108 tons of Aeolian dust to the atmosphere each

56 year (Peterson and Junge, 1971). Through substantial aerosol loading to the atmosphere,

57 dust storms can significantly alter the regional climate and physical environment (Park et

58 al., 2005; Goudie and Middleton, 2006). Dust can be transported over thousands of

59 kilometers, thereby influencing both the environment and society at great distances from

60 its source region (Goudie and Middleton, 2001, 2006; Middleton and Goudie, 2001). For

61 instance, the Saharan Desert contributes an estimated 40-66% of total Aeolian dust to the

62 global atmosphere (Junge, 1979; Morales, 1979; Schutz et al., 1981; Ganor and Mamane,

63 1982). In response to strong summertime heating of the land surface or gusty winds

64 associated with storms entering the Mediterranean Sea or North Africa, Saharan dust can

65 be lifted to heights in excess of 3-5 km above the ground (Escudero et al., 2005, 2011;

66 Dayan et al., 1991; Alpert and Ganor, 1993; Conte et al., 1996; Prospero, 1996). In extreme

67 cases, Saharan dust can reach China (Tanaka et al., 2005), the United States (Prospero,

68 1981; Gatz and Prospero, 1996), Barbados (Delany et al., 1967), and other remote locations,

69 even the (Barkan and Alpert, 2010).

70 Research on Aeolian dust is vitally important given its notable influence on

71 atmospheric and oceanic conditions, agriculture, soil, water quality, and human health. The

72 impact of dust on the atmosphere’s radiative balance (Hansen et al., 1998; Haywood and

73 Boucher, 2000) includes both direct effects on scattering and absorption (Tegen et al.,

74 1996; Haywood et al., 2003) and indirect effects related to the aerosols’ influence on cloud

75 microphysics (Rosenfeld et al., 1997). By altering the atmospheric temperature (Wong et 4

76 al., 2009) and concentration of condensation nuclei, dust storms can affect convective

77 activity, cloud formation, and precipitation efficiency (Bryson and Barreis, 1967; Maley,

78 1982; Lohmann and Feichter, 2005; Wong and Dessler, 2005). Dust aerosol radiative

79 heating can influence synoptic weather patterns, such as by strengthening the Saudi

80 Arabian heat low (Mohalfi et al., 1998). The impact of the dusty Saharan air layer on the

81 growth of easterly waves and tropical cyclones across the Atlantic Ocean continues to be

82 debated (Karyampudi and Carlson, 1988; Karyampudi and Pierce, 2002; Dunion and

83 Velden, 2004; Wu, 2007; Lau and Kim, 2007a,b; Sun et al., 2008). Iron is a key constituent

84 of aeolian dust (Zhu et al., 1997), and its deposition into the ocean enhances phytoplankton

85 blooms (Martin et al., 1991; Gruber and Sarmineto, 1997; Jickells et al., 1998; Sarthou et al.,

86 2003) and potentially leads to ocean cooling (Schollaert and Merrill, 1998). Dust can affect

87 atmospheric chemistry, including sulfur dioxide concentrations through physical

88 adsorption and heterogeneous reactions (Adams et al., 2005). Dust storms can damage

89 crops and reduce soil fertility (Fryrear, 1981; Thiagarajan and Lee, 2004). Furthermore,

90 dust storms dramatically affect human society. Reduced visibility can lead to traffic

91 accidents and vertigo in aircraft pilots (Morales, 1979; Hagen and Woodruff, 1973;

92 Middleton and Chaudhary, 1988; Dayan et al., 1991; Yong-Seung and Ma-Beong, 1996).

93 Dust storms can transport allergens and disease-spreading spores (Leathers, 1981; Shinn

94 et al., 2000; Pope et al., 2002; Kampa and Castanas, 2008), trigger asthma and respiratory

95 ailments (Kar and Takeuchi, 2004; Chen et al., 2004; Gyan et al., 2005; Thalib and Al-Taiar,

96 2012), and contaminate drinking water (Clements et al., 1963).

97 Saudi Arabia is a region of complex topography and extensive deserts (Fig. 1). Its

98 three primary desert regions are the Rub Al Khali (“Empty Quarter”, ≈600,000 km2) in the 5

99 southeast, An Nafud (≈65,000 km2) in the northwest, and Ad Dahna sand corridor (≈40,000

100 km2) in the east, connecting the previous two deserts. Remote desert regions that can

101 potentially serve as dust source regions to Saudi Arabia include the vast Saharan Desert to

102 the west and Syrian and Iraqi (Al-Hajarah and Al-Dibdibah) Deserts to the north. The

103 is bordered by the Mediterranean Sea to the northwest, Red Sea to the

104 west, Gulf of Aden and Arabian Sea to the south-southeast, and Persian (Arabian) Gulf to

105 the east, with the Sarawat Mountains (up to 3.3 km in elevation) along the peninsula’s west

106 coast.

107 According to Total Ozone Mapping Spectrometer (TOMS) data, the most prolific dust

108 source regions in the world are the Desert, particularly the Bodélé Depression in

109 Chad (most active in spring), and the Rub Al Khali along the Saudi Arabia-Oman border

110 (Goudie and Middleton, 2001, 2006; Giles, 2005). Within the Middle East, the TOMS

111 aerosol index peaks over the Rub Al Khali and Ad Dahna Deserts, and dust storms typically

112 occur in areas with a mean annual precipitation less than 100 mm and a mean annual

113 potential evapotranspiration greater than 1140 mm (Goudie and Middleton, 2002, 2006).

114 Middle Eastern dust storms are most frequent across Sudan, Iraq, Saudi Arabia, and the

115 Persian (Arabian) Gulf (Kutiel and Furman, 2003).

116 An extensive discussion of the causes of Middle Eastern dust storms is provided by

117 Goudie and Middleton (2006). According to Vishkaee et al. (2011), dust storms are

118 primarily triggered through dynamical lifting in the cool season, related to cold fronts and

119 their associated mid-latitude troughs, or diurnal vertical mixing in the warm season,

120 related to solar heating. The most frequent trigger for dust storms is a frontal passage,

121 with strong winds associated with intense baroclinicity. The concentration of atmospheric 6

122 dust is tightly correlated with wind velocity (Kutiel and Furman, 2003). Strong surface

123 cyclones can also stir up dust clouds. In monsoon regions, dust may be lifted into the

124 atmosphere along convergence zones between cold air masses, associated with cyclones,

125 and tropical anticyclonic air masses. In areas of complex terrain, katabatic winds can

126 trigger localized dust storms. Dust can be delivered into the atmosphere through

127 convective plumes and vortices (Koch and Renno, 2005). Haboobs and dust devils are local

128 causes of dust-raising and transport. A haboob is a convection-generated dust storm

129 associated with the cool outflow from a thunderstorm downdraft. Middle Eastern dust

130 storm activity usually peaks during the daylight hours, when intense solar heating of the

131 ground generates turbulence and local pressure gradients (Middleton, 1986). Dust activity

132 and the remotely-sensed aerosol index generally peak during May-August across the

133 Arabian Peninsula (Prospero et al., 2002; Washington et al., 2003; Barkan et al., 2004;

134 Goudie and Middleton, 2006), when solar heating and climatological wind speeds are

135 greatest. However, Sharav (Saharan) cyclones from the Mediterranean Sea (Trigo et al.,

136 1999) are responsible for the winter-spring peak in dust activity that characterizes

137 northern Saudi Arabia (Ganor et al., 1991; Herut and Krom, 1996; Kubilay et al., 2000,

138 2005; Shao, 2001; Kubilay et al., 2003).

139 A strong northerly Shamal wind can lift up dust from the Tigris-Euphrates Basin of

140 Iran/Iraq and transport it to the Persian (Arabian) Gulf and Arabian Peninsula (Middleton,

141 1986a,b), with severe Arabian dust storms often associated with the summer Shamal (Shao,

142 2001). The Shamal wind is usually generated by a strong baroclinic gradient between a

143 semi-permanent anticyclone over northern Saudi Arabia and a transient cyclones over

144 southern Iran, with strong turbulent winds along the convergence zone that are ideal for 7

145 lifting dust into the atmosphere (Membery, 1983; Goudie and Middleton, 2006). The

146 summer Shamal in JJA blows nearly continuously. In contrast, the rare winter Shamal

147 episodes during NDJFM persists for only one to five days and are characterized by gusty

148 northwesterly winds on the back side of a cold front, associated with an eastward or

149 southward-propagating mid-latitude disturbance from the Mediterranean Sea or Turkey

150 (Perrone, 1979; Vishkaee et al., 2012).

151 In the present study, we investigate the temporal and spatial characteristics of dust

152 storms across Saudi Arabia, with particular focus on the responsible air parcel trajectories

153 and dust source regions, using station and gridded weather observations and remotely-

154 sensed aerosol optical depth (AOD). Based on station observations, we formulate a list of

155 dust storm days for 13 unique locations across Saudi Arabia (Table 1, Figs. 1-2) and

156 examine the seasonal cycle of the dust storm activity. For each station, we develop a series

157 of 84-hour backward trajectories for these dust storm days. From these trajectories, we

158 determine the likely dust source regions. Next, we apply cluster analysis to the trajectories

159 to identify preferred air mass routes associated with the dust storms. Using a reanalysis

160 product and remotely-sensed AOD, we assess the time-evolving synoptic weather pattern

161 that generates the dust storms and their related AOD pattern.

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163 2. Data and Methods

164

165 2.1 Datasets

166 Present weather observations are retrieved from the National Climatic Data Center

167 (NCDC) Hourly Global and U.S. Integrated Surface Hourly Dataset for 2005-2012 at 13 8

168 stations across Saudi Arabia (Figs. 1-2). Here, modest dust activities are characterized by

169 station observations of “widespread dust in suspension in air”, “dust or sand raised by

170 wind”, “well-developed dust/sand whirl”, or “duststorm/sandstorm within sight”, while

171 intense dust activities are characterized by “slight/moderate dust/sandstorm” or “severe

172 duststorm/sandstorm”. For each day in a station’s record, a dust index is computed by

173 weighting hourly reports of modest dust activity by one and intense dust activity by three

174 and then summing the values for each day; while the weight of 3:1 is relatively arbitrary,

175 the results are largely insensitive to the weight selection. For each station, the top 100 dust

176 days are identified during 2005-2012 based on this index, with a dust index criterion that

177 ranges from 4 in Jeddah to 19 in ; dust storms are less common at the former

178 location, along the Red Sea, than the latter location, near the Ad Dahna Desert. Based on

179 hourly dust reports, the most active time of each day is determined (0Z, 3Z, …, 21Z), and

180 backward trajectories are developed using this list of 100 dust days and their central times

181 for each station.

182 Backward trajectories are computed based on six-hourly, three-dimensional wind

183 fields on a 1° x 1° grid from the National Centers for Environmental Prediction (NCEP)

184 Global Data Assimilation System (GDAS) (Kanamitsu, 1989), which applies the spectral

185 Medium Range Forecast (MRF) model. Numerous prior studies have applied GDAS in

186 developing backward air trajectories (e.g. Jorba et al., 2004; Brimelow and Reuter, 2005;

187 Moore et al., 2012). Time-evolving composites of daily sea-level pressure and 500-hPa

188 geopotential height anomalies are created using the NCEP-National Center for Atmospheric

189 Research (NCAR) Reanalysis on a 2.5° x 2.5° grid (Kalnay et al., 1996). 9

190 Daily Deep Blue aerosol optical depth (AOD) at 550 nm for 2005-2012, on a 1° x 1°

191 grid, is obtained from the National Aeronautics and Space Administration (NASA) as part of

192 the Moderate Resolution Imaging Spectroradiometer (MODIS) Terra and Aqua Daily Level-

193 3 dataset (Hsu et al., 2004). The MODIS instruments are onboard the NASA Earth

194 Observing System (EOS) Terra and Aqua satellites (Salomonson et al., 1989; Barnes et al.,

195 1998). The Deep Blue algorithm uses radiances from blue channels on the MODIS

196 instruments. The surface reflectance is minimal at these wavelengths, so aerosols may be

197 detected by an increase in total reflectance and spectral contrast (Hsu et al., 2004, 2006;

198 Ginoux et al., 2012). Estimates of AOD are only considered reliable over bright land

199 surfaces (Marey et al., 2011; Ginoux et al., 2012) and are characterized by substantial

200 uncertainties up to 25-30% (Hsu et al., 2006). More specifically, MODIS-derived AODs have

201 expected errors of ±(0.05+0.15*AOD) over land (Remer et al., 2005, 2008).

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203 2.2 Trajectory model

204 A Lagrangian trajectory model describes the paths of individual, infinitesimally

205 small air parcels as they travel through space and time (Dutton, 1986). The resulting

206 backward trajectories contain information on wind direction, wind speed, and atmospheric

207 stability (Dorling et al., 1992). Here, we apply the Hybrid Single Particle Lagrangian

208 Integrated Trajectory Model from the National Oceanic and Atmospheric Administration

209 (NOAA) Air Resources Laboratory (ARL) (Draxler and Hess, 1998; Rolph, 2003; Draxler,

210 2006; Draxler and Rolph, 2012). Prior studies have applied HYSPLIT backward trajectories

211 to examine the sources and pathways of dust events in China (Lee et al., 2010; Logan et al.,

212 2010), Iran (Vishkaee et al., 2011), Spain (Cabello et al., 2012; Valenzuela et al., 2012), the 10

213 Nile Delta (Prasad et al., 2010), and Indo-Gangetic Plains (Prasad and Singh, 2007), among

214 other regions.

215 Backward trajectories are computed using the Real-time Environmental

216 Applications and Display System (READY) website (Rolph, 2012). HYSPLIT uses the u- and

217 v-component of the wind, temperature, height, and pressure at different atmospheric levels,

218 typically from a reanalysis product (Banacos and Ekster, 2010) or operational model runs

219 (Moore et al., 2012), to compute backward trajectories for air parcels at specified heights above

220 the ground. For the current study, GDAS output is provided to the HYSPLIT model to compute

221 84-hour backward trajectories, using a dust arrival height of 500-m. Backward air trajectories

222 are typically computed for a maximum duration of three to four days, since excessive errors can

223 develop over longer time scales (Stohl, 1998). For all trajectories, hourly data is saved for height

224 above the ground, relative humidity, and atmospheric pressure (used to compute vertical motion).

225 For each of 13 Saudi Arabian stations, backward trajectories are computed from that station’s set

226 of 100 dust days during 2005-2012, and the trajectory ensemble option of HYSPLIT is applied

227 which results in 27 trajectories per day, or a total of 2700 backward trajectories per station. By

228 computing backward trajectories as ensembles, the inherent uncertainty of trajectory calculations

229 is addressed (Vishkaee et al., 2012). Each member of a trajectory ensemble is computed by

230 offsetting the meteorological GDAS data by a pre-determined grid factor, consisting of one grid

231 cell in the horizontal and 0.01 sigma units in the vertical, resulting in 27 ensemble members

232 based on all potential offsets in the X, Y, and Z directions.

233 For each of the six major desert regions noted in Section 1 (Rub Al Khali, An Nafud,

234 Ad Dahna, Sahara, Iraqi, and Syrian Deserts), a mask file is created with its approximate

235 spatial extent (Fig. 1). For all 2700 backward trajectories for each of 13 stations, the 11

236 percentage of trajectories passing over each desert is computed, along with the time spent

237 over the desert region during the 84-hour trajectories, in order to identify potential dust

238 source regions. In a similar fashion, Estellés et al. (2007) and Toledano et al. (2009)

239 identified air mass origin sectors by considering the amount of time spent over source

240 regions through trajectory analysis.

241 Each trajectory is classified as anticyclonic, neutral, or cyclonic, roughly following

242 the approach of Dong et al. (2011). First, the angle (α84) is computed between the latitude

243 and longitude at t0 (time of the dust storm event) and the latitude and longitude at t-84

244 (84-hours before the event). The Euclidean vector is determined between the former point

245 and latter point and its angle is computed, relative to true north. This is repeated for each

246 subsequent hour (e.g. t0 versus t-83 for α83). Then, the differences between neighboring

247 angles (e.g. α83-α84, α82-α83, …, α0-α1) are summed. If the sum is greater than 30 or less than

248 -30, then the trajectory is classified as anticyclonic or cyclonic, respectively; otherwise, it is

249 classified as neutral.

250

251 2.3 Cluster analysis

252 Cluster analysis is a multivariate statistical method for exploring structure within a

253 dataset (Anderberg, 1973; Everitt, 1980). In particular, non-hierarchical partitional

254 clustering techniques, such as the K-means clustering algorithm (Moody and Galloway,

255 1988; Kaufman and Rousseeuw, 1989; Dorling et al., 1992), are well designed for analyzing

256 large datasets (Čolović-Daul, 2007). Moody (1986) and Moody and Galloway (1988)

257 introduced the application of cluster analysis to air trajectories, leading to a series of

258 subsequent studies of trajectory clustering (e.g. Čolović-Daul, 2007; Žabkar et al., 2008; 12

259 Markou and Kassomenos, 2010). Briefly stated, the K-means method iteratively allocates a

260 set of objects, such as trajectories, among a predetermined number of clusters until the

261 sum of distances from each object to its cluster centroid over all clusters is minimized

262 (Žabkar et al., 2008).

263 According to the K-means algorithm, a set of trajectories is grouped into K clusters

264 according to a distance measure of metric space. Two common measures, also known as

265 metrics or distance functions, are the sum of square distance on the Euclidean plane

266 between end points (Moody and Galloway, 1988) and sums of the great-circle distance on a

267 Euclidean sphere between trajectory end points (Lin et al., 2001; Jorba et al., 2004). A

268 metric space is defined for quantifying similarities or differences between trajectories. For

269 each cluster, its cluster centre is determined as the mean trajectory for that cluster. Based

270 on the cluster centres, the distance between trajectories is computed. Trajectories are

271 grouped so as to minimize the variance of the distance between trajectories in the same

272 cluster and maximize the variance for trajectories belonging to different clusters (Crawford

273 et al., 2009).

274 One of the challenges with the K-means clustering technique is to determine the

275 appropriate number of clusters. The silhouette coefficient, which is a dimensionless

276 measure of both internal cluster cohesion and external cluster separation, can be used to

277 determine the appropriate number of clusters (Anderberg, 1973; Rousseaw, 1987). When

278 applied to trajectories, this method assesses how well the trajectories are clustered around

279 centroids into unique groupings and how distinct these clusters are from each other

280 (Anderberg, 1973). For each ith trajectory, the silhouette value is computed as:

281 =−()(,) . 13

282 If we assume that the ith trajectory is assigned to cluster A, then a(i) is the average

283 dissimilarity of the ith trajectory to all other trajectories in cluster A and b(i) is the average

284 dissimilarity of the ith trajectory to all trajectories in neighboring clusters, B. The silhouette

285 value ranges from -1 to +1. If S(i) is close to -1, then the trajectory is misclassified, but if

286 S(i) is close to +1, then the trajectory is well classified. The average Silhouette Coefficient,

287 computed as the mean value of S for all trajectories, is a measure of how well the cluster

288 structure fits the dataset and can be used to identify the ideal number of clusters to assign

289 to the dataset (Kaufman and Rousseeuw, 2005). The silhouette method generally leads to

290 clearer results than the traditional approach of identifying an elbow in a curve of the

291 number of clusters versus the within-cluster variance, particularly given that many curves

292 lack a distinct elbow. As pointed out by Salvador and Chan (2004), most studies that apply

293 the elbow approach to determine the appropriate number of clusters lack a clear statistical

294 justification.

295 In the current study, HYSPLIT backward trajectories (100 dust storm days * 27

296 ensemble members/day = 2700 trajectories per station) are clustered in Matlab using the

297 K-means technique based on the squared Euclidean distance metric, with 20 replicates.

298 Mean Silhouette Coefficients are then computed for cluster sizes ranging from three to ten,

299 with the highest coefficient determining the optimal number of clusters to apply. Any two

300 84-hour trajectories can be compared by computing the root-mean-square-difference

301 (RMSD) between their 84 latitudes and against between their 84 longitudes, and these two

302 values are then averaged for a net RMSD. The mean RMSD can be compared within-cluster

303 and across-cluster to assess the consistency within a cluster and uniqueness from other

304 clusters. 14

305

306 3. Results

307

308 3.1 Seasonal cycle of dust storms

309 Based on NCDC data for 13 Saudi Arabian stations (Table 1), the mean seasonal

310 cycle of dust storm activity is computed (Fig. 2). Averaged among these stations, Saudi

311 Arabian dust storms are most frequent from mid-winter to early summer, with 77% of dust

312 storms occurring during February-June. Dust storms are most active during March (19%)

313 and least active during November (1%). The pattern of preferred timing for dust storms is

314 heterogeneous across the country. Dust storm frequency peaks in mid-winter (February)

315 in proximity to the lower Sarawat Mountains (e.g. Jeddah and Al-Baha), in early spring

316 (April-May) over northern Saudi Arabia around the An Nafud and Syrian Deserts (e.g.

317 Turaif, Arar), and in early summer (June) over eastern Saudi Arabia around the Ad Dahna

318 Desert (e.g. Riyadh, Al-Ahsa). The station located at the highest elevation (1652 m in the

319 Sarawat Mountains), Al-Baha, exhibits a distinct bimodal peak in dust storm activity in

320 February-March and June-July; this is later attributed to south-southeasterly and

321 northwesterly trajectories, respectively.

322

323 3.2 Silhouette Coefficients

324 By computing the mean Silhouette Coefficients for a range from three to ten clusters

325 at each station, the optimal number of clusters for representing the pool of 2700 backward

326 trajectories at each station is determined (Fig. 3). In general, as the number of clusters

327 increases, the mean Silhouette Coefficient declines rather linearly, from 0.52±0.03 (mean ± 15

328 one standard deviation) at three clusters to 0.41±0.03 at ten clusters. For most stations,

329 three clusters are the best fit, with the exception of four clusters for Arar, Turaif, and

330 Jeddah and five clusters for Hafr Al-Batin. In agreement with Philipp et al. (2007), the

331 Silhouette Coefficient (along with other metrics) does not always provide a distinct

332 determination of the optimal number of clusters, but the selection of three to five clusters

333 is considered a manageable number for analysis and successfully leads to clear,

334 independent groupings of backward trajectories.

335

336 3.3 Trajectory clusters

337 According to the K-means clustering of the backward trajectories for 13 Saudi

338 Arabian stations and resulting mean Silhoutte Coefficients, the preferred 84-hour

339 trajectories for dust storms are grouped into three to five clusters and presented in Figs. 4-

340 6. In these figures, trajectories are assigned a color of red, green, blue, orange, or yellow in

341 order from the greatest AOD (red) to least AOD (yellow) measured at the station at time t0,

342 according to MODIS (as discussed later in Section 3.4). Furthermore, Table 1 includes the

343 percentage of trajectories for each station that pass over specified deserts, along with the

344 mean number of hours spent over the deserts; these statistics hint at potential dust source

345 regions. Based on the percentage of backward trajectories that pass over certain desert

346 regions in Saudi Arabia, the desert regions, in order from most to least important, are Rub

347 Al Khali (32%), Sahara (26%), Iraqi (25%), Ah Dahna (20%), Syrian (15%), and An Nafud

348 (13%). For Saudi Arabia, the Rub Al Khali is the most prominent local source of dust, while

349 the Saharan Desert is the greatest remote dust source. Further analysis indicates that the 16

350 Iranian Deserts are not substantial contributors of dust to Saudi Arabia, since few back

351 trajectories display a northeast to southwest path.

352 The individual trajectories for six select stations are shown in Fig. 7 to illustrate how

353 the K-means clustering technique grouped similar trajectories. For instance, the three

354 primary trajectories for dust storms in Sharorah (Figs. 4a, 7a) are northerly over the Rub Al

355 Khali Desert (39%, green), southeasterly from the Gulf of Aden and Yemen (33%, blue), and

356 northwesterly across the Mediterranean Sea, Iraqi Deserts, and Rub Al Khali Desert (28%,

357 red). From Fig. 7, it is evident that there is spread among the trajectories within a single

358 cluster but they generally follow a similar track in terms of distance and rotation. For

359 Sharorah, air parcels travel a longer distance on the northwesterly Mediterranean track

360 than the northerly Rub Al Khali track, while the southeasterly trajectories are largely

361 tropical maritime in nature. Based on Fig. 7, it is evident that the individual trajectories are

362 reasonable clustered, thereby supporting the relatively high Silhouette Coefficients. For

363 the 13 stations, the mean within-cluster RMSD and across-cluster RMSD are 4.67 and 9.61,

364 respectively, with a ratio between the two calculations of 2.06:1 (ranging from 1.73:1 for

365 Hail to 2.27:1 for Turaif). Clearly, trajectories within a single cluster are self-consistent and

366 unique from those in other clusters.

367 The vast majority of dust storm trajectories for Saudi Arabia are anticyclonic. On

368 average among the 13 stations, 56% of the 35,100 analyzed backward trajectories are

369 anticyclonic, 27% are neutral, and 17% are cyclonic. For Wadi Al-Dawasser and Riyadh, in

370 central Saudi Arabia, the dominant trajectory rotates clockwise out of Iraq (Fig. 4b,c), such

371 that 76% and 73% of their total trajectories are anticyclonic in nature, respectively. For 17

372 Tabuk (and other locations in northwestern Saudi Arabia), 33% of total trajectories are

373 cyclonic in nature, primarily those originating over the Mediterranean Sea (Fig. 5b).

374 Stations in Fig. 4, labeled here as Type I stations, generally have local dust sources

375 within Saudi Arabia, namely the Rub Al Khali (Sharorah, Wadi Al-Dawasser, Najran, and Al-

376 Baha), Ad Dahna (Riyadh), and An Nafud (Hail) Deserts (Table 1). The position of Najran,

377 Sharorah, and Wadi Al-Dawasser along the western fringe of the Rub Al Khali Desert makes

378 this desert a dominant source of dust to those locations. For Al-Baha, along the coast of the

379 Red Sea, the two dominant trajectories are south-southeasterly from Yemen and

380 northwesterly from the northern Sahara Desert (Fig. 4e), with preferred peaks in February-

381 March and June-July, respectively. These two preferred paths explain the bimodal seasonal

382 cycle of dust activity at Al-Baha as noted in Fig. 2. The northwesterly trajectory is

383 associated with the summer Shamal.

384 In contrast, stations in Figs. 5-6 generally receive their dust loadings from remote

385 sources outside of the country (Table 1). The primary remote dust sources are the Saharan

386 Desert, particularly for the “Type II” stations of Yenbo, Tabuk, Jeddah, and Turaif (Fig. 5),

387 and the Iraqi and Syrian Deserts, particularly for the “Type III” stations of Arar, Hafr Al-

388 Batin, and Al-Ahsa (Fig. 6). The Saharan Desert likely contributes the most dust to stations

389 in west-northwestern Saudi Arabia. For example, 68% of Yenbo’s trajectories cross the

390 Saharan Desert for a mean of 26.1 hours (Table 1). In eastern Saudi Arabia, close to the

391 Persian (Arabian) Gulf, the Iraqi Deserts are critical sources of dust, with 60% and 50% of

392 backward trajectories crossing these deserts for Hafr Al-Batin and Al-Ahsa, respectively

393 (Table 1). For stations bordering the northern Red Sea, such as Yenbo and Tabuk (Fig.

394 5a,b), the Mediterranean Sea track is quite active, with roughly three-fourths of total 18

395 trajectories crossing the sea with a preferred timing in mid-winter to early spring

396 (February-April). These dust events are associated with mid-latitude cold season cyclones

397 and their associated cold fronts, carrying Saharan dust to the region.

398

399 3.4 Aerosol Optical Depth statistics

400 The intensity of dust storms, in terms of aerosol loading, is assessed by quantifying

401 the mean AOD on dust storm days at each of 13 locations (Table 2). The mean AOD ranges

402 substantially from 0.43 at Tabuk, in northwest Saudi Arabia, to 1.10 at Najran, in southwest

403 Saudi Arabia. The highest AOD, on average close to 1.00, is associated with stations largely

404 impacted by the Rub Al Khali and Iraqi Deserts, namely Najran, Sharorah, Wadi Al-

405 Dawasser, and Hafr Al-Batin. In particular, the anticyclonic trajectory clusters that cross

406 the Rub Al Khali Desert into Sharorah (Fig. 4a, red), Wadi Al-Dawasser (Fig. 4b, red), and

407 Najran (Fig. 4d, red) generate an AOD in excess of 1.10, making these dust paths the most

408 efficient. In contrast, stations with trajectories that largely come off the Sahara Desert are

409 characterized by low AOD on dust storm days, including Yenbo and Tabuk with a mean

410 AOD of 0.52 and 0.43, respectively. As dust clouds travel a long distance from the Sahara

411 Desert to Saudi Arabia, much of the aerosols are lost through wet and dry deposition.

412 Trajectories that originate over the Mediterranean Sea and cross the Sahara Desert are the

413 least efficient dust paths, as evident by low AOD values at Tabuk (Fig. 5b, blue) and Yenbo

414 (Fig, 5a, blue) of 0.36 and 0.39, respectively. In general, stations with local dust sources

415 within Saudi Arabia (Type I) are characterized by greater AOD values during dust storms

416 than stations with remote dust sources from outside of the country, especially Type II. 19

417 For stations dominated by dust from the Rub Al Khali Desert, namely Najran,

418 Sharorah, Wadi Al-Dawasser, and Al-Baha, the trajectory cluster with the lowest mean

419 relative humidity in the final 24-hours is associated with the highest AOD, as the air mass

420 passes over favorable desert conditions. For example, the red and green trajectory clusters

421 for Sharorah (Fig. 4a) result in a mean AOD of 1.32 and 1.02 (Table 2), respectively. Their

422 paths are similar, yet the mean AOD is substantially different. Air masses associated with

423 the red trajectory are characterized by 10% lower relative humidity, favoring dust

424 production.

425

426 3.5 Synoptic and AOD characteristics of dust storms

427 The synoptic pattern (Fig. 9) that generates dust storms and the associated

428 characteristics of AOD (Fig. 8) are examined for three select stations, Najran (Type I), Al-

429 Ahsa (Type III), and Tabuk (Type II), which have unique dominant dust source regions of

430 the Rub Al Khali, Iraqi, and Sahara Deserts, respectively (Table 1). In particular, the

431 analysis focuses on the northerly trajectories at Najran (Fig. 4d, red), the short-distance

432 northwesterly trajectories at Al-Ahsa (Fig. 6c, green), and the long-distance northwesterly

433 trajectories at Tabuk (Fig. 5b, blue). The synoptic environment responsible for dust storms

434 in each of these three locations is found to be notably unique.

435 In the case of Najran, the anticyclonic trajectory initiates at 84-hours prior to the

436 dust events over southern Iraq, generating modest dust lifting, but as the trajectory passes

437 over the Rub Al Khali Desert, the mean AOD increases dramatically, indicating that this

438 desert is the primary source of dust (Fig. 8a-d). Following this specific trajectory cluster,

439 the mean AOD increases substantially from 0.72 on d-2 (2 days prior) to 1.02 on d-1 as the 20

440 air mass crosses the Rub Al Khali Desert (Fig. 10j). The anticyclonic trajectory is attributed

441 to a surface high-pressure system that propagates eastward from the eastern

442 Mediterranean Sea on d-2 (two days prior to the dust event) to the Caspian Sea at d0 (day

443 of the dust event) (Fig. 9a-c), while intensifying in the mid-troposphere (Fig. 9d-f). Winds

444 on the eastern and southern sides of this anticyclone stir up dust over the Rub Al Khali

445 Desert.

446 For Al-Ahsa, the northwesterly flow associated with dust storms is generated by the

447 pressure gradient between a surface anticyclone over North Africa and the Mediterranean

448 Sea and a surface cyclone east of the Caspian Sea (Fig. 9g-i). As these systems propagate

449 eastward, dust is channeled out of Iraq into eastern and southern Saudi Arabia (Fig. 8e-h).

450 The upper-level height anomalies are quite weak and dampen over time, leading up to the

451 dust event (Fig. 9j-l). As the air mass passes over the Iraqi Deserts, the mean AOD along

452 this trajectory cluster increases dramatically from 0.41 to 0.71 from d-2 to d-1 (Fig. 10a).

453 The mechanism for dust storms in Tabuk, generated by the long-range

454 northwesterly trajectory that originates in the Mediterranean and crosses the northern

455 Saharan Desert, is substantially different than that of Najran or Al-Ahsa. During the mid-

456 winter, the active Mediterranean storm track supports deep cyclones (-10 hPa anomalies)

457 passing over the Mediterranean and Black Seas, with an associated cold front that lifts dust

458 from the northern Sahara and carries it into northern Saudi Arabia, including Tabuk (Figs.

459 8i-k, 9m-o). A deep upper-level trough (anomalies < -70 m) shifts slightly eastward over

460 the Mediterranean Sea as its positive tilt on d-2 becomes neutral on d0 at the time of the

461 dust storm (Fig. 9p-r), indicative of a strengthening surface cyclone.

462 21

463 3.6 Along-trajectory meteorological conditions

464 Temporal changes in height above the ground of the air parcels, relative humidity,

465 and vertical motion are examined along the 84-hour backward trajectory clusters for four

466 select stations: Al-Ahsa, Riyadh, Arar, and Najran (Fig. 10). In general, air parcels along

467 trajectories that originate over the Mediterranean Sea are found at altitudes of 2-4 km at t-

468 84. This is most evident for the long-range northwesterly trajectories at Al-Ahsa (Fig. 6c,

469 blue), which initiate over the Mediterranean Sea at altitudes in excess of 4 km (Fig. 10a,

470 blue). The parcels rapidly descend during the 84 hours, particularly in the final 24 hours as

471 they cross the An Nafud and Iraqi Deserts. Dust storms at Al-Ahsa are characterized by the

472 greatest trajectory-mean subsidence of +2.45 hPa/hour (Fig. 10c) of any station. Typically,

473 air parcels remain at low altitudes of 400-1200 m, within the atmospheric planetary

474 boundary layer, for south-southeasterly trajectories originating over the Gulf of Aden,

475 Arabian Sea, Yemen, and Oman. For dust storms reaching Najran, tracked air parcels

476 remain at or below 1 km altitude during the entire 84-hour period (Fig. 10j) for all three

477 trajectory clusters (Fig. 4d), particularly the southeasterly trajectory from the Gulf of Aden

478 (blue). The southern Sarawat Mountains contribute towards a lifting of the air parcels in

479 the final 24 hours for dust storms in southwest Saudi Arabia, such as Najran (Fig. 10j,l),

480 Sharorah, and Wadi. Likewise, stations with primarily local dust sources, within Saudi

481 Arabia (Fig. 4), usually have trajectories at low altitudes, unlike dust events that originate

482 from the Mediterranean storm track.

483 The along-trajectory mean relative humidity ranges from 27.9% in Riyadh to 40.4%

484 in Najran, with the lowest relative humidity for locations in central Saudi Arabia, close to

485 the Ad Dahna Desert (e.g. Riyadh, Wadi Al-Dawasser, and Hail), and the highest for 22

486 locations in western Saudi Arabia, in close proximity to the Red and Mediterranean Seas

487 (e.g. Najran, Jeddah, and Turaif) (Fig. 10). For air parcels following a trajectory from the

488 Mediterranean Sea, once they pass over Saudi Arabia, the relative humidity abruptly

489 declines, as noted in Riyadh (Fig. 10e, blue). For Arar, trajectories from a maritime

490 environment, like the Mediterranean Sea (Fig. 6a, blue), or cooler environment, like Eastern

491 Europe (Fig. 6a, orange), exhibit relatively high relative humidity, in contrast to trajectories

492 that mostly pass over the Syrian (Fig. 6a, red) and Iraqi Deserts (Fig. 6a, green) (Fig. 10h).

493

494 4. Discussion and Conclusions

495 In the current study, backward trajectories are generated and clustered through the

496 K-means technique, based on mean Silhouette Coefficients, for dust storm days at 13

497 stations across Saudi Arabia. Furthermore, temporal and spatial patterns of remotely-

498 sensed AOD and meteorological conditions are assessed for these dust events to

499 understand the mechanisms and sources of the dust loading. Dust storms are most

500 common in Saudi Arabia during February-June, with a peak in March. Their activity

501 reaches a maximum during the mid-winter along the southern coast of the Red Sea (with

502 trajectories originating over Yemen and the Gulf of Aden), spring in northern Saudi Arabia,

503 and early summer in eastern Saudi Arabia, in the vicinity of the Ad Dahna Desert.

504 During February-April, cold fronts associated with Sharav cyclones from the

505 Mediterranean Sea can transport Saharan dust to Saudi Arabian stations along the northern

506 coast of the Red Sea, as verified from remotely-sensed AOD. Our trajectory-based finding of

507 the importance of cool-season Mediterranean cyclones to Saudi Arabian dust storms is

508 consistent with prior studies by Ganor et al. (1991), Herut and Krom (1996), Kubilay et al. 23

509 (2000, 2005), Shao (2001), and Kubilay et al. (2003). Likewise, Vishkaee et al. (2011)

510 indicated that dynamical lifting during the cool season from cold fronts is a primary trigger

511 of dust storms. The Mediterranean trajectories that support Saudi Arabian dust storms

512 have initial parcel altitudes of 2-4 km, in support of prior studies that Saharan dust can be

513 lifted to heights of several kilometers above the ground due to strong winds (Escudero et

514 al., 2005, 2011; Dayan et al., 1991; Alpert and Ganor, 1993; Conte et al., 1996; Prospero,

515 1996). Type II stations, such as Tabuk, generally experience a peak in dust activity during

516 April, associated with Mediterranean cyclones and transported Saharan Dust. Diurnal

517 heating and resulting turbulence are likely critical for the early summer dust storms in

518 eastern Saudi Arabia around the Ad Dahna Desert (Middleton, 1986; Vishkaee et al., 2011).

519 Strong heating over the Iraqi and Syrian Deserts lead to active dust periods over Type III

520 stations (e.g. Al-Ahsa) in June.

521 According to the backward trajectory analysis, the primary dust source regions,

522 from most to least important, are the Rub Al Khali, Saharan, Iraqi, Ad Dahna, Syrian, and An

523 Nafud Deserts. The primary local dust source, within the country, is the Rub Al Khali

524 Desert, while the primary remote dust sources are the Saharan Desert, for western Saudi

525 Arabia, and Iraqi Deserts, for northern / eastern Saudi Arabia. These findings agree with

526 studies of TOMS data by Goudie and Middleton (2001, 2006) and Giles (2005), which

527 identify the Saharan Desert and Rub Al Khali as the most prolific dust source regions in the

528 world. Based on MODIS data, the highest AOD is achieved during Saudi Arabian dust

529 storms that originate from the Rub Al Khali and Iraqi Deserts. The Saharan Desert is an

530 important remote source of dust, but Saudi Arabian dust storms associated with Saharan

531 dust rarely achieve large values of AOD. It is acknowledged that MODIS AOD has 24

532 substantial expected errors (Remer et al., 2005, 2008; Hsu et al., 2006), and in coastal

533 regions bordering the Red Sea, the satellite might also be detecting marine aerosols in

534 addition to Aeolian dust (Yu et al., 2012).

535

536 Acknowledgements

537 This study was funded by the King Saud University. The authors gratefully

538 acknowledge the NOAA Air Resources Laboratory for the READY website

539 (http://ready.arl.noaa.gov) for generating HYSPLIT trajectories used in this publication.

540 The authors are thankful for helpful discussions with Ms. Yan Yu, Dr. Zhengyu Liu, and Dr.

541 Guangshan Chen and comments from three anonymous reviewers. Nelson Center for

542 Climatic Research publication #.

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554 25

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847

848

849

850

851

852

853 38

854 Figure Captions

855

856 Figure 1. Map of the Middle East and North Africa, with shaded elevation in meters. The

857 source of the 0.25° x 0.25° elevation data is TerrainBase (TBASE) from the National Center

858 for Atmospheric Research (NCAR), obtained through the University of Washington. The 13

859 Saudi Arabian stations analyzed in this study are identified by large dots. Red, green, and

860 yellow dots indicate stations with dust sources primarily from the Rub Al Khali, Sahara, and

861 Iraqi Deserts, respectively. The six primary desert regions (Sahara, Rub Al Khali, An Nafud,

862 Ad Dahna, Syrian, and Iraqi) are labeled and identified with small dots.

863

864 Figure 2. Mean seasonal cycle of the percentage frequency of dust storms at 13 Saudi

865 Arabian stations during 2005-2012. The dark bars indicate the most active month for each

866 station. On the map, the stations’ locations are shown, along with the most active month.

867

868 Figure 3. Mean silhouette coefficients for each of 13 Saudi Arabian stations for trajectory

869 cluster sizes ranging from three to ten. Peaks in these silhouette curves indicate the

870 optimum cluster size for stations, including three (red lines) for Sharorah, Wadi Al-

871 Dawasser, Riyadh, Najran, Al-Baha, Hail, Yenbo, Al-Ahsa, and Tabuk; four (blue lines) for

872 Arar, Turaif, and Jeddah; and five (green lines) for Hafr Al-Batin.

873

874 Figure 4. K-means cluster analysis of 84-hour backward trajectories (at 500-m) for 100

875 dust storm days during 2005-2012 at (a) Sharorah, (b) Wadi Al-Dawasser, (c) Riyadh, (d)

876 Najran, (e) Al-Baha, and (f) Hail. These stations primarily have local dust sources within 39

877 Saudi Arabia. For these stations, the trajectories are grouped into three clusters, shown in

878 red, green, and blue, with the percent frequency and dominant month of each trajectory

879 cluster shown in the small black boxes. For each cluster, a representative trajectory is

880 shown based on the maximum within-cluster silhouette coefficient. The grey shading

881 indicates the percentage of total backward trajectories passing through each grid cell.

882

883 Figure 5. K-means cluster analysis of 84-hour backward trajectories (at 500-m) for 100

884 dust storm days during 2005-2012 at (a) Yenbo, (b) Tabuk, (c) Jeddah, and (d) Turaif.

885 These stations primarily have remote dust sources outside of Saudi Arabia, with a

886 significant component from the Sahara Desert. For these stations, the trajectories are

887 grouped into three or four clusters, shown in red, green, blue, and orange, with the percent

888 frequency and dominant month of each trajectory cluster shown in the small black boxes.

889 For each cluster, a representative trajectory is shown based on the maximum within-

890 cluster silhouette coefficient. The grey shading indicates the percentage of total backward

891 trajectories passing through each grid cell.

892

893 Figure 6. K-means cluster analysis of 84-hour backward trajectories (at 500-m) for 100

894 dust storm days during 2005-2012 at (a) Arar, (b) Hafr Al-Batin, and (c) Al-Ahsa. These

895 stations primarily have remote dust sources outside of Saudi Arabia, primarily from the

896 Iraqi and Syrian Deserts. For these stations, the trajectories are grouped into three or four

897 clusters, shown in red, green, blue, and orange, with the percent frequency and dominant

898 month of each trajectory cluster shown in the small black boxes. For each cluster, a

899 representative trajectory is shown based on the maximum within-cluster silhouette 40

900 coefficient. The grey shading indicates the percentage of total backward trajectories

901 passing through each grid cell.

902

903 Figure 7. Based on the trajectory clusters from Figs. 4-6, individual backward trajectories

904 are shown for (a) Sharorah, (b) Riyadh, (c) Hail, (d) Hafr Al-Batin, (e) Arar, and (f) Yenbo

905 using the same color scheme as in Figs. 4-6. For each station, every third trajectory from

906 the pool of 2700 is shown to limit clutter.

907

908 Figure 8. (a-d) Composite for Najran of daily-mean MODIS AOD for dust storm days during

909 2005-2012 for the northerly trajectory cluster (red, Fig. 4d) over the Ad Dahna and Rub Al

910 Khali on (a) d-3 (three days prior to dust storm), (b) d-2, (c) d-1, and (d) d0 (day of dust

911 storm). (e-h) Composite for Al-Ahsa of daily-mean MODIS AOD for dust storm days for the

912 northwesterly trajectory cluster (green, Fig. 6c) over the Iraqi Desert on (e) d-3, (f) d-2, (g)

913 d-1, and (h) d0. (i-k) Difference in composited daily-mean MODIS AOD for dust storm days

914 at Tabuk for its northwesterly trajectory cluster (blue, Fig. 5b) over the Mediterranean Sea

915 and Saharan Desert, consisting of (i) [d-2] minus [d-3], (j) [d-1] minus [d-2], and (k) [d0]

916 minus [d-1]. The upper and lower color bars pertain to (a-h) and (i-k), respectively. For

917 Tabuk, changes in AOD are shown to clearly illustrate their link to a passing cold front.

918

919 Figure 9. Composite of daily (a-c, g-i, m-o) sea-level pressure (hPa) and (d-f, j-l, p-r) 500-

920 hPa height (m) anomalies on dust days. Results are shown for (a-f) Najran’s northerly

921 trajectory cluster (red, Fig. 4d), (g-l) Al-Ahsa’s northwesterly trajectory cluster (green, Fig.

922 6c), and (m-r) Tabuk’s northwesterly trajectory cluster (blue, Fig. 5b). Anomalies, 41

923 computed from the NCEP-NCAR Reanalysis, are shown for d-2 (two days prior to the dust

924 event), d-1, and d0 (day of the dust event) in the first, second, and third columns,

925 respectively. The number of composited dust days is 28, 44, and 15 for Najran, Al-Ahsa,

926 and Tabuk, respectively. Hatching in the sea-level pressure anomaly panels indicates

927 MODIS AOD≥0.6 for Najran and Al-Ahsa and ≥0.45 for Tabuk. Surface cyclone and

928 anticyclone centers and associated fronts are also displayed in the sea-level pressure

929 anomaly panels.

930

931 Figure 10. Mean height above the ground (m), relative humidity (%), and vertical motion

932 (hPa/hour) of the tracked air parcels for (a-c) Al-Ahsa, (d-f) Riyadh, (g-i) Arar, and (j-l)

933 Najran, according to the 84-hour backward trajectories in Figs. 4-6 (using the same

934 trajectory colors). Data is shown hourly from 84 hours prior to the dust storm to the time

935 of the dust events (time 0). In (a,d,g,i), color dots indicate mean AOD following the relevant

936 trajectory cluster, with dot sizes increasing for intervals of 0.00-0.35, 0.36-0.55, 0.56-0.75,

937 and 0.76-1.20 (see legend in panel f).

938

939 Table Captions

940

941 Table 1. List of the 13 Saudi Arabian stations used in this study and their latitude,

942 longitude, and elevation (m). For each station, the percentage of total dust storms that

943 cross over specific deserts, along with the mean number of hours over those deserts, from

944 the 84-hour backward trajectories in Figs. 4-5 is given; italics indicate the highest values

945 per station. 42

946

947 Table 2. Mean MODIS AOD at each of 13 stations on dust storm days, for each trajectory

948 cluster shown in Figs. 4-5 and weighted across all clusters. Trajectory clusters that result

949 in a mean AOD ≥ 1.10 are identified in bold. Below each AOD value, two percentages are

950 provided, which represent the percentage of trajectories that achieve an AOD≥1.0 and ≥0.8,

951 respectively.