Multidisciplinary Chemistry Journals

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FREE access to top articles Inspiring Chemistry A journal of www.angewandte.org

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Chair of the Editor-in-Chief: Editorial Board:

Peter Gölitz Alois Fürstner (Mülheim)

Highlights: Editorial Board:

• Free App available: bit.ly/CHEMAPPS Annette G. Beck-Sickinger Andreas Kreimeyer - “The Angew. Chem. App is fantastic. (Leipzig) (Ludwigshafen) Very intuitive and informative. It is a Matthias Beller (Rostock) Christof M. Niemeyer very nice way to quickly find content Hans-Joachim Böhm (Basel) (Dortmund) relevant to one’s work” Stefan Buchholz (Essen) Wolfgang Parak (Marburg) (Chad A. Mirkin) Thomas Carell (Munich) Ferdi Schüth (Mülheim) - “I use the Angewandte app all the Claus Feldmann (Karlsruhe) Petra Schwille (Dresden) time. I love it! It’s great to be able Roland Fischer (Bochum) Martin Suhm (Göttingen) to download entire issues for offline Thomas Geelhaar (Darmstadt) Brigitte Voit (Dresden) reading.” (Phil S. Baran) Stefan Grimme (Bonn) Herbert Waldmann (Dortmund) • Follow us on Twitter and Facebook Hansjörg Grützmacher (Zurich) Hanno Wild (Wuppertal)

International Advisory Board: Comprising 44 world-renowned scientists, including Nobel Laureates Roald Hoffmann, Jean-Marie Lehn, Ryoji Noyori, and Ahmed Zewail.

“Angewandte Chemie combines a unique portfolio of publication types in a highly attractive format. Reading the journal daily online ensures that I keep up to date with the progress in my own fields of research and all other areas of chemistry.” (François Diederich)

2 Mixed Transition Metal Oxides: Design, Synthesis, and Energy Related Applications Changzhou Yuan, Hao Bin Wu, Yi Xie*, Xiong Wen (David) Lou* Full of energy: Recent advances in the rational design and synthesis of mixed transition-metal oxides (MTMOs, designated

as AxB3−xO4) with controllable compositions and structures and their applications in various electrochemical energy storage/ conversion technologies are summarized and discussed (see picture). Future trends and prospects for their further Angew. Chem. Int. Ed. DOI: 10.1002/anie.201303971 development are also discussed.

Chemistry with Graphene and Graphene Oxide – Challenges for Synthetic Chemists Siegfried Eigler*, Andreas Hirsch* The well-controlled synthesis of new graphene and graphene oxide derivatives as well as determination of the atomic structure are key challenges for synthetic chemists. Structure–property relationships must be exploited to use the full potential of graphene derivatives in upcoming applications. This Review focuses on

Angew. Chem. Int. Ed. concepts in the chemistry of graphene and graphene oxide with the DOI: 10.1002/anie.201402780 aim of encouraging chemists to enhance the field of research.

Sulfur(VI) Fluoride Exchange (SuFEx): Another Good Reaction for Click Chemistry Jiajia Dong, Larissa Krasnova, M. G. Finn, K. Barry Sharpless* Old chemistry in new glory: Sulfonyl fluoride exchange (SuFEx) forges rugged inorganic links between carbon centers. Like most click reactions, it is an old process now improved to allow the underappreciated sulfate connection to be made for a variety of

Angew. Chem. Int. Ed. purposes. The various exchange events uniquely enabled by the DOI: 10.1002/anie.201309399 use of fluoride are highlighted here in orange.

Engineered Nanoparticles for Drug Delivery in Cancer Therapy Tianmeng Sun, Yu Shrike Zhang, Bo Pang, Dong Choon Hyun, Miaoxin Yang, Younan Xia* On the way to nanomedicine: Considerable advances in the development of nanoparticles for cancer therapy have been made in recent years. Nanoparticle-based drug-delivery systems offer advantages with regard to multidrug resistance, systemic delivery, and clearance, and enable for example specific tumor targeting Angew. Chem. Int. Ed. and controlled release of therapeutic agents.use of fluoride are DOI: 10.1002/anie.201403036 highlighted here in orange.

3 ChemPubSoc Europe’s A journal of flagship journal www.chemeurj.org Free Sample Copy

Chair of the Editor-in-Chief: Editorial Board:

Neville Compton Jan-Erling Bäckvall Stockholms Universitet

Highlights: Editorial Board: • Celebrating 20 years of publication. Comprising 59 world-renowned scientists. Discover for free at Honorary Members: http://bit.ly/CEJ20: Vincenzo Balzani (Università degli Studi di Bologna), Italy • Top 20 all time most cited papers Gerhard Ertl (Fritz-Haber-Institut, Berlin), Germany • Top 20 most cited Reviews and Jean-Marie Lehn (Université de Strasbourg/Collège de Minireviews France, Paris), France • Top 20 most cited Concepts Armin de Meijere (Georg-August-Universitt Göttingen), Germany • Top 20 most cited Communications Kyriacos C. Nicolaou (Rice University, Houston), USA • Top 20 most cited Full Papers David Reinhoudt (University of Twente), The Netherlands • Top 20 most prolific authors J. Fraser Stoddart (Northwestern University, Evanston), USA • Free App available: bit.ly/CHEMAPPS Barry Trost (Stanford University, Stanford, CA), USA • Supported by ACES • Follow us on Twitter and Facebook • Cover Profiles: Find out more about the chemistry and the research groups “Chemistry – A European Journal has always been the gold highlighted on the front cover standard of chemistry for me.” (Martin Pumera, Editorial Board Member)

4 Masked Rhodamine Dyes of Five Principal Colors Revealed by Photolysis of a 2 Diazo 1 Indanone Caging Group: Synthesis, Photophysics, and Light Microscopy Applications Vladimir N. Belov*, Gyuzel Yu. Mitronova, Mariano L. Bossi*, Vadim P. Boyarskiy, Elke Hebisch, Claudia Geisler, Kirill Kolmakov, Christian A. Wurm, Katrin I. Willig, Stefan W. Hell* Masked fluorophores: New photoactivatable rhodamine dyes (see scheme) have been designed, decorated with a reactive group, conjugated with proteins, and used as labels in immunofluorescence and optical microscopy. These “hidden” markers can be readily and irreversibly “uncaged” with λ=375–420 nm or intense red light.conversion technologies are summarized and discussed (see picture). Future trends and prospects for their further Chem. Eur. J. DOI: 10.1002/chem.201403316 development are also discussed.

Palladium Catalysed Direct Cross Coupling of Organolithium Reagents with Aryl and Vinyl Triflates Carlos Vila, Valentín Hornillos, Massimo Giannerini, Martín Fañanás-Mastral, Ben L. Feringa* Cut out the middle man! A palladium-catalysed direct cross- coupling of organolithium reagents with aryl and vinyl triflates is presented. The reaction proceeds at 50 or 70 °C with short reaction Chem. Eur. J. times, and the corresponding products are obtained with moderate DOI:10.1002/chem.201404398 to high yields (see scheme).

Metal Nanoparticles and Supramolecular Macrocycles: A Tale of Synergy Verónica Montes-García, Jorge Pérez-Juste*, Isabel Pastoriza-Santos, Luis M. Liz-Marzán* Nanoparticles and macrocycles: Recent literature regarding the combination of supramolecular macrocycles and metal nanoparticles is reviewed, with particular emphasis on the synthesis, surface modification and assembly, as well as Chem. Eur. J. the potential applications of the obtained nanocomposites DOI: 10.1002/chem.201403107 (SERS = surface-enhanced Raman spectroscopy).

Transition-Metal-Free Catalytic Reduction of Carbon Dioxide Prof. Frédéric-Georges Fontaine, Marc-André Courtemanche and Marc-André Légaré Less is more: Metal-free systems, including frustrated Lewis pairs

(FLPs), have been shown to bind CO2. By reducing the Lewis acidity and basicity of the ambiphilic system, it is possible to generate active catalysts for the deoxygenative hydroboration of carbon dioxide to Chem. Eur. J. methanol derivatives with conversion rates comparable to those of DOI: 10.1002/chem.201304376 transition-metal-based catalysts (see scheme).

5 Rooted in Asia, A journal of read all over the world www.chemasianj.org Free Sample Copy

Editor-in-Chief: Chair of the Editorial Board:

Theresa Kueckmann Ryoji Noyori, Nagoya University, Japan, and RIKEN, Saitama, Japan Editorial Board: Ayyappanpillai Ajayaghosh (CSIR National Institute for Highlights: Interdisciplinary Science and Technology, Thiruvananthapuram) • Next day publication of accepted Jaephil Cho (Ulsan National Institute of Science and Technology) articles Insung S. Choi (Korea Advanced Institute of Science and Technology, Daejeon) • Celebrating 10 years of publication. Xinliang Feng (Technical University, Dresden) Discover at http://bit.ly/ChemAsia10: Makoto Fujita (University of Tokyo) 10 Most cited articles, Top authors, Top Itaru Hamachi (Kyoto University) referees, Special anniversary issues, Michael H. Huang (National Tsing Hua University, Hsinchu) Upcoming celebrations, The hottest Susumu Kitagawa (Kyoto University) topics covered Shū Kobayashi (University of Tokyo) • International readers and authors Aiwen Lei (Wuhan University) • Co-owned by the 13 chemical societies Xiaogang Liu (National University of Singapore) of ACES and supported by ChemPubSoc Jian Pei (Peking University, Beijing) Europe and FACS Thalappil Pradeep (Indian Institute of Technology Madras, Chennai) • Articles featured on Zhigang Shuai (Tsinghua University, Beijing) www.facebook.com/chemasianj Kazuyuki Tatsumi (Nagoya University) and twitter @chemasianj Yoshio Umezawa (Musashino University, Tokyo) Henry N. C. Wong (Chinese University of Hong Kong) • Free App available: bit.ly/CHEMAPPS Zhenzhong Yang (Institute of Chemistry, Chinese Academy of Sciences, Beijing) International Advisory Board: Comprising 72 world-renowned scientists, including Nobel Laureates Robert H. Grubbs, Jean-Marie Lehn, Richard R. Schrock, and K. Barry Sharpless.

6 Palladium-Catalyzed Cross Dehydrogenative Functionalization of C(sp2) — H Bonds Yinuo Wu, Jun Wang*, Fei Mao, Fuk Yee Kwong* Caught in the cross fire:This Review highlights the recent developments in catalytic cross-dehydrogenative coupling (CDC) reactions, which join together two

Chem. Asian J. aromatic C–H fragments through a palladium-catalyzed DOI: 10.1002/asia.201300990 dehydrogenative pathway.

Gold Nanorods with Phase-Changing Polymer Corona for Remotely Near-Infrared-Triggered Drug Release Ji Liu, Christophe Detrembleur*, Bruno Grignard, Marie-Claire De Pau-Gillet, Stéphane Mornet, Mona Treguer-Delapierre, Yannick Petit, Christine Jérôme*, Etienne Duguet* Remote control: The triggered release of doxorubicin (DOX) molecules from GNR@PCL-b-PEG hybrid nanoparticles was Chem. Asian J. achieved by conventional external heating or internal heating DOI: 10.1002/asia.201301010 induced by remote near-infrared (NIR) irradiation.

Toward Chemistry-Based Design of the Simplest Metalloenzyme-Like Catalyst That Works Efficiently in Water Taku Kitanosono, Shū Kobayashi* Water Music: We have designed the simplest metalloenzyme- like catalyst system model that can function in water, without any aid from an enzymatic structure itself. By compaction and precise orchestration of essential functions, this artificial system efficiently

Chem. Asian J. catalyzed enantioselective direct-type aldol reactions using DOI: 10.1002/asia.201403004 aqueous formaldehyde.

Self-Assembled Platinum Nanoflowers on Polydopamine-Coated Reduced Graphene Oxide for Methanol Oxidation and Oxygen Reduction Reactions Xueqing Yu, Huan Wang, Liping Guo, Liang Wang* Platinum in bloom! Self-assembled Pt nanoflowers on polydopamine-coated reduced graphene oxide are fabricated in a facile and efficient synthesis, and are a promising

Chem. Asian J. electrocatalyst for methanol oxidation and oxygen reduction DOI: 10.1002/asia.201402883 reactions.

7 Open Access Chemistry A journal of with Impact www.chemistryopen.org Browse The Journal

Co-Editors-in-Chief: Deputy Editor:

Karen Hindson Haymo Ross Natalia Ortúzar

Editorial Advisory Board Chairs:

Ramón Martínez-Máñez Thomas Wirth Jean-Marie Lehn Universitat Polytechnica de Cardiff University, UK Collège de France/Université Valencia, Spain de Strasbourg, France Highlights:

• Fully open access – articles are free to read • Communications, Full Papers, and Reviews are and reuse under the terms of Creative Commons stringently peer-reviewed to ensure the high-quality licenses of ChemistryOpen • Celebrate ChemistryOpen’s impressive first • An additional Thesis Treasury allows scientists to Impact Factor of 2.938 and publish for free publish an extended abstract describing their PhD until June 2015 research. These Thesis Summaries allow readers to • All accepted articles are published to a high browse and cite doctoral research like never before, standard, with electronic processing of text and helping to disseminate this important but largely graphics and a view to scientific accuracy and untapped reservoir of data rapid publication times • Next day publication of accepted articles • Free App available: bit.ly/CHEMAPPS

8 One-Pot Synthesis and Applications of N-Heteroaryl Iodonium Salts Marcin Bielawski, Joel Malmgren, Leticia M. Pardo, Ylva Wikmark, Berit Olofsson* N-Heteroarylation: An efficient one-pot synthesis of N-heteroaryl iodonium triflates from the corresponding N-heteroaryl iodide has been developed. The reactivity and chemoselectivity of these iodonium salts were demonstrated ChemistryOpen by selectively introducing a pyridyl moiety onto both oxygen DOI: 10.1002/open.201300042 and carbon nucleophiles in good yields.

Difluoro- and Trifluoromethylation of Electron-‐ Deficient Alkenes in an Electrochemical Microreactor Kenta Arai, Kevin Watts, Thomas Wirth* In the flow!In an electrochemical microreactor, Kolbe electrolysis of acetic acid derivatives allows facile difluoro- and trifluoromethylation of electrondeficient alkenes. Compared with ChemistryOpen bulk reactions, higher yields are achieved at room temperature DOI: 10.1002/open.201300039 and in short reaction times.

Understanding E2 versus SN2 Competition under Acidic and Basic Conditions Lando P. Wolters, Yi Ren*, F. Matthias Bickelhaupt* Titrating the LUMO: The character of the LUMO of a substrate

CH3CH2−LG (LG=leaving group) is found to be pH dependent: whereas it is Cβ−H bonding under acidic conditions, it is Cβ−H antibonding under basic conditions. This is an important factor ChemistryOpen behind the corresponding shift in reactivity towards an electron- DOI: 10.1002/open.201300043 donating agent Nu from substitution to elimination.

Synthesis and Photochromic Properties of Configurationally Varied Azobenzene Glycosides Vijayanand Chandrasekaran, Eugen Johannes, Hauke Kobarg, Frank D. Sönnichsen, Thisbe K. Lindhorst* Sweet switches: Azobenzene glycosides with systematically varied structural properties were synthesized using glycoside synthesis and Mills reaction. Their photochromic properties ChemistryOpen were tested to evaluate their usefulness in studies requiring DOI: 10.1002/open.201402010 temporal and spatial alteration of carbohydrate orientation.

9 A Multidisciplinary Journal A journal of Centering on Chemistry www.chempluschem.org Free Sample Copy

Editor-in-Chief:

Marisa Spiniello

Chairs of the Editorial Board:

Highlights: • Features multidisciplinary articles Matthias Driess Michal Hocek Nico Sommerdijk (Berlin Institute of (Institute of Organic (Eindhoven University covering at least two subfields of Technology, Germany) Chemistry and Biochemistry in of Technology, the Netherlands) chemistry Prague, Czech Republic) • Impressive first Impact Factor of Members of the Editorial Board: 3.242 (2013) Chi-Ming Che (The University of Hong Kong), China • Rigorous peer review and swift Avelino Corma (Universidad Politécnica de Valencia), Spain publication Luisa De Cola (Université de Strasbourg, ISIS), France • A fully electronic service with Chuan He (The University of Chicago), USA Free Color! Ivan Huc (Université Bordeaux 1), France • Cover Profiles for front cover articles Paul Knochel (Ludwig-Maximilians-Universitt München), Germany • Early Career Series and Interviews Tetsuro Majima (Osaka University), Japan • Free App available: bit.ly/CHEMAPPS Krzysztof Matyjaszewski (Carnegie Mellon University, • Follow us on Facebook and Pittsburgh), USA Twitter @ChemPlusChem Paolo Samorì (ISIS, Université de Strasbourg), France Itamar Willner (The Hebrew University of Jerusalem), Israel

International Advisory Board: Comprising 50 world-renowned scientists.

10 Design of a Nitrogen-Doped, Carbon-Coated

Li4Ti5O12 Nanocomposite with a Core-Shell Structure and Its Application for High-Rate Lithium-Ion Batteries Hongsen Li, Laifa Shen, Jie Wang, Bing Ding, Ping Nie, Guiyin Xu, Xiaoyan Wang, Xiaogang Zhang*

Made to fit:A nitrogen-doped, carbon-coated Li4Ti5O12 nanocomposite with a core–shell structure has been synthesized using the ionic liquid 1-ethyl-3-methylimdazolium tricyanomethanide as the carbon source. The well-defined nanocomposite displays better cycling and rate performances

ChemPlusChem than those of Li4Ti5O12 nanoparticles, and has a superior lithium- DOI: 10.1002/cplu.201300316 storage capability even at high rates (see picture).

Metal Coordination and Isomerization of a Hydrazone Switch Molly L. Croteau, Xin Su, Dean E. Wilcox*, Ivan Aprahamian* So many options! The interaction between a hydrazone-based switch and a Lewis acid can lead to coordination, followed by redistribution of metal and ligand, and isomerization. Based on isothermal titration calorimetry (ITC) and UV/Vis titration data,

ChemPlusChem the nature of the Lewis acid and its counterion determine which, DOI: 10.1002/cplu.201402134 if any, of these processes takes place (see picture).

Synthesis and Contact Angle Measurements of Janus Particles Alla Synytska*, M. Sc.Alina Kirillova, Lucio Isa* Two faced: Janus microparticles are a promising alternative to molecular surfactants for emulsion stabilisation. The synthesis of diverse Janus microparticles (figure, top) with a defined Janus ratio is reported and their position in situ at a water/oil interface using freeze-fracture, shadow-casting cryo- ChemPlusChem DOI: 10.1002/cplu.201400020 SEM is measured (figure, bottom).

Recyclable Heterogeneous and Low-Loading Homogeneous Chiral Imidazolidinone Catalysts for α-Alkylation of Aldehydes Anna Maria Pia Salvo, Francesco Giacalone, Renato Noto, Michelangelo Gruttadauria* Recycling drive: Is it possible to have a supported chiral imidazolidinone catalyst that is recyclable without loss in activity or a homogeneous counterpart catalytically active

ChemPlusChem at low loading? We have investigated this topic using the DOI: 10.1002/cplu.201400030 α-alkylation of aldehydes as a benchmark reaction (see figure).

11 Chemistry & Sustainability, A journal of Energy & Materials www.chemsuschem.org Free Sample Copy

Editor-in-Chief:

Guido Kemeling

Chairs of the Editorial Board:

Highlights:

• Free color images and no page charges • Impact Factor 7.117 (2013) • Cover Profiles for Front Cover images Matthias Beller Gabriele Centi Licheng Sun Leibniz-Institut für Katalyse, Università degli Studi di KTH Royal Institute of • Anywhere Article for easy online reading Rostock, Germany Messina, Italy Technology, Sweden and Dalian University of • Supported by: ACES Technology, P.R. China • @ChemSusChem - Follow us on Twitter! Members of the Editorial Board: • Free App available: bit.ly/CHEMAPPS Giuseppe Bellussi (Eni), Italy • Pioneering fully electronic services Claudio Bianchini (Istituto di Chimica dei Composti Organometallici), CNR, Firenze, Italy Nigel Brandon (Imperial College, London), UK Avelino Corma (Universidad Politécnica de Valencia), Spain Francesco De Angelis (Università degli Studi dell’Aquila), Italy Dirk Guldi (Universität Erlangen-Nürnberg), Germany Birgit Kamm (Forschungsinst. Bioaktive Polymersysteme, Teltow), Germany Toshiyasu Sakakura (AIST Research Institute for Innovation in Sustainable Chemistry, Tsukuba), Japan Joaquim Henrique Teles (BASF, Ludwigshafen), Germany International Advisory Board: Comprising 56 world-renowned scientists. 12 Solvent-Free and Catalysts-Free Chemistry: A Benign Pathway to Sustainability Manoj B. Gawande*, Vasco D. B. Bonifácio*, Rafael Luque, Paula S. Branco, Rajender S. Varma* Free chemistry: Various innovative sustainable organic reactions and methodologies using no solvents or catalysts and employing conventional and room-temperature heating conditions or alternative energy inputs such as ChemSusChem microwaves, sonication, mechanochemical mixing, and high speed ball milling DOI: 10.1002/cssc.201300485 are summarized.

Nanostructured Tungsten Trioxide Thin Films Synthesized for Photoelectrocatalytic Water Oxidation: A review Tao Zhu, Meng Nan Chong*, Eng Seng Chan

It′s all a matter of e: The synthesis of nanostructured WO3 to be used for photochemical water splitting using various electrochemical routes is reviewed. Key fundamental reaction mechanisms and various effects of synthesis methods and approaches on physical, chemical, optical, and photoelectrochemical properties

ChemSusChem of nanostructured WO3 are explained. Also, a summary of the current evaluation DOI: 10.1002/cssc.201402089 practices on the energy conversion efficiency of nanostructured WO3 is provided.

Paving the Way for Using Li2S Batteries Rui Xu, Xiaofeng Zhang, Cun Yu, Yang Ren, James C. M. Li, Ilias Belharouak*

Electrolyte my fire: Lithium disulfide “Li2S” cathode has gained great attention in

Li–S battery research recently. However, Li2S does not provide the full extent of its capacity in the cell because it is barely active due to its highly insulating character.

The use of a non-conventional electrolyte in a Li2S battery is described. This ChemSusChem electrolyte significantly improved the electrochemical activity of Li2S by delivering DOI: 10.1002/cssc.201402177 high capacity and good cycling.

Progress in Base-Metal Water Oxidation Catalysis Alexander Rene Parent*, Ken Sakai* Providing a platform: The development of water oxidation catalysts based on first-row transition metals has received increased interest in recent years as a method for storing solar fuels inexpensively. The homogeneous catalysts developed in the past two decades are reviewed, and commentary on ChemSusChem DOI: 10.1002/cssc.201402322 the development of the field is provided.

Catalytic Transfer Hydrogenation/Hydrogenolysis for Reductive Upgrading of Furfural and 5-(Hydroxymethyl) furfural David Scholz, Christof Aellig, Ive Hermans* To boldly flow: The next hydrogenation!The sequential transfer hydrogenation/ hydrogenolysis of furfural and 5-hydroxymethylfurfural to 2-methylfuran and

2,5-dimethylfuran is studied over in situ reduced, Fe2O3-supported Cu, Ni, and Pd catalysts, with 2-propanol as hydrogen donor. A significant enhancement in yield of

ChemSusChem 2-methylfuran and 2-methyltetrahydrofuran is observed under continuous DOI: 10.1002/cssc.201300774 flow conditions.

13 Advancing Chemistry A journal of www.wileyonlinelibrary.com/journal/hca

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Editorial Board: Editor-in-Chief Advisory Board M. Volkan Kisakürek Karl-Heinz Altmann, Zürich Michael Bühl, St. Andrews Senior Editors Christian Chapuis, Genève Hans-Jürg Borschberg Kuiling Ding, Shanghai Heinz Heimgartner Hans-Jürgen Hansen, Zürich Alan F. Williams Bernhard Jaun, Zürich Associate Editors Jean-Marie Lehn, Strasbourg Kathrin A. Brun Anthony Linden, Zürich Changchun Fu Esther Oliveros, Toulouse Richard J. Smith Inken Plitzko, Basel Olivier Potterat, Basel Assistant Editors Constanze Hofmann Helmut Rosemeyer, Osnabrück Yuzhu Song Helmut Schwarz, Berlin Bernard Testa, Lausanne Editorial Assistant Han van de Waterbeemd, Malgorzata Krause- Saint André Gruszczynska Andrea Vasella, Zürich Pierre Vogel, Lausanne Oliver Zerbe, Zürich Highlights:

• Up-to-date, peer-reviewed contributions from Founded by the Swiss Chemical Society, Helvetica Chimica Acta all over the world is now in its 98th year of publication and has a high reputation • Internationally renowned contributors amongst original full-paper chemistry journals. Helvetica Chimica Acta is a monthly multidisciplinary journal dedicated to the • Timely publication of original full-papers, dissemination of knowledge in all areas of chemistry and to the selected reviews, and short communications timely publication of original full-paper contributions from all over • Multidisciplinary scope; contributions from sub- the world. With emphasis on the multidisciplinary nature of the disciplines including, but not limited to, organic, journal, progress in subdisciplines including but not limited to inorganic, and physical chemistry organic, inorganic, physical, technical, and analytical chemistry is • Uniquely careful scientific editing (including reported. Outstanding referees review all contributions, and papers nomenclature) are published, on average, within three months of receipt if no revision needed. The journal publishes more than 250 papers per • High-quality layout, graphics, and printing year, and each monthly issue contains an average of 200 pages. • Publication of full experimental details There is no restriction on the length of their papers or the scope of • Commemorative issues that include the chemistry presented. Preliminary communications and review contributions from highly renowned chemists papers are considered as well.

14 Preparation and Structures of 2-Substituted 5-Benzyl-3-methylimidazolidin-4-one-Derived Iminium Salts, Reactive Intermediates in Organocatalytic Transformations Involving α,β- Unsaturated Aldehydes Uroš Grošelj*, Albert Beck, W. Bernd Schweizer, Dieter Seebach

Helv. Chim. Acta DOI: 10.1002/hlca.201400110

Confusing Quantitative Descriptions of Brønsted– Lowry Acid-Base Equilibria in Chemistry Textbooks – A Critical Review and Clarifications for Chemical Educators Erich C. Meister, Martin Willeke, Werner Angst, Antonio Togni, Peter Walde* Helv. Chim. Acta DOI: 10.1002/hlca.201300321

Functionalization of 2″-C-(Piperazinomethyl)- 2′,3′-BcNA (Bicyclic Nucleic Acids) with Pyren-1-ylcarbonyl Units Morten Borre Hansen, Nicolai Krog Andersen, Michael Raunkjær, Per Trolle Jørgensen, Jesper Wengel*

Helv. Chim. Acta DOI: 10.1002/hlca.201400141

How Small Amounts of Impurities Are Sufficient to Catalyze the Interconversion of Carbonyl Compounds and Iminium Ions, or Is There a Metathesis through 1,3-Oxazetidinium Ions? Experiments, Speculations, and Calculations Dieter Seebach*, Tomohiro Yoshinari, Albert K. Beck, Marc-Olivier Ebert, Alejandro Castro-Alvarez, Jaume Vilarrasa* and Markus Reiher* Helv. Chim. Acta DOI: 10.1002/hlca.201400221

15 Reviews and Records A journal of www.tcr.wiley-vch.de

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Editor-in-Chief:

Hisashi Yamamoto University of Chicago (USA) Editorial Board:

Shigeru Amemiya Masayuki Inoue Keiji Maruoka Noritaka Mizuno University of Pittsburgh, USA The University of Kyoto University, Japan The University of Tokyo, Japan Tokyo, Japan

Shigeru Nagase Hiroshi Sugiyama Yasuhiro Uozumi Eiji Yashima Jun-ichi Yoshida Fukui Institute for Kyoto University, Japan Institute for Molecular Nagoya University, Japan Kyoto University, Japan Fundamental Chemistry, Science, Okazaki, Japan Kyoto, Japan Highlights: • Free App available: bit.ly/CHEMAPPS discover history, and be a detective through the wiki- • The “Records and Challenges” platform of type website! The Chemical Record describes both world records • The Chemical Record Lecture (TCR Lecture) has and future challenges in chemistry – the “Record of established itself into a high-profile series with a view to Records” offers an archived overview of continually fostering international and interdisciplinary exchange, updated world records in chemistry and takes place annually in Japan as part of the spring • The Nozoe Autograph Books are now available online meeting of the Chemical Society of Japan as part of The Chemical Record. Browse the pages,

16 My Favorite Aromatic Compounds – A Tribute to Friedrich August Kekulé Henning Hopf* Hallowed halls of aromatic chemistry: Henning Hopf shares his personal views on the history of aromatic chemistry. Drawing from his nearly 55 years in the world of organic chemistry, he discusses his favorite aromatic compounds in a fitting tribute to Kekulé nearly 150 years after the hexagonal benzene structure was originally postulated. This Essay and the interactive website that accompanies the Nozoe Autograph Book project are

Chem. Rec. available free-access for at least a three-year period at DOI: 10.1002/tcr.201402056 [Essay] www.tcr.wiley-vch.de/nozoe.

Tricks of Light on Helices: Transformation of Helical Polymers by Photoirradiation Tamaki Nakano* Light does tricks to polymer chains, leading to remarkable changes in conformation and chemical structure. A preferred- handed helical structure was induced in a polyfluorene derivative using single-handed circularly polarized light in a reversible way. In this case, no photochromic group such as azobenzene was necessary to make the chain mutate; twist-coplanar transition of aryl–aryl moieties in the polymers triggers macromolecular conformational transition of the entire chain. Several examples Chem. Rec. of photoinduced stereomutation and reactions of chiral helical DOI: 10.1002/tcr.201300042 polymers are reviewed.

Continuous Flow Photochemistry Kerry Gilmore, Peter H. Seeberger* The efforts of the Seeberger group in continuous photochemical reactions, both visible and UV light, are described. These transformations include cyclizations, intermolecular couplings, radical polymeriztions, as well as a range of singlet oxygen oxygenations. Chem. Rec. DOI: 10.1002/tcr.201402035

Late-Stage Formation of Carbon – Fluorine Bonds Michael G. Campbell, Tobias Ritter* Selective C–F bond formation in the context of functionalized small molecules has been a longstanding synthetic challenge. In this Personal Account, we describe work from our lab that aims to address this challenge. Transition metal-mediated and – catalyzed fluorination reactions are highlighted, including potential 18 Chem. Rec. applications in F radiotracer synthesis for positron emission DOI: 10.1002/tcr.201402016 tomography (PET).

17 High Quality Topical issues A journal of www.ijc.wiley-vch.de

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Editor-in-Chief:

Ehud Keinan Benno Gitter and Ilana Ben Ami Professor of Chemistry, Technion – Israel Institute of Technology Editorial Board:

Lia Addadi Yitzhak Apeloig Yoram Cohen Weizmann Institute of Technion, Haifa, Israel Tel Aviv University, Israel Science, Rehovot, Israel

Ronnie Kosloff Ilan Marek David Milstein Avraham Nitzan Sason Shaik Hebrew University Technion, Haifa, Israel Weizmann Institute of Tel Aviv University, Israel Hebrew University, Jerusalem, Israel Science, Rehovot, Israel Jerusalem, Israel Highlights:

• Special Issues on timely topics from all areas of chemistry • Free App available: bit.ly/CHEMAPPS • The complete archive of the Israel

Reshef Tenne Ira Weinstock Arie Zaban Journal of Chemistry is now available Weizmann Institute of Ben Gurion University Bar-Ilan University, online. All articles are fully searchable Science, Rehovot, Israel of the Negev Ramat Gan, Israel and linked with thousands of related articles through CrossRef/DOI • Free color in all articles 18 Electrochemical CO2 Reduction: Recent Advances and Current Trends John-Paul Jones, G. K. Surya Prakash*, George A. Olah

Isr. J. Chem. DOI: 10.1002/ijch.201400081

Past and Future Solid-State NMR Spectroscopy Studies at the Convergence Point between Biology and Materials Research Gil Goobes*

Isr. J. Chem. DOI: 10.1002/ijch.201300113

Emergent Properties in Locally Ordered Molecular Materials Nicholas E. Jackson, Henry M. Heitzer, Brett M. Savoie, Matthew G. Reuter, Tobin J. Marks*, Mark A. Ratner*

Isr. J. Chem. DOI: 10.1002/ijch.201400021

Molecular Sensing Using Hyperpolarized Xenon NMR Spectroscopy Krishnan K. Palaniappan, Matthew B. Francis, Alexander Pines, David E. Wemmer*

Isr. J. Chem. DOI: 10.1002/ijch.201300128

19 Free Going International Sample Copy A journal of www.cjc.wiley-vch.de

Deputy Associate Editor-in-Chief: Editor-in-Chief:

Guozhen Ji Shengming Ma Shanghai Institute of Organic Chemistry Shanghai Institute of Organic Chemistry Chinese Academy of Sciences Chinese Academy of Sciences

Highlights: Associate Editors-in-Chief: • International peer-reviewed forum Shouhua Fen, Jilin University (Changchun, P.R. China) published in English Yulin Wu, SIOC, CAS (Shanghai, P.R. China) Yundong Wu, The Hong Kong University of Science and • Modern online publishing platform, Technology (P.R. China) covering all areas of chemistry Xinsheng Zhao, Peking University (P.R. China) • Publishes Reviews, Accounts, Hanfa Zou, Dalian Institute of Chemical Physics, CAS (P.R. China) Communications, Full Papers, and Notes International Advisory Board: • The complete archive of the Chinese Eric V. Anslyn, University of Texas (Austin, USA) Journal of Chemistry is now available Jinpei Cheng, Tsinghua University(Beijing, P.R. China) online. All articles are fully searchable Jiali Gao, University of Minnesota (Minneapolis, USA) and linked with thousands of related Maochun Hong, CAS (Fuzhou, P.R. China) articles through CrossRef/DOI Can Li, CAS (Dalian, China) Charles M. Lieber, Harvard University (Cambridge, USA) Jun O. Liu, John Hopkins University (Maryland, USA) Xiyan Lu, Chinese Academy of Sciences (Shanghai, P.R. China) Richard A. J. O’Hair, University of Melbourne (Australia) Mitsuo Sawamoto, Kyoto University (Kyoto, Japan) Fraser Stoddart, Northwestern University (Evanston,USA) Weihong Tan, University of Florida (USA) Ben Zhong Tang, The Hong Kong University of Science and Technology (Hong Kong, P.R. China) Younan Xia, Georgia Institute of Technology (Atlanta, USA) Vivan W.-W., Yam, The University of Hong Kong (Hong Kong, P.R. China) Jin-Quan Yu, The Scripps Research Institute (California, USA) 20 Imine-Linked Covalent Organic Framework on Surface for Biosensor Peiyuan Wang*, Mengmeng Kang, Shumin Sun, Qiang Liu, Zhihong Zhang, Shaoming Fang* Imine-linked covalent organic frameworks on amino functionalized silicon substrate were constructed via the reaction between 1,3,5-benzenetricarboxaldehyde and 1,4-diaminobenzene and used as biosensor for BSA Chin. J. Chem. adsorption and probe DNA immobilization. DOI: 10.1002/cjoc.201400430

Primary-Tertiary Diamine/Br-nsted Acid Catalyzed α-Allylation of Carbonyl Compounds with Allylic Alcohols Lingyun Cui, Long Zhang, Sanzhong Luo*, Jin-Pei Cheng* α-Allylic alkylation: The primary amine/Br-nsted acid promoted the direct α-allylation of unmodified aldehydes with allylic alcohols via an enamine process, affording the products Chin. J. Chem. in high yields (up to 88%) and with good diastereoselectivities DOI: 10.1002/cjoc.201400430 (up to 9:1).

Chincona Alkaloid-Catalyzed Enantioselective Trifluoromethylthiolation of Oxindoles Tao Yang, Qilong Shen*, Long Lu* An onganocatalytic asymmetric trifluoromethylthiolation of 3-aryl or 3-alkyloxindoles employing a trifluoromethyl-substituted thioperoxide as the electrophilic trifluoromethylthiolating reagent was described. Reactions occurred in good to excellent

Chin. J. Chem. enantioselectivities to generate enantiopure oxindoles with a SCF3- DOI: 10.1002/cjoc.201400392 substituted quaternary chiral center.

Sidearm as a Control in the Asymmetric Ring Opening Reaction of Donor-Acceptor Cyclopropane Qikai Kang, Lijia Wang, Zhongbo Zheng, Junfang Li*, Yong Tang* A new type of trisoxazoline and bisthiazoline based ligands have been developed, which are absent of chiral motif on the parent skeleton and contain a chiral backbone on sidearm. The ligands promote the amine nucleophilic ring opening reaction of Chin. J. Chem. 1,1-cyclopropane diesters smoothly, furnishing the γ-amino acid DOI: 10.1002/cjoc.201400053 derivatives in high yield with moderate to good enantioselectivity.

21 Global Visibility A journal of www.jccs.wiley-vch.de

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Editor-in-Chief:

Yu Tai Tao Institute of Chemistry, Academia Sinica Taipei (Taiwan, ROC)

Associate Editors: Chun-Hsien Chen, National Taiwan University, Taipei Chin-Ti Chen, Academia Sinica, Taipei King-Chuen Lin, National Taiwan University, Taipei Chien-Tien Chen, National Tsing Hua University, Hsinchu Wen-Feng Liaw, National Tsing Hua University, Hsinchu Highlights: International Editorial Advisory Board: • Oldest general chemistry journal Paul Attfield, University of Edinburgh (UK) in Taiwan Arthur J. Carty, Waterloo Institute for Nanotechnology (Canada) • Modern online publishing platform, Sunney I. Chan, California Institute of Technology, covering all areas of chemistry Pasadena (USA) • Publishes Reviews, Communications, Chi Ming. Che, Hong Kong University (China) Full Papers, and Notes Tahsin J. Chow, Academia Sinica, Taipei (Taiwan, ROC) • The complete archive of the Journal Hai-Lung Dai, Temple University, Phildelphia (USA) of the Chinese Chemical Society is Vadin Kukushkin, St. Petersburg State University (Russia) now available online. All articles are Hian Kee Lee, National Univ. Singapore fully searchable and linked with Chun-Chen Liao, Chung Yuan University, Chung-Li (Taiwan, ROC) thousands of related articles through Ching-Erh Lin, National Taiwan University, Taipei (Taiwan, ROC) CrossRef/DOI Sheng- Hsien Lin, National Chiao Tung University, Hsinchu (Taiwan, ROC) Shie-Ming Peng, National Taiwan University, Taipei (Taiwan, ROC) Peter M. Rentzepis, University of California, Irvine (USA) Ho-Hsiang Wei, Tamkang University, Taipei (Taiwan, ROC) Yoshinori Yamamoto, Tohoku Univ., Sendai (Japan) Edward Yeung, Iowa State University, Ames (USA)

22 Review on the Recent Progress in Low Band Gap Conjugated Polymers for Bulk Hetero-junction Polymer Solar Cells Hong-Jyun Jhuo, Po-Nan Yeh, Sih-Hao Liao, Yi-Lun Li, Yu-Shan Cheng, Show-An Chen* We classify the D–A polymers in accordance with the acceptor units that are commonly used, being Benzodiathiazole (BT), Thienopyrrolodione (TPD), and and Diketopyrrolopyrrole (DPP), with appropriate donors having promising efficiency. Low band gap polymers based on quinoid structure, thienothiophene (TT) J. Chin. Chem. Soc. DOI: 10.1002/jccs.201300333 having promising efficiency are also included.

Advances in Carbon-Incorporated Non-Noble Transition Metal Catalysts for Oxygen Reduction Reaction in Polymer Electrolyte Fuel Cells Tai-Feng Hung, Syuan-Hong Chen, Meng-Hsiu Tu, Zhi-Hsiang Lu, Chih Kai Chen, Ru-Shi Liu*, Heather F. Greer, Wuzong Zhou, Man-Yin Lo Recent advances in carbon-incorporated non-noble metal catalysts (NNMCs), specifically, carbon-incorporated iron nitride (FeCN)-based catalysts were reviewed. The oxygen reduction reaction (ORR) activities of FeCN-based catalysts were significantly affected by crystalline sizes, J. Chin. Chem. Soc. supporting materials, amounts of doped nitrogen, etc.in high yields (up to DOI: 10.1002/jccs.201300286 88%) and with good diastereoselectivities (up to 9:1).

Phosphonate Congeners of Oseltamivir and Zanamivir as Effective Anti-influenza Drugs: Design, Synthesis and Biological Activity Jiun-Jie Shie, Jim-Min Fang* The synthetic methods for oseltamivir, tamiphosphor, zanamivir, zanaphosphor and derivatives are reviewed. Their anti-influenza activities were compared by neuraminidase inhibition, cell-based assay and mice experiments. Guanidino-tamiphosphor and zanaphosphor showed remarkable activities against avian and human influenza viruses including J. Chin. Chem. Soc. the oseltamivir-resistant H275Y strain. The phosphonate monoalkyl esters DOI: 10.1002/jccs.201300544 were real active drugs, but not prodrugs of the parental phosphonic acids.

Synthesis, Characterization and Photoluminescence of Lanthanide Metal-organic Frameworks, Constructed from Triangular 4,4′,4″-s-triazine-1,3,5- triyl-p-aminobenzoate Ligands (pages 1115–1120) Ju-Hsiou Liao, Chien-Yuan Lai and Chih-Liang Yang

Eight isomorphous metal-organic frameworks, [Ln2(TATAB)2(H2O)

(DMA)6]·5H2O (Ln = Sm (1), Eu (2), Gd (3), Tb (4), Dy (5), Er (6), Tm (7), Yb (8)) were synthesized and characterized. They adopt 3-D interpenetrating

framework with (105·105·105) topology. Compound 4 exhibits bright green Tb J. Chin. Chem. Soc. emission upon UV excitation.derivatives in high yield with moderate to good DOI: 10.1002/jccs.201400116 enantioselectivity.

23 New with Wiley-VCH A journal of www.bkcs.wiley-vch.de

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Vice President of the Journal Editor-in-Chief: Publishing Committee:

Byeong Moon Kim Hyun-Joon Ha Seoul National University (Korea) Hankuk University of Foreign Studies (Korea)

Highlights: International Advisory Board: New at Wiley-VCH! From January Kyo Han Ahn (POSTECH, Korea) Daryl H. Busch (University of Kansas, USA) 2015 onwards, the Bulletin of the Song-Ho Byeon (Kyung Hee University, Korea) Korean Chemical Society is published Young Keun Chung (Seoul National University, Korea) with Wiley-VCH. It is the official Jean Etourneau (University of Bordeaux, France) research journal of the Korean W. James Feast (Durham University, UK) Chemical Society and cover all major Hubert Girault (Ecole Polytechnique Fédérale de Lausanne, Switzerland) Hyun-Joon Ha (HUFS, Korea) areas of chemistry. The Bulletin of the Mercouri G. Kanatzidis (Northwestern University, USA) Korean Chemical Society publishes Hoon Sik Kim (Kyung Hee University, Korea) a stimulating mixture of Accounts, Myoung Soo Lah (UNIST, Korea) Articles, Communications, and Notes. Duck-Hyung Lee (Sogang University, Korea) Hee-Yoon Lee (KAIST, Korea) Jin Yong Lee (Sungkyunkwan University, Korea) Myong-Hoon Lee (Chonbuk National University, Korea) Wan In Lee (Inha University, Korea) Yoon Sup Lee (KAIST, Korea) Heung Bin Lim (Dankook University, Korea) Guo-Qiang Lin (Shanghai Institute of Organic Chemistry, China) Sun-il Mho (Ajou University, Korea) Yuri N. Molin (Institute of Chemical Kinetics Com, Russia) Myeong Hee Moon (Yonsei University, Korea) Surk-Sik Moon (Kongju National University, Korea) Jong-Sang Park (Seoul National University, Korea) Seung Min Park (Kyung Hee University, Korea) Choong Kyun Rhee (Chungnam National University, Korea) George C. Schatz (Northwestern University, USA) Donald W. Setser (Kansas State University, USA) Seokmin Shin (Seoul National University, Korea) Hyuk Yu (University of Wisconsin, USA) 24 ACES Meeting 2005, Beijing ACES Meeting 2009, Shanghai

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Vera Koester

Most Viewed Articles: Highlights: Education Section: • Free-to-view Tips and Tricks for the Lab: • Comprehensive news and Column Choices information site Sarah Millar • Associated scientific online DOI: 10.1002/chemv.201200074 magazine (ChemViews Magazine) • Growing worldwide readership ChemViews Magazine: The Chemistry of Breaking Bad • Daily latest news and developments Falk Harnisch, Tunga Salthammer from research and industry DOI: 10.1002/chemv.201300114 • News, in-depth articles, commentary, additional feature material from ChemViews Magazine: leading authors What’s New in 3D Printing? • High quality scientific content Helena Dodziuk DOI: 10.1002/chemv.201300064

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Video: Carbonate Looping Elmar Zimmermann, Vera Köster (Video Editing: Lynsey Geldeard) 26 www.chempubsoc.eu Conference onCoordination Chemistry, Organometal- ChemPubSoc Europe Owners Meeting1999,Madrid lic Chemistry andCatalysis 2012,MétabiefMontd’Or www.chemeurj.org K. A.Jørgensen etal.K. Hydrogen-Bonding inAminocatalysis: From Proline andBeyond Concept CEUJED 20 (2) 337–612 (2014)·ISSN0947-6539 Vol. 20·No.CEUJED 20(2)337–612 2·2014 Speakers Launched Launched Launched Launched Launched Launched CPCHFT 14 (9) 1749 CPCHFT 14(9)1749 – 2004 (2013)·ISSN1439-4235 Vol. 14·No. 9·June2013 2000 200 1995 Symposium 2005,Strasbourg 8 Chemistry –AEuropean Journal 2014-20/2 A Journalof Launched Launched Launched Launched Launched Launched CHEMK3 6 (1) 1–362 (2014)·ISSN1867-3880Vol.6No.1January,2014 CHEMK3 6(1)1–362 2014 2009 2010

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ChemPubSoc Europe Owners Meeting2004,Lisbon EJOCFK (33) 7437–7636 (2013) · ISSN 1434-193X · No. 33/2013 No. · 1434-193X ISSN · (2013) 7437–7636 (33) EJOCFK A sister journal of journal sister A Open 2013·39 – 76 ·OnlineISSN2191-1363Vol.2No.April2013 Recent Developments in Amide Synthesis Amide in Developments Recent Rachel M. Lanigan and Tomand Lanigan Sheppard M. D. Rachel Microreviews Tetra(2-thienyl)ethyleneDerivatives Clara Baldoli, Emanuela Licandro et al. et Licandro Emanuela Baldoli, Clara CoverPicture Asian Journal of Organic Chemistry Organic of Journal Asian Wissenschaftsforum Chemie2013,Darmstadt Eur Enantioselective ArtiﬁcialMetalloenzymes Speakers (K. Tschulik,R.G.Compton) Nanoparticle Agglomeration CBCHFX 14(17)2221– 2376 (2013)·ISSN1439-4227 Vol. 14·No. 17·November 2013 Communication: Launched Launched Launched Launched Launched Launched (J. Eppinger) Full Paper: JOC Organic Chemistry Organic of Journal European 2012 1998 2000 Symposium 2010,Paris ChemBioChem /ChemPhysChem www.eurjoc.org 2/2013 3rd November Issue November 3rd 33 D55712 /2013 D 6093 D EJICFK (25) 4353–4525 (2013) · ISSN 1099-0682 · No. 25/2013 No. · 1099-0682 ISSN · (2013) 4353–4525 (25) EJICFK Biologically Relevant Silver(I)–N-Heterocyclic CarbeneComplexesSilver(I)–N-Heterocyclic Relevant Biologically Srinivasa Budagumpi et al. et Budagumpi Srinivasa Microreview White-Emitting CaWhite-Emitting Jun Lin et al. et Lin Jun CoverPicture Eur Cover Picture: Nanodiamond–TiO Minireview: Full Paper: Energy-Transfer inIr Mechanisms 9 MgNa(PO ChemPlusChem 78 (8) 749–884 (2013)·ISSN2192-6506Vol.78No.8August2013 ChemPlusChem 78(8)749–884 The Piers–Rubinsztajn (R. Reaction Wakabayashi Kuroda) andK. Launched Launched 4 Launched Launched ) 7 CHEMGX 8(8)1229 –1420 (2013)·ISSN1860-7179 Vol. 8·No. 8·August, 2013 Launched Launched :Ce 3+ /Tb JIC www.chempluschem.org 3+ 8/2013 2012 Inorganic Chemistry Inorganic of Journal European /Mn 2005 1998 2 Composites for Photocatalysis (A. M. T. Silvaetal.) 2+ Phosphors III –Eu www.eurjic.org III Complexes (Z.Bianetal.)

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