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Users Meeting PROGRAM and ABSTRACTS Advanced Photon Source • Center for Nanoscale Materials • Electron Microscopy Center 2014 Users Meeting PROGRAM AND ABSTRACTS User Science: discoveries for tomorrow i User Facilities at Argonne National Laboratory User Contacts Advanced Photon Source http://www.aps.anl.gov 630-252-9090 [email protected] Argonne Leadership Computing Facility http://www.alcf.anl.gov 630-252-0929 Argonne Tandem Linac Accelerator System http://www.phy.anl.gov/atlas 630-252-4044 Center for Nanoscale Materials http://nano.anl.gov 630-252-6952 [email protected] Electron Microscopy Center http://www.emc.anl.gov 630-252-4987 ii 2014 Users Meeting — May 12–15, 2014 Table of Contents Comprehensive Program ........................................................................................................................... 1 General Session Abstracts ...................................................................................................................... 11 Workshop Agendas and Abstracts ......................................................................................................... 21 Workshop A Beyond Lithium Ion Batteries: Chemistry, Materials, and Characterization .................................................................................... 23 Workshop B The APS MBA Upgrade: Introduction and Scientific Opportunities ............ 28 Workshop C A Historical Perspective: The First 100 Years of Crystallography ................ 30 APS Workshop 1 Inhomogeneities and Defects in Functional Materials: Future Opportunities with the APS MBA Lattice Upgrade .......................... 34 APS Workshop 2 Complex Liquid Interfaces ........................................................................... 41 APS Workshop 3 4D Imaging Applications in Dynamic Studies .............................................. 46 APS/CNM Workshop 4 Imaging at Nanometer and Picosecond Scales: Ultrafast Coherent X-ray Science at a Diffraction-limited Storage Ring ...... 56 APS Workshop 5 Frontier High-pressure Science at Synchrotron Facilities............................ 59 APS Workshop 7 New Advances and Future Opportunities in Phase Contrast Imaging ........ 64 CNM Workshop 8 Solar Energy Capture and Conversion at the Nanoscale ............................ 69 APS Workshop 10 Materials for a Sustainable Energy Future: Advances in Structural Science .................................................................................... 73 Poster Index .............................................................................................................................................. 79 Poster Abstracts ....................................................................................................................................... 91 Exhibitors/Sponsors ............................................................................................................................... 169 General Information ................................................................................................................................ 191 Practical Matters .................................................................................................................................. 193 Computer Access ................................................................................................................................ 195 Exhibitor Location Map/Lower Level .................................................................................................... 196 Exhibitor Location Map/Upper Level .................................................................................................... 197 Schedule at a Glance .....................................................................................................Inside back cover User Science: discoveries for tomorrow iii iv 2014 Users Meeting — May 12–15, 2014 Acknowledgments Overall Meeting Coordination: Constance A. Vanni Scientific Program Coordinators: Administrative Coordinators: APS: Eric Landahl Jane Andrew, APS CNM: Seungbum Hong Linda Carlson, APS EMC: Yasuo Ito Julie Emery, CNM Katie Carrado Gregar, CNM Tracey Stancik, CEP APS User Organization CNM Users Executive Committee Steering Committee Steven May, Drexel University (Chair) Peter Abbamonte, University of Illinois at Matthew Grayson, Northwestern University Urbana-Champaign Axel Hoffmann, Materials Science Div., Lahsen Assoufid, Argonne National Laboratory Argonne National Laboratory Leslie G. Butler, Louisiana State University Seungbum Hong, Nanoscience & Technology, Mark Daymond, Queen’s University Argonne National Laboratory (Vice Chair) Alan I. Goldman, Iowa State University/ Carmen Lilley, University of Illinois at Chicago Ames Laboratory Conal Murray, IBM TJ Watson Research Center Eric Landahl, DePaul University (Vice Chair) Steve Smith, South Dakota School of Mines Robert L. Leheny, Johns Hopkins University (Chair) and Technology Binhua Lin, The University of Chicago John Freeland, Advanced Photon Source, Argonne National Laboratory (ex officio) Karen Mulfort, Argonne National Laboratory Michael S. Pierce, Rochester Institute of Technology Oleg G. Shpyrko, University of California, San Diego EMC Users Executive Committee Yugang Sun, Argonne National Laboratory Carlos Alvarez, Northwestern University Pamela Focia, Northwestern University (ex officio) Phillip Heck, The Field Museum of Natural History Yasuo Ito, Northern Illinois University (Chair) Mitra Taheri, Drexel University User Science: discoveries for tomorrow v 2014 Users Meeting Organizing Committee Deena Blair— General support Rachel Reed — Signage, poster session, social events support, APS Users Organization arrangements, Virginia Brown— Building arrangements meeting coordination Linda Carlson — Web site, user elections, overall Ed Russell — Building arrangements, site coordination coordination, registration Becky Tasker — Building arrangements Jim Corsolini (CEP) — Video support Tara Videtic — Site access Jay Fisher (CEP) — Video support Carmie White, Argonne Guest House — On-site Beverly Knott — General support logistics and amenities coordination Jacquelin LeBreck (CEP) —General support Karin Widuch — Reimbursements, travel Michele Nelson (CEP) — Design and production arrangements, budget tracking, poster session of program book Sponsors is now About Argonne National Laboratory Argonne is a U.S. Department of Energy laboratory managed by the UChicago Argonne, LLC under contract number DE-AC02-06CH11357. The Laboratory is located southwest of Chicago at 9700 South Cass Avenue, Argonne, Illinois 60439. For information about Argonne, see www.anl.gov. vi 2014 Users Meeting — May 12–15, 2014 2014 Rosalind Franklin Award Julian Moosmann Karlsruhe Institute of Technology The APS Users Organization has named Julian The work recognized by this award provides an Moosmann as the winner of the 2014 Rosalind important new modality that could help answer Franklin Young Investigator Award. The award fundamental questions in developmental biology. recognizes Moosmann’s work to develop methods that Although the much-studied Xenopus laevis has have made it possible to obtain time-lapse 3D images been the source of many insights about embryonic of cells and tissues in living vertebrate embryos. The development, certain questions simply cannot be methods will also apply more generally to imaging answered with current technologies. Light microscopes of materials that have low absorption contrast in can’t show cells inside the optically opaque embryos, conventional x-ray imaging. and conventional absorption-based x-ray imaging is not sensitive enough, so phase-contrast techniques are Moosmann, a physics Ph.D. student at Karlsruhe needed. But it is still extremely challenging to capture Institute of Technology (KIT), Karlsruhe, Germany, is cell movement within the developing embryo without cited as an “original, visionary thinker” who is equally killing it. willing to undertake cumbersome experimental work and elaborate numerical simulations. Nominators also Moosmann and Hofmann did not set out to commended his scientific maturity, his ability to master revolutionize developmental biology. They work at techniques from several fields and to work as a team ANKA, the synchrotron light source at KIT, and were player, and his deep understanding of the concepts and interested in exploring the fundamental physics and physics behind the experiments. mathematics of x-ray phase-contrast imaging, which exploits differences in a sample’s refractive index—and Moosmann collaborated with his advisor, physicist the resulting phase changes in the transmitted x-rays— Ralf Hofmann, and an international team of physicists, to create a signal. beamline scientists, and biologists from KIT, Northwestern University, and the APS to apply the One of Moosmann’s key advances was to modify the new methods to image the movement of cells within application of the contrast transfer function (CTF), an embryo of the African claw-toed frog (Xenopus a standard technique used in phase-contrast imaging. laevis) over a period of about two hours. The results He wanted to improve the function’s resolution at a were published in Nature and the methods in Nature greater distance from the sample, that is, at large z. “We Protocols. The initial work was done at APS beamline decided to focus on propagation-based phase-contrast 2-BM-B, and additional experiments at APS beamline imaging because of the simplicity of the technique. 32-ID confirmed the results. The setup is free of additional optics
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