The Delimiting/Frontier Lines of the Constituents of Matter∗
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Hetc-3Step Calculations of Proton Induced Nuclide Production Cross Sections at Incident Energies Between 20 Mev and 5 Gev
JAERI-Research 96-040 JAERI-Research—96-040 JP9609132 JP9609132 HETC-3STEP CALCULATIONS OF PROTON INDUCED NUCLIDE PRODUCTION CROSS SECTIONS AT INCIDENT ENERGIES BETWEEN 20 MEV AND 5 GEV August 1996 Hiroshi TAKADA, Nobuaki YOSHIZAWA* and Kenji ISHIBASHI* Japan Atomic Energy Research Institute 2 G 1 0 1 (T319-11 l This report is issued irregularly. Inquiries about availability of the reports should be addressed to Research Information Division, Department of Intellectual Resources, Japan Atomic Energy Research Institute, Tokai-mura, Naka-gun, Ibaraki-ken, 319-11, Japan. © Japan Atomic Energy Research Institute, 1996 JAERI-Research 96-040 HETC-3STEP Calculations of Proton Induced Nuclide Production Cross Sections at Incident Energies between 20 MeV and 5 GeV Hiroshi TAKADA, Nobuaki YOSHIZAWA* and Kenji ISHIBASHP* Department of Reactor Engineering Tokai Research Establishment Japan Atomic Energy Research Institute Tokai-mura, Naka-gun, Ibaraki-ken (Received July 1, 1996) For the OECD/NEA code intercomparison, nuclide production cross sections of l60, 27A1, nalFe, 59Co, natZr and 197Au for the proton incidence with energies of 20 MeV to 5 GeV are calculated with the HETC-3STEP code based on the intranuclear cascade evaporation model including the preequilibrium and high energy fission processes. In the code, the level density parameter derived by Ignatyuk, the atomic mass table of Audi and Wapstra and the mass formula derived by Tachibana et al. are newly employed in the evaporation calculation part. The calculated results are compared with the experimental ones. It is confirmed that HETC-3STEP reproduces the production of the nuclides having the mass number close to that of the target nucleus with an accuracy of a factor of two to three at incident proton energies above 100 MeV for natZr and 197Au. -
1 11. Nuclear Chemistry 11.1 Stable and Unstable Nuclides Very Large
11. Nuclear Chemistry Chemical reactions occur as a result of loosing/gaining and sharing electrons in the valance shell which is far away from the atomic nucleus as we described in previous chapters in chemical bonding. In chemical reactions identity of the elements (atomic) and the makeup of the nuclei (mass due to protons and neutrons) is preserved which is reflected in the Law of Conservation of mass. This idea of atomic nucleus is always stable was shattered as Henri Becquerel discovered radioactivity in uranium compound where uranium nuclei changes or undergo nuclear reactions where nuclei of an element is transformed into nuclei of different element(s) while emitting ionization radiation. Marie Curie also began a study of radioactivity in a different form of uranium ore called pitchblende and she discovered the existence of two more highly radioactive new elements radium and polonium formed as the products during the decay of unstable nuclide of uranium-235. Curie measure that the radiation emanated was proportional to the amount (moles or number of nuclides) of radioactive element present, and she proposed that radiation was a property nucleus of an unstable atom. The area of chemistry that focuses on the nuclear changes is called nuclear chemistry. What changes in a nuclide result from the loss of each of the following? a) An alpha particle. b) A gamma ray. c) An electron. d) A neutron. e) A proton. Answer: a), c), d), e) 11.1 Stable and Unstable Nuclides There are stable and unstable radioactive nuclides. Unstable nuclides emit subatomic particles, with alpha −α, beta −β, gamma −γ, proton-p, neutrons-n being the most common. -
An Octad for Darmstadtium and Excitement for Copernicium
SYNOPSIS An Octad for Darmstadtium and Excitement for Copernicium The discovery that copernicium can decay into a new isotope of darmstadtium and the observation of a previously unseen excited state of copernicium provide clues to the location of the “island of stability.” By Katherine Wright holy grail of nuclear physics is to understand the stability uncover its position. of the periodic table’s heaviest elements. The problem Ais, these elements only exist in the lab and are hard to The team made their discoveries while studying the decay of make. In an experiment at the GSI Helmholtz Center for Heavy isotopes of flerovium, which they created by hitting a plutonium Ion Research in Germany, researchers have now observed a target with calcium ions. In their experiments, flerovium-288 previously unseen isotope of the heavy element darmstadtium (Z = 114, N = 174) decayed first into copernicium-284 and measured the decay of an excited state of an isotope of (Z = 112, N = 172) and then into darmstadtium-280 (Z = 110, another heavy element, copernicium [1]. The results could N = 170), a previously unseen isotope. They also measured an provide “anchor points” for theories that predict the stability of excited state of copernicium-282, another isotope of these heavy elements, says Anton Såmark-Roth, of Lund copernicium. Copernicium-282 is interesting because it University in Sweden, who helped conduct the experiments. contains an even number of protons and neutrons, and researchers had not previously measured an excited state of a A nuclide’s stability depends on how many protons (Z) and superheavy even-even nucleus, Såmark-Roth says. -
Compilation and Evaluation of Fission Yield Nuclear Data Iaea, Vienna, 2000 Iaea-Tecdoc-1168 Issn 1011–4289
IAEA-TECDOC-1168 Compilation and evaluation of fission yield nuclear data Final report of a co-ordinated research project 1991–1996 December 2000 The originating Section of this publication in the IAEA was: Nuclear Data Section International Atomic Energy Agency Wagramer Strasse 5 P.O. Box 100 A-1400 Vienna, Austria COMPILATION AND EVALUATION OF FISSION YIELD NUCLEAR DATA IAEA, VIENNA, 2000 IAEA-TECDOC-1168 ISSN 1011–4289 © IAEA, 2000 Printed by the IAEA in Austria December 2000 FOREWORD Fission product yields are required at several stages of the nuclear fuel cycle and are therefore included in all large international data files for reactor calculations and related applications. Such files are maintained and disseminated by the Nuclear Data Section of the IAEA as a member of an international data centres network. Users of these data are from the fields of reactor design and operation, waste management and nuclear materials safeguards, all of which are essential parts of the IAEA programme. In the 1980s, the number of measured fission yields increased so drastically that the manpower available for evaluating them to meet specific user needs was insufficient. To cope with this task, it was concluded in several meetings on fission product nuclear data, some of them convened by the IAEA, that international co-operation was required, and an IAEA co-ordinated research project (CRP) was recommended. This recommendation was endorsed by the International Nuclear Data Committee, an advisory body for the nuclear data programme of the IAEA. As a consequence, the CRP on the Compilation and Evaluation of Fission Yield Nuclear Data was initiated in 1991, after its scope, objectives and tasks had been defined by a preparatory meeting. -
Radioactive Decay
North Berwick High School Department of Physics Higher Physics Unit 2 Particles and Waves Section 3 Fission and Fusion Section 3 Fission and Fusion Note Making Make a dictionary with the meanings of any new words. Einstein and nuclear energy 1. Write down Einstein’s famous equation along with units. 2. Explain the importance of this equation and its relevance to nuclear power. A basic model of the atom 1. Copy the components of the atom diagram and state the meanings of A and Z. 2. Copy the table on page 5 and state the difference between elements and isotopes. Radioactive decay 1. Explain what is meant by radioactive decay and copy the summary table for the three types of nuclear radiation. 2. Describe an alpha particle, including the reason for its short range and copy the panel showing Plutonium decay. 3. Describe a beta particle, including its range and copy the panel showing Tritium decay. 4. Describe a gamma ray, including its range. Fission: spontaneous decay and nuclear bombardment 1. Describe the differences between the two methods of decay and copy the equation on page 10. Nuclear fission and E = mc2 1. Explain what is meant by the terms ‘mass difference’ and ‘chain reaction’. 2. Copy the example showing the energy released during a fission reaction. 3. Briefly describe controlled fission in a nuclear reactor. Nuclear fusion: energy of the future? 1. Explain why nuclear fusion might be a preferred source of energy in the future. 2. Describe some of the difficulties associated with maintaining a controlled fusion reaction. -
Heavy Element Nucleosynthesis
Heavy Element Nucleosynthesis A summary of the nucleosynthesis of light elements is as follows 4He Hydrogen burning 3He Incomplete PP chain (H burning) 2H, Li, Be, B Non-thermal processes (spallation) 14N, 13C, 15N, 17O CNO processing 12C, 16O Helium burning 18O, 22Ne α captures on 14N (He burning) 20Ne, Na, Mg, Al, 28Si Partly from carbon burning Mg, Al, Si, P, S Partly from oxygen burning Ar, Ca, Ti, Cr, Fe, Ni Partly from silicon burning Isotopes heavier than iron (as well as some intermediate weight iso- topes) are made through neutron captures. Recall that the prob- ability for a non-resonant reaction contained two components: an exponential reflective of the quantum tunneling needed to overcome electrostatic repulsion, and an inverse energy dependence arising from the de Broglie wavelength of the particles. For neutron cap- tures, there is no electrostatic repulsion, and, in complex nuclei, virtually all particle encounters involve resonances. As a result, neutron capture cross-sections are large, and are very nearly inde- pendent of energy. To appreciate how heavy elements can be built up, we must first consider the lifetime of an isotope against neutron capture. If the cross-section for neutron capture is independent of energy, then the lifetime of the species will be ( )1=2 1 1 1 µn τn = ≈ = Nnhσvi NnhσivT Nnhσi 2kT For a typical neutron cross-section of hσi ∼ 10−25 cm2 and a tem- 8 9 perature of 5 × 10 K, τn ∼ 10 =Nn years. Next consider the stability of a neutron rich isotope. If the ratio of of neutrons to protons in an atomic nucleus becomes too large, the nucleus becomes unstable to beta-decay, and a neutron is changed into a proton via − (Z; A+1) −! (Z+1;A+1) + e +ν ¯e (27:1) The timescale for this decay is typically on the order of hours, or ∼ 10−3 years (with a factor of ∼ 103 scatter). -
A Guide to Naturally Occurring Radioactive Materials (NORM)
ABOUT NORM SOME NORM NUCLIDES OF SPECIAL INTEREST A Guide to Naturally There are three types of NORM: Occurring Radioactive • Cosmogenic – NORM produced by cosmic rays interacting with the Earth’s Materials (NORM) Beryllium 7 atmosphere; the most important Developed by the 3 7 14 examples are H (tritium), Be, and C. 7Be is being continuously formed in the DHS Secondary Reachback Program • Primordial – Sufficiently long-lived atmosphere by cosmic rays. Jet engines can March 2010 NORM for some to have survived from accumulate enough 7Be to set off before the formation of the Earth; there radiological alarms when being cleaned. are 20 primordial NORM nuclides with As defined by the International Atomic the most important being 40K, 232Th, Energy Agency (IAEA), Naturally 235U, and 238U. Polonium 210 Occurring Radioactive Materials • Daughters – When 232Th, 235U and 238U In the 238U decay chain 210Po is a distant (NORM) include all natural radioactive decay 42 different radioactive nuclides daughter of 226Ra. 210Po gained notoriety in materials where human activities have are formed (see below) with the most the 1960s as a radioactive trace component increased the potential for exposure in important being 222Rn, 226Ra, 228Ra and in cigarette smoke. Heavy use of phosphate comparison with the unaltered natural 228 Ac. fertilizers (which have trace amounts of out here. fold Next situation. If processing has increased 226Ra) can triple the amount of 210Po found the concentrations of radionuclides in a When 232Th, 235U and 238U decay a in tobacco. material then it is Technologically radioactive “daughter” nuclide is formed, Enhanced NORM (TE-NORM). -
Mass Defect & Binding Energy
Sem-3 CC7 Nuclear Physics Mass Defect & Binding Energy According to nuclear particle experiments, the total mass of a nucleus (mnuc) is less than the sum of the masses of its constituent nucleons (protons and neutrons). For a nucleus with Z protons and mass number A, the mass difference or mass defect is given by Δm= Zmp + (A−Z)mn − mnuc where Zmp is the total mass of the protons, (A−Z)mn is the total mass of the neutrons, and mnuc is the mass of the nucleus. According to Einstein’s special theory of relativity, mass is a measure of the total energy of a system (E=mc2). The energy equivalent to mass defect is alled the binding energy B of the nucleus. Thus 2 B= [Zmp + (A−Z)mn − mnuc] c The binding energy is equal to the amount of energy released in forming the nucleus. Example 1. Calculate the mass defect and the binding energy of the deuteron. The mass of the −27 deuteron is mD=3.34359×10 kg or 2.014102u. Solution For the deuteron Z=1 and A=2. The mass defect for the deuteron is Δm=mp+mn−mD=1.008665 u+ 1.007825 u- 2.014102u = 0.002388u The binding energy of the deuteron is then B= Δm c2= Δm ×931.5 MeV/u=2.224MeV. Over two million electron volts are needed to break apart a deuteron into a proton and a neutron. This very large value indicates the great strength of the nuclear force. By comparison, the greatest amount of energy required to liberate an electron bound to a hydrogen atom by an attractive Coulomb force (an electromagnetic force) is about 10 eV. -
Iron-57 of Its Isotopes and Has an Sum of Protons + Neutrons 26 Fe Average Mass As Determined by a in the Nucleus
Elements - elements are pure homogeneous forms of matter Solid Liquid Gas Plamsa •constant volume & shape •constant volume but takes •varaible shape and volume •like a gas except it •very low compressibility on the shape of container that fills the container is composed of ions; •particles vibrate in place •low compressibility •high compressibility an ion is charged •highly ordered arrangement •random particle movement •complete freedom of motion atom or group of •do not flow or diffuse •moderate disorder •extreme disorder atoms. •strongest attractive forces •can flow and diffuse •flow and diffuse easily •examples: between particles •weaker attractive forces •weakest attractive forces - flames •generally more dense than •more dense than gases •least dense state - atmosphere of stars liquids •exert a pressure easily - a comet's tail Matter NO YES Pure Substance Can it be separated Mixture by physical means? Can it be decomposed by Is the mixture composition ordinary chemical means? identical throughout; uniform? NO YES YES NO element compound homogeneous heterogenous mixture mixture Co,Fe,S,H,O,C FeS, H2O, H2SO4 steel, air, blood, steam, wet iron, solution of sulfuric acid Cannot be separated Can be decomposed and rust on steel chemcially into simple chemcially separated Uniform appearance, Appearance, composition, substances into simple substances. composition and and properties are variable properties throughout in different parts of the sample Isotopes Is a mass number attached to the element? NO YES All atoms of the same element are not exactly alike mass number attached mass number equals the 57 The element is as a mixture also can be written as iron-57 of its isotopes and has an sum of protons + neutrons 26 Fe average mass as determined by a in the nucleus. -
1 Chapter 16 Stable and Radioactive Isotopes Jim Murray 5/7/01 Univ
Chapter 16 Stable and Radioactive Isotopes Jim Murray 5/7/01 Univ. Washington Each atomic element (defined by its number of protons) comes in different flavors, depending on the number of neutrons. Most elements in the periodic table exist in more than one isotope. Some are stable and some are radioactive. Scientists have tallied more than 3600 isotopes, the majority are radioactive. The Isotopes Project at Lawrence Berkeley National Lab in California has a web site (http://ie.lbl.gov/toi.htm) that gives detailed information about all the isotopes. Stable and radioactive isotopes are the most useful class of tracers available to geochemists. In almost all cases the distributions of these isotopes have been used to study oceanographic processes controlling the distributions of the elements. Radioactive isotopes are especially useful because they provide a way to put time into geochemical models. The chemical characteristic of an element is determined by the number of protons in its nucleus. Different elements can have different numbers of neutrons and thus atomic weights (the sum of protons plus neutrons). The atomic weight is equal to the sum of protons plus neutrons. The chart of the nuclides (protons versus neutrons) for elements 1 (Hydrogen) through 12 (Magnesium) is shown in Fig. 16-1. The Valley of Stability represents nuclides stable relative to decay. Examples: Atomic Protons Neutrons % Abundance Weight (Atomic Number) Carbon 12C 6P 6N 98.89 13C 6P 7N 1.11 14C 6P 8N 10-10 Oxygen 16O 8P 8N 99.76 17O 8P 9N 0.024 18O 8P 10N 0.20 Several light elements such as H, C, N, O, and S have more than one stable isotope form, which show variable abundances in natural samples. -
Quest for Superheavy Nuclei Began in the 1940S with the Syn Time It Takes for Half of the Sample to Decay
FEATURES Quest for superheavy nuclei 2 P.H. Heenen l and W Nazarewicz -4 IService de Physique Nucleaire Theorique, U.L.B.-C.P.229, B-1050 Brussels, Belgium 2Department ofPhysics, University ofTennessee, Knoxville, Tennessee 37996 3Physics Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 4Institute ofTheoretical Physics, University ofWarsaw, ul. Ho\.za 69, PL-OO-681 Warsaw, Poland he discovery of new superheavy nuclei has brought much The superheavy elements mark the limit of nuclear mass and T excitement to the atomic and nuclear physics communities. charge; they inhabit the upper right corner of the nuclear land Hopes of finding regions of long-lived superheavy nuclei, pre scape, but the borderlines of their territory are unknown. The dicted in the early 1960s, have reemerged. Why is this search so stability ofthe superheavy elements has been a longstanding fun important and what newknowledge can it bring? damental question in nuclear science. How can they survive the Not every combination ofneutrons and protons makes a sta huge electrostatic repulsion? What are their properties? How ble nucleus. Our Earth is home to 81 stable elements, including large is the region of superheavy elements? We do not know yet slightly fewer than 300 stable nuclei. Other nuclei found in all the answers to these questions. This short article presents the nature, although bound to the emission ofprotons and neutrons, current status ofresearch in this field. are radioactive. That is, they eventually capture or emit electrons and positrons, alpha particles, or undergo spontaneous fission. Historical Background Each unstable isotope is characterized by its half-life (T1/2) - the The quest for superheavy nuclei began in the 1940s with the syn time it takes for half of the sample to decay. -
The Nucleus and Nuclear Instability
Lecture 2: The nucleus and nuclear instability Nuclei are described using the following nomenclature: A Z Element N Z is the atomic number, the number of protons: this defines the element. A is called the “mass number” A = N + Z. N is the number of neutrons (N = A - Z) Nuclide: A species of nucleus of a given Z and A. Isotope: Nuclides of an element (i.e. same Z) with different N. Isotone: Nuclides having the same N. Isobar: Nuclides having the same A. [A handy way to keep these straight is to note that isotope includes the letter “p” (same proton number), isotone the letter “n” (same neutron number), and isobar the letter “a” (same A).] Example: 206 82 Pb124 is an isotope of 208 82 Pb126 is an isotone of 207 83 Bi124 and an isobar of 206 84 Po122 1 Chart of the Nuclides Image removed. 90 natural elements 109 total elements All elements with Z > 42 are man-made Except for technicium Z=43 Promethium Z = 61 More than 800 nuclides are known (274 are stable) “stable” unable to transform into another configuration without the addition of outside energy. “unstable” = radioactive Images removed. [www2.bnl.gov/ton] 2 Nuclear Structure: Forces in the nucleus Coulomb Force Force between two point charges, q, separated by distance, r (Coulomb’s Law) k0 q1q2 F(N) = 9 2 -2 r 2 k0 = 8.98755 x 10 N m C (Boltzman constant) Potential energy (MeV) of one particle relative to the other k q q PE(MeV)= 0 1 2 r Strong Nuclear Force • Acts over short distances • ~ 10-15 m • can overcome Coulomb repulsion • acts on protons and neutrons Image removed.