The Impact of Individual Nuclear Properties on $ R $-Process
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1 Chapter 16 Stable and Radioactive Isotopes Jim Murray 5/7/01 Univ
Chapter 16 Stable and Radioactive Isotopes Jim Murray 5/7/01 Univ. Washington Each atomic element (defined by its number of protons) comes in different flavors, depending on the number of neutrons. Most elements in the periodic table exist in more than one isotope. Some are stable and some are radioactive. Scientists have tallied more than 3600 isotopes, the majority are radioactive. The Isotopes Project at Lawrence Berkeley National Lab in California has a web site (http://ie.lbl.gov/toi.htm) that gives detailed information about all the isotopes. Stable and radioactive isotopes are the most useful class of tracers available to geochemists. In almost all cases the distributions of these isotopes have been used to study oceanographic processes controlling the distributions of the elements. Radioactive isotopes are especially useful because they provide a way to put time into geochemical models. The chemical characteristic of an element is determined by the number of protons in its nucleus. Different elements can have different numbers of neutrons and thus atomic weights (the sum of protons plus neutrons). The atomic weight is equal to the sum of protons plus neutrons. The chart of the nuclides (protons versus neutrons) for elements 1 (Hydrogen) through 12 (Magnesium) is shown in Fig. 16-1. The Valley of Stability represents nuclides stable relative to decay. Examples: Atomic Protons Neutrons % Abundance Weight (Atomic Number) Carbon 12C 6P 6N 98.89 13C 6P 7N 1.11 14C 6P 8N 10-10 Oxygen 16O 8P 8N 99.76 17O 8P 9N 0.024 18O 8P 10N 0.20 Several light elements such as H, C, N, O, and S have more than one stable isotope form, which show variable abundances in natural samples. -
Quest for Superheavy Nuclei Began in the 1940S with the Syn Time It Takes for Half of the Sample to Decay
FEATURES Quest for superheavy nuclei 2 P.H. Heenen l and W Nazarewicz -4 IService de Physique Nucleaire Theorique, U.L.B.-C.P.229, B-1050 Brussels, Belgium 2Department ofPhysics, University ofTennessee, Knoxville, Tennessee 37996 3Physics Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 4Institute ofTheoretical Physics, University ofWarsaw, ul. Ho\.za 69, PL-OO-681 Warsaw, Poland he discovery of new superheavy nuclei has brought much The superheavy elements mark the limit of nuclear mass and T excitement to the atomic and nuclear physics communities. charge; they inhabit the upper right corner of the nuclear land Hopes of finding regions of long-lived superheavy nuclei, pre scape, but the borderlines of their territory are unknown. The dicted in the early 1960s, have reemerged. Why is this search so stability ofthe superheavy elements has been a longstanding fun important and what newknowledge can it bring? damental question in nuclear science. How can they survive the Not every combination ofneutrons and protons makes a sta huge electrostatic repulsion? What are their properties? How ble nucleus. Our Earth is home to 81 stable elements, including large is the region of superheavy elements? We do not know yet slightly fewer than 300 stable nuclei. Other nuclei found in all the answers to these questions. This short article presents the nature, although bound to the emission ofprotons and neutrons, current status ofresearch in this field. are radioactive. That is, they eventually capture or emit electrons and positrons, alpha particles, or undergo spontaneous fission. Historical Background Each unstable isotope is characterized by its half-life (T1/2) - the The quest for superheavy nuclei began in the 1940s with the syn time it takes for half of the sample to decay. -
Nuclear Binding & Stability
Nuclear Binding & Stability Stanley Yen TRIUMF UNITS: ENERGY Energy measured in electron-Volts (eV) 1 volt battery boosts energy of electrons by 1 eV 1 volt -19 battery 1 e-Volt = 1.6x10 Joule 1 MeV = 106 eV 1 GeV = 109 eV Recall that atomic and molecular energies ~ eV nuclear energies ~ MeV UNITS: MASS From E = mc2 m = E / c2 so we measure masses in MeV/c2 1 MeV/c2 = 1.7827 x 10 -30 kg Frequently, we get lazy and just set c=1, so that we measure masses in MeV e.g. mass of electron = 0.511 MeV mass of proton = 938.272 MeV mass of neutron=939.565 MeV Also widely used unit of mass is the atomic mass unit (amu or u) defined so that Mass(12C atom) = 12 u -27 1 u = 931.494 MeV = 1.6605 x 10 kg nucleon = proton or neutron “nuclide” means one particular nuclear species, e.g. 7Li and 56Fe are two different nuclides There are 4 fundamental types of forces in the universe. 1. Gravity – very weak, negligible for nuclei except for neutron stars 2. Electromagnetic forces – Coulomb repulsion tends to force protons apart ) 3. Strong nuclear force – binds nuclei together; short-ranged 4. Weak nuclear force – causes nuclear beta decay, almost negligible compared to the strong and EM forces. How tightly a nucleus is bound together is mostly an interplay between the attractive strong force and the repulsive electromagnetic force. Let's make a scatterplot of all the stable nuclei, with proton number Z versus neutron number N. -
The Delimiting/Frontier Lines of the Constituents of Matter∗
The delimiting/frontier lines of the constituents of matter∗ Diógenes Galetti1 and Salomon S. Mizrahi2 1Instituto de Física Teórica, Universidade Estadual Paulista (UNESP), São Paulo, SP, Brasily 2Departamento de Física, CCET, Universidade Federal de São Carlos, São Carlos, SP, Brasilz (Dated: October 23, 2019) Abstract Looking at the chart of nuclides displayed at the URL of the International Atomic Energy Agency (IAEA) [1] – that contains all the known nuclides, the natural and those produced artificially in labs – one verifies the existence of two, not quite regular, delimiting lines between which dwell all the nuclides constituting matter. These lines are established by the highly unstable radionuclides located the most far away from those in the central locus, the valley of stability. Here, making use of the “old” semi-empirical mass formula for stable nuclides together with the energy-time uncertainty relation of quantum mechanics, by a simple calculation we show that the obtained frontier lines, for proton and neutron excesses, present an appreciable agreement with the delimiting lines. For the sake of presenting a somewhat comprehensive panorama of the matter in our Universe and their relation with the frontier lines, we narrate, in brief, what is currently known about the astrophysical nucleogenesis processes. Keywords: chart of nuclides, nucleogenesis, nuclide mass formula, valley/line of stability, energy-time un- certainty relation, nuclide delimiting/frontier lines, drip lines arXiv:1909.07223v2 [nucl-th] 22 Oct 2019 ∗ This manuscript is based on an article that was published in Brazilian portuguese language in the journal Revista Brasileira de Ensino de Física, 2018, 41, e20180160. http://dx.doi.org/10.1590/ 1806-9126-rbef-2018-0160. -
The R-Process of Stellar Nucleosynthesis: Astrophysics and Nuclear Physics Achievements and Mysteries
The r-process of stellar nucleosynthesis: Astrophysics and nuclear physics achievements and mysteries M. Arnould, S. Goriely, and K. Takahashi Institut d'Astronomie et d'Astrophysique, Universit´eLibre de Bruxelles, CP226, B-1050 Brussels, Belgium Abstract The r-process, or the rapid neutron-capture process, of stellar nucleosynthesis is called for to explain the production of the stable (and some long-lived radioac- tive) neutron-rich nuclides heavier than iron that are observed in stars of various metallicities, as well as in the solar system. A very large amount of nuclear information is necessary in order to model the r-process. This concerns the static characteristics of a large variety of light to heavy nuclei between the valley of stability and the vicinity of the neutron-drip line, as well as their beta-decay branches or their reactivity. Fission probabilities of very neutron-rich actinides have also to be known in order to determine the most massive nuclei that have a chance to be involved in the r-process. Even the properties of asymmetric nuclear matter may enter the problem. The enormously challenging experimental and theoretical task imposed by all these requirements is reviewed, and the state-of-the-art development in the field is presented. Nuclear-physics-based and astrophysics-free r-process models of different levels of sophistication have been constructed over the years. We review their merits and their shortcomings. The ultimate goal of r-process studies is clearly to identify realistic sites for the development of the r-process. Here too, the challenge is enormous, and the solution still eludes us. -
CHAPTER 2 the Nucleus and Radioactive Decay
1 CHEMISTRY OF THE EARTH CHAPTER 2 The nucleus and radioactive decay 2.1 The atom and its nucleus An atom is characterized by the total positive charge in its nucleus and the atom’s mass. The positive charge in the nucleus is Ze , where Z is the total number of protons in the nucleus and e is the charge of one proton. The number of protons in an atom, Z, is known as the atomic number and dictates which element an atom represents. The nucleus is also made up of N number of neutrally charged particles of similar mass as the protons. These are called neutrons . The combined number of protons and neutrons, Z+N , is called the atomic mass number A. A specific nuclear species, or nuclide , is denoted by A Z Γ 2.1 where Γ represents the element’s symbol. The subscript Z is often dropped because it is redundant if the element’s symbol is also used. We will soon learn that a mole of protons and a mole of neutrons each have a mass of approximately 1 g, and therefore, the mass of a mole of Z+N should be very close to an integer 1. However, if we look at a periodic table, we will notice that an element’s atomic weight, which is the mass of one mole of its atoms, is rarely close to an integer. For example, Iridium’s atomic weight is 192.22 g/mole. The reason for this discrepancy is that an element’s neutron number N can vary. -
Nuclear Mass and Stability
CHAPTER 3 Nuclear Mass and Stability Contents 3.1. Patterns of nuclear stability 41 3.2. Neutron to proton ratio 43 3.3. Mass defect 45 3.4. Binding energy 47 3.5. Nuclear radius 48 3.6. Semiempirical mass equation 50 3.7. Valley of $-stability 51 3.8. The missing elements: 43Tc and 61Pm 53 3.8.1. Promethium 53 3.8.2. Technetium 54 3.9. Other modes of instability 56 3.10. Exercises 56 3.11. Literature 57 3.1. Patterns of nuclear stability There are approximately 275 different nuclei which have shown no evidence of radioactive decay and, hence, are said to be stable with respect to radioactive decay. When these nuclei are compared for their constituent nucleons, we find that approximately 60% of them have both an even number of protons and an even number of neutrons (even-even nuclei). The remaining 40% are about equally divided between those that have an even number of protons and an odd number of neutrons (even-odd nuclei) and those with an odd number of protons and an even number of neutrons (odd-even nuclei). There are only 5 stable nuclei known which have both 2 6 10 14 an odd number of protons and odd number of neutrons (odd-odd nuclei); 1H, 3Li, 5B, 7N, and 50 23V. It is significant that the first stable odd-odd nuclei are abundant in the very light elements 2 (the low abundance of 1H has a special explanation, see Ch. 17). The last nuclide is found in low isotopic abundance (0.25%) and we cannot be certain that this nuclide is not unstable to radioactive decay with extremely long half-life. -
Nuclear Physics and Astrophysics SPA5302, 2019 Chris Clarkson, School of Physics & Astronomy [email protected]
Nuclear Physics and Astrophysics SPA5302, 2019 Chris Clarkson, School of Physics & Astronomy [email protected] These notes are evolving, so please let me know of any typos, factual errors etc. They will be updated weekly on QM+ (and may include updates to early parts we have already covered). Note that material in purple ‘Digression’ boxes is not examinable. Updated 16:29, on 05/12/2019. Contents 1 Basic Nuclear Properties4 1.1 Length Scales, Units and Dimensions............................7 2 Nuclear Properties and Models8 2.1 Nuclear Radius and Distribution of Nucleons.......................8 2.1.1 Scattering Cross Section............................... 12 2.1.2 Matter Distribution................................. 18 2.2 Nuclear Binding Energy................................... 20 2.3 The Nuclear Force....................................... 24 2.4 The Liquid Drop Model and the Semi-Empirical Mass Formula............ 26 2.5 The Shell Model........................................ 33 2.5.1 Nuclei Configurations................................ 44 3 Radioactive Decay and Nuclear Instability 48 3.1 Radioactive Decay...................................... 49 CONTENTS CONTENTS 3.2 a Decay............................................. 56 3.2.1 Decay Mechanism and a calculation of t1/2(Q) .................. 58 3.3 b-Decay............................................. 62 3.3.1 The Valley of Stability................................ 64 3.3.2 Neutrinos, Leptons and Weak Force........................ 68 3.4 g-Decay........................................... -
Nuclei at the Limits of Particle Stability
0» Nuclei at the limits of particle stability Alex C. Mueller Bradley M. Sherrill IPNO-DRE 9,3-10 t MSU CL 883 \ Vr - J Michigan State University National Superconducting Cyclotron Laboratory Nuclei at the limits of particle stability Alex C. Mueller Bradley M. SherriJl IPNO-DRE 93-10 MSU CL 883 Michigan State University National Superconducting Cyclotron Laboratory NUCLEI AT THE LIMITS OF PARTICLE STABILITY Alex C. Mueller CNRS-IN2P3, Institut de Physique Nucléaire, F-91406 Orsay, France and Bradley M. Sherritt National Superconducting Cyclotron Laboratoiy, Michigan State University, East Lansing, MI48824, USA KEY WORDS: nuclear ^-stability, production of unstable nuclei, on-line isotope separators and recoil spectrometers, reactions induced by unstable nuclei, properties of nuclei at the drip-lines, neutron-halo, nuclei far off stability in astrophysics Shortened Title: Exotic Nuclei (to appear in Annual Review of Nuclear and Particle Science, Volume 43) CONTENTS !.INTRODUCTION 3 2. THE LIMITS OF STABILITY 4 3. TECHNIQUES OF PRODUCTION 7 3.1 Overview 7 3.2 ISOL techniques 7 3.3 Recoil separators 9 4. PROTON-RICH NUCLEI 13 4.1 Searches for the location of the proton drip-line 13 4.2 Properties of proton rich nuclei 16 4.3 Beyond the proton drip-line 20 4.4 Astrophysics: breakout from the CNO-cvcle and the rp-process 22 4.5 Properties and synthesis of the heaviest elements 24 5. NEUTRON-RICH NUCLEI 26 5.1 Mapping of the neutron drip-line 26 5.2 Nuclear masses along the neutron drip-line 28 5.3 Decay studies 30 5.4 Nuclear moments 32 5.5 Nuclear radii, matter and charge distributions 33 5.6 Reaction studies of the halo nuclei: cross-sections, momentum distributions and neutron correlations 35 5.7 Some comments on the neutron halo. -
Microscopic Calculations of Beta-Decay Rates for R-Process
Vol. 48 (2017) ACTA PHYSICA POLONICA B No 3 MICROSCOPIC CALCULATIONS OF β-DECAY RATES FOR r-PROCESS∗ Tomislav Marketina, André Sieverdingb, Meng-Ru Wub Nils Paara, Gabriel Martínez-Pinedob;c aDepartment of Physics, Faculty of Science, University of Zagreb 10000 Zagreb, Croatia bInstitut für Kernphysik (Theoriezentrum), Technische Universität Darmstadt 64289 Darmstadt, Germany cGSI Helmholtzzentrum für Schwerionenforschung Planckstraße 1, 64291 Darmstadt, Germany (Received January 17, 2017) Elements heavier than iron are being created in massive, explosive as- trophysical scenarios such as core-collapse supernovae and neutron star mergers. Heavy element nucleosynthesis is a very complex process that requires the knowledge of the properties, mainly nuclear masses, neutron capture and beta-decay rates, of thousands of nuclei. However, due to the limitations of current experimental facilities, only a relatively small num- ber of nuclei have so far been studied experimentally. Given the amount of nuclei, and the regions of the nuclear chart involved in the heavy element nucleosynthesis, it is necessary to use models that can be reliably applied to even the most exotic nuclei. Thus, the use of microscopic nuclear structure models presents itself as the logical choice, because the underlying micro- scopic theory of nuclear interaction is expected to be valid across the whole nuclear chart. In this manuscript, we present the results of a large-scale cal- culation of β-decay rates using a fully self-consistent theoretical framework based on the relativistic nuclear energy density functional. Taking into ac- count the first-forbidden transitions, we are able to determine the regions of the nuclear chart where these transitions are critical for the description of the decay rates. -
Nuclear Physics
Phys 239 Quantitative Physics Lecture 18 Nuclear Physics What can a non-nuclear physicist tell you about nuclear physics that would be worth your while? Admittedly, I will only scratch the surface of the rich subject, and offer some quantitative tools and big-picture perspective. The Physicist’s Periodic Table Hanging in virtully every classroom is the Chemist’s Periodic Table of Elements. Child’s play. Physicists need a Chart of the Nuclides. An interactive version can be found at http://www.nndc.bnl.gov/chart/. An excerpt at the bottom end appears below. Proton number (Z) runs up the left side and neutron number (N) along the bottom. Ask a periodic table for the mass of a lithium atom and it’ll say 6.941 a.m.u. The chart of the nuclides will say that lithium has two stable isotopes: 6Li at mass 6.015122 a.m.u. comprising 7.59% of natural abundance, and 7Li at 7.016004 a.m.u. making up the lion’s share at 92.41%. Show off. You can also learn that 8Li has a lifetime of 0.84 s, decaying by β− to 8Be, which itself lasts less than 10−16 s before breaking into two 4He nuclei. And so it goes. The chart of the nuclides is a treasure trove of quantitative information about nuclei: masses, abundances, decay chains, half-lives, energy, neutron absorption cross section, excited states, nuclear spin. Really amazing. 1 You can see, for instance, that starting with four hydrogen atoms in the Sun (okay; nuclei, but their elec- trons are somewhere nearby) and ending up with a helium nucleus goes from 4 times 1.007825032 a.m.u. -
The Mass of a Nucleus
The mass of a nucleus • Energy generation in stars • which nuclei are stable • which nuclei exist in principle 1 SOHO, 171A Fe emission line Nucleons Mass Spin Charge size: ~1 fm Proton 938.272 MeV/c2 1/2 +1e Neutron 939.565 MeV/c2 1/2 0 Nuclei nucleons attract each other via the strong force ( range ~ 1 fm) a bunch of nucleons bound together create a potential for an additional : neutron proton (or any other charged particle) V V l Coulomb Barrier V 1/3 l c a a i R ~ 1.3 x A fm 2 i t t n Z1 Z 2 e n e e t V = t c o R o R P P … R … r r Nucleons in a Box: Discrete energy levels in nucleus Æ Nucleons are bound by attractive force. Therefore, mass of nucleus is smaller than the total mass of the nucleons by the binding energy dm=B/c2 2 Nuclear Masses and Binding Energy Energy that is released when a nucleus is assembled from neutrons and protons 2 m Z N(,)= Zmp +n Nm −/ B c mp = proton mass, mn = neutron mass, m(Z,N) = mass of nucleus with Z,N 0 > •B • With B the mass of the nucleus is determined. • B is very roughly ~A Masses are usually tabulated as atomic masses m = mnuc + Z me - Be Nuclear Mass Electron Mass Electron Binding Energy ~ 1 GeV/A 511 keV/Z 13.6 eV (H) to 116 keV (K-shell U) / Z 2 Most tables give atomic mass excess Δ in MeV:m= Amu +/ Δ c (so for 12C: Δ=0) (see nuclear wallet cards for a table) 3 Q-value Energy released in a nuclear reaction (>0 if energy is released, 0 if energy is use<d Example: The sun is powered by the fusion of hydrogen into helium: 4 + 4p Æ He + 2 e + 2νe Mass difference dM released as eneryg dE = dM c2 2 (using nuclear masses !) Q/ c=nuc 4 m p − nuc4 m 2m − He e 2 −ν m 4 In practice one often uses mass excess Δ and atomic masses.