Light Nuclides Produced in the Proton-Induced Spallation of U at 1
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Hetc-3Step Calculations of Proton Induced Nuclide Production Cross Sections at Incident Energies Between 20 Mev and 5 Gev
JAERI-Research 96-040 JAERI-Research—96-040 JP9609132 JP9609132 HETC-3STEP CALCULATIONS OF PROTON INDUCED NUCLIDE PRODUCTION CROSS SECTIONS AT INCIDENT ENERGIES BETWEEN 20 MEV AND 5 GEV August 1996 Hiroshi TAKADA, Nobuaki YOSHIZAWA* and Kenji ISHIBASHI* Japan Atomic Energy Research Institute 2 G 1 0 1 (T319-11 l This report is issued irregularly. Inquiries about availability of the reports should be addressed to Research Information Division, Department of Intellectual Resources, Japan Atomic Energy Research Institute, Tokai-mura, Naka-gun, Ibaraki-ken, 319-11, Japan. © Japan Atomic Energy Research Institute, 1996 JAERI-Research 96-040 HETC-3STEP Calculations of Proton Induced Nuclide Production Cross Sections at Incident Energies between 20 MeV and 5 GeV Hiroshi TAKADA, Nobuaki YOSHIZAWA* and Kenji ISHIBASHP* Department of Reactor Engineering Tokai Research Establishment Japan Atomic Energy Research Institute Tokai-mura, Naka-gun, Ibaraki-ken (Received July 1, 1996) For the OECD/NEA code intercomparison, nuclide production cross sections of l60, 27A1, nalFe, 59Co, natZr and 197Au for the proton incidence with energies of 20 MeV to 5 GeV are calculated with the HETC-3STEP code based on the intranuclear cascade evaporation model including the preequilibrium and high energy fission processes. In the code, the level density parameter derived by Ignatyuk, the atomic mass table of Audi and Wapstra and the mass formula derived by Tachibana et al. are newly employed in the evaporation calculation part. The calculated results are compared with the experimental ones. It is confirmed that HETC-3STEP reproduces the production of the nuclides having the mass number close to that of the target nucleus with an accuracy of a factor of two to three at incident proton energies above 100 MeV for natZr and 197Au. -
An Octad for Darmstadtium and Excitement for Copernicium
SYNOPSIS An Octad for Darmstadtium and Excitement for Copernicium The discovery that copernicium can decay into a new isotope of darmstadtium and the observation of a previously unseen excited state of copernicium provide clues to the location of the “island of stability.” By Katherine Wright holy grail of nuclear physics is to understand the stability uncover its position. of the periodic table’s heaviest elements. The problem Ais, these elements only exist in the lab and are hard to The team made their discoveries while studying the decay of make. In an experiment at the GSI Helmholtz Center for Heavy isotopes of flerovium, which they created by hitting a plutonium Ion Research in Germany, researchers have now observed a target with calcium ions. In their experiments, flerovium-288 previously unseen isotope of the heavy element darmstadtium (Z = 114, N = 174) decayed first into copernicium-284 and measured the decay of an excited state of an isotope of (Z = 112, N = 172) and then into darmstadtium-280 (Z = 110, another heavy element, copernicium [1]. The results could N = 170), a previously unseen isotope. They also measured an provide “anchor points” for theories that predict the stability of excited state of copernicium-282, another isotope of these heavy elements, says Anton Såmark-Roth, of Lund copernicium. Copernicium-282 is interesting because it University in Sweden, who helped conduct the experiments. contains an even number of protons and neutrons, and researchers had not previously measured an excited state of a A nuclide’s stability depends on how many protons (Z) and superheavy even-even nucleus, Såmark-Roth says. -
Compilation and Evaluation of Fission Yield Nuclear Data Iaea, Vienna, 2000 Iaea-Tecdoc-1168 Issn 1011–4289
IAEA-TECDOC-1168 Compilation and evaluation of fission yield nuclear data Final report of a co-ordinated research project 1991–1996 December 2000 The originating Section of this publication in the IAEA was: Nuclear Data Section International Atomic Energy Agency Wagramer Strasse 5 P.O. Box 100 A-1400 Vienna, Austria COMPILATION AND EVALUATION OF FISSION YIELD NUCLEAR DATA IAEA, VIENNA, 2000 IAEA-TECDOC-1168 ISSN 1011–4289 © IAEA, 2000 Printed by the IAEA in Austria December 2000 FOREWORD Fission product yields are required at several stages of the nuclear fuel cycle and are therefore included in all large international data files for reactor calculations and related applications. Such files are maintained and disseminated by the Nuclear Data Section of the IAEA as a member of an international data centres network. Users of these data are from the fields of reactor design and operation, waste management and nuclear materials safeguards, all of which are essential parts of the IAEA programme. In the 1980s, the number of measured fission yields increased so drastically that the manpower available for evaluating them to meet specific user needs was insufficient. To cope with this task, it was concluded in several meetings on fission product nuclear data, some of them convened by the IAEA, that international co-operation was required, and an IAEA co-ordinated research project (CRP) was recommended. This recommendation was endorsed by the International Nuclear Data Committee, an advisory body for the nuclear data programme of the IAEA. As a consequence, the CRP on the Compilation and Evaluation of Fission Yield Nuclear Data was initiated in 1991, after its scope, objectives and tasks had been defined by a preparatory meeting. -
Heavy Element Nucleosynthesis
Heavy Element Nucleosynthesis A summary of the nucleosynthesis of light elements is as follows 4He Hydrogen burning 3He Incomplete PP chain (H burning) 2H, Li, Be, B Non-thermal processes (spallation) 14N, 13C, 15N, 17O CNO processing 12C, 16O Helium burning 18O, 22Ne α captures on 14N (He burning) 20Ne, Na, Mg, Al, 28Si Partly from carbon burning Mg, Al, Si, P, S Partly from oxygen burning Ar, Ca, Ti, Cr, Fe, Ni Partly from silicon burning Isotopes heavier than iron (as well as some intermediate weight iso- topes) are made through neutron captures. Recall that the prob- ability for a non-resonant reaction contained two components: an exponential reflective of the quantum tunneling needed to overcome electrostatic repulsion, and an inverse energy dependence arising from the de Broglie wavelength of the particles. For neutron cap- tures, there is no electrostatic repulsion, and, in complex nuclei, virtually all particle encounters involve resonances. As a result, neutron capture cross-sections are large, and are very nearly inde- pendent of energy. To appreciate how heavy elements can be built up, we must first consider the lifetime of an isotope against neutron capture. If the cross-section for neutron capture is independent of energy, then the lifetime of the species will be ( )1=2 1 1 1 µn τn = ≈ = Nnhσvi NnhσivT Nnhσi 2kT For a typical neutron cross-section of hσi ∼ 10−25 cm2 and a tem- 8 9 perature of 5 × 10 K, τn ∼ 10 =Nn years. Next consider the stability of a neutron rich isotope. If the ratio of of neutrons to protons in an atomic nucleus becomes too large, the nucleus becomes unstable to beta-decay, and a neutron is changed into a proton via − (Z; A+1) −! (Z+1;A+1) + e +ν ¯e (27:1) The timescale for this decay is typically on the order of hours, or ∼ 10−3 years (with a factor of ∼ 103 scatter). -
A Guide to Naturally Occurring Radioactive Materials (NORM)
ABOUT NORM SOME NORM NUCLIDES OF SPECIAL INTEREST A Guide to Naturally There are three types of NORM: Occurring Radioactive • Cosmogenic – NORM produced by cosmic rays interacting with the Earth’s Materials (NORM) Beryllium 7 atmosphere; the most important Developed by the 3 7 14 examples are H (tritium), Be, and C. 7Be is being continuously formed in the DHS Secondary Reachback Program • Primordial – Sufficiently long-lived atmosphere by cosmic rays. Jet engines can March 2010 NORM for some to have survived from accumulate enough 7Be to set off before the formation of the Earth; there radiological alarms when being cleaned. are 20 primordial NORM nuclides with As defined by the International Atomic the most important being 40K, 232Th, Energy Agency (IAEA), Naturally 235U, and 238U. Polonium 210 Occurring Radioactive Materials • Daughters – When 232Th, 235U and 238U In the 238U decay chain 210Po is a distant (NORM) include all natural radioactive decay 42 different radioactive nuclides daughter of 226Ra. 210Po gained notoriety in materials where human activities have are formed (see below) with the most the 1960s as a radioactive trace component increased the potential for exposure in important being 222Rn, 226Ra, 228Ra and in cigarette smoke. Heavy use of phosphate comparison with the unaltered natural 228 Ac. fertilizers (which have trace amounts of out here. fold Next situation. If processing has increased 226Ra) can triple the amount of 210Po found the concentrations of radionuclides in a When 232Th, 235U and 238U decay a in tobacco. material then it is Technologically radioactive “daughter” nuclide is formed, Enhanced NORM (TE-NORM). -
Spallation Neutron Sources for Science and Technology
Proceedings of the 8th Conference on Nuclear and Particle Physics, 20-24 Nov. 2011, Hurghada, Egypt SPALLATION NEUTRON SOURCES FOR SCIENCE AND TECHNOLOGY M.N.H. Comsan Nuclear Research Center, Atomic Energy Authority, Egypt Spallation Neutron Facilities Increasing interest has been noticed in spallation neutron sources (SNS) during the past 20 years. The system includes high current proton accelerator in the GeV region and spallation heavy metal target in the Hg-Bi region. Among high flux currently operating SNSs are: ISIS in UK (1985), SINQ in Switzerland (1996), JSNS in Japan (2008), and SNS in USA (2010). Under construction is the European spallation source (ESS) in Sweden (to be operational in 2020). The intense neutron beams provided by SNSs have the advantage of being of non-reactor origin, are of continuous (SINQ) or pulsed nature. Combined with state-of-the-art neutron instrumentation, they have a diverse potential for both scientific research and diverse applications. Why Neutrons? Neutrons have wavelengths comparable to interatomic spacings (1-5 Å) Neutrons have energies comparable to structural and magnetic excitations (1-100 meV) Neutrons are deeply penetrating (bulk samples can be studied) Neutrons are scattered with a strength that varies from element to element (and isotope to isotope) Neutrons have a magnetic moment (study of magnetic materials) Neutrons interact only weakly with matter (theory is easy) Neutron scattering is therefore an ideal probe of magnetic and atomic structures and excitations Neutron Producing Reactions -
Production and Properties Towards the Island of Stability
This is an electronic reprint of the original article. This reprint may differ from the original in pagination and typographic detail. Author(s): Leino, Matti Title: Production and properties towards the island of stability Year: 2016 Version: Please cite the original version: Leino, M. (2016). Production and properties towards the island of stability. In D. Rudolph (Ed.), Nobel Symposium NS 160 - Chemistry and Physics of Heavy and Superheavy Elements (Article 01002). EDP Sciences. EPJ Web of Conferences, 131. https://doi.org/10.1051/epjconf/201613101002 All material supplied via JYX is protected by copyright and other intellectual property rights, and duplication or sale of all or part of any of the repository collections is not permitted, except that material may be duplicated by you for your research use or educational purposes in electronic or print form. You must obtain permission for any other use. Electronic or print copies may not be offered, whether for sale or otherwise to anyone who is not an authorised user. EPJ Web of Conferences 131, 01002 (2016) DOI: 10.1051/epjconf/201613101002 Nobel Symposium NS160 – Chemistry and Physics of Heavy and Superheavy Elements Production and properties towards the island of stability Matti Leino Department of Physics, University of Jyväskylä, PO Box 35, 40014 University of Jyväskylä, Finland Abstract. The structure of the nuclei of the heaviest elements is discussed with emphasis on single-particle properties as determined by decay and in- beam spectroscopy. The basic features of production of these nuclei using fusion evaporation reactions will also be discussed. 1. Introduction In this short review, some examples of nuclear structure physics and experimental methods relevant for the study of the heaviest elements will be presented. -
The Discoverers of the Ruthenium Isotopes
•Platinum Metals Rev., 2011, 55, (4), 251–262• The Discoverers of the Ruthenium Isotopes Updated information on the discoveries of the six platinum group metals to 2010 http://dx.doi.org/10.1595/147106711X592448 http://www.platinummetalsreview.com/ By John W. Arblaster This review looks at the discovery and the discoverers Wombourne, West Midlands, UK of the thirty-eight known ruthenium isotopes with mass numbers from 87 to 124 found between 1931 and 2010. Email: [email protected] This is the sixth and fi nal review on the circumstances surrounding the discoveries of the isotopes of the six platinum group elements. The fi rst review on platinum isotopes was published in this Journal in October 2000 (1), the second on iridium isotopes in October 2003 (2), the third on osmium isotopes in October 2004 (3), the fourth on palladium isotopes in April 2006 (4) and the fi fth on rhodium isotopes in April 2011 (5). An update on the new isotopes of palladium, osmium, iridium and platinum discovered since the previous reviews in this series is also included. Naturally Occurring Ruthenium Of the thirty-eight known isotopes of ruthenium, seven occur naturally with the authorised isotopic abun- dances (6) shown in Table I. The isotopes were fi rst detected in 1931 by Aston (7, 8) using a mass spectrograph at the Cavendish Laboratory, Cambridge University, UK. Because of diffi cult experimental conditions due to the use of poor quality samples, Aston actually only detected six of the isotopes and obtained very approximate Table I The Naturally Occurring Isotopes of Ruthenium Mass number Isotopic Abundance, % 96Ru 5.54 98Ru 1.87 99Ru 12.76 100Ru 12.60 101Ru 17.06 102Ru 31.55 104Ru 18.62 251 © 2011 Johnson Matthey http://dx.doi.org/10.1595/147106711X592448 •Platinum Metals Rev., 2011, 55, (4)• percentage abundances. -
Fusion and Spallation Irradiation Conditions Steven J
Fusion and Spallation Irradiation Conditions Steven J. Zinkle Metals and Ceramics Division Oak Ridge National Laboratory, Oak Ridge, TN International Workshop on Advanced Computational Science: Application to Fusion and Generation-IV Fission Reactors Washington DC, March 31-April 2, 2004 Comparison of fission and fusion (ITER) neutron spectra Stoller & Greenwood, JNM 271-272 (1999) 57 • Main difference between fission and DT fusion neutron spectra is the presence of significant flux above ~4 MeV for fusion –High energy neutrons typically cause enhanced production of numerous transmutation products including H and He –The Primary Knock-on Atom (PKA) spectra are similar for fission and fusion at low energies; fusion contains significant high-energy PKAs (>100 keV) Displacement Damage Mechanisms are being investigated with Molecular Dynamics Simulations Damage efficiency saturates when subcascade formation occurs Avg. Avg. fission fusion Molecular dynamics modeling of displacement cascades up to 50 keV PKA 200 keV and low-dose experimental tests (microstructure, tensile (ave. fusion) properties, etc.) indicates that defect production from fusion and fission neutron collisions are similar 10 keV PKA => Defect source term is similar for fission and fusion conditions (ave. fission) Peak damage state in iron cascades at 100K 5 nm A critical unanswered question is the effect of higher transmutant H and He production in the fusion spectrum Radiation Damage can Produce Large Changes in Structural Materials • Radiation hardening and embrittlement -
1 Chapter 16 Stable and Radioactive Isotopes Jim Murray 5/7/01 Univ
Chapter 16 Stable and Radioactive Isotopes Jim Murray 5/7/01 Univ. Washington Each atomic element (defined by its number of protons) comes in different flavors, depending on the number of neutrons. Most elements in the periodic table exist in more than one isotope. Some are stable and some are radioactive. Scientists have tallied more than 3600 isotopes, the majority are radioactive. The Isotopes Project at Lawrence Berkeley National Lab in California has a web site (http://ie.lbl.gov/toi.htm) that gives detailed information about all the isotopes. Stable and radioactive isotopes are the most useful class of tracers available to geochemists. In almost all cases the distributions of these isotopes have been used to study oceanographic processes controlling the distributions of the elements. Radioactive isotopes are especially useful because they provide a way to put time into geochemical models. The chemical characteristic of an element is determined by the number of protons in its nucleus. Different elements can have different numbers of neutrons and thus atomic weights (the sum of protons plus neutrons). The atomic weight is equal to the sum of protons plus neutrons. The chart of the nuclides (protons versus neutrons) for elements 1 (Hydrogen) through 12 (Magnesium) is shown in Fig. 16-1. The Valley of Stability represents nuclides stable relative to decay. Examples: Atomic Protons Neutrons % Abundance Weight (Atomic Number) Carbon 12C 6P 6N 98.89 13C 6P 7N 1.11 14C 6P 8N 10-10 Oxygen 16O 8P 8N 99.76 17O 8P 9N 0.024 18O 8P 10N 0.20 Several light elements such as H, C, N, O, and S have more than one stable isotope form, which show variable abundances in natural samples. -
Quest for Superheavy Nuclei Began in the 1940S with the Syn Time It Takes for Half of the Sample to Decay
FEATURES Quest for superheavy nuclei 2 P.H. Heenen l and W Nazarewicz -4 IService de Physique Nucleaire Theorique, U.L.B.-C.P.229, B-1050 Brussels, Belgium 2Department ofPhysics, University ofTennessee, Knoxville, Tennessee 37996 3Physics Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 4Institute ofTheoretical Physics, University ofWarsaw, ul. Ho\.za 69, PL-OO-681 Warsaw, Poland he discovery of new superheavy nuclei has brought much The superheavy elements mark the limit of nuclear mass and T excitement to the atomic and nuclear physics communities. charge; they inhabit the upper right corner of the nuclear land Hopes of finding regions of long-lived superheavy nuclei, pre scape, but the borderlines of their territory are unknown. The dicted in the early 1960s, have reemerged. Why is this search so stability ofthe superheavy elements has been a longstanding fun important and what newknowledge can it bring? damental question in nuclear science. How can they survive the Not every combination ofneutrons and protons makes a sta huge electrostatic repulsion? What are their properties? How ble nucleus. Our Earth is home to 81 stable elements, including large is the region of superheavy elements? We do not know yet slightly fewer than 300 stable nuclei. Other nuclei found in all the answers to these questions. This short article presents the nature, although bound to the emission ofprotons and neutrons, current status ofresearch in this field. are radioactive. That is, they eventually capture or emit electrons and positrons, alpha particles, or undergo spontaneous fission. Historical Background Each unstable isotope is characterized by its half-life (T1/2) - the The quest for superheavy nuclei began in the 1940s with the syn time it takes for half of the sample to decay. -
Nuclear Binding & Stability
Nuclear Binding & Stability Stanley Yen TRIUMF UNITS: ENERGY Energy measured in electron-Volts (eV) 1 volt battery boosts energy of electrons by 1 eV 1 volt -19 battery 1 e-Volt = 1.6x10 Joule 1 MeV = 106 eV 1 GeV = 109 eV Recall that atomic and molecular energies ~ eV nuclear energies ~ MeV UNITS: MASS From E = mc2 m = E / c2 so we measure masses in MeV/c2 1 MeV/c2 = 1.7827 x 10 -30 kg Frequently, we get lazy and just set c=1, so that we measure masses in MeV e.g. mass of electron = 0.511 MeV mass of proton = 938.272 MeV mass of neutron=939.565 MeV Also widely used unit of mass is the atomic mass unit (amu or u) defined so that Mass(12C atom) = 12 u -27 1 u = 931.494 MeV = 1.6605 x 10 kg nucleon = proton or neutron “nuclide” means one particular nuclear species, e.g. 7Li and 56Fe are two different nuclides There are 4 fundamental types of forces in the universe. 1. Gravity – very weak, negligible for nuclei except for neutron stars 2. Electromagnetic forces – Coulomb repulsion tends to force protons apart ) 3. Strong nuclear force – binds nuclei together; short-ranged 4. Weak nuclear force – causes nuclear beta decay, almost negligible compared to the strong and EM forces. How tightly a nucleus is bound together is mostly an interplay between the attractive strong force and the repulsive electromagnetic force. Let's make a scatterplot of all the stable nuclei, with proton number Z versus neutron number N.