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Glaciological Studies at Siple Station (Antarctica): Potential Ice-Core Paleoclimatic Record

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Glaciological Studies at Siple Station (Antarctica): Potential Ice-Core Paleoclimatic Record Journal of Glaciology, Vol. 37, No. 125, 1991 Glaciological studies at Siple Station (Antarctica): potential ice-core paleoclimatic record E. MOSLEY-THOMPSON, J. DAI, L. G. THOMPSON, Byrd Polar Research Center, The Ohio State University, Columbus, Ohio 43210-1308, U.S.A. P. M . GROOTES, Q_uat~rnary Isotope Laboratory, University of Washington, Seattle, Washington 98195, U.S.A. JAMES K. ARBOGAST AND j. F. PASKIEVITCH Byrd Polar Research Center, The Ohio State University, Columbus, Ohio 43210-1308, U.S.A. ABSTRACT. The quality and utility of the records of oxygen-isotopic abundances, dust concentrations and anionic concentrations preserved in the ice at Siple Station (75°55' S, 84°15' W) are assessed from four shallow (20m) cores. The combination of high accumu lation (0.56 m a- 1 w.e. ) and low mean annual temperature (-24°C) preserves the prominent seasonal variations in 818 0 which are very spatially coherent. Sulfate concentrations vary seasonall y and, in conjunction with 818 0, will allow accurate dating of deeper cores from Siple Station. The concentrations of insoluble dust are the lowest measured in Antarctica, making Siple Station an excellent location to examine large increases in atmospheric tubidity. The seasonal variations and annual fluxes of the anions are examined for the last two decades (AD 1966-85) with regard to probable sources. An unusually high sulfate flux in 1976 may reflect the February 1975 eruption of Mount Ngauruhoe, New Zealand. No annual signal in nitrate concentration is confirmed and no unusually high nitrate fluxes support the suggestion of nitrate production by large solar flares. However, nitrate flux is higher for the latter half of the 1970s and early 1980s, possibly reflecting the recent loss of stratospheric ozone. Finally, comparison of the 8180 record with available surface-temperature data (AD 195 7- 85) reveals that multi-year trends along the western coast of the Antarctic Peninsula are recorded at Siple. More importantly, comparison with areally weighted temperature reconstructions suggests that the 8180 record may reflect larger-scale, persistent trends in the high southern latitudes. The strong spatial coherence of the preserved records, the potential for accurate dating, and possible relevance to larger­ scale processes make Siple Station an excellent site for paleoenvironmental reconstruction from ice cores. INTRODUCTION chemical records anticipated from a 302 m core for reconstruction of paleoenvironmental conditions in the Current emphasis upon the comprehensive investigation of high southern latitudes. the global environmental system (National Research In support of deeper cores (302 and 132 m) drilled at Council, 1986, p. 1-6, 1988) has drawn attention to ice Siple Station, Antarctica (75°55'S, 84°15'W, 1054m sheets and ice caps which continuously record and a .s.I.; Fig. 1), during the 1985-86 austral summer preserve the physical and chemical character of the (Mosley-Thompson and others, 1986), eight additional atmosphere. The extraction of an environmental history shallow cores (20 m) were collected and samples were from an ice core requires evaluation of both the temporal taken from three pits. The 20 m core records encompass 20 quality and spatial variability of the record which limits its years (AD 1966-85) and in combination with pit studies 2 utility as an environmental proxy. The gases trapped in ice represent a sampling area of several km . These have been bubbles at Siple Station have provided a unique, high­ used to examine the potential for accurate dating, to resolution record of atmospheric chemistry (Stauffer and obtain basic glaciological information such as annual Oeschger, 1985; Friedli and others, 1986). Here we accumulation rate and density variations with depth, to explore the potential of the 8180, particulate, and examine the spatial reproducibility of the preserved 11 Journal ef Glaciology records, and to assess their relevance to larger-scale processes. Soluble impurities in Antarctic snow and ice provide unique information about both present and past atmos­ pheric chemical composition. Siple Station, located near the base of the Antarctic Peninsula (Fig. I), offers the opportunity to study precipitation chemistry at a site intermediate between the coastal areas, where sea-salt aerosol has a strong infl uence and the interior where secondary aerosol tends to be dominant. For the purposes of this paper, the Antarctic seasons are loosely defined as : summer, December-February; winter, March-September; and spring, October-November. SAMPLE ACQUISITION, PREPARATION AND ANALYSES Fig. 1. Antarctic sites for results cited in the text and in Table 1. Drilling and pit sampling were conducted 2 km upwind of Table 1. Chloride, nitrate and sulfate in Antarctic snow Location (Fig . 1) Years Number of er SO/- Annual (Reference) samples accumulation average in µeq /l mm w.e Siple 1965-85 284 2.48 0.4·5 0.77 540 (this work) Siple -2.0 -0.5 -0.7 -400 (Herron, 1982) Gomez Nunatak 1942-80 612 2.3 -0.4 -0.8 880 (Mulvaney and Peel, 1988) Dolleman Island 1973-85 143 11.8 -0.4 -5.0 51·0 (Mulvaney and Peel, 1988) Jam es Ross Island 1964-78 312 > 10.0 0.4 1.8 490 (Aristarain and others, 1982) South Pole 1959-69 100 1.25 1.44 1. 50 85 (Legrand and Delmas, 1984) Dome C 1960-78 -0.23 -1.9 34 (Delmas and others, 1982) Site D57 pre-1900 0.7 0.5 30 (Zanolini and others, 1985) Ross Ice Shelf (Windless Bight) 1971-86 90 -2.0 200 (Zeller and others, 1986) - Estimated from diagrams. - Information not available. the station to reduce the potential of contamination. All improved over the method previously reported by cores and pit samples were stored below - 20°C until just Legrand and others ( 1984) which has been recently prior to laboratory analysis. Samples were initially upgraded by Saigne and others (1987). The use of a prepared in a cold working room (-15°C) where a band relatively large injection loop (0.64 ml ) eliminated the saw was used to cut the samples directly from the core. A need for a concentrator column (Arbogast, 1987), while minimum of20mm ofmaterial was removed from all sides preserving the desired detection limits ( c. ~ 1 ppb for er, to obtain fresh samples of the desired size which were N03, and So/-). Working standards were prepared daily placed in pre-cleaned containers. With the exception of from stock solutions and procedural blanks were included the 8 180 samples, further cleaning, melting and analysis in each analytical session for every step in sample were conducted in a Class-100 clean-room laboratory. handling, beginning with the cutting by band saw. Only Millipore Milli-Q ultra-pure, deionized, filtered water minor amounts ( < 5 ppb) of er were observed in a few was used for cleaning of all samples and containers and for cases. The time required for each analysis (injection) is preparing elu ants and standards. The concentration of approximately 10 min. The ionic concentrations are insoluble microparticles with diameters ~0.63µm mr1 comparable to previously published values (Table 1), (MPG) were measured by a Model TA II Coulter suggesting that the contamination control procedures counter, using a procedure described elsewhere (Thomp­ employed are effective. son, 1977 ). The electrical conductivity (EC) of liquid samples was measured using a Beckman RC-20 conduc­ 18 tivity bridge. The 8 0 measurements were made with a SHALLOW-CORE RESULTS: (AD 1966-85) stable-isotope mass spectrometer at the Quaternary Isotope Laboratory of the University of Washington. Oxygen-isotope ratios (8 180) The anion concentrations were determined with a Dionex Model 20 1Oi ion chromatograph equipped with an Figure 2 illustrates () 180 for three 20 m cores (cores 2, 6 AS4A anion separator column and a micro-membrane and 8) and the upper 18 m of core A which was drilled in a suppressor column. Carbonate/bicarbonate (0.00 12 / 2 m trench. The depth in firn was converted to water­ 1 0.00038 mol r ) eluant was used, a long with equivalen t depth using the depth-density relationship 1 0.1mol1" H 2S04 as regenerant for the suppressor. derived from density measurements in pits and on cores. Analytical precision and sensitivity were significantly Figure 2 clearly demonstrates that 8 180 exhibits a Siple Station, Antarctica, 1985 16 O Oto 1001 Core 2 Core 6 Core A -3 7 - 33 -29 -2 5 -37 - 33 -29 - 25 - 37 -33 - 29 -25 0.0 _ L_ L.J ..._ L .:-Jr:::- ~ -l-~~~-~_J=-L J ''i~: , .... -- '1900 / R5 2 .5 ~ c Q) ro > =i O' 5.0 Q) 0 N I E .r: ~a. 75-] Q) 0 10 .0 66 65 1964 Average= -29.3 Average=-29.5 Average=-29.6 Average=-29.4 Fig . 2. Oxygen-isotope (8 180) ratios for three 20 cm cores (2, 6 and 8) and the upper lBm of core A illustrate the spatial reproducibility of the record. The firn depths were converted to water-equivalent depths using a depth-density relationship derived empirically from pit- and core-density data. 13 Journal of Glaciology Table 2. 818 0 results from four 20 m cores (AD 1966-85). Pearson correlation coefficients and significance levels (A) Annual averages Core 2 6 8 A 2 0.644 0.734 0.403 (99 .0) (99 .0) (90 .0) 6 0.742 0.432 (99.9) (93.0) 8 0.537 (95 .0) ( B) Winter averages Core 2 6 8 A 2 0.594 0.870 0.552 (99 .0) (99 .9) (95.0) 6 0.567 0.747 (99.0) (99 .0) 8 0.529 (95.0) (C) Summer averages Core 2 6 8 A 2 0.600 0.680 NS (99 .0) (99 .0) 6 0.467 NS (95 .0) 8 NS NS: Not significant at any acceptable level ( < 90% ).
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