Qualitative Nuclear Mechanics from a NLHV Design
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Hetc-3Step Calculations of Proton Induced Nuclide Production Cross Sections at Incident Energies Between 20 Mev and 5 Gev
JAERI-Research 96-040 JAERI-Research—96-040 JP9609132 JP9609132 HETC-3STEP CALCULATIONS OF PROTON INDUCED NUCLIDE PRODUCTION CROSS SECTIONS AT INCIDENT ENERGIES BETWEEN 20 MEV AND 5 GEV August 1996 Hiroshi TAKADA, Nobuaki YOSHIZAWA* and Kenji ISHIBASHI* Japan Atomic Energy Research Institute 2 G 1 0 1 (T319-11 l This report is issued irregularly. Inquiries about availability of the reports should be addressed to Research Information Division, Department of Intellectual Resources, Japan Atomic Energy Research Institute, Tokai-mura, Naka-gun, Ibaraki-ken, 319-11, Japan. © Japan Atomic Energy Research Institute, 1996 JAERI-Research 96-040 HETC-3STEP Calculations of Proton Induced Nuclide Production Cross Sections at Incident Energies between 20 MeV and 5 GeV Hiroshi TAKADA, Nobuaki YOSHIZAWA* and Kenji ISHIBASHP* Department of Reactor Engineering Tokai Research Establishment Japan Atomic Energy Research Institute Tokai-mura, Naka-gun, Ibaraki-ken (Received July 1, 1996) For the OECD/NEA code intercomparison, nuclide production cross sections of l60, 27A1, nalFe, 59Co, natZr and 197Au for the proton incidence with energies of 20 MeV to 5 GeV are calculated with the HETC-3STEP code based on the intranuclear cascade evaporation model including the preequilibrium and high energy fission processes. In the code, the level density parameter derived by Ignatyuk, the atomic mass table of Audi and Wapstra and the mass formula derived by Tachibana et al. are newly employed in the evaporation calculation part. The calculated results are compared with the experimental ones. It is confirmed that HETC-3STEP reproduces the production of the nuclides having the mass number close to that of the target nucleus with an accuracy of a factor of two to three at incident proton energies above 100 MeV for natZr and 197Au. -
1 11. Nuclear Chemistry 11.1 Stable and Unstable Nuclides Very Large
11. Nuclear Chemistry Chemical reactions occur as a result of loosing/gaining and sharing electrons in the valance shell which is far away from the atomic nucleus as we described in previous chapters in chemical bonding. In chemical reactions identity of the elements (atomic) and the makeup of the nuclei (mass due to protons and neutrons) is preserved which is reflected in the Law of Conservation of mass. This idea of atomic nucleus is always stable was shattered as Henri Becquerel discovered radioactivity in uranium compound where uranium nuclei changes or undergo nuclear reactions where nuclei of an element is transformed into nuclei of different element(s) while emitting ionization radiation. Marie Curie also began a study of radioactivity in a different form of uranium ore called pitchblende and she discovered the existence of two more highly radioactive new elements radium and polonium formed as the products during the decay of unstable nuclide of uranium-235. Curie measure that the radiation emanated was proportional to the amount (moles or number of nuclides) of radioactive element present, and she proposed that radiation was a property nucleus of an unstable atom. The area of chemistry that focuses on the nuclear changes is called nuclear chemistry. What changes in a nuclide result from the loss of each of the following? a) An alpha particle. b) A gamma ray. c) An electron. d) A neutron. e) A proton. Answer: a), c), d), e) 11.1 Stable and Unstable Nuclides There are stable and unstable radioactive nuclides. Unstable nuclides emit subatomic particles, with alpha −α, beta −β, gamma −γ, proton-p, neutrons-n being the most common. -
An Octad for Darmstadtium and Excitement for Copernicium
SYNOPSIS An Octad for Darmstadtium and Excitement for Copernicium The discovery that copernicium can decay into a new isotope of darmstadtium and the observation of a previously unseen excited state of copernicium provide clues to the location of the “island of stability.” By Katherine Wright holy grail of nuclear physics is to understand the stability uncover its position. of the periodic table’s heaviest elements. The problem Ais, these elements only exist in the lab and are hard to The team made their discoveries while studying the decay of make. In an experiment at the GSI Helmholtz Center for Heavy isotopes of flerovium, which they created by hitting a plutonium Ion Research in Germany, researchers have now observed a target with calcium ions. In their experiments, flerovium-288 previously unseen isotope of the heavy element darmstadtium (Z = 114, N = 174) decayed first into copernicium-284 and measured the decay of an excited state of an isotope of (Z = 112, N = 172) and then into darmstadtium-280 (Z = 110, another heavy element, copernicium [1]. The results could N = 170), a previously unseen isotope. They also measured an provide “anchor points” for theories that predict the stability of excited state of copernicium-282, another isotope of these heavy elements, says Anton Såmark-Roth, of Lund copernicium. Copernicium-282 is interesting because it University in Sweden, who helped conduct the experiments. contains an even number of protons and neutrons, and researchers had not previously measured an excited state of a A nuclide’s stability depends on how many protons (Z) and superheavy even-even nucleus, Såmark-Roth says. -
Compilation and Evaluation of Fission Yield Nuclear Data Iaea, Vienna, 2000 Iaea-Tecdoc-1168 Issn 1011–4289
IAEA-TECDOC-1168 Compilation and evaluation of fission yield nuclear data Final report of a co-ordinated research project 1991–1996 December 2000 The originating Section of this publication in the IAEA was: Nuclear Data Section International Atomic Energy Agency Wagramer Strasse 5 P.O. Box 100 A-1400 Vienna, Austria COMPILATION AND EVALUATION OF FISSION YIELD NUCLEAR DATA IAEA, VIENNA, 2000 IAEA-TECDOC-1168 ISSN 1011–4289 © IAEA, 2000 Printed by the IAEA in Austria December 2000 FOREWORD Fission product yields are required at several stages of the nuclear fuel cycle and are therefore included in all large international data files for reactor calculations and related applications. Such files are maintained and disseminated by the Nuclear Data Section of the IAEA as a member of an international data centres network. Users of these data are from the fields of reactor design and operation, waste management and nuclear materials safeguards, all of which are essential parts of the IAEA programme. In the 1980s, the number of measured fission yields increased so drastically that the manpower available for evaluating them to meet specific user needs was insufficient. To cope with this task, it was concluded in several meetings on fission product nuclear data, some of them convened by the IAEA, that international co-operation was required, and an IAEA co-ordinated research project (CRP) was recommended. This recommendation was endorsed by the International Nuclear Data Committee, an advisory body for the nuclear data programme of the IAEA. As a consequence, the CRP on the Compilation and Evaluation of Fission Yield Nuclear Data was initiated in 1991, after its scope, objectives and tasks had been defined by a preparatory meeting. -
Heavy Element Nucleosynthesis
Heavy Element Nucleosynthesis A summary of the nucleosynthesis of light elements is as follows 4He Hydrogen burning 3He Incomplete PP chain (H burning) 2H, Li, Be, B Non-thermal processes (spallation) 14N, 13C, 15N, 17O CNO processing 12C, 16O Helium burning 18O, 22Ne α captures on 14N (He burning) 20Ne, Na, Mg, Al, 28Si Partly from carbon burning Mg, Al, Si, P, S Partly from oxygen burning Ar, Ca, Ti, Cr, Fe, Ni Partly from silicon burning Isotopes heavier than iron (as well as some intermediate weight iso- topes) are made through neutron captures. Recall that the prob- ability for a non-resonant reaction contained two components: an exponential reflective of the quantum tunneling needed to overcome electrostatic repulsion, and an inverse energy dependence arising from the de Broglie wavelength of the particles. For neutron cap- tures, there is no electrostatic repulsion, and, in complex nuclei, virtually all particle encounters involve resonances. As a result, neutron capture cross-sections are large, and are very nearly inde- pendent of energy. To appreciate how heavy elements can be built up, we must first consider the lifetime of an isotope against neutron capture. If the cross-section for neutron capture is independent of energy, then the lifetime of the species will be ( )1=2 1 1 1 µn τn = ≈ = Nnhσvi NnhσivT Nnhσi 2kT For a typical neutron cross-section of hσi ∼ 10−25 cm2 and a tem- 8 9 perature of 5 × 10 K, τn ∼ 10 =Nn years. Next consider the stability of a neutron rich isotope. If the ratio of of neutrons to protons in an atomic nucleus becomes too large, the nucleus becomes unstable to beta-decay, and a neutron is changed into a proton via − (Z; A+1) −! (Z+1;A+1) + e +ν ¯e (27:1) The timescale for this decay is typically on the order of hours, or ∼ 10−3 years (with a factor of ∼ 103 scatter). -
A Guide to Naturally Occurring Radioactive Materials (NORM)
ABOUT NORM SOME NORM NUCLIDES OF SPECIAL INTEREST A Guide to Naturally There are three types of NORM: Occurring Radioactive • Cosmogenic – NORM produced by cosmic rays interacting with the Earth’s Materials (NORM) Beryllium 7 atmosphere; the most important Developed by the 3 7 14 examples are H (tritium), Be, and C. 7Be is being continuously formed in the DHS Secondary Reachback Program • Primordial – Sufficiently long-lived atmosphere by cosmic rays. Jet engines can March 2010 NORM for some to have survived from accumulate enough 7Be to set off before the formation of the Earth; there radiological alarms when being cleaned. are 20 primordial NORM nuclides with As defined by the International Atomic the most important being 40K, 232Th, Energy Agency (IAEA), Naturally 235U, and 238U. Polonium 210 Occurring Radioactive Materials • Daughters – When 232Th, 235U and 238U In the 238U decay chain 210Po is a distant (NORM) include all natural radioactive decay 42 different radioactive nuclides daughter of 226Ra. 210Po gained notoriety in materials where human activities have are formed (see below) with the most the 1960s as a radioactive trace component increased the potential for exposure in important being 222Rn, 226Ra, 228Ra and in cigarette smoke. Heavy use of phosphate comparison with the unaltered natural 228 Ac. fertilizers (which have trace amounts of out here. fold Next situation. If processing has increased 226Ra) can triple the amount of 210Po found the concentrations of radionuclides in a When 232Th, 235U and 238U decay a in tobacco. material then it is Technologically radioactive “daughter” nuclide is formed, Enhanced NORM (TE-NORM). -
22.101 Applied Nuclear Physics (Fall 2006) Problem Set No. 1 Due: Sept
22.101 Applied Nuclear Physics (Fall 2006) Problem Set No. 1 Due: Sept. 13, 2006 Problem 1 Before getting into the concepts of nuclear physics, every student should have some feeling for the numerical values of properties of nuclear radiations, such as energy and speed, wavelength, and frequency, etc. This involves some back of the envelope calculations using appropriate universal constants. (i) A thermal neutron in a nuclear reactor is a neutron with kinetic energy equal to kBT, where kB is the Boltzmann’s constant and T is the temperature of the reactor. Explain briefly the physical basis of this statement. Taking T to be the room temperature, 20C, calculate the energy of the thermal neutron (in units of ev), and then find its speed v (in cm/sec), the de Broglie wavelength λ (in A) and circular frequency ω (radian/sec). Compare these values with the energy, speed, and interatomic distance of atoms that make up the materials in the reactor. What is the point of comparing the neutron wavelength with typical atomic separations in a solid? (ii) Consider a 2 Kev x-ray, calculate the frequency and wavelength of this photon. What would be the point of comparing the x-ray wavelength with that of the thermal neutron? For an electron with wavelength equal to that of the thermal neutron, what energy would it have? 2 2 (iii) The classical radius of the electron, defined as e / mec , with e being the electron charge, me the electron rest mass, and c the speed of light, has the value of 2.818 x 10-13 cm. -
Production and Properties Towards the Island of Stability
This is an electronic reprint of the original article. This reprint may differ from the original in pagination and typographic detail. Author(s): Leino, Matti Title: Production and properties towards the island of stability Year: 2016 Version: Please cite the original version: Leino, M. (2016). Production and properties towards the island of stability. In D. Rudolph (Ed.), Nobel Symposium NS 160 - Chemistry and Physics of Heavy and Superheavy Elements (Article 01002). EDP Sciences. EPJ Web of Conferences, 131. https://doi.org/10.1051/epjconf/201613101002 All material supplied via JYX is protected by copyright and other intellectual property rights, and duplication or sale of all or part of any of the repository collections is not permitted, except that material may be duplicated by you for your research use or educational purposes in electronic or print form. You must obtain permission for any other use. Electronic or print copies may not be offered, whether for sale or otherwise to anyone who is not an authorised user. EPJ Web of Conferences 131, 01002 (2016) DOI: 10.1051/epjconf/201613101002 Nobel Symposium NS160 – Chemistry and Physics of Heavy and Superheavy Elements Production and properties towards the island of stability Matti Leino Department of Physics, University of Jyväskylä, PO Box 35, 40014 University of Jyväskylä, Finland Abstract. The structure of the nuclei of the heaviest elements is discussed with emphasis on single-particle properties as determined by decay and in- beam spectroscopy. The basic features of production of these nuclei using fusion evaporation reactions will also be discussed. 1. Introduction In this short review, some examples of nuclear structure physics and experimental methods relevant for the study of the heaviest elements will be presented. -
The Discoverers of the Ruthenium Isotopes
•Platinum Metals Rev., 2011, 55, (4), 251–262• The Discoverers of the Ruthenium Isotopes Updated information on the discoveries of the six platinum group metals to 2010 http://dx.doi.org/10.1595/147106711X592448 http://www.platinummetalsreview.com/ By John W. Arblaster This review looks at the discovery and the discoverers Wombourne, West Midlands, UK of the thirty-eight known ruthenium isotopes with mass numbers from 87 to 124 found between 1931 and 2010. Email: [email protected] This is the sixth and fi nal review on the circumstances surrounding the discoveries of the isotopes of the six platinum group elements. The fi rst review on platinum isotopes was published in this Journal in October 2000 (1), the second on iridium isotopes in October 2003 (2), the third on osmium isotopes in October 2004 (3), the fourth on palladium isotopes in April 2006 (4) and the fi fth on rhodium isotopes in April 2011 (5). An update on the new isotopes of palladium, osmium, iridium and platinum discovered since the previous reviews in this series is also included. Naturally Occurring Ruthenium Of the thirty-eight known isotopes of ruthenium, seven occur naturally with the authorised isotopic abun- dances (6) shown in Table I. The isotopes were fi rst detected in 1931 by Aston (7, 8) using a mass spectrograph at the Cavendish Laboratory, Cambridge University, UK. Because of diffi cult experimental conditions due to the use of poor quality samples, Aston actually only detected six of the isotopes and obtained very approximate Table I The Naturally Occurring Isotopes of Ruthenium Mass number Isotopic Abundance, % 96Ru 5.54 98Ru 1.87 99Ru 12.76 100Ru 12.60 101Ru 17.06 102Ru 31.55 104Ru 18.62 251 © 2011 Johnson Matthey http://dx.doi.org/10.1595/147106711X592448 •Platinum Metals Rev., 2011, 55, (4)• percentage abundances. -
Problem Set 3 Solutions
22.01 Fall 2016, Problem Set 3 Solutions October 9, 2016 Complete all the assigned problems, and do make sure to show your intermediate work. 1 Activity and Half Lives 1. Given the half lives and modern-day abundances of the three natural isotopes of uranium, calculate the isotopic fractions of uranium when the Earth first formed 4.5 billion years ago. Today, uranium consists of 0.72% 235U, 99.2745% 238U, and 0.0055% 234U. However, it is clear that the half life of 234U (245,500 years) is so short compared to the lifetime of the Earth (4,500,000,000 years) that it would have all decayed away had there been some during the birth of the Earth. Therefore, we look a little closer, and find that 234U is an indirect decay product of 238U, by tracing it back from its parent nuclides on the KAERI table: α β− β− 238U −! 234T h −! 234P a −! 234U (1) Therefore we won’t consider there being any more 234U than would normally be in equi librium with the 238U around at the time. We set up the two remaining equations as follows: −t t ;235 −t t ;238 = 1=2 = 1=2 N235 = N0235 e N238 = N0238 e (2) Using the current isotopic abundances from above as N235 and N238 , the half lives from n 9 t 1 1 the KAERI Table of Nuclides t =2;235 = 703800000 y; t =2;238 = 4:468 · 10 y , and the lifetime of the earth in years (keeping everything in the same units), we arrive at the following expressions for N0235 and N0238 : N235 0:0072 N238 0:992745 N0235 =−t = 9 = 4:307N0238 =−t = 9 = 2:718 (3) =t1 ;235 −4:5·10 =7:038·108 =t1 ;238 −4:5·10 =4:468·109 e =2 e e =2 e Finally, taking the ratios of these two relative abundances gives us absolute abundances: 4:307 2:718 f235 = = 0:613 f238 = = 0:387 (4) 4:307 + 2:718 4:307 + 2:718 235U was 61.3% abundant, and 238U was 38.7% abundant. -
Background and Derivation of ANS-5.4 Standard Fission Product Release Model
NUREG/CR-7003 PNNL-18490 Background and Derivation of ANS-5.4 Standard Fission Product Release Model Office of Nuclear Regulatory Research AVAILABILITY OF REFERENCE MATERIALS IN NRC PUBLICATIONS NRC Reference Material Non-NRC Reference Material As of November 1999, you may electronically access Documents available from public and special technical NUREG-series publications and other NRC records at libraries include all open literature items, such as NRC’s Public Electronic Reading Room at books, journal articles, and transactions, Federal http://www.nrc.gov/reading-rm.html. Register notices, Federal and State legislation, and Publicly released records include, to name a few, congressional reports. Such documents as theses, NUREG-series publications; Federal Register notices; dissertations, foreign reports and translations, and applicant, licensee, and vendor documents and non-NRC conference proceedings may be purchased correspondence; NRC correspondence and internal from their sponsoring organization. memoranda; bulletins and information notices; inspection and investigative reports; licensee event reports; and Commission papers and their attachments. Copies of industry codes and standards used in a substantive manner in the NRC regulatory process are NRC publications in the NUREG series, NRC maintained at— regulations, and Title 10, Energy, in the Code of The NRC Technical Library Federal Regulations may also be purchased from one Two White Flint North of these two sources. 11545 Rockville Pike 1. The Superintendent of Documents Rockville, MD 20852–2738 U.S. Government Printing Office Mail Stop SSOP Washington, DC 20402–0001 These standards are available in the library for Internet: bookstore.gpo.gov reference use by the public. Codes and standards are Telephone: 202-512-1800 usually copyrighted and may be purchased from the Fax: 202-512-2250 originating organization or, if they are American 2. -
The Delimiting/Frontier Lines of the Constituents of Matter∗
The delimiting/frontier lines of the constituents of matter∗ Diógenes Galetti1 and Salomon S. Mizrahi2 1Instituto de Física Teórica, Universidade Estadual Paulista (UNESP), São Paulo, SP, Brasily 2Departamento de Física, CCET, Universidade Federal de São Carlos, São Carlos, SP, Brasilz (Dated: October 23, 2019) Abstract Looking at the chart of nuclides displayed at the URL of the International Atomic Energy Agency (IAEA) [1] – that contains all the known nuclides, the natural and those produced artificially in labs – one verifies the existence of two, not quite regular, delimiting lines between which dwell all the nuclides constituting matter. These lines are established by the highly unstable radionuclides located the most far away from those in the central locus, the valley of stability. Here, making use of the “old” semi-empirical mass formula for stable nuclides together with the energy-time uncertainty relation of quantum mechanics, by a simple calculation we show that the obtained frontier lines, for proton and neutron excesses, present an appreciable agreement with the delimiting lines. For the sake of presenting a somewhat comprehensive panorama of the matter in our Universe and their relation with the frontier lines, we narrate, in brief, what is currently known about the astrophysical nucleogenesis processes. Keywords: chart of nuclides, nucleogenesis, nuclide mass formula, valley/line of stability, energy-time un- certainty relation, nuclide delimiting/frontier lines, drip lines arXiv:1909.07223v2 [nucl-th] 22 Oct 2019 ∗ This manuscript is based on an article that was published in Brazilian portuguese language in the journal Revista Brasileira de Ensino de Física, 2018, 41, e20180160. http://dx.doi.org/10.1590/ 1806-9126-rbef-2018-0160.