arXiv:1006.5179v1 [cond-mat.stat-mech] 27 Jun 2010 ae a enetne oteFrigs ti already of is It Fermi two-component gas. neutral ultracold Fermi the an to that observed extended quantum been in has magnetism of exploration the recently, in condensate[5]. Very spinor observed ferromagnetic typical directly experiments, a In been condensate, have studied. been domains ever magnetic have the gas leading Theoretically, neutral Bose active, a -1 in magnetism. [8–10] becomes and of freedom [7] manifestation of the 4], traps[3, degree to optical in spin confined gases[3– are their quantum gases atomic of When magnetism 6]. the in interest dia- research and para- causes relativistic spin the intrinsic the magnetism[2]. upon that effects found important and pair- Daicic magnetized gases the for investigation. mechanics extensive statistical developed under been also free altogether. the paramagnetism stronger exhibits so times susceptibility, gas two diamagnetic the is than susceptibility paramagnetic field h eprtrso lcrn n osaea o s100 as low as atoms[11]. are ions cold and of of photoionization cold by far, The created So been atoms. has ultracold neutral from gases atoms[6]. between interactions pulsive ∗ te.FreetoswoeLande-factor whose each electrons with For compete other. Landau paramag- the Pauli and The netism diamagnetic diamagnetism)[1]. de- the Landau induces charge (the field part to magnetic para- in due Pauli freedom motion of (the gree orbital part the elec- paramagnetic while of two the magnetism), moment of in magnetic consists results spin gas trons The electron field, free parts. magnetic a independent In of magnetization physics. the matter condensed in studied orsodn uhr [email protected] author: Corresponding h td futaodaoshssiuae renewed stimulated has atoms ultracold of study The have gases Fermi relativistic of properties Magnetic utemr,i spsil oraiecagdquantum charged realize to possible is it Furthermore, ants feeto ae a enconsiderably been has gases electron of Magnetism optto ewe aaants n imgeimi cha in diamagnetism and paramagnetism between Competition 6 iaosehbt ermgeimcue yre- by caused ferromagnetism exhibits atoms Li antcfils eas opr the compare also We fields. magnetic ASnmes 53.k 16.a 51.p 75.20.-g 75.10.Lp, res 51.60.+a, gases, 05.30.Fk, Boltzmann numbers: of PACS that than smaller and larger is gases ae,spoigtepril a he emnlevels Zeeman three has particle the supposing gases, larger a h i-adpr-antcrgos ntewa-edlimit, weak-field the In regions. para-magnetic and dia- the o temperatures, low eateto hsc,Uiest fSineadTechnolog and Science of University Physics, of Department h hre em a ihasalLande-factor small a with gas Fermi charged The .INTRODUCTION I. g ol eprmgei.W aclt h rtclvleo th of value critical the calculate We paramagnetic. be could g c 1 = ioigJa,Jhn i,adQagGu Qiang and Qin, Jihong Jian, Xiaoling / √ 2 Nevertheless, 12. g ,tezero- the 2, = Dtd oebr1,2018) 10, November (Dated: g c tal. et 87 au fFrigsswt hs fBlzanadBose and Boltzmann of those with gases Fermi of value Rb g c nrae ihtetmeauerdcn nfinite in reducing the with increases g sepesdas expressed is rm0t 2. to 0 the from electrons, from Different there g dia- electrons. freedom, in and of as paramagnetism degrees magnetism, between gas charge competition quantum and the the spin arises Once the gases. both Fermi has or Bose charged as 10 and mK ne fZea state Zeeman of index where ω with emo ihcharge with fermion u aaants nlarge in paramagnetism but ak h eeeayo ahLna ee with level Landau each of degeneracy the marks fti ae st aclt h rtclvleof value critical the calculate to is paper this of that expected small is in diamagnetism It displays gas effect. quantum the paramagnetic of intensity the where h ffcieHmloinwitnas written Hamiltonian effective the previously[12]. obtained spin-1 been charged have of which results gases with Bose comparison a present also ie adueeg ntemgei field magnetic the in energy Landau tized oa eto rai ,ydrcin ftesystem. the of directions y x, in area section total eoe h emnenergy, Zeeman the denotes fco o ieetmgei osi ies,ranging diverse, is ions magnetic different for -factor sepce ob imgei,wieta with that while diamagnetic, be to expected is σ h rn hroyai oeta fteFrigas Fermi the of potential thermodynamic grand The The ecnie hre em a of gas Fermi charged a consider We = = j qB/ ± H Ω ¯ µ g g 0 = 1 g T fco sacaatrsi aaee omeasure to parameter characteristic a is -factor , pectively. c − steceia oeta and potential chemical the is steLnefco and Lande-factor the is ,adfidthat find and 0, 6=0 ( a h aevlebt thg and high at both value same the has m ejn,Biig108,China 100083, Beijing Beijing, y µN , 1 µ ∗ = , ǫ c ,rsetvl.Tein a eregarded be can ions The respectively. K, 2 σ ǫ en h yoantcfeunyo a of frequency gyromagnetic the being ) − = jk . . . , = β z 1 D I H MODEL THE II. − D ( = e L ∗ q aeigdffrn adulvl and levels Landau different labeling g L g j,k n mass and m X fco hc separates which -factor 2 j,k 1 ~ | X z ,σ F, ∗ q + ,σ g z c c ,σ σB ( j fBs n Fermi and Bose of ǫ i n1+ ln[1 ) jk . g ~ gdFrigases Fermi rged ω z = ein h anpurpose main The region. m + + − ∗ ǫ e σ gσ . ~ 2 σ − 2 m D − β eest h spin- the to refers k ~ ∗ L ( z 2 ω, ǫ µ N jk ǫ = ) jk z n + atce,with particles, qBS z B jk ǫ σ stequan- the is , z − σ xy µ , ) g ] / S , region, (2 g xy We . π the ~ (4) (3) (2) (1) ǫ c σ z ) 2

−1 0.50 where β = (kBT ) . Performing Taylor expansions and

(a) then integrating out kz, Eq. (4) becomes

ωV m∗ 3/2 Ω = T =06 2 0.00

− ~ 2πβ  M ∞ 3 ~ω ~ ( 1)l+1l− 2 e−lβ( 2 −gσ ω−µ) − , (5) × 1 e−lβ~ω Xl=1 Xσ −

-0.50 where V is the volume of the system. For simplicity, the (b) following notation is introduced, 0.80

∞ p l+1 α/2 −lx(ησ+δ) σ ( 1) l e

Fτ [α, δ]= − , (6) M (1 e−lx)τ 0.40 Xl=1 − ~ ~ ~ where x = β ω and η = ( ω/2 µ + ǫ )/( ω). Then σ − σ Eq. (5) is rewritten as 0.00

(c)

∗ 3/2 ωV m -0.44 Ω = F σ[ 3, 0]. (7) T =06 ~2 1 − 2πβ  − d Xσ

M For a system with the given particle density n = N/V , the is obtained according to the fol- -0.48 lowing equation

∗ 3/2 0.0 0.4 0.8 1 ∂Ω m σ n = = x 2 F1 [ 1, 0]. (8) −V  ∂µ  2πβ~  − g T,V Xσ

A similar treatment has been employed to study diamag- FIG. 1: (a) The total magnetization density (M), (b) the netism of the charged spinless [13] and extended paramagnetization density (M p), and (c) the diamagnetiza- to the study of competition of diamagnetism and param- tion density (M d) as a function of g at t = 0.2. The dotted agnetism in charged spin-1 Bose gases[12]. This method and dashed lines correspond to ω = 5 and 10, respectively. is more applicable at relatively high temperatures. To determine gc, we need calculate the magnetization and density M as a function of the magnetic field B and tem- perature T . The system is paramagnetic when M > 0 3/2 σ 1 M 6 =t F [ 3, 0]+ x(gσ ) while diamagnetic when M < 0. M can be derived from T =0  1 − − 2 Xσ the thermodynamic potential by the standard procedure 1 ∂Ω M 6 = , which yields σ σ T =0 − V ∂B T,V F1 [ 1, 0] xF2 [ 1, 1] . (11)  × − − −  ~ ∗ 3/2 q m σ In following discussions, ω is used to indicate the magni- M 6 = F [ 3, 0] T =0 m∗c 2πβ~2   1 − tude of magnetic field since it is proportional to B. Xσ 1 + x(gσ )F σ[ 1, 0] xF σ[ 1, 1] . (9) − 2 1 − − 2 −  III. RESULTS AND DISCUSSIONS

For carrying out numerical calculations, it is useful 1 First, we look at a spin- 2 Fermi gas, setting σ = 1 to make the parameters dimensionless, such as M = to present the two Zeeman levels. The dimensionless± ∗ ~ ~ ∗ ∗ ∗ m cM/(n q), ω = ω/(kBT ), and t = T/T . Here T magnetization density M as a function of g is shown in is the characteristic temperature of the system, which is 2 Fig. 1(a). As expected, M is negative in the small g ∗ 2 ∗ given by kB T = 2π~ n 3 /m . Then we have x = ω/t, ′ ′ ∗ region, which means that the diamagnetism dominates. ησ =1/2 µ /ω gσ and µ = µ/(kBT ) in the notation For each given value of ω, M grows with g and changes σ − − Fτ [α, δ]. Equations (8) and (9) can be re-expressed as its sign from negative to positive in the larger g region, indicating that the paramagnetic effect is enhanced due 1= ωt1/2 F σ[ 1, 0] (10) to increase of g. This phenomenon is also observed in the 1 − Xσ Bose system[12]. gc is just the value of g where M = 0. 3

0.50

= 10

0.49

0.45

0.42 = 5 c c g

g

= 20

0.40 = 10 0.35

= 5

0.28

0.35

0 5 10 15 20

0 5 10 15 20

1/t

1/t

FIG. 2: Plots of the critical value of g-factor as a function of FIG. 3: The gc 1/t curves for charged spin-1 gases obey- 1/t. The magnetic field is chosen as ω = 20 ( line), 10 ing the Bose-Einstein− (BE, dotted line), Maxwell-Boltzmann (dashed line) and 5 (dotted line), respectively. (MB, solid line) and Fermi-Dirac (FD, dashed line) statistics, respectively. The magnetic field is chosen as ω = 10 and 5. The total magnetization M shown in Fig. 1(a) con- 1 1 sists of both the paramagnetic and diamagnetic contri- where λ = hβ 2 /(2πm∗) 2 , z = eβ(µ−ǫσ) and the Fermi- butions. Figure 1(b) depicts the pure paramagnetic con- Dirac integral fn(z) is normally defined as tribution to M, which is calculated by M p = gm where m = n n− . Figure 1(c) plots the diamagnetic con- ∞ n−1 1 − 1 1 x tribution to M, M d = M M p. For each fixed value fn(z) −1 x dx, (14) − ≡ Γ(n) Z0 z e +1 of ω, the diamagnetization M d is slightly weakened with increasing g. Interestingly, for a charged spin-1 Bose gas where Γ(n) is a usual gamma function and x = βǫ. Then in a constant magnetic field, the diamagnetism is not the magnetization density, M, is obtained from grand suppressed but enhanced as g becomes larger[12]. Com- thermodynamic potential in Eq. (13), paring Figs 1(a), 1(b) and 1(c), it can be seen clearly 1/2 that the increase of M with g is mainly owing to the 3/2 ′ ωt ′ M T =06 =gt σf 3 (z ) f 1 (z ) paramagnetization M p. 2 − 12 2 Xσ Xσ gc is an important parameter to describe the competi- 2 −1/2 tion between the diamagnetism and paramagnetism. Fig- ω t ′ 1 g σf− 1 (z ), (15) ure 2 plots gc for the charged spin- Fermi gas. The tem- − 24 2 2 Xσ perature is described by 1/t and the magnetic fields are ′ chosen to be relatively larger, since the method adopted where z′ = e(µ +gσω)/t. After some algebra, we get from here is more applicable at higher temperatures or in Eq. (15) that gc ω→0 =1/√12 0.28868. So in the weak stronger fields. In the high temperature limit, gc tends | ≈ field limit, gc has the same value both at the high and to a universal value, gc t→∞ =0.28868, regardless of the | low temperature limit. This implies that the gc 1/t strength of the magnetic field. In a fixed magnetic field, curve is likely to flatten out in the weak-field limit.− gc increases monotonically as the temperature falls down. To proceed, we make a comparison between Fermi But the trend of increasing is slowed down if the magnetic and Bose gases. Considering that gc for charged spin- field is weakened. 1 Bose gas has already been studied[12], we discuss a Present method can not produce valid results in the Fermi gas with three sublevels, σ = 1, 0 (a pseudo- low temperature region if a small magnetic field is chosen. ± ′ spin-1 Fermi gas) to ensure the comparability. Results In this case that gω t µ , the grand thermodynamic for the spin-1 Boltzmann gas are also obtained. Fig- potential in Eq. (4)≪ can≪ be calculated using the Euler- ure 3 shows the gc 1/t curves for the three kinds of Maclaurin formula − charged spin-1 gases. In a given value of ω, gc of all the ∞ 1 ∞ 1 three gases displays similar temperature-dependence: gc ψ(j + ) ψ(x)dx + ψ′(0), (12) increases monotonously as t reduces. In the high tem- 2 ≈ Z0 24 Xj=0 perature limit, gc goes to the same value in all magnetic fields, gc t→∞ = 1/√8, reflecting that the Bose-Einstein and then Eq. (4) is transformed into (BE) and| Fermi-Dirac (FD) statistics coincide with the Maxwell-Boltzmann (MB) statistics in this case. V Vβ 2 ΩT =06 = f 5 (z)+ (~ω) f 1 (z), (13) Figure 3 also demonstrates the difference among the −βλ3 2 24λ3 2 Xσ Xσ three kinds of statistics. For each given fixed value of ω, 4 the gc 1/t curves of Bose and Fermi gases always locate critical value of g and gc increases monotonically as the at the− two sides of that of the Boltzmann gas. Given the temperature t decreases in a fixed magnetic field ω, and same temperature and magnetic field, gc of Fermi gas the rise in gc is lowered as ω is reduced. We conjecture is the smallest. According to our previous research[12], that gc holds a constant at all temperatures in the weak 1 g → = 1/2 for the Boltzmann gas regardless of the field limit. For a spin- Fermi gas, g → =1/√12. We c|t 0 2 c|ω 0 magnetic field. This means that gc of the Fermi gas does also briefly compare gc of charged spin-1 gases obeying never exceed 1/2 in the low temperature, no matter how the Fermi-Dirac, Bose-Einstein and Maxwell-Boltzmann strong the field is. statistics. The gc 1/t curves of Boltzmann gases are al- ways between those− of Bose and Fermi gases in the same magnetic field. In the high temperature limit, gc of all IV. SUMMARY the three gases tends to the same value. This work was supported by the Fok Ying Tung Educa- In summary, we study the interplay between paramag- tion Foundation of China (No. 101008), the Key Project netism and diamagnetism of charged Fermi gases suppos- of the Chinese Ministry of Education (No. 109011), and ing that the Lande-factor g is a variable. The gas under- the Fundamental Research Funds for the Central Univer- goes a shift from diamagnetism to paramagnetism at the sities of China.

[1] L.D. Landau, E.M. Lifshitz, Statistical Physics. Part 1, Simkin, E.G.D. Cohen, Phys. Rev. A 59 (1999) 1528. Butterworth-Heinemann, Oxford, 1980. [8] T.-L. Ho, Phys. Rev. Lett. 81 (1998) 742; T. Ohmi, K. [2] J. Daicic , N.E. Frankel, R.M. Gailis, V. Kowalenko, Machida, J. Phys. Soc. Jpn. 67 (1998) 1822. Phys. Rep. 63 (1994) 237 and references therein. [9] Q. Gu, R.A. Klemm, Phys. Rev. A 68 (2003) 031604(R); [3] D.M. Stamper-Kurn, M.R. Andrews, A.P. Chikkatur, S. C. Tao, P. Wang, J. Qin, Q. Gu, Phys. Rev. B 78 (2008) Inouye, H.-J. Miesner, J. Stenger, W. Ketterle, Phys. 134403. Rev. Lett. 80 (1998) 2027. [10] K. Kis-Szabo, P. Szepfalusy, G. Szirmai, Phys. Rev. A [4] J. Stenger, S. Inouye, D.M. Stamper-Kurn, H.-J. Mies- 72 (2005) 023617; S. Ashhab, J. Low Tempt. Phys. 140 ner, A.P. Chikkatur, W. Ketterle, Nature 396 (1998) 345. (2005) 51. [5] L.E. Sadler, J.M. Higbie, S.R. Leslie, M. Vengalattore, [11] T.C. Killian, S. Kulin, S.D. Bergeson, L.A. Orozco, C. D.M. Stamper-Kurn, Nature 443 (2006) 312. Orzel, S.L. Rolston, Phys. Rev. Lett. 83 (1999) 4776. [6] G.B. Jo, Y.R. Lee, J.H. Choi, C.A. Christensen, T.H. [12] X. Jian, J. Qin, Q. Gu, unpublished. Kim, J.H. Thywissen, D.E. Pritchard, W. Ketterle, Sci- [13] G.B. Standen, D.J. Toms, Phys. Rev. E 60 (1999) 5275. ence 325 (2009) 1521. [7] K. Yamada, Prog. Theor. Phys. 76 (1982) 443; M.V.