Nonlinear Optics, Quantum Optics, Vol. 51, pp. 265–316 ©2019 Old City Publishing, Inc. Reprints available directly from the publisher Published by license under the OCP Science imprint, Photocopying permitted by license only a member of the Old City Publishing Group.
Pulsed Solid State Laser Systems Using ABCD Matrix Method: A Review
,∗ Y. S. NADA1,J.M.EL-AZAB2,S.M.MAIZE1 AND Y. H. E LBASHAR3
1Physics Department, Faculty of Science, Menoufia University, Shebeen-Elkoom, Menoufia, Egypt 2National Institute of laser Enhanced Sciences, Cairo University, Giza, Egypt 3Egypt Nanotechnology Center (EGNC), Cairo University, Giza, Egypt
Received: March 12, 2019. Accepted: April 14, 2019.
Although the laser diode and fiber laser are better than CW microchip lasers as they have the smallest size, compact design and wide range of emission laser wavelengths, the Q-switched solid state microchip laser is better than laser diode and fiber laser, because the energy storage capacity and laser induced threshold damage of laser diode are less than those of Q-switched microchip laser and long cavity of the fiber laser prevents achieving very short laser pulses. Yb:YAG was chosen as active medium due to its simple energy level scheme, long upper laser level lifetime (951 μs) which is suitable for storing energy, low quantum defects, large emission cross section, and large absorption cross-section for InGaAs laser emission. The combination of Cr4+: YAG and a doped- YAG gain medium, such as Yb:YAG, is particularly attractive from the point of view of an extremely robust device. Since both materials use the same host crystal, YAG, they can be diffusion-bonded to each other in a way that blurs the distinction between a monolithic and a composite- cavity device. Both materials have the same thermal and mechanical properties and the same refractive index, and the bond between them can be sufficiently strong that the composite device acts in all ways as if it were a single crystal. Due to better mechanical and thermal properties compared to the glass and single crystal, transparent ceramics became high power end-pumping lasers candidate in numerous fields. Ceramic active medium can be heavily and homogeneously doped with laser- active ions.
Keywords: ABCD Matrix, Pulsed lasers, laser systems, ultra short pulse lasers
∗ Corresponding author: e-mail: [email protected]
265 266 Y. S. NADA et al.
1. INTRODUCTION 1.1. Solid state lasers According to the case of active medium, lasers can be classified into solid, liquid or gas. The first invented laser was solid state laser (Ruby laser) [1]. Laser science has many branches like laser safety, material processing, and measurements, and all these applications depend on the active medium wave- length and switching technique [2–22]. The achieving gain with a given solid state laser system performance, the host material with its unique macroscopic and microscopic properties, the activator ions, and optical pump source should be selected self-consistently [23]. Solid state laser materials must have sharp fluorescent lines, strong absorption band and high quantum efficiency. Solid state laser materials are mainly crystal or glass doped by transitions or rare earth ions, in which optical transitions can occur between states of inner incomplete electron shells, (4f-4f) transition for rare earth and (3d-3d) transi- tion for transition ions doped materials. The laser radiation of solid state laser emits in the range of visible and near –IR spectrum (0.4-3μm) [23, 24]. Solid state laser material can be expressed as a physical system of active ions doped in host materials (crystal or glass). For best understanding of the solid state laser system, it can be approached by interaction among active ions with cer- tain electronic states, that be immersed in the local electrostatic crystal field of the host, a phonon field, and a photon field (see Figure 1) [25].
1.1.1. Active ions With an efficient absorption of the pump radiation and an efficient emission, the ions will be useful for giving the optical dynamics of laser material at
FIGURE 1 Physical system of a solid state laser. PULSED SOLID STATE LASER SYSTEMS 267
FIGURE 2 (a) Weak electron–phonon coupling of RE ions; (b) relatively strong electron–phonon coupling of TM ions described by the configurational coordinate model. certain wavelengths. In the case of ions with excellent absorption and weak emission, or vice versa, the solution is using two ions in the same host mate- rial, the first called sensitizer, which absorbs the pump energy, and the other called activator which emits the laser radiation. This operation takes place by having efficient nonradiative energy transfer from the sensitizer to the activa- tor through the strong overlap of the emission spectrum of the sensitizer and absorption spectrum of the activator [25]. Due to the electronic transitions of the active ions in the local ligand field environment of the host material, the optical spectral properties of a laser material are determined, and the active ions categorized into two main types. The first type is the transition metal ions (TM ions) which have the nonshielded 3d-electrons that can couple eas- ily with the phonons of the surrounding oxygen ligands, resulting in broad (3d-3d) transition bands. The other type are the rare earth ions (RE ions) with 4f-electrons which are shielded by the electrons of 5s and 5p orbitals leading to narrow (4f-4f) transitions, due to the weak interaction with the crystal field produced by the ligands as seen in Figure 2 [25-26].
1.1.2. Host material For achieving a highly efficient solid state laser material the active medium with a high optical quality should be fabricated with the absence of absorp- tion and scattering centers. Therefore, choosing the host material depends on its good optical properties, as inhomogeneous propagation of light through the crystal, which leads to poor beam quality, comes from the variation in the refractive index of the host material. Also, choosing the host material 268 Y. S. NADA et al. depends on its good mechanical and thermal properties such as, hardness, thermal conductivity and fracture strength. On the other side, the possibility of scaling the growth of impurity-doped crystal with maintaining high pro- duction should be obtained [23, 25-26]. The active ion properties such as: the size, disparity, valence, and the spectroscopic properties limit the number of useful materials for the solid state lasers. So, the crystal must have lat- tice sites that have local crystal fields of symmetry and strength required for achieving the desired spectroscopic properties and can accept ions with long radiative lifetimes with emission cross sections near 10−20 cm2 [23]. The two main groups of host materials are crystalline solids and glasses. Compared to glasses, the crystalline materials have the advantages of higher thermal con- ductivity, narrower fluorescence linewidths, and larger hardness. However, the crystalline materials show problems of poor optical quality and doping homogeneity as well as narrower absorption lines and limited dimension of laser medium. Rods of glasses up of to 1m in length and over 10 cm in diam- eter and disks of up to 90 cm in diameter and several centimeters thick, which are useful in high energy applications, have been produced with higher opti- cal quality [23].
1.2. Ceramic laser “Ceramics" is gotten from the Greek keramos, meaning porcelain and pottery. Ceramics are composed of randomly oriented microcrystallites, as shown in Figure 3, so the opaque and translucent cement and clay, used often in tableware, cannot be used as a laser medium. It is due to the existence of many scattering sources, such as grain boundary phases, residual pores and
FIGURE 3 Schematic presentation of the microstructure of conventional transparent ceramics, light scat- tering and the attenuation of input power through the ceramic body. Strong scattering owing to (28) a grain boundary, (30) residual pores, (32) secondary phase, (33) double refraction, (5) inclusions and (6) surface roughness in ceramics prohibits applications in optics [6]. PULSED SOLID STATE LASER SYSTEMS 269
FIGURE 4 Brief overview of the fabrication process of highly transparent Nd: YAG ceramics. secondary phases, which give rise to considerable scattering losses that block laser oscillation in the translucent ceramic laser gain medium [27]. In 1995 the first, highly efficient Nd: YAG ceramic laser medium with average grain size of 50 μm, was fabricated by a solid state reaction method using a high purity powder (> 99.99 wt% purity) [28]. Also Nd: YAG mate- rial with average grain size of 10 μm [29] and 3-4 μm [30] was made by using Nanocrystalline Technology and Vacuum Sintering method (NTVS) as illustrated in Figure 4. The first demonstration of polycrystalline Nd-doped YAG ceramics with high conversion efficiency of pore-free polycrystalline Nd:YAG ceramics and high optical quality comparable to the commercial one as well as single crys- tals with new structures were fabricated from ceramic with Solid–State Crys- tal Growth (SSCG) method, as illustrated in Figure 5 [31]; exhibiting a high degree of transparency. Dense Nd:YAG ceramic samples were prepared by conventional sintering and post- Hot Isostatic Pressing (HIP) treatment [32- 33]. As a result of these different techniques, transparent ceramics with very high optical quality were obtained, because. On the macroscopic scale these materials show no refractive index fluctuation or double refraction. On the microscopic one no secondary phases, residual pores or optically inhomoge- neous parts are observed [27]. Comparing ceramic composite and composite crystalline Nd:YAG rod used for high power diode end–pumping laser system 270 Y. S. NADA et al.
FIGURE 5 Fabrication process of a polycrystalline and a single crystal of Nd:YAG material.
[34-35] a maximum CW laser output power of 113 W, and a maximum opti- cal to optical transformation efficiency of 47% were achieved for ceramic rod. For crystalline rods these numbers were: 121 W fowerpower and 48% for effi- ciency. Also, most of the radiative spectral properties such as, cross sections of the intermanifold transitions, emission cross sections of the inter-Stark transitions as well as the fluorescence branching ratios of ceramic and single crystal Nd:YAG, are in good agreement [25].Therefore, ceramic technology can be considered as a good approach for overcoming the technological and economic problems of using single crystal. It has emerged as a promising candidate because it can be produced in large volumes, what is very suitable for high-power laser generation. It can also provide a gain medium for fiber lasers with high beam quality and can also be heavily and homogeneously doped with laser-active ions [27]. The Yb:YAG laser characteristics indicate a great potential for highly efficient and high power Diode Pumped Solid State (DPSS) lasers [36-40]. In 2003, the first cw Yb:YAG laser beam with 345 mw output power and 26% slope efficienc, was demonstrated. It was fab- ricated by nanocrystalline technology and a vacuum sintering method [37]. An output power 7.7 W with a slope efficiency of 60% in continuous wave (cw) operation and an output power of 9 W with a slope efficiency of 73% and a threshold of 1 W at 1030 nm in the quasi-continuous wave (qcw) oper- ation were obtained [36]. Output power of up to 5.1W with slope efficiency up to 44.3% (cw) has been achieved. 4.4 W power at 48 kHz, with 7-ns pulses were obtained by using passive Q-switching with Cr:YAG saturable absorber [38]. An average output power of 3.80W with a pulse duration of 433 fs at a repetition rate of 90.9 MHz and a peak power of 96.5kW was achieved at the wavelength of 1050 nm using a 2% output coupler in mode locked PULSED SOLID STATE LASER SYSTEMS 271
FIGURE 6 Energy levels in Yb:YAG.
Yb-YAG ceramic laser [39]. A maximum average output power of 2.55 W, with pulse duration of 11.5 ns, repetition rate of 5.71 kHz, pulse energy of 446.25 μJ and peak power of 38.8 kW were obtained by using composite Yb:YAG/Cr4+:YAG/YAG crystal with passive Q-switching at 1030 nm [40]. These results are mainly due to the distinctive physical properties of ytter- bium ion as a long life time emission, a broad emission band and a wide range of tunability, a simple energy level scheme (just two manifolds), a low quantum defect; this in addition to the accessibility of suitable ceramic hosts with good thermo-mechanical properties [36,37].
1.3. Microchip laser Solid state laser systems are composed of discreet optical components that must be carefully assembled and critically aligned. Thus, the laser assembly must be carried out by trained technicians what results in a large cost and consuming time. Also the laser is of large size and become unreliable. The solution to these problems of high cost, time consuming, large size and unre- liability is the Microchip laser. The term ‘microchip laser’ was coined at MIT Lincoln Laboratory in the early 1980s to draw an analogy between this new class of device and semiconductor electronic microchips with their inherent small size, reliability, and low-cost mass production [26,41].
1.3.1. Microchip laser construction Microchip lasers are miniature diode-pumped solid-state devices formed by dielectrically coating thin platelets of gain media [42]. As illustrated in Figure 7 a microchip laser consists of a small piece of solid-state gain medium polished flat and parallel on two sides. Cavity mir- rors are dielectrically deposited directly onto the polished surfaces and the 272 Y. S. NADA et al.
FIGURE 7 Monolithic microchip laser. laser is longitudinally pumped with a semiconductor diode laser. Microchip lasers that consist of a single dielectrically coated material are referred to as monolithic. There are several aspects of the microchip laser that make it interesting. First, the cavity length can be made sufficiently short that only a single longitudinal mode falls under the gain profile, thereby ensuring single- frequency output. By using a flat-flat cavity and longitudinally pumping the microchip laser, the TEM00 mode is strongly favorized and only one trans- verse mode may oscillate. When only one spatial mode oscillates (both lon- gitudinal and transverse), the two orthogonal polarization modes of the laser compete for exactly the same gain and the device operates in a single polar- ization. Another extremely important aspect of microchip lasers is that all of their surfaces are flat. This allows large wafers of microchip lasers to be pol- ished and coated before the wafers are cut into 1-mm-square pieces, with each piece being a complete device. As a result of their small size and simple fab- rication, microchip lasers are potentially mass producible at low cost. Other interesting aspects, for dynamic applications of microchip lasers, are their short cavity lifetimes and small mode volumes. It allows for rapid changes of the operating parameters of the lasers, leading to high rates of frequency modulation and a short-pulse operation. Yb:YAG material was successfully used in microchip lasers operating at 1.05 mm [43], which is becoming more popular, particularly in passively Q-switched devices because of its longer upper-state lifetime [26].
1.3.2. Pumping microchip lasers Microchip lasers are pumped by semiconductor diode lasers. In the simplest configuration one places the microchip laser in close proximity to the output PULSED SOLID STATE LASER SYSTEMS 273
FIGURE 8 Photograph of passively Q-switched microchip laser bonded to the ferrule of the fiber used to pump it. facet of the diode with no intervening optics [41]. An alternative configura- tion for pumping microchip lasers uses a fiber coupled diode laser. This con- figuration decouples the diode-laser system from the microchip cavity and offers several practical advantages. It facilitates an extremely compact laser head which can fit into small places, coupled to the rest of the system by a single, flexible optical fiber, as shown in Figure 8 [26].
1.3.3. Passively Q-switched laser A passive Q-switching provides an attractive alternative to the active one for many applications. A passively Q-switched laser contains a gain medium and a saturable absorber. As the gain medium is pumped it accumulates energy and emits photons. Over many round trips in the resonator the photon flux sees gain, fixed loss, and a saturable loss. If the gain medium saturates before the saturable absorber andthe laser will tend to oscillate in cw mode. On the other hand, if the photon flux builds up to a level that saturates, or bleaches, the saturable absorber first, the resonator will see a dramatic reduction in intracavity loss and the laser will Q-switch, generating a short, intense pulse of light, without the need for any high-voltage or high-speed switching elec- tronics. In addition to simplicity of implementation, the advantages of a pas- sively Q-switched laser include the generation of pulses with a well-defined energy and duration that are insensitive to pumping conditions. In contrast to actively Q-switched lasers, the population inversion at the time the cavity Q-switches is fixed by material parameters and the design of the laser. In the absence of pulse bifurcation it is identical from pulse to pulse. The most com- monly used saturable absorber for passive Q-switching of microchip lasers is Cr4+: YAG. It has been used to Q-switch Nd:YAG microchip lasers operating at 1.064 mm [44,45], 946 nm [45], and 1.074 mm [46]; Nd:YVO4 microchip lasers operating at 1.064 mm [47]; Nd:GdVO4 microchip lasers operating at 1.062 mm [48]; and Yb:YAG microchip lasers operating at 1.03 mm [49, 50]. The combination of Cr4+: YAG and a doped-YAG gain medium, such as Nd:YAG, is particularly attractive from the point of view of an extremely robust device. Since both materials use the same host crystal, YAG, they can 274 Y. S. NADA et al.
FIGURE 9 Schematic presentation of a composite-cavity Yb:YAG/Cr4+:YAG passively Q-switched microchip laser. be diffusion-bonded to each other in a way that blurs the distinction between a monolithic and a composite-cavity device. Both materials have the same thermal and mechanical properties and the same refractive index, and the bond between them can be sufficiently strong that the composite device acts in all ways as if it were a single crystal.
2. ATOMIC PROCESSES 2.1. Light absorption and emission Absorption and spontaneous emission processes are the two main atomic pro- cesses required to obtain an incoherent light emission. In case of producing laser, stimulated emission process takes place. This process is similar to spon- taneous emission except that emission is stimulated to occur by a “seed” pho- ton, which is “cloned” to produce two identical photons which are coherent photon as they have the same wavelength and are in phase [51]. As illustrated in Figure 10, both the absorption and the stimulated emis- sion are stimulated processes and are opposite of each other. Stimulated emis- sion requires an initial photon: an atom already at the upper energy level is stimulated to produce a photon by proximity to an existing photon. In the course of the process the original photon is not destroyed but rather passes through the medium with an identical clone produced in the process [51]. To introduce probabilities of these absorption and emission processes, let us consider two energy levels system as illustrated in Figure 11, with N1 as PULSED SOLID STATE LASER SYSTEMS 275
FIGURE 10 Atomic processes in laser.
FIGURE 11 Schematic presentation of (a)Spontaneous emission (b) Stimulated emission (c) Absorption pro- cesses.
the population of the ground state and N2 as the population of the excited state. For the spontaneous emission (see Figure 11(a)) the decay rate of the excited state (dN/dt)sp must be proportional to the population N2. dN2 =−AN2 (1) dt sp where A is a positive constant named the rate of spontaneous emission or Einstein A coefficient. The quantity (τsp = 1/A) is the spontaneous emission (radiative) life time. For the stimulated emission (Figure 11(b)) the decay rate can be written as dN2 =−W21 N2 (2) dt st
dN2 where ( dt )st is the rate at which transition from upper energy level to lower energy level (2-1) occurs due to the stimulated emission and (W21) is the rate of stimulated emission which has the dimension of (time−1) and depends on 276 Y. S. NADA et al. both the 2-1 transition and the flux of incident photons. For a plane wave it can be written that, W21 = σ21θ, where θ is the photon flux of the incom- ing wave and σ21 is the stimulated emission cross section, which depends on the transition characteristics. Similarly the stimulated absorption can be expressed as follows dN1 =−W12 N1 (3) dt ab dN1 where the derivative dt ab is the transition rate from lower to the upper energy level (1-2) due to absorption (Figure (c)) and (W12) is the rate of absorption process which can be written as,
W12 = σ12 (4) where σ12 is the absorption cross section which depends on the 1-2 transition characteristics. Rate equations that describe the population in the laser levels and number of photons in the laser cavity can be derived by using the probabilities of the absorption and emission processes.
2.2. Population rate equation In this chapter we will derive the population rate equation for two -, three -, four - and quasi-three level lasers which are considered in the current study.
2.2.1. Population rate equations for two level lasers In the two level lasers, the rate of change of N2 due to both absorption and stimulated emission is given by
dN 2 = (absorption rate)N − (stimulated emission rate)N (5) dt 1 2
The stimulated processes are characterized by the stimulated emission and absorption cross-sections σ21 and σ12, respectively. Einstein showed at the beginning of the twentieth century that, if the two levels are nondegenerate, one has W21 =W12 and thus σ21 = σ12 [52]. Thus we can write,
dN 2 = absorption rate(N − N ) (6) dt 1 2 and
dN 2 = σ(N − N ) (7) dt 1 2 PULSED SOLID STATE LASER SYSTEMS 277
Similarly the rate of change of N1 due to both absorption and stimulated emission can be expressed as,
dN 1 = σ(N − N ) (8) dt 2 1
Also the spontaneous emission has an effect on the population of these two levels. Thus the complete rate equations will be obtained by adding the term of spontaneous emission from Equation (28) to Equations (7 & 8).
dN 2 = σ(N − N ) − A N (9) dt 1 2 21 2
dN 1 = σ(N − N ) + A N (10) dt 2 1 12 2
We must account also for the pumping process that produces the (positive) population inversion (N2 − N1). To do this the most simply we add a term Wp to the population equation and call it the pumping rate into the upper level. Therefore Equation (36) will read as,
dN 2 = σ(N − N ) − A N + W (11) dt 1 2 21 2 p
2.2.2. Population rate equations for three level laser In fact, in the two level system the probabilities of the excitation and de- excitation are the same, i. e., by irradiating the medium, the radiation will induce both upward transitions 1– 2 (absorption) and downward transitions 2 –1 (stimulated emission). Therefore there no population inversion takes place. The solution of this problem is by using of a third energy level, as in the three-level laser inversion scheme, which is shown in Figure 12 [53].
FIGURE 12 Three-level laser. Level 1 is the ground stat. Laser oscillation occurs on the 2 –1 transition. 278 Y. S. NADA et al.
In this three level system, such as the ruby laser, level 3 is depopulated rapidly via fast decay to the upper laser level 2 which does not give the pumping process much chance to act in reverse and repopulate the ground level 1. Also, it can be considered that the pumping process occurs directly from lower laser level (level 1) to the upper laser level (level 2), because any atom in level 3 converts quickly to level 2. The change of population of dN1 =− level (28) due to pumping is; dt PN1 , where (P) is the pumping rate which is the number of atoms per cubic centimeter per second that are excited from level 1 to level 3. According to the assumption that, level 3 decays very rapidly to level 2 we can write for the rate of change of population of level 2 due to pumping the following expression:
dN dN dN 2 ≈ 3 =− 1 = PN (12) dt dt dt 1
Atoms in level 2 are decaying form level 2 to level 1 via the spontaneous and stimulated emissions, respectively. Thus the changes in the populations of these two levels can be written as:
dN 1 = σ(N − N ) + A N − PN (13) dt 2 1 21 1 1 and
dN 2 = PN − σ(N − N ) − A N (14) dt 1 2 1 21 1
2.2.3. Population rate equation for Four level laser As illustrated in Figure 13 another useful system for achieving population inversion is possible. The lower laser level (level 1) is not the ground level but, an excited level that can itself decay into the ground level what enhances the population inversion [53]. In four level lasers such as Nd:YAG the pumping proceeds from the ground level 0 to level 3, which, as in the three-level laser, decays rapidly into the upper laser level 2. Also level 1 is decaying rapidly into ground level, thus we can write N3 = N1 ≈ 0 and, the population inversion (N2 − N1) ≈ N2 = N. The change in level 2 population due to the spontaneous emission and stimulated emission with the effect of pumping process can be expressed in the following equation.
dN 2 = PN − σN − A N (15) dt 21 PULSED SOLID STATE LASER SYSTEMS 279
FIGURE 13 A four-level laser. The lower laser level 1 decays into the ground level 0.
2.2.4. Population rate equation for a Quasi-three level system In a quasi-three level lasers such as Yb:YAG which is the active medium used in this study; the lower laser level is sublevel of the ground level states which are strongly coupled and in thermal equilibrium therefore non-negligible fraction of the ground state population is present in the lower laser level because the energy separation between sublevels 0 and 1 is comparable to KT. This results in laser photon absorption. See Figure 14 [52]. As illustrated in Figure 14 pumping state decays very rapidly into the upper laser level, so that we can deal with N1 and N2 as the total popula- tion in the laser. The rate equations for upper state laser sublevels can be
FIGURE 14 Quasi – three- level laser. 280 Y. S. NADA et al. written in terms of the total populations N1 and N2 as follows;
dN N 2 = PN − (σ N − σ N ) − 2 (16) dt 1 e 2 a 1 τ where σe and σa are the emission and absorption cross sections of laser pho- tons, respectively.
2.3. Photons rate equation Laser rate equations are derived on the basis of a simple notion that there should be a balance between the total number of atoms undergoing a transi- tion and the total number of photons being created or annihilated [52]. The change in intensity of the laser beam I(ν) due to the stimulated emis- sion and absorption is described in plane wave approximation by the follow- ing equation [53]: 1 ∂ ∂ g2 − ) I (ν) = σ(ν) N2 − I (ν) (17) c ∂t ∂z g1
As we postulate that these two levels of the same degeneracy, i. e. g1 = g2 and by neglecting the population of the ground state, Equation (44) will take + the form in the forward direction of the propagation, where I(ν) is the intensity of the laser beam in the forward direction of propagation.
∂ I +(ν) 1 ∂ I +(ν) + = σ(ν)N I +(ν) (18) ∂z c ∂t 2
− In the backward direction of propagation case, where (I(ν)) is the correspond- ing intensity of the laser beam, the equation can be written as,
∂ I −(ν) 1 ∂ I −(ν) − + = σ(ν)N I −(ν) (19) ∂z c ∂t 2
Addition of the two Equations (18 & 19) gives
∂(I +(ν) − I −(ν)) 1 ∂(I +(ν) + I −(ν)) + = σ(ν)N (I +(ν) + I −(ν)) (20) ∂z c ∂t 2
There is a very little variation of I +(ν)&I −(ν) with z in many lasers [30], therefore Equation (46) can be approximated by:
d (I +(ν) + I −(ν)) = cσ(ν)N (I +(ν) + I −(ν)) (21) dt 2 PULSED SOLID STATE LASER SYSTEMS 281
FIGURE 15 Energy level diagram of (a) Yb:YAG laser medium and (b) Cr4+:YAG saturable absorber.
If the gain medium does not completely fill the resonator i.e. l < L, where L is the cavity length and l is the active medium length, the left side of Equation 20,which is independent of z, is simply multiplied by L. However, the right side is multiplied by l, which is less than L, Thus,
d (I +(ν) + I −(ν))L = cσ(ν)N (I +(ν) + I −(ν))l (22) dt 2
Since the number of photons inside the cavity is proportional to the total intensity I +(ν) + I −(ν) we may write,
d = σ ν l (2 ( )N2) (23) dt tr
= 2L where is the photon flux and (tr c ) is the cavity round trip time.
2.4. Steady state laser rate equations model Two differential equations which control the process of stimulated emission in the period that after the switching, had been formulated with concerning only with the fast switching case in which no significant changes of popula- tion inversion takes place. Also, the processes of slow effects in comparison to the formation of the giant pulse, such as continued pumping and sponta- neous emission have been neglected. The population inversion, total energy and peak power can be obtained by solving these two equations [54]. Gener- alized theory which includes the effect of the absorber in the cavity flux and population inversion rate have been formulated and results in three rate equa- tions [55]. Solution of these rate equations for the key laser parameter such as the output energy and pulse width had been obtained without considering the saturable absorber excited state absorption [56]. The three rate equations 282 Y. S. NADA et al. considering the Cr:YAG saturable absorber excited state absorption had been solved to obtain pulse characteristics such as output energy, peak power and pulse width [57]. In this Chapter a laser rate equation model will be intro- duced to describe the behavior of Yb:YAG/Cr:YAG composite ceramic pas- sively Q switched microchip laser. Including the excited state absorption of the saturable absorber, the pump term and the reabsorption loss of the quasi- three-level laser medium, the modified coupled rate equations of photons and the saturable absorber in the passively q-switched resonator are given in Refs [55–58]. d 1 = [ 2σ (ν)Nl − 2σg Ngls − 2σe Nels − ln − L − 2αLl ] (24) dt tr R
dN N =−γσcN − + W (25) dt τ p
dNg Nso − Ng =−σgcNg + (26) dt τs
Ng + Ne = Nso (27)
All the mentioned parameters are defined in Table 1. Equations (24-26) describes the behavior of the resonator photon flux with time. This equation includes all mechanisms contributing to the intracavity photon flux. The first term (2σ Nl) is the gain of the active medium. The second term (−2σg Ngls ) and the third term (−2σe Nels ) express the losses of the intracavity photon flux as a result of absorbing atomic transitions of the q-switch ground and excited states over the saturable absorber length, − 1 respectively. The fourth term ( ln R ) is the useful loss due to laser output extracted from the cavity. The fifth term (−L) is the remaining loss due to other cavity optical processes, such as material scattering, quantum defects, etc. the sixth term (−2αLl) is the loss due to the reabsorption of quasi-three- level Yb:YAG laser material. Equation (25) represents the time behavior of the population inversion density of the laser gain medium as a result of stim- ulated emission, spontaneous emission and the volumetric pump rate into the upper laser level which is proportional to the continuous-wave pump power, αl Wp = Pp[1 − e ]/(hvp A pl), respectively. where (Pp) is the incident pump power, (hvp) is the pump photon energy, (A p) is the pump beam area and (α) is the absorption coefficient of gain medium at the pump wavelength [58]. ?? is the inversion reduction factor which indicates the population inver- sion change in the laser active medium when the population inversion of the upper laser level is decreased by one. It is equal 2 for Yb3+ doped three-level PULSED SOLID STATE LASER SYSTEMS 283
TABLE 1 Rate equation model parameters. Symbol Meaning The photon density in the laser cavity
tr Cavity round trip time = 2lc/c
lc Optical length of the laser cavity c Speed of light in vacuum σ Stimulated emission cross section of the laser medium N Population inversion density of the gain medium l Length of the laser gain medium
σg Absorption cross section of the ground state of the saturable absorber
Ng Ground state population of the saturable absorber
ls Length of the saturable absorber
σe Absorption cross section of the excied state of the saturable absorber
Ne excited state population of the saturable absorber R Reflectivity of the output coupler L Nonsaturable intracavity round-trip dissipative optical loss
αL Absorption coefficient at lasing wavelength of gain medium γ Inversion reduction factor τ Life time of the upper laser level of the gain medium
Wp Volumetric pump rate into the upper laser level
Nso Total population density of the saturable absorber
τs Excited state life time of the saturable absorber solid-state lasers [58–60]. Equation (26) shows the variation of the population density of the q-switch element ground state depending on stimulated absorp- tion and the spontaneous emission, respectively. As the photon flux increases, the ground state population density decreases until bleaching. The effect of pumping process and spontaneous decay of the laser population inversion density during pulse duration can be neglected, because they take a quite long time in comparison to the pulse build up time. Therefore the Equation (25) becomes:
dN =−γσcN (28) dt
Before saturation of the saturable absorber, the initial population inversion density (Ni ) can be approximated to zero. Because, the photon density is low 284 Y. S. NADA et al. the most of the population of the saturable absorber is in the ground state. Thus we can assume that
d = 0, N = N , N = 0, N = N . (29) dt g so e i
By substituting in Equation (24), the initial population inversion can be writ- ten as 1 2σg Nsols + ln + L + 2αLl N = R (30) i 2σl
After the bleaching of the saturable absorber with highest photon intensity, almost all the saturable absorber ground state population is excited. Thus we can assume that
d = 0, N = 0, N = N , N = N . (31) dt g e so th
By substituting in Equation (24), the threshold population inversion (Nth) can be written as: 1 2σe Nsols + ln + L + 2αLl N = R (32) th 2σl
Using Equation (32) we rewrite Equation (24) in the form:
d = (2σ Nl − 2σ N l) (33) dt t th
Dividing Equation (33) by Equation (28) in order to get;
d l N − N =− th (34) dN lc γ N
Equation (34) can be integrated from the time of Q-switch opening to an arbitrary time (t) by