EXISTENCE OF WEAK SOLUTIONS FOR A PSEUDO-PARABOLIC SYSTEM COUPLING CHEMICAL REACTIONS, DIFFUSION AND MOMENTUM EQUATIONS∗
ARTHUR J. VROMANS†‡ , FONS VAN DE VEN† , AND ADRIAN MUNTEAN‡
Abstract. We study the weak solvability of a nonlinearly coupled system of parabolic and pseudo-parabolic equations describing the interplay between mechanics, chemical reactions, diffusion and flow in a mixture theory framework. Our approach relies on suitable discrete-in-time energy-like estimates and discrete Gronwall inequalities. In selected parameter regimes, these estimates ensure the convergence of the Rothe method for the discretized partial differential equations.
Key words. System of nonlinear parabolic and pseudo-parabolic equations, reaction-diffusion, weak solutions, existence, Rothe method.
AMS subject classifications. Primary, 35A01, 35K51; Secondary, 35D30, 35K70, 74D05, 74F10, 74F20, 74F25
1. Introduction. We investigate the existence of weak solutions to a system of partial differential equations coupling chemical reaction, momentum transfer and diffusion, cast in the framework of mixture theory [4]. We use the Rothe method [17, 30] as main tool. For simplicity, we restrict ourselves to a model with a single non-reversible chemical reaction in a one-dimensional bounded spatial domain [0, 1] enclosed by unlimited (or instantly replenished) reservoirs of the reacting chemicals. The chemical reaction is of the N-to-1-type with the reacting chemicals consisting out of solids and a sin- gle fluid, while the produced chemical is a solid. New mathematical challenges arise due to the strong nonlinear coupling between all unknowns and their transport fluxes.
Evolution systems, in which chemical reactions, momentum transfer, diffusion and stresses interplay, occur practically in every physical or biological system where there is enough knowledge to describe completely the balances of masses and forces; see e.g. [7, 10, 13, 26]. In all these situations, the interest lies in capturing the ef- fects flows have on deformations, deformations and chemical reactions on structures, and structures on chemical reactions and flow. In biology, such a system is used, for instance, to better understand and eventually forecast the plant growth and develop- ment [26]. In structural engineering, one wants to delimit the durability of a concrete sample exposed to ambiental corrosion, for example sulfate attack in sewer pipes [13]. Our initial interest in this topic originates from mathematical descriptions of sulfate corrosion [2]. We have realized that the mathematical techniques used for a system
arXiv:1702.02481v1 [math.AP] 8 Feb 2017 describing sulfate attack [when within a porous media (concrete) sulfuric acid reacts with slaked lime to produce gypsum], could be equally well applied to some more gen- eral systems sharing similar features (e.g. types of flux couplings and nonlinearities).
At a general level, the system outlined in this paper is a combination of parabolic
∗Submitted to the editors February 7th, 2017. Funding: This work was funded by the Netherlands Organization for Scientific Research (NWO) under contract no. NWO-MPE 657.000.004. †Centre for Analysis, Scientific Computing and Applications (CASA), Technische Universiteit Eindhoven, Eindhoven, The Netherlands ([email protected], [email protected]). ‡Department of Mathematics and Computer Science, Karlstads Universitet, Karlstad, Sweden ([email protected]). 1 2 A. J. VROMANS, A. A. F. VAN DE VEN AND A. MUNTEAN equations of diffusion-drift type with production terms by chemical reactions and pseudo-parabolic stress equations based on viscoelastic terms. On their own, both parabolic equations (cf. e.g. [11, 19, 20], and pseudo-parabolic equations (see e.g. [3, 12, 14, 28, 29, 31]) are well-understood from mathematical and numerical analysis perspectives. However, coupling these objects leads to systems of equations with a less understood structure. Many systems in the literature seem similar to ours at a first glance. A coupling remotely resembling our case appears in [1], but with differ- ent nonlinear terms, others like those in [1,7] do not have the pseudo-parabolic part, [10, 13] refer to a different domain situation, while in [26] higher-order derivatives are involved.
Due to the strong coupling present in our system, we chose to investigate in this paper the simplest case: a one-dimensional bounded domain, benefiting this way of an easier control of the nonlinearities by relying on the embedding H1 ,→ L∞ within a decoupling strategy of the model equations inspired by the method of Rothe. The study of the multidimensional case will be done elsewhere.
We apply our techniques to a general system introduced in Section 2, which covers e.g. mathematical models describing sulfate attack on concrete. In this section, we also introduce a set of assumptions based on which the existence of weak solutions can be proven. In our setting, the parabolic equations contain only coupling terms consisting of time-derivative terms of the unknowns of the pseudo-parabolic equations, while the pseudo-parabolic equations contain only coupling terms through Lipschitz- like non-linearities coupling back to the parabolic part of the system. In Section 3, we apply a time discretization decoupling the evolution system, inspired by the method of Rothe, such that the Lipschitz functions are evaluated at a different time-slice than the unknowns involved in the pseudo-parabolic part. The decoupled pseudo-parabolic equations can now be solved given the solution of the parabolic system posed at the previous time slice, while the new parabolic part can be solved with the just obtained solution of the pseudo-parabolic equations. The discrete-in-time a priori energy-like estimates are derived in Section 4 by testing the discretized system with suitable functions leading to quadratic terms and then by applying the discrete Gronwall lemma to the resulting quadratic inequalities. Based on these a-priori estimates, we show in Section 5 that our assumptions stated in Section 2 are valid in certain parameter regions. Furthermore, based on our a-priori estimates, we prove in Section 6 that the linear interpolation functions of the solutions to the discrete system converge strongly to a weak solution of the original system.
2. Description of the system. We define our system on a time-space domain [t0,T ]×[0, 1], where t0 is the initial time and T is the final time defined at a later stage by Claim 3. The unknowns of our system d d d−1 d−1 are two vector functions, φ : ([t0,T ]×[0, 1]) → R and w : ([t0,T ]×[0, 1]) → R , and one scalar function v :[t0,T ] × [0, 1] → R. The vector φ consists of the volume fractions of the d chemical components active in a chemical reaction mechanism of redox type. The vector w refers to the displacements of the mixture components with respect to a reference coordinate system. The scalar function v denotes the velocity of the single chemical fluid. We identify the different components of the vectors with the different chemicals and use the following convention. The subscript 1 is related to the produced chemical. The subscript d is related to the fluid. All the other subscripts are related to the remaining solid chemicals. The unknowns interplay in the following EXIST. OF WEAK SOL. FOR COUPLED PARAB. AND PSEUDO-PARAB. SYS. 3
system of the evolution equations: For l ∈ {1, . . . , d}, m ∈ {1, . . . , d − 1}, we have
d−1 1 2 X X i j (1a) ∂tφl − δl∂z φl + Il(φ)∂z (Γ(φ)v) + ∂z Blijm(φ)∂t wm = Gφ,l(φ) m=1 i,j=0 d−1 1 X X j (1b) ∂z (Γ(φ)v) + ∂z Hjm(φ)∂t wm = Gv(φ) m=1 j=0 2 2 (1c) ∂twm − Dm∂z wm − γm∂z ∂twm + Fm(φ)v d−1 1 X X i n + ∂z Eminj(φ)∂z∂t wj = Gw,m(φ) j=1 i+n=0 i,n≥0 1,∞ d with functions Il, Γ,Blijm,Hjm,Fm,Eminj,Gφ,l,Gv,Gw,m ∈ W (0, 1) and constants δl,Dm, γm ∈ R+. Furthermore, abuse notation with kf(·)kW 1,∞((0,1)d) ≤ Pd f ∈ R+. Notice that this system must satisfy the conditions l=1 φl = 1, the fundamental equation of fractions, which allows for the removal of the l = d − 1 component of Equation (1a). We assume the volume fractions are insulated at the boundary, thus implying ∂zφ = 0 at the boundaries z = 0 and z = 1. The boundary at z = 0 is assumed to be fixed, while the boundary at z = 1 has a displacement W (t) = h(t) − 1, where h(t) is the height of the reaction layer at the present time t. The Rankine-Hugoniot relation, see e.g. [24], states that the velocity of a chemical at a boundary is offset from the velocity, U, of the boundary by influx or outflux of the chemical, i.e. ( φm (U − ∂twm) · nˆ = JˆmL (φm,res − φm)
φd (U − v) · nˆ = JˆdL (φd,res − φd) In general the function L(·) denotes the concentration jump across the boundary. However, we assume the boundary to be semi-permeable in such a way that only influx can occur. Hence L(f) := fH(f) = f+ denotes the positive part of f. Furthermore, we assume that the fluid reservoir is at the boundary z = 1: φd,res is positive at z > 1, but 0 at z < 0. The produced chemical does not have any reservoir at the boundaries. Therefore φ1,res = 0 at both z < 0 and z > 1. The other chemicals have a reservoir below the z = 0 boundary: φm,res is positive at z < 0 and 0 at z > 1 for 1 < m < d. We generalize the Rankine-Hugoniot relations by replacing φm with H1m(φ) and φd with Γ(φ).
The influx due to the Rankine-Hugoniot relations shows that the displacement wm|z=1 will not be equal to the boundary displacement W (t). This will result in stresses, which we incorporate with a Robin boundary condition at these locations [25, section 5.3]. Collectively for all t ∈ [t0,T ] these boundary conditions are ∂ φ | = 0, l 6= d − 1 (3a) z l z=0 ∂zφl|z=1 = 0, l 6= d − 1 w | = 0 1 z=0 ∂ w | = A (w | − W (t)) z 1 z=1 1 1 z=1 H (φ)∂ w | = Jˆ L (φ − φ | ) , 1 < m < d (3b) 1m t m z=0 m m,res m z=0 ∂ w | = A (w | − W (t)) , 1 < m < d z m z=1 m m z=1 v| = 0 z=0 ˆ Γ(φ)(∂th(t) − v)|z=1 = JdL (φd,res − φd|z=1) 4 A. J. VROMANS, A. A. F. VAN DE VEN AND A. MUNTEAN
It is worth noting that in the limit |Am| → ∞ one formally obtains the Dirichlet boundary conditions, which are the natural boundary conditions for this system from a physical perspective. The initial conditions describe a uniform and stationary equilibrium solution at t = t0:
(4) φl(t0, z) = φl0 and wm(t0, z) = 0 for all z ∈ [0, 1]. The collection of Equations (1a)–(1c), (3a), (3b), and (4) forms our continuous system. Notice that this continuous system needs the pseudo-parabolic terms: our existence method (of weak solutions) fails when we choose γm = 0. Moreover, the height func- tion h(t) in Equation (3b) cannot be chosen freely. Integration of Equation (1b) in both space and time together with Equation (3b) will yield an ODE of h(t), and, in special cases, a closed expression of h(t). Furthermore, the initial conditions (4) do not contain a description of v(t0, z), because this function can be calculated ex- plicitly: Equation (4) together with Equations (1b) and (1c) define a subsystem of ∂wm the variables ∂t (t, z), v(t, z) on (t, z) ∈ {t0} × (0, 1) with boundary conditions of Equation (3b). This subsystem can be written in the form on to which Theorem 4 can be applied, which shows that there exists a unique solution of this subsystem in 2 d (C (0, 1)) iff both Γ(φ(t0, z)) 6= 0 and H1m(t0, 0) 6= 0 are satisfied.
Our existence proof relies on the following set of assumptions: Assumption 1. d ≥ 2, Jˆd, Jˆm ≥ 0 and φd,res, φm,res ∈ [0, 1] for 1 ≤ m < d and Pd l=1 φl,res = 1. All chemical reactions, where d − 1 chemicals react to form 1 chemical, are allowed. The reacting solid chemicals (1 < m < d) flow into the domain from a reservoir at z < 0, while the reacting liquid chemical flows into the domain from a reservoir at z > 1. Moreover, the reservoir volume fractions are in the physical range [0, 1]. Assumption 2. For all 0<α<1/d introduce Iα as (α, 1 − (d − 1)α). Then Γα := inf Γ(φ) ∈ R+ and Hα := min inf H1m(φ) ∈ R+. d d φ∈Iα 1≤m Next to these assumptions, we want our solutions to be physical at almost every time t. So, the volume fractions must lie in [0, 1] and the velocity v(t) must be both essentially bounded and of bounded variation, which implies that both v and ∂zv 2 2 must be functions in the Bochner space L (t0,T ; L (0, 1)). However, the volume frac- tions φ cannot become 0 without creating problems for the original Rankine-Hugoniot boundary conditions or allowing singularities in the domain implying φ ∈ ((0, 1))d. To this end, we introduce a new time interval for which all of these constraints hold EXIST. OF WEAK SOL. FOR COUPLED PARAB. AND PSEUDO-PARAB. SYS. 5 and we claim that such an interval exists. Claim 3. There exists a time domain [t0,T ], a velocity V > 0 and a volume fraction φmin ∈ (0, 1/d) such that R t R 1 |v(s, z)|2dzds > V 2, t0 0 R t R 1 2 2 t 0 |∂zv(s, z)| dzds > V , T = inf t 0 , inf min φl(t, z) < φmin z∈(0,1) 1≤l≤d which, in line with Assumption 1, implies φl(t, z) ∈ Iφmin = [φmin, 1 − (d − 1)φmin] ⊂ (0, 1) for all (t, z) ∈ [t0,T ] × [0, 1] and 1 ≤ l ≤ d. This claim guarantees that all chemicals are omnipresent, while velocities and defor- mations remain bounded. This claim can be related to the theories on parabolic and pseudo-parabolic equations. The claim, which will be proven in Section 5, mimics the necessary L2(0, 1) and H1(0, 1) regularity of the coefficients in the parabolic and pseudo-parabolic equation theory. Combining the claim with Assumption 2 directly introduces the constants Γφmin and Hφmin respectively as lower bounds of Γ(φ) and d all H1m(φ) for φ ∈ Iφmin . In this paper we shall prove the existence of a volume fraction φmin ∈ (0, 1/d), a velocity V > 0 and a nonempty time interval [t0,T ] such that a weak solution of the continuous system exists if Assumptions 1,2,9, 17, 21 and 25 are satisfied. We will prove this statement in 4 steps: • First, we discretise the continuous system in time with a regular grid of step size ∆t, apply a specific Euler scheme and prove that this new discretised system can be solved iteratively in the classical sense at each time slice. • Second, we make a weak version of the discretised system and prove that there exists a weak solution of the continuous system. This will be done by choosing specific test functions such that we obtain quadratic inequalities. By application of Young’s inequality and using the Gronwall lemmas we obtain the energy-like estimates called the a priori estimates, which are step size ∆t independent upper bounds of the Sobolev norms of the weak solutions. • Third, we prove Claim 3 by showing that the upper bounds of the a priori estimates are increasing functions of T −t0 and V that have to satisfy specific upper bounds in order to guarantee the validity of Claim 3. Then, in certain parameter regions, regions in (T − t0,V )-space exist for which Claim 3 holds. • Fourth, we will introduce temporal interpolation functions u(t) = uk and k−1 k uˆ(t) = u +(t−tk−1)D∆t(u) to justify the existence of functions on [t0,T ]× [0, 1] and we will show that the weak limit for ∆t ↓ 0 exists and is a weak solution of the continuous system. 3. The discretised system and its classical solution. We discretise time with regular temporal grid tk = t0 + k∆t for ∆t > 0. This discretization is applied to Claim 3 with the infimum replaced with a minimum, the time t replaced with the discrete time tk and the time integrals replaced with Riemann sums. Consequently, the time T is now dependent on the discretization. To highlight this fact we introduce the notation T∆t for the time T of Claim 3 with regular tem- poral grid tk = t0 + k∆t. 6 A. J. VROMANS, A. A. F. VAN DE VEN AND A. MUNTEAN We discretise the continuous system in such a way that the equations become lin- ear elliptic equations with respect to evaluation at time tk, and only contain two time evaluations: at tk and tk−1. The time derivative ∂tu is replaced with the standard first k uk−uk−1 k order finite difference D∆t(u) := ∆t , where u (z) := u(tk, z). The discretised system takes the form k 2 k k−1 k−1 k−1 (5a) D∆t(φl) − δl∂z φl + Il(φ )∂z Γ(φ )v d−1 1 X X i k−1 k−1 k−1 k k−1 + ∂z Bli0m(φ )wm + Bli1m(φ )D∆t(wm) = Gφ,l(φ ) m=1 i=0 d−1 X k−1 k−1 k−1 k (5b) ∂z H0m(φ )wm + H1m(φ )D∆t(wm) m=1 k−1 k k−1 +∂z Γ(φ )v = Gv(φ ) k 2 k 2 k k−1 k−1 (5c) D∆t(wm) − Dm∂z wm − γm∂z D∆t(wm) + Fm(φ )v d−1 1 X X k−1 i k−1 k−1 k k−1 + ∂z Emi0j(φ )∂zwj + Em01j(φ )D∆t(wj) = Gw,m(φ ) j=1 i=0 with boundary conditions k ∂zφl z=0 = 0, l 6= d − 1 (6a) k ∂zφl z=1 = 0, l 6= d − 1 H (φk−1| )Dk (w ) = Jˆ L φ − φk−1 1m z=0 ∆t m z=0 m m,res m z=0 ∂ wk = A wk − Wk (6b) z m z=1 m m z=1 vk = 0 z=0 k−1 k k−1 ˆ k−1 Γ φ |z=1 D∆t(W) − v z=1 = JdL φd,res − φd z=1 , k where W := W (tk), and Jˆ1 = 0 in accordance with the first boundary condition of (3b), and initial conditions (4). A powerful property of this discretised system is its sequential solvability at time tk: the existence of a natural hierarchy in attacking this problem. First we obtain results for Equation (5c), then we use these results to obtain similar results for both Equations (5a) and (5b). Moreover, the structure of the discretised system is that of an elliptic system. Hence, the general existence theory for elliptic systems can be extended directly to cover our situation: n n Theorem 4. Let Ω ⊂ R bounded, A±,B±,C± ∈ M(R , R ), D a diagonal 2 n positive definite matrix of size n × n, and Eij, fi ∈ (L (Ω)) for all i, j ∈ {1, . . . , n}. There exists a unique solution u ∈ (C2(Ω))n of the system ( 2 ∂z u − ∂z(E(z)u) − Du = f on (x−, x+) =: Ω 0 A±u(x±) + B±u (x±) = C±. Moreover, if the conditions A+ + B+E(x+) B+ 6= 0 and min |Tr (E(z)) | > 0 A− + B−E(x−) B− z∈Ω EXIST. OF WEAK SOL. FOR COUPLED PARAB. AND PSEUDO-PARAB. SYS. 7 are satisfied, then the solution u is given by −1 u(z) Z z 0 A + B E(x ) B C = Ψ(z) Ψ(s) ds + + + + + + U(z) f(s) A + B E(x ) B C x− − − − − − A + B E(x ) B Z x+ 0 + + + + + Ψ(x ) Ψ(s) ds 0 0 + f(s) x− with U(z) = ∂zu − E(z)u, and with Ψ(z) ∈ M(Rn, Rn) for all z ∈ Ω satisfying E(z) ∂ Ψ(z) = In Ψ(z) for z ∈ Ω z D−1 0 Ψ(x−) = In Proof. See [27, p.130] for the general calculus result or see Chapter 6 of [11] for the elliptic theory result. In specific: rewrite system in terms of u and U. This system has a fundamental matrix Ψ(z) yielding the above solution after satisfying boundary conditions. k−1 d Corollary 5. Let ∆t > 0. For all t0 < tk such that φ ∈ (0, 1) there exists a 2d−1 unique solution uk := (φk, wk, vk) ∈ C2(0, 1) × C1(0, 1) of the system (5a)–(5c) with boundary conditions (6a) and (6b) and initial conditions (4). Proof. The result follows with induction with respect to k ≥ 0 from applying The- 1,∞ d orem 4 and using both Il, Γ,Blijm,Hjm,Fm,Eminj,Gφ,l,Gv,Gw,m ∈W (0, 1) and δl,Dm, γm ∈ R+. This result shows that there exists a solution of the discrete system even if the solution does not satisfy Assumptions 1,2,9, 17, 21 and 25 and Claim 3. The solution might therefore be non-physical. Furthermore these solutions might not have a weakly convergent limit as ∆t ↓ 0. We will use a weak solution framework to show the existence of physical solutions for which the weak convergence as ∆t ↓ 0 does exist. 4. A priori estimates. The estimates in this section rely on the validity of Claim 3. This validity will be proven in Section 5. Notice that from this moment onwards the notation l 6= d − 1 denotes l ∈ {1, . . . , d − 2, d}. We create a weak form of the discretised system by multiplying the equations with a function in H1(0, 1), integrating over (0, 1) and applying the boundary conditions k k where needed. To this end we test Equation (5a) with φl and D∆t(φl), and Equa- k k tion (5c) with wm and D∆t(wm). In Appendix A these tests are evaluated in detail 8 A. J. VROMANS, A. A. F. VAN DE VEN AND A. MUNTEAN and it is shown there how we obtain the following quadratic inequalities: d−1 ! 1 k X 2 2 (11) D kw k 2 + (γ + D )k∂ w k 2 2 ∆t m L m m z m L m=1 d−1 X ∆t k 2 ∆t ∆t k 2 + 1 + D (wm) 2 + γm 1 + + Dm D (∂zwm) 2 2 ∆t L 2 2 ∆t L m=1 d−1 X k 2 k 2 k−1 2 k−1 2 ≤ Kw0 + Kw1mkwmkL2 +Kw2mk∂zwmkL2 +Kw3mkwm kL2 +Kw4mk∂zwm kL2 m=1 k 2 k 2 k−1 2 k−1 2 +Kw5m D∆t(wm) L2 +Kw6m D∆t(∂zwm) L2 +Kw7kv kL2 +Kw8k∂zv kL2 , k 2 k 2 k 2 (12) D∆t kφlkL2 + 2δlk∂zφl kL2 + ∆t D∆t(φl) L2 k−1 2 k 2 X k−1 2 ≤ Kaφ0 + Kaφ1k∂zv kL2 + Kaφ2lkφl kL2 + Kaφ3lnk∂zφn kL2 n6=d−1 d−1 1 X X h i k−1 2 k i 2 i + Kaφ(4+i)m ∂zwm L2 + Kaφ(6+i)m D∆t(∂zwm) L2 , m=1 i=0 and k X 2 X 2 k 2 k 2 (13) D∆t k∂zφlkL2 + D∆t(φl) L2 + ∆t D∆t (∂zφl) L2 δl l6=d−1 l6=d−1 k−1 2 X h k 2 k−1 k−1 2 i ≤ Kbφ0 + Kbφ1k∂zv kL2 + Kbφ2l D∆t(φl) L2 + Kbφ3l k∂zφl kL2 l6=d−1 d−1 1 X Xh i k−1 2 k i 2 i + Kbφ(4+i)m ∂zwm L2 + Kbφ(6+i)m D∆t(∂zwm) L2 . m=1 i=0 The constants Kindex for x ∈ {a, b} can be found in Appendix A as Equations (74a)– (74i) and Equations (75a)–(75i). We are now able to apply two versions of the Discrete Gronwall lemma. The 1st version (of Lemma 6) will be applied to Equations (11) and (12), while the 2nd ver- sion (of Lemma 7) will be applied to Equation (13). Lemma 6 (1st Discrete Gronwall lemma). Suppose h ∈ (0,H). Let (xk), (yk+1) k and (z ) for k = 0, 1,... be sequences in R+ satisfying k−1 xk − xk−1 X (14) yk + ≤ A + zk−1 + Bxk + Cxk−1 and zjh ≤ Z h j=0 for all k = 1,... with constants A,B,C and Z independent of h satisfying A > 0, Z > 0,B + C > 0, and BH ≤ 0.6838, EXIST. OF WEAK SOL. FOR COUPLED PARAB. AND PSEUDO-PARAB. SYS. 9 then C + 1.6838B (16a) xk ≤ x0 + Z + A kh e(C+1.6838B)kh and C + B k X (16b) yjh ≤ x0 + Z + Ahk e(C+1.6838B)kh. j=1 Proof. We rewrite Equation (14) such that xk is on the left-hand side and xk−1 is on the right-hand side. We can discard the yk term since it is always positive. The partial sum of the geometric series yields Z A 1 + Ch k A xk ≤ x0 + + − 1 + Ch B + C 1 − Bh B + C from which we obtain Equation (16a) by applying the inequalities 1 2 (18) 1 + a ≤ ea ≤ 1 + aea for a ≥ 0 and ≤ ea+a for 0 ≤ a ≤ 0.6838. 1 − a With Bh − 1 ≤ BH − 1 < 0 we rewrite Equation (14) into k k−1 X X yjh ≤ Ahk + Z + (1 + Ch)x0 + (C + B)h uj. j=1 j=1 We insert Equation (16a) for xj and use j < k for the factor in brackets. Then the sum over exponentials can be seen as a partial sum of a geometric series, yielding k X C + 1.6838B e(C+1.6838B)kh − 1 yjh ≤ x0 +Z +Ahk+(C +B)h x0 + Z + A kh . C + B e(C+1.6838B)h − 1 j=1 With 1/(ea − 1) ≤ 1/a for a ≥ 0 one immediately obtains Equation (16b). Lemma 7 (2nd Discrete Gronwall lemma). Let c > 0 and (yk), (gk) be positive sequences satisfying X (21) yk ≤ c + gjyj for k ≥ 0, 0≤j then X (22) yk ≤ c exp gj for k ≥ 0. 0≤j Proof. The proof can be found in [15]. We introduce a set of new constants, which aid us in the application of the Gronwall lemmas: 10 A. J. VROMANS, A. A. F. VAN DE VEN AND A. MUNTEAN Definition 8. k A := max Kw0, t0≤tk≤T∆t B Kw2m := max Kw1m, , 2 m γm + Dm C Kw4m := max Kw3m, , 2 m γm + Dm 2 C+1.6838B (C+1.6838B)(T∆t−t0) (Kw7 + Kw8)V + A C+B (T∆t − t0) e C˜2 := , min {1 − Kw5m, γm − Kw6m} m k gbk := max Kbφ3l∆t, l6=d−1 d−1 X Kφ3l2m + Kφ3l3m K := , φ3l4 min{1 − K , γ − K } m=1 w5m m w6m 2 Kbφ5m 2 cb := Kbφ0(T∆t − t0) + Kbφ1V + max Kbφ4m, C˜ (T∆t − t0) m γm + Dm K K + max bφ6m , bφ7m C˜2, m 1 − Kw5m γm − Kw6m n 2 2o Db := max 2Kφ3l1V + Kφ3l4C˜ . l6=d−1 The constants Kindex not introduced here can be found in Equations (74a)–(74i) and Equations (75a)–(75i) of Appendix A. Moreover, introduce the constants Kaφ5m 2 Aa := Kaφ0 + cb exp(Db) max Kaφ3lj + max Kaφ4m, C˜ , l,j6=d−1 m γm + Dm 2 Kaφ6m Kaφ7m 2 Za := Kaφ1V + max , C˜ , m 1 − Kw5m γm − Kw6m Da := max Kaφ2l. l6=d−1 With these new notations, we obtain several simple expressions for the upper bounds by applying the Gronwall inequalities. However these expressions are only valid if the following assumptions are met. Assumption 9. Let B and C be given by Definition 8 and Mm01j as introduced in Equation (69b). Assume B + C > 0 and √ Mm11j + Mj11m + Mm01j γm = √ 2γ γ |A | + γ |A | + E (1 + γ ) + E < m . m m j j m01j m j01m d − 1 The second condition guarantees the pseudo-parabolicity, because it guarantees the conditions 1 > Kw5m and γm > Kw6m in Corollary 11. Assumption 10. Let B be given by Definition 8. Assume H = 0.6838/B. With these two assumptions the Gronwall inequalities imply the following upper bounds: EXIST. OF WEAK SOL. FOR COUPLED PARAB. AND PSEUDO-PARAB. SYS. 11 Corollary 11. Let ∆t ∈ (0,H). Introduce the sequences d−1 k X k 2 k 2 x = kwmkL2 + (γm + Dm)k∂zwmkL2 m=1 d−1 k X h k 2 k 2 i y = (1 − Kw5m) D∆t(wm) L2 + (γm − Kw6m) D∆t (∂zwm) L2 m=1 k k 2 k 2 z = Kw7kv kL2 + Kw8k∂zv kL2 . The inequality C + 1.6838B xk ≤ (K + K )V 2 + A (t − t ) e(C+1.6838B)(tk−t0) w7 w8 C + B k 0 is valid for all tk ∈ [t0,T∆t]. Furthermore, 1 > Kw5m and γm > Kw6m and the inequality k X j 2 (C+1.6838B)(tk−t0) y ∆t ≤ (Kw7 + Kw8)V + A(tk − t0) e j=1 is valid for all tk ∈ [t0,T∆t]. Proof. We first need to show that we can choose the η-indices such that 1 > Kw5m and γm > Kw6m, as otherwise we have insufficient information to bound all terms. There are d − 1 couplings between K and K through η . These √ w5m w6m √ Mm01j1 couplings only give Mm01j < 2 γm/(d − 1) and ηMm01j1 = 1/ γm as conditions. However Kw6m is coupled to itself as well through ηMm11j1. With ηMm11j1 = 1 it is immediately clear that the constraint of Assumption 9 allows one to choose the remaining η-indices in Kw5m and Kw6m freely to satisfy the inequalities. Hence, 1 > Kw5m and γm > Kw6m is guaranteed by Assumption 9. Next we apply Lemma 6 to Equation (11) in the form of Equation (14) with xk, yk k and z as above. With use of the identity k∆t = tk − t0 and with the initial condition 0 0 wm(z) = 0 for z ∈ (0, 1), yielding x (z) = 0, the two inequalities of Corollary 11 directly follow from Lemma 6. For the next result, we choose ηindex > 0 such that 2 > Kbφ2lδl holds. Corollary 12. Let t0 < tk ≤ T∆t. Introduce the sequence k X k 2 xb = k∂zφl kL2 l6=d−1 k X 2 k 2 yb = 2 − Kbφ2l D∆t(φl) L2 . δl l6=d−1 The inequalities k xb ≤ cb exp(Db) k X j y ∆t ≤ cb (1 + Db exp(Db)) j=1 are valid for all tk ∈ (t0,T ]. 12 A. J. VROMANS, A. A. F. VAN DE VEN AND A. MUNTEAN Proof. We can always choose ηindex > 0 in Kφ2l such that 2 > δlKφ2l holds. With the newly introduced notations cb, Db and gbn, and with the initial condition 0 0 ∂zφ (z) = 0 for z ∈ (0, 1), yielding xb = 0, we can sum inequality (13) and rewrite it into the inequality k−1 k−1 k−1 k k X j 0 X j X j xb ≤ xb + yb ∆t ≤ cb + xb + gbjxb = cb + gbjxb. j=0 j=0 j=0 Pk−1 k With j=0 gbj ≤ Db, direct application of Lemma 7 yields the bound of xb . Substi- k Pk j tuting this upper bound for xb will directly yield the upper bound of j=1 yb ∆t. We need an extra upper bound on H to guarantee the successful application of the k Discrete Gronwall lemma for φl . Assumption 13. Let B and Da be given by Definition 8. Assume 0.6838 0.6838 H = min , . B Da k Now an upper bound for kφl kL2 can be determined. k 2 Corollary 14. For ∆t ∈ (0,H) the sequence kφl kL2 satisfies the inequality k 2 2 1.6838Da(tk−t0) kφl kL2 ≤ φl0 + Za + 1.6838Aa(tk − t0) e for all tk ∈ [t0,T∆t] and all l 6= d − 1, if Assumptions 9 and 13 hold. Proof. We insert the bounds from Corollaries 11 and 12 in Equation (12), and we k k 2 use the new notations xa := kφl kL2 , and d−1 1 k k−1 2 X X k i 2 za := Kaφ1k∂zv kL2 + Kaφ(6+i)m D∆t(∂zwm) L2 , m=1 i=0 to obtain k k k D∆t (xa) ≤ Aa + za + Daxa from Equation (14). Once more apply Lemma 6 to obtain the result of Corollary 14. 5. Proof of Claim 3. The a priori estimates of the previous section depend heavily on Claim 3. This claim restricts the time interval (t0,T∆t) for which the physical volume fraction restriction k φj (z) ∈ [φmin, 1 − (d − 1)φmin] for all j 6= d − 1, and the physical velocity restrictions Pk j 2 2 Pk j 2 2 j=0 kv kL2 ∆t ≤ V , and j=0 ∂zv L2 ∆t ≤ V are valid. We need to prove that the interval (t0,T∆t) is non-empty. On closer inspection, we see that Claim 3 can be proven with upper bounds only. Lemma 15. Let t0 ≤ tk = k∆t ≤ T∆t. Let Pd be the set of cyclic permutations of k k P j 2 (1, . . . , d). The constraints φl (z)∈[φmin,1−(d−1)φmin] for l 6= d−1, kv kL2 ∆t ≤ j=0 EXIST. OF WEAK SOL. FOR COUPLED PARAB. AND PSEUDO-PARAB. SYS. 13 k 2 P j 2 2 V , and ∂zv L2 ∆t ≤ V are implied by j=0 2 2 X 1 1 − φmin φk ≤ for all α ∈ P , αj d H1 2 C∞ j6=d k X j 2 2 and ∂zv L2 ∆t ≤ V . j=0 Proof. The 3rd condition of Equation (6b) allows the application of the Poincar´e j inequality, which in one-dimensional space immediately gives the inequality kv kL2 ≤ j k k∂zv kL2 . With this relation we can reduce the number of constraints on v from two to one. k For the constraints on φl we randomly pick an α ∈ Pd and start with reversing 2 2 Young’s inequality on P φk ≤ 1 1−φmin , which yields P φk ≤ j6=d αj 2 C j6=d αj H1 ∞ H1 1−φmin C . This inequality is transformed by the Sobolev embedding theorem into ∞ P k k 2 j6=d φα ≤ 1 − φmin. With φα ∈ C (0, 1) for j 6= d, which is shown in Theo- j L∞ j rem 4, we can change the L∞ norm into a proper supremum on (0, 1). Hence we obtain inf φk ≥ φ from the identity 1 = P φk. Since α was chosen randomly, z∈(0,1) αd min 1≤l≤d l k we conclude that this result holds for all α ∈ Pd. Hence, min inf φl (z) ≥ φmin. 1≤l≤d z∈(0,1) With the d infima established it is immediately clear that the d suprema follow auto- matically from the same identity. Pd k The volume fraction identity 1 = l=1 φl cannot be used directly to satisfy the desired bound of Lemma 15. It would use a circular argument involving φmin: proving the lower bound φmin by a more stringent upper bound found in Lemma 15 and proving that upper bound with the volume fraction identity and the lower bound φmin. Indirectly, the volume fraction identity can be used as is shown in Appendix A, where k a differential equation for φd−1 is constructed and tested such that new inequalities (76) and (77) are found. Thus, from these new inequalities (76) and (77), Lemma 6 together with Corollaries 11, 12 and 14 yields an upper bound k 2 (35) φd−1 H1 ≤ P (T∆t − t0,V ) 2 The function P(x, y) has P(0, y) = φ(d−1)0 and it is a strictly increasing continu- ous function. Hence, for all cyclic permutations α of (1, . . . , d) there exist strictly increasing continuous functions P (T −t ,V ) with P (0, 0) = Pd−1 φ2 , such that α ∆t 0 α j=1 αj 0 d−1 X k 2 kφ k 1 ≤ P (T − t ,V ) αj H α ∆t 0 j=1 for all t0 ≤ tk ≤ T∆t. With this upper bound at hand, we are now able to show the existence of a non- empty time interval (t0,T ) for which the volume fraction condition of Claim 3 holds. Before we proceed, we need to introduce a geometric solid, the Steinmetz solid. 14 A. J. VROMANS, A. A. F. VAN DE VEN AND A. MUNTEAN Definition 16. Introduce a d-dimensional solid cylinder with central axis lc and radius r as the set of points at a distance at most r from the line lc. Following [16, 18] we introduce the d-dimensional Steinmetz solid Sd(r) as the intersection of d d-dimensional solid cylinders with radius r such that the axes lc intersect orthogonally at the origin. In particular we assume the orientation of the Steinmetz solid to be such d that the cylinder axes lc are spans of Cartesian basis elements in R . Hence d X 2 2 Sd(r) = (x1, . . . , xd) ∈ R x ≤ r for all 1 ≤ i ≤ d . j j6=i With the Steinmetz solid we obtain conditions for φmin, V and T − t0 to obtain k φl (z) ∈ (φmin, 1 − (d − 1)φmin) for all l and all t0 ≤ tk ≤ T∆t. For k = 0 these conditions impose constraints on the initial volume fractions. Therefore we need an extra assumption. 0 Assumption 17. Let φ = (φ10, . . . , φd0) ∈ S, where ( d ) 1 − φmin X √ 0 d 0 d S = Sd ∩ φ ∈ R φl = 1 ∩ [φmin, ∞) , 2C∞ l=1 with Sd(·) the Steinmetz solid as defined in Definition 16 and assume p 2(d − 1)C∞ < 1 − for 2 < d ≤ 5, d φ min 1 ≤ p for 5 < d. 1 + 2(d − 1)C∞ Denote the set of cyclic permutations of (1, . . . , d) with Pd. 2 Lemma 18. There exists an open simply connected region S ⊂ R+ with (0, 0) ∈ S, such that 2 1 1 − φmin (x, y) ∈ S ⇒ Pα(x, y) < for all α ∈ Pd, 2 C∞ 2 1 1 − φmin (x, y) ∈ ∂S ⇒ Pα(x, y) ≤ for all α ∈ Pd, 2 C∞ 2 1 1 − φmin (x, y) ∈/ S ⇒ Pα(x, y) > for at least one α ∈ Pd, 2 C∞ if Assumption 17 holds. Proof. Remark that√ the largest hypercube contained in the Steinmetz solid Sd(r) has edges of length√ 2r/ d − 1, which is equal to the set of points with maximum norm at most r/ d − 1. We have the value r = 1√−φmin , for which the interior of the 2C∞ 1−φmin hypercube is given by the inequality max {φl0} < √ . The upper bound for 1≤l≤d 2(d−1)C∞ all volume fractions is 1−φmin and this is a bound on the hypercube, which implies d ≥ 2 1 + 1/(2C∞) = 5/4. The Steinmetz solid exists only for r > 0. However, the volume 1−φmin fractions have a lower bound φmin > 0, which gives the inequality √ ≥ φmin 2(d−1)C∞ 1 and therefore the condition φmin ≤ √ . Another bound follows from the 1+ 2(d−1)C∞ EXIST. OF WEAK SOL. FOR COUPLED PARAB. AND PSEUDO-PARAB. SYS. 15 lowest value for the maximum. The condition 1 − φmin 1 > = min max {φl0} p d 1≤l≤d 2(d − 1)C∞ d P φl0=1 l=1 √ 2 d−1C∞ implies the condition φmin < 1 − d . The lower bound must satisfy φmin > 0, 2 p 2 which yields d > 2 = C∞ + C∞< C∞ − 2 and conveniently satisfies the d ≥ 5/4 condition. The two upper bounds for φmin are not equal. The last bound is the lesser 2 of the two for d < 2C∞ + 1 = 5, while the second bound is the lesser of the two for 2 d > 2C∞ + 1 = 5. Hence, the minimum of the two upper bounds for φmin guarantees d that there exists a subset of initial conditions in [φmin, 1 − (d − 1)φmin] such that 2 1 1−φmin for all α ∈ Pd we have Pα(0, 0) < . Because all Pα(x, y) are strictly 2 C∞ increasing and continuous functions, we immediately obtain simply connected open sets Sα for each Pα(x, y) for which (0, 0) ∈ Sα hold with the properties 2 1 1 − φmin (x, y) ∈ Sα ⇒ Pα(x, y) < , 2 C∞ 2 1 1 − φmin (x, y) ∈ ∂Sα ⇒ Pα(x, y) = , 2 C∞ 2 1 1 − φmin (x, y) ∈/ Sα ⇒ Pα(x, y) > . 2 C∞ Hence, S = T S . α∈Pd α Now, we only need to prove that we can choose a value V > 0 for which Claim 3 holds. 2 To this end we use the function Q∆t(T∆t − t0,V ) introduced in Appendix A as an Pk j 2 2 2 upper bound to j=0 k∂zv kL2 ∆t. Hence, we need to prove Q∆t(T∆t − t0,V ) ≤ V for all ∆t ∈ (0,H). Assumption 19. Assume 2 4d − 2 H1m max (Kw7 + Kw8) < 1. Γ2 m γ − K φmin m w6m Lemma 20. If Assumption 19 holds, then there exist H∗,V ∗ > 0 and an open 2 ∗ simply connected region R ⊂ R+ with (0,V ) ∈ R such that 2 (x, y) ∈ R ⇒ QH∗ (x, y) < y , 2 (x, y) ∈ ∂R ⇒ QH∗ (x, y) = y , 2 (x, y) ∈/ R ⇒ QH∗ (x, y) > y . 2 2 ∗ Furthermore R ⊂ {(x, y) ∈ R+|Q∆t(x, y) ≤ y } for all ∆t ∈ (0,H ). Proof. Using Corollaries 11, 12 and 14 we obtain: 0 2 4d − 2 2 2 2 Q∆t(x, y) = ∂zv 2 ∆t + 8Γ C (d − 1)cb(x, y) exp(Db(x, y))y L Γ2 ∞ φmin 2 2 H0m 2 2 ˆ2 + Gvx + x max , 4(d − 1)C∞H0mcb(x, y) exp(Db(x, y)) C (x, y) m γm + Dm H2 4(d − 1)C2 H2 c (x, y) exp(D (x, y)) + max 1m , ∞ 1m b b Cˆ2(x, y) , m γm − Kw6m 1 − Kw5m 16 A. J. VROMANS, A. A. F. VAN DE VEN AND A. MUNTEAN with C + 1.6838B Cˆ2(x, y) := (K + K )y2 + A x exp((C + 1.6838B)x) w7 w8 C + B 2 2 2 cb(x, y) := cb1x + cb2y + cb3xCˆ (x, y) + cb4Cˆ (x, y) 2 2 Db(x, y) := max {Db1ly + Db2lCˆ (x, y)}. l6=d−1 Introduce the constants cˆb := cb2 + cb4(Kw7 + Kw8), Dˆ b := max {Db2l + Db3l(Kw7 + Kw8)} l6=d−1 2 2 satisfying cb(0, y) =c ˆby and Db(0, y) = Dˆ by . Since Q∆t(x, y) is differentiable with strictly increasing positive derivative in x and y and strictly positive derivative in ∆t, it is sufficient to prove that there exists a ∗∗ ∗∗∗ 2 region y ∈ (y , y ) for which QH∗ (0, y) < y . Because of the positive derivatives, this result guarantees for all ∆t ∈ (0,H∗) that there exists an open simply connected 2 2 region such that Q∆t(x, y) < y in the region and Q∆t(x, y) ≤ y on the boundary of the region. The function Q∆t(0, y) satisfies the inequality 2 4 2 Q∆t(0, y) ≤ Q∆t(y) = Q0∆t + Q1y + Q2y exp(Q3y ) with 0 2 Q0 = k∂zv kL2 2 4d − 2 H1m Q1 = max (Kw7 + Kw8) Γ2 m γ − K φmin m w6m 2 (4d − 2)(4d − 4) 2 2 H1m Q2 = C∞cˆb max 2Γ + (Kw7 + Kw8) Γ2 m 1 − K φmin w5m Q3 = Dˆ b. If Q1 < 1, as is assumed in Assumption 19, then ∂Q∆t(y) 2 = Q1 < 1. ∂y y=0 By the strictly increasing derivative in y there exists for every ∆t small enough a ∗ ∂Q∆t(0,y) 0 ∗ unique point y such that ∂y2 =: Q∆t(0, y ) = 1, which implies y=y∗ ∗ 2 ∗ 2 ∗ 2 Q1 = 1 − Q2(y ) 2 + Q3(y ) exp(Q3(y ) ) and ∗ ∗ 2 ∗ 4 ∗ 2 ∗ 2 Q∆t(0, y ) = Q0∆t + (y ) − Q2(y ) 1 + Q3(y ) exp(Q3(y ) ). Hence choose ∗ Q2 ∗ 4 ∗ 2 ∗ 2 H = (y ) 1 + Q3(y ) exp(Q3(y ) ), Q0 such that every ∆t < H∗ is small enough to satisfy Assumption 19. Bolzano’s theorem 2 immediately gives the existence of an intersection point between QH∗ (y) and y . EXIST. OF WEAK SOL. FOR COUPLED PARAB. AND PSEUDO-PARAB. SYS. 17 Hence by the strictly positive derivative there exists a unique point y∗∗ ∈ (0, y∗) ∗∗ ∗∗ 2 0 ∗∗ such that QH∗ (y ) = (y ) and QH∗ (y ) < 1. Moreover by the strictly positive ∗∗∗ ∗ ∗∗∗ derivative larger than 1 there exists a unique point y > y such that QH∗ (y ) = ∗∗∗ 2 0 ∗∗∗ ∗∗ ∗∗∗ (y ) and QH∗ (y ) > 1. Hence we have found the interval (y , y ) for which 2 QH∗ (0, y) ≤ QH∗ (y) < y . To be more precise about the implications of Q1 < 1 we need a new assumption. Assumption 21. Assume