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Atmos. Chem. Phys., 8, 637–653, 2008 www.atmos-chem-phys.net/8/637/2008/ Atmospheric © Author(s) 2008. This work is distributed under Chemistry the Creative Commons Attribution 3.0 License. and Physics Observations of iodine monoxide columns from satellite A. Schonhardt¨ 1, A. Richter1, F. Wittrock1, H. Kirk1, H. Oetjen1,*, H. K. Roscoe2, and J. P. Burrows1 1Institute of Environmental Physics, University of Bremen, Otto-Hahn-Allee 1, 28359 Bremen, Germany 2British Antarctic Survey, Natural Environment Research Council, High Cross, Madingley Road, Cambridge CB3 0ET, UK *now at: School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK Received: 23 July 2007 – Published in Atmos. Chem. Phys. Discuss.: 5 September 2007 Revised: 3 January 2008 – Accepted: 9 January 2008 – Published: 11 February 2008 Abstract. Iodine species in the troposphere are linked to methods to determine iodine compounds in the atmosphere ozone depletion and new particle formation. In this study, were initially developed on account of radioactive iodine a full year of iodine monoxide (IO) columns retrieved from isotopes released from nuclear power installations and the measurements of the SCIAMACHY satellite instrument is need to understand their distribution and deposition (Cham- presented, coupled with a discussion of their uncertainties berlain and Chadwick, 1953; Chamberlain, 1960; Chamber- and the detection limits. The largest amounts of IO are found lain et al., 1960). Models for the investigation of tropo- near springtime in the Antarctic. A seasonal variation of io- spheric iodine chemistry further evolved after the recogni- dine monoxide in Antarctica is revealed with high values in tion of significant release of methyl iodide into the tropo- springtime, slightly less IO in the summer period and again sphere (Chameides and Davis, 1980; Chatfield and Crutzen, larger amounts in autumn.
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