Residual Radioactive Contamination from Decommissioning

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Residual Radioactive Contamination from Decommissioning - - - NUREG/CR-55 12 PNL-7994 Vol. 1 Residual Radioactive Contamination From Decommissioning Technical Basis for Translating Contamination Levels to Annual Total Effective Dose Equivalent Final Report Prepared by W. E. Kennedy, Jr., D. L. Strenge Pacific Northwest Laboratory Operated by Battelle Memorial Institute Prepared for I U.S. Nuclear Regulatory Commission ---- I I. AVAILABILITY NOTICE Availability of Reference Matenals Cited in NRC Publicabons Most documents cited in NRC publications will be available from one of the following sources: 1. The NRC Public Document Room, 2120 L Street. NW., Lower Level. Washington, DC 20555 2. The Superintendent of Documents. U.S. Government Printing Office, P.O. Box 37082, Washington, DC 20013-7082 3. The National Technical Information Service, Springfield, VA 22161 Although the listing that follows represents the majority of documents cited in NRC publications. It Is not Intended to be exhaustive. Referenced documents available for Inspection and copying for a fee from the NRC Public Document Room Include NRC correspondence and Internal NRC memoranda; NRC bulletins, circulars, Information notices. Inspection and investigation notices: licensee event reports: vendor reports and correspondence; Commis- sion papers; and applicant and licensee documents and correspondence. The following documents In the NUREG series are available for purchase from the GPO Sales Program: formal NRC staff and contractor reports. NRC-sponsored conference proceedings. International agreement reports, grant publications, and NRC booklets and brochures. Also available are regulatory guides, NRC regulations In the Code of Federal Regulations, and Nuclear Regulatory Commission Issuances. Documents available from the National Technical Information Service Include NUREG-serles reports and technical reports prepared by other Federal agencies and reports prepared by the Atomic Energy Commis- sion. forerunner agency to the Nuclear Regulatory Commission. Documents available from public and special technical libraries include all open literature items, such as books, Journal articles, and transactions. Federal Register notices, Federal and State legislation, and con- gressional reports can usually be obtained from these libraries. Documents such as theses, dissertations. foreign reports and translations, and non-NRC conference pro- ceedings are available for purchase from the organization sponsoring the publication cited Single copies of NRC draft reports are available free, to the extent of supply, upon written request to the Office of Administration, Distribution and Mall Services Section, U.S. Nuclear Regulatory Commission, Washington. DC 20555. CopIes of Industry codes and standards used In a substantive manner In the NRC regulatory process are maintained at the NRC Library, 7920 Norfolk Avenue, Bethesda, Maryland, for use by the public. Codes and standards are usually copyrighted and may be purchased from the originating organization or, If they are American National Standards, from the American National Standards Institute, 1430 Broadway, New York, A NY 10018. DISCLAIMER NOTICE This report was prepared as an account of work sponsored by an agency of the United States Govemment. Neitherthe United States Government nor any agency thereof. orany of their employees, makes any warranty, expressed or Implied, or assumes any legal liability of responsibility for any third party's use, or the results of such use, of any information, apparatus, product or process disclosed in this report, or represents that its use by such third party would not infringe privately owned rights. J NUREG/CR-5512 PNL-7994 Vol. 1 Residual Radioactive Contamination From Decommissioning Technical Basis for Translating Contamination Levels to Annual Total Effective Dose Equivalent Final Report Manuscript Completed: September 1992 Date Published: October 1992 Prepared by W. E. Kennedy, Jr., D. L. Strenge R. A. Meek, Ph.D., NRC Project Manager Christine Daily, NRC -technical Specialist Pacific Northwest Laboratory Richland, WA 99352 Prepared for Division of Regulatory Applications Office of Nuclear Regulatory Research U.S. Nuclear Regulatory Commission Washington, DC 20555 NRC FIN B2908 - Abstract This document is the first volume of a three-volume report to provide generic and site-specific estimates of radiation dose for exposures to residual radioactive contamination after the decommissioning of facilities licensed by the U.S. Nuclear Regulatory Commission (NRC). This first volume provides the details of the generic scenario and pathway modeling analysis. The level of detail included in this volume serves as the basis for user-friendly computer software to be developed under strict quality-assurance procedures. This volume is intended to be used as a reference to Vol- ume 2, a full description of the computer software. Included in Volume 1 are descriptions of the scenarios, models, mathematical formulations, assumptions, and justifications of parameter selections. Volume 1 was produced after consideration of public comments received on the January 1990 review draft. The generic modeling addresses residual radioactive contamination inside buildings and in soils. For buildings, two scenarios are presented to relate volume and surface contamination levels to estimates of the annual total effective dose equivalent (TEDE) or the TEDE (as defined in 10 CFR 20) received during a year of exposure with the conditions defined in the scenarios. Because of concerns regarding potential ground-water contamination from residual radioactive contamination in soil, a generic water-use model was developed to permit evaluation of the annual TEDE for drinking water from wells. The generic water-use model was also used in the evaluation of multiple pathways associated with contaminated soil. The generic treatment of potentially complex ground-water systems used here provides a conservative analysis that may only indi- cate that additional site data and more sophisticated modeling are warranted. The scenarios, models, mathematical formulations, and selected parameter values in this volume are intended to serve as the technical basis for the NRCs derivation of screening values supporting its development of policy applied to residual radioactive contamination from decommissioning. .H.i NUREG/CR-55 12 Contents Page Abstract ............ , ................................................................... iii Executive Summary . ............................................................................. xiii Foreword ........................................... Xv Acknowledgments................................................................................ xix 1 Introduction ............................................ 1.1 2 Methodology and Nomenclature .2.1 2.1 Dosimetry Definitions .2.1 2.2 Symbol Nomenclature .2.2 3 Scenario Descriptions for the Release of Buildings .. 3.1 3.1 Building Renovation Scenario .3.1 3.1.1 Time Frame for Building Renovation Scenario 3.2 3.1.2 Exposure Pathways for Building Renovation Scenario .3.3 3.1.3 External Dose .3.5 3.1.4 Inhalation Dose for Renovation .3.7 3.1.5 Ingestion Dose for Renovation .3.7 3.1.6 Annual TEDE Rate for the Building Renovation Scenario .3.8 3.2 Building Occupancy Scenario .3.9 3.2.1 Time Frame of Building Occupancy Scenario .3.9 3.2.2 Exposure Pathways ........... ..... 3.9 3.23ExtrnaDoe fr Buldig Ocupncy................................................................ 31 3.2.4 Inhalation Dose for Building Occupancy ..................... I .......................... 3.12 3.2.5 Ingestion Dose for Building Occupancy ................................................ 3.13 3.2.6 Annual TEDE Rate for Building Occupancy Scenario: ................................... 3.14 4 Drinking Water Scenario ....................................................................... 4.1 4.1 Water-Use Model ................................ 4.2 4.1.1 Characteristics of Water-Use Model Suitable for Screening .4.2 4.1.2 Three-Box Water-Use Model .4.3 4.1.3 Equations for Radionuclide Transfer in Soil Using the Water-Use Model .4.5 v NUREG/CR-5512 Contents 4.2 Calculation of Annual TEDE .............................. ................................ 4.11 5 Residential Scenario . .......................................................................... 5.1 5.1 Residential Scenario: Concepts and Assumptions ........ ............. ....................... 5.2 5.1.1 Time Frame for the Residential Scenario ............................................... 5.2 5.1.2 Exposure Pathways for the Residential Scenario ......................................... 5.2 5.2 Steps for Calculating Annual Dose from Agricultural Pathways ............. .. .................. 5.5 53 Concentrations and TIansfer Factors for Resuspension and Root Uptake From Soil ...... ......... 5.9 5.3.1 Soil-Plant-Human Pathway ..................... .......................... ....... 5.9 5.3.2 Animal Products Contaminated by Soil Sources ......................................... 5.14 5.4 Concentrations and Transfer Factors for Irrigation Water as the Contaminating Medium .... ....... 5.24 5.4.1 Food Crops Contaminated by Irrigation Water .......................................... 5.24 5.4.2 Animal Products Contaminated by Irrigation Water ...................................... 5.33 5.5 Calculation of Pathway Transfer Factors ......................... ............................ 5.51 5.6 Calculation of Total Dose From Pathways for the Residential Scenario .............. ... ........
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