APPENDIX B-20
EVALUATION OF POTENTIAL HAZARDS OF DEPLETED URANIUM V.
"E77AJWATION OF POTENTIAL HAZAFDS 0V DEPT= UPANIU o 'aximur. Amount of Source Paterial Involved in Each -A Process process at Mn7 One Time ",--Itir'9 500 lbs. Ca t 1mg 500 lbs. :ieat Treatment 200 lbs. 7-, r-• n; 250 lbs.
_*tr-dinr 250 lbs. 2'.,' r' 150 lbs. ,qas-ýiriZ,500 lbs.
...ran•.•u.- presents a two fold hazard: first from its chemical toxicity; e~d scond, frcm the ionizing alpha, beta, and garma radiation emitted in the process of radicactive decay. The ionizing radiations are hazardous or when relatively -,h en srall rcLur.ts of uraniun are taken into the body "ar2,e a*ounts are present in close proximity to the body. However, the c'•<'a yprorerties of uran!u'=. -resent a hazard only after it is absorbed limited Intc the blood streams. rortunately, uranriun is absorbed to n very and its specific extent through unbroken sl:in or the gastronintestinal tract, elements. actlvity is quite low in comparison with most other radioactive Ma.z.T'ful exposures to either hazard can be prevented by careful handling technIques and cc.-on sense. a. External. The isotopes of uranium found in normal or depleted mixtures emit alpha particles accompanied bl' very low energ a rad ation nrc hazarrý in t he nrcces of radioactive decay. The alpha radiaticn nresents low unless the uraniur'. gets into the body. Th•.e ga-rma radiation Is of such no hazard exce-t to parts of the hcd:, in contact energL" that it constitutes time. *Af .Ith larse quantit.es of urcniur. for extended periccds nr ,-3 and chemicýl refiýnn%" the beta particle emissions of UJX, and UTX2 ( 9ý1a23'), the first t;'o dau7ghters of n2U23°, rnre up near, al- the rcnctrat'lrC racli;iticn asszooa.eJ -. w1th'et),= normal cr r'em~lete-l uranlu-.. of rletal sl( I 7-. raitationd dose rate at the surrape2 a bare uranw-. Pnd tre 2r3 nrZr./hr. Te 2.3, •-0 Cevrom 9 P 3a contributes 240 mrer/h•r n. 1 r . 'ev B- from %,Th2&7acds 9nother 20 rmaem/hr. -he gamra ras are ail qu'ut soft and! all tr.ly 2.7 mrem/hr. ••he nelting and casting of urnanlur surface of the resujt In the nigration of the ",71 and IJX2 daughters to the cnst!,. The concentration of these beta. emitters on the interior surfaces of ncl-Is and crucibles, on the exterior surfaces of castings, and in the slag results in dose rates as high as 2 R/hr. These surface deposits are re-cid quicklTy and easily by washinzr resulting In limited exnosure tn rersonnel. ,. Internal. Uranluri ca: g;in access to the "c(:y by way of injection, estion, or inhalation. Alsor1ptlon t)rcu) unbro-e shin is negligible; -rsorption via injection is likely to occur onlyv in such cases as contamina tion of open wounds; and absorpt!:)n via i is a:croximateiv 1% of intake. Inhalan o: uranium ccmtA4s 'F the ;nficant,io mode of entry. Once in the bo raniumt cai cailse d b,' rcj:a-iOn and by chemical toxicity.
c. Chemical Toxicity. Once uranium enters the blood stream in cally active a chemi form, its toxicity i.: comparable to that of arsenic, mercury. Fortunately, lead, or the dusts ri:ost likely to be encountered in industrial processing of uranium are relitively insoluble and so inert physiologically that they are considered as r-idiclorical hazard-; rather than toxic chemicals. These-are deposited prima-ily in the res-liral-cri system from which they are mobilized slowly. The more soluL_,ý corMIpouInd or uranium are quickly taken into the blood stream via lunrs or ccntan,-inatý-J wounds and may result in significant deposits of U0 2 in the kidney. There some of the uranium combines with the protein of cell walls, poisoning the cells and interfering with the vital functions of waste eliminaticn ana maintenance of electrolyte balance. The uranium does not remain fixed in the kidney, but is eliminated at the rate of about half every two weeks. Moderately severe damage to the kidney as a result of acute exposure is reparable, and a return toward normal kidney function may occur even during continued exposure.
d. Radiation Hazards. The principal radiation hazard from internal deposits of uranium is the intense ionization in tissue produced by the alpha particles emitted during radioactive decay. The more than 4 of the alpha particles Mev energy is absorbed in the first 0.1 mm of tissue, resulting in localized cellular damage. On thie otherhand, particles dissipate their gamma rays and beta energies 1n •latively larger volumes of tissue and produce comparatively little dariargj Many industrialF uranium dusts are relatively insoluble and are deposited primarily in the respiratory system. A fixed deposit of uranium in the lung is eliminated at the rate of about half every 120 days.
2. Hazard Control and Evaluation.
a. External. Uranium does not constitute a serious external radiation hazard. The time honored methods for controlling exposure to external sources of radiation are distance, time, and shielding. The intensity of gamma radiation from a point source rapidly decreases with distance away from the source. Beta radiation intensity is decreased even more rapidly with distance. In the case of uranium there is relatively little radiation exposure at a few feet from the material. The length of: time a person may remain in any given area or at any particular jab can be limited on the basis of instrument evalua tions of the radiation conditions. It is not necessary to use massive shield ing or special manipulating devices to decrease exposures in working with normal or depleted uranium. The 2.32 Hev betas from these materials will be stopped completely by about 0.5 in. of water, even less plastic (Lucite), or less than 0.25 in. of glass. A horse-hide leather glove can decrease the radiation dose to the hands as much as 80%.
2 P'17 '.
with t 1. Since the principal health hazard in dealing -mpounds is that of inhalation, the b sic methods of control are andoure ventilation. Depleted uraniun. ptocessilng areas are provided appropriate and special or local ventilation u adequate general ventilation Commercially available respiratory or the kind of operations performed. term high concentra for protection against short protective devices are used that place programs and administrative procedures tions. Educational supplement mechanical handling techniques are used to emphasis on proper in the atmosphere, Usually the sampling of uranium particulates controls. is accomplished by method of evaluating inhalation hazards, the standard of uranium, a filter at a measured rate. The amount drawing air through determined filter from a known volume of air is UX and UX2 collected on the 1 radioactivity. The procedure for by measurement of the alpha and beta follows: determining airborne activity is as air through a filter (1) Air samples are collected by filtering time. Routine spot samples at a known rate of flow and for a predetermined for a 20 minute period. are collected by running the air sampler for holding the (2) Counting technique utilizes a 2" planchet is placed in the planchet and counted sample to be counted. The filter paper for 30 minutes. by the counting time to (3) The total count obtained is divided per minute. determine the counting rate in counts is subtracted from (4) The background ccunt rate of theldetectcr giunts per minutes. the counts per minute to obtain the corrected is divided by the efficiency (5) The corrected counts per minute per minute (dpm). of the detector to determine the disintegrations as follows: (6) The airborne activity is then computed
airborne activity = dpm (2.22 X lO~dpm/uc) (volume of air sampled)
with limits specified (7) The calculated activity is then compared in AEC Reg 10 CFR Part 20. and cast under either a c. Melting and Casting. Uranium is melted all radiation and contamination vacuum or some inert gas. This contains the radioactive daughter during the melt. During melting and casting, They are found mostly in the crucible products segregate from the uranium. This segregation is so pro residues and on surfaces of rough castings. will be found. nounced that very real radiation hazards
LI
3 (1) Melting. The vacuum melting operation is uiique in that the .,grhtO~j oducts of uranium are brought to the surface of the melt and are found In're , the surface of the melt, and the lining of the furnace. 'This radioaco material must be removed. After pouring, the top surface of the ingot is cropped and the sides are machined under local exhaust ventilation. Patching of the furnace lining periodically results another health physics ?roblem in involving external radiation and airborne culate matter. Shielding parti the personnel who perform this job because of the is difficult freedom of movement required for the operation. lead aprons are unsatisfactory. Gloves and One solution is to use a movable aluminum shield which is placed Inside the furnace. Aluminum was chosen higher atomic number since elements produce Dremstahlung radiation to beta radiation. when exposed The beta radiation associated with has an effective the daughter products range of 1100 centimeters. This trate is more than enough to pene the epidermes layer of skin and may potentially cause beta burns. How ever, the aluminum shield is only open in that quadrant in which the worker is either cleaning or patching the lining. Even with the shield, worker must be limited the as to the amount of time spent in Respirators the furnace. are required during the patching operation.
(2) Casting. When graphite crucibles are used they must be machined after for casting uranium, each heat. Considering that the crucible contaminated with radioactive is now daughter products, the ventilation during machining problem operation requires careful consideration. particulate matter Airborne may be far above the MPC. The ventilating this system used for operation utilizes a hood enclosure of a combination of sheet metal and luci 'alastic in conjunction with the exhaust system. d. t Tlatment. No special measures are required operations. for heat treatment
e. Hot Working.
(1) rorging. Health physics precautions are not press forging because stringent in there is very little airborne contamination.
(2) Extrudina. No special health physics precautions are considered necessary with the exception of conducting proper clean up after extrusion was completed. The heating of the billets is conducted in properly vented salt baths.
f. Cold )Jorkin),(Sviaging). ho special measures are required for normal swaging operations.
g. Machining. To maintain the level of airborne particulate below the MPC, all machining uranium operations are provided with local exhaust ventilation. The degree or extent of ventilation varies with the nature, amount, and method of release of the contaminant. All machining is performed under coolant. Since uranium is pyrophoric, a generous supply of coolant is used to flood both the tool and work piece to prevent fires and to reduce airborne contamination. All machines are thoroughly cleaned at least once a month.
4 r-"
ory Protection.
S(I) Respirators are required for all operations in which airborne adi•oactivity concentrations might exceed 10% of the maximum permissible they will be concentrations established in Title 10 Part 20. In addition, worn when directed by the Health Physicist.
(2) The type respirator to be used is the American Optical R-6057 Sure Guard Respirator with the Super Micro-Toxisol R-57 Filter. See Figure I for manufacturer's instructions regarding fitting, cleaning and maintenance of these respirators.
(3) The supervisors are responsible for insuring that personnel are instr.ucted in the proper use of respirators and wear them as required. Work will be programed in such a manner that respirators will not be worn for periods longer than 45 minutes at any one time nor more than 5 hours in any one work week.
(4) Experience has shown that the average concentrations encountered in areas occupied by employees fall within three to five times the MPC established in 10 CFR 20.
FLJAL7.ACI1N 0F P=TLIAL HAZAPDS Or 77.07I.1
. . .r-c.urnt of,. urce "aterial Invclve&ý in Each llrcces.. ".t Tny .. "'--
•.'{-z n. .ds
The thcria is used as P crucible rm-terial because of it7,-.- tr--err -..... ','-st 7.-crci. . .. r.ts no h-zar,.9 In the • u~eK ' r t,'.¶ -"c 7..-. e thoria cruciae is set ½nsl, a tantulhTv cr'r:cb]e ýnr •-'* -. r-turp of 20CC - 23000 0 in a high Vacuur syste7. T t -' 'ru•'r ,- - t_.ct. durrtis the meltinf cycle. T-he crucibles Pre iis'vul u-rp r'c -5 K •r~cweK of as radioactive .... te.
Of-•R--. _ C .- t .. L U. .. APPENDIX C ARGONNE NATIONAL LABORATORY DATA ý\7*rf DOE/EV-0005138 1 0 ANL-OHS/H P-83.108 01 C 'C.,.
FORMERLY UTILIZED MED/AEC SITES REMEDIAL ACTION PROGRAM
RADIOLOGICAL SURVEY OF THE FOR MER WATER WN ARSENAL PROPERTY GSA SITE VVATERTOWN, MASSACHUSEl TS
OCCUPATIONAL HEALTH AND SAFETY DIVISION Health Physics Section ARGONNE NATIONAL LABORATORY, ARGONNE, ILLINOIS
(-f Operated by THE UNIVERSITY OF CHICAGO for the U. S. DEPARTMENT OF ENERGY under Cc'-.ract W.31.109.Eng.38 233 234 m NI 229 0 193 192 191 190 L 230 185 21 18 @7 133
232
235 220 20 238 I 239 237 194 195 196 1971 - 243 241 242 236
0 FEET 30 n SMAR ET ES Q OVERHEAD SMEAR 0 METERSI 0 N AIR SAMPLE
Q GAMMA BACKGROUJN
Fig. 9. Building 234. ANL-IIP Dwg. No. 82-13
f ( ( I
6 5A
v9 9 I 109 J12 120 ,,,©,190 2©@ ,,o2 ,,g(430®- 0 02-8 4o 1 A'" L- 11 57(100 1073ýý 10 11
3/ If ROOM NUMBER
n SMEAR
(D OVERHEAD SMEAR FEET oI- -- 30 ! A
0 METERS 10 N A, AIR SAMPLE
Q GAMMA BACKGROUND
Fig. 10. Building 235. ANL-II1 Dwg. No. 82-12. 174 III Li Li
I 168 169 170 171 172
GARAGE 1 (9 200 199 A 199 OFFICE AREA 2 175 0 RADIO SHOP 3
-E ROOM NUMBER 0 FEET I0 n SMEAR I I 0 METERS 3 N 0 OVERHEAD SMEAR A AIR SAMPLE Q GAMMA BACKGROUND
Fig. I. Building 236. ANL-IlP Dwg. No. 82-14 ( ( 181
1AA
1o 179
N
0 FEET I0 -- - - Im.- n SMEAR
0 METERS 3 /A AIR SAMPLE
Q GAMMA BACKGROUND
Fig. 12. Building 237. ANL-IIP Dwg. No. 82-15 37
TABLE 2
AMBIENT RADIATION LEVELS
Duration of Radiation Level Corresponding 0 Location Measurement RSS-111 PRM-7 Measurement Area No. Grid (h) (pR/h) (PR/h)
INTERIOR
Bldg. 234 18 65.5 8.9 7 Bldg. 235 11 4.0 8.8 7 12 3.0 8.3 7 13 4.0 9.0 8 14 3.0 10.2 8 16 3.4 8.9 8 17 4.1 9.4 8 19 6.0 11.2 8 Bldg. 236 15 6.2 8.6 8
Bldg. 237 20 4.1 8.8 8 ------EXTERIOR I 1 M-2 2 M-2 2.5 11.6 13 II 3 .-- 3 4.5 9.8 7 4 K-3 2.1 11.7 10 7 H-2 6.2 7.5 IlI 5 5 H-3 3.0 10.7 9 6 F-4 3.8 12.6 11 10 E-4 2.3 10.0 10 IV 9 1-1 2.5 10.2 10 V 8 0-2 1.8 9.6 10 21 Q-2 2.9 14.6 15 22 Q-1 3.1 12.4 12 aLocations are shown on maps in Figures 5 and 9 through 12. 38
TABLE 3 a RADON-CONCENTRATION DETERMINATIONS
Radon Air Sample b (2i/£ pCi/9 Number Location
0.74 4 Building 235, 0.0074 -Room 1
0.65 5 Building 235, 0.0065 Room 2
1.02 6 Building 235, 0.0102 Room 3 East
0.85 7 Building 235, 0.0085 Room 3 West
0.38 8 Building 235, 0.0038 Room 5
0.58 9 Building 235, 0.0058 Room 10
0.46 10 Building 236, 0.0046 Office
0.15 11 Building 236, 0.0015 Garage
0.04 12 Building 237, 0.0004 Shed
0.06 13 Building 236, 0.0006 Radio Shop
0.10 14 Building 234, 0.0010 East
0.96 15 Building 235, 0.0096 Pistol Range
0.27 16 Building 234, 0.0027 Center
0.54 17 Building 234, 0.0054 West 39
TABLE 3 (coat'd.)
Air Sample Number Location WLb
18 Building 237, No actinon Shed
20 c Building 236, No actinon Garage
Building 235, No actinon Room 3 Center
22 Building 234, No actinon Center
aLocations are shown on maps in Figures 9 through 12. b A Working Level (WL) is defined in 10 CFR 712 as any combination of short-lived radon-daughter products in 1 liter of air that will result in the ultimate emission of 1.3 x 105 MeV of potential alpha energy. The numerical value of the WL is derived from the alpha energy released by the total decay through RaC' of the short-lived radon-daughter products, RaA, RaB, and RaC at radioactive equilibrium w'ith 100 pCi of 222Rn per liter of air.
Actinon determination. TA ILE) DATA SHEET OF AREA SURVEYS I Window~EndI Percent of Area I'AC 4G-3 8 Accessible Air Direct Rleadings (M PRiM-7 PRM-5-3 Smear flesultr. Room or for Survey Sample (dis/nin-l0O cmI) (miR/h) (pR/h) w/PG-2 (dim/min Area No. Floor Wall (WL) Both Alpha Contact I meter (cts/rain) 100 cml) Comments
AREA 1: 2 cm IlKGI) 0.8 40 45000 100 34 I000 2 c-m 50000 100 2500 RKGI 0.03 40 35 2 c-m 20000 100 400 KGDI) 0.03 30 36 2 100 cm 500 BK(;I) 0.07 10 10000 37 100 0.04 20 3000 )00 2 38 Cm 10000 ( 100 15000 0.2 20 39b 2 100 cm b 5.0 20 35000 4 0 50000 400 2 cm ( 100 0.1 20 5000 w- 41 2000 2 100 cm FIKGI) 0.1 20 5000 42 500 100 BKGI) 0.15 20 15000 43 3000 100 BKGI) 0.5 20 15000 3000 2 44 Cm 100 20 10000 2000 100 0.6 45 2 20 5000 < 100 cm 500 BKGI) 0.05 46
AREA I:I
< 700 CM2 BKGI) 0.14 30 30000 47-53, N-ý 4500 2 50000 < 200 cm b 451000 250 7.0 30 54 , 60, N-3 TABLE I DATA SHIEET OF AREA SURVEYS
I 1 1 - Percent of Aroa PAC 4G-3 End Window Accessible Air Direct Rnoadinsa GM PRM-7 PRM-5-3 CImOar Resultr floom or for Survey Sample (dlis/ in-100 crul) (mR/h) (pR/h) w/PG-2 (dis/rnin Area No. Floor Wall (WI1) srpin Alpha 1 mnoler 10[) era1 Contact (cts/nin) Cormnin n t r, . 100 C.1...
55-5 7, N-3 IlKG(I) 2 0.7 30 30000 1100 cm 59, 61-63, 25010101 )00 0.7 2 N-3 30 50000 47000 cm
58, H-3 400 IK(;I) 2 0.03 30 2000 900 cm 71, L-2 300 OK OIl 0.03 2 30 2100 3700 cm 64-66, L-3 BK(;1) 1000 0.08 30 2 10000 < 300 cm 67-70, K-3 HKGI) 0.02 30 50000 < 400 CM2
AREA III t-n General 11K(;ID 1000 1(0GD I0 2000
AREA IV General 500 IKGD 20 3000
AREA V
72. 73, 2510 2 "1K(;I) 0.03 20 10000 < 300 cm 77, N-I
( ( TABLE 1 DATA SHEET OF AREA SURVEYS
i'AC 4G-3 Window PercentAccessible of Aiea Air Direct Readingsa GM PRM-7 PRM-5-3 Smear Results
Boom or for Survey Sample (dis/min-100 cml) (mR/h) (pn/h) w/PG-2 (diu/min Area No. Floor Wall (WL) fla Alpha Contact I meter (cts/min) 100 cmI) Comments
AREA V
(cont'd.)
2 cM 74-76, N 15000 PK(;I) 3.0 20 25000 ( 300 2 flK(WD 3000 300 cm 79-82, 0 250 0.04 20 2 2000 100 78, 0-2 250 0.04 20 Cm BKGD 2000 ( 100 2 83, P-I 250 0.03 20 cm BK(;,D 0.03 20 3000 ( 100 89, P-2 250 2 cm BKGI) 0.03 20 2000 100 84, Q-I 250 2 HKGI) cm aI' 0.03 20 7000 300 85-88, Q- 400
All instr ment reii ings I clude bardgrounds (P4 C-4GR, 250 4im, PRM-!-3, 400 cpni. G", 0.03 mR, I'RK-7, I'I pR).
b etsl chills were 4ound at these loc tLi oilii.
t" "Grid loclkions arq shown n Fipt,,re 37
TABLE 2
A{fBIEN-T RADIATION LEVELS
Duration of Radiation Level Corresponding a Location Measurement RSS-11l PRM-7 Measurement Area No. Grid (h) (pR/h) (pR/h)
INTERIOR
Bldg. 234 18 65.5 8.9 7
Bldg. 235 11 4.0 8.8 7 12 3.0 8.3 7 13 4.0 9.0 8 14 3.0 10.2 8 16 3.4 8.9 8 17 4.1 9.4 8 19 6.0 11.2 8
Bldg. 236 15 6.2 8.6
Bldg. 237 20 4.1 8.8 ------10P EXT.ERI OR I 1 M-2 3.3 17.7 34.
2 M-2 2.5 11.6 13 !I 3 M-3 4.5 9.8 7 4 K-3 2.1 11.7 10 7 H-2 6.2 7.5 5 III H- 3 5 3.0 10.7 9 6 F-4 3.8 12.6 11 10 E-4 2.3 10.0 10 iv 9 1-1 2.5 10.2 10 ',7 8 0-2 1.8 9.6 10 21 Q-2 2.9 14.6 15 22 Q-I 3.1 12.4 12
TLocations are shown on i-aps in Figures 5 and 9 through 12. 38
TABLE 3
RADON-CONCENTRATION DETERMINATIONS
Radon Air (2i/£ Sample b Location Number
0.0074 0.74 4 Building 235, -Room 1
0.0065 0.65 5 Building 235, Room 2
0.0102 1.02 6 Building 235, Room 3 East
0.0085 0.85 7 Building 235, Room 3 West
0.0038 0.38 8 Building 235, Room 5
0.0058 0.58 9 Building 235, Room 10
0.0046 0.46 10 Building 236, Office
0.0015 0.15 11 Building 236, Garage
0.0004 0.04 12 Building 237, Shed
0.0006 0.06 13 Building 236, Radio Shop
0.0010 0.10 14 Building 234, East
0.0096 0.96 15 Building 235, Pistol Range
0.0027 0.27 16 Building 234, Center
0.0054 0.54 17 Building 234, West 39
TABLE 3 (cont' d.)
A: r Sample Number Location WLb
16Cc U, I -; No actinon Shed c 2 0 Building 236, No actinon Garage
Building 235, No actinon Room 3 Center
Building 234, No actinon Center a Locations are shown on maps in Figures 9 through 12. b A Working Level (WL) is defined in 10 CFR 712 as any combination of short-lived radon-daughter products in I liter of air that will result in the ultimate emission of 1.3 x I10 MeV of potential alpha energy. The numerical value of the WIL is derived from the alpha energy released by the total decay through RaC' of the short-lived radon-daughter products, RaA, RaB, and RaC at radioactive equilibrium W- 100 2 2 2 th pCi of Rn per liter of air. cActinon determination. TABLE 4
(;AMtIA SIECIIAL AND URANIIUR FLUOROME'RIC ANALYSES OF SOIL SAMIPLES
Gatunn Sjpectra, yCi/&!-J
2 32.rI, 226H, Fluorouetric a Decay Decay Uranium Sample 3 (Chain Chain PR/8 1 10% pCt/g 1 10% No. 1 7c
SOIL COHINGS
33.4 :1 1.36 ± 0.09 824.0 t 82.4 334.0 t b I-S47-A 1.54 f 0.11 1.03 0.07 ± 902.0 90.2 0.07 1.21 ± 0.09 2227.0 222.7 B 1.96 t 0.14 1.04 ± 2 9 . b ± 1 .52 ± 0.11 736.0 ± 73.6 298.0 b 0.53 0.05 0.86 t 0.07 C 46.2 ± 4.6 18.7 1.9 <0.03 0.35 1 0.07 0.62 ± 0.06 D ± t 241.0 t 24.1 1.03 1.60 t 0.11 595.0 t 59.5 1-548-A 1.10 ± 0.08 t 0.07 48.4 196.0 t 19.6 t 0.09 1.89 ± 0.13 484.0 ± B 0.79 0.07 1.33 40.5 41. ± t t 0.13 100.0 t 10.0 0.04 1.24 0.09 1.81 C 0.24 ± 47.0 t 4.7 19.0 1.9 0 0.98 ± 0.07 1.53 t 0.11 D 0.08 0.03 ± 151.0 15.1 b 1.21 t 0.12 372.0 37.2 ± b 1 .48 ± 0.15 i-549-A 1.08 it 0.11 t 412.0 ±f 41.2 167.0 ± 16.7b it 1 .62 ± 0.16 0.92 0.09 B 0.90 0.09 88.3 ± 8-8b 1.30 ± 0.13 218.0 t 21.8 0.05 I .05 it 0. 11 C 0.51 it ± 84.3 8.4 34.1 t 3.4 1 .08 it 0.11 I .•4 0.10 ± D 0.29 0.03 ± b it 16-3b 0.83 0.08 403.0 40.3 0. 10 0.67 it 0.07 it 163.0 1-S50-A 1.03 761 .0 ± 76.1 308 .0 ± 30.8b 0.83 it 0.08 0.97 0.10 B 0.67 0.07 ± 348.0 ± 34.8b it 1.03 0.10 859.0 85.9 0.05 0.73 it 0.07 ± ± ± 25.8 C 0.53 it 637.0 63.7 258.0 0.87 it 0.09 1 .40 0.14 D 0.63 0.06 ± ± it 2.4 1.6 ± 0.2 it 0.0 7 1 .08 0.11 ± 0.2 0.33 0.03 0.70 ± 1 it 0.2 I-S51-A it 0.10 3.3 0.3 2.3 0.78 it 0.08 1 .00 ± ± B 0.70 it 0.07 3.8 0.4 2.6 ± 0.2 1.18 0.12 ± 0.10 1.01 it 0.10 ± it 0.2 C 1.01 it 0.10 2.2 0.2 1.5 0.84 it 0.08 0.97 D 0.35 0.04 ± ± ± 4.4 ± 0.4 1 0.19 0.6 I .25 it 0.13 .85 it 6.4 ± !-S52-A 1.12 it 0.11 5.2 0.5 3.6 ± 0.4 0.14 1 .84 0.18 ± 0.81 o.08 1.36 it 3.0 it 0.3 B it 't 0.18 4.4 0.4 1.22 "t 0.12 1 .76 ± C 0.58 it 0.06 't 1.9 0.2 1.3 £ 0.2 .010 it 0.10 0.90 0.09 D 0.04 0.02, TaI'iie 4
(uoniSii.d . )
Giminn Spec-tra1 jpCI/8ti•
2 24BRaq Sample Iirca y Uraniim 1'luoronetci/ No. I 37c(:t Chai iti CIh I n Pg/g ± (lPci/g f 107. I-$53-A 1.91 0.19 0. 76 (I. OR 1 .35 7 . 0 B it 00.14 0.7 3.9 t 0.4 2.11 0.21 1 .20 0. 12 2.02 - 0.20 5.7 it 0.6 C 4 3.9 I .42 0. 14 1.15 0.12 1 t it .60 ± 0.16 3.7 0.4 2.5 ± 0.3 D 0.20 0.04 1.26 + 0. 13 1.61 i0. 16 2.4 0.2 1.6 1 0.2 it I-S54-A 2.49 0.25 0.67 0. 07 it 1.10 .t 0. II 10.6 1.1 5.2 0.5c B 2.68 0.27 it it 0.96 0. I0 1 .20 0. 12 6.6 0. 7 3.6 0.4 itit C 0.59 0.06 0.94 0.09 1.12 0.11 0.2 it it 2.9 0.3 2.0 ± D it it 0.12 0.04 I .44 it 0. 14 1.15 0.12 2.1 it 0.2 1.4 0.2 it it 1± I-S55-A 1 .55 0.16 1.10 0.11 it 0.2 it 0.49 0.05 1.8 ± 0.2 1.2 B 1.74 0.17 1 .20 0.12 0.88 +. 0. 09 it 2.6 0.3 1.8 it 0.2 C 1 .62 0.16 I. 00 0.10 4 it '-. it 1.31 0.13 4.4 0.4 3.0 it 0.3 D 0.36 0.04 1.51 it 0. 15 1.31 0.13 2.2 0.2 1.5 0.2
I -956-A 0.20 0.04 <0.06 0.15 it0.05 <0.7 8 0.03 0.04 (1.0 0.11 0.05 <0.02 <1 .0 <0. 7 C 0.21 0.04 it 0.34 it 0.06 0.53 it 0.05 (1.0 <0.7 D 0.13 0.04 1. 05 it 0. 11 1.35 f 0.14 2.0 it0.2 1.4 t 0.2
I-S57-A 5.01 0.50 <0.06 it 0.91 0.09 2.1 it 0.2 1.4 it 0.2 B 7.80 0.78 0. RO 0.08 it 1.15 it 0.12 1.8 it 0.2 1.2 it 0.2 C 2.35 0.24 1.07 0.11 1.12 0.11 1.7 it 0.2 1.2 it 0.2 D 0.99 0.10 0.70 0.07 it 1.20 it 0.12 2.1 it 0.2 1.4 it 0.2 it it I-S58-A 1.44 0.14 I .38 0.14 it 0.80 0.08 1.9 it 0.2 1.3 it 0.2 B 1.65 it 0.17 it 0.94 0.09 0.88 0.09 1.9 it 0.2 1.3 0.2 it it C 0.93 0.09 1.10 0.11 1 .24 0.12 1.8 0.2 t it 1.2 0.2 D 0.45 1.06 it 0.05 0.11 1.01 0.10 1.7 0.2 1.2 0.2
( TA F1F. 4
G a cnctJra)Ci r a [&to
232-11, 22nRa Sample D)ecay Decay Urniijum Fluorometric No. asic, Chla Ii Ch init Pg/g ± 1O% pCi/g t 10%
1-559-A 1.55 ± 0.16 0. 1 1 1.86 0.19 4.2 0.4 2.9 ± 0.3 B 2.74 t 0.27 1.18 0. 12 1.72 0. 17 4.8 0.5 3.3 £ 0. 1 C 2.27 t 0.23 0.68 0.07 1.46 0.15 3.6 0.4 2.5 ± D 0.33 t 0.04 0.3 1.11 0.11 2.01 0.20 3.6 0.4 2.5 ± i-S60-A 5.19 t 0.52 1.47 0.15 2.07 0.21 3.9 0.4 2.7 ± 0.3 B 3.48 t 0.35 2. 1Q 0.22 3.39 0.34 6.9 0.7 4.7 ± 0.5 C 0.78 t 0.08 3.32 0.33 4.85 0.49 8.9 0.9 6.1 ± 0.6 ± D 0.20 0.04 1 .09 0.11 1.45 0.15 2.5 0.3 1.7 ± 0.2 ± I-S61-A 0.97 0.10 1.15 0.12 0.81 0.08 2.3 0.2 1.6 ± 0.2 ± B 0.62 0.06 I .39 0.14 0.73 0.07 2.5 0.3 1.7 ± 0.2 ± C 0.61 0.06 0.88 0.09 0.76 0.08 2.6 0.3 1.8 ± 0.2 D 0.95 0.10 1 .03 0.16 0.84 0.08 3.0 0.3 2.1 ± 0.2
it 1-$62-A 1.10 0.11 1 .59 0.16 1.10 0.11 27.0 2.7 11.8 ± 1.2c ± B 0.50 0.05 0.80 0.08 1.67 0.17 15.5 1.6 7.6 ± 0.8c ± C 0.11 0.03 1 .28 0.13 1.20 0.12 4.6 0.5 3.2 ± 0.3 D <0.03 0.90 0.09 1.21 0.12 2.5 0.3 1.7 ± 0.2
1.63 t 0.16 0.07 1 0.04 1.34 ± 0.13 1.9 1 0.2 1.3 ± 0.2
0.48 1 0.05 1.75 ± 0. I0 3.84 t 0.38 962.0 ±96.0 390.0 139.0
SOIL. BORINGS
1-SI7-1 0.23 ± 0.04 0.58 t 0.06 0.72 ± 0.07 3.5 it 0.4 2.0 ±" 0.2c it it 2 0.30 0.04 0.73 0.07 0.43 0.04 3.8 it 0.4 1.9 0.2 it it 0.34 0.04 0.49 t 0.05 0.36 0.04 1.1 it 0.1 0.8 0.1 4 it it i" 5 0.51 0.05 1.21 t 0.12 0.78 0.08 2.6 it 0.3 1.8 0.2 ± it it 6 0.17 0.04 0.83 0.08 0.74 0.07 2.6 0.3 1.8 it 0.2 1AII.E 4 (( -nlt , d. )
t;RhIw1l,1 j f( Liii, j'L. I /$J
213 11h 22n in SAmple I~rn y Ilech y Utrlijum Fll1oromietric No. 37Cp, (:hn t n c hmi IR/R t 10% I)Ci/g ± 10% 1-578-1 0.35 ± 0.04 2.29 0. 23 2.42 0.24 11.2 ± I1 2 ± 6.5 t 0.7" 0.57 1 0.06 1. 14 0.11 I.II 0.11 8.3 ± 0.8 4.3 t 0.4c + 3 0.57 ± 0.06 3.66 0.37 2.32 0.23 7.5 ± 0.8 5.1 f 0.5 4 0.21 t 0.03 4. 1 .98 0.20 1 .69 0.17 3.0 + ± 0.3 2.0 ± 0.2 5 0.24 ± 0.03 1 . 76 0. I8 I .76 0.18 3.2 ± 0.3 it 2.2 t 0.2 6 0.25 ± 0.04 I .82 it 0. i8 1 .69 0.17 3.6 ± 0.4 2.5 ± 0.3 4` ± 1-S79-1 0.53 it 0.05 1.65 0.17 ±t 1.78 0. 18 22.5 it 2.3 10.6 2 0.44 it 0.04 it 1.1 1 .29 0. 13 1.25 0.12 4.9 it 0.5 it it ± 2.9 0.3 3 0.18 0.04 0.15 0.05 0.29 0.03 0.9 it 0. 1 0.6 it 0.1 4 1.70 it 0.17 0.33 it 0.07 0.68 S.3 it 0.1 it it 0.07 0.9 0.1 5 <0.03 0.23 0.04 0.60 + 0.06 2.0 it 0.2 0.1 6 <0.03 it 1.4 .r- 1.15 0.12 0.69 1.6 0.2 + it 0.07 i. 1 0.1 !-980-I 0.36 t 0.04 0.89 t 0.09 1.07 it 0.11 23.3 2.3 C 2 10.3 it I . o <0.03 1 .85 t 0.19 2.10 ± 0.21 6.7 0.7 4.4 0.4 3 <0.03 <0.06 0.48 it o .05 1.7 + 0.2 1.2 4 <0.03 0.68 t 0.07 it 0.38 0.04 4.1 + 0.4 2.0 0.1 5 it 0.14 1.35 1.01 it 0. 10 1 .48 + 0.15 7.0 + 0.7 4.0 it 0.24 6 0.22 i 0.02 0.98 ± 0. 10 + 0.60 0. 06 7.4 + 0.7 3.5 0.4c
1-S 1-I 0.20 0.04 0.95 0. 10 1 .41 0.14 622.0 it 62.2 252.0 1t25.2 2 0.77 0.08 0.24 0.02 I .36 0.14 1400.0 it140.0 567.0 ±56.7 4 0.22 0.04 0.60 4. 1.44 it 0.06 0.14 232.0 + 23.2 94.0 i 9.4 5 0.34 0.03 0.78 it 0.08 4` 0.83 0. OR 101.0 it 10.1 40.9 6 <0.03 0.60 it 0.06 1 0.1") 1 1.19 0.12 14.2 1.4 6.7 it it 1-$82-1 0.57 it 0.06 1 .32 it 0.13 1.06 it 0.11 119.0 + 12.0 48.2 2 0.51 0.05 1 .42 0.14 1.15 0.12 62.4 6.2 fit it +` 25.3 2.Ab 3 0.88 0.09 1.18 0.12 1.17 0.12 it it it 54.3 5.4 22.0 2.2 4 0.21 0.02 I .35 0.14 0.74 4. 0.07 10.4 1 . 0 4.8 it 0.5 5 it 0.21 0.02 0.25 0.05 0.36 0.04 2.0 0.2 1.4 it 0.2
6 0.25 i 0.02 0.63 t 0.06 0.79 it 0.08 1.6 t 0.2 1.1 t 0.1 ( ( TABILE 4 (cont'd.)
Gammsn Spc~ctra. PCi/pit?
2 3 2 Th 2 2 Oia
Sample Deciay Decay Uranium Fluorometric 7 No0. 13 Cu Chlion ch ain,| pg/K 1 10% pCi/R ± 10C I) 1-883-1 0.08 4 0.05 0.60 ±. 0.06 1.13 0.11 136.0 ±. 13.6 55.1 ± 5.5 2 0.37 1 0.04 o.61 ± 0.06 1 .56 0.16 928.0 ±. 92.8 376.0 :t37.6 ± 3 <0.03 0.31 ± 0.09 0.60 0.06 33.4 ±. 3.4 13.5 ± 1. 4 I 4 <0.03 0.34 ±. 0.07 0.83 t 0.08 15.2 ±. 1.5 6.8 1 0.7 .± ± ±. 5 <0.03 0. 13 0.05 1 .04 0.10 39.0 3.9 15.8 4. 1.6 b 6 0.08 ± 0.05 0.46 ±. 0.07 0.99 0.10 35.9 ±. 3.6 14.5 t 1.5 ± ±. ±. !-S84-1 0.90 0.09 0.89 0.09 1.06 ±t 0.11 257.0 26.0 104.0 ±10.4 ±. ±. ±. 2 0.35 ± 0.04 1.07 0.01 1 .35 4.t 0.14 136.0 14.0 55. 1 t 5±.5 ± ±. "±" 3 0.63 I 0.06 1.14 0.11 0.28 4± 0.03 8.9 0.9 3.6.±t 0.4 ±. ±. 5 0.13 0.03 0.73 0.07 0.91 ±. 0.09 6.1 0.6 3.2 ± 0.3 ±. ±. 6 <0.03 0.58 0.09 1.01 0.10 5.8 0.6 3.2 ± 0.3 4
±.28.b 1-185-1 3.62 t 0.4 0.94 ± 0.09 0.68 0.07 710.0 ± 71.0 288.0 2 0.68 0.07 1.75 0.18 1.62 0.16 1452.0 ±145.2 588.0 ±58. 8 ± 3.81 ± 0.38 2.42 0.24 254.0 t 25.4 70.1 "t 7.0 3 0.47 0.05 b 4 0.23 0.02 0.40 0.08 1 .00 0.10 27.4 ± 2.7 11.1 ± 1.1b ±. 5 0.38 ± 0.04 1 .46 0.15 1.07 t 0.11 18.9 ± 1.9 7.6 ± 0.8 t t t" 0.4b 6 0.47 0.05 0.62 t 0.06 0.78 ±.± 0.08 10.1 ± 1.0 4.1 ± t ±.t b ±. I-586-1 0.57 ± 0.06 0.36 ±. 0. 07 0.78 I 0.08 393.0 39.3 159.0 ±15.9 ±. 597.0 ±. t.24. 2 1.18 1 0.12 0.57 0.09 1.41 0.14 59.7 242.0 2 ± t ±. ±. b 3 0.55 1 0.06 1.12 ±. 0.11 1 .04 0.10 33.5 3.4 13.6 ± ±. 8.1 f. 0.8 b 4 <0.03 1.18 ± 0.12 1.25 0.12 19.9 2.0 ±. ± 0.4 5 0.03 ± 0.02 o.84 ± 0.08 1 .30 0.13 8.2 4± 0.8 4.4 6 <0.03 0.56 0.08 0.90 ±. 0.09 2.4 0.2 i.6 ± 0.2 ± ± ±. 1-$87-1 1 .00 ± 0.10 1.74 ± 0. 17 11.02 1.10 14.1 ± 1.4 9.6 f 1.0 :t ±! 2 0.19 t 0.02 1 .03 0.10 1.72 0.17 2.4 ± 0.2 1.6 t 0.2 ±. ±. ±" 3 0.42 t 0.04 I .56 0.16 2.11 0.21 4.5 "± 0.5 3.1 0.3 ±. -t ±. 4 0.15 0.04 2.21 0.22 2.32 0.23 5.7 ± 0.6 3.9 0.4 5 0.15 ± 0.04 2.15 0.22 2.44 0.24 5.8 0.6 4.0 0.4 4.4 1. 0.4 f. 6 0. 13 f. 0.03 2.35 1 0.24 2.05 ± 0.20 3.0 0.3 lABLl.E 4 (-o ll 'i . )
(3nnwna SJ eCArn, pCi/gIu
232Thi 22f3Rt Sample lIeray I)eray Urnnium Fluorometric Me. 1-3 C7 Chlin Clhbnini I'R/R ± I o pCi/a if I(IV
I-S8-I 0.76 ± 0.08 0.65 4 0.06 1.03 0. 10 9.0 ± 0.9 4 4.5 it 0.4 2 0.29 it 0.04 0. 14 1 40 ± 1.06 0.11 4.8 4+ 0.5 2.8 0.3 3 1 .24 ± 0.12 0.33 4 ± 0. 10 1 .21 0.12 3.0 ± 0.3 2.0 it 0.2 4 ± ± 0.36 0.04 0.99 0. 10 0.93 0.09 2.9 ± ± ± 0.3 2.0 0.2 5 0.61 £ 0.06 2.04 0. 21 + 1.77 0.18 3.8 0.4 2.6 0.3 6 ± ± 1.19 0.12 2. 1 0.22 2.65 0.26 3.7 0.4 t 4 2.5 0.3 it ± 1-589-I it 0.15 t 0.04 0.57 0.09 0.56 0.06 8.7 0.9 t ± 4.0 0.4 2 0.16 1 0.04 0.08 0.04 it 0.3c t 0.40 0.04 5.5 it 0.6 2.6 3 <0.03 0.48 ± 0.07 0.89 0.09 3.2 0.3 2.2 4 t ± 0.2 0.11 t 0.03 0.50 0.08 0.89 0.09 2.1 it t ± it 0.2 1.4 0.1 5 0.33 t 0.04 0.67 it 0.07 0.75 0. 0R 1.8 it 0.2 1.2 0.1 6 ± 0.33 it 0.04 0.83 0.08 0.99 0. 10 2.4 ± 0.2 it ± 1.6 0.2 1-990-1 1.50 t 0.15 1.14 0.11 1.07 0.11 42.3 it 4.2 17.1 t 1.7b 2 ± 0.21 -i 0.04 0.70 0.07 0.82 0.08 6.6 it 0.7 ± 3.3 itf (1.3 3 0.15 i 0.04 0.47 it 0.09 0.73 0.07 3.7 it 0.4 ± 2.1 0.2c 4 <0.03 0.71 0.07 0.75 0.08 1.4 it 0.2 1.0 0.1 t ± 5 0.14 0.04 1.12 0.11 0.85 0.08 1.8 it 0.2 ± 1.2 0.1 6 0.06 t 0.02 <0.06 0.78 0.08 1.7 ± 0.2 it ± 1.2 0.1 it 1-S91-1 0.44 ±- 0.04 2.96 0.3(0 3.61 0. 36 11.6 ± it it 1.2 7.9 it 0.8 2 0.03 t 0.02 !.13 0.11 4 0.91 0.09 2.5 it 0.3 1.7 ± Itit 0.2 3 <0.03 I .43 0.14 I .29 0.13 2.8 it + it 0.3 1.9 0.2 4 <0.03 2.21 0.22 it 0. 1 it 1.70 0.17 3.7 it 0.4 2.5 5 <0.03 0.43 ± "it 0.06 0.39 0.04 2.2 t 0.2 1.5 0.2 6 ± <0.03 1.72 0.17 1.02 0.10 4.4 it 0.5 ± 3.0 0.3
( ( TABLE 4 E(-ont' d. )
Garga Sj ectra, plgi_/Ao
232Th 22ORS
Sample Decay Decay Uranium Fluorowetric 1 No. 37C, Chain Chain pg/g f 10% pCi/K 1 10%
I-S92-1 BIDLR 2.84 ± 0.28 13.66 t 1.37 1.4 t 0.2 1.0 t 0.1 2 0.19 t 0.06 2.08 t 0.21 11.67 t 1.17 2.5 t 0.3 1.7 t 0.2 3 0.14 f 0.04 0.94 t 0.09 4.44 1 0.44 2.3 t 0.2 1.6 t 0.2 4 0.09 - 0.04 0.93 t 0.09 1.98 t 0.20 1.9 t 0.2 1.3 t 0.1 5 BDL 0.35 1 0.07 0.97 ± 0.10 1.0 1 0.1 0.7 t 0.1 6 BDL 0.55 t 0.08 0.87 t 0.09 1.2 t 0.1 0.8 1 0.1
t i-$93-1 0.25 t 0.04 0.79 1 0.08 1.65 ± 0.16 2.7 1 0.3 1.8 0.2 2 0.22 1 0.04 0.92 1 0.09 1.34 t 0.13 2.0 ± 0.2 1.4 1 0.2 3 0.04 ± 0.02 1.10 t 0.11 1.32 t 0.13 2.3 1 0.2 1.6 t 0.2 4 <0.03 0.83 ± 0.08 0.95 ± 0.10 2.9 ± 0.3 2.0 1 0.2 ± 5 <0.03 1.06 t 0.11 1.72 t 0.17 3.3 t 0.3 2.3 0.2 t 6 0.03 t 0.02 0.95 t 0.10 1.28 t 0.13 2.7 1 0.3 1.8 0.2
l-S94-1 0.63 t 0.06 2.08 ± 0.21 5.54 t 0.55 17.8 ± 1.8 12.2 t 1.2 t 0.7 2 0.03 t 0.02 1.63 t 0.16 7.99 ± 0.80 10.3 1 1.0 7.0 t 9.6 t 1.0 3 0.17 t 0.05 1.15 1 0.12 3.44 t 0.34 14.1 1.4 1.6 t 0.2 4 <0.03 - 1.46 ± 0.15 2.4 ± 0.2 t 0.2 1.2 t 0.1 5 <0.03 0.77 ± 0.08 1.23 t 0.12 1.8 ± 1.6 1 0.2 6 <0.03 0.58 ± 0.09 1.85 ± 0.18 2.4 0.2
t 0.3 1.8 1 0.2 i-595-1 0.55 t 0.06 2.18 f 0.22 5.04 t 0.50 2.6 1 2.0 t 0.7 2 0.12 f 0.04 1.88 1 0.19 4.24 1 0.42 2.9 0.3 t 0.2 1.6 t 0.2 3 0.28 t 0.04 1.76 ± 0.18 4.14 t 0.41 2.3 ± 2.8 ± 0.3 4 0.09 t 0.04 0.97 1 0.10 2.41 ± 0.24 4.1 0.4 4.3 ± 0.4 2.9 t 0.3 5 0.15 ± 0.04 0.31 1 0.03 2.09 t 0.21 t 9.2 t 0.9 6 <0.03 1.00 1 0.10 4.18 t 0.42 13.5 1.4
1 1-R96 f BDL 274.0 ±27.0 215.0 122.0 708.0 71.0 483.0 ±48 TAIIIE 4 (cfjmt d'. )
(;Ofvnun_ pcupc~ l
2321h 226pa IVrcay S mple IDecay 1 7 Urnnlum FbjoromeLrjc No. a. Cn Cha I ) Chain I'R/R ± I0% pCi/R 1 10%
1-597-A 0.84 ± O.O0 0.R5 t 0.08 1.01 1 0.10 3.4 ± 0.3 2.3 t 0.2 B 0.24 t 0.05 1.11 f 0.11 1.07 ± 0.11 3.4 f 0.3 2.3 ± 0.2 C 0.16 t 0.05 0.92 t 0.09 1.24 ± 0.12 2.4 f 0.2 1.6 t 0.2 D 0.30 ± 0.04 0.95 1 0. t0 1.45 ± 0.14 2.6 ± 0.3 1.8 : 0.2
I-S98-A 1 .39 1 0.14 0. 70 0.07 0.88 ±t 0.09 3.3 0.3 2.1 ± 0.2 C B 0.79 0. OR 0.8R. 0.08 0.85 0.08 t± 6.0 0.6 3.1 :t 0.3 C 0.35 0.04 0.64 O.06 0.48 0.05 7.6 0. 4c "± ± 0.8 3.5 :± D 0.26 it 0.04 I .09 0.11 0.4 c 0.82 0.04 7.5 0.8 3.7 ± ±1 ±t 1-599-A 0.47 -± 0.05 1 .82 0. 1R ± 2.04 0.20 251.0 25. 1 102.0 f 10.2, B 0.16 0.05 0.24 ± 2.45 4.08 ±t 0.41 322.0 32.2 130.0 ±13.0 C 0.16 0.05 2.25 ± ±I ± 0.22 5.89 0.59 545.0 54.5 221.0 ± 22.01 D (0.03 ± 1.16 ±t 0.12 5.42 0.54 272.0 27.2 110.0 ±t ± ±11.0 ±I 1-5100-A ± 1.17 0.12 1 .75 0. 18 2.10 0.21 5.3 ± 0.5 3.6 ±t 0.4 B 0.66 ± 0.07 1 .90 0.19 2.06 0.21 5.8 0.6 4.0 0.4 C ±" ± ±t 0.60 0.06 2.22 0.22 I .95 0.20 8.8 0.9 ± 3.6 0.4 D 0.69 0.07 3.70 0.37 3.09 0.31 8.3 ±t 0.8 ± ± 3.4 0.4c ±f I-S1OI-A 0.51 ±! 0.05 0. R6 0.09 ± 0.77 0.08 4.5 ±t 0.5 3.1 0.3 B 0. 05 0.02 it ± 1.15 0.12 1.01 0.10 3.0 0.3 2.0 +t ± ±t 0.2 C 0.21 0.04 1 .224 0.12 0.90 0.09 3.8 0.4 ± D ± + 2.6 0.3 0.34 0.05 I .00 0.10 I .25 0.12 3.3 0.2 ± 0.2 2.3 1 -9102 e 1.55 ± 0.16 1.29 it 0.13 3.06 it 0.31 12.8 f 1.3 7.7 1 0.8c
1-S103 h-A 3.82 It 0.38 0.94 it 3 0.09 1.73 it 0.17 1. 75x 104 it 1. 75x103 7.1x 0l It 7.1xlO2b 1 .48 2 B it 0.15 1.10 it 0.11 2. 73x 103 73x10 1.lx103 j it 2. ,.•? O2b C 0.18 0.05 1.09 1 0.11 1 .40 0.14 463.0 46.3 188.0 D 0.07 0.04 1.30 t (0.13 1 .65 it 0.16 343.0 118.8 34.3 139.0 ft3 E (0.03 1.22 1 it 3.91 0.12 2.17 0.22 146.0 14.6 59.1 t 5.9
( ( IAIII.E 4 (cont. d. )
Ga mm.ua Lr a 2 __,Ci IsU
3 2 2 2 2 Tit e1na Sample I)Chiay D)ecay Uranium Fluorometric No. 137c -Cl Chn 1in Cli. in Pg/8 t 10% pCi/g ± 10).
3 1. 3xO2b 1-S104-A 3.13 ± 0.31 IIDL 1.88 1 0.19 3. lOXI3 t 3. Ix102 1.3xlO ± ±t ± 2.6x10 3 b B 1.01 ± 0.10 BDIL 1.34 ± 0.13 6. 39x 10' 6. 4x 03 (2.6x10' ± 5.3x10 2 ±: b C 2.14 ± 0.21 0.72 t 0.07 1.23 t 0.12 5. 26x 103 2. 1xlO1 2. 1 xO 2
4 3 ± . ;XiO 2 b 2.53 t 0.25 0.30 1 0.09 1.45 t 0.14 1.67x10 ± 1.7x10 6.8x103 6 1
4 3 t 6.8± 102b 2.62 t 0.26 0.85 - 0.08 1.05 1 0. 10 1.67x10 ± 1.7x10 6.8xi03
BACKGROUND SOIL ENVIRONMENTAL
I-SBI07-A 1.25 t 0.06 1.2 ± 0.1 0.96 1 0.06 3.4 ± 0.5 2.3 t It 0. A B 4.3 t 0.6 2.9 ± C 4.1 t 0.6 2.8 0. 4 ± D 3.1 t 0.4 2.1 0..
I-SD108-A 0.91 ± 0.05 1.5 t 0.1 1.00 1 0.07 2.5 t 0.5 1.7 t 0.3 4.6 B 6.8 1 0.6 t O.4 t 0.3 C 3.5 f 0.5 2.4 2.2 t 0.3 D 3.2 ± 0.4
1.7 0.3 I-SBI09-A 2.20 ± 0.10 0.9 t 0.1 0.68 1 0.06 2.5 t 0.4 ± 0.4 1.5 0.3 B 2.2 t ± 0.9 £ 0.3 C 1.3 0.4 t 1.6 0.3 D 2.4 0.4 ± ± 0.91 1 0.1 0.72 ± 0.06 4.0 t 0.4 2.7 0.3 i-SBIIO-A <0.05 ± 17.4 1 0.8 11.8 0.5 B ± 5.0 ± o.4 3.4 0.3 C 3.2 ± 0.4 2.2 0.3 D TAIIE 4 it-+-i! 'd.)
Conversion per Appesidix S.
Ilpleted uranium coniver•mun factor of 0.406(, 1 dCI/R/g Rad oui RialnInuin-Pr given its Table 6'.
IDepleted uranium 7 2 6 corrected for natiirntl iraltir •Inredrni (in Rn Cotkc sit rat ion. dSoil from sewer (see FiR. 14). r Surface scrapingm. fRock sample from surface (see Fig. 8).
BDL = Below Detectable Limits hsample subdivided into 2-in, 2-in, 2-in, 6-in, and I-in segments.
-tD
( 50
TABLE 5
GA_-"biA SPECTMAL AN-'D URANTUM FLUORODTRIC ANALYSES OF WATER (W) AND SLUDGE (SS) SA--PLES
Gamma Spectra (pCi/m.tc)
2 3 2 Th 2 2 GRa Sample Volume Decay Decay Uranium Fluorometric No. (•.f) Chain Chain pg/m•m.±10% pCi/mslO~a
DISSOLVED SOLIDS
I-W63 132 <0.01 <0 .01 0.0011±0.0001 7.5xl0 4±7.5xlOs
3 I-SS64 41 0.36±0.07 <0.01 0.0027±0.0003 1.8x10 ±1.8x10 '
1-SS65 43 BDLb 0.21±0.03 0.0012±0.0001 8.2x10'4-8.2xlO0s
I -W66 147 <0.01 <0.01 0.0014±0.0001 9.6x10 4±9.6x1O 5
I-W67 125 0.05±0.02 <0.01 0.0002±0.0001 1.4x10 4±1.4xi0 S
1-SS68 42 BDL 0.09±0.03 0.0010±0.0001 6.8x10 4l6. 8xi0 5
1 -W69 135 <0.01 <0.01 0.0007±0.0001 2.8x10"'±2.8xlO-sc
I -Ss70 58 0 .05±0.02 <0.01 0.0022±0.0002 1.5x10-3+i.5xxO-4
1 -W71 135 <0.01 <0.01 0.0002±0.0001 1.4x10 4±1.4x10 5
I-SS72 85 0.04±0.01 <0.01 0.0012±0.0001 8.2x10 4 ±8.2x10l5
1 -W73 132 0.12±0.05 <0.01 0.0008±0.0001 5.5xO0 4-5.5x10 5
4 5 I-SS74 47 BDL 0.07±0.02 0.0006±0.0001 4.ix10 -4.1x10
-4c 1 -W86 135 0.04±0.02 0.03±0.02 0.0215±0.0022 8.7x10-3±8. 7 x 1 0
5 I -W90 38 BDL <0.01 0.0011±0.0001 7.5x10 -47.5x10
3 c 1-W91 147 BDL 0.02±0.01 0.0038±0.0004 1.5x10 ±1.Sxl0"
1 -W92 137 BDL <0.01 0.0035±0.0004 2.4x10 -3 2.4x10 4
1-W93 134 <0.01 <0.01 0.0014±0.0002 9.6x10-4±9.6x10"s
I-W95 142 0.04±0.02 <0.01 0.0134±0.0013 9.2x10 4±9.2x10 5 51
TABLE 5 (cont'd.)
Gamma Spectra (pCi/mZ±a) 232Th 2 2 6 Ra Sample Weight Decay Decay Uranium Fluorometric No. (g) Chain Chain pg/g±10, pCi/g±10•
SUSPEhNED SOLIDS
I-W63 0. 033 BDL <0. 02 3.0 ± 0.3 2.0 0.2
I-SS64 109 .2 1.00±0.10 <0.02 3.4 ±0.3 2.3 0.2
1-SS65 97.4 0.36±0.07 1.04±0.10 2.5 ±0.3 1.7 0.2
1-W66 0.027 <0.06 <0. 02 3.3 ± 0.3 2.3 0.2
I-W67 0 .009 <0.06 6.4 ±0.64 2.4 ±0.3 1.6 0.2
1-SS68 159 .0 0.6 1±0.06 0. 60±0.06 1.2 ± 0.2 0.8 0.1
I -W69 0.008 1.5 ±0.15 <0. 02 6.8 ± 0.7 4.6 0.5
I-SS70 165.5 0.46±0.07 0. 82±0.08 1.8 ± 0.2 1.2 0.1
I -'W7 1 0.011 <0. 06 <0. 02 2.7 ± 0.3 1.8 0.2
I-SS72 19.6 <0. 06 2.46±0. 25 2.2 ± 0.2 1.5 0.2
1 -W73 0.008 <0.06 <0 02 2.5 t 0.3 1.7 0.2
121.6 0. 78±0.08 0. 63±0.06 1.0 ± 0.1 0.7 0.1 I-SS76 I -WS6 12. 3 <0. 06 1. 06±0. 11 135.0 ±13.5 54. 7 5.5c
i09 .1 0.65±0. 06 0. 85±0.08 4.4 ± 0.5 3.0 0.3 I -W91 0.29 <0. 02 10.3 ± 1.0 4.2 o.4c 1 -W92 10.2 2.03±0.20 1 26±0. 13 2.8 ± 0.3 1.9 0.2
1 -W93 13.0 <0.06 1 .80±0. 18 5.1 ± 0.5 3.5 0.4
1 -W95 5.1 <0. 06 7.11±0.71 5.1 ± 0.5 3.5 0.4
aConversion for Appendix 5. BDL = Below Detectable Limits cDepleted uranium concentration factor of 0.405 as in Table 4. 52
TABLE 6
UJRANIUM MASS SPECTROMETRIC ANALYSES OF SELECTED SOIL SAM'PLES
U Isotopic, Atom Sample No. 233 234 235 236 238
J-S47-A <0.001 0.001 0.228 0.005 99.766 D <0.001 0.001 0.235 0.005 99.759
I-S48-A <0.001 0.001 0.237 0.005 99.757 D <0.001 0.001 0.273 0.005 99.271
1-S49-A <0.001 0.001 0.230 0.005 99.764 D <0.001 0.001 0.236 0.005 99.758
I-SSO-A <0.001 0.001 0.227 0.005 99.767 D <0.001 0.001 0.228 0.005 99.766
I-S76 <0.001 0.001 0.226 0.005 99.768
1-SI03-A <0.001 0.001 0.226 0.005 99.768
1-S105-A <0.001 0.001 0.225 0.006 99.768
I-R96 <0.001 0.005 0.711 <0.001 99.283 54
APPENDIX 1
I NSTRUMENTAT ION
I. PORTABLE RADIATION SURVEY METERS
A. Gas-Flow Proportional Survey Meters
The Eberline PAC-4G-3 was the primary instrument used for surveying. This instrument is a gas-flow proportional counter which utilizes a propane gas 2 2 proportional detector, 51 cm (AC-21) or 325 cm "(AC-22) in area, with a thin 2 double-aluminized Mylar window (- 0.85 mg/cm ).
Since this instrument has multiple high-voltage settings, it can be used to distinguish between alpha and beta-gamma contamination. This instrument was initially used in the beta mode. In the beta mode, the detector responds to alpha and beta paticles and x- and gamma-rays. When areas indicated a higher count rate than the average instrument background, the beta-mode reading was recorded, and the instrument was then switched to the alpha mode to determine any alpha contribution. In the alpha mode, the instrument responds only to particles with high-specific ionization. This instrument is calibrated in the 2 3 alpha mode with a flat-plate infinitely-thin NBS traceable 9Pu standard, and 9 9 0 in the beta mode with a flat-plate infinitely-thin NBS traceable SSr- Y stan dard. The PAC-4G-3 instruments are calibrated to an apparent 50% detection efficiency. An input discriminator threshold sensitivity of 1.5 mV is used with these detectors.
B. Beta-Gamma End Window Survey Meter
When an area of contamination was found with a PAC instrument, a reading was taken with an Eberline Beta-gamma Geiger-Mueller Counter Model E-530 with a HP-190 probe. This probe has a thin mica end window and is, therefore, sen sitive to alpha and beta particles and x- and gamma-rays. A thin piece of 2 aluminum is added to the mica, thus making the window density -7 mg/cm . At this density, the instrument is not sensitive to alpha particles. A maximum reading is obtained with the probe placed in contact with the area of con tamination. In this position, the response (in mR/h) to gamma radiation is generally conservative relative to a determination of mrad/h at I cm. Another reading is obtained with the probe held 1 m from the contaminated area. This 2 2 6 instrument is calibrated in mR/h with a Ra standard source.
C. Low Energy Gamma Scintillation Survey Meter
An Eberline Model PRM-5-3 with a PG-2 gamma scintillation detector was used to determine low energy x and gamma radiation. The PG-2 detector consists of a thin NaI(T£) scintillation crystal 5 cm in diameter by 2 mm thick. This instrument is calibrated on three separate discriminators for three energy 2 4 1 2 regions using 2 3 9 Pu (17 keV), Am (59.5 keV) and 3SU (185.7 keV) sources. This instrument can be operated in either a differential (to discriminate between different energy regions) or integral mode. 55
APPENDIX I (cont'd.)
D. High Energy Micro "R" Scintillation Survey Meter
An Eberline Micro "R" meter model PRM-7 was used to detect high-energy gamma radiation. This instrument contains an internally mounted NaI(Tk) scin tillation crystal 2.5 cm in diameter by 2.5 cm thick and can be used for measuring fields of low-level radiation between 10 pR/h and 5000 VR/h. This instrument is also calibrated with a 2 2 6 Ra standard source.
E. Integrating Radiation Meter
In addition to the PRM-7, a pressurized ion chamber (Reuter Stokes Model RSS-1l1) was used at selected locations to determine the ambient radiation field. The RSS-111 has three output modes; (1) instantaneous exposure rate, (2) strip chart differential readout, and (3) integrated exposure. This instrument is mounted on a tripod, 3 ft (- I m) above the surface and has a uniform energy response from about 0.2 MeV to about 4 MeV. A 3-h period of operation is usually sufficient to obtain significant data.
II. SMEAR COUNTING INSTRUMENTATION
An ANL-designed gas-flow proportional detector connected to an Eberline Mini Scaler Model MS-2 was used to count multiple smears simultaneously. This 2 detector has a double-aluminized Mylar window (400 cm ) and uses P-10 (90% argon and 10% methane) as the counting gas. The metal sample holder for this detector has been machined to hold ten smear papers. This particular system consists of two Mini Scalers and two detectors. One is used for counting in the alpha mode; the other is used in the beta mode. Up to ten samples can be counted simul taneously.
Any smear taken from a contaminated area was counted individually in a Nuclear Measurements Corporation (PC-5 or PC-3A) gas-flow proportional counter. These instruments have been modified to contain a double-aluminized Mylar spun top. This top is placed over non-conducting media (e.g. paper smears) to negate the dielectric effect on the counter. These counters also use P-10 counting gas. Smears are counted in both the alpha and beta modes. These instruments are calibrated by determining the input sensitivity using an alpha source.
III. AIR SAMPLING DEVICE
Air samples were collected using a commercially available (ANL-modified filter queen) vacuum cleaner identified as a "Princess Model." The air was 3 drawn through a filter media at a flow rate of 40 m /h. The filter media consist 2 of 200 cm sheets of Hollingsworth-Vose (HV-70 or LB5211-9 mil) filter paper. The collection efficiency at these flow rates for 0.3-micron particles is about 99.9%.
A separate air sample can be taken with a positive displacement pump drawing about 20 liters/min through a millipore (0.5 to 0.8 micron) filter paper 56
"APPENDIX I (cont' d. ) for abcut -ne hour. An alpha spectrum can be measured from a section of this 2 1 9 2 2 2 filter paper. The ratio of actinon ( Rn - 6.62 MeV a AcC) to radon ( Rn 7.69 MeV o FaC') can be determined from this spectrum.
IV. GAMIA SPECTRAL INSTRUMENTATION
A Nuclear Data Multichannel Analyzer Model ND-100, utilizing a 7.6-cm diameter by 7.6-cm-thick NaI(Tk) scintillation crystal is commonly used for determining gamma spectrum. This instrument is calibrated with NBS traceable gamma sources. Samples from contaminated areas were analyzed using this sytem and the contamination radionuclides were identified.
Hyperpure Germanium detectors (ORTEC - 17% efficiency right-circular cylinders) can be used when more sophisticated gamma-ray analyses are required. These detectors are coupled to Nuclear Data Multichannel Analyzers (Models ND-60, ND-66 or ND-100). 57
APPENrDIX 2
CONVERSION FACTORS
I. INSTRUMENTATION
The factors used to convert the instrument readings to units of disintegra tions per minute per 100 cm2 (dis/min-]O0 cm 2 ) and the derivation of those factors are listed below.
A. Conversion Factors
Floor PAC-4G-3 Monitor (FM-4G) Alpha Beta Alpha Beta
2 To 100 cm 1.96 1.96 0.31 0.31
cts/min per dis/min - 2 - 2 for 9 0 Sr- 90 Y
2 3 9 cts/min per dis/min for pu 2 2
cts/min per dis/min for 3.1 3.0 2.9 2.9 normal U
2 2 6 cts/min per dis/min Ra 1.6 1.7 1.6 1.7 plus daughters
B. Derivation of Conversion Factors
Floor Monitor
2 Window Area: - 325 cm Conversion to 100 cm2 = 0.31 times Floor Monitor readings
PAC-4G-3
2 Window Area: - 51 Cm Conversion to 100 cm2 = 1.96 times PAC reading
22n Internal Gas-Flow Counter. PC counter
Geometry: Solid Steel Spun Top - 0.50
Geometry: Mylar Spun Top - 0.43 Mylar spun top counting {double-aluminized Mylar window (-- 0.85 mg/cm2 )) utilizes the well of the PC counter and is a method developed and used by the Argonne National Laboratory Health Physics Section for negating the dielec tric effect in counting samples on nonconducting media. 58
APPENDIX 2 (cont' d.
The PAC-4G-3 and PC counters are calibrated (see Appendix 1) using a flat plate, infinitely thin 2 2 6Ra (including all short-lived daughters) standard as a source of alpha emissions. The plate was counted in a 2n Internal Gas-Flow Counter (PC counter) with the source leveled to an apparent 2n geometry. The alpha counts per minute (cts/min) reading was found to be 1.9 x 104 cts/min, or 1.9 x 104 - 0.51* = 3.8 x 104 disintegrations per minute (dis/min) alpha. Since the source was infinitely-thin, the alpha component was used as the total alpha dis/min of the source.
The same 2 2 6 Ra plus daughters source, when counted with the PAC instrument in the alpha mode, was found to be 2.3 x 104 cts/min at contact. The conversion factor for cts/min to dis/min for the PAC instrument is 3.8 x 104 - 2.3 x 104 1.6 dis/min alpha to cts/min alpha.
The same source was covered with two layers of conducting paper, each 6.31 mg/cm2 , to absorb the alpha emissions. With the PC counter in the beta mode and the paper in good contrast with the chamber, the count was found to be 1.25 x 104 cts/min or 1.25 x 104 - 0.50 = 2.45 x 104 dis/min beta. With the PAC-4G-3 in the beta mode and in contact with the covered source in the center of the probe, the count was found to be 1.45 x 10' cts/min. This indicates a con version factor of 2.45 x 104 1.45 x 104 = 1.7 dis/min alpha to cts/min beta gamma. All three detectors (51 cm2 , 100 cm 2 , and 325 cm 2 ) gave readings similar to those reported above for the alpha and beta-gamma mode.
A similar method was used to determine the conversion factors for normal uranium.
II. SMEAR COUNT
The conversion factors for cts/min-100 cm 2 to dis/min-100 cm 2 for smear counts are given below:
A. Conversion Eouation (Alpha)
cts/min - (Bkgd) = dis/min a g x bf x sa x waf
A geometry (g) of 0.43 is standard for all flat-plate counting using the Mylar spun top.
A backscatter factor (bf) of 1.0 was used when determining alpha acti vity on a filter media.
The self-absorption factor (sa) was assumed to be 1, unless otherwise determined.
*The value of 0.51 includes the following factors: geometry (g) = 0.50; back scatter factor (bf) = 1.02; sample absorption factor (sa) = 1.0; window air factor (waf) = 1.0. The product of g x bf x sa x waf is 0.51.
*~~~~y. ,*. My 59
APPENDIX 2 (Cont'd.)
If the energies of the isotope were known, the appropriate window air factor (waf) was used; if the energies of the isotopes were not known, 2 3 9 the (waf) of pu (0.713) was used.
2 2 6 The (waf) for alpha from Ra plus daughters is 0.55.
B. Conversion Equation (Beta)
cts/min - {P Bkgd (cts/min) + G cts/min = g x bf x sa x waf
A geometry (g) of 0.43 is standard for all flat-plate counting using the Mylar spun top.
A backscatter factor (bf) of 1.1 was used when determining beta activi ty on a filter media.
A self-absorption factor (sa) was assumed to be 1, unless otherwise determined.
If the energies of the isotopes were known, the appropriate window air factor (waf) was used; if the energies of the isotopes were unknown, 9 9 the (waf) of °Sr- 0 Y (0.85) was used.
2 2 6 The (waf) for betas from Ra plus daughters is 0.85. APPENDIX D CHEM-NUCLEAR SYSTEMS, INC. DATA Comprehensive Site Assessment General Services Administration (GSA) Federal Property Resources Center Watertown, Massachusetts
Volume IV
Radiological Survey Records
prepared by Chem-Nuclear Systems, Inc. O'Brien and Gere Engineers, Inc.
October 1990 zu
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Air Sampler Type/No. ,6C-O,/'20s..T- Filter Used Gti--Alej N& Activity (uCi/ml) = (net cpm)x(C.F.) x (4.505 x 10-' uCi/dpm) X Fa Fa = 1.25 for Alpha (Sample volume) x (10' mI/I) or (2.83 x 10' ml/ft3) Fa = 1.00 for Other Emitters Time Sampler on Sampler off Total time X Flow Rate Sample Volume ,6-\ 31 Counting inst./Serial# Cý5f-/ 7z 11y,; C. F. 4-. 1 c- MDA 1.',22xio /-I Total Counts + Count Time cpm cpm - Cb = Net cpm Activity (uCi/ml) 30______t 30 3-1 01 Counting lnst./Serial# C.F.-__ MDA Total Counts * Count Time = cpm cpm Cb = Net cpm Activity (uCi/ml) Sample Location n 1E - 10OA Technician Si.itLY,, Air Sampler/# R#nbeC. /Los-s" Filter Used GIL MN 1q, r Time Sampler on Sampler off Total time X Flow Rate Sample Volume 3 ,8 -/ 3- Counting Inst./Serial# E5P- I ./ 111k C.F..'_.' MDA LS.2,I D Total Counts Count Time cpm cpm Cb = Net cpm Activity (uCi/ml) _,10 _ _ _ <_ _. _ _ZZ 0k' Counting lnst./Serial#______C.F.-__ MDA ____ Total Counts -Count Time cpm cpm b-C Net cpm Activity (uCi/mI) 10, CONTAMINATC ýADIATION '0 SUTIVEY TIEp(ý. PAOETFL 17 ? ~ TIMSTIM TIME,TOIMEB/ 0- tfS~1 as4 WYEEKL' WELWEEKLYCONTAMINATION AND OI 0 ADIATION r?7MO__NTHL MONTHLY SURIVEY 0 _DPILL 317E 'WvSA 't'SS~LELEYISCSCA AnEA CONTROL LEVELS 0 OTHEn 0- 1/0 Cm',(,~ Al rHAa 0.0/lsiOcn,'ALPHA (SEECOmmENISI I O"'Y5PI/3100 SETA GAA.iLIA _ ____ dT"n,1I:Y3cn9 BETA-GAMMA U NO ACTION FTEOO S'~YG CHC, DAA ONTMIATIN URVYSRADIATION CONTAMIN.TATION ALPHA BETA-GAMMA ______ALPHA BETA/GAMMA - BETA"/GAMMA INSTRUMENT t YPE'TAGONO I/,' CuE1 L)-2-9RADIATION NEUTRON BT.AM SOUIICE STRENGTH INTUMNT YE/TA NOALH E-CMA Tac m",mR/ 'N7fm" tYEIA END 0 ' SFIUMENT RSPNSE - ,fA, IACO lIEVE I-D A C-NC I CoRC T O TzT~ T -oS I A LP H A B ET A -GA M M A P'e m / i, Q1 PROBSYIE/ EOUIV -- EtftZg ýG.AMMA *ITEM P*CK~nOUNO . 0 Q-!Ls NEUTRONU 3 , O I~A OR ______TM ~ 'dm EUTAm 0~ LOCATION ROBE '00 C.' PROBE 10 Cc,~O ~ nEASOTJ FOP 'SUFVEY C] PnOCYORN ______1A IO'RT jJ IN t SPECIAL______ BROUTNE V-d")rK IS) f 213 j BE TAGAMMA "LP"HA m".-Ih 0 21 TRA, ,_ c,-, 0,T_" NEUTRON Ql LOCATION ,`pas' D ImI ,2 Iý 7.2on 211. 29 _____ I _____ 300 17 y ______fld Wio/@ mInat Ion Survey Grid Map) FA CIITA /V ',"-, XLLOAIN&nWTR0 "M A 4'vco T rV A. 4 R, - IL 33 -jIQD m F? I z INCLO 101, 70? 0 'rn y 1 2 3 .20 6 7 8 9 10 1 12 13 14 150 16 17 18 19 20 21 22 5 !326 27 28 29 3 31 2 33 4 35 3 37 3 39 4( I ~~ ~ ~ ~ ~ _ / D 0 O I 2 ~ ~ ~ L~ ~ [~ 1 ~ __ ~ ~ ~ ~ ~ 2 30 31MEf32_ 133_ _ 34/_ _ 3______CONTAMINA AOIATION '0 (OCAICNACT"IvIcom, c1 -- wrt CUnVMIATIlAt wEE it les R 1ADITINU ~~C)URCEPIINCHECRy COTMNTOCSOESRDATO DAT OT NATI MNTONAPA NC DAALYAMA SURLYVEYKY `';0 1 nALPA IEAGAMDE AIAINSRE AM INTRM.ENTs TAPEHI NF! 0A _ tAITO VE SCSA.GMCNTOLLEAL NEURO EEECIECYALPHACO (2)J....BEACTORM ALPHAy BEAETM-G.l~ATEMA A I O A . S T UN S A T SW I P MEN T TY P E.`T A- N O O M U-33RDAINNEUTRON ROBEEI 0O AI, BETAE(OUWVT GAMMA Q AG MM T NOVENEUEUTRO ROPAK BED 'OT np. Vp.. PROB TOBCmi PROB .$CIO /1'. 0 LOP on RUIN vv PhOUIIN PRVt - 20 InR on 22 7.I f e) I 26c - ~ ______III _ 27 T/ y' I I ILq 332 333_ 4 I _ 3T0 ~ rn ly NWTGAWILl FPPI IE COTOniNG OFFAGr SE. PICT ICI OUS. OR FRAAUDTL ENT ST ATEM E NTIS on EN TRIES5ON T-HISDOC UME NT MAY BE PUNISHAatAA r n M DER..&DEA ALSTcnJ PAntrAI fl('OIrAl rr)I`ITnnT~ fladiallon/O ~minationSurvey -GrId-MMa-p W ATIVIT-Y/ M L CAT ION 6-, W 76 a , ( 4 D 9 U c ro ,VPAGE W S~n VEYOR DAll ______NOTIE: THlEKNO WINO $ WILLFUL AECOAOINOOF FALSE. TfllS DOCUMENtTMAY BE PUNISHABLEAS A FELONYFICTICIOUS,0Ft UNDERFEDERAL FRAUDULENTSTATUTES.RENRESO STATEMENTSORETISO 3.. 2(6 L. R r, Czm leii 2 313 74 7 81 9 1610 171 121 19 20 1 2 C, ;sYi/ tVIN 23 4 2 27 28 9 30 31 2 3 34 35 3 37 38 9 m ______~Gtf m CHEM NUCLEAR SYSTEMS INC AIRBORNE RADIOACTIVITY SAMPLE/MONITOR REPORT No. "-z;-e' () * Project Name/No. .jgg- I 4rtv~rorI/, Date 2e JiuN 'Iq Sample Location W-I&A Technician I. JcwezeN Air Sampler Type/No. RAbcr'O!,/z,,_• Filter Used CFLfl'xN A&E Activity (uCi/ml) = (net cpm)x(C.F.) x (4.505 x 10-7 uCi/dpm) X Fa Fa = 1.25 for Alpha (Sample volume) x (101 ml/I) or (2.83 x 10' ml/ft3) Fa = 1.00 for Other Emitters Time Sampler on Sampler off Total time X Flow Rate = Sample Volume Counting lnst./Seriala-. c'- /vu C.F. 5-, MDA 2 .. Total Counts - Count Time = cpm cpm Cb- = Net cpm Activity (uCi/ml) '7 47 <2. 1.- 10 OY Counting Inst./Serial_ C.F.- MDA Total Counts * Count Time = cpm cpm - C = Net cpm Activity (uCi/ml) , i,35 Sample Location WeC--,A Technician f;. Joqms,-, 3 Air Sampler/# PADErCO/,4(.(t9 Filter Used G.Lr,•,1, A/E Time Sampler on Sampler off Total time X Flow Rate = Sample Volume ,8-/ 3- Counting Inst./Serial# "P- / C.F. s.c MDA ' z Total Counts - Count Time = cpm cpm -- C = Net cpm Activity (uCi/ml) -- i2 a Counting Inst./Serial# C.F.__ MDA Total Counts * Count Time cpm cpm C Net cpm b Activity (uCi/ml) 1 11 .... J -U.11 A- 11 V .1 l.UVk JU I.. 0, SE, , I LIP sflý I 6( I 4ý 1 i Jrly I I I IU, n f, I ýc VýA. 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OAMMA ,eý/hfl, ITEM 01 ODFE IOU, C- SWIPEI ITEM ECUIVR L a on EouIvý - EOUIV __ BETA-GAMMA 0l 11"v- No1C NEUTRON LOCATION OR 0l NEUTRON LOCATION NO I rpl%..i 0 P"IC0 .G " PROOF IJ " -"IM SAll, I oopcnM~'P m I 'I I PROSE11 Ile. -v R'0 0 I I I! I - i I - l< Ing 1 It I -70 IC 1 + - 40- "(4..f MAr' 4~c-la-0 I_-2-Il- ' 1 I I I I 'S I ______ 2- ______I I I 9.co ______I I ______ (4 I I ______I ______I I I I -Li--- ___ I I I ______I -4-- I _____ I -i-1______I I ______ •3 __ __ I I ______ '-F __ I i ______I ______ _ I I _____ I ______ __ Il I J I ______ ______I-______I ____ I ______I______ilL -+ I ------4 I I I I t 4 If -4- t I F IA- i 11 1 i i -1- 4- 11--t F F 4 m F I IL--f F F 4 - I 1Ir - .- I I 4i 1 1 t 4 I t ii -r - C 4- ______I ______K C - L I API eF-o 4eAh-fThNT Rad latlo n/Q~mina lion Survey Grid Map I- ACTIVITY/\W, LOCATION r,"rzrA PAGE SURVEYOR POUt LAflt A DATE JA 6 "~'A~ " 0J INOTE: THE KNOWING&£ WILLFUL RECORDING OF FALSE. FICTICIOUS. On FRAUDULENTSTATEMENTS OR ENTRIES ON THISDOCUMENT MAYOf OUNISHAOLEASA FELONY UNDERFED ALSTATUTES. r--- T T I r I T - t - I - - t - - 1-1-4 -- 4-4-4-F -- 4----- 4-4-4-4- - L- I - - I - J .....i .1 1 T-- t-t1-tt-t-ti-t-t-1-±-+-f- -1-f-f-I-4-4-I-f- -l-4-1-I-4-L-IL11 I - I - I -- I - 1 t - I -11 4- I - I-4-1- t - +-f - i-I- I-4-4 - 4-4-1-4- - 4-4 - 1-4 -.1 ...... 1- I - I i t - -1 1 4- I - I t -4-1- +-1-1- +- f - I - +- +- f-I-I-I-I-] -4-l-1-4-J-4 1 i 1 I I -T -- I -- T-1- I 4 - -- F----- i1 --- -- 4--4 L olil F b _( _ I I I_ #lfl' LCR F21 - - - : -- - IF -f--I--f -1-1--4-+-f-4--+-4-4--4-4-4'-4---4--4--1-I4 ± 0 __ J -J j flj woL jb z -I 'A 2 r~~~~~~--- 1 t I t I------i-f--f -4-1-4---4-4-rTY4-4---I I L 41' t- IJ I u J - - I - - t - --1 t - 11- - I - -4 +- f-f-f-I-I-I- 4-1-1-4-1-i -'4-I - I..... 1.... 1.1 In I Ajc -j z/ 'I 0A ~3 4 (6 8 9 10 11 12 13 14 15 16 17 IS 19 20 21 22 23 26 - 5 29 30 32+33 34 35 36 37 38 39 40 CHEM NUCLA SSTEMS INC 2 > 0 U) .3 0 1..... 1 0.ir - T - - - - i--i-i - - - f - -4-4- -4-4-J-4.. . 1* iv0 f4O Cc 2 K.I 2 4 C C 0.G. 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MDA Total Counts + Count Time cpm cpm - -b = Net cpm Activity (uCi/mI) Sample Location Technician Air Sampler/# Filter Used Time Sampler on Sampler off Total time X Flow Rate Sample Volume 2-,Counting Inst/Serial# C.F.__ MDA Total Counts - Count Time = cpm cpm - b = Net cpm Activity (uCi/mI) 0( Counting Inst./Serialt C. F.__ MDA Total Counts ' Count Time = cpm cpm b - Net cpm Activity (uCi/ml) siinivis ivujoij w3oNn ANO I I AV SY 310VNSINnd 30 AVN IN 3"fIDOO SII4I NO $I I UiN3 UO S I NJn3lvis I Nj1IlUnvUA UU flu, J I I ')Ij ASIVA JO t)t41GUOD3U 111,111M QN-0- 3.11 0, LI U z 9ZI 61 Ln > 1C 9C > L U z T U 4C CC 64 oz > it If p 9z r -T- S. I I FZ ý5(11I-a Cz 0 ýd 00- ý3 00, 30OU-13p I --ý.- pý JUOUT-.10 N 11V cl NOULA314 - '42 JUL)uj UO, VV4nVO ta A e-4_ý A1110 3 ýInC)3 k4,.a,. 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A3AunS N011VIOVU 1AIM33M ONY N01i'vNI"ViNOZ) 0 Al )133M N Q 1 Ti -' uz7N..,v Z,0 8 A)Iva 1 AIVO , S/4 0 'WrAOD f)d3U A3AUnS (0ý8 0 luvis O'ý 01 -oliviov 4 1VUMVINOD CONTAM(10ON/R AOIATIOH SURVEY REPORT 0 9 oOTIU,iON SHEE NOETHE KNOWINO & WIL.LFUL.RECORDING OF FALSE. FICTITIOUS. OR FRAUDULENT STATEMENTS OR ENTRIES ON4 TH IS DOCUMENT MAY BE PUNISH4ABLEAS A FELONY UNDER FEDERAL STATUTE. ALý-A PETA GAMMA -IN ALPHA BETA-GAMMA n,,.m/pw 0 S-~ G~AL4IA ITE SWPE EOUIV [O4Ji - BETA-GAMMA 0 ITEM EOU~v EGUICý-:, 14 on PROBE on ,O R NEUTRON 0l LOCA~ION NO dn~ 4~J df~ pl' NEUTRON 0 LOCATION _ mE.1. PROS"'E:F 00,T PRS 0c Ico Rib, RPOBE I Ooc"" f~l D cm icro on" B I ~~ ~ ~ ~ ~ ~ fm~,t 01.__ MAP___I______ z 0 cI, rm (A, I II T t 1- -F ______.1 4' I Il--i F + 4 I 'I RADIOL('OGICAL CONTROL1 Radlation/C ,-mInatlon SurveyGrid Map I nJ7 PAGE SLOCATIONAC TIVIT Y/ qw '/ ~4'mneA'// 3 3 £VILT ,7 SURVEYOR DATE 5, Jo~t)'To/1, 2/ J4 /,"v -7 NOTE: THE KNOWINO &WILLFUL RECORDINO OF FALSE, FICTICIOUS. OR FRAUDULENT STATEMENTs OR ENTRIES ON THIS DOCUMENT MAY BE PUNISHABLE AS A FELONY UNDER FEDERAL STATUTES. I I T 11ITTr11rr1 I I I I I I ( 'CrR "Lt'f E3, ____ ------ .15 C, C,---- -a[------ S .r,6. . . . ---- . ------. ------I I ------ fx 1---14f--+--444--- - r r - r - - C I - r - - I - r - 1 - C-- - r - r - 1 - I - I- - I - - 4 - + - I - 4- 4 - + - I - 4 - I - L - - . - z K. 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' FIEASON FOR SUPvEy 0 PnoCEOUBE-NO______ Ol SPECIAL t 14M~ *ROUTINE WOCK IIJ PRO~rC_; 20 .&20 AL.PAA BETA.GAMMA ITEM,~,, 21, (Ou'v eouiUIVU39 OC; 4GAMMA onTE "0VB NETO Q LOCATION "-08E CT) '_ PROBE 100 C,,, m~co BYI,. U23 AI3 5 131. 30 12 1 B~' .1 1 .?ft 14 SVAZFP1 ______ITT3C ___ __ 3 . Ol T .,s~ r5IK 16' X45~C.~'ý TAT t IiI34I-O SfUT- 1' CHEM NUCLEAR SYSTEMS. INC 02 2 C- f o 0. 0 9 ' r- 2 04 0' ci10 0u4~ -I - o3z 10 I 0 7P1 z N 00 c 0 0 tjl 00 c in C 0 z J 07c I ~71 -J I.' I- fladlallo n/C41fmInatlon Survey Grid Map ACTIVITY/ *W LOCATION G4WT~m A PAGE w *1. ------I I - - DATE S. J(HN50 Zr JIJPJE ' o zi JVmc qt% * OTE! THEEKNOWINOG& WILLFUL. RECORDING OF FALSE. FICTICIOUSOR FRAUDULENTSTATE!MNTwS DATE ORENTRIES ON THIS DOCUMENT MAY Of PUNISHABLE AS A FELONY UNDER FEDERAL STATUTES.&I Yi 1 I T *g - -!- _ 1 - - a -~r --- F- 12 d- - - - - p ------I - - '3 3 IF;~~~ -- -- _ -~~ - L _ 4 _ 1. 31 I _ 3 '5 4& LI P.7fi I m z1 m r, 3 4j f, 1 7 [ 8 [:ý 170 12 1=3 14 [15: M6511 7 1S 1=9 2 0 1 2 1 2 2 23 265 1,5133 127 1280129 110 111 132 13313 I CHEM-NUCLEAR SYSTEMS INC AIRBORNE RADIOACTIVITY SAMPLE/MONITOR REPORT No. Q-z2-oL,0) * Project Name/No. G W.eT.,/V,./, Date -z J,,,' 20 Sample Location D.,.L.L 5"C r-It. r.-'.3. Technician S. Air Sampler Type/No. Tbt• C-0 Filter Used GCLr-,N 41C Activity (uCi/ml) = (net cpm)x(C.F.) x (4.505 x 10- uCi/dpm) X Fa Fa = 1.25 for Alpha (Sample volume) x (101 mIA) or (2.83 x 101 ml/ft3) Fa = 1.00 for Other Emitters Time Sampler on Sampler off Total time X Flow Rate Sample Volume -\Z 8-\?I- Counting Inst./Serial# C'NF P-/I1 C.F. LO MDA /./4'$/i Total Counts - Count Time = cpm cpm -- C = Net cpm Activity (uCi/ml) a Counting Inst./Serial# CCF._ MDA Total Counts + Count Time = cpm cpm C b- = Net cpm Activity (uCi/ml) Sample Location Technician Air Sampler/# Filter Used Time Sampler on Sampler off Total time X Flow Rate Sample Volume ,3/ -/' Counting Inst./Serial# C.F.__ MDA Total Counts - Count Time = cpm cpm C Net cpm Activity (uCi/ml) 0 Counting Inst./Serial# C.F__ MDA Total Counts + Count Time cpm cpm - Net cpm Activity (uCi/ml) biLilivi5 lvuj(jij ujuNn Atjolýj v 5V lie d I UAW I N iýnDoo 51141 NOS J IU IN I UO SIN 1. 3 1, Is IN 3 In any Ui Uo Snc) I D, I DO 3" 1, A AU 'J 1,"). 0 L V UN-u- 3", Gc vtn U, c >. 9c LI sjlý T TZ r---41 S51. ssi. SSI, ic u tj 0 '-si, sso. 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N011VI(IYU 0 A3AunS 0 Al-13M a A1'.0 ONY N011WAIMINOD 0 IIA331 t-oscjHur C,-,, UOA]AtlnS Al-I (ý,i r i 71Y I -j OILVIOVJ& 13U k3AUlll E ---tftf- v--II'IT I z - ",I N VNINVINO D CONTAM* ON/RADIATION SURVEY REPORT r7ONTINUA OH SHEET in OP'oJECT F ILL --- -% 5, _ L,-1 • (. *.3 _•C.- 5. JOHtJroiJ I Zz Jv" -,to NOTE: THE KNOWVNO & WILLtUL RECORDING OF FALSE. FICTITIOUS. OR FRAUOULENT STATEMENTS THIS DOCUMENT MAY BE OR ENTRIIS ON PUNISHABLE AS A FELONY UNDER FEDERAL STATUTES. ALPHA BETA-GAMMA mremnh. 0 SWIPE] EOUIV - EOUIV 0AW--O AMMA U ITEM NEUTON LOCATION P1OBE 100 cm' P'OIE 100 cm micro R/N U S/ _-/- -, ...... .1m -C cl I.I 'In z CONTAMI H/RA DIATION SURVEY REPORT CONTINUAl) SHEET ACTIVITY/ 6 - IM- LAUA17- P'C- X~J J IApIOPAE O r) OCAT ION L0TfT)-,l 6Z-O~ 15A( 32- O !~~P.QJ/7('7Z ~eI.j 4-I( * NOTE: THEKNOWING &WILLFUIL IECOR DING OFFALSE. FICTITIOUS. OAt F AUDVULENT STATEMENTS ORtENTRIES O N THIS DOCUMENT MAY BE PUNISHABLE AS A FELONY UNDER FEDERAL STATUTES. 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