Mark Stockman, the Knight of Plasmonics
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SPASER As a Complex System: Femtosecond Dynamics Traced by Ab-Initio Simulations
SPASER as a complex system: femtosecond dynamics traced by ab-initio simulations Item Type Conference Paper Authors Gongora, J. S. Totero; Miroshnichenko, Andrey E.; Kivshar, Yuri S.; Fratalocchi, Andrea Citation Juan Sebastian Totero Gongora ; Andrey E. Miroshnichenko ; Yuri S. Kivshar and Andrea Fratalocchi " SPASER as a complex system: femtosecond dynamics traced by ab-initio simulations ", Proc. SPIE 9746, Ultrafast Phenomena and Nanophotonics XX, 974618 (March 14, 2016); doi:10.1117/12.2212967; http:// dx.doi.org/10.1117/12.2212967 Eprint version Publisher's Version/PDF DOI 10.1117/12.2212967 Publisher SPIE-Intl Soc Optical Eng Journal Ultrafast Phenomena and Nanophotonics XX Rights Copyright 2016 Society of Photo Optical Instrumentation Engineers. One print or electronic copy may be made for personal use only. Systematic reproduction and distribution, duplication of any material in this paper for a fee or for commercial purposes, or modification of the content of the paper are prohibited. Download date 27/09/2021 00:14:10 Link to Item http://hdl.handle.net/10754/619757 SPASER as a complex system: femtosecond dynamics traced by ab-initio simulations Juan Sebastian Totero Gongoraa, Andrey E. Miroshnichenkob, Yuri S. Kivsharb, and Andrea Fratalocchia aPRIMALIGHT, King Abdullah University of Science and Technology (KAUST),Thuwal 23955-6900, Saudi Arabia bNonlinear Physics Centre, Australian National University, Canberra ACT 2601, Australia. ABSTRACT Integrating coherent light sources at the nanoscale with spasers is one of the most promising applications of plasmonics. A spaser is a nano-plasmonic counterpart of a laser, with photons replaced by surface plasmon polaritons and the resonant cavity replaced by a nanoparticle supporting localized plasmonic modes. -
CV Hamed Koochaki
1 curriculum vitae Hamed Koochaki Kelardeh Hamed Koochaki Kelardeh, PhD Department of Physics & Astronomy Center for Nano Optics (CeNO), Georgia Stae University Science Annex, Suit 411, Atlanta, GA 30303 Tel: (404) 566 - 1283 Email: [email protected] Web site: www.physics.gsu.edu/hamed-koochaki-kelardeh Employment 2017–present: Postdoctoral Fellow Georgia State University Atlanta, GA, USA Center for Nano Optics (CeNO), Department of Physics & Astronomy Advisor: Mark Stockman Education 2012–2016: Ph.D., Physics, Georgia State University, Atlanta, GA, USA. GPA 4.12/4.0 Dissertation: Ultrafast laser-induced kinetics in two-dimensional materials. 2012–2015: M.Sc., Physics, Georgia State University, Atlanta, GA, USA. GPA 4.10/4.0 Thesis: Theoretical study of graphene under strong electric field. 2006–2009: M.Sc., Atomic & Molecular Physics, Magna Cum Laude Iran University of Science and Technology, Tehran, Iran. GPA 3.5/4.0 Thesis: Numerical study of K-alpha x-ray emission from multi-layered cold and shocked targets. 2002–2006: B.Sc., Applied Physics, Magna Cum Laude University of Tabriz, Tabriz, Iran. GPA 3.3/4.0 Thesis: High-efficiency semiconductor thermocouples: design & characterization. Research Interests Computational and theoretical physics; Ultrafast dynamics in condensed matter; Optical and transport properties of low-dimensional materials, Nonequilibrium carrier transport and relaxation dynamics, Dirac materials, Laser-plasma interactions, Relativistic interaction, Coherent optics, SPASER and Nano-laser. Honors and Awards . Outstanding Student of the year 2017 recognized by Physics Department Executive Committee . Center for Nano-Optics (CeNO) fellowship 2014-2017 Georgia State University . President at Physics Graduate Student Association (PGSA) 2016-2017 Georgia State University . -
Citation Data All Indices 2014 2000
MARK I. STOCKMAN CURRICULUM VITAE PAGE 1 OF 43 Dr. Mark I. Stockman Residence: Phone:678-438-1093 Phone: (678)438-1093 29 Peachtree Center Ave. Department of Physics and Astronomy Georgia State University Atlanta, GA 30302 USA Phone (worldwide): +1-678-457-4739 E-mail: [email protected] Internet: http://www.phy- Mark I. Stockman,astr.gsu.edu/stockman PhD, DSc, Professor of Physics Regents’ Professor GSU Center for Nano-Optics (CeNO), Director American Physical Society (APS), Fellow Optical Society of America (OSA), Fellow SPIE – The International Society for Optical Engineering, Fellow h-index: 64 On line at http://www.phy-astr.gsu.edu/stockman/ Contents p. # 1. PERSONAL ..................................................................................................................2 2. BRIEF NARRATIVE .....................................................................................................2 3. EDUCATION ................................................................................................................3 4. RESEARCH AND ACADEMIC POSITIONS ....................................................................4 5. RESEARCH .................................................................................................................4 5.1. Major Results ......................................................................................................................... 5 5.2. Other Significant Results ........................................................................................................ 6 5.3. -
Synthesis and SERS Application of Sio2@Au Nanoparticles
Synthesis and SERS application of SiO2@Au nanoparticles A. Saini, T. Maurer*, I. Izquierdo Lorenzo, A. Ribeiro Santos, J. Béal, J. Goffard, D. Gérard, A. Vial and J. Plain Laboratoire de Nanotechnologie et d’Instrumentation Optique, ICD CNRS UMR n°6281, Université de Technologie de Troyes, CS 42060, 10004 Troyes, France In this letter, we report a chemical route for synthesizing SiO2@Au core-shell nanoparticles. The process includes four steps: i) preparation of the silica cores, ii) grafting gold nanoparticles over SiO2 cores, iii) priming of the silica-coated gold nanoparticles with 2 and 10 nm gold colloids and finally iv) formation of complete shell. The optical extinction spectra were experimentally measured and compared to numerical calculations in order to confirm the dimensions deduced from SEM images. Finally, the potential of such core- shell nanoparticles for biosensing was probed by means of Surface Enhanced Raman Scattering measurements and revealed higher sensitivities with much lower gold quantity of such core-shell nanoparticles compared to Au nanoparticles exhibiting similar diameters. SiO2 core-Au shell nanoparticles have attracted much attention for the past ten years due to potential applications in various fields such as cancer imaging and treatment(Loo et al., 2004), Surface-Enhanced Raman Spectroscopy (SERS) detection of molecules(Wang et al., 2006, Maurer et al., 2013), catalytic degradation of environmental pollutants(Ma et al., 2009) or even fabrication of SPASER (Surface Plasmon Amplification by Stimulated Emission of radiation) devices when the silica is dye-doped(Stockman, 2008). However, the growth of a complete gold shell around silica nanoparticles is very hard to achieve. -
Mark Stockman: Evangelist for Plasmonics
pubs.acs.org/journal/apchd5 Editorial Mark Stockman: Evangelist for Plasmonics Cite This: ACS Photonics 2021, 8, 683−698 Read Online ACCESS Metrics & More Article Recommendations ABSTRACT: Mark Stockman was a founding member and evangelist for the plasmonics field for most of his creative life. He never sought recognition, but fame came to him in a different way. He will be dearly remembered by colleagues and friends as one of the most influential and creative contributors to the science of light from our generation. ■ A SHORT BIOGRAPHY OF PROFESSOR MARK projects involved large groups and implied very long STOCKMAN experimental cycles. He moved to the neighboring Institute of Mark Stockman was born on the 21st of July 1947 in Kharkov, a Automation and Electrometry in Novosibirsk to work on the major cultural, scientific, educational, and industrial center in the fundamentals of nonlinear optics with Sergey Rautian. He mainly Russian-speaking northern Ukraine, a part of the Soviet habilitated in 1989 with a D.Sc. dissertation on nonlinear optical Union at that point in time. His father, Ilya Stockman, was a phenomena in macromolecules. mining engineer by training, who fought in World War II and Around this time, the political regime in the Soviet Union became a highly decorated enlisted officer. After the war, Ilya softened and the Iron Curtain was lifted. In 1990, on the Stockman embraced an academic career and eventually became invitation of Professor Thomas F. George, Mark was permitted to leave Russia with his family to take a research post at the State a Professor at the Dnepropetrovsk Higher Mining School. -
Experiment and Theory: No Spasing from Core-Shell Spasers
Experiment and Theory: No Spasing from Core-Shell Spasers Günter Kewes,1 Kathrin Höfner,2 Andreas Ott,3 Rogelio Rodriguez-Oliveros,2 Alexander Kuhlicke,1 Yan Lu,3 Matthias Ballauff,3 Kurt Busch,2, 4 and Oliver Benson1 1AG Nanooptik, Institut für Physik, Humboldt-Universität zu Berlin, Newtonstrasse 15, 12489 Berlin, Germany 2AG Theoretische Optik & Photonik, Institut für Physik, Humboldt-Universität zu Berlin, Newtonstrasse 15, 12489 Berlin, Germany 3Helmholtz-Zentrum Berlin für Materialien und Energie GmbH (HZB), Hahn-Meitner-Platz 1, 14109 Berlin, Germany 4Max-Born Institut, Max-Born-Strasse 2a, 12489 Berlin, Germany In 2009 the smallest laser-device consisting of a single 14 nm gold sphere and a dye-doped coating was “demonstrated” [1] based on the proposal of the “spaser” from 2003 [2]. Here, we critically evaluate so far reported results on both an experimental and on a theoretical basis. Experiments: Core-shell spasers were chemically synthesized or metal nanoparticles were coated with dye-doped polymer films. Various excitation schemes were tested, yielding laser or laser-like signatures. All of them, however, were later identified to stem from sources other than spasing. Theory: A fully analytic model for spherical core-shell spasers was developed: Within this model, we drop the widely used quasi-static approximation of the electromagnetic field in favor of fully electromagnetic Mie theory. This allows for precise incorporation of realistic gain relaxation rates (quenching and cavity-to-gain coupling) that so far have only been estimated (and massively underestimated) in spaser theory. The model unravels multiple severe limitations (that exist all over the VIS) concerning the threshold-pump, the extreme gain-medium requirements and the unavoidable heat production (independent of excitation scheme). -
Plasmon Lasers
Plasmon Lasers Wenqi Zhu1,2, Shawn Divitt1,2, Matthew S. Davis1, 2, 3, Cheng Zhang1,2, Ting Xu4,5, Henri J. Lezec1 and Amit Agrawal1, 2* 1Center for Nanoscale Science and Technology, National Institute of Standards and Technology, Gaithersburg, MD 20899 USA 2Maryland NanoCenter, University of Maryland, College Park, MD 20742 USA 3Department of Electrical Engineering and Computer Science, Syracuse University, Syracuse, NY 13244 USA 4National Laboratory of Solid-State Microstructures, Jiangsu Key Laboratory of Artificial Functional Materials, College of Engineering and Applied Sciences, Nanjing University, Nanjing, China 5Collaborative Innovation Center of Advanced Microstructures, Nanjing, China Corresponding*: [email protected] Recent advancements in the ability to design, fabricate and characterize optical and optoelectronic devices at the nanometer scale have led to tremendous developments in the miniaturization of optical systems and circuits. Development of wavelength-scale optical elements that are able to efficiently generate, manipulate and detect light, along with their subsequent integration on functional devices and systems, have been one of the main focuses of ongoing research in nanophotonics. To achieve coherent light generation at the nanoscale, much of the research over the last few decades has focused on achieving lasing using high- index dielectric resonators in the form of photonic crystals or whispering gallery mode resonators. More recently, nano-lasers based on metallic resonators that sustain surface plasmons – collective electron oscillations at the interface between a metal and a dielectric – have emerged as a promising candidate. This article discusses the fundamentals of surface plasmons and the various embodiments of plasmonic resonators that serve as the building block for plasmon lasers. -
Coherent Control at Gold Needle Tips Approaching the Strong-Field Regime
Nanophotonics 2021; aop Research article Philip Dienstbier*, Timo Paschen and Peter Hommelhoff Coherent control at gold needle tips approaching the strong-field regime https://doi.org/10.1515/nanoph-2021-0242 interaction [1, 2] resulting in unique sensing capabilities Received May 15, 2021; accepted June 22, 2021; from detecting single-molecule Raman-scattering [3]to published online July 5, 2021 scanning-nearfield microscopy [4]. Abstract: We demonstrate coherent control in photoemis- Plasmonics also gained more and more interest in sion from a gold needle tip using an − 2 field composed the realm of strong-field physics as field-driven phenom- of strong few-cycle laser pulses with a nearfield inten- ena such as high-harmonic generation (HHG), attosecond sity of ∼ 4TW/cm2. We obtain the nearfield intensity pulse generation, and electron rescattering were explored from electron energy spectra, showing the tell-tale plateau for dielectrics and metals [5–9]. The solid-state nature of field-driven electron rescattering at the metal surface of plasmonic structures and their strong enhancement of induced by the fundamental field. Changing the relative incident fields resulted in on-chip structures sensitive to phase between the fundamental field centered at 1560 nm the waveform of light [10, 11], ultrafast electron emitters and its second harmonic modulates the total emitted pho- [12–18], and hybrid devices providing nearfield-enhanced tocurrent with visibilities of up to 80% despite the strong HHG from solids [19]. and broadband excitation of the plasmonic material. Our Apart from specially designed targets, using tailored work combines a two-color coherent control scheme and waveforms has proven extremely successful in coherently strong-field physics enabled by a nanoplasmonic emitter. -
SPASERS: Nano-Lasers Going Beyond the Diffraction Limit
SPASERS: Nano-Lasers Going Beyond the Diffraction Limit Belinda Pacheco Literature Seminar November 9, 2017 A SPASER (Surface Plasmon Amplification by Stimulated Emission of Radiation) is a nanoscale version of a laser that has been recently theorized and experimentally demonstrated.1,2 SPASERs can be considered counterparts to the laser since they are intense, coherent light sources and require a resonator cavity-like structure with gain media. However, SPASERs dramatically differ from lasers in two ways: 1) their resonator and gain medium structures are on the nanoscale, and 2) the stimulated emission originates from overpopulation of surface plasmons in excited states, and not population inversion in the gain medium. Consequently, SPASERs can uniquely overcome the diffraction limit which is detrimental to the spatial footprint and physical size of the 3 typical laser. Based on these characteristics SPASERs (a) show tremendous prospects in fields where lasers have become limiting factors such as in ultramicroscopy, spectroscopy, ultrasensitive detection, imaging, biomedical applications, optical communications, and lab-on-a-chip devices.1,4–6 However, SPASERs have not been successfully implemented into these technologies because of their inherent lack of beam directionality and significant radiative losses.4 Despite their shortcomings, recent efforts in materials chemistry, materials science, and nano-optics (b) have provided routes for overcoming these limitations. To understand the lasing action of a SPASER, it is essential to understand the fundamentals of surface plasmons. In essence, surface plasmons (SPs) are oscillations of conduction band electrons at the interface between materials of different dielectric permittivity.7 SPs are naturally coupled to electromagnetic waves allowing them to be considered a type of boson (a polariton), thereby acting similarly to photons (i.e. -
Open Resonator Electric Spaser Bobo Liu,† Weiren Zhu,‡ Sarath D
Article www.acsnano.org Open Resonator Electric Spaser Bobo Liu,† Weiren Zhu,‡ Sarath D. Gunapala,§ Mark I. Stockman,# and Malin Premaratne*,† † Advanced Computing and Simulation Laboratory (AχL), Department of Electrical and Computer Systems Engineering, Monash University, Clayton, Victoria 3800, Australia ‡ Department of Electronic Engineering, Shanghai Jiao Tong University, Shanghai 200240, People’s Republic of China § Jet Propulsion Laboratory, California Institute of Technology, Pasadena, California 91109, United States # Center for Nano-Optics and Department of Physics and Astronomy, Georgia State University, Atlanta, Georgia 30303, United States *S Supporting Information ABSTRACT: The inception of the plasmonic laser or spaser (surface plasmon amplification by stimulated emission of radiation) concept in 2003 provides a solution for overcoming the diffraction limit of electromagnetic waves in miniaturization of traditional lasers into the nanoscale. From then on, many spaser designs have been proposed. However, all existing designs use closed resonators. In this work, we use cavity quantum electrodynamics analysis to theoretically demonstrate that it is possible to design an electric spaser with an open resonator or a closed resonator with much weak feedback in the extreme quantum limit in an all-carbon platform. A carbon nanotube quantum dot plays the role of a gain element, and Coulomb blockade is observed. Graphene nanoribbons are used as the resonator, and surface plasmon polariton field distribution with quantum electrodynamics features can be observed. From an engineering perspective, our work makes preparations for integrating spasers into nanocircuits and/or photodynamic therapy applications. KEYWORDS: spaser, graphene, Coulomb blockade, carbon nanotube, plasmon n nanoplasmonics, the spaser (surface plasmon amplifica- in which, the gain medium employed a semiconductor cascade tion by stimulated emission of radiation) is a promising quantum well structure. -
Magneto-Optical Spaser
2002 OPTICS LETTERS / Vol. 38, No. 12 / June 15, 2013 Magneto-optical spaser D. G. Baranov,1,2 A. P. Vinogradov,1,2 A. A. Lisyansky,3,* Yakov M. Strelniker,4 and David J. Bergman5 1Moscow Institute of Physics and Technology, 9 Institutskiy per., Dolgoprudniy, Moscow 141701, Russia 2Institute for Theoretical and Applied Electromagnetics, 13 Izhorskaya, Moscow 125412, Russia 3Department of Physics, Queens College of the City University of New York, Queens, New York 11367, USA 4Department of Physics, Bar-Ilan University, Ramat-Gan IL-52900, Israel 5Raymond and Beverly Sackler School of Physics and Astronomy, Faculty of Exact Sciences, Tel Aviv University, Tel Aviv IL-69978, Israel *Corresponding author: [email protected] Received December 26, 2012; revised April 28, 2013; accepted May 8, 2013; posted May 8, 2013 (Doc. ID 182465); published June 3, 2013 We present an electrodynamical model of a quantum plasmonic device—the magneto-optical (MO) spaser. It is shown that a spherical gain nanoparticle coated with a metallic MO shell can operate as a spaser amplifying circularly polarized surface plasmons. The MO spaser may be used in design of an optical isolator in plasmonic transmission lines as well as in spaser spectrometry of chiral molecules. © 2013 Optical Society of America OCIS codes: (240.6680) Surface plasmons; (140.3410) Laser resonators; (310.6628) Subwavelength structures, nanostructures; (350.4238) Nanophotonics and photonic crystals; (230.3810) Magneto-optic systems. http://dx.doi.org/10.1364/OL.38.002002 Recently, nanosources of coherent light have attracted Maxwell’s equation, while the dynamics of the polariza- significant attention [1]. After [2], different plasmonic- tion and the population inversion of active atoms n are based light sources have been studied theoretically governed by the equations following from the density [3–5] and realized experimentally [6–8]. -
A Novel Metal Nanoparticles-Graphene Nanodisks-Quantum Dots Hybrid-System-Based Spaser
nanomaterials Article A Novel Metal Nanoparticles-Graphene Nanodisks-Quantum Dots Hybrid-System-Based Spaser Mariam M. Tohari 1,* , Andreas Lyras 2 and Mohamad S. AlSalhi 2,3 1 Department of Physics, College of Science, King Khalid University, P.O. Box 9004, Abha 62529, Saudi Arabia 2 Department of Physics and Astronomy, College of Science, King Saud University, P. O. Box 11451, Riyadh 11451, Saudi Arabia; [email protected] (A.L.); [email protected] (M.S.A.) 3 Research Chair on Laser Diagnosis of Cancers, College of Science, King Saud University, Riyadh 11451, Saudi Arabia * Correspondence: [email protected] Received: 01 January 2020; Accepted: 22 February 2020; Published: 27 February 2020 Abstract: Active nanoplasmonics have recently led to the emergence of many promising applications. One of them is the spaser (surface plasmons amplification by stimulated emission of radiation) that has been shown to generate coherent and intense fields of selected surface plasmon modes that are strongly localized in the nanoscale. We propose a novel nanospaser composed of a metal nanoparticles-graphene nanodisks hybrid plasmonic system as its resonator and a quantum dots cascade stack as its gain medium. We derive the plasmonic fields induced by pulsed excitation through the use of the effective medium theory. Based on the density matrix approach and by solving the Lindblad quantum master equation, we analyze the ultrafast dynamics of the spaser associated with coherent amplified plasmonic fields. The intensity of the plasmonic field is significantly affected by the width of the metallic contact and the time duration of the laser pulse used to launch the surface plasmons.