Geological Disposal of Highly Radioactive Waste Is Based on a Multi-Barrier Approach to Safely Isolate the Waste from the Environment

Total Page:16

File Type:pdf, Size:1020Kb

Geological Disposal of Highly Radioactive Waste Is Based on a Multi-Barrier Approach to Safely Isolate the Waste from the Environment Geological disposal of highly radioactive waste is based on a multi-barrier approach to safely isolate the waste from the environment. In a number of countries, research is being done at underground laboratories. (Credits: SKB, ANORA) A storage building for low- level radioactive wastes in the USA. (Credit: USDOE) At the Institute of Reactor Research in Switzer- land, some low-level radioactive wastes are stored on site. (Credit: UNIPEDE) IAEA BULLETIN, 4/1989 Features Radioactive waste management: World overview An update of trends and developments by J.L. Zhu and C.Y. Chan With a history of over 40 years of development, the what is being done on an international basis in this field. use of the atom can be classified as a maturing technol- The perspective of this summary is primarily from ogy. However, the benefits that result from the use of civilian nuclear power programmes. the atom are not without concerns. Few topics have commanded as much attention from scientists, govern- Trends and strategies ments, and the general public over the past 30 years as the subject of "nuclear waste" (radioactive waste) and As countries pursue, plan, and implement national what to do with it. In many countries, the future and con- programmes to manage various types of radioactive tinued use of nuclear power is contingent on acceptable waste, there are similar issues and some apparent trends solutions for waste management and disposal. in the approaches and strategies. In summary: • Emphasis is being placed upon demonstrating that Almost every one of the IAEA's 113 Member States all radioactive wastes, even the most highly radioactive generates some radioactive wastes. These wastes have wastes, can be safely isolated for the required time various forms and characteristics and they arise from period from man and the environment. Most countries nuclear generation of electricity, nuclear fuel cycle with nuclear power have programmes to study, develop, activities, industrial application, and work at research and demonstrate technical solutions to safely manage centres and hospitals, for example. The actual volumes radioactive waste. The purpose of many projects for of wastes from nuclear electricity generation and other research and development and demonstration is to show nuclear applications are small compared to those of that acceptable methods exist for long-term safe disposal other technologies or industries (i.e. coal-burning power of such wastes. These developments and continued stations). However, a major concern is that some radio- studies are important for several reasons: they will test active wastes can pose a threat to man and the environ- the latest conceptual solutions and options for waste ment for long periods of time. management and disposal; they will yield further test This report summarizes the national trends and strate- data that will help to improve computerized mathemati- gies for radioactive waste management and disposal, and cal models used to make safety assessments and evalua- tions of potential geological disposal conditions; and Mr Zhu is Director of the IAEA Division of Nuclear Fuel Cycle and Waste Management and Ms Chan is a staff member of the Division. they will help assess, through analytical modelling and In the United Kingdom each year, more than 4 million cubic metres of toxic waste are produced. Only 1.1% of this amount is radioactive waste. Of this HLW small fraction, most of the waste con- tains low levels of radioactivity. Source: UKAEA 0.1% IAEA BULLETIN, 4/1989 Features Radioactive waste terms For safety and technical reasons, the various forms of • Intermediate-level wastes (ILW) contain lower levels nuclear wastes are usually categorized by their levels of of radioactivity and heat content than high-level wastes, radioactivity, heat content, and potential hazard. The but they still must be shielded during handling and trans- IAEA has established definitions describing the technical port. Such wastes may include resins from reactor opera- features of radioactive wastes that are applied to their tions or solidified chemical sludges, as well as pieces of management in many countries. For general purposes, equipment or metal fragments. Commercial engineering however, more simplified descriptions and explana- processes are being used to treat and immobilize these tions of important terms may be useful to a basic wastes; disposal in surface structures or shallow burial is understanding: practiced widely. Some countries have built or plan to build shallow repositories in rock formations on land or • Half-life. This term refers to the time it takes for any under the sea. given radionuclide to lose half of its radioactivity. Most • High-level wastes (HLW) arise from the reprocessing significant fission products, which are highly radioactive, of spent fuel from nuclear power reactors through which have half-lives of about 30 years or less; for example, uranium and plutonium can be recovered for re-use. caesium-137. A few, such as iodine-129, have half-lives These wastes contain transuranic elements, and fission in the thousands of years. For perspective, natural products that are highly radioactive, heat-generating, uranium has a half-life of about 4500 million years, or and long-lived. Liquid HLW has been effectively stored in roughly the age of the earth. tanks at specially constructed facilities. Before final • Short-lived and long-lived wastes. These terms disposal and isolation from the biosphere, they require refer to a given radioactive element's half-life. Those with treatment and solidification. Spent fuel that is not half-lives longer than approximately 30 years are gener- reprocessed may be considered a high-level waste. ally considered long-lived. • Alpha-bearing wastes (also called transuranic, • Low-level wastes (LLW) contain a negligible amount plutonium-contaminated material, or alpha wastes) of long-lived radionuclides. Produced by peaceful include wastes that are contaminated with enough long- nuclear activities in industry, medicine, research, and by lived, alpha-emitting nuclides to make disposal at a nuclear power operations, such wastes may include shallow land burial site unacceptable. They arise prin- items such as packaged gloves, rags, glass, small tools, cipally from spent fuel reprocessing and mixed-oxide fuel paper, and filters which have been contaminated by fabrication. The wastes may be disposed of in a similar radioactive material. manner to HLW. validation and laboratory research, the capability of a waste repository to protect public health safely over the Environmental assessment long-term. Additional assurance on the long-term Following the recommendations of the Post-Accident behaviour of waste is being obtained from studies of Review Meeting on the Chernobyl Accident in 1986, the natural radioactive conditions, including the behaviour IAEA established an international study aimed at utilizing of radionuclides from uranium ore bodies that have been the environmental data which exist as a result of the fall- present and undisturbed in the earth's crust for millions out from the Chernobyl release. This study, known as the of years. Validation of Model Predictions (VAMP), seeks to take the advantage of the "natural laboratory" for validating • Several countries are building or planning environmental transfer models. Such models find appli- commercial-scale reprocessing and vitrification facili- cation in assessing the radiological impacts in all parts of ties. The reprocessing of spent fuel is planned or being the nuclear fuel cycle. It operates with four separate implemented by almost one-half of the countries with working groups of experts from research institutions in nuclear power. France and the United Kingdom have more than 20 Member States and has attracted co- sponsorship from the Commission of the European Com- had commercial reprocessing capabilities for nearly a munities (CEC). VAMP is scheduled to continue until decade. However, by the early 1990s, most of the other 1992. countries planning reprocessing will have operational The IAEA is also participating in a similar interna- facilities. tional study, the Biospheric Model Validation Study To improve vitrification technologies (the immobili- (BIOMOVS), initiated in 1986 by the Swedish National zation of waste into glass or glass-like form), some Institute of Radiation Protection (SSI). This study, which countries have built or plan to build small-scale pilot began prior to the Chernobyl accident, tests models for ecological transfer and bioaccumulation of the plants to demonstrate the technology at hand. A few full- radionuclides and other tracer substances. The study scale vitrification plants are presently in operation and has changed its original schedule to consider post- other plants are either in the planning or construction Chernobyl accident data and will now continue until phase. The Australian Nuclear Science and Technology 1991. — S. Hossain, Division of Nuclear Fuel Cycle and Organization (ANSTO) has recently started integrating Waste Management its Synroc small-scale demonstration plant with a larger plant where alternative calcination methods will be developed and studied. IAEA BULLETIN, 4/1989 Features • Most countries with nuclear power programmes are developing technology for deep geologic disposal facili- ties for high-level radioactive waste (HLW). The factors Synthetic rock influencing nuclear waste management depend on the country's policy and involvement in the various stages of At
Recommended publications
  • DOE EA-2146 Final Environmental Assessment for the MARVEL
    DOE/EA-2146 Final Environmental Assessment for the Microreactor Applications Research, Validation, and Evaluation (MARVEL) Project at Idaho National Laboratory June 2021 DOE/ID-2146 Final Environmental Assessment for the Microreactor Applications Research, Validation, and Evaluation (MARVEL) Project at Idaho National Laboratory June 2021 Prepared for the U.S. Department of Energy DOE Idaho Operations Office i i CONTENTS 1. INTRODUCTION .............................................................................................................................. 1 1.1 Background .............................................................................................................................. 1 1.2 Purpose and Need ..................................................................................................................... 1 2. ALTERNATIVES .............................................................................................................................. 2 2.1 Proposed Action - Microreactor Applications Research, Validation and Evaluation (MARVEL) Project .................................................................................................................. 3 2.1.1 Reactor Structure System ............................................................................................ 5 2.1.2 Secondary Containment Structure .............................................................................. 5 2.1.3 Core System ...............................................................................................................
    [Show full text]
  • INTERSCALAR VEHICLES for an AFRICAN ANTHROPOCENE: on Waste, Temporality, and Violence
    INTERSCALAR VEHICLES FOR AN AFRICAN ANTHROPOCENE: On Waste, Temporality, and Violence GABRIELLE HECHT Stanford University http://orcid.org/0000-0003-1445-0785 Brightly painted concrete houses, equipped with running water and elec- tricity, arranged in dozens of identical rows: this photograph (Figure 1) depicts the newly built company town of Mounana in eastern Gabon. The road is clean, the children happy. In the late 1970s, this image represented Gabonese “expec- tations of modernity” (Ferguson 1999) through national and corporate projects. By the end of this essay, I hope you will also see it as an image of the African Anthropocene. The idea of an African Anthropocene may seem like a paradox. After all, the biggest appeal of the idea of the Anthropocene has been its “planetarity” (DeLoughrey 2014). For some geologists, the Anthropocene signals the start of a new epoch, one in which humans permanently mark the stratigraphic record with their “technofossils” (Zalasiewicz et al. 2014). Other earth scientists adopt the notion to signal humanity’s catastrophic effects on the planet’s physical and biochemical systems. During the past decade, the term has become a “charismatic mega-category” (Reddy 2014) across the humanities, arts, and natural and social sciences (Steffen et al. 2011; Ellsworth and Kruse 2012). Inevitably, debates rage about origins and nomenclature. Did the Anthropocene begin with the dawn of human agriculture? Or with the Columbian exchange of the sixteenth and sev- enteenth centuries? How about the start of European industrialization in the eigh- CULTURAL ANTHROPOLOGY, Vol. 33, Issue 1, pp. 109–141, ISSN 0886-7356, online ISSN 1548-1360.
    [Show full text]
  • Toxicological Profile for Plutonium
    PLUTONIUM 153 5. PRODUCTION, IMPORT/EXPORT, USE, AND DISPOSAL 5.1 PRODUCTION No information is available in the TRI database on facilities that manufacture or process plutonium because this chemical is not required to be reported under Section 313 of the Emergency Planning and Community Right-to-Know Act (Title III of the Superfund Amendments and Reauthorization Act of 1986) (EPA 1998). Plutonium was the first human-made element to be synthesized in weighable amounts. 238Pu was discovered in 1940 by Seaborg and co-workers; it was synthesized by the bombardment of uranium with deutrons (2H). Isotopes with mass numbers 228–247 have been identified; all are radioactive (Clark et al. 2006). Trace amounts of plutonium are found worldwide, mostly due to fall-out from atmospheric nuclear testing, which ended in 1980 and released several isotopes of plutonium, including 238Pu, 239Pu, 240Pu, and 241Pu (Clark et al. 2006; DOE 2005a; Eisenbud and Gesell 1997). Plutonium is not considered a naturally occurring element; however, trace amounts of 239Pu are found in naturally occurring uranium ores, but the amounts are in such small amounts that extraction is not practical (Clark et al. 2006; EPA 2006b; Lide 2008). Small amounts of 244Pu exist in nature from remnants of primordial stellar nucleosynthesis (Clark et al. 2006). Small amounts of plutonium were produced in natural reactors, such as the Oklo natural reactor in Gabon, which existed about 2 billion years ago (DOE 2005a). The most common form of plutonium found in the environment is 239Pu, followed by 240Pu (DOE 1999a). Large quantities of plutonium were first produced during the 1940’s as part of the Manhattan Project in order to produce the atomic bomb.
    [Show full text]
  • Oklo Nature’S Nuclear Reactor the Ranger Uranium Mine in Northern Australia
    Mike Follows Oklo Nature’s nuclear reactor The Ranger uranium mine in northern Australia When Enrico Fermi and his team constructed In May 1972 a scientist at the nuclear fuel- processing plant at Pierrelatte in France performed Key words their nuclear fission reactor at Stagg Field in a routine mass spectrometry analysis on a uranium nuclear fission Chicago in 1942 they would have assumed ore sample. It had been sent from the Franceville chain reaction uranium ore deposits near Oklo in Gabon, a that it was the first time a fission reaction had isotopes former French colony in West Africa. It contained taken place on the planet. But, as Mike Follows 0.7171% of U-235. The slight shortfall in the uranium explains, Nature beat them to it – and by almost expected proportion of U-235 sparked a thorough investigation. Other samples were taken. About two billion years. 500 tonnes of uranium had an average U-235 There are three principal isotopes of uranium, concentration of 0.62%, with one sample as low summarised in the table. U-235 is the most valuable as 0.44%. This meant that about 500 kg of U-235 as it is the only one that can sustain a nuclear was missing – enough to make at least half a dozen chain reaction, useful for generating power. But nuclear weapons with the destructive power of the everywhere you look – the Earth’s crust, the Moon, one dropped on Hiroshima in August 1945. even meteorites – its natural abundance is only In 1956 Paul Kuroda had published calculations 0.7202%.
    [Show full text]
  • Technetium 1 Technetium
    Technetium 1 Technetium Technetium Appearance shiny gray metal General properties Name, symbol, number technetium, Tc, 43 Pronunciation /tɛkˈniːʃiəm/ tek-NEE-shee-əm Element category transition metal Group, period, block 7, 5, d Standard atomic weight [98] g·mol−1 Electron configuration [Kr] 4d5 5s2 Electrons per shell 2, 8, 18, 13, 2 (Image) Physical properties Phase solid Density (near r.t.) 11 g·cm−3 Melting point 2430 K,2157 °C,3915 °F Boiling point 4538 K,4265 °C,7709 °F Heat of fusion 33.29 kJ·mol−1 Heat of vaporization 585.2 kJ·mol−1 Specific heat capacity (25 °C) 24.27 J·mol−1·K−1 Vapor pressure (extrapolated) P/Pa 1 10 100 1 k 10 k 100 k at T/K 2727 2998 3324 3726 4234 4894 Atomic properties [1] [2] Oxidation states 7, 6, 5, 4, 3 , 2, 1 , -1, -3 (strongly acidic oxide) Electronegativity 1.9 (Pauling scale) Ionization energies 1st: 702 kJ·mol−1 2nd: 1470 kJ·mol−1 3rd: 2850 kJ·mol−1 Atomic radius 136 pm Covalent radius 147±7 pm Miscellanea Technetium 2 Crystal structure hexagonal close packed Magnetic ordering Paramagnetic Thermal conductivity (300 K) 50.6 W·m−1·K−1 Speed of sound (thin rod) (20 °C) 16,200 m/s CAS registry number 7440-26-8 Most stable isotopes iso NA half-life DM DE (MeV) DP 95mTc syn 61 d ε - 95Mo γ 0.204, - 0.582, 0.835 IT 0.0389, e 95Tc 96Tc syn 4.3 d ε - 96Mo γ 0.778, - 0.849, 0.812 97 6 97 Tc syn 2.6×10 y ε - Mo 97mTc syn 91 d IT 0.965, e 97Tc 98Tc syn 4.2×106 y β− 0.4 98Ru γ 0.745, 0.652 - 99Tc trace 2.111×105 y β− 0.294 99Ru 99mTc syn 6.01 h IT 0.142, 0.002 99Tc γ 0.140 - Technetium is the chemical element with atomic number 43 and symbol Tc.
    [Show full text]
  • ()I'i'nfi.Ktil" \ ,.& 8444'' ''' ,..4.+4":".^
    NikI*011.1) 111,1i III ()1(i,\NII \ I I()N.. t.i..(11()1\t..,\ )le..11( 1 I OR Ilk()P1 ()I'I'Nfi.ktil" \ ,.& 8444'' ''' ,..4.+4":".^ ' ' ... Cover: The Advanced Gas -Cooled Reactor at Windscale, England. Reproduced by kind permission of the United Kingdom Atomic Energy Authority. WHO Regional Publications European Series No. 3 HEALTH IMPLICATIONS OF NUCLEAR POWER PRODUCTION Report on a Working Group Brussels, 1 -5 December 1975 WORLD HEALTH ORGANIZATION REGIONAL OFFICE FOR EUROPE COPENHAGEN 1978 ISBN 92 9020 103 7 © World Health Organization 1977 Publications of the World Health Organization enjoy copyright protec- tion in accordance with the provisions of Protocol 2 of the Universal Copy- right Convention. For rights of reproduction or translation, in part or in toto, of publications issued by the WHO Regional Office for Europe application should be made to that Office, Scherfigsvej 8, DK -2100 Copenhagen 0, Denmark. The Regional Office welcomes such applications. The designations employed and the presentation of the material in this publication do not imply the expression of any opinion whatsoever on the part of the Secretariat of the World Health Organization concerning the legal status of any country, territory, city or area or of its authorities, or con- cerning the delimitation of its frontiers or boundaries. The mention of specific companies or of certain manufacturers' products does not imply that they are endorsed or recommended by the World Health Organization in preference to others of a similar nature that are not men- tioned. Errors and omissions excepted, the names of proprietary products are distinguished by initial capital letters.
    [Show full text]
  • “Advanced” Isn't Always Better
    SERIES TITLE OPTIONAL “Advanced” Isn’t Always Better Assessing the Safety, Security, and Environmental Impacts of Non-Light-Water Nuclear Reactors “Advanced” Isn’t Always Better Assessing the Safety, Security, and Environmental Impacts of Non-Light-Water Nuclear Reactors Edwin Lyman March 2021 © 2021 Union of Concerned Scientists All Rights Reserved Edwin Lyman is the director of nuclear power safety in the UCS Climate and Energy Program. The Union of Concerned Scientists puts rigorous, independent science to work to solve our planet’s most pressing problems. Joining with people across the country, we combine technical analysis and effective advocacy to create innovative, practical solutions for a healthy, safe, and sustainable future. This report is available online (in PDF format) at www.ucsusa.org/resources/ advanced-isnt-always-better and https:// doi.org/10.47923/2021.14000 Designed by: David Gerratt, Acton, MA www.NonprofitDesign.com Cover photo: Argonne National Laboratory/Creative Commons (Flickr) Printed on recycled paper. ii union of concerned scientists [ contents ] vi Figures, Tables, and Boxes vii Acknowledgments executive summary 2 Key Questions for Assessing NLWR Technologies 2 Non-Light Water Reactor Technologies 4 Evaluation Criteria 5 Assessments of NLWR Types 8 Safely Commercializing NLWRs: Timelines and Costs 9 The Future of the LWR 9 Conclusions of the Assessment 11 Recommendations 12 Endnotes chapter 1 13 Nuclear Power: Present and Future 13 Slower Growth, Cost and Safety Concerns 14 Can Non-Light-Water Reactors
    [Show full text]
  • OKLO REACTORS : 2 Billion Years Before Fermi !
    OKLO REACTORS : 2 billion Years before Fermi ! Bertrand BARRÉ, AREVA « The italian Navigator has landed in the New World » And not even a photographer… 2 - B. Barré OKLO séminaire GIFT - 2005 Then and Now X 2000 million years ago X Today 3 - B. Barré OKLO séminaire GIFT - 2005 Detective Story X June 1972 X Pierrelatte Nuclear Fuel Enrichment plant was using ore from Gabon (deposits discovered in 60’s) X Shipment of U routine mass spec. measurements of 235U/ 238U ratio (0.7171% instead of 0.7202%), and no 236U… X Talk about paying attention to details! X Pierrelatte > Malvesi > Gueugnon > Mounana > Oklo (north) 4 - B. Barré OKLO séminaire GIFT - 2005 Where is Oklo? 5 - B. Barré OKLO séminaire GIFT - 2005 Franceville Basin 6 - B. Barré OKLO séminaire GIFT - 2005 7 - B. Barré OKLO séminaire GIFT - 2005 Oklo, Gabon (CEA 1974) 8 - B. Barré OKLO séminaire GIFT - 2005 OKLO Mining Operations Nov1970-Dec1971 9 - B. Barré OKLO séminaire GIFT - 2005 Open Pit Mining in Oklo Mined ore Excavation Ore in place Drillings Very rich « lens » 10 - B. Barré OKLO séminaire GIFT - 2005 The OKLO Mine 11 - B. Barré OKLO séminaire GIFT - 2005 Mounana Plant Nov1970-Dec1971 U concentration in ore vs 235U abundance 12 - B. Barré OKLO séminaire GIFT - 2005 Reminder… X 235U is desired form of Uranium for thermal fission X Reactors (other than CANDU and Magnox) require enrichment : X MTR (old) :93% X MTR (new): 20% X LWR : 3.2-4.5% 13 - B. Barré OKLO séminaire GIFT - 2005 A Window in Time X Before 2.2 billion years ago, no uranium deposit, because not enough oxygen in atmosphere and therefore water X After 1.4 billion years ago, 235U abundance too low Remember… The Americas separated from EurAsia and Africa less than 200 million years ago 14 - B.
    [Show full text]
  • Nuclear Energy Today
    Cov-Nuc Energy Today 4/06/03 11:38 Page 1 Nuclear Development Nuclear Energy Today NUCLEAR•ENERGY•AGENCY 1-RefBook 20 May 2003 23/05/03 19:09 Page 1 Nuclear Development Nuclear Energy Today NUCLEAR ENERGY AGENCY ORGANISATION FOR ECONOMIC CO-OPERATION AND DEVELOPMENT 1-RefBook 20 May 2003 23/05/03 19:09 Page 2 Foreword All the forecasts of world energy demand for the next 50 years point towards very significant increases in consumption. A big share of this new demand will come from areas of the world where existing energy consumption is now relatively low in comparison with the OECD countries, and which are becoming increasingly integrated in the global economy. As energy demand grows, all societies worldwide will face a real challenge in providing the energy needed to feed economic growth and improve social development, while enhancing protection of the environment. In this context, it is not difficult to conclude that it is the responsibility of policy makers to establish energy policies that meet that challenge while being robust enough to cope with the risks associated with the globalisation of the world economy. Diversification, security of supply, protection of the environment and technology development are key elements of any energy policy that tries to put into the markets enough energy at a reasonable price in a sustainable way. Among the different energy sources that are contributing significantly to world supply none appears to policy makers as more complex than nuclear energy. The economic, technological and social implications of nuclear power makes any decision something that goes far beyond the normal actors of the market place.
    [Show full text]
  • Interscalar Vehicles for the African Anthropocene: on Waste, Temporality, and Violence
    Interscalar Vehicles for the African Anthropocene: On Waste, Temporality, and Violence Gabrielle Hecht author correspondence to [email protected] Mounana, Gabon, late 1970s. Courtesy of Cogéma. Used with Permission. Brightly painted concrete houses, equipped with running water and electricity, arranged in dozens of identical rows: this photograph depicts the newly built company town of Mounana in eastern Gabon. The road is clean, the children happy. In the late 1970s, this image aimed to represent the success of national and corporate modernity projects. By the end of this essay, I hope you will also see it as an image of the African Anthropocene. manuscript under review. do not cite without explicit author permission. not for circulation beyond seminar participants. 2 The idea of an African Anthropocene may seem like a paradox. After all, the biggest appeal of the Anthropocene idea has been its “planetarity.”1 For some geologists, the Anthropocene signals the start of a new epoch, in which humans permanently mark the stratigraphic record with their “technofossils.”2 Other earth scientists adopt the notion to signal humanity’s catastrophic effects on the planet’s physical and biochemical systems. Over the last decade, the term has become a “charismatic mega-category”3 across the humanities, arts, and natural and social sciences.4 Inevitably, debates rage about origins and nomenclature. Did the Anthropocene begin with the dawn of human agriculture? Or with the Columbian exchange of the 16th and 17th centuries? How about the start of European industrialization in the 18th century? Some favor July 16, 1945, date of the first nuclear weapons test at Alamogordo.5 While geologists ponder the stratigraphic signals left by each of these options, humanists and social scientists worry about their political and ethical implications.
    [Show full text]
  • Oklo Natural Nuclear Reactor
    Oklo Natural Nuclear Reactor Brandon Clary HUGS 2016 6/16/2016 Outline • Before Oklo • Discovery of the Oklo anomaly • Explanation of anomaly • Operation of Oklo • Implications of Oklo research Aerial view of the Oklo open mine pit in Gabon, Africa. Before Oklo • (1942) Chicago Pile goes online, and is self-sustaining. • (1953) George W. Wetherill & Mark Inghram find evidence of neutron induced fission in a Congo pitchblende. • (1956) A chemist by the name Kuroda sketches out the requirements necessary for natural nuclear fission. • From 1957 until mid 1973 no known Chicago Pile-1, the first self-sustaining manmade natural fission detected. nuclear reactor. Kuroda’s Requirement • Quantity: Abundance of fissile uranium 235U isotope. • Size: Uranium deposit should exceed the average length that fission-inducing neutrons travel (~2/3 meter). ~3% weapons grade. • Moderator: Neutron moderator, a substance that can slow down neutrons produced through Isotopic amount of 235U as a function fission. of millions of years ago [1] • Lack of poisons: Elements that absorb neutrons Uranium Absorption cross Isotope section should not be present (boron, lithium, etc). U-235 680.9 barns Reported cross section for uranium- 235 [2] Oklo Anomaly • French uranium enrichment center detects anomaly in isotopic ratio for UF6. • Analysis reveals isotopic abundance of 235U in sample core from Gabon is 238U 99.2744 0.6000% instead of 235U 0.7202 0.7202%.[3] 234 • Corresponds to U 0.0054 approximately 200 Percent present day abundances kilograms of missing 235U. of common uranium isotopes [4] Explanation of Oklo Anomaly • CEA and International Atomic Energy Agency form committee for investigation.
    [Show full text]
  • February 2005
    The natural Reactors at Oklo (Gabon): 2 billion Years before Fermi! Bertrand BARRÉ, AREVA (Synopsis) 1. The Italian Navigator has landed in the New World. On December 2, 1942, this cryptic message announced that the team gathered around Enrico Fermi in Chicago had managed to sustain a fission chain reaction in the first ever man made nuclear reactor, CP1. This was the climax of a decade long search, starting with the discovery by Chadwick in 1932 of the neutron, a particle able to interact with the nuclei without being hampered by their electric charges, the series of experiments by Fermi sending “moderated” neutrons against every nucleus of the Mendeleyev Table, the discovery of the fission of uranium by Otto Hahn and Lise Meitner in 1938. When the team led by Joliot discovered, a few months later, that 2 to 3 new neutrons were emitted during the fission, they were able to conceptually design a nuclear reactor, a facility using a sustained fission chain reaction to generate vast amounts of energy, but World War 2 shifted the research efforts to America. And for three decades, it was believed that CP1 was not only the first man made reactor, but the first nuclear reactor ever – full stop. 2. Radioactive Earth. Not everybody realizes that geothermal energy is just another name to describe the radioactivity of our planet. Among the heavier elements retained during the formation of Earth (most of the lightest elements escaped its too small gravity), a number have only radioactive isotopes. Potassium1, Thorium and Uranium are the most abundant remaining today.
    [Show full text]