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This Issue Is Dedicated to Professor Francesco De Simone on the Occasion of His 72Nd Birthday

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This Issue Is Dedicated to Professor Francesco De Simone on the Occasion of His 72Nd Birthday This Issue is Dedicated to Professor Francesco De Simone on the Occasion of his 72nd Birthday Volume 4. Issue 12. Pages 1615-1798. 2009 ISSN 1934-578X (printed); ISSN 1555-9475 (online) www.naturalproduct.us NPC Natural Product Communications EDITOR-IN-CHIEF HONORARY EDITOR DR. PAWAN K AGRAWAL PROFESSOR GERALD BLUNDEN Natural Product Inc. The School of Pharmacy & Biomedical Sciences, 7963, Anderson Park Lane, University of Portsmouth, Westerville, Ohio 43081, USA Portsmouth, PO1 2DT U.K. [email protected] [email protected] EDITORS PROFESSOR ALESSANDRA BRACA ADVISORY BOARD Dipartimento di Chimica Bioorganicae Biofarmacia, Universita di Pisa, Prof. Berhanu M. Abegaz Prof. Hartmut Laatsch via Bonanno 33, 56126 Pisa, Italy Gaborone, Botswana Gottingen, Germany [email protected] Prof. Viqar Uddin Ahmad Prof. Marie Lacaille-Dubois PROFESSOR DEAN GUO Karachi, Pakistan Dijon, France State Key Laboratory of Natural and Biomimetic Drugs, Prof. Øyvind M. Andersen Prof. Shoei-Sheng Lee School of Pharmaceutical Sciences, Bergen, Norway Taipei, Taiwan Peking University, Beijing 100083, China Prof. Giovanni Appendino Prof. Francisco Macias [email protected] Novara, Italy Cadiz, Spain PROFESSOR J. ALBERTO MARCO Prof. Yoshinori Asakawa Prof. Anita Marsaioli Departamento de Quimica Organica, Tokushima, Japan Campinas, Brazil Universidade de Valencia, Prof. Lee Banting E-46100 Burjassot, Valencia, Spain Prof. Imre Mathe Portsmouth, U.K. Szeged, Hungary [email protected] PROFESSOR YOSHIHIRO MIMAKI Prof. Anna R. Bilia Prof. Joseph Michael Florence, Italy Johannesburg, South Africa School of Pharmacy, Tokyo University of Pharmacy and Life Sciences, Prof. Maurizio Bruno Prof. Ermino Murano Horinouchi 1432-1, Hachioji, Tokyo 192-0392, Japan Palermo, Italy Trieste, Italy [email protected] Prof. Josep Coll Prof. Virinder Parmar PROFESSOR STEPHEN G. PYNE Barcelona, Spain Delhi, India Department of Chemistry University of Wollongong Prof. Geoffrey Cordell Prof. Luc Pieters Chicago, IL, USA Antwerp, Belgium Wollongong, New South Wales, 2522, Australia [email protected] Prof. Samuel Danishefsky Prof. Om Prakash PROFESSOR MANFRED G. REINECKE New York, NY, USA Manhattan, KS, USA Department of Chemistry, Prof. Duvvuru Gunasekar Prof. Peter Proksch Texas Christian University, Tirupati, India Düsseldorf, Germany Forts Worth, TX 76129, USA [email protected] Prof. A.A. Leslie Gunatilaka Prof. Satyajit Sarker Tucson, AZ, USA Wolverhampton, UK PROFESSOR WILLIAM N. SETZER Department of Chemistry Prof. Stephen Hanessian Prof. Raffaele Riccio The University of Alabama in Huntsville Montreal, Canada Salerno, Italy Huntsville, AL 35809, USA Prof. Kurt Hostettmann [email protected] Prof. Monique Simmonds Lausanne, Switzerland Richmond, UK PROFESSOR YASUHIRO TEZUKA Prof. Martin A. Iglesias Arteaga Institute of Natural Medicine Prof. Valentin Stonik Mexico, D. F, Mexico Institute of Natural Medicine, University of Toyama, Vladivostok, Russia 2630-Sugitani, Toyama 930-0194, Japan Prof. Jerzy Jaroszewski Prof. Hiromitsu Takayama [email protected] Copenhagen, Denmark Chiba, Japan PROFESSOR DAVID E. THURSTON Prof. Leopold Jirovetz Prof. Karen Valant-Vetschera Department of Pharmaceutical and Biological Chemistry, Vienna, Austria Vienna, Austria The School of Pharmacy, Prof. Teodoro Kaufman Prof. Peter G. Waterman University of London, 29-39 Brunswick Square, Rosario, Argentina Lismore, Australia London WC1N 1AX, UK [email protected] Prof. Norbert De Kimpe Prof. Paul Wender Gent, Belgium Stanford, USA INFORMATION FOR AUTHORS Full details of how to submit a manuscript for publication in Natural Product Communications are given in Information for Authors on our Web site http://www.naturalproduct.us. Authors may reproduce/republish portions of their published contribution without seeking permission from NPC, provided that any such republication is accompanied by an acknowledgment (original citation)-Reproduced by permission of Natural Product Communications. Any unauthorized reproduction, transmission or storage may result in either civil or criminal liability. The publication of each of the articles contained herein is protected by copyright. Except as allowed under national “fair use” laws, copying is not permitted by any means or for any purpose, such as for distribution to any third party (whether by sale, loan, gift, or otherwise); as agent (express or implied) of any third party; for purposes of advertising or promotion; or to create collective or derivative works. Such permission requests, or other inquiries, should be addressed to the Natural Product Inc. (NPI). A photocopy license is available from the NPI for institutional subscribers that need to make multiple copies of single articles for internal study or research purposes. To Subscribe: Natural Product Communications is a journal published monthly. 2009 subscription price: US$1,695 (Print, ISSN# 1934-578X); US$1,395 (Web edition, ISSN# 1555-9475); US$2,095 (Print + single site online). Orders should be addressed to Subscription Department, Natural Product Communications, Natural Product Inc., 7963 Anderson Park Lane, Westerville, Ohio 43081, USA. Subscriptions are renewed on an annual basis. Claims for nonreceipt of issues will be honored if made within three months of publication of the issue. All issues are dispatched by airmail throughout the world, excluding the USA and Canada. Natural Product Communications Vol. 4 (12) 2009 Published online (www.naturalproduct.us) Editorial In Honor of the 72nd Birthday of Professor Francesco De Simone It is our great privilege and pleasure to introduce this issue, which is dedicated to Prof. Francesco De Simone, Professor of Pharmaceutical Technology, Faculty of Pharmacy, Department of Pharmaceutical Science, University of Salerno, on the occasion of his 72nd birthday. Prof. De Simone has made many outstanding contributions to the field of natural products science, particularly for the conservation of biodiversity through drug discovery. His research has been based on various aspect of modern pharmacognosy, offering valuable contributions to phytochemistry, food chemistry, and, more recently, pharmaceutical technology applied to herbal drug preparations. During his distinguished and productive career, spanning over 45 years, Francesco De Simone has either authored or co- authored over 200 peer-reviewed scientific publications, 15 book chapters, some patent applications, and a great number of contributions in congress proceedings. Prof. De Simone, during his research activity, has paid particular attention to the enhancement of the value of traditional medicine in Latin American countries, including the conservation of their cultural and natural value. His efforts have represented an excellent opportunity to improve collaboration and to re-enforce networks between Italian and Latin American research groups. This issue, on the occasion of his 72nd birthday on June 27, 2009, represents a tribute to his outstanding scientific contributions and an opportunity to express congratulations and best wishes from all of us, colleagues and friends. Our personal thanks go also to all the authors, mostly of them Prof. De Simone’s friends, and reviewers who have contributed to the success of this special issue. Nunziatina De Tommasi Alessandra Braca Pawan K. Agrawal Natural Product Communications Vol. 4 (12) 2009 Published online (www.naturalproduct.us) Preface It is a pleasure for me, as a colleague and friend, to send wishes to Prof. Francesco De Simone on the occasion of his 72ns birthday. The first time I met Prof. De Simone was in October 1969, when I entered, as a student, the Institute of Medicinal and Toxicological Chemistry of the University of Naples. A strong friendship was quickly created between us: I have always appreciated the ecleptic knowledge of Prof. De Simone and his open minded vision of the world. From the beginning of the 1980s and for almost 20 years, we have been collaborating in very productive scientific work, studying the phytochemistry of medicinal plants from all over the world, but mainly from South America. During this period, mainly due to his efforts, a generation of highly able scientists has been created operating in the field of natural products. Apart from the high scientific value of Prof. De Simone as a chemist, I also recognize his ability in organizing and promoting science. From the end of the 1980s Prof. De Simone has been the main player in the activation of the Faculty of Pharmacy at the University of Salerno, which is now a well organized and active Faculty. Prof. De Simone also deserves great credit for his efforts as Dean in the periods 1994-1999 and 2004-2008. Prof. Francesco De Simone’s research has focused on all major aspects of natural product science, including isolation, structure elucidation, and the biological evaluation of natural compounds in medicinal plants, foods and cosmetics. To Francesco, a very outstanding scientist, sincere thanks for his contribution to Phytochemistry! Prof. Cosimo Pizza Chairman of Italian Society of Phytochemistry University of Salerno, Department of Pharmaceutical Sciences Via Ponte Don Melillo 84084 Fisciano (SA), Italy A Friend Named Ciccio I met for the first time Professor Francesco De Simone (friends call him ‘Ciccio’) in the Spring of 1995 when he, as Dean of the Faculty of Pharmacy, asked me to move from University of Naples to the University of Salerno. I was somewhat sceptical, but, at the same time, I was impressed by his ability to list all
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