PHYSICAL REVIEW RESEARCH 2, 013231 (2020)
Chiral magnonic edge states in ferromagnetic skyrmion crystals controlled by magnetic fields
Sebastián A. Díaz ,1 Tomoki Hirosawa ,2 Jelena Klinovaja,1 and Daniel Loss 1 1Department of Physics, University of Basel, Klingelbergstrasse 82, 4056 Basel, Switzerland 2Department of Physics, University of Tokyo, Bunkyo, Tokyo 113-0033, Japan
(Received 5 November 2019; accepted 23 January 2020; published 28 February 2020)
Achieving control over magnon spin currents in insulating magnets, where dissipation due to Joule heating is highly suppressed, is an active area of research that could lead to energy-efficient spintronics applications. However, magnon spin currents supported by conventional systems with uniform magnetic order have proven hard to control. An alternative approach that relies on topologically protected magnonic edge states of spatially periodic magnetic textures has recently emerged. A prime example of such textures is the ferromagnetic skyrmion crystal which hosts chiral edge states providing a platform for magnon spin currents. Here we uncover that an external magnetic field can drive a topological phase transition in the spin-wave spectrum of a ferromagnetic skyrmion crystal. The topological phase transition is signaled by the closing of a low-energy bulk magnon gap at a critical field. In the topological phase, below the critical field, two topologically protected chiral magnonic edge states lie within this gap, but they unravel in the trivial phase, above the critical field. Remarkably, the topological phase transition involves an inversion of two magnon bands that at the point correspond to the breathing and counterclockwise modes of the skyrmions in the crystal. Our findings suggest that an external magnetic field could be used as a knob to switch on and off magnon spin currents carried by topologically protected chiral magnonic edge states.
DOI: 10.1103/PhysRevResearch.2.013231
I. INTRODUCTION nascent field of topological magnonics [19–21] is ferromag- netic (FM) skyrmion crystals (SkXs) [22,23], whose magnetic A major obstacle to meeting the demand for ever smaller texture is shown in Fig. 1. Although their low-energy spin- logic and storage devices, based on expectations set by wave modes have been investigated before [24–27], only re- Moore’s law, is the pernicious effect of Joule heating [1]. cently were they predicted to host chiral magnonic edge states Two diverging approaches relying on spin degrees of freedom protected by the nontrivial topology of their bulk magnon instead of electric charges have come to the rescue. Embracing bands [28]. heating effects and trying to utilize them to produce electronic In contrast to electronic topological insulators, ground- spin currents is the goal of the field of spin caloritronics [2]. state magnetic phases such as FM SkXs, and consequently the Alternatively, avoiding displacing electric charges altogether spin-wave spectrum they support, depend crucially on applied can be achieved via spin currents carried by magnons in magnetic fields. Therefore, it is a nontrivial question whether insulating magnets [3–6]. While several magnonic analogs of a magnetic field can drive a topological phase transition in electronic phenomena that could help design the next gener- ation of energy efficient devices have already been identified the spin-wave spectrum without drastically modifying the [3,7–9], a growing niche for magnon spin current applications ground-state texture. Quite remarkably, we discover that there that stray from those inspired by conventional electronics has is a window of magnetic-field values where such a phase tran- recently emerged [10,11]. sition between two topologically distinct spin-wave spectra of Despite progress on launching and getting a handle on the the FM SkX can be observed. It involves two low-energy bulk directionality of magnon spin waves [12–15], reliable control magnon bands, which at the point correspond to the counter- of their propagation and robustness against sample imperfec- clockwise and breathing modes [26]. Experimental studies in tions are still lacking. Realizing such control could be attained bulk chiral magnets showed that the energy difference of these in topological magnon insulators [16–18], systems with a modes gets smaller with increasing magnetic field, but it does spatially periodic magnetic texture that support topologically not vanish upon reaching the boundary with the conical phase protected magnonic edge states. A promising platform for the [27]. On the other hand, our two-dimensional model predicts a critical magnetic-field value at which these two bands touch at the point, closing a magnon gap and signaling the topological phase transition. Increasing the magnetic field past this critical value reopens the gap, the bands exchange Chern Published by the American Physical Society under the terms of the numbers, and band inversion takes place in the vicinity of Creative Commons Attribution 4.0 International license. Further the gap-closing point. Furthermore, topologically protected distribution of this work must maintain attribution to the author(s) chiral magnonic edge states within this gap are only supported and the published article’s title, journal citation, and DOI. in the phase below the critical field. Therefore, an external
2643-1564/2020/2(1)/013231(9) 013231-1 Published by the American Physical Society DÍAZ, HIROSAWA, KLINOVAJA, AND LOSS PHYSICAL REVIEW RESEARCH 2, 013231 (2020)
partitioned as r = R + r j. The Hamiltonian of free spin waves is then obtained, by taking a lattice Fourier transform, as the O(S) piece in the expansion 1 H = S † H (k) + E . (2) SW 2 ki ij k j 0 k;i, j − · + Here = (a , a† )T , a = √1 e ik (R r j )a , E = ki ki −ki k j N R R j 0 − 1 2 NS i i, with N the total number of magnetic unit cells, (k) − (k) H = ij ij , ij(k) − ∗ − ∗ − (3) ij( k) ij( k)
where (k) = 1 [J (k)e+ · e+ + D (k) · e+ × e+], (k) ij 2 ij i j ij i j ij = δ − 1 + · − + · + × − = ij i 2 [Jij(k)ei e j Dij(k) ei e j ], i j[Jij FIG. 1. Ferromagnetic skyrmion crystal texture. Triangular crys- = 3 · 3 + = · 3 × 3 − 3 · = μ (k 0)ei e j Dij(k 0) ei e j ] bJei zˆ, with b g B tal of ferromagnetic Néel skyrmions obtained from the classical −ik·(R+r −r ) B/JS, J (k) = J + , e i j , and mutatis mutandis ground-state texture of the spin-lattice Hamiltonian model for D/J = ij R R ri r j { 1, 2, 3} 1.0andb = 0.8. The out-of-plane component of the moments is for Dij(k). The orthonormal frame e j e j e j is defined at 3 color coded. each magnetic unit cell site j, where e j is parallel to the ± = 1 ± 2 classical ground-state spin texture and e j e j ie j . magnetic field could be used to control the propagation of A paraunitary Bogoliubov transformation Tk diagonalizes robust magnon spin currents with a defined directionality the above spin-wave Hamiltonian yielding along the edge of FM SkXs in thin films. † 1 H = S E λ α α λ + + E , (4) SW k kλ k 2 0 II. SPIN WAVES IN A FERROMAGNETIC k,λ SKYRMION CRYSTAL α† where kλ creates magnons with crystal momentum k at The FM SkX is obtained from the classical ground-state the λth band whose energy is given by Ekλ. Each band can texture of spin-S operators on a triangular lattice (with lattice be classified by their Chern number, a topological index constant a) governed by the Hamiltonian defined in reciprocal space, given by an integral over the first Cλ = i dk μν {Pλ k ∂ Pλ k ∂ Pλ k }/ π 1 Brillouin zone, Tr ( )[ kμ ( )] kν ( ) 2 , † H =− (Jr,r Sr · Sr + Dr,r · Sr × Sr ) = σ σ with Pλ(k) Tk λ zTk z a projection operator and 2 r,r ( λ) = δλ δ [16]. ij i ij We numerically compute the bulk magnon band structure + gμ B S · zˆ, (1) B r and the Chern number of the lowest-energy bands as a func- r tion of external magnetic field. Using magnon coherent states = including nearest-neighbor exchange Jr,r J and interfacial (details in Appendix B), we also obtain the time evolution Dzyaloshinskii-Moriya (DM) interactions Dr,r = D zˆ × (r − of the real-space deformation of the FM SkX for those same r )/|r − r | as well as a coupling to an external magnetic bands. field Bzˆ, where g is the gyromagnetic ratio and μB is the Bohr magneton. Focusing on zero temperature, we use Monte III. NEARLY FLAT AND DISPERSIVE BANDS Carlo simulated annealing [29] followed by further time evo- lution employing a restricted Landau-Lifshitz-Gilbert (LLG) Now we discuss the magnon bands. Figures 2(a)–2(d) show equation [30] to obtain the classical ground-state spin texture the lowest-energy bulk magnon bands for increasing values of as a function of the magnetic field. The magnetic moment the (rescaled) external magnetic field b. The majority of the texture of the FM SkX is related to the classical ground-state bands are dispersive, but a few of them appear to be nearly spin texture by Mr =− g.s.|Sr|g.s. , whose direction mˆ r = flat. As the magnetic field increases, the nearly flat bands are Mr/|Mr| is shown in Fig. 1. shifted to higher energies, while the dispersive bands remain Spin waves are described by rotating the spin quantization almost unaffected. Moreover, overlapping bands belonging axis at each lattice site along the direction of the FM SkX to these two different classes hybridize less the lower their spin texture so that the rotated spin operators model collective energy is. At the point, for k = 0, time evolution reveals excitations about this classical ground state. Assuming small that the nearly flat bands correspond to elliptical, triangular, deviations, we employ a standard transformation mapping the square, and pentagonal distortions of the individual skyrmions rotated spin operators to Holstein-Primakoff bosons [31] ar in the FM SkX [see Fig. 2(e)]. As time evolves, these localized † / and ar to then expand in powers of 1 S [32]. deformations rotate clockwise, retaining their shape, about the The FM SkX is a triangular crystal of skyrmions. Its center of each skyrmion and uniformly across the FM SkX. magnetic unit cell, a single skyrmion, consists of many spins. For k = 0, the distortions of individual skyrmions are iden- This is naturally described by a triangular Bravais lattice R tical up to a phase eik·r, as expected of spatially modulated, with a basis r j. Therefore, the triangular lattice of spins is propagating spin waves (see Fig. 5 in Appendix B).
013231-2 CHIRAL MAGNONIC EDGE STATES IN FERROMAGNETIC … PHYSICAL REVIEW RESEARCH 2, 013231 (2020)
b =0.5 b =0.6 b =0.7 b =0.8 E m =5 (a) (b) (c) (d) (e) JS 2.5 m =4 m =5 m =4 m =4 2.0 m =4 m =4 1.5 m =3 m =3 m =3 1.0 m =3 m =3 m =2 0.5 m =2 m =2 m =2
0.0 m =2
FIG. 2. Magnetic-field dependence of the magnon spectrum. (a)–(d) Bulk magnon spectra of the FM SkX along the first Brillouin zone loop K- -M-K for increasing values of the applied magnetic field b = gμBB/JS. Nearly flat (dispersive) bands are depicted in purple (gray). The counterclockwise (A), breathing (B), and clockwise (C) modes are respectively denoted in blue, red, and green. (e) Localized skyrmion distortions corresponding to the nearly flat bands from (a)–(d), labeled by their azimuthal number m.
The above modes are expected to be part of the magnon number of the lowest-energy bands as the magnetic field is spectrum because they also appear in the spectrum of isolated increased, we observe no exchange of Chern number between skyrmions [33,34] and are known to affect their dynamics nearly flat and dispersive bands. Therefore, these two distinct [35]. In analogy to small distortions of a circular domain classes of bands are topologically decoupled. wall, which can be classified by their azimuthal number m ∈ {0, 1, 2,...}, we also label these magnon bands by m [36,37]. IV. TOPOLOGICAL PHASE TRANSITION Although not as flat as the others, but sharing the same real-space time evolution features, the second lowest-energy Next we turn to the topological phase transition. As shown band corresponds to m = 2. Note, however, that it flattens in the sequence from Fig. 2, the counterclockwise and breath- out with increasing magnetic field because, as skyrmions ing modes approach each other when the magnetic field shrink, their overlap with nearest neighbors decreases, hence increases. By further ramping up the field we observe the approaching the isolated skyrmion limit. The lowest-energy third bulk magnon gap closing and then reopening with the band corresponds to a localized gyrotropic mode, a remnant of two bands touching at the point at a critical field bc = 0.88 the translational modes (m = 1) of the isolated skyrmion [25]. forming a Dirac-like point [see Fig. 3(b)]. This gap closing Remarkably, the Chern number of all the nearly flat bands is is profoundly different from the others involving nearly flat zero. bands as evidenced by the spin-wave modes in the vicinity Among the dispersive modes there are three of special of the point. For magnetic fields smaller than the critical importance: counterclockwise (A), breathing (B), and clock- value b < bc, the third band corresponds to the counterclock- wise (C). They correspond to skyrmion distortions in the wise mode and the fourth band to the breathing mode [see = vicinity of k 0 [see Figs. 2(a)–2(d)]. First predicted by LLG Fig. 3(a)]. On the other hand, for b > bc, these spin-wave simulations [26], these three low-energy modes can be excited modes are inverted [see Fig. 3(c)]. However, band inversion by spatially uniform AC magnetic fields: out of plane for the does not guarantee the occurrence of a topological phase breathing mode and in plane for the counterclockwise and transition [41]. clockwise modes. They have been observed experimentally in A better assessment of the nature of the spin-wave spec- bulk samples of chiral [27,38,39] and polar magnets [40]. trum changes with magnetic field is given by tracking the Isolated skyrmions also support a localized breathing Chern numbers. For external magnetic fields larger than the = mode, with azimuthal number m 0, characterized by axially critical value, the third band exhibits a change from C3 = 1to symmetric distortions of their size, periodically shrinking C3 = 0[seeFig.3(d)], becoming topologically trivial, while and expanding. However, the breathing mode present in the the fourth band jumps from C4 = 1toC4 = 2: A transfer of FM SkX magnon spectrum is not localized because of the Chern number takes place. strong overlap experienced by neighboring skyrmions as they Increasing the magnetic field in this range merely shrinks expand. the size of the skyrmions in the FM SkX without breaking any When a nearly flat band passes through a dispersive symmetries. Nevertheless, the bulk magnonic band structure one, the spin-wave mode associated with each band remains experiences a clear change in its topology. Thus, the system largely the same. Despite their overlap in energy, the bands indeed is expected to undergo a topological phase transition hardly hybridize with each other. By tracking the Chern at bc.
013231-3 DÍAZ, HIROSAWA, KLINOVAJA, AND LOSS PHYSICAL REVIEW RESEARCH 2, 013231 (2020)
E (a) (b) (c) Obtaining a finite system by simply cutting the infinite JS bulk texture of the FM SkX arbitrarily is likely to result in a 1.5 spin configuration that is neither the global nor a local energy minimum and for which magnons cannot be properly defined. To avoid this issue, we place our system on a generic strip
1.0 geometry where the edges are a result of sample termination. By recomputing the minimum-energy spin configuration of the system in this new geometry, we make sure we obtain more physical bulk and edge textures. 0.5 On the new geometry, the FM SkX reconstructs near the b
0.4 0.04 Topologically protected edge state bands are expected to extend across the gaps connecting consecutive sets of bulk 0.2 0.02 0.0 subbands. 0.00 0.6 0.7 0.8 0.9 0.80 0.85 0.90 0.95 In Figs. 4(a) and 4(c) we show the one-dimensional band b b structure for b = 0.80 and b = 0.95, respectively, of the pris- (f) tine FM SkX. Consistent with the prediction of the bulk-edge correspondence, while there are no edge states within either the first or second gap, they appear within the third gap for both magnetic-field values. However, only in the topological < (g) phase b bc are edge states extending across the third gap present (blue and red), while topologically trivial edge states (purple) can be seen in the third gap of both phases. To expose the topologically protected edge states while t =0 t = T/4 t = T/2 t =3T/4 at the same time removing the topologically trivial ones, we introduce a special type of disorder by applying a larger FIG. 3. Magnetic-field-driven topological phase transition. (a)– magnetic field along a narrow sliver near the strip edges. (c) Bulk magnon spectrum of the FM SkX in the vicinity of the The texture is then relaxed to a new, stable configuration. topological phase transition for (a) b = 0.80, (b) b = bc = 0.88, and As depicted in Figs. 4(b) and 4(d), this model of disorder (c) b = 0.95. The counterclockwise (A) and breathing (B) modes, predominantly changes the edge state bands, leaving the shown respectively in blue and red, get inverted. (d) Chern numbers bulk subbands mostly invariant. Adding this disorder to the of the three lowest energy bands {C1,C2,C3} as functions of the topologically trivial phase completely removes the edge states magnetic field. Here C3 exhibits a sudden decrease from one to zero from the third gap [see Fig. 4(d)]. In contrast, only two edge as the magnetic field increases past bc, rendering the third band states remain within the third gap in the topological phase [see topologically trivial. (e) Size of the third gap 3 as a function of the Fig. 4(b)]. Moreover, these edge states are chiral as confirmed magnetic field, which vanishes at bc and grows linearly in the vicinity by their magnonic wave function. The right-moving (blue) and of the topological phase transition. (f) and (g) Snapshots of the time left-moving (red) edge states are localized at opposite edges evolution of the out-of-plane magnetization of the counterclockwise of the strip, consistent with a positive winding as predicted by and breathing modes, respectively. Here T denotes the period of both the sign of ν3 (see Appendix C for details). spin-wave modes, for simplicity. In agreement with the predictions of the bulk-edge corre- spondence, the above results suggest that the magnonic edge V. MAGNONIC EDGE STATES AND DISORDER states that remain after introducing disorder are topologically Besides the inversion of the counterclockwise and breath- protected. Conversely, the edge states that connect a bulk ing modes, there is another measurable consequence of the subband set with itself and which unravel with disorder are topological phase transition. The bulk-edge correspondence topologically trivial. We observe two topologically protected postulates that the number of edge states within the ith bulk edge states in Figs. 4(a) and 4(b) instead of one, as expected ν ν = gap, i, is related to the Chern numbers of the bulk bands from 3 1, because we use a strip of infinite extension with ν = below that gap via i ji Cj [42,43]. Accordingly, since two spatially separated edges. If we made our strip geometry ν3 = 1, a topologically protected chiral magnonic edge state of finite size, we would observe a single state propagating should be present within the third bulk gap for b < bc, but not clockwise along the edge. for bc < b. However, the predictions of this correspondence still must be checked. As a matter of fact, a stringent require- VI. DISCUSSION ment of the bulk-edge correspondence is that the finite-size bulk should consist of an integer number of unit cells [44], Profound differences exist between systems that support which is not necessarily expected to hold for every sample. the ferromagnetic SkXs considered here and antiferromag-
013231-4 CHIRAL MAGNONIC EDGE STATES IN FERROMAGNETIC … PHYSICAL REVIEW RESEARCH 2, 013231 (2020)
(a) Pristine (b) Disordered Long-range dipolar interactions were neglected in the E E present work, since in the microscopic approach to thin mag- JS JS netic films, which we have focused on here, they amount to a small correction to nearest-neighbor ferromagnetic ex- 2.0 2.0 change. However, they are of paramount importance in the description of spin waves in magnonic crystals [4–6] and could also give rise to topological magnon insulators [16]. 1.5 1.5 Dipolar interactions in thin films can also give rise to a demag- netizing field that is believed to enlarge the stability region of FM SkXs [23,45]. Previous studies [39] have shown that 1.0 1.0 the magnon spectrum of bulk FM SkXs agrees qualitatively with experiments if dipolar interactions are neglected and that quantitative agreement is achieved when they are taken into 0.5 0.5 account. Moreover, the strength of dipolar interactions could b
013231-5 DÍAZ, HIROSAWA, KLINOVAJA, AND LOSS PHYSICAL REVIEW RESEARCH 2, 013231 (2020) of Science through Program for Leading Graduate Schools these eigenstates. While having a fixed number of magnons (MERIT), JSPS KAKENHI (Grant No. 16J07110) and Young (hence dubbed number states), these states have an arbitrary Researchers’ Exchange Program between Japan and Switzer- phase which makes them unsuitable to describe coherent time land 2018. This work was supported by the Swiss National evolution of magnon modes. The standard solution to this Science Foundation and NCCR QSIT. This project received problem is to resort to magnon coherent states [50,51], i.e., funding from the European Union’s Horizon 2020 research eigenstates of the magnon annihilation operators. They are and innovation program (ERC Starting Grant, Grant Agree- explicitly constructed as ment No. 757725). 2 † −|zkλ| /2 zkλα λ |zkλ =e e k |0 , (B2)
APPENDIX A: BOGOLIUBOV TRANSFORMATION where αkλ |0 =0, and they of course satisfy αkλ |zkλ = | |α† α | =| |2 = zkλ zkλ . Note that zkλ kλ kλ zkλ zkλ n¯kλ is the av- To diagonalize the spin-wave Hamiltonian HSW [Eq. (2)], λ the Bogoliubov transformation erage number of magnons in the th band with crystal mo- mentum k. = jλα + jλ ∗α† ak j Uk kλ V−k −kλ (A1) To lowest order in Holstein-Primakoff√ bosons, the spin operators are given by S = 2S (e−a + e+a† ) + Se3.The must be used, where the indices j and λ run over {1,...,p} R j 2 j R j j R j j expectation value we must now compute reads for a magnetic unit cell comprised of p spins. By introducing √ T † † † T − ak = (ak1,...,akp) and a = (a ,...,a ) , and similarly | | = | | + 3. k k1 kp zkλ SR j (t ) zkλ 2SRe[e j zkλ aR j (t ) zkλ ] Se j (B3) for α and α†, the Bogoliubov transformation can be written k k = From the inverse lattice Fourier transform aR j as · + √1 eik (R r j )a , where N is the total number of magnetic N k k j ak αk = T , (A2) unit cells, and the Bogoliubov transformation defined in † k α† a−k −k Eq. (A1), we note that computing the time-dependent operator aR j (t ) reduces to finding αkλ(t ). Solving the where Heisenberg equation U V ∗ = k −k d i i Tk ∗ (A3) α = ,α =− E α , V U kλ(t ) [HSW kλ] S kλ kλ(t ) (B4) k −k dt h¯ h¯
−(i/h¯)SE λt is a paraunitary matrix that enforces the bosonic algebra on we arrive at α λ(t ) = α λe k . Employing the above α α† k k kλ and kλ. relations, we finally get