Atmos. Chem. Phys., 20, 7955–7977, 2020 https://doi.org/10.5194/acp-20-7955-2020 © Author(s) 2020. This work is distributed under the Creative Commons Attribution 4.0 License. Sea spray aerosol organic enrichment, water uptake and surface tension effects Luke T. Cravigan1, Marc D. Mallet1,a, Petri Vaattovaara2, Mike J. Harvey3, Cliff S. Law3,4, Robin L. Modini5,b, Lynn M. Russell5, Ed Stelcer6;, David D. Cohen6, Greg Olsen7, Karl Safi7, Timothy J. Burrell3, and Zoran Ristovski1 1School of Earth and Atmospheric Sciences, Queensland University of Technology, Brisbane, Australia 2Department of Environmental Science, University of Eastern Finland, Kuopio, Finland 3National Institute of Water and Atmospheric Research, Wellington, New Zealand 4Department of Marine Sciences, University of Otago, Dunedin, New Zealand 5Scripps Institute of Oceanography, University of California, San Diego, La Jolla, California, USA 6Centre for Accelerator Science, NSTLI, Australian Nuclear Science and Technology Organisation, Menai, NSW, Australia 7National Institute of Water and Atmospheric Research, Hamilton, New Zealand anow at: Australian Antarctic Program Partnership, Institute for Marine and Antarctic Science, University of Tasmania, Hobart, Australia bnow at: Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232 Villigen PSI, Switzerland deceased Correspondence: Zoran Ristovski (
[email protected]) Received: 4 September 2019 – Discussion started: 19 September 2019 Revised: 9 May 2020 – Accepted: 27 May 2020 – Published: 9 July 2020 Abstract. The aerosol-driven radiative effects on marine concentration ratios of approximately 0.1–0.2. The enrich- low-level cloud represent a large uncertainty in climate sim- ment of organics was compared to the output from the ulations, in particular over the Southern Ocean, which is also chlorophyll-a-based sea spray aerosol parameterisation sug- an important region for sea spray aerosol production.