https://doi.org/10.5194/acp-2020-885 Preprint. Discussion started: 2 October 2020 c Author(s) 2020. CC BY 4.0 License. Assessing and improving cloud-height based parameterisations of global lightning flash rate, and their impact on lightning-produced NOx and tropospheric composition 5 Ashok K. Luhar1, Ian E. Galbally1, Matthew T. Woodhouse1, and Nathan Luke Abraham2,3 1CSIRO Oceans and Atmosphere, Aspendale, 3195, Australia 2National Centre for Atmospheric Science, Department of Chemistry, University of Cambridge, Cambridge, UK 3Department of Chemistry, University of Cambridge, Cambridge, UK 10 Correspondence to: Ashok K. Luhar (
[email protected]) Abstract. Although lightning-generated oxides of nitrogen (LNOx) account for only approximately 10% of the global NOx source, it has a disproportionately large impact on tropospheric photochemistry due to the conducive conditions in the tropical upper troposphere where lightning is mostly discharged. In most global composition models, lightning flash rates used to calculate LNOx are expressed in terms of convective cloud-top height via the Price and Rind (1992) (PR92) 15 parameterisations for land and ocean. We conduct a critical assessment of flash-rate parameterisations that are based on cloud-top height and validate them within the ACCESS-UKCA global chemistry-climate model using the LIS/OTD satellite data. While the PR92 parameterisation for land yields satisfactory predictions, the oceanic parameterisation underestimates the observed flash-rate density severely, yielding a global average of 0.33 flashes s-1 compared to the observed 9.16 -1 flashes s over the ocean and leading to LNOx being underestimated proportionally. We formulate new/alternative flash-rate 20 parameterisations following Boccippio’s (2002) scaling relationships between thunderstorm electrical generator power and storm geometry coupled with available data.