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Transparent Paper-Based Triboelectric Nanogenerator As Page Mark and Anti-Theft Sensor

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Transparent Paper-Based Triboelectric Nanogenerator As Page Mark and Anti-Theft Sensor Nano Research 1 DOINano 10.1007/s12274Res -014-0484-1 Transparent paper-based triboelectric nanogenerator as page mark and anti-theft sensor Li Min Zhang1†, Fei Xue1†, Weiming Du1, Chang Bao Han1, Chi Zhang1, and Zhong Lin Wang1,2 () Nano Res., Just Accepted Manuscript • DOI: 10.1007/s12274-014-0484-1 http://www.thenanoresearch.com on April 18, 2014 © Tsinghua University Press 2014 Just Accepted This is a “Just Accepted” manuscript, which has been examined by the peer-review process and has been accepted for publication. A “Just Accepted” manuscript is published online shortly after its acceptance, which is prior to technical editing and formatting and author proofing. Tsinghua University Press (TUP) provides “Just Accepted” as an optional and free service which allows authors to make their results available to the research community as soon as possible after acceptance. After a manuscript has been technically edited and formatted, it will be removed from the “Just Accepted” Web site and published as an ASAP article. Please note that technical editing may introduce minor changes to the manuscript text and/or graphics which may affect the content, and all legal disclaimers that apply to the journal pertain. In no event shall TUP be held responsible for errors or consequences arising from the use of any information contained in these “Just Accepted” manuscripts. To cite this manuscript please use its Digital Object Identifier (DOI® ), which is identical for all formats of publication. TABLE OF CONTENTS (TOC) Transparent paper-based triboelectric nanogenerator as page mark and anti-theft sensor Li Min Zhang1†, Fei Xue1†, Weiming Du1, Chang Bao 1 1 1,2 Han , Chi Zhang , and Zhong Lin Wang 1Beijing Institute of Nanoenergy and Nanosystems, Chinese Academy of Sciences, Beijing, 100083, China. 2School of Material Science and Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332, USA. We integrate grating-structured PTENGs into a book as a self-powered anti-theft sensor, which can effectively convert mechanical triggering agitated during handling the book pages into an electric output to either drive a commercial electronic device or trigger a warning buzzer. Furthermore, different grating-structures on each page produce different number of output peaks which can accurately position the turned pages and record the pages flipped over. Zhong Lin Wang, http://www.nanoscience.gatech.edu/ Nano Research DOI (automatically inserted by the publisher) Research Article Transparent paper-based triboelectric nanogenerator as page mark and anti-theft sensor Li Min Zhang1†, Fei Xue1†, Weiming Du1, Chang Bao Han1, Chi Zhang1, and Zhong Lin Wang1,2 () † Received: day month year ABSTRACT Revised: day month year The triboelectric nanogenerator (TENG), based on the well-known triboelectric Accepted: day month year effect and electrostatic induction effect, has been proven to be a simple, cost (automatically inserted by effective approach for self-powered systems to convert ambient mechanical the publisher) energy into electricity. We report a flexible and transparent paper-based triboelectric nanogenerator (PTENG) consisting of an indium tin oxide (ITO) © Tsinghua University Press film and a polyethylene terephthalate (PET) film as the triboelectric surfaces, and Springer-Verlag Berlin which not only acts as an energy supply but also a self-powered active sensor. It Heidelberg 2014 can harvest kinetic energy when the papers contact, bend or relatively slide by a combination of vertical contact-separation mode and lateral sliding mode. In KEYWORDS addition, we also integrate grating-structured PTENGs into a book as a self-powered anti-theft sensor. The mechanical triggering agitated during paper-based triboelectric handling the book pages can be effectively converted into an electric output to nanogenerator, either drive a commercial electronic device or trigger a warning buzzer. self-powered systems, Furthermore, different grating-structures on each page produce different anti-theft sensor, position, number of output peaks by relatively sliding, which can accurately act as a page indium tin oxide mark and record the pages flipped over. This work is a significant step forward in self-powered paper-based devices. 1 Introduction health monitoring, infrastructure and environmental monitoring, internet of things and With the enormous development of the world defense technologies [4-7]. Now a sensor network is technology towards miniaturization, portability and usually integrated by several different functional functionality in the recent years [1-3], sensor sensors and many small electronic devices. A network has been a powerful driving force for the practical challenge for portable sensor network is next phase of information technology. More and the huge number of batteries used in the system, more types of sensors have been widely used in Address correspondence to [email protected] 2 Nano Res. which needs to be recharged, replaced, monitored trigger a warning buzzer. Furthermore, different and maintained. This will cause not only a grating-structures on each page produce different horrendous task but also environmental and health number of output peaks, which can accurately concerns. A self-powered system aiming at position the turned pages and record the pages harvesting energy from the environment [8-11] to flipped over. This work provides a potential power sensor networks is proposed to offset or even method to develop the self-powered, durable, cost replace the reliance of small portable electronics on effective anti-theft system for books, paintings and batteries [2, 12, 13], which will make great any other flexible materials in the future. contribution to the whole environment in the next few decades. So far, portable and renewable human 2 Experimental section motion-driven self-powered systems have been scavenged with diverse approaches based on 2.1 Fabrication of the PTENG piezoelectrics [14-17], electrostatics [18, 19], and electromagnetics [20, 21]. Recently, triboelectric Two pieces of commercial printing paper (33 nanogenerator (TENG) [22, 23] has been mm × 33 mm) with a thickness of 0.2 mm were demonstrated as an efficient device to convert cleaned and then deposited with a 1 m layer of different types of mechanical energy such as human ITO on one side to form ITO-paper. Then a layer of motion, vibration, sonic wave, automobile motion PET film with the thickness of 0.1 mm was adhered and more into electricity. on one piece paper, contacting with the ITO film to Paper has been widely used for thousands of form PET-ITO-paper. Finally, the two parts were years in human civilization [24], for the outstanding assembled together with the PET film facing to the advantages of lightweight, cheap, flexible and ITO film, as shown in Figure 1a. The PTENG was environment friendly. Over the past decades, driven with a linear motor (Linmot E1100) at an paper-based functional electronic devices have acceleration rate of ±10 m/s2 and the maximum opened up a new era of applications in circuits, velocity of 0.6 m/s. The transferred charge and chips and sensors. Although the development of open-circuit voltage were measured by an integrated technology has enlarged the range of electrometer with very large input resistance applications of paper-based electronic devices, the (Kethily, 6514). The short-circuit current of the fatal weakness for the paper-based systems is too PTENG was measured using a Stanford low-noise much dependence on external power supply. Hence current preamplifier (Model SR570). making the paper-based systems work independently and sustainably has profound 2.2 Fabrication of a self-powered page mark and significance. In this paper, we demonstrate a new anti-theft sensor based on the PTENG type of paper-based triboelectric nanogenerator (PTENG) using indium tin oxide (ITO) film and Grating-structured PTENGs were applied into polyethylene terephthalate (PET) film as each page of a book to form a self-powered triboelectric surfaces and it can be made in a book anti-theft sensor. The grating-structured PTENGs or any other paper products to harvest kinetic were made on the adjacent pages, as shown in energy when the papers contact, bend or relatively Figure 4a. The one-grating-structures were adhered slide with the advantages of both transparent and on the even pages, and the multi-grating-structures flexible. In addition, we also integrate were adhered on the odd pages. Assuming the grating-structured PTENGs into a book as a number of grating is n, the number of odd page is self-powered anti-theft sensor. The mechanical (2n-1). Each grating has a dimension of 5 mm × 20 triggering agitated during handling the book pages mm. can be effectively converted into an electric output to either drive a commercial electronic device or 3 Result and discussion | www.editorialmanager.com/nare/default.asp Nano Res. 3 of the PTENG in vertical contact-separation mode. Figure 1a illustrates the basic structure of the A periodic contact and separation drives the fabricated PTENG. The lower part is a thin layer of induced electrons go back and forth through the ITO film deposited on a commercial printing paper, external circuit. Furthermore, Figure 1e illustrates a where the ITO film acts as both the triboelectric cycle of electricity generation process in lateral surface and the electrode. The upper part is sliding mode. Similarly, the upper film slides in and fabricated by pasting another layer of PET on the out, producing electric potential
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