Chapter 10 Nuclear Fission
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Spontaneous Fission of U234, Pu236, Cm240, and Cm244
Lawrence Berkeley National Laboratory Lawrence Berkeley National Laboratory Title Spontaneous Fission of U234, Pu236, Cm240, and Cm244 Permalink https://escholarship.org/uc/item/0df1j1qm Authors Ghiorso, A. Higgins, G.H. Larsh, A.E. et al. Publication Date 1952-04-21 eScholarship.org Powered by the California Digital Library University of California TWO-WEEK LOAN COPY This is a Library Circulating Copy which may be borrowed for two weeks. For a personal retention copy, call Tech. Info. Division, Ext. 5545 UCRL-1772 Unclassified-Chemistry Distribution UNIVEBSITY OF CALIFCEiNIil Radiation Laboratory Contract No, ti-7405-eng-4.8 24.4 SPONTANEOUS FISSION OF' I'Zu6, ~m~~~~ AND Gm A, Ghiorso, G. H, Higgins, A. E. Larsh, Go To Seaborg, and So G, Thompson April 21, 1752 Berkeley, California A. Ghiorso, G. H. Higgins, A. E. Larsh, G. T. Seaborg, and S. Go Thompson Radiation Laboratory and Department of Chemistry Uni versity of California, Berkeley, Californf a April 21, 1952 In a recent communication commenting on the mechanism of fission we called attention to the simple exponential dependence of spontaneous fission rate on Z~/Aand to the effect of an odd nucleon in slowing the fission process.1 Since it is of interest to test further the simple correlation of the spontaneous fission rate for even-even nuclides wfth z~/A~a further number of such rates have been determined, The spontaneous fission rates were measured by pladng the chemically purified samples on one electrode of a parallel plate ionization chamber, filled with a mixture of argon and carbon dioxide, which was connected with an amplifier f ollawed by a register and a stylus recorder. -
Hetc-3Step Calculations of Proton Induced Nuclide Production Cross Sections at Incident Energies Between 20 Mev and 5 Gev
JAERI-Research 96-040 JAERI-Research—96-040 JP9609132 JP9609132 HETC-3STEP CALCULATIONS OF PROTON INDUCED NUCLIDE PRODUCTION CROSS SECTIONS AT INCIDENT ENERGIES BETWEEN 20 MEV AND 5 GEV August 1996 Hiroshi TAKADA, Nobuaki YOSHIZAWA* and Kenji ISHIBASHI* Japan Atomic Energy Research Institute 2 G 1 0 1 (T319-11 l This report is issued irregularly. Inquiries about availability of the reports should be addressed to Research Information Division, Department of Intellectual Resources, Japan Atomic Energy Research Institute, Tokai-mura, Naka-gun, Ibaraki-ken, 319-11, Japan. © Japan Atomic Energy Research Institute, 1996 JAERI-Research 96-040 HETC-3STEP Calculations of Proton Induced Nuclide Production Cross Sections at Incident Energies between 20 MeV and 5 GeV Hiroshi TAKADA, Nobuaki YOSHIZAWA* and Kenji ISHIBASHP* Department of Reactor Engineering Tokai Research Establishment Japan Atomic Energy Research Institute Tokai-mura, Naka-gun, Ibaraki-ken (Received July 1, 1996) For the OECD/NEA code intercomparison, nuclide production cross sections of l60, 27A1, nalFe, 59Co, natZr and 197Au for the proton incidence with energies of 20 MeV to 5 GeV are calculated with the HETC-3STEP code based on the intranuclear cascade evaporation model including the preequilibrium and high energy fission processes. In the code, the level density parameter derived by Ignatyuk, the atomic mass table of Audi and Wapstra and the mass formula derived by Tachibana et al. are newly employed in the evaporation calculation part. The calculated results are compared with the experimental ones. It is confirmed that HETC-3STEP reproduces the production of the nuclides having the mass number close to that of the target nucleus with an accuracy of a factor of two to three at incident proton energies above 100 MeV for natZr and 197Au. -
CME Search Before Isobar Collisions and Blind Analysis from STAR
CME Search Before Isobar Collisions and Blind Analysis From STAR Prithwish Tribedy for the STAR collaboration The 36th Winter Workshop on Nuclear Dynamics 1-7th March, 2020, Puerto Vallarta, Mexico In part supported by Introduction Solenoidal Tracker at RHIC (STAR) RHIC has collided multiple ion species; year 2018 was dedicated to search for effects driven by strong electromagnetic fields by STAR Isobars: Ru+Ru, Zr+Zr @ 200GeV (2018) Low energy: Au+Au 27 GeV (2018) Large systems : U+U, Au+Au @ 200 GeV P.Tribedy, WWND 2 The Chiral Magnetic Effect (Cartoon Picture) Quarks Quarks randomly aligned oriented along B antiquarks I II III IV More More right left handed handed quarks quarks J || B J || -B CME converts chiral imbalance to observable electric current P.Tribedy, WWND 2020 3 New Theory Guidance : Complexity Of An Event Magnetic field map Pb+Pb @ 2.76 TeV Axial charge profile b=11.4 fm, Npart=56 Pb+Pb 2.76 TeV, b=11.4 fm, dN5/dxT [a.u.] 0.3 6 uR>uL 0.2 4 uR<uL 0.1 2 0 0 y [fm] -2 -0.1 -4 -0.2 -6 -0.3 -6 -4 -2 0 2 4 6 x [fm] Based on: Chatterjee, Tribedy, Phys. Rev. C 92, Based on: Lappi, Schlichting, Phys. Rev. D 97, 011902 (2015) 034034 (2018) Going beyond cartoon picture: 1) Fluctuations dominate e-by-e physics, 2) B-field & domain size of axial-charge change with √s P.Tribedy, WWND 2020 4 New Theory Guidance : Complexity Of An Event Pb+Pb @ 2.76 TeV Magnetic field b=11.4 fm, N Axial charge profile Pb+Pb 2.76 TeV, b=11.4 fm, dN5/dxT [a.u.] 0.3 6 u 0.2 4 u 0.1 2 0 0 y [fm] -2 -0.1 -4 -0.2 -6 -0.3 -6 -4 -2 0 2 4 6 x [fm] Based on: Chatterjee, -
Search for Isobar Nuclei in Mass Distributions of Heavy Fission Fragments of 235U Nuclei by Thermal Neutrons
International Conference “Nuclear Science and its Application”, Samarkand, Uzbekistan, September 25-28, 2012 SEARCH FOR ISOBAR NUCLEI IN MASS DISTRIBUTIONS OF HEAVY FISSION FRAGMENTS OF 235U NUCLEI BY THERMAL NEUTRONS Abdullaeva G.A., Koblik Yu.N., Nebesniy A.F., Pikul V.P. Institute of Nuclear Physics, Tashkent, Uzbekistan To search for isobar nuclei in mass distributions of 235U nuclei heavy fission fragments (FF) caused by thermal neutrons we used experimental data from [1]. In [1] experimental data of yields for each value of mass number in FF mass numbers range from A=125 to A=155 a.m.u. depending on effective charge state z* are published. In figure 1 such experimental dependence of FF yields Yi (Ai) =f(z*) and processing of this dependence by Gauss distribution with an error to one σ for each z* is presented. The basic difficulty consisted in correct transition from measured z* to charges of heavy fragments at the moment of nuclear fission. For this purpose we used the modified expression from [2] in the form of: k * α k1 i i ii VzV1zz 0 . Here zi* and zi - the measured effective charge of the i-th ion with mass number Ai and a charge of corresponding fragment, Vi - velocity of ion, Vo - average velocity of electrons interacting with fragment in the target matter and influencing to formation of an effective charge of the ion. Velocity Vi was defined with use of measured value Ek for each fragment. Velocity Vo can 8 changes in limits from Vo = 2.2×10 cm/s - electron velocity in the first orbit of hydrogen atom to 3.6×108 cm/s [2], constants: α =0.45 and k =0.6 are taken as from [2]. -
Spontaneous Fission Half-Lives of Heavy and Superheavy Nuclei Within a Generalized Liquid Drop Model
Spontaneous fission half-lives of heavy and superheavy nuclei within a generalized liquid drop model Xiaojun Bao1, Hongfei Zhang1,∗ G. Royer2, Junqing Li1,3 June 4, 2018 1. School of Nuclear Science and Technology, Lanzhou University, Lanzhou 730000, China 2. Laboratoire Subatech, UMR: IN2P3/CNRS-Universit´e-Ecole des Mines, 4 rue A. Kastler, 44 Nantes, France 3. Institute of Modern Physics, Chinese Academy of Science, Lanzhou 730000, China Abstract We systematically calculate the spontaneous fission half-lives for heavy and superheavy arXiv:1302.7117v1 [nucl-th] 28 Feb 2013 nuclei between U and Fl isotopes. The spontaneous fission process is studied within the semi-empirical WKB approximation. The potential barrier is obtained using a generalized liquid drop model, taking into account the nuclear proximity, the mass asymmetry, the phenomenological pairing correction, and the microscopic shell cor- rection. Macroscopic inertial-mass function has been employed for the calculation of the fission half-life. The results reproduce rather well the experimental data. Rela- tively long half-lives are predicted for many unknown nuclei, sufficient to detect them if synthesized in a laboratory. Keywords: heavy and superheavy nuclei; half-lives; spontaneous fission ∗Corresponding author. Tel.: +86 931 8622306. E-mail address: [email protected] 1 1 Introduction Spontaneous fission of heavy nuclei was first predicted by Bohr and Wheeler in 1939 [1]. Their fission theory was based on the liquid drop model. Interestingly, their work also con- tained an estimate of a lifetime for fission from the ground state. Soon afterwards, Flerov and Petrzak [2] presented the first experimental evidence for spontaneous fission. -
An Octad for Darmstadtium and Excitement for Copernicium
SYNOPSIS An Octad for Darmstadtium and Excitement for Copernicium The discovery that copernicium can decay into a new isotope of darmstadtium and the observation of a previously unseen excited state of copernicium provide clues to the location of the “island of stability.” By Katherine Wright holy grail of nuclear physics is to understand the stability uncover its position. of the periodic table’s heaviest elements. The problem Ais, these elements only exist in the lab and are hard to The team made their discoveries while studying the decay of make. In an experiment at the GSI Helmholtz Center for Heavy isotopes of flerovium, which they created by hitting a plutonium Ion Research in Germany, researchers have now observed a target with calcium ions. In their experiments, flerovium-288 previously unseen isotope of the heavy element darmstadtium (Z = 114, N = 174) decayed first into copernicium-284 and measured the decay of an excited state of an isotope of (Z = 112, N = 172) and then into darmstadtium-280 (Z = 110, another heavy element, copernicium [1]. The results could N = 170), a previously unseen isotope. They also measured an provide “anchor points” for theories that predict the stability of excited state of copernicium-282, another isotope of these heavy elements, says Anton Såmark-Roth, of Lund copernicium. Copernicium-282 is interesting because it University in Sweden, who helped conduct the experiments. contains an even number of protons and neutrons, and researchers had not previously measured an excited state of a A nuclide’s stability depends on how many protons (Z) and superheavy even-even nucleus, Såmark-Roth says. -
Re-Examining the Role of Nuclear Fusion in a Renewables-Based Energy Mix
Re-examining the Role of Nuclear Fusion in a Renewables-Based Energy Mix T. E. G. Nicholasa,∗, T. P. Davisb, F. Federicia, J. E. Lelandc, B. S. Patela, C. Vincentd, S. H. Warda a York Plasma Institute, Department of Physics, University of York, Heslington, York YO10 5DD, UK b Department of Materials, University of Oxford, Parks Road, Oxford, OX1 3PH c Department of Electrical Engineering and Electronics, University of Liverpool, Liverpool, L69 3GJ, UK d Centre for Advanced Instrumentation, Department of Physics, Durham University, Durham DH1 3LS, UK Abstract Fusion energy is often regarded as a long-term solution to the world's energy needs. However, even after solving the critical research challenges, engineer- ing and materials science will still impose significant constraints on the char- acteristics of a fusion power plant. Meanwhile, the global energy grid must transition to low-carbon sources by 2050 to prevent the worst effects of climate change. We review three factors affecting fusion's future trajectory: (1) the sig- nificant drop in the price of renewable energy, (2) the intermittency of renewable sources and implications for future energy grids, and (3) the recent proposition of intermediate-level nuclear waste as a product of fusion. Within the scenario assumed by our premises, we find that while there remains a clear motivation to develop fusion power plants, this motivation is likely weakened by the time they become available. We also conclude that most current fusion reactor designs do not take these factors into account and, to increase market penetration, fu- sion research should consider relaxed nuclear waste design criteria, raw material availability constraints and load-following designs with pulsed operation. -
Photofission Cross Sections of 238U and 235U from 5.0 Mev to 8.0 Mev Robert Andrew Anderl Iowa State University
Iowa State University Capstones, Theses and Retrospective Theses and Dissertations Dissertations 1972 Photofission cross sections of 238U and 235U from 5.0 MeV to 8.0 MeV Robert Andrew Anderl Iowa State University Follow this and additional works at: https://lib.dr.iastate.edu/rtd Part of the Nuclear Commons, and the Oil, Gas, and Energy Commons Recommended Citation Anderl, Robert Andrew, "Photofission cross sections of 238U and 235U from 5.0 MeV to 8.0 MeV " (1972). Retrospective Theses and Dissertations. 4715. https://lib.dr.iastate.edu/rtd/4715 This Dissertation is brought to you for free and open access by the Iowa State University Capstones, Theses and Dissertations at Iowa State University Digital Repository. It has been accepted for inclusion in Retrospective Theses and Dissertations by an authorized administrator of Iowa State University Digital Repository. For more information, please contact [email protected]. INFORMATION TO USERS This dissertation was produced from a microfilm copy of the original document. While the most advanced technological means to photograph and reproduce this document have been used, the quality is heavily dependent upon the quality of the original submitted. The following explanation of techniques is provided to help you understand markings or patterns which may appear on this reproduction, 1. The sign or "target" for pages apparently lacking from the document photographed is "Missing Page(s)". If it was possible to obtain the missing page(s) or section, they are spliced into the film along with adjacent pages. This may have necessitated cutting thru an image and duplicating adjacent pages to insure you complete continuity, 2. -
Compilation and Evaluation of Fission Yield Nuclear Data Iaea, Vienna, 2000 Iaea-Tecdoc-1168 Issn 1011–4289
IAEA-TECDOC-1168 Compilation and evaluation of fission yield nuclear data Final report of a co-ordinated research project 1991–1996 December 2000 The originating Section of this publication in the IAEA was: Nuclear Data Section International Atomic Energy Agency Wagramer Strasse 5 P.O. Box 100 A-1400 Vienna, Austria COMPILATION AND EVALUATION OF FISSION YIELD NUCLEAR DATA IAEA, VIENNA, 2000 IAEA-TECDOC-1168 ISSN 1011–4289 © IAEA, 2000 Printed by the IAEA in Austria December 2000 FOREWORD Fission product yields are required at several stages of the nuclear fuel cycle and are therefore included in all large international data files for reactor calculations and related applications. Such files are maintained and disseminated by the Nuclear Data Section of the IAEA as a member of an international data centres network. Users of these data are from the fields of reactor design and operation, waste management and nuclear materials safeguards, all of which are essential parts of the IAEA programme. In the 1980s, the number of measured fission yields increased so drastically that the manpower available for evaluating them to meet specific user needs was insufficient. To cope with this task, it was concluded in several meetings on fission product nuclear data, some of them convened by the IAEA, that international co-operation was required, and an IAEA co-ordinated research project (CRP) was recommended. This recommendation was endorsed by the International Nuclear Data Committee, an advisory body for the nuclear data programme of the IAEA. As a consequence, the CRP on the Compilation and Evaluation of Fission Yield Nuclear Data was initiated in 1991, after its scope, objectives and tasks had been defined by a preparatory meeting. -
Uranium (Nuclear)
Uranium (Nuclear) Uranium at a Glance, 2016 Classification: Major Uses: What Is Uranium? nonrenewable electricity Uranium is a naturally occurring radioactive element, that is very hard U.S. Energy Consumption: U.S. Energy Production: and heavy and is classified as a metal. It is also one of the few elements 8.427 Q 8.427 Q that is easily fissioned. It is the fuel used by nuclear power plants. 8.65% 10.01% Uranium was formed when the Earth was created and is found in rocks all over the world. Rocks that contain a lot of uranium are called uranium Lighter Atom Splits Element ore, or pitch-blende. Uranium, although abundant, is a nonrenewable energy source. Neutron Uranium Three isotopes of uranium are found in nature, uranium-234, 235 + Energy FISSION Neutron uranium-235, and uranium-238. These numbers refer to the number of Neutron neutrons and protons in each atom. Uranium-235 is the form commonly Lighter used for energy production because, unlike the other isotopes, the Element nucleus splits easily when bombarded by a neutron. During fission, the uranium-235 atom absorbs a bombarding neutron, causing its nucleus to split apart into two atoms of lighter mass. The first nuclear power plant came online in Shippingport, PA in 1957. At the same time, the fission reaction releases thermal and radiant Since then, the industry has experienced dramatic shifts in fortune. energy, as well as releasing more neutrons. The newly released neutrons Through the mid 1960s, government and industry experimented with go on to bombard other uranium atoms, and the process repeats itself demonstration and small commercial plants. -
Radioactive Decay
North Berwick High School Department of Physics Higher Physics Unit 2 Particles and Waves Section 3 Fission and Fusion Section 3 Fission and Fusion Note Making Make a dictionary with the meanings of any new words. Einstein and nuclear energy 1. Write down Einstein’s famous equation along with units. 2. Explain the importance of this equation and its relevance to nuclear power. A basic model of the atom 1. Copy the components of the atom diagram and state the meanings of A and Z. 2. Copy the table on page 5 and state the difference between elements and isotopes. Radioactive decay 1. Explain what is meant by radioactive decay and copy the summary table for the three types of nuclear radiation. 2. Describe an alpha particle, including the reason for its short range and copy the panel showing Plutonium decay. 3. Describe a beta particle, including its range and copy the panel showing Tritium decay. 4. Describe a gamma ray, including its range. Fission: spontaneous decay and nuclear bombardment 1. Describe the differences between the two methods of decay and copy the equation on page 10. Nuclear fission and E = mc2 1. Explain what is meant by the terms ‘mass difference’ and ‘chain reaction’. 2. Copy the example showing the energy released during a fission reaction. 3. Briefly describe controlled fission in a nuclear reactor. Nuclear fusion: energy of the future? 1. Explain why nuclear fusion might be a preferred source of energy in the future. 2. Describe some of the difficulties associated with maintaining a controlled fusion reaction. -
Arxiv:1901.01410V3 [Astro-Ph.HE] 1 Feb 2021 Mental Information Is Available, and One Has to Rely Strongly on Theoretical Predictions for Nuclear Properties
Origin of the heaviest elements: The rapid neutron-capture process John J. Cowan∗ HLD Department of Physics and Astronomy, University of Oklahoma, 440 W. Brooks St., Norman, OK 73019, USA Christopher Snedeny Department of Astronomy, University of Texas, 2515 Speedway, Austin, TX 78712-1205, USA James E. Lawlerz Physics Department, University of Wisconsin-Madison, 1150 University Avenue, Madison, WI 53706-1390, USA Ani Aprahamianx and Michael Wiescher{ Department of Physics and Joint Institute for Nuclear Astrophysics, University of Notre Dame, 225 Nieuwland Science Hall, Notre Dame, IN 46556, USA Karlheinz Langanke∗∗ GSI Helmholtzzentrum f¨urSchwerionenforschung, Planckstraße 1, 64291 Darmstadt, Germany and Institut f¨urKernphysik (Theoriezentrum), Fachbereich Physik, Technische Universit¨atDarmstadt, Schlossgartenstraße 2, 64298 Darmstadt, Germany Gabriel Mart´ınez-Pinedoyy GSI Helmholtzzentrum f¨urSchwerionenforschung, Planckstraße 1, 64291 Darmstadt, Germany; Institut f¨urKernphysik (Theoriezentrum), Fachbereich Physik, Technische Universit¨atDarmstadt, Schlossgartenstraße 2, 64298 Darmstadt, Germany; and Helmholtz Forschungsakademie Hessen f¨urFAIR, GSI Helmholtzzentrum f¨urSchwerionenforschung, Planckstraße 1, 64291 Darmstadt, Germany Friedrich-Karl Thielemannzz Department of Physics, University of Basel, Klingelbergstrasse 82, 4056 Basel, Switzerland and GSI Helmholtzzentrum f¨urSchwerionenforschung, Planckstraße 1, 64291 Darmstadt, Germany (Dated: February 2, 2021) The production of about half of the heavy elements found in nature is assigned to a spe- cific astrophysical nucleosynthesis process: the rapid neutron capture process (r-process). Although this idea has been postulated more than six decades ago, the full understand- ing faces two types of uncertainties/open questions: (a) The nucleosynthesis path in the nuclear chart runs close to the neutron-drip line, where presently only limited experi- arXiv:1901.01410v3 [astro-ph.HE] 1 Feb 2021 mental information is available, and one has to rely strongly on theoretical predictions for nuclear properties.