Photon Statistics of Light Resonantly Scattered from a Three-Level Atom Rollin Michael Evans Iowa State University
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Iowa State University Capstones, Theses and Retrospective Theses and Dissertations Dissertations 1984 Photon statistics of light resonantly scattered from a three-level atom Rollin Michael Evans Iowa State University Follow this and additional works at: https://lib.dr.iastate.edu/rtd Part of the Nuclear Commons Recommended Citation Evans, Rollin Michael, "Photon statistics of light resonantly scattered from a three-level atom " (1984). Retrospective Theses and Dissertations. 8160. https://lib.dr.iastate.edu/rtd/8160 This Dissertation is brought to you for free and open access by the Iowa State University Capstones, Theses and Dissertations at Iowa State University Digital Repository. It has been accepted for inclusion in Retrospective Theses and Dissertations by an authorized administrator of Iowa State University Digital Repository. For more information, please contact [email protected]. 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Universi^ Micrdnlms International 300 N. Zeeb Road Ann Arbor, Ml 48106 8505814 Evans, Rollin Michael PHOTON STATISTICS OF LIGHT RESONANTLY SCATTERED FROM A THREE-LEVEL ATOM Iowa State University PH.D. 1984 University Microfilms Intsrnâtionâl 300 N. zeeb Road, Ann Arbor, Ml 48106 Photon statistics of light resonantly scattered from a three-level atom by Rollin Michael Evcins A Dissertation Submitted to the Graduate Faculty in Partial Fulfillment of the Requirements for the Degree of DOCTOR OF PHILOSOPHY Department: Physics Major; Nuclear Physics Approved: Members of the Committee: Signature was redacted for privacy. Signature was redacted for privacy. In Charge of Major Mork Signature was redacted for privacy. FW^ the Major Department Signature was redacted for privacy. For the 'Grabuate College Iowa State University Ames, Iowa 1984 il TABLE OF CONTENTS Pacre CHAPTER I. INTRODUCTION "l Nuclear Structure Information Through Optical Means 2 Review of Spectroscopic Methods 3 Photon Statistics and the Photon-Burst Method 6 The Doppler Effect and Fluorescence Lineshapes 11 Equipment 12 Photon Burst and On-Line Methods 13 Photon Burst and Exotic Atom Searches 15 Thesis Structure 17 CHAPTER II. EQUIPMENT 18 Review of Dye Lasers 18 DC Lock 33 Heterodyne Lock 40 Transfer Etalon 45 Havemeter 51 Atomic-Beam Chamber 54 Photon-Burst Counting Electronics 67 CHAPTER III. PHOTON STATISTICS AND FLUORESCENCE LINESHAPES 71 Two-Level System and the Burst Method 71 Photon Number Distributions in a Three-Level System 81 0 Parameters 91 Lineshape Calculations 95 ill CHAPTER IV. BACKGROUND AND ATOMIC VELOCITY EFFECTS 106 Mode 2 Counting and Background 107 Dark Counts 113 Chain Breaking 122 Background Interference 125 CHAPTER V. DATA AND ANALYSIS 139 Photodiode Calibration and Laser Intensity Profile Measurements 140 Upper Level Population Probability 143 Photon Number Distributions 146 Line shape. Data suid Calculations 163 CHAPTER VI. CONCLUSIONS 176 System Sensitivity 176 Photon Number Distributions 180 Spectral Lineshapes 181 REFERENCES 183 PARTIAL TABLE OF SYMBOLS 188 APPENDIX 191 Background Interference 191 1 CHAPTER I. INTRODUCTION Through the study of -atomic spectra nuclear magnetic moments, spins, spectroscopic quadrupole moments and changes in mean square charge radii can be obtained. For the past fifty years, atomic spectra have provided information on stable amd long-lived nuclei. It is now possible to extend these studies to short-lived (half life of less than one second) species. The major advantage of spectroscopic techniques over others is their extreme sensitivity. Nuclear scattering experiments, muonic atom or X-ray isotope shift experiments may provide more information than spectroscopic methods, but require macroscopic amounts of material. It is possible with spectroscopic techniques to work with as few as 10,000 atoms/sec (1). This sensitivity opens up exciting possibilities. All the basic laws of nuclear physics have been derived from an intensive study of some 500 nuclei, namely those that are stable or can be reached from stable nuclei by simple nuclear reactions. The number of nuclei that have been produced is close to 1700, and it is conjectured that 7000 nuclei could eventually be identified (2). In exploring these new regions of short-lived nuclei, new nuclear properties or even new nuclear effects might well be discovered. Already nuclear structure and systematics qualitatively different from stable nuclei have 2 emerged In the measurements of a loner chain of neutron deficient Hg isotopes (3). A primary purpose of this work is to extend the sensitivity of optical detection techniques to the one atom/sec level through the use of the photon-burst method. The sensitivity increase is obtained by scattering large numbers of photons from a single atom. Â number of new and interesting effects in the statistics of the resonantly scattered light then become important. Nuclear Structure Information Through Optical Means The addition of neutrons to a nucleus changes its mass, radiusr magnetic moment and shape. Changes in the mass and electromagnetic moments of nuclei can be detected through their effects upon the electrons of the atoms (4). The change in nuclear mass and radius from the addition of neutrons causes a shift in the electron energy levels. This isotope shift can be broken into two parts, one part arising from the change in size of the nucleus and the other arising from the change in mass. Electrons with orbits which penetrate the nucleus (S and states) are sensitive to nuclear size changes. However, the addition of a neutron also changes 'the center of mass of the nucleus-electron- cloud system shifting the electron energy levels. The exact size of this mass shift depends upon correlations between all electrons in the atom,, which makes calculation of this 3 effect very difficult. The estimate of the specific mass shift is the single largest source of error in the determination of the change in nuclear size for this type of experiment. The outer electrons are sensitive to the magnetic dipole and the spectroscopic quadrupole moments of the nucleus. The effect of these moments upon the electronic structure is to split a level into several sublevels. The number of these sublevels depends upon the nuclear and electronic spin. The splitting separations depend upon the electron wavefunction and the sizes of the electromagnetic moments of the nucleus. Review of Spectroscopic Methods A relatively new tool for spectroscopy is the high- power, narrow-frequency tunable laser. The resonant • inte^raction cross section between atoms and photons 'is large 7 17 ("x ) and beam fluxes of 10 photons per sec are not difficult to obtain. The spectral purity aind high degree of polarization of a laser makes possible great selectivity in the atomic transition smd sublevel being probed. The major spectroscopic techniques that have been used to probe short-lived nuclei can be arouped into three types; 1) RAdiation Detected Optical Pumping (RADOP), in which radiation from the nuclear decay is detected; 2) Atomic Beam Resonance (ABR), in which the atom itself is detected; and 4 3) Resonance Fluorescence, in which light scattered by the atom is detected. All of these techniques have been used for many years, but recently lasers have been used to increase their sensitivity. In RÂDOP (3), as well as in the later LINO (Laser Induced Nuclear Orientation (5)) and LINUP (Laser Induced NUclear Polarization (6)) techniques an atom is optically pumped, partially aligning the nucleus with the polarization of the light source. An angular asymmetry may exist in the nuclear decay of the aligned nucleus. This alignment occurs when the laser is in resonance with one of the atomic hyperfine components. The hyperfine structure can be obtained by monitoring the anisotropic nuclear decay as a function of laser frequency. The great strength of this technique is the sensitivity of nuclear radiation detection. The technique of atomic-beam resonance is among the oldest used for hyperfine structure work (7). Huber et al. (8) updated this technique to probe long chains of radioactive alkali isotopes (8, 9). In this system, a laser beam is used to alter the population distribution of the atomic m^ sublevels.