A Nuclear Reactor Can Be
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An Investigation of How Powerful a Nuclear Reactor Can Be by Tammy L. Stoops Submitted to the Department of Nuclear Engineering in partial fulfillment of the requirements for the degrees of Bachelor of Science in Nuclear Engineering and Master of Science in Nuclear Engineering at the MASSACHUSETTS INSTITUTE OF TECHNOLOGY June 1996 © 1996 Massachusetts Institute of Technology All Rights Reserved. Author ......... ............................................... bepartment of Nuclear Engineering May 10. 1996 Certified by ... .......... Michael W. Golay Professor of Nuclear Engineering Thesis Supervisor Certified by ................................................. rfes Jefferson W. Tester fessor ofChemical Engineering Thesis Reader Certified by ............ Michael J. Driscoll Professor Emeritus of Nuclear Engineering Thesis Reader A ccepted by ................................. ............................... - ' Jeffrey P. Freidberg Chairman, Departmental Committee on Graduate Students I'ASSACHUSETTS INS •'"CL OF TECHNOLOGY JUN 2 01996 Science LIBRARIES An Investigation of How Powerful a Nuclear Reactor Can Be by Tammy L. Stoops Submitted to the Department of Nuclear Engineering on May 10, 1996, in partial fulfillment of the requirements for the degrees of Bachelor of Science in Nuclear Engineering and Master of Science in Nuclear Engineering Abstract Nuclear power technologies, emitting no greenhouse gases, may be used to mitigate glo- bal warming by replacing fossil fuel energy sources. Current versions of this technology are not well-suited for this purpose, however. In order to create a suitable nuclear power system, an investigation was performed to identify and improve upon a breeder reactor system capable of large-scale power production. The system would be required to produce hydrogen as a transportable energy source, actively reduce its fission product inventory during operation, and resist nuclear proliferation. An examination of solid, gaseous, and liquid fuel reactors indicated that the molten salt breeder reactor was most capable of meeting future needs. The development of advanced alloys is expected to reduce the problem of corrosion of the structural materials. The coat- ing of the reactor graphite with pyrolytics or silicon carbide and the sizing of the flow channels maximize the graphite moderator lifetime. Also, chemical processing systems have been developed which appear to be adequate for the removal of the fission products, however lack of funding halted their refinement and industrial implementation. The latest designs of molten salt breeder reactors require improvement. The chemical pro- cessing system may be simplified to a one-step, metal transfer process for fission product removal, significantly reducing the residual reactor decay power. The use of a helium- based gas turbine system eliminates hazardous interactions between the fuel and coolant. By elevating the primary heat exchanger, natural circulation may be induced to ease the cooling burden of pump failure. The decay heat can be removed using specially designed cooling tanks which allow both radiative heat losses and natural convection of air over the fuel salt. The questions of economic performance are not considered in the work reported here. The results of this investigation show that this molten salt breeder reactor concept is pas- sively safe. The reactor power may be increased without bound, provided that an increase is made in reactor fuel salt volume, thereby reducing the decay power density. The ability of this concept to meet the desired characteristics for a global warming response is very powerful. Thesis Supervisor: Michael W. Golay Title: Professor of Nuclear Engineering Acknowledgments I would like to thank the many individuals who provided the guidance for this project. Without the patience and advice of Professors Michael W. Golay, Michael J. Driscoll, Larry M. Lidsky, and Jefferson W. Tester, this work would never have become a reality. Without the soothing words of my fiance, Lee Carson, in times of difficulty, I would never have seen the light. I would like to extend a special thanks to Uri Gat, Kazuo Furukawa, and Dick Engel. Their genuine interest and willingness to share their invaluable experi- ence even under the extreme conditions of a hospital stay were greatly appreciated. I truly stand on the shoulders of giants as I reach for a higher star. I would also like to thank my mother, Anne Stoops. Despite the numerous setbacks, you have helped me maintain my hope and determination. Your confidence in me was an endless source of encouragement. As I worked diligently in a field dominated by men, your influence reminded me to never forget who I am, a woman. I love you, Mom. Thank you. Finally, I would like to dedicate this work to my father, Richard Stoops. You have always seen the best in me, Dad, and gave me the faith to believe in myself. Because of you, I strove to reach seemingly unreachable goals and succeeded. When I stumbled, you were always there to pick me up, brush me off, and put me back on track. You have made me who I am, and taught me to acknowledge and accept what I am not. I love you, Dad. Thank you. Contents 1 Introduction ............................................................................................................... 13 1.1 General .............................................................................................................. 13 1.2 Background ....................................................................................................... 14 1.3 M ethod of Investigation .................................................................................... 16 1.4 Scope of the W ork Reported Here .................................................................... 17 2 Required Technology and Reactor Concepts ............................................................ 19 2.1 G eneral .............................................................................................................. 19 2.1.1 Large-Scale Breeding Capability .......................................................... 19 2.1.2 H ydrogen Production Capability .......................................................... 19 2.1.3 Reduction of the Core Fission Product Inventory ................................. 20 2.1.4 N uclear Proliferation Resistance ........................................................... 20 2.2 Solid Fuel Reactors ........................................................................................... 22 2.3 Fluid Fuel Reactors ........................................................................................... 24 2.3.1 G aseous Fuel ......................................................................................... 25 2.3.2 Liquid Fuel ............................................................................................ 25 2.4 Choice of Technology ....................................................................................... 27 3 Status of M olten Salt Reactor D evelopm ent ............................................................. 29 3.1 G eneral .............................................................................................................. 29 3.2 The Fuel Cycle and Reactor Physics ................................................................ 29 3.3 Fuel Chem istry .................................................................................................. 31 3.3.1 Interactions of the Base Fuel Salt ......................................................... 31 3.3.2 Fission Product D istribution ................................................................. 33 3.4 Selection of Salt Container and Piping Materials ............................................. 34 3.5 Graphite ............................................................................................................. 36 3.6 Cooling .............................................................................................................. 39 3.7 Fuel Processing ................................................................................................. 40 3.8 Required Improvem ents .................................................................................... 47 4 Chem ical Processing .................................................................................................. 49 4.1 General .............................................................................................................. 49 4.2 One Step Processing ........................................................................................ 49 4.3 Process Efficiency and Cycle Time .................................................................. 50 4.4 The Fuel D ecay H eat ........................................................................................ 51 5 H eat Transfer Perform ance ........................................................................................ 57 5.1 General .............................................................................................................. 57 5.2 LiF-BeF 2, Helium , and G as Turbines ............................................................... 58 5.3 Natural Circulation of the Fuel Upon Pump Failure ......................................... 59 5.3.1 The Core ............................................................................................... 61 5.3.2 The Prim ary H eat Exchanger ............................................................... 61 5.3.3 The Pum p .............................................................................................