Chapter 2 – General Background Information Chapter 2 General Background Information
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16 European Atlas of Natural Radiation | Chapter 2 – General background information Chapter 2 General background information This chapter provides the background information geology of Europe, one can already form a general necessary to understand how ionising radiation works, and large-scale idea of the level of natural radioactiv- why it is present in our environment, and how it can be ity that can be expected. For instance, young and mo- represented on a map. bile unconsolidated sediments (like clay or sand) that are found in many regions in northern and northwest- The ionising radiation discussed in this chapter consists ern Europe contain generally fewer radionuclides than of alpha, beta and neutron particles as well as gamma certain magmatic or metamorphic rocks found in for rays. Each interacts with matter in a specific way, caus- example Scandinavia (Fennoscandian Shield), Central ing biological effects that can be hazardous. Health risk Europe (Bohemian Massif), France (Bretagne and Cen- from radiation is described by the absorbed dose, tral Massif) and in Spain (Iberian Massif). The more equivalent dose and effective dose, calculated using recent alpine mountain belts are composed of many specific weighting factors. The effects of ionising radia- different types of rocks, leading to strong spatial vari- tion on humans can be deterministic and stochastic. All ations in radiological signature and radiological back- this information leads to the general principles of radi- ground. Some types of volcanic rocks have a higher ation protection. Natural ionising radiation is emitted by radionuclide content and can lead to increased indoor a variety of sources, both cosmogenic and terrigenous, gamma dose rates and radon or thoron concentra- and can be primordial (existing since the origin of the tions. Another specific case are karstic limestone are- Solar System) or secondary (created by the interaction as, where the radiological risk varies locally, leading to of radiation with matter). The most important terrestrial strong hot-spots of natural radioactivity. Organic-rich 238 235 primordial radionuclides are uranium ( U and U de- shale and slate can also be enriched in uranium lead- 232 cay series), thorium Th decay series and potassium ing to an increased radiological risk. Other geological 40K. One particular descendant from uranium and thori- factors like fractures such as faults can favour radio- um is radon gas, having a particular impact on human nuclide concentration and radon migration to the sur- health. As radon forms by radioactive decay inside min- face. The topmost layer of the Earth's surface is often eral grains, part of it escapes into the pore-space (em- covered by a soil layer, which can influence the local anation), and migrates to the atmosphere (exhalation). content in radionuclides and affect the natural radio- Once present in indoor air, radon becomes a potential activity presented in this Atlas. source of hazardous exposure to the occupants. Being radioactive, it produces progeny that partly attaches to The final section of this chapter describes the process aerosol particles, leading to an attached fraction and of generating a map based on available knowledge an unattached fraction. The relation between radon and experimental data. Statistical analysis is the tool gas, aerosol particle size and concentration and those used to interpret the data and knowledge and the attached and unattached fractions determines the principles are illustrated and described in detail in this health risk (by inhalation) to humans. In this way, scien- part. Concepts like accuracy and precision have very tists can estimate the different sources and contribu- specific meanings in statistical terms, and it is impor- tions to radiation doses to humans, presented in a dose tant to appreciate them when dealing with data. pie-chart. A case study about Ukraine shows how the Measurement uncertainty, sample bias, choice of highest radiation exposure to the population comes scale and resolution are other examples, just to men- from natural radiation sources. Due to the radiation tion a few of the considerations going into the design protection measures imposed, the exposure due to the of a survey or map. Without data there could be no Chernobyl accident is less. map but without a detailed knowledge of the quality, the limitations and the different ways in which data The composition and structure of the sub-surface, de- could be sampled and interpreted, one cannot hope to scribed by geology, has a strong influence on the local create a useful map. The complexity of the process is level of natural background radiation, along with other demonstrated, and it concludes with a case study on conditions such as altitude and climate. Looking at the designing a soil-gas survey. Clockwise from top-left: Borkum sand island, North Sea coast, Germany. Source: Peter Bossew. Törvajöe variegated limestone in blocks fallen from klint escarpment. Törvajöe, Estonia. Source: Tınis Saadre. The Aurora Borealis, or Northern Lights, shines above Sauðárkrókur, Iceland. Source: Vincent Guth on Unsplash. Folded limestone flysch, San Rocco, Liguria, Italy. Source: Rotraud Stiegler. Chapter 2 – General background information | European Atlas of Natural Radiation 17 General background information 2.1 Radiation physics Ionising radiation (hereafter called radiation) is radiation neutrons), ions or atoms moving at high speeds (usually greater under emitting ionising radiation is called radioactivity. that carries enough energy to liberate electrons from atoms or than 1 % of the speed of light), and electromagnetic waves on the The following section briefly describes radiation, together with molecules, thereby ionising them. Ionising radiation is made up of high-energy end of the electromagnetic spectrum. The ability of its biological effects on humans, and the general principle of energetic subatomic particles (alpha particles, beta particles and atomic nuclei to convert spontaneously (without exterior action) radiation protection. 2.1.1 Different kinds of radiation Alpha 4 + Alpha radiation is the emission of an alpha particle from the alpha particle must overcome to penetrate or escape from the Alpha decay α 2He nucleus of an atom, changing the originating atom to one of an nucleus. element with an atomic number 2 less and mass number 4 less The least penetrating alpha particle is positively charged and Nucleus than it started with. An alpha particle consists of two protons and quite massive in comparison to the more penetrating negatively two neutrons, essentially the nucleus of a helium-4 atom, and charged beta-, and the most penetrating, gamma and neutron Alpha gets out from the nucleus by tunnel effect. radiations. Due to its charge and mass: particle The alpha decay equation may be described in general terms • an alpha particle interacts strongly with matter and stops as follows: within 100 µm in most materials. In air, alpha particles may Proton travel only a few centimetres, e.g. an 5.5 MeV alpha particle A A-4 4 Neutron Z P Z-2 D+ 2He (2-1) travels 4 cm in air and 48 µm in water. A A-4 4 • travel distance depends on several variables including the energy where Z P is theZ-2 D parent+ 2He nucleus of atomic(2-1) number Z and mass with atomic electrons. Thus alpha particle produces thousands of A A-4 4 of the alpha particle, the atomic number and atomic weight of numberZ P A, Z-2 D+ is2 Hethe daughter nucleus of(2-1) atomic number Z-2 and ion pairs until its kinetic energy has been completely dissipated A A-4 4 the absorber and the density of the absorber. mass numberP A-4, andD+ He is the alpha particle.(2-1) The total energy Z Z-2 2 • an alpha particle dissipates its energy in matter mainly by two within the substance it traverses. It is the most ionising radiation released is shared between the alpha particle, recoil daughter mechanisms, ionisation and electron excitation. emitted by natural sources, with the extremely rare exception of nucleus,E γand= hgamma-radiationν = E1 - E 2 from the daughter(2-2) nucleus when the spontaneous fission of uranium. (2-2) • direct collisions with an atomic nucleus are few and far Eit isγ E leftγ == inh hanνν =excitedE=1 - EenergyE 21 - stateE 2 and decays(2-2) to its ground state. between. The energyE ofγ the= h alphaν = E particles1 - E 2 typically ranges(2-2) between 2 and 10 MeV and its value is characteristic of the emitting nucleus. Double positive charge of alpha particles allows ionisation Radionuclidesln 2 emitting alpha particles of low energy decay with within a given substance (solid, liquid, or gas) by the formation of The amount of energy required to produce ion pairs is a function of the = (2-3) λ T long half-lives,ln 2 1/2 whereas those emitting alpha particles of high ion pairs due to coloumbic attraction between a traversing alpha absorbing medium. For example, air absorbs an average of 35 eV, argon = (2-3) λ T particle and atomic electrons of the atoms within the material gas absorbs approximately 25 eV, and a semiconductor material requires energy have1/2 shortln 2 half-lives. The shorter half-lives exhibited = (2-3) λ T only 2-3 eV to produce an ion pair. This gives semiconductor materials by radionuclides1/2 with high alpha decay energies compared to the alpha particle travels. The two neutrons of the alpha particle ln 2 an important advantage as radiation detectors compared to gases when the longer half-lives of nuclides with lower decay energies(2-3) is give it additional mass, which further