Wintertime aerosol dominated by solid fuel burning emissions across Ireland: insight into the spatial and chemical variation of submicron aerosol Chunshui Lin1,2,3, Darius Ceburnis1, Ru-Jin Huang1,2,3*, Wei Xu1,2, Teresa Spohn1, Damien Martin1, Paul 5 Buckley4, John Wenger4, Stig Hellebust4, Matteo Rinaldi5, Maria Cristina Facchini5, Colin O’Dowd1*, and Jurgita Ovadnevaite1 1School of Physics, Ryan Institute’s Centre for Climate and Air Pollution Studies, National University of Ireland Galway. University Road, Galway. H91 CF50, Ireland 2State Key Laboratory of Loess and Quaternary Geology and Key Laboratory of Aerosol Chemistry and Physics, Chinese 10 Academy of Sciences, 710061, Xi’an, China 3Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi’an 710061, China 4School of Chemistry and Environmental Research Institute, University College Cork, Cork, Ireland 5Istituto di Scienze dell’Atmosfera e del Clima, Consiglio Nazionale delle Ricerche, 40129, Bologna, Italy 15 Correspondence to: Ru-Jin Huang (
[email protected]) and Colin O’Dowd (
[email protected]) Abstract. To get an insight into the spatial and chemical variation of the submicron aerosol, a nationwide characterization of wintertime PM1 was performed using an Aerosol Chemical Speciation Monitor (ACSM) and Aethalometer at four representative sites across Ireland. Dublin, the capital city of Ireland, was the most polluted area with an average PM1 -3 -3 -3 concentration of 8.6 μg m , ranging from <0.5 μg m to 146.8 μg m in December 2016. The PM1 in Dublin was mainly 20 composed of carbonaceous aerosol (organic aerosol (OA) + black carbon (BC)) which, on average, accounted for 80% of total PM1 mass during the monitoring period.