Abraham Nitzan

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Abraham Nitzan, University of Pennsylvania Title: Transport and optical response in illuminated molecular junctions Abstract: The interaction of light with molecular conduction junction is attracting growing interest as a challenging experimental and theoretical problem on one hand, and because of its potential application as a characterization and control tool on the other. From both its scientific aspect and technological potential it stands at the interface of two important fields: molecular electronics and molecular plasmonics. I shall review the present state of the art of this field and our work on optical response, switching, Raman scattering, temperature measurements, light generation and photovoltaics in such systems. Bio Abraham Nitzan was born in Israel in 1944, received B.Sc. and M.Sc. degrees from the Hebrew University, and Ph.D degree from Tel Aviv University (TAU) in 1972. Following post doctoral studies at MIT and the University of Chicago he has returned to Tel Aviv University in 1975 where he is a professor of Chemistry since 1982 (Emeritus since 2014). Since 2015 he is a professor of Chemistry at the University of Pennsylvania, USA. At TAU he has served as Chairman of the School of Chemistry in 1984-7, Dean of the Faculty of Sciences in 1995-8 and director of the Institute of Advanced Studies 2003-15. His research focuses on the interaction of light with molecular systems, chemical reactions in condensed phases and interfaces and charge transfer processes in such environments. He has published over 350 papers, a comprehensive text ("Chemical Dynamics in Condensed Phases", Oxford U. Press, 2006), was assigned one patent and has given invited talks in over 150 scientific meetings. During 1992-2014 Nitzan was the incumbent of the Kodesh Chair of Chemical Dynamics at Tel Aviv University and since 2018 he holds the Donner Chair of Physical Sciences at UPenn. Among his main recognitions are the Humboldt Award, the Israel Chemical Society Prize (2004) and Medal (2015), the Emet Prize, the Hirschfelder Prize, the Plyler Prize and the Israel Prize in Chemistry. He is a Fellow of the American Physical Society and of the American Association for the Advancement of Science, a Foreign Honorary member of the American Academy of Arts and Sciences, a Foreign Associate of the US National Academy of Sciences and a member of the Israel Academy of Arts and Sciences. In 2010 he has received an honorary doctorate (Dr. Honoris Causa) from th e University of Konstanz. .

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1944, TEL AVIV, ISRAEL ZAHAL (Israeli) Military Service: 1966‐1969 Marital Status (No
ABRAHAM NITZAN, Ph.D. University of Pennsylvania February 2018 CURRICULUM VITAE Born: 1944, TEL AVIV, ISRAEL ZAHAL (Israeli) Military Service: 1966‐1969 Marital Status (No. of children): Married, 2 children EDUCATION 1961‐1964 Hebrew University, Jerusalem Chemistry B.Sc. Summa cum laude 1964‐1966 Hebrew University, Jerusalem Chemistry M.Sc. Summa cum laude 1970‐1972 Tel‐Aviv University Chemistry Ph.D. Summa cum laude Master's Thesis: On the Radiation Chemistry of Water Supervisor: Professor G. Czapski Doctoral Dissertation: Radiationless Transitions in Molecular Systems Supervisor: Professor J. Jortner ACADEMIC AND PROFESSIONAL EXPERIENCE Period Institute Department Function 2015‐ University of Chemistry Professor Pennsylvania 2014‐2015 Free University Berlin Physics Visiting Professor 2013‐ Tel Aviv University Chemistry Prof. Emeritus 1981‐2013 Tel Aviv University Chemistry Professor 2006‐2012 Northwestern Univ Chemistry Adjunct Professor 2003‐2015 Tel Aviv University Sackler Institute of Director Advanced Studies 1995‐1998 Tel Aviv University Sackler Faculty of Dean Exact Sciences 1990‐1991 Weizmann Institute Chemistry Professor 1984‐1987 Tel Aviv University Chemistry Chairman 1975‐1981 Tel Aviv University Chemistry Assoc. Prof. 1974‐1975 Northwestern Univ Chemistry Assistant Prof 1974‐1975 Univ. of Chicago Chemistry Research Assoc. 1972‐1974 M.I.T. Chemistry Research Assoc. 1 ABRAHAM NITZAN, Ph.D. University of Pennsylvania RESEARCH INTERESTS Theoretical studies of activation, relaxation and energy transfer processes in molecular systems. Theory of transport phenomena in condensed phases and on surfaces. Theory of chemical reaction rates in condensed phases. Theory of ionic diffusion and conductivity in solid ionic conductors, in polymers and in confined systems. Electromagnetic and electronic interactions in small particles and clusters Theoretical investigations of charge transfer and charge separation phenomena in condensed phases, at interfaces and in nano‐junctions.
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Equilibrium Consideration
On the origin of ground-state vacuum-field catalysis: Equilibrium consideration Cite as: J. Chem. Phys. 152, 234107 (2020); https://doi.org/10.1063/5.0006472 Submitted: 02 March 2020 . Accepted: 27 May 2020 . Published Online: 15 June 2020 Tao E. Li , Abraham Nitzan , and Joseph E. Subotnik COLLECTIONS Paper published as part of the special topic on Photocatalysis and Photoelectrochemistry Note: This paper is part of the JCP Special Topic on Photocatalysis and Photoelectrochemistry. ARTICLES YOU MAY BE INTERESTED IN State-pairwise decoherence times for nonadiabatic dynamics on more than two electronic states The Journal of Chemical Physics 152, 234105 (2020); https://doi.org/10.1063/5.0010081 Modeling voltammetry curves for proton coupled electron transfer: The importance of nuclear quantum effects The Journal of Chemical Physics 152, 234108 (2020); https://doi.org/10.1063/5.0010412 Polaritonic normal modes in transition state theory The Journal of Chemical Physics 152, 161101 (2020); https://doi.org/10.1063/5.0007547 J. Chem. Phys. 152, 234107 (2020); https://doi.org/10.1063/5.0006472 152, 234107 © 2020 Author(s). The Journal ARTICLE of Chemical Physics scitation.org/journal/jcp On the origin of ground-state vacuum-field catalysis: Equilibrium consideration Cite as: J. Chem. Phys. 152, 234107 (2020); doi: 10.1063/5.0006472 Submitted: 2 March 2020 • Accepted: 27 May 2020 • Published Online: 15 June 2020 Tao E. Li,1,a) Abraham Nitzan,1,2,b) and Joseph E. Subotnik1,c) AFFILIATIONS 1 Department of Chemistry, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA 2School of Chemistry, Tel Aviv University, Tel Aviv 69978, Israel Note: This paper is part of the JCP Special Topic on Photocatalysis and Photoelectrochemistry.
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Arxiv:2103.06749V1 [Physics.Chem-Ph] 11 Mar 2021
Collective vibrational strong coupling effects on molecular vibrational relaxation and energy transfer: Numerical insights via cavity molecular dynamics simulations Tao E. Li,1, ∗ Abraham Nitzan,1, 2, y and Joseph E. Subotnik1, z 1Department of Chemistry, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA 2School of Chemistry, Tel Aviv University, Tel Aviv 69978, Israel For a small fraction of hot CO2 molecules immersed in a liquid-phase CO2 thermal bath, classical cavity molecular dynamics simulations show that forming collective vibrational strong coupling (VSC) between the C O asymmetric stretch of CO2 molecules and a cavity mode accelerates hot- molecule relaxation. The physical mechanism underlying this acceleration is the fact that polaritons, especially the lower polariton, can be transiently excited during the nonequilibrium process, which facilitates intermolecular vibrational energy transfer. The VSC effects on these rates (i) resonantly depend on the cavity mode detuning, (ii) cooperatively depend on molecular concentration or Rabi splitting, and (iii) collectively scale with the number of hot molecules, which is similar to Dicke’s superradiance. For larger cavity volumes, due to a balance between this superradiant-like behavior and a smaller light-matter coupling, the total VSC effect on relaxation rates can scale slower than 1=N, and the average VSC effect per molecule can remain meaningful for up to N ∼ 104 molecules forming VSC. Moreover, we find that the transiently excited lower polariton prefers to relax by transferring its energy to the tail of the molecular energy distribution rather than equally distributing it to all thermal molecules. Finally, we highlight the similarities of parameter dependence between the current finding with VSC catalysis observed in Fabry–Pérot microcavities.
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Raman Scattering from Nonequilibrium Molecular Conduction Junctions Michael Galperin, Mark A
Subscriber access provided by TEL AVIV UNIV (AO) Letter Raman Scattering from Nonequilibrium Molecular Conduction Junctions Michael Galperin, Mark A. Ratner, and Abraham Nitzan Nano Lett., 2009, 9 (2), 758-762• DOI: 10.1021/nl803313f • Publication Date (Web): 21 January 2009 Downloaded from http://pubs.acs.org on February 18, 2009 More About This Article Additional resources and features associated with this article are available within the HTML version: • Supporting Information • Access to high resolution figures • Links to articles and content related to this article • Copyright permission to reproduce figures and/or text from this article Nano Letters is published by the American Chemical Society. 1155 Sixteenth Street N.W., Washington, DC 20036 NANO LETTERS 2009 Raman Scattering from Nonequilibrium Vol. 9, No. 2 Molecular Conduction Junctions 758-762 Michael Galperin,*,† Mark A. Ratner,‡ and Abraham Nitzan§ Department of Chemistry & Biochemistry, UniVersity of California at San Diego, La Jolla, California 92093, Department of Chemistry, Northwestern UniVersity, EVanston Illinois 60208, and School of Chemistry, The Sackler Faculty of Science, Tel AViV UniVersity, Tel AViV 69978, Israel Received November 3, 2008; Revised Manuscript Received December 26, 2008 ABSTRACT Raman scattering is a potentially important probe of structure, dynamics, and thermal properties of single-molecule conduction junctions. We combine a nonequilibrium Green’s function description of the junction with a generalized scattering theory of the Raman process, which provides the ﬁrst theoretical description of Raman scattering from such systems. The voltage dependence of the Raman ﬂux shows a characteristic behavior at the conductance threshold resulting from (a) partial populations in the ground and excited molecular levels that give rise to two scattering pathways as well as interference between them and (b) junction heating that affects the Raman intensities.
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Biography of Mark A. Ratner BIOGRAPHY
Biography of Mark A. Ratner BIOGRAPHY ark Ratner describes him- theory is a relatively simple mathemati- self as a theoretical materi- cal model of a disordered system that als chemist. Arguably the relates concentration of conductor sites M youngest of the chemical within a theoretical lattice structure to sciences, materials chemistry is con- the flow (or percolation) of charge, par- cerned with how chemical interactions ticularly ionic diffusion. Below a thresh- control and determine the properties of old concentration, or the percolation materials. Throughout his career, Rat- threshold, the substance is an insulator, ner has aimed to develop models to de- and above that concentration it is a con- fine a theoretical language for how the ductor. Over the past 10 years, Ratner molecular structures of a material are and Nitzan have examined the proper- manifested in its physical properties. His ties both of electron transfer within work has focused on several areas in- molecules and electron transport in mo- cluding charge transport (1, 2), ion lecular wire junctions (11, 12). In such transfer (3), nonlinear optical behavior junctions, single molecules or small (4), and quantum dynamics (5, 6). Elec- groups of molecules conduct electrical tron-transfer reactions, so fundamental current between two electrodes. Because to life, underlie biological processes such of the very small size of the structures, as photosynthesis, cytochrome p450 re- both the molecular electronic structure actions, and cellular respiration as well and the connection between the mole- as materials processes such as electro- chemistry and corrosion. ‘‘It’s one of the cule and the electrodes strongly influ- most important reactions in chemistry, Mark A.
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Curriculum Vitae
Date of Revision: May 6, 2021 CURRICULUM VITAE A. BIOGRAPHICAL INFORMATION 1. PERSONAL Name: Dvira Segal University Address: Department of Chemistry, University of Toronto, 80 St. George Street, Toronto, Ontario, M5S 3H6 Oﬃce Phone: 416 946 0559 Email address: [email protected] 2. DEGREES 2004 Ph.D. (direct program) in Chemistry, Tel Aviv University Title of Graduate thesis: Electron transfer in molecular conductors Supervisor: Professor Abraham Nitzan 1998 B.Sc. in Chemistry Major-Computer Science Minor, CUM LAUDE, Tel Aviv University 3. EMPLOYMENT July 2017- Professor, Department of Chemistry, University of Toronto July 2012-2017 Associate Professor, Department of Chemistry, University of Toronto July 2007-2012 Assistant Professor, Department of Chemistry, University of Toronto 2006-2007 Postdoctoral Fellow Department of Chemistry, Columbia University, New York 2003-2005 Concurrent Postdoc position in: Chemical Physics Department, Weizmann Institute of Science, Rehovot, Israel Department of Chemistry University of British Columbia, Vancouver, Canada 4. HONOURS 2014-2023 Canada Research Chair (Tier II) in Theoretical Chemistry 2010-2012 Alfred P. Sloan Research Fellow 2010-2015 Early Research Award 2000-2003 The Clore scholarship for Ph.D. students 1995, 1996 The Dean's list for academic achievements in the Faculty of Exact Sciences, Tel-Aviv University 5. PROFESSIONAL AFFILIATIONS AND ACTIVITIES Chemical Institute of Canada (CIC): Member Quantum Transport and Thermodynamics Society (QTTS) 1 B. ACADEMIC HISTORY 6A. RESEARCH ENDEAVOURS Field: Theoretical Chemical Physics (a) Quantum transport and dissipation. Our research is focused on the development of analytical and computational methods for describing charge and energy transport processes in condensed phases. This includes: (i) Formulation of methodologies for following the dynamics of many-body quantum sys- tems driven out-of-equilibrium by a potential bias or/and a temperature gradient.
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HSING-TA (THETA)CHEN Department of Chemistry University of Pennsylvania 908-489-4996 231 S
HSING-TA (THETA)CHEN Department of Chemistry University of Pennsylvania 908-489-4996 231 S. 34 Street, 263 Cret [email protected] Philadelphia, PA 19104 [email protected] CURRENT POSITION Postdoctoral Researcher, University of Pennsylvania, PA 1/2017 – Present - Developed mixed quantum-classical electrodynamics theory and simulation - Analyzed semiclassical simulation of resonance energy transfer and molecular spectroscopy - Explored strong coupling quantum optics using semiclassical and numerically exact approaches EDUCATION Columbia University, NY 10/2016 Ph.D. in Chemical Physics (Advisor: Prof. David Reichman) Thesis: Delving Into Dissipative Quantum Dynamics: From Approximate to Numerically Exact Approaches. Thesis committee: Prof. Bruce Berne, Prof. Andrew Millis, Prof. Richard Friesner, Prof. Seogjoo Jang National Taiwan University, Taiwan 6/2010 M.Sc. in Physics (Advisor: Prof. Shih-I Chu) Thesis: Generalized Floquet approach for time-dependent electron transport: memory effect on the photon-assisted tunneling via a single quantum dot. National Taiwan University, Taiwan 6/2006 B.Sc. in Physics B.Sc. in Mathematics RESEARCH EXPERIENCE Visiting Scholar, IAMS, Academia Sinica, Taiwan 7/2019 – 8/2019 Visiting Postdoctoral Researcher, SLAC/Stanford University, CA 1/2017 – 7/2017 Sackler Postdoctoral Fellow, Tel Aviv University, Israel 6/2016 – 8/2016 Ph.D. Thesis Research, Columbia University, NY 6/2012 – 6/2016 Research Assistant, Center for Quantum Science and Engineering, Taiwan 7/2010 – 7/2011 PUBLICATIONS [17] Tao E. Li, Hsing-Ta Chen, Abraham Nitzan, Joseph E. Subotnik, Quasiclassical Modeling of Cavity Quantum Electrodynamics. arXiv:1910.02299 (2019) [16] Zeyu Zhou, Hsing-Ta Chen, Abraham Nitzan, Joseph E. Subotnik, Non-adiabatic Dynamics in a Laser Field with Floquet Fewest Switches Surface Hopping: The Need for An Accurate Treatment of Coherence and De- coherence Remains.
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CURRICULUM VITAE Vladimiro Mujica
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