Nuclear Fuel Cycle
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Spent Nuclear Fuel Pools in the US
Spent Nuclear Fuel Pools in the U.S.: Reducing the Deadly Risks of Storage front cover WITH SUPPORT FROM: WITH SUPPORT FROM: By Robert Alvarez 1112 16th St. NW, Suite 600, Washington DC 20036 - www.ips-dc.org May 2011 About the Author Robert Alvarez, an Institute for Policy Studies senior scholar, served as a Senior Policy Advisor to the Secre- tary of Energy during the Clinton administration. Institute for Policy Studies (IPS-DC.org) is a community of public scholars and organizers linking peace, justice, and the environment in the U.S. and globally. We work with social movements to promote true democracy and challenge concentrated wealth, corporate influence, and military power. Project On Government Oversight (POGO.org) was founded in 1981 as an independent nonprofit that investigates and exposes corruption and other misconduct in order to achieve a more effective, accountable, open, and ethical federal government. Institute for Policy Studies 1112 16th St. NW, Suite 600 Washington, DC 20036 http://www.ips-dc.org © 2011 Institute for Policy Studies [email protected] For additional copies of this report, see www.ips-dc.org Table of Contents Summary ...............................................................................................................................1 Introduction ..........................................................................................................................4 Figure 1: Explosion Sequence at Reactor No. 3 ........................................................4 Figure 2: Reactor No. 3 -
Table 2.Iii.1. Fissionable Isotopes1
FISSIONABLE ISOTOPES Charles P. Blair Last revised: 2012 “While several isotopes are theoretically fissionable, RANNSAD defines fissionable isotopes as either uranium-233 or 235; plutonium 238, 239, 240, 241, or 242, or Americium-241. See, Ackerman, Asal, Bale, Blair and Rethemeyer, Anatomizing Radiological and Nuclear Non-State Adversaries: Identifying the Adversary, p. 99-101, footnote #10, TABLE 2.III.1. FISSIONABLE ISOTOPES1 Isotope Availability Possible Fission Bare Critical Weapon-types mass2 Uranium-233 MEDIUM: DOE reportedly stores Gun-type or implosion-type 15 kg more than one metric ton of U- 233.3 Uranium-235 HIGH: As of 2007, 1700 metric Gun-type or implosion-type 50 kg tons of HEU existed globally, in both civilian and military stocks.4 Plutonium- HIGH: A separated global stock of Implosion 10 kg 238 plutonium, both civilian and military, of over 500 tons.5 Implosion 10 kg Plutonium- Produced in military and civilian 239 reactor fuels. Typically, reactor Plutonium- grade plutonium (RGP) consists Implosion 40 kg 240 of roughly 60 percent plutonium- Plutonium- 239, 25 percent plutonium-240, Implosion 10-13 kg nine percent plutonium-241, five 241 percent plutonium-242 and one Plutonium- percent plutonium-2386 (these Implosion 89 -100 kg 242 percentages are influenced by how long the fuel is irradiated in the reactor).7 1 This table is drawn, in part, from Charles P. Blair, “Jihadists and Nuclear Weapons,” in Gary A. Ackerman and Jeremy Tamsett, ed., Jihadists and Weapons of Mass Destruction: A Growing Threat (New York: Taylor and Francis, 2009), pp. 196-197. See also, David Albright N 2 “Bare critical mass” refers to the absence of an initiator or a reflector. -
The Nuclear Waste Primer September 2016 What Is Nuclear Waste?
The Nuclear Waste Primer September 2016 What is Nuclear Waste? Nuclear waste is the catch-all term for anything contaminated with radioactive material. Nuclear waste can be broadly divided into three categories: • Low-level waste (LLW), comprised of protective clothing, medical waste, and other lightly-contaminated items • Transuranic waste (TRU), comprised of long-lived isotopes heavier than uranium • High-level waste (HLW), comprised of spent nuclear fuel and other highly-radioactive materials Low-level waste is relatively short-lived and easy to handle. Currently, four locations for LLW disposal exist in the United States. Two of them, Energy Solutions in Clive, Utah and Waste Control Specialists in Andrews, Texas, accept waste from any U.S. state. Transuranic waste is often a byproduct of nuclear weapons production and contains long-lived radioactive elements heavier than uranium, like plutonium and americium. Currently, the U.S. stores TRU waste at the Waste Isolation Pilot Plant (WIPP) near Carlsbad, New Mexico. High-level waste includes spent nuclear fuel and the most radioactive materials produced by nuclear weapons production. Yucca Mountain is the currently designated high-level waste repository for the United States. 1 | What is Spent Nuclear Fuel? Spent nuclear fuel (SNF), alternatively referred to as used nuclear fuel, is the primary byproduct of nuclear reactors. In commercial power reactors in the U.S., fuel begins as uranium oxide clad in a thin layer of zirconium-aluminum cladding. After several years inside of the reactor, around fi ve percent of the uranium has been converted in some way, ranging from short-lived and highly radioactive fi ssion products to long-lived actinides like plutonium, americium, and neptunium. -
Nuclear Transmutation Strategies for Management of Long-Lived Fission
PRAMANA c Indian Academy of Sciences Vol. 85, No. 3 — journal of September 2015 physics pp. 517–523 Nuclear transmutation strategies for management of long-lived fission products S KAILAS1,2,∗, M HEMALATHA2 and A SAXENA1 1Nuclear Physics Division, Bhabha Atomic Research Centre, Mumbai 400 085, India 2UM–DAE Centre for Excellence in Basic Sciences, Mumbai 400 098, India ∗Corresponding author. E-mail: [email protected] DOI: 10.1007/s12043-015-1063-z; ePublication: 27 August 2015 Abstract. Management of long-lived nuclear waste produced in a reactor is essential for long- term sustenance of nuclear energy programme. A number of strategies are being explored for the effective transmutation of long-lived nuclear waste in general, and long-lived fission products (LLFP), in particular. Some of the options available for the transmutation of LLFP are discussed. Keywords. Nuclear transmutation; long-lived fission products; (n, γ ) cross-section; EMPIRE. PACS Nos 28.41.Kw; 25.40.Fq; 24.60.Dr 1. Introduction It is recognized that for long-term energy security, nuclear energy is an inevitable option [1]. For a sustainable nuclear energy programme, the management of long-lived nuclear waste is very critical. Radioactive nuclei like Pu, minor actinides like Np, Am and Cm and long-lived fission products like 79Se, 93Zr, 99Tc, 107Pd, 126Sn, 129I and 135Cs constitute the main waste burden from a power reactor. In this paper, we shall discuss the management strategies for nuclear waste in general, and long-lived fission products, in particular. 2. Management of nuclear waste The radioactive nuclei which are produced in a power reactor and which remain in the spent fuel of the reactor form a major portion of nuclear waste. -
小型飛翔体/海外 [Format 2] Technical Catalog Category
小型飛翔体/海外 [Format 2] Technical Catalog Category Airborne contamination sensor Title Depth Evaluation of Entrained Products (DEEP) Proposed by Create Technologies Ltd & Costain Group PLC 1.DEEP is a sensor analysis software for analysing contamination. DEEP can distinguish between surface contamination and internal / absorbed contamination. The software measures contamination depth by analysing distortions in the gamma spectrum. The method can be applied to data gathered using any spectrometer. Because DEEP provides a means of discriminating surface contamination from other radiation sources, DEEP can be used to provide an estimate of surface contamination without physical sampling. DEEP is a real-time method which enables the user to generate a large number of rapid contamination assessments- this data is complementary to physical samples, providing a sound basis for extrapolation from point samples. It also helps identify anomalies enabling targeted sampling startegies. DEEP is compatible with small airborne spectrometer/ processor combinations, such as that proposed by the ARM-U project – please refer to the ARM-U proposal for more details of the air vehicle. Figure 1: DEEP system core components are small, light, low power and can be integrated via USB, serial or Ethernet interfaces. 小型飛翔体/海外 Figure 2: DEEP prototype software 2.Past experience (plants in Japan, overseas plant, applications in other industries, etc) Create technologies is a specialist R&D firm with a focus on imaging and sensing in the nuclear industry. Createc has developed and delivered several novel nuclear technologies, including the N-Visage gamma camera system. Costainis a leading UK construction and civil engineering firm with almost 150 years of history. -
Spent Fuel Reprocessing
Spent Fuel Reprocessing Robert Jubin Oak Ridge National Laboratory Reprocessing of used nuclear fuel is undertaken for several reasons. These include (1) recovery of the valuable fissile constituents (primarily 235U and plutonium) for subsequent reuse in recycle fuel; (2) reduction in the volume of high-level waste (HLW) that must be placed in a geologic repository; and (3) recovery of special isotopes. There are two broad approaches to reprocessing: aqueous and electrochemical. This portion of the course will only address the aqueous methods. Aqueous reprocessing involves the application of mechanical and chemical processing steps to separate, recover, purify, and convert the constituents in the used fuel for subsequent use or disposal. Other major support systems include chemical recycle and waste handling (solid, HLW, low-level liquid waste (LLLW), and gaseous waste). The primary steps are shown in Figure 1. Figure 1. Aqueous Reprocessing Block Diagram. Head-End Processes Mechanical Preparations The head end of a reprocessing plant is mechanically intensive. Fuel assemblies weighing ~0.5 MT must be moved from a storage facility, may undergo some degree of disassembly, and then be sheared or chopped and/or de-clad. The typical head-end process is shown in Figure 2. In the case of light water reactor (LWR) fuel assemblies, the end sections are removed and disposed of as waste. The fuel bundle containing the individual fuel pins can be further disassembled or sheared whole into segments that are suitable for subsequent processing. During shearing, some fraction of the radioactive gases and non- radioactive decay product gases will be released into the off-gas systems, which are designed to recover these and other emissions to meet regulatory release limits. -
Re-Examining the Role of Nuclear Fusion in a Renewables-Based Energy Mix
Re-examining the Role of Nuclear Fusion in a Renewables-Based Energy Mix T. E. G. Nicholasa,∗, T. P. Davisb, F. Federicia, J. E. Lelandc, B. S. Patela, C. Vincentd, S. H. Warda a York Plasma Institute, Department of Physics, University of York, Heslington, York YO10 5DD, UK b Department of Materials, University of Oxford, Parks Road, Oxford, OX1 3PH c Department of Electrical Engineering and Electronics, University of Liverpool, Liverpool, L69 3GJ, UK d Centre for Advanced Instrumentation, Department of Physics, Durham University, Durham DH1 3LS, UK Abstract Fusion energy is often regarded as a long-term solution to the world's energy needs. However, even after solving the critical research challenges, engineer- ing and materials science will still impose significant constraints on the char- acteristics of a fusion power plant. Meanwhile, the global energy grid must transition to low-carbon sources by 2050 to prevent the worst effects of climate change. We review three factors affecting fusion's future trajectory: (1) the sig- nificant drop in the price of renewable energy, (2) the intermittency of renewable sources and implications for future energy grids, and (3) the recent proposition of intermediate-level nuclear waste as a product of fusion. Within the scenario assumed by our premises, we find that while there remains a clear motivation to develop fusion power plants, this motivation is likely weakened by the time they become available. We also conclude that most current fusion reactor designs do not take these factors into account and, to increase market penetration, fu- sion research should consider relaxed nuclear waste design criteria, raw material availability constraints and load-following designs with pulsed operation. -
Compilation and Evaluation of Fission Yield Nuclear Data Iaea, Vienna, 2000 Iaea-Tecdoc-1168 Issn 1011–4289
IAEA-TECDOC-1168 Compilation and evaluation of fission yield nuclear data Final report of a co-ordinated research project 1991–1996 December 2000 The originating Section of this publication in the IAEA was: Nuclear Data Section International Atomic Energy Agency Wagramer Strasse 5 P.O. Box 100 A-1400 Vienna, Austria COMPILATION AND EVALUATION OF FISSION YIELD NUCLEAR DATA IAEA, VIENNA, 2000 IAEA-TECDOC-1168 ISSN 1011–4289 © IAEA, 2000 Printed by the IAEA in Austria December 2000 FOREWORD Fission product yields are required at several stages of the nuclear fuel cycle and are therefore included in all large international data files for reactor calculations and related applications. Such files are maintained and disseminated by the Nuclear Data Section of the IAEA as a member of an international data centres network. Users of these data are from the fields of reactor design and operation, waste management and nuclear materials safeguards, all of which are essential parts of the IAEA programme. In the 1980s, the number of measured fission yields increased so drastically that the manpower available for evaluating them to meet specific user needs was insufficient. To cope with this task, it was concluded in several meetings on fission product nuclear data, some of them convened by the IAEA, that international co-operation was required, and an IAEA co-ordinated research project (CRP) was recommended. This recommendation was endorsed by the International Nuclear Data Committee, an advisory body for the nuclear data programme of the IAEA. As a consequence, the CRP on the Compilation and Evaluation of Fission Yield Nuclear Data was initiated in 1991, after its scope, objectives and tasks had been defined by a preparatory meeting. -
GAO-15-141, SPENT NUCLEAR FUEL MANAGEMENT: Outreach
United States Government Accountability Office Report to Congressional Requesters October 2014 SPENT NUCLEAR FUEL MANAGEMENT Outreach Needed to Help Gain Public Acceptance for Federal Activities That Address Liability GAO-15-141 D October 2014 SPENT NUCLEAR FUEL MANAGEMENT Outreach Needed to Help Gain Public Acceptance for Federal Activities That Address Liability Highlights of GAO-15-141, a report to congressional requesters Why GAO Did This Study What GAO Found DOE is responsible for disposing of Spent nuclear fuel—the used fuel removed from nuclear power reactors—is commercial spent nuclear fuel. DOE expected to accumulate at an average rate of about 2,200 metric tons per year in entered into contracts with owners and the United States. This spent nuclear fuel is mostly stored wet, submerged in generators of spent nuclear fuel to pools of water. However, since pools have been reaching their capacities, begin disposing of it beginning in 1998, owners and generators of spent nuclear fuel (typically utilities and reactor with plans for disposal in a national operators) have been transferring it to canisters that are placed in casks on repository. DOE, however, was unable concrete pads for dry storage—which is an expensive and time-consuming to meet the 1998 date and, as a result process. When operating reactors’ licenses begin to expire in the 2030s, the rate of lawsuits, the federal government has of spent nuclear fuel accumulation is expected to decrease, but the amount in dry paid out about $3.7 billion for storage storage will increase as the pools are closed and all spent nuclear fuel is costs. -
Nuclear Energy & the Environmental Debate
FEATURES Nuclear energy & the environmental debate: The context of choices Through international bodies on climate change, the roles of nuclear power and other energy options are being assessed by Evelyne ^Environmental issues are high on international mental Panel on Climate Change (IPCC), which Bertel and Joop agendas. Governments, interest groups, and citi- has been active since 1988. Since the energy Van de Vate zens are increasingly aware of the need to limit sector is responsible for the major share of an- environmental impacts from human activities. In thropogenic greenhouse gas emissions, interna- the energy sector, one focus has been on green- tional organisations having expertise and man- house gas emissions which could lead to global date in the field of energy, such as the IAEA, are climate change. The issue is likely to be a driving actively involved in the activities of these bodies. factor in choices about energy options for elec- In this connection, the IAEA participated in the tricity generation during the coming decades. preparation of the second Scientific Assessment Nuclear power's future will undoubtedly be in- Report (SAR) of the Intergovernmental Panel on fluenced by this debate, and its potential role in Climate Change (IPCC). reducing environmental impacts from the elec- The IAEA has provided the IPCC with docu- tricity sector will be of central importance. mented information and results from its ongoing Scientifically there is little doubt that increas- programmes on the potential role of nuclear ing atmospheric levels of greenhouse gases, such power in alleviating the risk of global climate as carbon dioxide (CO2) and methane, will cause change. -
Fast-Spectrum Reactors Technology Assessment
Clean Power Quadrennial Technology Review 2015 Chapter 4: Advancing Clean Electric Power Technologies Technology Assessments Advanced Plant Technologies Biopower Clean Power Carbon Dioxide Capture and Storage Value- Added Options Carbon Dioxide Capture for Natural Gas and Industrial Applications Carbon Dioxide Capture Technologies Carbon Dioxide Storage Technologies Crosscutting Technologies in Carbon Dioxide Capture and Storage Fast-spectrum Reactors Geothermal Power High Temperature Reactors Hybrid Nuclear-Renewable Energy Systems Hydropower Light Water Reactors Marine and Hydrokinetic Power Nuclear Fuel Cycles Solar Power Stationary Fuel Cells U.S. DEPARTMENT OF Supercritical Carbon Dioxide Brayton Cycle ENERGY Wind Power Clean Power Quadrennial Technology Review 2015 Fast-spectrum Reactors Chapter 4: Technology Assessments Background and Current Status From the initial conception of nuclear energy, it was recognized that full realization of the energy content of uranium would require the development of fast reactors with associated nuclear fuel cycles.1 Thus, fast reactor technology was a key focus in early nuclear programs in the United States and abroad, with the first usable nuclear electricity generated by a fast reactor—Experimental Breeder Reactor I (EBR-I)—in 1951. Test and/or demonstration reactors were built and operated in the United States, France, Japan, United Kingdom, Russia, India, Germany, and China—totaling about 20 reactors with 400 operating years to date. These previous reactors and current projects are summarized in Table 4.H.1.2 Currently operating test reactors include BOR-60 (Russia), Fast Breeder Test Reactor (FBTR) (India), and China Experimental Fast Reactor (CEFR) (China). The Russian BN-600 demonstration reactor has been operating as a power reactor since 1980. -
Characteristics of Spent Nuclear Fuel and Cladding Relevant to High-Level Waste Source Term-CNWRA 93-006 Property of CNWRA 93-006 CNWRA Library
CNWRA 93-006 :~~~~~~~~~ I I S _~~~~~~~~~~~ Prepared for Nuclear Regulatory Commission Contract NRC-02-88-005 Prepared by Center for Nuclear Waste Regulatory Analyses San Antonio, Texas May 1993 462.2 --- T19930511000 8 Characteristics of Spent Nuclear Fuel and Cladding Relevant to High-Level Waste Source Term-CNWRA 93-006 Property of CNWRA 93-006 CNWRA Library CHARACTERISTICS OF SPENT NUCLEAR FUEL AND CLADDING RELEVANT TO HIGH-LEVEL WASTE SOURCE TERM Prepared for Nuclear Regulatory Commission Contract NRC-02-88-005 Prepared by Hersh K. Manaktala Center for Nuclear Waste Regulatory Analyses San Antonio, Texas May 1993 PREVIOUS REPORTS IN SERIES Number Name Date Issued CNWRA 92-017 An Assessment of Borosilicate Glass as a High-Level Waste Form September 1992 CNWRA 92-018 Leaching of Borosilicate Glass Using Draft ASTM Procedure for High-Level Waste August 1992 ii --- ABSTRACT This report, based on literature study, describes characteristics of light water reactor (LWR) fuel assemblies for boiling water reactors (BWR) and pressurized water reactors (PWR) and the changes that take place in both cladding and uranium dioxide fuel during service in commercial power reactors. This information is provided as a background for the evaluation of important factors related to fuel stability under geologic repository conditions. Data related to discharged fuel storage (both wet and dry) are also provided, along with the condition of the fuel in terms of damaged and leaking fuel assemblies. The degradation of spent fuel and cladding while in service in the reactor and likely degradation in a geologic repository are discussed in terms of cladding oxidation and corrosion, and fuel-pellet cracking, fuel restructuring, microstructure and fission product mobility, inventory and distribution of fission products, fuel pellet rim effect, and fission gas release and pressure increase.