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Mixing of Quantum States: a New Route to Creating Optical Activity Anvar S
www.nature.com/scientificreports OPEN Mixing of quantum states: A new route to creating optical activity Anvar S. Baimuratov1, Nikita V. Tepliakov1, Yurii K. Gun’ko1,2, Alexander V. Baranov1, Anatoly V. Fedorov1 & Ivan D. Rukhlenko1,3 Received: 7 June 2016 The ability to induce optical activity in nanoparticles and dynamically control its strength is of great Accepted: 18 August 2016 practical importance due to potential applications in various areas, including biochemistry, toxicology, Published: xx xx xxxx and pharmaceutical science. Here we propose a new method of creating optical activity in originally achiral quantum nanostructures based on the mixing of their energy states of different parities. The mixing can be achieved by selective excitation of specific states orvia perturbing all the states in a controllable fashion. We analyze the general features of the so produced optical activity and elucidate the conditions required to realize the total dissymmetry of optical response. The proposed approach is applicable to a broad variety of real systems that can be used to advance chiroptical devices and methods. Chirality is known to occur at many levels of life organization and plays a key role in many chemical and biolog- ical processes in nature1. The fact that most of organic molecules are chiral starts more and more affecting the progress of contemporary medicine and pharmaceutical industry2. As a consequence, a great deal of research efforts has been recently focused on the optical activity of inherently chiral organic molecules3, 4. It can be strong in the ultraviolet range, in which case it is difficult to study and use in practice. -
Chapter 16 – Electrostatics-I
Chapter 16 Electrostatics I Electrostatics – NOT Really Electrodynamics Electric Charge – Some history •Historically people knew of electrostatic effects •Hair attracted to amber rubbed on clothes •People could generate “sparks” •Recorded in ancient Greek history •600 BC Thales of Miletus notes effects •1600 AD - William Gilbert coins Latin term electricus from Greek ηλεκτρον (elektron) – Greek term for Amber •1660 Otto von Guericke – builds electrostatic generator •1675 Robert Boyle – show charge effects work in vacuum •1729 Stephen Gray – discusses insulators and conductors •1730 C. F. du Fay – proposes two types of charges – can cancel •Glass rubbed with silk – glass charged with “vitreous electricity” •Amber rubbed with fur – Amber charged with “resinous electricity” A little more history • 1750 Ben Franklin proposes “vitreous” and “resinous” electricity are the same ‘electricity fluid” under different “pressures” • He labels them “positive” and “negative” electricity • Proposaes “conservation of charge” • June 15 1752(?) Franklin flies kite and “collects” electricity • 1839 Michael Faraday proposes “electricity” is all from two opposite types of “charges” • We call “positive” the charge left on glass rubbed with silk • Today we would say ‘electrons” are rubbed off the glass Torsion Balance • Charles-Augustin de Coulomb - 1777 Used to measure force from electric charges and to measure force from gravity = - - “Hooks law” for fibers (recall F = -kx for springs) General Equation with damping - angle I – moment of inertia C – damping -
Applied Spectroscopy Spectroscopic Nomenclature
Applied Spectroscopy Spectroscopic Nomenclature Absorbance, A Negative logarithm to the base 10 of the transmittance: A = –log10(T). (Not used: absorbancy, extinction, or optical density). (See Note 3). Absorptance, α Ratio of the radiant power absorbed by the sample to the incident radiant power; approximately equal to (1 – T). (See Notes 2 and 3). Absorption The absorption of electromagnetic radiation when light is transmitted through a medium; hence ‘‘absorption spectrum’’ or ‘‘absorption band’’. (Not used: ‘‘absorbance mode’’ or ‘‘absorbance band’’ or ‘‘absorbance spectrum’’ unless the ordinate axis of the spectrum is Absorbance.) (See Note 3). Absorption index, k See imaginary refractive index. Absorptivity, α Internal absorbance divided by the product of sample path length, ℓ , and mass concentration, ρ , of the absorbing material. A / α = i ρℓ SI unit: m2 kg–1. Common unit: cm2 g–1; L g–1 cm–1. (Not used: absorbancy index, extinction coefficient, or specific extinction.) Attenuated total reflection, ATR A sampling technique in which the evanescent wave of a beam that has been internally reflected from the internal surface of a material of high refractive index at an angle greater than the critical angle is absorbed by a sample that is held very close to the surface. (See Note 3.) Attenuation The loss of electromagnetic radiation caused by both absorption and scattering. Beer–Lambert law Absorptivity of a substance is constant with respect to changes in path length and concentration of the absorber. Often called Beer’s law when only changes in concentration are of interest. Brewster’s angle, θB The angle of incidence at which the reflection of p-polarized radiation is zero. -
APPENDICES 206 Appendices
AAPPENDICES 206 Appendices CONTENTS A.1 Units 207-208 A.2 Abbreviations 209 SUMMARY A description is given of the units used in this thesis, and a list of frequently used abbreviations with the corresponding term is given. Units Description of units used in this thesis and conversion factors for A.1 transformation into other units The formulas and properties presented in this thesis are reported in atomic units unless explicitly noted otherwise; the exceptions to this rule are energies, which are most frequently reported in kcal/mol, and distances that are normally reported in Å. In the atomic units system, four frequently used quantities (Planck’s constant h divided by 2! [h], mass of electron [me], electron charge [e], and vacuum permittivity [4!e0]) are set explicitly to 1 in the formulas, making these more simple to read. For instance, the Schrödinger equation for the hydrogen atom is in SI units: È 2 e2 ˘ Í - h —2 - ˙ f = E f (1) ÎÍ 2me 4pe0r ˚˙ In atomic units, it looks like: È 1 1˘ - —2 - f = E f (2) ÎÍ 2 r ˚˙ Before a quantity can be used in the atomic units equations, it has to be transformed from SI units into atomic units; the same is true for the quantities obtained from the equations, which can be transformed from atomic units into SI units. For instance, the solution of equation (2) for the ground state of the hydrogen atom gives an energy of –0.5 atomic units (Hartree), which can be converted into other units quite simply by multiplying with the appropriate conversion factor (see table A.1.1). -
Gauss' Theorem (See History for Rea- Son)
Gauss’ Law Contents 1 Gauss’s law 1 1.1 Qualitative description ......................................... 1 1.2 Equation involving E field ....................................... 1 1.2.1 Integral form ......................................... 1 1.2.2 Differential form ....................................... 2 1.2.3 Equivalence of integral and differential forms ........................ 2 1.3 Equation involving D field ....................................... 2 1.3.1 Free, bound, and total charge ................................. 2 1.3.2 Integral form ......................................... 2 1.3.3 Differential form ....................................... 2 1.4 Equivalence of total and free charge statements ............................ 2 1.5 Equation for linear materials ...................................... 2 1.6 Relation to Coulomb’s law ....................................... 3 1.6.1 Deriving Gauss’s law from Coulomb’s law .......................... 3 1.6.2 Deriving Coulomb’s law from Gauss’s law .......................... 3 1.7 See also ................................................ 3 1.8 Notes ................................................. 3 1.9 References ............................................... 3 1.10 External links ............................................. 3 2 Electric flux 4 2.1 See also ................................................ 4 2.2 References ............................................... 4 2.3 External links ............................................. 4 3 Ampère’s circuital law 5 3.1 Ampère’s original -
Polarization and Dichroism
Polarization and dichroism Amélie Juhin Sorbonne Université-CNRS (Paris) [email protected] 1 « Dichroism » (« two colors ») describes the dependence of the absorption measured with two orthogonal polarization states of the incoming light: Circular left Circular right k k ε ε Linear horizontal Linear vertical k k ε ε 2 By extension, « dichroism » also includes similar dependence phenomena, such as: • Low symmetry crystals show a trichroic dependence with linear light • Magneto-chiral dichroism (MχD) is measured with unpolarized light • Magnetic Linear Dichroism (MLD) is measured by changing the direction of magnetic ield and keeping the linear polarization ixed … Dichroism describes an angular and /or polarization behaviour of the absorption 3 Linear dichroism (LD) : difference measured with linearly polarized light Circular dichroism (CD) : difference measured with left / right circularly polarized light. Natural dichroism (ND) : time-reversal symmetry is conserved Non-Reciprocal (NR): time-reversal symmetry is not conserved Magnetic dichroism (MD) : measured in (ferro, ferri or antiferro) magnetic materials Dichroism Time reversal Parity symmetry symmetry Natural Linear (NLD) + + Magne6c Linear (MLD) + + Non Reciprocal Linear (NRLD) - - Natural Circular (NCD) + - Magne6c Circular (MCD) - + Magneto-op6cal (MχD) - - 4 The measurement of dichroism is often challenging… … but provides access to properties that cannot be measured in another way isotropic spectra polarized spectra 9 Al K edge Al K edge [6] beryl Al 6 6 corundum -Al O α -
Gem-Quality Tourmaline from LCT Pegmatite in Adamello Massif, Central Southern Alps, Italy: an Investigation of Its Mineralogy, Crystallography and 3D Inclusions
minerals Article Gem-Quality Tourmaline from LCT Pegmatite in Adamello Massif, Central Southern Alps, Italy: An Investigation of Its Mineralogy, Crystallography and 3D Inclusions Valeria Diella 1,* , Federico Pezzotta 2, Rosangela Bocchio 3, Nicoletta Marinoni 1,3, Fernando Cámara 3 , Antonio Langone 4 , Ilaria Adamo 5 and Gabriele Lanzafame 6 1 National Research Council, Institute for Dynamics of Environmental Processes (IDPA), Section of Milan, 20133 Milan, Italy; [email protected] 2 Natural History Museum, 20121 Milan, Italy; [email protected] 3 Department of Earth Sciences “Ardito Desio”, University of Milan, 20133 Milan, Italy; [email protected] (R.B.); [email protected] (F.C.) 4 National Research Council, Institute of Geosciences and Earth Resources (IGG), Section of Pavia, 27100 Pavia, Italy; [email protected] 5 Italian Gemmological Institute (IGI), 20123 Milan, Italy; [email protected] 6 Elettra-Sincrotrone Trieste S.C.p.A., Basovizza, 34149 Trieste, Italy; [email protected] * Correspondence: [email protected]; Tel.: +39-02-50315621 Received: 12 November 2018; Accepted: 7 December 2018; Published: 13 December 2018 Abstract: In the early 2000s, an exceptional discovery of gem-quality multi-coloured tourmalines, hosted in Litium-Cesium-Tantalum (LCT) pegmatites, was made in the Adamello Massif, Italy. Gem-quality tourmalines had never been found before in the Alps, and this new pegmatitic deposit is of particular interest and worthy of a detailed characterization. We studied a suite of faceted samples by classical gemmological methods, and fragments were studied with Synchrotron X-ray computed micro-tomography, which evidenced the occurrence of inclusions, cracks and voids. -
Bright Γ Rays Source and Nonlinear Breit-Wheeler Pairs in the Collision of High Density Particle Beams
PHYSICAL REVIEW ACCELERATORS AND BEAMS 22, 023402 (2019) Bright γ rays source and nonlinear Breit-Wheeler pairs in the collision of high density particle beams † ‡ F. Del Gaudio,1,* T. Grismayer,1, R. A. Fonseca,1,2 W. B. Mori,3 and L. O. Silva1, 1GoLP/Instituto de Plasmas e Fusão Nuclear, Instituto Superior T´ecnico, Universidade de Lisboa, 1049-001 Lisbon, Portugal 2DCTI/ISCTE Instituto Universitário de Lisboa, 1649-026 Lisboa, Portugal 3Departments of Physics & Astronomy and of Electrical Engineering, University of California Los Angeles, Los Angeles, California 90095, USA (Received 13 April 2018; published 8 February 2019) The collision of ultrashort high-density e− or e− and eþ beams at 10s of GeV, to be available at the FACET II and in laser wakefield accelerator experiments, can produce highly collimated γ rays (few GeVs) with peak brilliance of 1027 ph=smm2 mrad20.1%BW and up to 105 nonlinear Breit-Wheeler pairs. We provide analytical estimates of the photon source properties and of the yield of secondary pairs, finding excellent agreement with full-scale 3D self-consistent particle-in-cell simulations that include quantum electrodynamics effects. Our results show that beam-beam collisions can be exploited as secondary sources of γ rays and provide an alternative to beam-laser setups to probe quantum electrodynamics effects at the Schwinger limit. DOI: 10.1103/PhysRevAccelBeams.22.023402 I. INTRODUCTION speed of light, e is the elementary charge and ℏ is the Planck constant. The classical regime is identified by χ ≪ 1, the full Colliders are a cornerstone of fundamental physics of quantum regime by χ ≫ 1 and the quantum transition paramount importance to probe the constituents of matter. -
Investigation of Dichroism by Spectrophotometric Methods
Application Note Glass, Ceramics and Optics Investigation of Dichroism by Spectrophotometric Methods Authors Introduction N.S. Kozlova, E.V. Zabelina, Pleochroism (from ancient greek πλέον «more» + χρόμα «color») is an optical I.S. Didenko, A.P. Kozlova, phenomenon when a transparent crystal will have different colors if it is viewed from Zh.A. Goreeva, T different angles (1). Sometimes the color change is limited to shade changes such NUST “MISiS”, Russia as from pale pink to dark pink (2). Crystals are divided into optically isotropic (cubic crystal system), optically anisotropic uniaxial (hexagonal, trigonal, tetragonal crystal systems) and optically anisotropic biaxial (orthorhombic, monoclinic, triclinic crystal systems). The greatest change is limited to three colors. It may be observed in biaxial crystals and is called trichroic. A two color change may be observed in uniaxial crystals and called dichroic. Pleochroic is often the term used to cover both (2). Pleochroism is caused by optical anisotropy of the crystals Dichroism can be observed in non-polarized light but in (1-3). The absorption of light in the optically anisotropic polarized light it may be more pronounced if the plane of crystals depends on the frequency of the light wave and its polarization of incident light matches plane of polarization of polarization (direction of the electric vector in it) (3, 4). light that propagates in the crystal—ordinary or extraordinary Generally, any ray of light in the optical anisotropic crystal is wave. divided into two rays with perpendicular polarizations and The difference in absorbance of ray lights may be minor, but different velocities (v1, v2) which are inversely proportional to it may be significant and should be considered both when the refractive indices (n1, n2) (4). -
Sauter–Schwinger Effect with a Quantum Gas
PAPER • OPEN ACCESS Sauter–Schwinger effect with a quantum gas To cite this article: A M Piñeiro et al 2019 New J. Phys. 21 083035 View the article online for updates and enhancements. This content was downloaded from IP address 129.2.180.214 on 21/08/2019 at 18:49 New J. Phys. 21 (2019) 083035 https://doi.org/10.1088/1367-2630/ab3840 PAPER Sauter–Schwinger effect with a quantum gas OPEN ACCESS A M Piñeiro , D Genkina, Mingwu Lu and I B Spielman RECEIVED Joint Quantum Institute, National Institute of Standards and Technology and University of Maryland, Gaithersburg, MD 20899, United 26 March 2019 States of America REVISED 18 July 2019 E-mail: [email protected] and [email protected] ACCEPTED FOR PUBLICATION Keywords: quantum gases, Sauter–Schwinger effect, particle creation, quantum simulation 2 August 2019 PUBLISHED 21 August 2019 Abstract Original content from this The creation of particle–antiparticle pairs from vacuum by a large electric field is at the core of work may be used under the terms of the Creative quantum electrodynamics. Despite the wide acceptance that this phenomenon occurs naturally when − Commons Attribution 3.0 18 1 electric field strengths exceed Ec≈10 Vm , it has yet to be experimentally observed due to the licence. fi Any further distribution of limitations imposed by producing electric elds at this scale. The high degree of experimental control this work must maintain present in ultracold atomic systems allow experimentalists to create laboratory analogs to high-field attribution to the author(s) and the title of phenomena. -
Nonperturbative QED Vacuum Birefringence
Prepared for submission to JHEP Nonperturbative QED vacuum birefringence V.I.Denisov E.E.Dolgaya and V.A.Sokolov Physics Department, Moscow State University, Moscow, 119991, Russia E-mail: [email protected], [email protected], [email protected] Abstract: In this paper we represent nonperturbative calculation for one-loop Quantum Electrodynamics (QED) vacuum birefringence in presence of strong magnetic field. The dispersion relations for electromagnetic wave propagating in strong magnetic field point to retention of vacuum birefringence even in case when the field strength greatly exceeds Sauter-Schwinger limit. This gives a possibility to extend some predictions of perturbative QED such as electromagnetic waves delay in pulsars neighbourhood or wave polarization state changing (tested in PVLAS) to arbitrary magnetic field values. Such expansion is especially important in astrophysics because magnetic fields of some pulsars and magnetars greatly exceed quantum magnetic field limit, so the estimates of perturbative QED effects in this case require clarification. Keywords: QED vacuum birefringence, Electromagnetic processes in strong field, Non- perturbative effects arXiv:1612.09086v2 [hep-ph] 30 Dec 2016 Contents 1 Introduction 1 2 Constitutive relations for nonperturbative QED 2 3 Electromagnetic wave propagation in strong magnetic field 4 4 QED vacuum birefringence extension on nonperturbative regime 6 5 Conclusion 9 1 Introduction From the very beginning, radiative corrections to the QED Lagrangian coming from the vacuum fluctuations have been the subject of a great interest. Such corrections, accounted on background of constant and homogeneous electromagnetic field, lead to Heisenberg- Euler effective Lagrangian [1]. The scale parameter for nonlinearities in Heisenberg-Euler electrodynamics (characteristic quantum electrodynamic induction or Schwinger limit for electric field) B = E = m2c3/e~ = 4.41 1013G distinguishes different regimes of the c c · theory. -
Investigation of Magnetic Circular Dichroism Spectra of Semiconductor Quantum Rods and Quantum Dot-In-Rods
nanomaterials Article Investigation of Magnetic Circular Dichroism Spectra of Semiconductor Quantum Rods and Quantum Dot-in-Rods Farrukh Safin 1,* , Vladimir Maslov 1, Yulia Gromova 2, Ivan Korsakov 1, Ekaterina Kolesova 1, Aliaksei Dubavik 1, Sergei Cherevkov 1 and Yurii K. Gun’ko 2 1 School of Photonics, ITMO University, 197101 St. Petersburg, Russia; [email protected] (V.M.); [email protected] (I.K.); [email protected] (E.K.); [email protected] (A.D.); [email protected] (S.C.) 2 School of Chemistry, Trinity College, Dublin 2 Dublin, Ireland; [email protected] (Y.G.); [email protected] (Y.K.G.) * Correspondence: farruhsafi[email protected] Received: 20 April 2020; Accepted: 12 May 2020; Published: 30 May 2020 Abstract: Anisotropic quantum nanostructures have attracted a lot of attention due to their unique properties and a range of potential applications. Magnetic circular dichroism (MCD) spectra of semiconductor CdSe/ZnS Quantum Rods and CdSe/CdS Dot-in-Rods have been studied. Positions of four electronic transitions were determined by data fitting. MCD spectra were analyzed in the A and B terms, which characterize the splitting and mixing of states. Effective values of A and B terms were determined for each transition. A relatively high value of the B term is noted, which is most likely associated with the anisotropy of quantum rods. Keywords: magnetic circular dichroism; quantum nanocrystals; quantum rods; Dot-in-Rods 1. Introduction Anisotropic colloidal semiconductor nanocrystals of various shapes have attracted a lot of attention over recent years due to their unique properties and potential applications.