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Aerosol Effective Radiative Forcing in the Online Aerosol Coupled CAS
atmosphere Article Aerosol Effective Radiative Forcing in the Online Aerosol Coupled CAS-FGOALS-f3-L Climate Model Hao Wang 1,2,3, Tie Dai 1,2,* , Min Zhao 1,2,3, Daisuke Goto 4, Qing Bao 1, Toshihiko Takemura 5 , Teruyuki Nakajima 4 and Guangyu Shi 1,2,3 1 State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China; [email protected] (H.W.); [email protected] (M.Z.); [email protected] (Q.B.); [email protected] (G.S.) 2 Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters/Key Laboratory of Meteorological Disaster of Ministry of Education, Nanjing University of Information Science and Technology, Nanjing 210044, China 3 College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing 100029, China 4 National Institute for Environmental Studies, Tsukuba 305-8506, Japan; [email protected] (D.G.); [email protected] (T.N.) 5 Research Institute for Applied Mechanics, Kyushu University, Fukuoka 819-0395, Japan; [email protected] * Correspondence: [email protected]; Tel.: +86-10-8299-5452 Received: 21 September 2020; Accepted: 14 October 2020; Published: 17 October 2020 Abstract: The effective radiative forcing (ERF) of anthropogenic aerosol can be more representative of the eventual climate response than other radiative forcing. We incorporate aerosol–cloud interaction into the Chinese Academy of Sciences Flexible Global Ocean–Atmosphere–Land System (CAS-FGOALS-f3-L) by coupling an existing aerosol module named the Spectral Radiation Transport Model for Aerosol Species (SPRINTARS) and quantified the ERF and its primary components (i.e., effective radiative forcing of aerosol-radiation interactions (ERFari) and aerosol-cloud interactions (ERFaci)) based on the protocol of current Coupled Model Intercomparison Project phase 6 (CMIP6). -
Studying Geoengineering with Natural and Anthropogenic Analogs
Studying Geoengineering with Natural and Anthropogenic Analogs Alan Robocka, Douglas G. MacMartinb, Riley Durenc, and Matthew W. Christensend aDepartment of Environmental Sciences, Rutgers University, 14 College Farm Road, New Brunswick, NJ 08901 bControl and Dynamical Systems, California Institute of Technology, 1200 E. California Blvd., Pasadena, CA 91125 cJet Propulsion Laboratory, California Institute of Technology, 4800 Oak Grove Dr., Pasadena, CA 91109 dDepartment of Atmospheric Science, Colorado State University, Fort Collins, CO 80523 Submitted to Climatic Change November 2012 Corresponding Author: Alan Robock Department of Environmental Sciences Rutgers University 14 College Farm Road New Brunswick, NJ 08901 Phone: 848-932-5751 Fax: 732-932-8644 E-mail: [email protected] 1 Abstract 2 Solar radiation management (SRM) has been proposed as a possible option for offsetting 3 some anthropogenic radiative forcing, with the goal of reducing some of the associated climatic 4 changes. There are clearly significant uncertainties associated with SRM, and even small-scale 5 experiments that might reduce uncertainty would carry some risk. However, there are also 6 natural and anthropogenic analogs to SRM, such as volcanic eruptions in the case of 7 stratospheric aerosol injection and ship tracks in the case of marine cloud albedo modification. It 8 is essential to understand what we can learn from these analogs in order to validate models, 9 particularly because of the problematic nature of outdoor experiments. It is also important to 10 understand what we cannot learn, as this might better focus attention on what risks would need to 11 be solely examined by numerical models. Stratospheric conditions following a major volcanic 12 eruption, for example, are not the same as those to be expected from intentional geoengineering, 13 both because of confounding effects of volcanic ash and the differences between continuous and 14 impulsive injection of material into the stratosphere. -
Estimation of Cloud Condensation Nuclei Concentration from Aerosol Optical Quantities: Influential Factors and Uncertainties
Open Access Atmos. Chem. Phys., 14, 471–483, 2014 Atmospheric www.atmos-chem-phys.net/14/471/2014/ doi:10.5194/acp-14-471-2014 Chemistry © Author(s) 2014. CC Attribution 3.0 License. and Physics Estimation of cloud condensation nuclei concentration from aerosol optical quantities: influential factors and uncertainties Jianjun Liu1,2 and Zhanqing Li1,2 1State Laboratory of Earth Surface Process and Resource Ecology, GCESS, Beijing Normal University, Beijing, China. 2Department of Atmospheric and Oceanic Science and Earth System Science Interdisciplinary Center, University of Maryland, College Park, Maryland, USA Correspondence to: Zhanqing Li ([email protected]) Received: 26 July 2013 – Published in Atmos. Chem. Phys. Discuss.: 2 September 2013 Revised: 7 November 2013 – Accepted: 30 November 2013 – Published: 15 January 2014 Abstract. Large-scale measurements of cloud condensation significant increase in σsp and decrease in CCN with increas- nuclei (CCN) are difficult to obtain on a routine basis, ing SSA is observed, leading to a significant decrease in their whereas aerosol optical quantities are more readily available. ratio (CCN / σsp) with increasing SSA. Parameterized rela- This study investigates the relationship between CCN and tionships are developed for estimating CCN, which account aerosol optical quantities for some distinct aerosol types us- for RH, particle size, and SSA. ing extensive observational data collected at multiple Atmo- spheric Radiation Measurement (ARM) Climate Research Facility (CRF) sites around the world. The influences of rel- ative humidity (RH), aerosol hygroscopicity (fRH) and sin- 1 Introduction gle scattering albedo (SSA) on the relationship are analyzed. Better relationships are found between aerosol optical depth Aerosols play important roles in Earth’s climate and the hy- (AOD) and CCN at the Southern Great Plains (US), Ganges drological cycle via their direct and indirect effects (IPCC, Valley (India) and Black Forest sites (Germany) than those at 2007). -
Aerosols, Their Direct and Indirect Effects
5 Aerosols, their Direct and Indirect Effects Co-ordinating Lead Author J.E. Penner Lead Authors M. Andreae, H. Annegarn, L. Barrie, J. Feichter, D. Hegg, A. Jayaraman, R. Leaitch, D. Murphy, J. Nganga, G. Pitari Contributing Authors A. Ackerman, P. Adams, P. Austin, R. Boers, O. Boucher, M. Chin, C. Chuang, B. Collins, W. Cooke, P. DeMott, Y. Feng, H. Fischer, I. Fung, S. Ghan, P. Ginoux, S.-L. Gong, A. Guenther, M. Herzog, A. Higurashi, Y. Kaufman, A. Kettle, J. Kiehl, D. Koch, G. Lammel, C. Land, U. Lohmann, S. Madronich, E. Mancini, M. Mishchenko, T. Nakajima, P. Quinn, P. Rasch, D.L. Roberts, D. Savoie, S. Schwartz, J. Seinfeld, B. Soden, D. Tanré, K. Taylor, I. Tegen, X. Tie, G. Vali, R. Van Dingenen, M. van Weele, Y. Zhang Review Editors B. Nyenzi, J. Prospero Contents Executive Summary 291 5.4.1 Summary of Current Model Capabilities 313 5.4.1.1 Comparison of large-scale sulphate 5.1 Introduction 293 models (COSAM) 313 5.1.1 Advances since the Second Assessment 5.4.1.2 The IPCC model comparison Report 293 workshop: sulphate, organic carbon, 5.1.2 Aerosol Properties Relevant to Radiative black carbon, dust, and sea salt 314 Forcing 293 5.4.1.3 Comparison of modelled and observed aerosol concentrations 314 5.2 Sources and Production Mechanisms of 5.4.1.4 Comparison of modelled and satellite- Atmospheric Aerosols 295 derived aerosol optical depth 318 5.2.1 Introduction 295 5.4.2 Overall Uncertainty in Direct Forcing 5.2.2 Primary and Secondary Sources of Aerosols 296 Estimates 322 5.2.2.1 Soil dust 296 5.4.3 Modelling the Indirect -
ALBEDO ENHANCEMENT by STRATOSPHERIC SULFUR INJECTIONS: a CONTRIBUTION to RESOLVE a POLICY DILEMMA? an Editorial Essay
ALBEDO ENHANCEMENT BY STRATOSPHERIC SULFUR INJECTIONS: A CONTRIBUTION TO RESOLVE A POLICY DILEMMA? An Editorial Essay Fossil fuel burning releases about 25 Pg of CO2 per year into the atmosphere, which leads to global warming (Prentice et al., 2001). However, it also emits 55 Tg S as SO2 per year (Stern, 2005), about half of which is converted to sub-micrometer size sulfate particles, the remainder being dry deposited. Recent research has shown that the warming of earth by the increasing concentrations of CO2 and other greenhouse gases is partially countered by some backscattering to space of solar radiation by the sulfate particles, which act as cloud condensation nuclei and thereby influ- ence the micro-physical and optical properties of clouds, affecting regional precip- itation patterns, and increasing cloud albedo (e.g., Rosenfeld, 2000; Ramanathan et al., 2001; Ramaswamy et al., 2001). Anthropogenically enhanced sulfate particle concentrations thus cool the planet, offsetting an uncertain fraction of the anthro- pogenic increase in greenhouse gas warming. However, this fortunate coincidence is “bought” at a substantial price. According to the World Health Organization, the pollution particles affect health and lead to more than 500,000 premature deaths per year worldwide (Nel, 2005). Through acid precipitation and deposition, SO2 and sulfates also cause various kinds of ecological damage. This creates a dilemma for environmental policy makers, because the required emission reductions of SO2, and also anthropogenic organics (except black carbon), as dictated by health and ecological considerations, add to global warming and associated negative conse- quences, such as sea level rise, caused by the greenhouse gases. -
Automated Underway Oceanic and Atmospheric Measurements from Ships
AUTOMATED UNDERWAY OCEANIC AND ATMOSPHERIC MEASUREMENTS FROM SHIPS Shawn R. Smith (1), Mark A. Bourassa (1), E. Frank Bradley (2), Catherine Cosca (3), Christopher W. Fairall (4), Gustavo J. Goni (5), John T. Gunn (6), Maria Hood (7), Darren L. Jackson (8), Elizabeth C. Kent (9), Gary Lagerloef (6), Philip McGillivary (10), Loic Petit de la Villéon (11), Rachel T. Pinker (12), Eric Schulz (13), Janet Sprintall (14), Detlef Stammer (15), Alain Weill (16), Gary A. Wick (17), Margaret J. Yelland (9) (1) Center for Ocean-Atmospheric Prediction Studies, Florida State University, Tallahassee, FL 32306-2840, USA, Emails: [email protected], [email protected] (2) CSIRO Land and Water, PO Box 1666, Canberra, ACT 2601, AUSTRALIA, Email: [email protected] (3) NOAA/PMEL, 7600 Sand Point Way NE, Seattle, WA 98115, USA, Email: [email protected] (4) NOAA/ESRL/PSD, R/PSD3, 325 Broadway, Boulder, CO 80305-3328, USA, Email: [email protected] (5) USDC/NOAA/AOML/PHOD, 4301 Rickenbacker Causeway, Miami, FL 33149, USA, Email: [email protected] (6) Earth and Space Research, 2101 Fourth Ave., Suite 1310, Seattle, WA, 98121, USA, Emails: [email protected], [email protected] (7) Intergovernmental Oceanographic Commission UNESCO, 1, rue Miollis, 75732 Paris Cedex 15, FRANCE, Email: [email protected] (8) Cooperative Institute for Research in Environmental Sciences, NOAA/ESRL/PSD, 325 Broadway, R/PSD2, Boulder, CO 80305, USA, Email: [email protected] (9) National Oceanography Centre, European Way, Southampton, SO14 3ZH, UK, Emails: [email protected], -
The Monterey Area Ship Track Experiment
Calhoun: The NPS Institutional Archive Faculty and Researcher Publications Faculty and Researcher Publications 2000-08-15 The Monterey Area Ship Track Experiment Durkee, Philip A. Journal of the Atmospheric Sciences, Vol. 57, 15 August 2000, pp. 2523-2541. http://hdl.handle.net/10945/46745 15 AUGUST 2000 DURKEE ET AL. 2523 The Monterey Area Ship Track Experiment PHILIP A. DURKEE Department of Meteorology, Naval Postgraduate School, Monterey, California KEVIN J. NOONE Stockholm University, Stockholm, Sweden ROBERT T. B LUTH Office of Naval Research, Arlington, Virginia (Manuscript received 14 November 1996, in final form 23 February 1999) ABSTRACT In June 1994 the Monterey Area Ship Track (MAST) experiment was conducted off the coast of California to investigate the processes behind anthropogenic modification of cloud albedo. The motivation for the MAST experiment is described here, as well as details of the experimental design. Measurement platforms and strategies are explained, and a summary of experiment operations is presented. The experiment produced the largest dataset to date of direct measurements of the effects of ships on the microphysics and radiative properties of marine stratocumulus clouds as an analog for the indirect effects of anthropogenic pollution on cloud albedo. 1. Introduction ever, the upper limit of the indirect aerosol forcing es timate was 21.5 W m22. Clearly, reducing the uncer Determining the effects of atmospheric aerosol par tainty in, or even arriving at, a central value for the ticles on the radiative balance of the earth has been a estimates of the indirect radiative effect of aerosols is major focus of recent climate research. -
Climate Intervention (July 2021)
State of the Science FACT SHEET Climate Intervention Climate Intervention (CI), also called climate engineering or geoengineering, refers to deliberate, large‐scale actions intended to counteract aspects of climate change. This Fact Sheet explains some of the fundamental principles and issues associated with CI (1). Why Might Climate Intervention Be Considered? The main driver of climate change over the past century has been anthropogenic emissions of carbon dioxide (CO2), a greenhouse gas (GHG). Increasing emission rates have caused present‐day atmospheric CO2 to reach the highest value in over a million years based on studies of emissions of atmospheric CO2 and its accumulation in the atmosphere, ocean, and terrestrial biosphere. The increased emissions of other GHGs, such as methane, nitrous oxide and ozone, also contribute to anthropogenic climate change. The increased accumulation of GHGs has led to warming over much of the globe, to acidification of ocean surface waters (from CO2) (2), and to many other well‐documented climate impacts (3). As climate change continues, if the world does not make the desired greenhouse gas emissions reductions (4) such as those initiated by the Paris agreement (5), governments and other entities might turn to CI to counteract increasing climate change impacts. CI could potentially be implemented by consensus or unilaterally; either way, a thorough understanding of CI methods, and their associated uncertainties and unintended side effects is essential. Principal CI methods are divided into two How might CDR be accomplished? general categories (6) (see figure): Oceanic sequestration: Adding nutrients, such as iron, to “ferti‐ lize” the ocean enhances biological growth (e.g., phytoplank‐ Carbon dioxide removal (CDR): CDR is a process to remove ton), which removes CO2 from surface waters and leads to lower CO2 from the atmosphere for long‐term storage on land or atmospheric levels. -
Oceanic Phytoplankton, Atmospheric Sulphur, Cloud Albedo and Climate Robert J
_N_A_TU_R_E~V_O_L_._32_6~16_A_P_R_I_L_1_9_87~~~~~~~~~~~1:\/IE:.\fV ~~"'fl~LJ:.~~~~~~~~~~~~~~~~~~~6_55 Oceanic phytoplankton, atmospheric sulphur, cloud albedo and climate Robert J. Charlson*, James E. Lovelockt, Meinrat 0. Andreae* & Stephen G. Warren* *Department of Atmospheric Sciences AK-40, University of Washington, Seattle, Washington 98195, USA t Coombe Mill Experimental Station. Launceston, Cornwall PL15 9RY, UK :j: Department of Oceanography, Florida State University, Tallahassee, Florida 32306, USA The major source of cloud-condensation nuclei (CCN) over the oceans appears to be dimethylsulphide, which is produced by planktonic algae in sea water and oxidizes in the atmosphere to form a sulphate aerosol. Because the reflectance (albedo) of clouds (and thus the Earth's radiation budget) is sensitive to CCN density, biological regulation of the climate is possible through the effects of temperature and sunlight on phytoplankton population and dimethylsulphide production. To counteract the warming due to doubling of atmospheric C02' an approximate doubling of CCN would be needed. CLIMATIC influences of the biota are usually thought of in a volcano is of regional importance only. Large eruptions, on connection with biological release and uptake of C02 and CH4 the other hand, which emit enough gaseous sulphur compounds and the effect of these gases on the infrared radiative properties to influence wider areas, are relatively rare events. For this 1 of the atmosphere • However, the atmospheric aerosol also discussion, we shall assume that the contribution of CCN from participates in the radiation balance, and Shaw2 has proposed volcanic sulphur to the global atmosphere is proportional to its that the aerosol produced by the atmospheric oxidation of contribution to the total sulphur flux, that is, 10-20% of the sulphur gases from the biota may also affect climate. -
Experimental Studies on Particle Emissions from Cruising Ship, Their Characteristic Properties, Transformation and Atmospheric Lifetime in the Marine Boundary Layer
Atmos. Chem. Phys., 8, 2387–2403, 2008 www.atmos-chem-phys.net/8/2387/2008/ Atmospheric © Author(s) 2008. This work is distributed under Chemistry the Creative Commons Attribution 3.0 License. and Physics Experimental studies on particle emissions from cruising ship, their characteristic properties, transformation and atmospheric lifetime in the marine boundary layer A. Petzold1, J. Hasselbach1, P. Lauer2, R. Baumann1, K. Franke3, C. Gurk4, H. Schlager1, and E. Weingartner5 1Dt. Zentrum fur¨ Luft- und Raumfahrt, Inst. fur¨ Physik der Atmosphare,¨ Oberpfaffenhofen, 82234 Wessling, Germany 2MAN Diesel SE, Stadtbachstr. 1, 86135 Augsburg, Germany 3Institute for Environmental Physics, University of Bremen, Otto-Hahn-Allee 1, 28359 Bremen, Germany 4Max-Planck-Institute for Chemistry, Johann-Joachim-Becher-Weg 27, 55128 Mainz, Germany 5Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland Received: 9 October 2007 – Published in Atmos. Chem. Phys. Discuss.: 19 October 2007 Revised: 17 March 2008 – Accepted: 15 April 2008 – Published: 6 May 2008 Abstract. Particle emissions from ship engines and their ship exhaust particle number concentrations in an expanding atmospheric transformation in the marine boundary layer plume, a maximum plume life time of approx. 24 h is esti- (MBL) were investigated in engine test bed studies and in mated for a well-mixed marine boundary layer. airborne measurements of expanding ship plumes. During the test rig studies, detailed aerosol microphysical and chem- ical properties were measured in the exhaust gas of a serial 1 Introduction MAN B&W seven-cylinder four-stroke marine diesel engine under various load conditions. The emission studies were Shipping represents a major contribution to the international complemented by airborne aerosol transformation studies in transportation sector which, however, is not well quantified the plume of a large container ship in the English Chan- in terms of global emissions and climate impacts. -
Observations of Ship Tracks from Ship-Based Platforms
JANUARY 1999 PORCH ET AL. 69 Observations of Ship Tracks from Ship-Based Platforms W. P ORCH,* R. BORYS,1 P. D URKEE,# R. GASPAROVIC,@ W. H OOPER,& E. HINDMAN,** AND K. NIELSEN# * Los Alamos National Laboratory, Los Alamos, New Mexico 1 Atmospheric Sciences Center, Desert Research Institute, Reno, Nevada # Department of Meteorology, Naval Postgraduate School, Monterey, California @ The Johns Hopkins University, APL, Laurel, Maryland & Naval Research Laboratory, Washington, D.C. ** Earth and Atmospheric Sciences Department, City College of New York, New York, New York (Manuscript received 17 October 1997, in ®nal form 17 February 1998) ABSTRACT Ship-based measurements in June 1994 provided information about ship-track clouds and associated atmo- spheric environment observed from below cloud levels that provide a perspective different from satellite and aircraft measurements. Surface measurements of latent and sensible heat ¯uxes, sea surface temperatures, and meteorological pro®les with free and tethered balloons provided necessary input conditions for models of ship- track formation and maintenance. Remote sensing measurements showed a coupling of ship plume dynamics and entrainment into overlaying clouds. Morphological and dynamic effects were observed on clouds unique to the ship tracks. These morphological changes included lower cloud bases early in the ship-track formation, evidence of raised cloud bases in more mature tracks, sometimes higher cloud tops, thin cloud-free regions paralleling the tracks, and often stronger radar returns. The ship-based lidar aerosol measurements revealed that ship plumes often interacted with the overlying clouds in an intermittent rather than continuous manner. These observations imply that more must be learned about ship-track dynamics before simple relations between cloud condensation nuclei and cloud brightness can be developed. -
Earth Energy Budget and Balance
Earth energy budget and balance 31% total reflection (23% clouds. 8% surface) Reflection is frequency dependent but will be 69% absorption( 20% clouds, 49% surface) treated as average value for visible light range. Simplified scheme of the balance between the incident, reflected, Fi transmitted, and absorbed radiation Fr Ft Box Model Fa Kirchhoff’s law Efficiency factors F F F : emissivity (=absorptivity) F F F F r a t 1 i r a t α: albedo Fi Fi Fi : opacity (=1-transmittivity) 1 Black body: =1, α=0 Albedo, Absorption, Opacity Opaque body: =0 The incident, absorbed, reflected, and transmitted flux depends sensitively on the wavelength of the radiation! Albedo The ratio of reflected to incident solar energy is called the Albedo α At present cloud and climate conditions: 31% The Albedo depends on the Surface Albedo nature and characteristics of Asphalt 4-12% the reflecting surface, a light surface has a large Albedo Forest 8-18% (maximum 1 or 100%), a dark Bare soil 17% surface has a small Albedo Green grass 25% (minimum 0 or 0%). Desert sand 40% New concrete 55% Ocean Ice 50-70% Fresh snow 80-90% Albedo of Earth αice >35% αforest 12% αforest 12% αagriculture 20% αagriculture 20% αdesert 30% αdesert 30% αdesert 30% αforest 12% αforest 12% αocean <10% αocean <10% αice >35% Tundra 20% Arctic ocean 7 % New snow 80% Melting ice 65% Melt pond 20% Clear skies versus clouds At clear skies Albedo is relatively low because of the high Albedo value of water. This translates in an overall variation of 5-10%.