Atmos. Chem. Phys., 14, 12763–12779, 2014 www.atmos-chem-phys.net/14/12763/2014/ doi:10.5194/acp-14-12763-2014 © Author(s) 2014. CC Attribution 3.0 License. Surface-to-mountaintop transport characterised by radon observations at the Jungfraujoch A. D. Griffiths1, F. Conen2, E. Weingartner3,*, L. Zimmermann2, S. D. Chambers1, A. G. Williams1, and M. Steinbacher4 1Australian Nuclear Science and Technology Organisation, New South Wales, Australia 2Environmental Geosciences, Department of Geosciences, University of Basel, Basel, Switzerland 3Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232 Villigen, Switzerland 4Swiss Federal Laboratories for Materials Science and Technology (Empa), Dübendorf, Switzerland *now at: Institute for Aerosol and Sensor Technology, University of Applied Sciences, 5210 Windisch, Switzerland Correspondence to: A. D. Griffiths (alan.griffi
[email protected]) Received: 5 May 2014 – Published in Atmos. Chem. Phys. Discuss.: 4 July 2014 Revised: 30 September 2014 – Accepted: 17 October 2014 – Published: 5 December 2014 Abstract. Atmospheric composition measurements at masses which have travelled far from emission sources and Jungfraujoch are affected intermittently by boundary-layer had time to mix. But local sources can still have an influence, air which is brought to the station by processes including depending largely on the recent history of vertical transport thermally driven (anabatic) mountain winds. Using obser- and associated mixing. This necessitates the development of vations of radon-222, and a new objective analysis method, carefully considered data selection techniques. we quantify the land-surface influence at Jungfraujoch hour The task of understanding vertical transport becomes par- by hour and detect the presence of anabatic winds on a ticularly complicated in mountainous terrain (Rotach and daily basis.