Ex-Vessel Steam Explosion Analysis for Pressurized Water Reactor and Boiling Water Reactor
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A Window Into the Meltdown Events at the Fukushima Daiichi Nuclear
www.nature.com/scientificreports OPEN Caesium-rich micro-particles: A window into the meltdown events at the Fukushima Daiichi Nuclear Received: 12 October 2016 Accepted: 12 January 2017 Power Plant Published: 15 February 2017 Genki Furuki1,*, Junpei Imoto1,*, Asumi Ochiai1, Shinya Yamasaki2, Kenji Nanba3, Toshihiko Ohnuki4, Bernd Grambow5, Rodney C. Ewing6 & Satoshi Utsunomiya1 The nuclear disaster at the Fukushima Daiichi Nuclear Power Plant (FDNPP) in March 2011 caused partial meltdowns of three reactors. During the meltdowns, a type of condensed particle, a caesium-rich micro-particle (CsMP), formed inside the reactors via unknown processes. Here we report the chemical and physical processes of CsMP formation inside the reactors during the meltdowns based on atomic- resolution electron microscopy of CsMPs discovered near the FDNPP. All of the CsMPs (with sizes of 2.0–3.4 μm) comprise SiO2 glass matrices and ~10-nm-sized Zn–Fe-oxide nanoparticles associated with a wide range of Cs concentrations (1.1–19 wt% Cs as Cs2O). Trace amounts of U are also associated with the Zn–Fe oxides. The nano-texture in the CsMPs records multiple reaction-process steps during meltdown in the severe FDNPP accident: Melted fuel (molten core)-concrete interactions (MCCIs), incorporating various airborne fission product nanoparticles, including CsOH and CsCl, proceeded via SiO2 condensation over aggregates of Zn-Fe oxide nanoparticles originating from the failure of the reactor pressure vessels. Still, CsMPs provide a mechanism by which volatile and low-volatility radionuclides such as U can reach the environment and should be considered in the migration model of Cs and radionuclides in the current environment surrounding the FDNPP. -
Nuclear Reactor Realities
Page 1 of 26 Nuclear Reactor Realities NUCLEAR REACTOR REALITIES (An Australian viewpoint) PREFACE Now that steam ships are no longer common, people tend to forget that nuclear power is just a replacement of coal, oil or gas for heating water to form steam to drive turbines, or of water (hydro) to do so directly. As will be shown in this tract, it is by far the safest way of doing so to generate electricity economically in large quantities – as a marine engineer of my acquaintance is fond of saying. Recently Quantum Market Research released its latest Australian Scan (The Advertiser, Saturday April 17, 2012, p 17). It has been tracking social change by interviewing 2000 Australians annually since 1992. In the concerns in the environment category, “[a]t the top of the list is nuclear accidents and waste disposal” (44.4 per cent), while “global warming” was well down the list of priorities at No 15, with only 27.7 per cent of people surveyed rating the issue as “extremely serious.” Part of the cause of such information must be that people are slowly realising that they have been deluded by publicity about unverified computer models which indicate that man’s emissions of CO2 play a major part in global warming. They have not yet realised that the history of the dangers of civilian nuclear power generation shows the reverse of their images. The topic of nuclear waste disposal is also shrouded in reactor physics mysteries, leading to a mis-placed general fear of the unknown. In this article only nuclear reactors are considered. -
Implications of the Accident at Chernobyl for Safety Regulation of Commercial Nuclear Power Plants in the United States Final Report
NUREG-1251 Vol. I Implications of the Accident at Chernobyl for Safety Regulation of Commercial Nuclear Power Plants in the United States Final Report Main Report U.S. Nuclear Regulatory Commission p. o AVAILABILITY NOTICE Availability of Reference Materials Cited in NRC Publications Most documents cited in NRC publications will be available from one of the following sources: 1. The NRC Public Document Room, 2120 L Street, NW, Lower Level, Washington, DC 20555 2. The Superintendent of Documents, U.S. Government Printing Office, P.O. Box 37082, Washington, DC 20013-7082 3. The National Technical Information Service, Springfield, VA 22161 Although the listing that follows represents the majority of documents cited in NRC publica- tions, it is not intended to be exhaustive. Referenced documents available for inspection and copying for a fee from the NRC Public Document Room include NRC correspondence and internal NRC memoranda; NRC Office of Inspection and Enforcement bulletins, circulars, information notices, inspection and investi- gation notices; Licensee Event Reports; vendor reports and correspondence; Commission papers; and applicant and licensee documents and correspondence. The following documents in the NUREG series are available for purchase from the GPO Sales Program: formal NRC staff and contractor reports, NRC-sponsored conference proceed- ings, and NRC booklets and brochures. Also available are Regulatory Guides, NRC regula- tions in the Code of Federal Regulations, and Nuclear Regulatory Commission Issuances. Documents available from the National Technical Information Service include NUREG series reports and technical reports prepared by other federal agencies and reports prepared by the Atomic Energy Commission, forerunner agency to the Nuclear Regulatory Commission. -
Calculating Nuclear Accident Probabilities from Empirical Frequencies Minh Ha-Duong, V
Calculating nuclear accident probabilities from empirical frequencies Minh Ha-Duong, V. Journé To cite this version: Minh Ha-Duong, V. Journé. Calculating nuclear accident probabilities from empirical frequencies. Environment Systems and Decisions, Springer, 2014, 34 (2), pp.249-258. 10.1007/s10669-014-9499-0. hal-01018478v2 HAL Id: hal-01018478 https://hal.archives-ouvertes.fr/hal-01018478v2 Submitted on 21 Jul 2014 HAL is a multi-disciplinary open access L’archive ouverte pluridisciplinaire HAL, est archive for the deposit and dissemination of sci- destinée au dépôt et à la diffusion de documents entific research documents, whether they are pub- scientifiques de niveau recherche, publiés ou non, lished or not. The documents may come from émanant des établissements d’enseignement et de teaching and research institutions in France or recherche français ou étrangers, des laboratoires abroad, or from public or private research centers. publics ou privés. Distributed under a Creative Commons Attribution - NonCommercial - ShareAlike| 4.0 International License Manuscript to appear in Environment, Systems and Decisions CALCULATING NUCLEAR ACCIDENT PROBABILITIES FROM EMPIRICAL FREQUENCIES Minh Ha-Duong et Venance Journé1 2014-04-10 Summary Since there is no authoritative, comprehensive and public historical record of nuclear power plant accidents, we reconstructed a nuclear accident dataset from peer-reviewed and other literature. We found that, in a sample of five random years, the worldwide historical frequency of a nuclear major accident, defined as an INES level 7 event, is 14%. This value is 67 % to have at least one nuclear accident rated at level ≥ 4 on the INES scale. These numbers are subject to uncertainties because the fuzziness of the definition of a nuclear accident. -
The SL-1 Accident Consequences
The SL-1 Accident Consequences Key Things to Remember On the night of January 3, 1961, the SL-1 nuclear reactor, a About prototype for a military installation to be used in remote Arctic SL-1 Accident Consequences: locations, exploded, killing the three-member military crew. The crew had been performing the routine process of re-assembling 1. The SL-1’s highly enriched fuel the reactor control rod drive mechanisms during a reactor outage. had high burnup and had The SL-1 was a small 3 Mega-Watt-thermal (MWt) boiling water operated for 932 MW-days, reactor, complete with a turbine-generator and condenser building up fission products in designed to generate both electric power and building heat. 1 the fuel before the accident. 2. The SL-1 condensers were on The SL-1 was designed, constructed and initially operated by the top of the building and the Argonne National Laboratory. It was located at the Idaho reactor was in a ventilated National Laboratory, then called the National Reactor Testing building with no containment. Station. Combustion Engineering became the operating 3. About 30 percent of SL-1’s fuel contractor for the Atomic Energy Commission (now the was absent from the reactor Department of Energy) for SL-1 on February 5, 1959. vessel after the accident. 4. The AEC claimed that basically The SL-1 had first gone critical on August 1, 1958 and by only iodine-131 was in the July 1, 1959 had accumulated 160 Mega-Watt operating days radioactive plume from the (MWD). By August 21, 1960, the reactor had accumulated 680 accident. -
On Vapor/Steam Explosion Analysis
THE NUCLEAR NEWS INTERVIEW Fauske and Henry: On vapor/steam explosion analysis Vapor explosions are an integral part of reactor safety evaluations when accident conditions could lead to molten fuel coming in contact with liquid coolant. he book Experimental Technical Bases for Evalu- involving these types of explosions must be evaluated ating Vapor/Steam Explosions in Nuclear Reactor in a manner consistent with the available experimen- TSafety was recently published by the American tal technical bases. Their new book, they say, provides a Nuclear Society. The authors, Hans Fauske and Robert common reference that includes the total experimental Henry, say that the possibility of vapor/steam explo- database for vapor/steam explosions, as well as informa- sions occurring at nuclear power plants is an important tion directly related to molten materials and the coolant consideration for safety assessments of events wherein a of interest. high-temperature molten mass could come into contact Early in his career, Fauske joined Argonne National with a liquid coolant. Laboratory, where he focused on reactor safety evalua- The authors stress that potential accident conditions tions for both fast and light-water reactors. Vapor explo- sions were a key element of the safety evaluations for the Fast Flux Test Fa- cility and the Clinch River Breeder Reactor designs, and steam explo- sions were an important part of the safety assessments for water-cooled reactors. Fauske left ANL in 1980 to establish, with Robert Henry and Michael Grolmes, Fauske & Associ- ates. In 2011, Fauske stepped away from management responsibilities at the company to spend more time on engineering evaluations and writing. -
A Comparative Study of Flammability Limit Models for H2/CO Mixture on the Applicability of Severe Accident Conditions
Transactions of the Korean Nuclear Society Spring Meeting Jeju, Korea, May 23-24, 2019 A Comparative Study of Flammability Limit Models for H2/CO Mixture on the Applicability of Severe Accident Conditions 1 1 1 1,2 Yeon Soo Kim , Joongoo Jeon , Wonjun Choi , Sung Joong Kim * 1Department of Nuclear Engineering, Hanyang University 2Institutte of Nano Science and Technology, Hanyang University 222 Wangsimni-ro, Seongdong-gu, Seoul 04763, Republic of Korea *Corresponding author: [email protected] 1. Introduction sustainably. Lower flammability limit (LFL) is the minimum concentration while upper flammability limit Through the Fukushima accident, it was proved that (UFL) is the maximum concentration. As the amount of hydrogen released into containment building may cause combustible gas which can be generated in nuclear explosion under severe accident (SA). After the accident, power plant is limiting, LFL is mainly applied in researches have been actively conducted to predict and flammability evaluation under severe accident. mitigate the combustion risk. On the other hand, as the Because hydrogen and carbon monoxide coexist in the accident progresses to ex-vessel phase, carbon monoxide containment building at ex-vessel phase, the LFL of is generated in the containment by molten corium- H2/CO mixture should be obtained separately. In this concrete interaction (MCCI). Carbon monoxide is also section, the various method to predict the LFL of H2/CO flammable gas, which can increase the combustion risk is described in three categories; MELCOR default option, when coexisting with hydrogen. However, most of the empirical correlations and method based on the theory. previous studies have mainly focused on hydrogen and paid relatively less attention to carbon monoxide. -
SKI Report 02:16 a Review of Steam Explosions with Special Emphasis
The APRI 4 (Accident Phenomena of Risk Importance) research project is accomplished by: • Swedish Nuclear Power Inspectorate • Ringhals AB • OKG Aktiebolag • Forsmarks Kraftgrupp AB • Barsebäck Kraft AB • Teollisuuden Voima Oy (TVO) and supervised by the Project Board, consisting of: OKG Aktiebolag Mauritz Gärdinge, chairman Swedish Nuclear Power Inspectorate Oddbjörn Sandervåg Ringhals AB Anders Henoch Forsmarks Kraftgrupp AB Ingvar Berglund Barsebäcks Kraft AB Erik Larsen TVO Heikki Sjövall Contents Abstract v 1 Introduction 1 1.1 Study objectives and workscope . .................. 2 1.2 References . ............................. 3 2 Task 1: A general review of the phenomenology of a steam explosion during a postulated severe accident in nuclear power plants 4 2.1 General picture on MFCI . ......................... 4 2.1.1 Fuel Coolant Interaction (FCI) . .................. 5 2.2 Molten fuel-coolant premixing . .................. 7 2.2.1 Status of current research and recent results . ........... 7 2.2.2 Inter-relations and uncertainties of molten fuel-coolant premixing . 9 2.2.3 Self-limiting mechanisms in melt-water premixing . .... 11 2.3 Molten fuel-coolant triggering . .................. 12 2.3.1 Status of current research and recent results . ........... 12 2.3.2 Triggering experiments . .................. 14 2.3.3 Analytical work on triggering . .................. 17 2.3.4 Conclusions . ............................. 18 i 2.4 Results from steam explosion experiments with different melt materials . 19 2.5 Computational investigation of steam explosion . ........... 20 2.5.1 PM-ALPHA and ESPROSE.m codes . ........... 20 2.5.2 MC3D code . ............................. 22 2.5.3 Computations of the KROTOS tests with the codes COMETA, TEXAS and SEURBNUK/EURDYN . .................. 23 2.6 Summary . ............................. 24 2.6.1 Premixing/Quenching . -
The Results of Two Recent Corium-Water Thermal Interaction (CWTI)
CONF-850810—10 DE85 007897 CORIUM QUENCH IN DEEP POOL MIXING EXPERIMENTS* by B. W. Spencer, L. McUmber, D. Gregorash, R. Aeschlimann, and J. J. Sienicki Reactor Analysis and Safety Division Argonne National Laboratory Argonne, IL 60439 ABSTRACT The results of two recent corium-water thermal interaction (CWTI) tests are described in which a stream of molten corium was poured into a deep pool of water in order to determine the mixing behavior, the corf urn-to-water heat transfer rates, and the characteristic sizes of the quenched debris. The corium composition was 60% UOg, 16% ZrO2, and 24% stainless steel by weight; its initial temperature was 3080 K, ~ 160 K above the oxide phase liquidus temperature. The corium pour stream was a single-phase 2.2 cm dia liquid column which entered the water pool in film boiling at ~ 4 m/s. The water subcooling was 6 and 75C in the two tests. Test results showed that with low subcooling, rapid steam generation caused the pool to boil up into a high void fraction regime. In contrast, with large subcooling no net steam generation occurred, and the pool remained relatively quiescant. Breakup of the jet appeared to occur by surface stripping. In neither test was the breakup com- plete during transit through the 32 cm deep water pool, and molten corium channeled to the base where it formed a melt layer. The characteristic heat transfer rates measured 3.5 MJ/s and 2.7 MJ/s during the fall stage for small and large subcooling, respectively; during the initial stage of bed quench, the surface heat fluxes measured 2.4 MW/m2 and 3.7 MW/m2, respectively. -
Historical Loss Experiences in the Global Power Industry August 2014 Contents
MARSH RISK MANAGEMENT RESEARCH HISTORICAL LOSS EXPERIENCES IN THE GLOBAL POWER INDUSTRY AUGUST 2014 CONTENTS 1 INTRODUCTION 2 PART ONE: PRINCIPLES OF GENERATING ELECTRICITY 8 PART TWO: HISTORICAL LOSSES 48 CONCLUSION HISTORICAL LOSS EXPERIENCES IN THE GLOBAL POWER INDUSTRY ii marsh.com MARSH RISK MANAGEMENT RESEARCH INTRODUCTION At Marsh, our claims management and power industry experience enables us to present an accurate description of the types of events that commonly lead to insurance claims. To compile this study, we used data and an analysis of global trends that many power clients will already be acquainted with. The purpose of this document is to provide commentary on the world of power generation, the risks affecting that industry, and the importance of effective risk management in preventing or mitigating these risks. The report is divided into two parts: ȫ Part one provides a brief overview of some of the key technologies being used in power generation, including details of some areas that are either emergent or in the research-and-development stage at the time of writing. ȫ Part two features a narrative description of some of the historical loss experiences that have affected the power generation industry in recent years. It may be helpful to review this document along with the following recent Marsh Risk Management Research briefings on power generation: ȫ The Impact of Large Losses in the Global Power Industry. ȫ Common Causes of Large Losses in the Global Power Industry. We trust that you will find this document both illuminating and helpful as you consider the risks your own organization faces. -
NUREG/CR-6042, Rev. 2 [3:4] Appendix
Reactor Safety Course (R-800) 3.7 Special Consideration for BWR Facilities 3.7 Special Considerations for BWR for reactor vessel pressure control when run Facilities continuously in the recirculation mode, pumping water from the condensate storage Boiling water reactors have unique features tank back to the condensate storage tank and that would cause their behavior under severe periodically diverting a small portion of the accident conditions to differ significantly flow into the reactor vessel as necessary to from that expected for the pressurized water maintain the desired water level. The steam reactor design.1,2 This section addresses taken from the reactor vessel by the turbine several special considerations affecting BWR is passed to the pressure suppression pool as severe accident progression and mitigation. turbine exhaust, which provides a slower In this endeavor, many implications of the rate of pool temperature increase than if the phenomena described in Sections 3.1 through vessel pressure control were obtained by 3.6 (such as zirconium oxidation) will be direct passage of steam from the vessel to demonstrated by example. First, however, it the pool via the SRVs. Plants having both is necessary to review some of the BWR HPCI and RCIC systems can employ the features pertinent to severe accident HPCI turbine exclusively for pressure considerations. control while the RCIC system is used to maintain the reactor vessel water level. The 3.7.1 Pertinent BWR Features HPCI turbine is larger than the RCIC turbine and, therefore, is more effective for pressure An important distinction of the BWR design control. These systems require DC power for is that provisions are made for direct valve and turbine governor control, but have operator control of reactor vessel water level no requirement for control air. -
09 Fr0200361
09 FR0200361 ^r.^r IQ 34. IMPORTANCE OF PROTOTYPIC-CORIUM EXPERIMENTS FOR SEVERE ACCIDENT RESEARCH P. PILUSO, C. JOURNEAU, G. COGNET, D. MAGALLON*, J.M. SEILER** CEA Cadarache 13108 St Paul les Durance cedex, France *: detached from the Joint Research Centre of the European Commission ** CEA Grenoble KEY WORDS: Severe accidents, Nuclear materials, Experiments Introduction: In case of a severe accident in a nuclear reactor, very complex physical and chemical phenomena would occur. Parallel to the development of mechanistic and scenario codes, experiments are needed to determine key phenomena and coupling, develop and qualify specific models, validate codes. Due to lower costs and constraints, experiments using low temperature simulant materials (such as CORINE [1] or Scaled Simulant Spreading Experiments (S3C) [2] for spreading or BALI [3,4] for in-vessel pools) allow the testing of a large number of configurations and the determination of correlations. But some crucial corium phenomena and behaviours such as the importance of radiation heat transfer or the presence of a large liquidus-solidus interval (up to 1000 K) are not reproduced in low temperature experiments. Consequently, it is attempted to simulate real corium with high temperature simulant materials: alumina, thermite, widely used (e.g. KATS [5] or COMET [6] facilities); high temperature salts or mixtures with zirconia and/or hafnia. However, it is not feasible to simulate all the aspects of corium phenomenology, especially its high temperature behaviour. Therefore, experiments with prototypic material are performed to check the results obtained with simulants and identify possible differences. In this context, CEA has undertaken a large program on severe accidents with prototypic corium [7].