Requirements for a Next Generation Nuclear Data Format
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Computing ATOMIC NUCLEI
UNIVERSAL NUCLEAR ENERGY DENSITY FUNCTIONAL Computing ATOMIC NUCLEI Petascale computing helps disentangle the nuclear puzzle. The goal of the Universal Nuclear Energy Density Functional (UNEDF) collaboration is to provide a comprehensive description of all nuclei and their reactions based on the most accurate knowledge of the nuclear interaction, the most reliable theoretical approaches, and the massive use of computer power. Science of Nuclei the Hamiltonian matrix. Coupled cluster (CC) Nuclei comprise 99.9% of all baryonic matter in techniques, which were formulated by nuclear sci- the Universe and are the fuel that burns in stars. entists in the 1950s, are essential techniques in The rather complex nature of the nuclear forces chemistry today and have recently been resurgent among protons and neutrons generates a broad in nuclear structure. Quantum Monte Carlo tech- range and diversity in the nuclear phenomena that niques dominate studies of phase transitions in can be observed. As shown during the last decade, spin systems and nuclei. These methods are used developing a comprehensive description of all to understand both the nuclear and electronic nuclei and their reactions requires theoretical and equations of state in condensed systems, and they experimental investigations of rare isotopes with are used to investigate the excitation spectra in unusual neutron-to-proton ratios. These nuclei nuclei, atoms, and molecules. are labeled exotic, or rare, because they are not When applied to systems with many active par- typically found on Earth. They are difficult to pro- ticles, ab initio and configuration interaction duce experimentally because they usually have methods present computational challenges as the extremely short lifetimes. -
Nuclear Data
CNIC-00810 CNDC-0013 INDC(CPR)-031/L NUCLEAR DATA No. 10 (1993) China Nuclear Information Center Chinese Nuclear Data Center Atomic Energy Press CNIC-00810 CNDC-0013 INDC(CPR)-031/L COMMUNICATION OF NUCLEAR DATA PROGRESS No. 10 (1993) Chinese Nuclear Data Center China Nuclear Information Centre Atomic Energy Press Beijing, December 1993 EDITORIAL BOARD Editor-in-Chief Liu Tingjin Zhuang Youxiang Member Cai Chonghai Cai Dunjiu Chen Zhenpeng Huang Houkun Liu Tingjin Ma Gonggui Shen Qingbiao Tang Guoyou Tang Hongqing Wang Yansen Wang Yaoqing Zhang Jingshang Zhang Xianqing Zhuang Youxiang Editorial Department Li Manli Sun Naihong Li Shuzhen EDITORIAL NOTE This is the tenth issue of Communication of Nuclear Data Progress (CNDP), in which the achievements in nuclear data field since the last year in China are carried. It includes the measurements of 54Fe(d,a), 56Fe(d,2n), 58Ni(d,a), (d,an), (d,x)57Ni, 182~ 184W(d,2n), 186W(d,p), (d,2n) and S8Ni(n,a) reactions; theoretical calculations on n+160 and ,97Au, 10B(n,n) and (n,n') reac tions, channel theory of fission with diffusive dynamics; the evaluations of in termediate energy nuclear data for 56Fe, 63Cu, 65Cu(p,n) monitor reactions, and of 180Hf, ,8lTa(n,2n) reactions, revision on recommended data of 235U and 238U for CENDL-2; fission barrier parameters sublibrary, a PC software of EXFOR compilation, some reports on atomic and molecular data and covariance research. We hope that our readers and colleagues will not spare their comments, in order to improve the publication. Please write to Drs. -
Nuclear Data Library for Incident Proton Energies to 150 Mev
LA-UR-00-1067 Approved for public release; distribution is unlimited. 7Li(p,n) Nuclear Data Library for Incident Proton Title: Energies to 150 MeV Author(s): S. G. Mashnik, M. B. Chadwick, P. G. Young, R. E. MacFarlane, and L. S. Waters Submitted to: http://lib-www.lanl.gov/la-pubs/00393814.pdf Los Alamos National Laboratory, an affirmative action/equal opportunity employer, is operated by the University of California for the U.S. Department of Energy under contract W-7405-ENG-36. By acceptance of this article, the publisher recognizes that the U.S. Government retains a nonexclusive, royalty- free license to publish or reproduce the published form of this contribution, or to allow others to do so, for U.S. Government purposes. Los Alamos National Laboratory requests that the publisher identify this article as work performed under the auspices of the U.S. Department of Energy. Los Alamos National Laboratory strongly supports academic freedom and a researcher's right to publish; as an institution, however, the Laboratory does not endorse the viewpoint of a publication or guarantee its technical correctness. FORM 836 (10/96) Li(p,n) Nuclear Data Library for Incident Proton Energies to 150 MeV S. G. Mashnik, M. B. Chadwick, P. G. Young, R. E. MacFarlane, and L. S. Waters Los Alamos National Laboratory, Los Alamos, NM 87545 Abstract Researchers at Los Alamos National Laboratory are considering the possibility of using the Low Energy Demonstration Accelerator (LEDA), constructed at LANSCE for the Ac- celerator Production of Tritium program (APT), as a neutron source. Evaluated nuclear data are needed for the p+ ¡ Li reaction, to predict neutron production from thin and thick lithium targets. -
Nuclear Energy Agency Nuclear Data Committee
NUCLEAR ENERGY AGENCY NUCLEAR DATA COMMITTEE SUMMARY RECORD OF THE lWEEFPY-FIRST MEETING (Technical Sessions) CBNM, Gee1 (Belgium) 24th-28th September 1979 Compiled by C. COCEVA (Scientific Secretary) OECD NUCLEAR ENERGY AGENCY 38 Bd. Suchet, 75016 Paris TABLE OF CONTENTS TECHNICAL SESSIONS Participants in meeting 1. Isotopes 2. National Progress Reports 3. Meetings 4. Technical Discussions 5. Topical Meeting on "Progress in Neutron Data of Structural Materials for Fast ~eactors" 6. Neutron and Related Nuclear Data Compilations and Evaluations Appendices 1 Meetings of the IAEA/NDS planned for 1980, 1981 and 1982 2 Progranme of the Topical Meeting on "Progress in Neutron Data of Structural Materials for Fast Reactors " 3 Summary of the general discussion on the works presented at the Topical Meeting TECmTICAL SESSIONS Perticipants in the 21st Meeting were as follows : For Canada : Dr. W.G. Cross Atomic Energy of Canada Ltd. Chalk River For Japan : Dr. K. Tsukada Japan Atomic Energy Research Institute Tokai-blur a For the United States of America : Dr. R.E. Chrien (Chairman) Brookhaven National Laboratory Dr. S.L. Wl~etstone U.S. Department of Energy Dr. 8.T. Motz Los Alamos Scientific Laboratory Dr. F.G. Perey Oak Ridge National Laboratory For the countries of the European Communities and the European Commission acting together : Dr. R. Iiockhoff (Local Secretary) Central Bureau for Nuclear Pleasurements Geel, Belgium Dr. C. Coceva (Scientific Secretary) Comitato Nazionale per 1'Energia Nucleare Bologna, Italy Dr. S. Cierjacks Kernforschungszentrum Karlsruhe Federal Republic of Germany Dr. C. Fort Conunissariat i 1'Energie Atomique Cadaroche, France Dr. A. Michaudon (Vice-chairman) Commissariat 2 1'Energie Atomique Bruysrcs-1.e-ChZtel Dr. -
The JEFF-3.1.1 Nuclear Data Library
Data Bank ISBN 978-92-64-99074-6 The JEFF-3.1.1 Nuclear Data Library JEFF Report 22 Validation Results from JEF-2.2 to JEFF-3.1.1 A. Santamarina, D. Bernard, P. Blaise, M. Coste, A. Courcelle, T.D. Huynh, C. Jouanne, P. Leconte, O. Litaize, S. Mengelle, G. Noguère, J-M. Ruggiéri, O. Sérot, J. Tommasi, C. Vaglio, J-F. Vidal Edited by A. Santamarina, D. Bernard, Y. Rugama © OECD 2009 NEA No. 6807 NUCLEAR ENERGY AGENCY Organisation for Economic Co-operation and Development ORGANISATION FOR ECONOMIC CO-OPERATION AND DEVELOPMENT The OECD is a unique forum where the governments of 30 democracies work together to address the economic, social and environmental challenges of globalisation. The OECD is also at the forefront of efforts to understand and to help governments respond to new developments and concerns, such as corporate governance, the information economy and the challenges of an ageing population. The Organisation provides a setting where governments can compare policy experiences, seek answers to common problems, identify good practice and work to co-ordinate domestic and international policies. The OECD member countries are: Australia, Austria, Belgium, Canada, the Czech Republic, Denmark, Finland, France, Germany, Greece, Hungary, Iceland, Ireland, Italy, Japan, Korea, Luxembourg, Mexico, the Netherlands, New Zealand, Norway, Poland, Portugal, the Slovak Republic, Spain, Sweden, Switzerland, Turkey, the United Kingdom and the United States. The Commission of the European Communities takes part in the work of the OECD. OECD Publishing disseminates widely the results of the Organisation’s statistics gathering and research on economic, social and environmental issues, as well as the conventions, guidelines and standards agreed by its members. -
Separation of Nuclear Isomers for Cancer Therapeutic Radionuclides
www.nature.com/scientificreports OPEN Separation of nuclear isomers for cancer therapeutic radionuclides based on nuclear decay after- Received: 03 November 2016 Accepted: 06 February 2017 effects Published: 13 March 2017 R. Bhardwaj1,2, A. van der Meer1, S. K. Das1, M. de Bruin1, J. Gascon2, H. T. Wolterbeek1, A. G. Denkova1 & P. Serra-Crespo1 177Lu has sprung as a promising radionuclide for targeted therapy. The low soft tissue penetration of its β− emission results in very efficient energy deposition in small-size tumours. Because of this, 177Lu is used in the treatment of neuroendocrine tumours and is also clinically approved for prostate cancer therapy. In this work, we report a separation method that achieves the challenging separation of the physically and chemically identical nuclear isomers, 177mLu and 177Lu. The separation method combines the nuclear after-effects of the nuclear decay, the use of a very stable chemical complex and a chromatographic separation. Based on this separation concept, a new type of radionuclide generator has been devised, in which the parent and the daughter radionuclides are the same elements. The 177mLu/177Lu radionuclide generator provides a new production route for the therapeutic radionuclide 177Lu and can bring significant growth in the research and development of177 Lu based pharmaceuticals. Lutetium-177 (177Lu) has emerged as a promising radionuclide for targeted therapy. The low energy β− emissions, a half-life of 6.64 days and the emission of low energy and low abundance γ-rays has made 177Lu a solid candidate to be the most applied therapeutic radionuclide by 20201. Its low energy β − particles with a tissue penetration of less than 3 mm make it suitable for targeting small primary and metastatic tumours, like prostate, breast, mela- noma, lung and pancreatic tumours, for bone palliation therapy and other chronic diseases2–4. -
Neutron Drip Line Nuclei HUGE D I F F U S E D PA IR ED
Neutron Drip line nuclei HUGE D i f f u s e d PA IR ED 4He 5He 6He 7He 8He 9He 10He Pairing and binding The Grand Nuclear Landscape (finite nuclei + extended nucleonic matter) superheavy Z=118, A=294 nuclei known up to Z=91 82 126 terra incognita known nuclei protons proton drip line 50 82 neutron stars 28 20 50 stable nuclei neutron drip line 8 28 2 20 probably known only up to oxygen 2 8 neutrons Binding Blocks http://www.york.ac.uk/physics/public-and-schools/schools/secondary/binding-blocks/ http://www.york.ac.uk/physics/public-and-schools/schools/secondary/binding- blocks/interactive/ https://arxiv.org/abs/1610.02296 http://www.nishina.riken.jp/enjoy/kakuzu/kakuzu_web.pdf The limits: Skyrme-DFT Benchmark 2012 120 stable nuclei 288 known nuclei ~3,000 drip line two-proton drip line N=258 80 S2n = 2 MeV Z=82 SV-min two-neutron drip line N=184 Asymptotic freedom ? 110 Z=50 40 N=126 100 proton number Z=28 N=82 proton number Z=20 90 230 244 N=50 232 240 248 256 N=28 Nuclear Landscape 2012 neutron number 0 N=20 0 40 80 120 160 200 240 280 fromneutron B. Sherrill number How many protons and neutrons can be bound in a nucleus? Literature: 5,000-12,000 Erler et al. Skyrme-DFT: 6,900±500 Nature 486, 509 (2012) syst HW: a) Using http://www.nndc.bnl.gov/chart/ find one- and two-nucleon separation energies of 6He, 7He, 8He, 141Ho, and 132Sn. -
Radioactive Decay & Decay Modes
CHAPTER 1 Radioactive Decay & Decay Modes Decay Series The terms ‘radioactive transmutation” and radioactive decay” are synonymous. Many radionuclides were found after the discovery of radioactivity in 1896. Their atomic mass and mass numbers were determined later, after the concept of isotopes had been established. The great variety of radionuclides present in thorium are listed in Table 1. Whereas thorium has only one isotope with a very long half-life (Th-232, uranium has two (U-238 and U-235), giving rise to one decay series for Th and two for U. To distin- guish the two decay series of U, they were named after long lived members: the uranium-radium series and the actinium series. The uranium-radium series includes the most important radium isotope (Ra-226) and the actinium series the most important actinium isotope (Ac-227). In all decay series, only α and β− decay are observed. With emission of an α particle (He- 4) the mass number decreases by 4 units, and the atomic number by 2 units (A’ = A - 4; Z’ = Z - 2). With emission β− particle the mass number does not change, but the atomic number increases by 1 unit (A’ = A; Z’ = Z + 1). By application of the displacement laws it can easily be deduced that all members of a certain decay series may differ from each other in their mass numbers only by multiples of 4 units. The mass number of Th-232 is 323, which can be written 4n (n=58). By variation of n, all possible mass numbers of the members of decay Engineering Aspects of Food Irradiation 1 Radioactive Decay series of Th-232 (thorium family) are obtained. -
Overview of Nuclear Data
Overview of Nuclear Data Michal Herman National Nuclear Data Center Brookhaven National Laboratory Nuclear Data Program Link between basic science and applications Nuclear Science Community ✦ experiments Eur. Phys.✦ J.theory A (2012) 48:113 Page 11 of 39 10Nuclear2 Data Application Cross section (barn) 10Community Community ✦ natural needs data: compilationLu(n,γ) @ DANCE 1 ENDF/B−VII.0 SAMMY7.0 broadened and fitted 10−1 1 10 102 ✦ ✦ evaluation Neutron energy (eV) complete Fig. 15. Cross-section for the 175Lu(n, γ) reaction measured with a natural Lutetium sample in the resolved resonance ✦ organized ✦range.archival 176Lu(n,γ) @ DANCE ✦ 104 ENDF/B−VII.0 SAMMY7 broadened and fitted traceable DANCE detector ✦ dissemination 103 ✦ readable LANSCE Cross section (barn) 102 Fig. 14. The DANCE detector (picture credits: LANSCE-NSM. Herman Berkeley, May 27-19, 2015 LA-UR-0802953). 10 1 processed into physical quantities, like the total γ cascade 10−1 1 10 102 energy, γ multiplicity, individual gamma ray energies, and Neutron energy (eV) neutron time of flight. After analysis of these data and sev- 176 eral corrections (calibration, dead time correction, back- Fig. 16. Cross-section for the Lu(n, γ)reactioninthere- solved resonance range. ground subtraction) the neutron radiative capture cross- section σ(n,γ)(En) is obtained. Results are presented here 176 2 Lu(n,γ) @ DANCE for three energy ranges: i) thermal energy, ii) resolved res- 10 onance region, and iii) above 1 keV in the unresolved res- ENDF/B−VII.0 onance region. K. Wisshak et al, 2006 H. Beer et al, 1984 i) For an incident neutron energy of 0.025 eV, the mea- BRC sured cross-sections for 175Lu(n, γ)and176Lu(n, γ), are in Cross section (barn) good agreement with published values [64] while improv- 10 ing their precisions. -
Nuclear Data: Serving Basic Needs of Science and Technology an Overview of the IAEA's International Nuclear Data Centre by Alex Lorenz and Joseph J
Information services for development Nuclear data: Serving basic needs of science and technology An overview of the IAEA's international nuclear data centre by Alex Lorenz and Joseph J. Schmidt In today's world, the transfer and spread of informa- number and sophistication of requests for information tion implies the systematic collection, classification, have increased considerably. As of now, scientists in storage, retrieval, and dissemination of knowledge with more than 70 Member States have received IAEA the essential use of computers. nuclear data services. The number of requests received To be able to take best advantage of information tech- annually by the IAEA Nuclear Data Section has doubled nology that has been developing over the last decades, over the last 5 years. Several developing Member States scientific knowledge has to be reduced to concentrated in the last few years have started development of nuclear factual statements or data. Today, the volume of infor- power and fuel cycle technologies. Many more have mation published prevents anyone from being fully become increasingly motivated to introduce nuclear informed in his or her own field, not to speak of keeping techniques entailing the use of nuclear radiations and up with developments in other fields. Consequently, it isotopes in science and industry. has become necessary to supplement conventionally These developments have put an ever-increasing published information (such as books, journals, and demand on the IAEA to provide a growing number of reports) kept in libraries with condensed information, users with an extensive amount of up-to-date nuclear amenable to computer processing and presented to users data, and the required computer codes for processing in easily accessible and conveniently utilized form. -
Quantum Optics with Gamma Radiation
FEATURES gamma rays of 14.4 keY emitted by the excited 57mFe state (r= 141 ns,I=312), the coherencelength is about 40 m. Forthe 6.2 Quantum optics with keV gammaradiationfrom 181~a ,having alifetime of8.73 flS, the coherence length is 4 km. The appreciable coherence length of these gamma photons allows us to observe the interference gamma radiation between the transition amplitudes from two paths ofthe single , photon, passing through two different samples. In one path the Romain Coussement'·2, Rustem Shahkmoumtov ,3, Gerda Neyens' photon interacts withnuclei ofa reference sample and inthe other and Jos Odeurs1 path it interacts with the nuclei ofa sample under investigation. lInstituut voor Kern- en Stmlingsfysica, Katholieke Universiteit The distance betweenthe samples canbeas large as the coherence Leuven, Celestijnenlaan 200 D, B-3001 Leuven, Belgium length ofthe photon. Interference ofthese two transition ampli 2Optique Nonlineaire Theorique, Universite Libre de Bruxelles, tudes provides spectroscopic CP 231, Bid du Triomphe, B-lOS0 Bruxelles, Belgium information about the hyper- 3Kazan Physico- Technical Institute ofRussian Academy of fine interaction ofthe nuclei in Sciences, 10/7 Sibirsky tmkt, Kazan 420029, Russia the investigated sample, pro vided the hyperfine spectrum Since the discovery of the nuclei in the reference AN one slow down a gamma photon to a group velocity ofa sample is known. Suchinterfer of optical lasers, the Cfew m/s, or can one stop it in a piece ofmaterial only a few ence phenomena have been micron thick and release it? Can one, on command, induce trans explored using synchrotron scientific community parency ofa nuclear resonant absorber for gamma radiation and radiation [5) and are nowadays make a gate? Can one change the index ofrefraction for gamma used as a tool for solid state has been challenged rays in such a way that one could think of optical devices for physics studies. -
Towards a Nuclear Clock with the 229Th Isomeric Transition
Dissertation SUBMITTED TO THE Combined Faculties of the Natural Sciences and Mathematics of the Ruperto-Carola-University of Heidelberg, Germany FOR THE DEGREE OF Doctor of Natural Sciences Put forward by Pavlo V. Bilous Born in: Kherson, Ukraine Oral examination: 13.12.2018 Towards a nuclear clock with the 229Th isomeric transition The first referee: PD Dr. Adriana Pálffy-Buß The second referee: Prof. Dr. Klaus Blaum Zusammenfassung Der Kern 229Th mit seinem Isomerzustand bei 7.8 eV ist ein einzigartiger Kandidat für die erste nukleare optische Uhr mit außerordentlicher Genauigkeit von 10−19. Auf- grund der niedrigen Isomerübergangsenergie ist die Kopplung an die atomare Hülle bei den Prozessen der inneren Konversion (IK) oder Elektronenbrücke (EB) sehr stark. In dieser Arbeit untersuchen wir theoretisch die IK- und EB-Mechanismen und entwerfen neuartige lasergestützte Systeme, die auf (i) eine genauere Bestimmung der Isomerenen- ergie Em und (ii) effiziente Anregung des Isomers abzielen. Einerseits zeigen wir, wie die IK von angeregten elektronischen Zuständen von Th-Ionen zur Bestimmung der Iso- merübergangsenergie verwendet werden kann. Wir schlagen auch einen neuen Ansatz zur Messung der Isomerenergie mit Laserspektroskopie-Genauigkeit mit der laserinduzierten EB in 229Th3+ Ionen vor. Andererseits stellen wir mögliche Isomeranregungsschemata vor, die auf dem EB-Prozess in hochgeladenen Th-Ionen oder auf lasergestützter Ker- nanregung durch Elektroneneinfang des 29.19 keV-Kernzustands direkt über dem Isomer beruhen. Durch die Anwendung von hochgeladenen Ionen wird möglich, die EB optisch mit Hochleistungslasern zu treiben, was laut unserer Ergebnisse zu einer effizienten An- regung führen sollte. Ein solcher Aufbau mit Ionenfallen könnte für die zukünftige Entwicklung der Atomkernuhr relevant werden.