PHYSICS OF PLASMAS 21, 082115 (2014)

Magnetobound and protonium J. R. Correa and C. A. Ordoneza) Department of Physics, University of North Texas, Denton, Texas 76203, USA (Received 3 June 2014; accepted 5 August 2014; published online 27 August 2014) The formation of magnetobound positronium and protonium is investigated via classical trajectory simulations of binary point charge interactions in an external magnetic field. A magnetobound state is a predicted pair- system that is temporarily bound due to the presence of an external mag- netic field. The magnetic field constrains the motion of charged in the direction perpendic- ular to it, while allowing them to move freely in the parallel dimension. At large separations, each particle undergoes helical motion with an adiabatically invariant magnetic moment. As the charges approach each other, the electric interaction breaks the adiabatic constant of the motion, and the particles may temporarily behave as a highly correlated pair. The results of computer simulations of the fully three-dimensional trajectories of classical and non-relativistic point charges with the same mass, equal charge magnitude, and opposite sign are reported. The simulations show the for- mation of magnetobound positronium and protonium. The results yield formation cross sections, which are compared to analytical expressions. Additionally, the results reveal that magnetobound states drift across magnetic field lines. Observations on the drift distance, lifetime, and drift speed of simulated magnetobound states are reported. VC 2014 AIP Publishing LLC. [http://dx.doi.org/10.1063/1.4894107]

I. INTRODUCTION energy are impacted onto a gas covered target or cold surfaces immersed in a magnetic field.3,5 In experiments A magnetobound state is a pair particle- sys- being conducted at CERN that aim at the production and tem of positive energy that is temporarily bound due to the study of cold antihydrogen, the formation of Pn has presence of an external magnetic field. Here, the potential been identified inside strong magnetic fields.6 In addition, energy of the binary charge system is defined as zero when the interaction of positrons or antihydrogen atoms with the the particles are at infinite separation. These systems are trap electrodes may lead to Ps production.7 studied via classical trajectory simulations. The three- Furthermore, the formation of excited states of Ps atoms dimensional numerical trajectory solutions show the forma- inside strong magnetic fields has been identified as a possible tion of magnetobound states. avenue for the production of antihydrogen.8–10 Quasibound states are a similar phenomenon to the mag- Section II describes the equations of motion and meth- netobound states predicted here but concern particles of dis- odology used to carry out numerical studies regarding the parate masses, while magnetobound states concern particles formation of magnetobound states. Section III shows the der- of equal masses. Quasibound states of antihydrogen (or ivation of an analytical expression for the formation cross ) are positive energy systems of a and a nu- section of magnetobound states. Section IV presents the cleus that are temporarily bound due to the presence of a results of the numerical studies and includes comparisons magnetic field.1 Quasibound states may form when positrons with analytical expressions. Also, a brief report is provided and interact in antihydrogen production experi- regarding some patterns in the behavior of magnetobound ments at the European Organization for Nuclear Research states. Section V discusses the possibility of using the forma- (CERN). tion of magnetobound states as an intermediate step in anti- Magnetized positronium (Ps) atoms (negative energy hydrogen synthesis in the laboratory. Finally, some states), magnetized protonium (Pn) atoms, and guiding cen- concluding remarks are provided in Sec. VI. ter drift atoms are two-particle systems that are similar to the magnetobound states described here. A guiding center drift atom is a loosely of a magnetized lepton and a II. CLASSICAL TRAJECTORY SIMULATIONS 2 3 nucleus. A magnetized Ps atom is a loosely bound Consider a charged particle in an external magnetic field and pair in which, similarly to guiding center drift B and in the electric field produced by a point charge Q. 4 atoms, the lepton oscillates axially along a magnetic field Classically, its trajectory is governed by the Lorentz force line about the other particle (due to that particle’s electric potential well) with a frequency that is much larger than the j q Q R^ k q €r u u u Lu u r_ B : (1) lepton’s frequency of azimuthal drift rotation about the other u 2 u u ¼ mu Ru þ mu  particle. Magnetized Ps atoms have been reported when low Unnormalized coordinates, physical constants, and the mag- a) netic field are denoted with the subscript u. m is mass, q Ze Author to whom correspondence should be addressed. Electronic mail: ¼ [email protected] is charge, e is the charge of a positron, Z is a positive or

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negative integer, j is the Coulomb force constant [e.g., r ). Thus, in Cartesian coordinates, the equations of motion 1 À j (4p )À in SI units, where  is the permittivity of free in each of the three orthogonal directions are u ¼ 0 0 space], kL is the Lorentz force constant (e.g., kLu 1 in SI units), R is a vector identifying one particle’s position¼ rela- Xt x00 t 7 ðÞ y0 t B ; (6) tive to the other particle, R^ is the corresponding unit vector, 6ðÞ¼ R3 t À 6ðÞ ðÞ r is a vector identifying a particle’s position from the origin of a coordinate system, and the dots denote derivatives with Yt y600 t 7 ðÞ x60 t B ; (7) respect to the unnormalized time t . A dimensionless form of ðÞ¼ R3 t þ ðÞ u ðÞ Eq. (1) and

quQu R^ qu r00 r0 B; (2) Zt ¼ q2 R2 þ q  z00 t 7 ðÞ: (8) n n 6ðÞ¼ R3 t ðÞ can be obtained, where the dimensionless system of coordi- Here, R t X2 t Y2 t Z2 t ; X t x t x t ; nates and parameters are defined such that þ À Y t yð Þ¼t y tð ,Þþ and Zð(tÞþ) z (ðt)–Þ zð Þ¼(t). ð ÞÀ ð Þ þ pffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiÀ þ À ð Þ¼Theð secondÞÀ ð orderÞ coupled¼ differential equations of v v u : (3) motion, Eqs. (6)–(8), are solved numerically. The solution is ¼ vn cast in parametric form and used to render a three- Here, the normalization factors are signified by the subscript dimensional trajectory for each of the particles. The equa- n, and the primes denote derivatives with respect to the nor- tions of motion have only one parameter, B, which is directly malized time t. The normalization factors are related to the magnetic field strength. Therefore, in order to produce a unique trajectory solution, six initial conditions and one parameter need to be specified. The results are pre- 2m2e3 ju u u sented as they pertain to the interaction of electron-like Bn 3 ; ¼ kLu"hu masses. Nonetheless, the results apply equally well to the "h2 interaction of a and an since Eqs. (6)–(8) r u ; (4) n 2 apply to any system of two particles of equal mass, equal ¼ jumueu rn charge magnitude, and opposite charge sign. tn ; Figure 1 depicts the initial positions of two particles ¼ acu with respect to a Cartesian coordinate system. Let quantities where "h is the reduced Planck constant, a is the fine structure with a subscript 0 refer to values assigned at t 0. Numerous constant, c is the speed of light, and ac j e2="h . The nor- binary trajectory simulations were carried out.¼ Typical initial u ¼ u u u malization factor for charge, qn, equals eu, the unnormalized conditions are charge of the positron. Additionally, the normalization factor for mass, m , is the unnormalized mass of the positron or pro- b n x06 6 ; ton, depending on whether and positrons or ¼ 2 and antiprotons are being considered. Other normalization y06 6rc; ¼ factors can be constructed from the normalization factors al- z0 z0 6 ; ready specified. For instance, the normalization factors for 6 ¼ 2 (9)

speed, acceleration, force, and energy, respectively, are as fol- x06 v 0; lows: v r =t ; a r =t2; F m a , and K F r . ¼ ? n n n n n n n n n n n n y0 0; Here, the SI¼ system of¼ units is employed.¼ All normalization¼ 06 ¼ z0 7v 0: factors are written in terms of four unnormalized quantities: 06 ¼ z mu, eu, ju, and "hu. Thus, the corresponding normalized quanti- Here, v 0 is the initial speed associated with motion perpen- ties are unity, m e j "h 1 and k 1. The corre- ? ¼ ¼ ¼ ¼ L ¼ dicular to the local magnetic field, b is the guiding center sponding normalization factors are m m , q e , j j ; n ¼ u n ¼ u n ¼ u "hn "hu, and kLn 1. ¼Consider a¼ system of two particles where m m ¼ þ m ; Z6 61; B B^z, and ^z is a unit vector parallel to a uniform¼ À magnetic¼ field.¼ The and – signs in the subscript 6 correspond to the positive andþ negative charge, respectively. ^ ^ 2 2 Let R t R t ; R6 t 6R t , and R6 t R t . Then, Eq.ð Þ(2) becomesþð Þ ð Þ¼ ð Þ ð Þ¼ ð Þ FIG. 1. Schematic of initial positions and velocities of a particle and an anti- R^ particle. The magnetic field direction is out of the page, and it is parallel to r600 7 2 r60 B ; (5) the z axis. The circle segments indicate the cyclotron orbit of the correspond- ¼ R À Â ing particle for a particular value of magnetic field strength. The dots indicate the initial positions of the particles in the xy-plane, and the ( ) and ( ) where R t r t r t , and r6 is the normalized vector denote the charge sign of the corresponding particle. The axial positionþ of theÀ ð Þ þð ÞÀ Àð Þ from the origin to the positive or negative particle (i.e., r or particles is z0/2 for the positive particle and z0/2 for the negative particle. þ À

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impact parameter, rc is the cyclotron radius, and z0 is the ini- tial axial separation between the particles. Particles would undergo cyclotron motion near t 0, provided that v 0 0 ¼ ? 6¼ and z0 is sufficiently large. Cyclotron motion is the gyration that charged particles experience in a magnetic field. The axis of the cyclotron motion of a particle is referred to as the guiding center of that particle. The initial phase of cyclotron motion is implicitly defined by the choice of x06 and y06. The initial phase of the particles was uniformly sampled in two of the three compu- tational studies reported here. The initial conditions are chosen such that the guiding center of each particle is on the xz-plane. The guiding cen- ter motion of a particle is the motion that is obtained when averaging over the cyclotron period. Guiding center theory hinges on the assumption that the magnetic moment associ- ated with each particle’s cyclotron motion is an adiabatic constant. The guiding center impact parameter b is the per- pendicular (to the direction of the magnetic field z^) distance between the initial guiding centers of the charges. Hereafter, the term “impact parameter” is used in place of FIG. 2. Example of a magnetobound state. The lines represent the trajecto- “guiding center impact parameter” for brevity. The initial ries of a particle and an antiparticle in a magnetic field, with the positive par- ticle approaching from the positive z-direction and the negative particle cyclotron radius is rc v 0/xc,wherexc kLqB/m and approaching from the negative -direction. Here, coordinates are normalized ¼ ? ¼ z q q6 . according to Eq. (3). ¼ Forj j large enough values of the initial axial separation, the results of the simulation studies are independent of z0. Figure 2 shows a sample solution that resulted in a mag- The initial conditions, Eq. (9),chosenareconsistentwith netobound state. The equations of motion are solved numeri- that expectation. The simulation begins when the particles cally for 0 t s. The numerical differential equation solver are far enough from each other to ensure that they undergo utilized to solve the equations of motion progressively guiding center motion. For very large separations, the elec- reduces the step size until it is able to track the solution well tric potential between the particles is very small due to its over the entire region.11 A magnetobound state is defined to inverse dependence on R.Thesimulatedmotionbegins have been formed when both particles reverse the sign of when K0 (1 )K ,where 1 is a chosen constant, their axial velocity component two or more times. An 2¼ þ 12  K0 mv0; K mv , K denotes the kinetic energy of the unmagnetized particle will experience such sign changes at ¼ 1 ¼ 1 two-particle system, the subscript refers to quantities most once. For a magnetobound state, that number can be 1 when the particles are an infinite distance apart, and the much higher. This is illustrated in Fig. 3, which shows the subscript zero denotes initial time, t 0 (i.e., at the begin- axial position versus time for a sample solution. ¼ ning of the simulation). Energy conservation requires that Three numerical studies were carried out to investigate U0 K0 K ,whereU denotes the potential energy of the the formation of magnetobound states. Each study consists of þ ¼ 1 guiding centers. Solving the energy conservation equation seven series of simulations. Each series of simulations con- 2 with U0 jq /R0 gives sists of numerous trajectory solutions to the equations of ¼À

2 4 j q 2 z0 b : (10) ¼ sffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi2m2v4 À 1 In deriving Eq. (10), the distance between the particles is approximated using the separation between their guiding centers. This is no more consequential than choosing a slightly different . For the simulations,  1/100 was cho- sen. Additionally, it was required that b ¼r .  1 ensures  c  that U0 K0. This, along with the range of values of b chosen,j j ensures that z b. For all trajectory solutions, 0  FIG. 3. Plot of the normalized axial positions with respect to normalized it was verified that v s=5 v t 0 =v t 0 time for two particles that form a magnetobound state. The normalization ½ ?ð ÞÀ ?ð ¼ ÞŠ ?ð ¼ Þ Շ 1=10 000. Here, s is the simulation duration. s 2s0 is convention is the same as that of Fig. 2. Each line represents the trajectory ¼ of one of the particles, with the positive particle approaching from the posi- chosen, where s0 z0/vz0 is twice the time that the particles would require to¼ reach zero axial separation if they did not tive z-direction and the negative particle approaching from the negative z- direction. Initially, the guiding centers of the particles lie on the xz-plane. interact with one another and vz0 is the axial speed of each Each time the trajectories cross the horizontal axis, the particles are at particle at the beginning of the simulation. approximately zero axial separation.

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motion for two of opposite charge, equal charge mag- tmbs l=g ; (14) nitude, and the same mass in an external magnetic field. Each ¼ k series of simulations differs from the other series only by the where g is the relative speed between the guiding centers of k strength of the magnetic field. Each simulation within a series the particles (which is assumed to be parallel to the magnetic is identical to the other simulations in its series except for the field due to the strength of the magnetic field). Equation (14) initial impact parameter. b is increased in multiples of rc from is used in Sec. IV B for a comparison of timescales. twice the cyclotron radius to bmax, which is chosen to be a length beyond which magnetobound states are not expected. B. Formation impact parameter The initial conditions of the simulations impart equal ki- The adiabatic invariance of the magnetic moments of netic energy to each particle. The first two studies also charged particles in a constant magnetic field can be broken impart equal speeds in each of the three orthogonal dimen- as the charges approach each other. Guiding center motion sions for each particle. In contrast, the third study assigns ceases, and the particles behave as a correlated system. most of the initial kinetic energy of each particle to that par- Otherwise, the particles reflect or pass by one another axi- ticle’s axial velocity component. ally, resuming guiding center motion at sufficient separation. The parameters and initial conditions for the first compu- The formation impact parameter of magnetobound tational study are as follows: 1 T Bu 7 T; 2rc b bmax,     states, rmbs, is hypothesized to be approximately equal to the in increments of rc; vz0 v0=p3; v 0 v0 2=3; v0 v ¼ ? ¼ ¼ 1 distance between the particles at zero axial separation at 1  ; and v kBT=m, where kB is the Boltzmann 1 ffiffiffi pffiffiffiffiffiffiffiffi which the magnitude of the electric force on each charge constantð þ Þ and T 5¼ K. The second study considers T 15 K. pffiffiffiffiffiffiffiffiffiffiffiffiffiffi u ¼ pffiffiffiffiffiffiffiffiffiffiffiffiffiffi u ¼ equals the maximum magnitude of the magnetic force on ei- The third study considers particles with Tu 15 K and near- ther particle. This would guarantee the breaking of the invar- zero speed perpendicular to the magnetic field.¼ In all other iance of the magnetic moment. With the assumption rmbs aspects, the third study is the same as the second study. 2 2  rc, the condition is expressed as kLqv ;bB jq =rmbs or ?  III. ANALYTICAL FORMATION CROSS SECTION jq rmbs : (15)  kLBv ;b A. Formation cross section, mean free path, rffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi? and formation timescale Here, v ,b is the perpendicular speed of either particle at the ? Consider a particle and its antiparticle interacting in a point of zero axial separation (i.e., when the position vector strong magnetic field. Here, the particles are treated as non- from one charge to the other is perpendicular to the magnetic field). If different values of are obtained depending on relativistic classical point charges with rc b, and the mag- rmbs netic field is assumed to be uniform and extend over all which particle is considered, the value that yields the largest should be chosen. Particles of equal charge magnitude space. Let rmbs be a formation impact parameter such that rmbs are being considered. Additionally, the guiding center impact b rmbs leads to a magnetobound state being formed  parameter of the particles is assumed to remain unaffected (expressions for rmbs will be derived in the following subsec- tion). A formation cross section of the form during the portion of the trajectories prior to the breaking of the magnetic moment invariance. If the breaking of the mag- 2 rmbs prmbs (11) netic moment invariance does not take place at approxi- ¼ mately zero axial separation (i.e., R b in the guiding center is constructed. approximation), then it is assumed¼ to not occur at larger Consider the interaction of a test particle and a mono- impact parameters since the particles experience the largest energetic collection of its corresponding anti-particles (field electric field at approximately zero axial separation. particles) uniformly distributed over space interacting in a The kinetic and potential energies of the particles will be strong magnetic field. The field particles are assumed to be considered using a coordinate system whose origin coincides uncorrelated and do not interact among themselves or drift with the center of mass of the system when the particles are relative to each other. Given a formation cross section of the an infinite distance apart, before they interact. (However, the form of Eq. (11), the probability that a magnetobound state present work does not utilize the center of mass equations or will form during a sufficiently small time period Dt is the reduction of a two particle system to a single reduced mass and a center of force.) The total energy of the system P nr Ds: (12) mbs ¼ mbs equals the instantaneous kinetic energy of the particles 2 2 2 at infinity, K 1=2 m1v1; 1=2 m2v2; 1=2 lg , Here, Ds is the distance travelled by the test particle’s guid- 1 ¼ð Þ 1 þð Þ 1 ¼ð Þ 1 ing center relative to the guiding centers of the field particles where l m1m2/(m1 m2). Here, g denotes the relative speed between¼ the particlesþ at infinity, and denote the masses during a time Dt, and n is the field particle density. The m1 m2 mean free path for the formation of a magnetobound state is of particle 1 and particle 2, respectively. If the particles have arrived at by setting the probability in Eq. (12) equal to one, different masses, the subscript 2 denotes the particle with the largest mass. The particles are first considered to have dispar- 1 ate masses to illustrate the connection between the theory l nrmbs À (13) ¼ð Þ being presented and prior theory. (i.e., Ds l when Pmbs 1). Once l is known, the formation When the invariance of the magnetic moment of a parti- timescale¼ can be obtained¼ as cle is broken, the perpendicular speed of one or both

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2 2 particles can change drastically. However, energy conserva- Considering disparate masses and g 2jq = m1rmbs tion limits the speeds of the particles such that in Eq. (18) leads to 1  ð Þ

2 1 2 1 2 jq jq m1v1 m2v2 K ; (16) rmbs5 : (20) 2 þ 2 À R ¼ 1 ¼ kLg B rffiffiffiffiffiffiffiffiffiffiffiffiffiffi1 where v1 and v2 are the speeds of particle 1 and particle 2, In Ref. 12, Eq. (20) was obtained for describing the forma- respectively. Thus, the maximum speed possible is the limit tion of quasibound states of antihydrogen by comparison of 2 in which the energy K jq /R is assigned to the lightest of maximum forces, but neglecting the change in potential 1 þ the two masses at R b, where the electric force is at its energy. ¼ maximum. In this limit, the magnetic force is at its maximum For equal masses, m m m, l m/2, and Eq. (16) 1 ¼ 2 ¼ ¼ if, additionally, v1,b v 1,b (i.e., the total speed of particle 1 becomes v2 v2 2 2 1 4 2 . The maxi- ? m 1 2 = jq =R = mg ¼ ð þ Þ À ¼ð Þ 1 at a separation b from particle 2, v1,b, equals its perpendicular mum speed for any particle in the binary system considered speed at that same separation, v 1,b). Thus, with m2 m1, here must be equal-to-or-smaller-than the speed obtained ?  l m1, the speed to utilize for the hypothesized condition when the kinetic energy of one of the particles is zero (e.g.,  for the formation impact parameter of magnetobound states 2 v2 0). Similarly to Eqs. (17) and (18), one obtains v ;b is 2 ¼ 2jq2 ? ’ g =2 mb and 1 þ 2 2 2 2jq v ;b g : (17) q2 g2 2 q2 ? ’ 1 þ m1b j j 2 kLqB 1 : (21) rmbs ¼ sffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi2 þ mrmbs Using Eq. (17) in Eq. (15), one obtains the following expres- sion for the formation impact parameter of magnetobound Equations (18) and (21) are quartic functions. They can 4 3 states, rmbs1, be cast in the form rmbs rmbs 0. Here, ; , and are real coefficientsA whichþ B guaranteesþ E ¼ real solutions.A B The 2 2 exactE solutions can be found, of which the positive real solu- jq 2 2jq 2 kLqB g : (18) 2 r ¼ 1 þ m1rmbs1 tion must be chosen. For Eq. (21), 1; 4jq = mbs1 sffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi 2 2 2 2 2 2 A ¼ B ¼ mg ; 2j q = kLB g . Thus, ð 1Þ E ¼À ð 1Þ Hereafter, rmbsN symbols with N being an even number refer to equal masses, while an odd subscript refers to cases of 3 N 1 2 2 2 disparate masses. Thus, the N subscript is used to differenti- rmbs d B 2 d ; ¼ 4 0ÀB À B þ þ sffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi2 d þ B À 1 ate different expressions for the magnetobound state forma- pffiffiffiffiffiffiffiffiffiffiffiffiffiffi B þ tion impact parameter, which differ due to the different @ pffiffiffiffiffiffiffiffiffiffiffiffiffiffi A(22)

limiting cases being considered. 13=3 1=3 1 5=3 2=3 2 where d 2 3À cÀ 2 3À c and c 9 Equation (18) has two interesting limiting cases, that for 4 ¼2 3 1=E3 þ ¼ð B E 2 2 81 768 . Equation (22) will be evaluated which g 2jq = m1r and the reverse. That is, these mbs þand comparedB E À to theE Þ simulation results that will be discussed cases represent1  the extremesð Þ of how the initial kinetic energy pffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi of the particles in the center of mass frame at infinity, in Sec. IV. 2 Equation (21) also has two limiting cases. Considering 1=2 lg , compares to the magnitude of the potential 2 2 ð Þ 1 the limit in which g =2 2jq = mrmbs leads to energy of the particles at the distance of closest approach, 1  ð Þ jq2/r . The first of these choices leads to mbs jm 1=3 1=3 1=3 rmbs2 2 2 : (23) jm1 jm1 ¼ 2kLB rmbs3 : (19)  ¼ 2k2B2  k2B2 L L 2 2  The limit g =2 2jq = mrmbs in Eq. (21) leads to 1  ð Þ The scale length given by Eq. (19) has been obtained in Ref. 2 in association with guiding center drift atoms. Such 1 jq rmbs4 24 ; (24) atoms satisfy the condition that the cyclotron frequency is ¼ kLg B much greater than the axial bounce frequency, which in turn rffiffiffiffiffiffiffiffiffiffiffiffiffiffi1 is much greater than the E B drift rotation frequency.2 which, neglecting a factor of p4 2 1:19, is the same as This condition leads to the scale length given by Eq. (19),2 Eq. (20).  which has been used with a different multiplicative factor in The theory presented here, whenffiffiffi applied to disparate experimental reports pertaining magnetized Ps atoms.3 A masses and certain limiting cases, has produced Eqs. (19) timescale analysis leads to Eq. (19) in Ref. 1, which regards and (20), which have been previously found to apply to guid- quasibound states of antihydrogen. It is interesting that Eq. ing center drift atoms and/or quasibound states. When the (19) can be derived from different physical considerations: same theory has been applied to the case of a charged parti- the comparison of maximum electric and magnetic forces cle and its antiparticle, Eqs. (22), (23), and (24) have experienced by the particles, or an analysis of timescales. resulted. Equations (23) and (24) are more easily used than Another interesting aspect of Eq. (19) is that it is independ- Eq. (22). These equations apply to magnetobound states, ent of speed. which have not been previously predicted or empirically

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zero and 2p in increments of p/4. The phase seemed to affect the formation of magnetobound states insofar as it may change the phase of each particle as they approach zero axial separation. Thus, the initial phase can change the particles’ distance of closest approach by up to 4rc. The average and maximum error percentages between the data represented by the seven solid squares in Fig. 4 and Eqs. (22), (23), and (24) are summarized in Table I. The percent error is calculated as Numerical Prediction Error j NumericalÀ j 100%, where Numerical repre- sents¼ the values observed in the numerical study and Prediction represents the values given by the corresponding analytical expression. Using a multiplicative fitting factor i (i.e., f1 if0), all analytical predictions for the magneto- FIG. 4. Plot of the results of the numerical study regarding the formation bound state¼ formation cross section agreed to within 10% impact parameter of magnetobound states considering Tu 5 K. The vertical axis represents the normalized impact parameter and the horizontal¼ axis rep- with the numerical results. In the figures and in the equa- resents the magnetic field strength in SI units. The normalization convention tions, the fitting parameter is i 1 while the error tables use is the same as that of Fig. 2. The squares are the initial impact parameter a variety of values. A simple¼ multiplicative factor is used below which at least 84% of trajectories resulted in magnetobound states. with the analytical predictions because the electric-to-mag- The dots are the impact parameter above which no magnetobound trajecto- ries were observed. The dotted line is the prediction from Eq. (22). The solid netic-force ratio at which the electric force between the line is the prediction from Eq. (23). The dotted-dashed line is the prediction charges breaks the adiabatic invariance of the magnetic from Eq. (24). No fitting parameter was used. moment of either particle (due to the external magnetic field) is not precisely known, and the breaking of this invariance shown to our knowledge. In the following section, Eqs. (22), forms the basis for the analytical predictions presented here. (23), and (24) are compared to numerical simulations. A second numerical study was performed using a differ- ent value for the initial speeds of the particles, but otherwise the same as the first. The initial speeds of the particles were IV. NUMERICAL RESULTS chosen to correspond to T 15 K. All other parameters u ¼ A. Formation impact parameter remained unchanged. The results of this study are presented in Fig. 5, which is similar to Fig. 4 in its labeling conven- The first numerical study consisted of 360 classical tra- tions. In a similar fashion to Table I, the average and maxi- jectory simulations of binary point charge interactions in an mum error percentages between Eqs. (22), (23), and (24) and external magnetic field. The results of this numerical study the data represented by the seven solid squares in Fig. 5 are regarding the formation impact parameter are summarized in summarized in Table II. Fig. 4, where the horizontal axis represents magnetic field Thus far, the computational studies assumed that the ini- strength, and the vertical axis represents the initial impact tial kinetic energy of the particles was equally divided parameter. The dotted line is the prediction from Eq. (22). between the orthogonal components of the motion when The solid line is the prediction from Eq. (23). The dotted- averaged over the initial cyclotron period. A final study was dashed line is the prediction from Eq. (24). The solid dots conducted in which the perpendicular component of the ini- and squares represent the numerical results for the formation tial speed of each particle corresponded to 1/11th of the total impact parameter of magnetobound states. The solid squares initial speed, and the rest was allocated to the axial compo- mark the initial impact parameter below which at least 84% nent of the motion. In all other aspects, the third study was of trajectories resulted in magnetobound states, while the identical to the second numerical study, with one exception: solid dots mark the impact parameter above which no mag- the initial phase of the particles was not varied. The netobound trajectories were observed. (This is similar to the antihydrogen quasibound states studied in Ref. 1, where most but not all trajectories below a certain threshold-impact parameter were found to result in quasibound states.) The initial phase of the particles was only varied for the trajecto- ries that lie in the region between the squares and the dots. There, the initial phase of one particle was varied between

TABLE I. Formation impact parameter percent errors from the numerical study considering T 5 K. The data chosen for the comparisons are that u ¼ which is represented by the solid squares in Fig. 4.

Formation Cross Section Avg. (%) Max. (%) i Avg. (%) Max. (%)

Eq. (22) 74.4 76.4 3.82 5.9 8.4 Eq. (23) 73.9 76.0 3.83 6.5 9.2 Eq. (24) 31.6 39.6 1.49 5.1 10.1 FIG. 5. Same as Fig. 4, except T 15 K. u ¼

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TABLE II. Formation impact parameter percent errors from the numerical TABLE III. Formation impact parameter percent errors from the numerical

study considering Tu 15 K. The data chosen for the comparisons are that study considering Tu 15 K and vz0 v 0. The data chosen for the compar- which is represented by¼ the solid squares in Fig. 5. isons are that which is¼ represented by the? solid squares in Fig. 6.

Formation cross section Avg. (%) Max. (%) i Avg. (%) Max. (%) Formation cross section Avg. (%) Max. (%) i Avg. (%) Max. (%)

Eq. (22) 69.0 71.2 3.07 8.4 11.9 Eq. (22) 65.5 69.1 2.87 7.2 11.3 Eq. (23) 68.4 70.9 2.98 9.7 13.4 Eq. (23) 65.7 68.7 2.79 8.2 12.8 Eq. (24) 37.2 41.7 1.57 5.1 8.5 Eq. (24) 32.0 34.4 1.46 2.7 4.2

increments of the impact parameter were very small for the Tu 5 K study were analyzed. Limitations of the numerical third study. The initial impact parameter was increased in root¼ solver employed required the lifetimes of magneto- multiples of the initial cyclotron radius, which is very small bound states to also be checked by eye. Consequently, the due to the low initial perpendicular speeds of the particles. number of magnetobound trajectories analyzed for these fea- The results of the third study, which pertains to particles tures is small, and the sample is not regarded as statistically with a small ratio of perpendicular to parallel initial speeds, significant. The simulated data to be discussed in this section (v 0/v0 1/11), are presented in Fig. 6. This figure retains are shown in Figs. 7–9 and were obtained from analyzing 98 the? labeling¼ conventions of Figs. 4 and 5. Table III lists the trajectory simulations that resulted in magnetobound states. average and maximum error percentages between the data Of these, 10 trajectories were analyzed for the data points represented by the seven solid squares in Fig. 6 and Eqs. associated with Bu 1 T, 16 trajectories for Bu 2 T, 11 for (22)–(24). Here, the data points below which 84% are only ¼ ¼ shown because they were very close to the data points above which no magnetobound states were observed. An observa- tion that is not shown in Fig. 6 or Table III (that is, for the study pertaining Tu 15 K and vz0 v 0) is that magneto- bound states did not¼ form if the initial impact? parameter was below 7rc. Each of these cases resulted in a p-radian reflec- tion of the particles. A similar observation was made for 12% of the cases with impact parameters below 7rc in the study pertaining Tu 15 K. For the study pertaining T 5 K, magnetobound¼ states were consistently observed u ¼ for small impact parameters as small as b 2rc (the lower limit of the range). ¼

B. Lifetime, drift, and drift speed

FIG. 7. Plot of the ratio smbs/sc versus the strength of the magnetic field as All magnetobound states observed in the simulations observed in the Tu 5 K computational study. Here, smbs is the average life- drifted across the magnetic field. The drift, drift speed, and time of the magnetobound¼ states and it is defined as the time between the lifetime of a subset of the magnetobound trajectories of the first and last time that the charges of a magnetobound state pass each other axially. sc is the initial cyclotron period, which is itself a function of the magnetic field strength.

FIG. 6. Plot of the results of the numerical study pertaining to particles ini- tially with vz0 v 0. The vertical axis represents the normalized impact pa- rameter and the horizontal? axis represents the magnetic field strength in SI FIG. 8. Plot of the average drift speed (perpendicular to the magnetic field) units. The normalization convention is the same as that of Fig. 2. The of magnetobound states as a fraction of the total initial speed of each particle squares are the initial impact parameter below which at least 84% of trajec- versus magnetic field strength in SI units as observed in the Tu 5 K compu- tories resulted in magnetobound states. The dotted line is the prediction tational study. The dots represent the average drift speed of¼ the magneto- from Eq. (22). The solid line is the prediction from Eq. (23). The dotted- bound states that formed at that particular value of the magnetic field dashed line is the prediction from Eq. (24). No fitting parameter was used. strength.

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V. ANTIHYDROGEN SYNTHESIS

Magnetobound states may be useful as an intermediate step in the production of neutral antimatter. Two scenarios will be very briefly speculated in this section. In antihydrogen experiments being conducted at CERN, a nested Penning trap is used to confine antiprotons and posi- trons. In a nested Penning trap, radial confinement is pro- vided by a magnetic field, and an electric field produced by biased cylindrical electrodes provides the axial confinement of the particles. A nested Penning trap uses five or more elec- trodes to produce nested electric wells of opposite sign. Therefore, charges of opposite sign can be stored in different FIG. 9. Plot of the average drift perpendicular to the magnetic field of a sections of the trap. In order to achieve overlap between magnetobound state as a function of the magnetic field strength as observed charges of opposite sign, the energy of one of the species is in the Tu 5 K computational study. The dots represent the average drift of the magnetobound¼ states that formed at that particular value of the magnetic increased such that the particles gain enough kinetic energy field strength. to overcome the potential barrier separating them from the other species. Antihydrogen may be produced primarily via B 3 T, 13 for B 4 T, 12 for B 5 T, 12 for B 6 T, three-body recombination. However, the antihydrogen that is u ¼ u ¼ u ¼ u ¼ and 24 trajectories were analyzed for the Bu 7 T data produced is energetic due to the process that is used to points. For each value of magnetic field strength,¼ the values achieve overlap. This makes these antihydrogen atoms diffi- of b were chosen to approximately uniformly cover the range cult to confine given the limited magnetic field well depth between b 2rc and the points marked by the solid squares available to confine neutral atoms via their magnetic dipoles. in Fig. 4. ¼ Consider a nested Penning trap, with antiprotons in the Figure 7 shows the ratio of smbs/sc, where sc is the initial inner well and positrons in the outer wells. Allow the two cyclotron period. The lifetime of a magnetobound state, smbs, species to remain at low temperatures and in their respective was defined as the time between the first and last time that wells. Introduce an electron beam traveling axially through the particles of a magnetobound state reverse their axial the trap. As the electron beam encounters the positrons of motion. The average smbs/sc was calculated to be approxi- the well closest to the origin of the beam, magnetobound Ps 3 mately 3.3 10 . The average smbs was calculated to be may be produced. Magnetobound Ps may overcome the elec- between 346Â (for B 1 T) and 6000 (for B 7 T) times tric potential separating the positrons from the antiprotons. u ¼ u ¼ larger than sc. The average smbs was calculated to be about This is because magnetobound states are neutral systems. three orders of magnitude smaller than tmbs, the magneto- The magnetobound Ps would then travel axially, due the mo- bound state formation time as given by Eq. (14) considering mentum provided by the beam’s particle (and radially due to 12 3 n 10 mÀ . the drift discussed in the previous section), and interact with ¼ The drift of a magnetobound state across magnetic field the species in the inner well. Thus, cold antihydrogen may lines in a direction perpendicular to the plane of the initial be produced via three-body recombination between magne- guiding centers can be seen in Fig. 2. As a system, magneto- tobound Ps and the antiprotons of the inner well. bound states are neutral. Every magnetobound state observed The radial drift observed in the simulations may be det- in the simulations displayed said drift. The direction of the rimental to the scenario discussed thus far. However, it may magnetobound state drift seemed to be determined by the ini- be useful for antihydrogen synthesis in a modified scheme. tial conditions. That is, if the direction of the magnetic field Consider a hollow antiproton plasma confined in a Penning defines the positive z axis and the plane of the initial guiding trap, as well as an electron plasma confined in the volume centers defines the xz-plane, then whether the particles within the inner radius of the antiproton plasma. If positrons drifted in the positive or negative y-direction depended only are sent to stream through the electron plasma, magneto- upon whether the positive charge approached the yz-plane bound Ps may form. As the magnetobound Ps drifts axially from the positive or negative z-direction (and the negative and radially, it may undergo three-body recombination charge thus approached the mid-plane from the complemen- within the antiproton plasma and result in the production of tary direction). These statements regarding the direction of cold antihydrogen atoms. said drift are an observation that held true for every magne- These schemes for achieving antihydrogen synthesis via tobound state seen in the simulations, and they were checked magnetobound states utilize the ability of magnetobound by reversing the initial conditions of about twenty trajectory states to drift across magnetic fields and possibly electric simulations that led to magnetobound states. fields. In antihydrogen experiments such as those conducted Figure 8 shows the average drift speed observed in the at CERN, this may represent a practical way to overcome the simulations for each value of Bu, while Fig. 9 shows the total difficulties related to matching the kinetic energy of the spe- drift. The speed of the drift of magnetobound states across cies in the outer wells to the values necessary to overcome magnetic field lines is a large fraction of the initial speed of the electric potential of the inner well without reaching lev- the particles. This drift may be detrimental to the radial con- els that prevent the production of cold antihydrogen. Thus, finement of the charges that form a magnetobound state. further studies of these aspects of magnetobound states are

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desirable. Additionally, further studies regarding the forma- Prior to the formation of a magnetobound state, and after tion of magnetobound and quasibound states at larger ener- its disassociation, the center of mass of the two particle system gies ( 50 K) may be useful, as these states may have already experiences zero net displacement in the guiding center been formed in experiments working near those energy lev- approximation. However, during the lifetime of a magneto- els. It is of interest to note that, under certain conditions, the bound state, the simulations showed that the center of mass scenarios discussed may also work if the particles are acquires a drift velocity that is perpendicular to the magnetic exchanged for their oppositely signed counterparts. In such a field. case, magnetobound Pn would be produced instead of mag- In summary, the formation of temporarily bound sys- netobound Ps. tems of positive energy formed by a charged particle and its antiparticle have been studied via full trajectory simulation of point charges in a strong magnetic field. Several analytical VI. CONCLUDING REMARKS expressions for the formation impact parameter of magneto- The interaction of a charged particle and its antiparticle bound states were proposed and found to be in good agree- in a strong magnetic field has been investigated. As a ment with the numerical results over the range of conditions charged particle and its antiparticle approach one another, considered. In addition, the observation of cross-field drift the electric field does work on the particles. This results in distance, lifetime, and drift speed of the magnetobound states an increased kinetic energy and changes in each particle’s formed in the simulations was reported. Finally, possible pitch angle. The adiabatic invariance of the magnetic avenues for the use of magnetobound states as an intermedi- moment may be broken as the electric force between the ate step in antihydrogen synthesis were described. charges approaches or overcomes the magnetic force due to the external field. The particles may then behave as a tempo- ACKNOWLEDGMENTS rarily bound system. The authors thank Dr. Francis Robicheaux for his Three numerical studies of the interactions of a particle valuable input and Aimee Ayton for helpful discussions. This and an antiparticle of the same mass under a strong magnetic material is based upon work supported by the Department of field have been conducted. The formation of temporarily Energy under Grant No. DE-FG02-06ER54883 and by the bound states of positive energy, called magnetobound states, National Science Foundation under Grant No. PHY-1202428. was revealed. Several analytical expressions for the forma- tion cross section of magnetobound states were developed 1C. E. Correa, J. R. Correa, and C. A. Ordonez, Phys. Rev. E 72, 046406 and compared to numerical results. In one of its limiting (2005). cases and considering disparate masses, the theory presented 2S. G. Kuzmin, T. M. O’Neil, and M. E. Glinsky, Phys. Plasmas 11, 2382 (2004). here gave rise to a scale length that has been associated with 3 2 D. P. van der Werf, C. J. Baker, D. C. S. Beddows, P. R. Watkeys, C. A. guiding center drift atoms in other work. In another limiting Isaac, S. J. Kerrigan, M. Charlton, and H. H. Telle, in XV International case and also considering disparate masses, the formation Workshop on Low Energy Positron and Positronium Physics [J. Phys.: impact parameter that has been associated with quasibound Conf. Ser. 199, 012005 (2010)]. 4 states of antihydrogen was found.1 M. E. Glinsky and T. M. O’Neil, Phys. Fluids B 3, 1279 (1991). 5C. J. Baker, D. P. van der Werf, D. C. S. Beddows, P. R. Watkeys, C. A. Magnetobound states may have important implica- Isaac, S. J. Kerrigan, M. Charlton, and H. H. Telle, J. Phys. B: At. Mol. tions. For instance, the formation of magnetobound states Opt. Phys. 41, 245003 (2008). increases the time that two particles remain close together, 6L. Venturelli, M. Amoretti, C. Amsler, G. Bonomi, C. Carraro, C. L. which may allow participation in three body recombination Cesar, M. Charlton, M. Doser, A. Fontana, R. Funakoshi, P. Genova, R. S. Hayano, L. V. Jørgensen, A. Kellerbauer, V. Lagomarsino, R. Landua, E. of said particles. In three body recombination, the two par- Lodi Rizzini, M. Macrı, N. Madsen, G. Manuzio, D. Mitchard, P. ticles that are near each other would experience a collision Montagna, L. G. Posada, H. Pruys, C. Regenfus, A. Rotondi, G. Testera, with a third particle, and one of the particles may take suf- D. P. Van der Werf, A. Variola,Y. Yamazaki, and N. Zurlo (ATHENA Collaboration), Nucl. Instrum. Methods Phys. Res. B 261, 40 (2007). ficient energy away to result in the formation of an atom. 7M. Amoretti, C. Amsler, G. Bazzano, G. Bonomi, A. Bouchta, P. Bowe, A magnetobound state is a neutral system. As would be C. Carraro, C. L. Cesar, M. Charlton, M. Doser, V. Filippini, A. Fontana, consistent with that expectation, the study revealed that M. C. Fujiwara, R. Funakoshi, P. Genova, J. S. Hangst, R. S. Hayano, L. magnetobound states drift across magnetic field lines. V. Jørgensen, V. Lagomarsino, R. Landua, D. Lindel€of, E. Lodi Rizzini, M. Macri, N. Madsen, G. Manuzio, M. Marchesotti, P. Montagna, H. Observations on the drift distance, lifetime, and drift speed Pruys, C. Regenfus, P. Riedler, A. Rotondi, G. Rouleau, G. Testera, A. of the magnetobound states formed in one of the computa- Variola, and D. P. van der Werf, Phys. Lett. B 578, 23 (2004). tional studies were reported. The formation of magneto- 8B. I. Deutch, M. Charlton, M. H. Holzscheiter, P. Hvelplund, L. V. bound states may thus reduce the confinement times of Jørgensen, H. Knudsen, G. Laricchia, J. P. Merrison, and M. R. Poulsen, Hyp. Int. 76, 151 (1993). plasmas where pair particles interact. However, magneto- 9M. Charlton, Phys. Lett. A. 143, 143 (1990). bound states may be useful as an intermediate step in the 10E. A. Hessels, D. M. Homan, and M. J. Cavagnero, Phys. Rev. A 57, 1668 production of antihydrogen. Two possible scenarios were (1998). 11 briefly discussed that may open opportunities for the pro- Wolfram Research, Inc., “Numerical Solution of Differential Equations” Mathematica, Version 8.0, Champaign, IL, 2010. duction of neutral antimatter at lower temperatures than 12C. E. Correa, S. A. Khan, J. R. Correa, and C. A. Ordonez, Nucl. Instrum. currently achieved. Methods Phys. Res. B 241, 165 (2005).

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