molecules Review Shape-Memory Polymeric Artificial Muscles: Mechanisms, Applications and Challenges 1, 1, 1, , 1 2 2 Yujie Chen y , Chi Chen y, Hafeez Ur Rehman * y, Xu Zheng , Hua Li , Hezhou Liu and Mikael S. Hedenqvist 3,* 1 State Key Laboratory of Metal Matrix Composites, School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China;
[email protected] (Y.C.);
[email protected] (C.C.);
[email protected] (X.Z.) 2 Collaborative Innovation Centre for Advanced Ship and Dee-Sea Exploration, Shanghai Jiao Tong University, Shanghai 200240, China;
[email protected] (H.L.);
[email protected] (H.L.) 3 Department of Fibre and Polymer Technology, School of Engineering Sciences in Chemistry, Biotechnology and Health, KTH Royal Institute of Technology, SE-100 44 Stockholm, Sweden * Correspondence:
[email protected] (H.U.R.);
[email protected] (M.S.H.) These authors contributed equally to this work. y Academic Editor: Laura Peponi Received: 7 July 2020; Accepted: 3 September 2020; Published: 16 September 2020 Abstract: Shape-memory materials are smart materials that can remember an original shape and return to their unique state from a deformed secondary shape in the presence of an appropriate stimulus. This property allows these materials to be used as shape-memory artificial muscles, which form a subclass of artificial muscles. The shape-memory artificial muscles are fabricated from shape-memory polymers (SMPs) by twist insertion, shape fixation via Tm or Tg, or by liquid crystal elastomers (LCEs). The prepared SMP artificial muscles can be used in a wide range of applications, from biomimetic and soft robotics to actuators, because they can be operated without sophisticated linkage design and can achieve complex final shapes.