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Anomalous Density of States of a Luttinger Liquid in Contact with A

Anomalous Density of States of a Luttinger Liquid in Contact with A

Anomalous of a Luttinger in contact

with a sup erconductor

1 2 3 1;4

C. Winkelholz , Rosario Fazio , F.W.J. Hekking , and Gerd Schon

1

Institut fur  Theoretische Festkorperphysik, Universtitat Karlsruhe, 76128 Karlsruhe, Germany

2

Istituto di Fisica, Universit a di Catania, viale A. Doria 6, 95129 Catania, Italy

3

Cavendish Laboratory, University of Cambridge, Madingley Road, Cambridge CB3 0HE, UK

4

Department of Technical Physics, Helsinki University of Technology, 02150 Espoo, Finland

Abstract

We study the frequency and space dep endence of the lo cal tunneling density

of states of a Luttinger liquid LL which is connected to a sup erconduc-

tor. This coupling strongly mo di es the single-particle prop erties of the LL.

It signi cantly enhances the density of states near the Fermi level, whereas

this quantityvanishes as a p ower law for an isolated LL. The enhancement

is due to the interplaybetween -electron interactions and multiple

back-scattering pro cesses of low-energy at the interface b etween the

LL and the sup erconductor. This anomalous b ehavior extends over large dis-

tances from the interface and may b e detected by coupling normal prob es to

the system.

Typ eset using REVT X

E 1

Transp ort in low-dimensional structures is strongly in uenced by electron-electron in-

teractions. A paradigm mo del to describ e interactions in one-dimensional systems is the

Luttinger liquid LL. The low-lying excitations of the electron system consist of charge and

waves, rather than [1,2]. As a consequence, the presence of a barrier

in the liquid leads to p erfectly re ecting for repulsiveinteractions or transmitting for

attractiveinteractions b ehavior at low energies [3].

One of the most striking characteristic prop erties of Luttinger is the b ehavior of

the density of states DOS close to the Fermi energy. Contrary to Fermi liquids, whose

residue is nite, LLs have a DOS whichvanishes near the Fermi energy as a

power law,

g +4=g 4=8

 

N !   ! : 1

The exp onent g dep ends on the strength of the electron-electron interaction: it is smaller



larger than two for repulsive attractive interactions. In the non-interacting case g =2,



and the DOS is constantasinFermi liquids [4].

Recently it b ecame p ossible to fabricate interfaces b etween a sup erconductor S and a

two-dimensional electron 2DEG [5]. An excess low-voltage conductance due to Andreev

scattering has b een observed in Nb-InGaAs junctions [6], as well as a sup ercurrent through a

2DEG in an InGaAs/InAlGaAs heterostructure with Nb contacts [7,8]. If the 2DEG is gated

to form a , it should b e p ossible to study transp ort through Sup erconductor

- Luttinger Liquid S-LL interfaces. The Josephson current through a S-LL-S system has

b een calculated [9,10], as well as the I -V characteristics of a tunnel junction b etween a

sup erconductor and a chiral LL [11]. The latter can b e realized, e.g., in the fractional

quantum Hall regime.

The proximity e ect [12] mo di es the prop erties of a normal metal N in contact with

a sup erconductor. The leakage of Co op er pairs induces a non-vanishing pair amplitude in

N, de ned as F ~r =h ~r ~ri, where  ~r  is the annihilation op erator for an electron

"  s

with spin s. The pair amplitude is a two-particle prop erty, related to the probability to nd

two time-reversed electrons at a p osition ~r . In a clean normal metal at zero temp erature,

F ~r  decays as 1=r away from the N-S interface. In a LL with repulsiveinteraction in con-

tact with a sup erconductor, F ~r  decays as 1=r , where >1 dep ends on the strength of

interaction [10]. These results hold as long as ~r lies within the temp erature-dep endent coher-

ence length  =hv =k T from the interface to the sup erconductor. At larger distances,

N F B

F ~r  decays exp onentially on the length scale  . The reason for the decay of the pair

N

amplitude is that the two electrons lo ose their relative coherence over this distance.

Single electrons, however, lo ose phase coherence only at a much larger distance, namely the

phase-breaking length L . Indeed, recent exp eriments [8,13] have shown that interference



e ects due to single quasiparticles in N-S systems p ersist over distances much larger than

 .We, therefore, exp ect quite generally a considerable in uence of sup erconductivityon

N

single particle prop erties over distances where the pair amplitude has already decayed.

In order to investigate these prop erties in a strongly interacting system we study the lo cal

single-particle density of states DOS of a LL in contact with a sup erconductor. We nd

that the lo cal DOS is substantially enhanced near the Fermi energy as compared to the p ower

law decay of an isolated LL cf. Eq.1. This result should b e contrasted with the b ehavior

of the pair amplitude a two-particle prop erty whichis suppressed in the interacting system. 2

The anomalous enhancement is a result of the interplaybetween the scattering of low-energy

electrons at the S-LL interface and the electron-electron interactions in the LL [14]. As for

the space dep endence, the DOS do es not decay in the same fashion as the pair amplitude

away from the S-LL interface. It remains enhanced up to distances of the order of the mean

free path, whichmaybemuch larger than  for a clean quantum wire. Hence, the e ect

N

cannot simply b e explained in terms of a nite density of Co op er pairs in the LL. Both the

frequency and the space dep endence of the DOS can b e detected exp erimentally by coupling

normal metal tunneling prob es to the LL at some distance from the sup erconductor.

In the inset of Fig. 1 weschematically draw a 'clean' S-LL interface, consisting of a

LL in go o d contact with S. The shaded area indicates a tunnel junction b etween the LL

and a normal metal prob e. We will also study a LL of nite length connected to two

sup erconductors S-LL-S system. In such a system Andreev b ound states exist b elow the

gap [15]. Finally,we will comment on the case of a LL connected to S by means of a tunnel

barrier. The anomalous enhancement of the DOS is found in this case as well.

The Hamiltonian of a LL can b e written in b osonized form as h =1

" 

Z

X

1 g 2

j

2 2

^

H = dx r  ; 2 v r  +

L j j j

2 2 g

j

j

where j = ;  , and v =2=g v are the renormalized interaction-dep endentFermi velo c-

j j F

ities. We restrict ourselves to repulsive, spin-indep endentinteractions; hence g < 2 and



g = 2. The Fermi eld op erators are decomp osed in terms of right- and left-moving



ik x ik x

F F

op erators  and  , resp ectively,  = e  + e  , where k is the Fermi

+;s ;s s +;s ;s F

wavevector. The elds  in turn can b e expressed through Boson op erators

;s

p

p

y

i  [ x+ x]

s s

 =  e ; 3

0

;s

1 1

p p

where =  + s  and  =  + s . The density of electrons p er spin in the LL

s   s  

2 2

is  = k =2 . Maslovetal. [10] recently develop ed a b osonization scheme to treat clean

0 F

S-LL interfaces. For a LL coupled to two sup erconductors at a distance L, they obtained

the following normal mo de expansion for the the elds

r r

X

 x i g



y

^ ^

x= J +  + sinqxb b ; 4

 q ;q

;q

2 2L 2 2

q>0

r

X

i 1 g



0 y

^ ^

p

+ sinqxb + b ; 5 x=

q ;q 

 ;q

 2 2

q>0

s

r

X

 2 x i

y

^ ^

 x= b ; 6 M + sinqxb

 ;q q

;q

2 2L 2 g



q>0

s

X

1 i 2

0 y

^ ^

p

 x=  + sinqxb + b  : 7

 q ;q

 ;q

 2 g



q>0

y

^

Here, b are Bose op erators and = expfq =2g where is a short range cut-o . The

q

j;q

phase di erence b etween the two sup erconductors is ; J and M describ e the top ological

0 0

excitations satisfying the constraint J + M = o dd. Finally, and  are canonically

 

conjugate to J;M resp ectively. The lo cal density of states p er spin of the LL measured at 3

a distance x from the sup erconducting contact is obtained from the retarded one-electron

0 y 0

Green's function of the LL, G x; x ; t ihf x; t; x ;0gi t,

R s

s

Z

1

1

i! t

N x; ! = Im dte G x; x; t : 8

R



1

We rst discuss the space and frequency dep endence of the DOS of a LL contacted at

x = 0 with a sup erconductor, which corresp onds to the limit L !1 in the mo de expansion

given by Eqs. 4 { 7. In this case only the non-zero mo des q>0 contribute to the

y

lo cal DOS. The correlation function h x; t x; 0i can b e evaluated using the b oson

s

s

representation Eq. 3 with the result

Y

2 2

j

j

2

+2x

y

h x; 0 x; ti =2

s 0

2 2

s

 iv t

j

j=;

h i

j

2

 ; 9

 i2x+v t +i2xv t

j j

at a distance x from the LL-S interface, where =g=16 1=4g  and =g=16 +

j j j j j

1=4g . At small energies the DOS b ehaves as

j

g =41=2



N !   ! : 10

S LL

The exp onent of the DOS is negativeg < 2, which implies a strong enhancement at



low energies whereas in the absence of S the DOS of the LL vanishes at the Fermi energy.

The presence of the sup erconductor thus changes the prop erties of the Luttinger liquid in

a qualitativeway. Recently, Oreg and Finkel'stein [14] have found a similar enhancement

of the lo cal DOS of a LL in the presence of an impurity. They interpret their result as

a consequence of the interplaybetween the back-scattering induced by the impurity and

the repulsiveinteractions in the LL. A similar interplay exists in our system. Although

we consider a clean S-LL interface, backscattering is induced by the sup erconducting gap,

which re ects low-energy electrons either directly or via multiple Andreev pro cesses. The

enhanced DOS as a function of frequency, Eq. 10, is schematically drawn in Fig. 1; for

comparison we also show the vanishing DOS in absence of the sup erconductor, Eq. 1.

Atlow energies ! the enhancement of the DOS p ersists over large distances x!   v =!



from the interface. On the other hand, the induced pair amplitude in the LL, whichis

characteristic of the presence of the sup erconductor, decays as a p ower [10] of the distance

x. This profound di erence in the space dep endence demonstrates that the DOS provides

di erent information compared to the proximity e ect. The reason why the DOS do es not

approach the well-known b ehaviour of an Luttinger liquid far from the sup erconducting

contact is in part related to the fact that we are considering a clean wire. In this case the

states in the LL are extended and the DOS enhancement do es not dep end on x.

Wenow turn to the prop erties of the DOS for a S-LL-S system. The two sup erconductors

are separated by the distance L and are kept at a phase di erence . The latter can b e

achieved, e.g., byemb edding this junction in a SQUID. As we consider a LL of nite length,

the top ological excitations should b e taken into account; moreover the contribution from the

non-zero mo des consists of a discrete sum rather than a continuous integral over q states.

The correlator reads 4

Y

y

i v 1 = t=2L

F

h x; 0 x; ti = e D x; t: 11

;s j

;s

j =;

The exp onential prefactor originates from the top ological part; we used the fact that J =1

and M = 0 in the ground state for < <. The -dep endence is related to the phase-

dep endent shift of the Andreev levels see b elow. The contribution from the non-zero mo des

is given by

 !  !

2

j j

  +2ix=L   2ix=L   iv t=L

j

1 e 1 e  1 e

D x; t= 

j 0

 =L 2  =L

1 e  1 e

 !

j

 =L 2

1 e 

 : 12

 [ i2x+v t]  [ +i2xv t]

j j

1 e 1 e 

As in the previous case of a single S-LL interface, the anomalous b ehavior of the DOS

at low ! extends over large distances, measured now relative to the p osition of one of the

interfaces, hence the phase-dep endent contribution to the DOS p ersists over distances much

larger than the Josephson coupling. If the interaction constant can b e written as a ratio of

twointegers g = m =n , we can express the DOS, using Eq. 11, as

 0 0

XX

N x; ! =  a x[ ! E +!+E ] : 13

0 n ;n ;n

n

s;

Here a x are the Fourier co ecients of the function D x; t corresp onding to the energies

n

n 

E = E 2 +1  v ;

;n F F

n 2Lk 2L

0 F

where E is the Fermi energy. The E are the energies of the Andreev levels [15] in the

F ;n

interacting quantum wire. The phase-di erence lifts the degeneracy for right- and left

moving electrons, giving rise to the Josephson e ect. In the noninteracting case g = 2,



all the  -functions have the same weight and the lo cal DOS shows a p eak whenever the

frequency ! coincides with an Andreev level E . When the electron-electron interaction is

;n

switched on, the charge and spin part in Eq. 12 obtain di erent p erio dicities due to spin-

charge separation. As a consequence the co ecients a show a more structured b ehaviour.

n

In Fig. 2 the DOS is plotted for g = 1 as a function of the frequency and of the distance from



one of the two sup erconductors. For claritywe use a realistic, broadened version of the  -

functions in Eq. 13. We, further, xed the phase di erence between the sup erconductors

to zero. One clearly sees a strong enhancement of the DOS close to the interface. Away from

the sup erconductor the DOS remains enhanced, but the energy scale of the enhancementis

reduced to lower frequencies. The oscillatory contribution to the DOS is reminiscent of the

Friedel-oscillations, characterized by a p erio d 2k . In the general case 6= 0, the DOS for

F

the rightmoving electrons di ers from that of the left moving electrons due to the phase

factor in Eq. 11. Although this leads to a more complicated dep endence of DOS on x and

! , the anomalous enhancement is still present.

So far we discussed the case in which the S-LL interface has a high transparency. Let

us shortly comment on the opp osite limit, in which the Luttinger liquid is connected to the

sup erconductor by a tunnel junction. In this case at low energies, we nd for the DOS close

g =21+1=2g g =8

  

to the junction N  ! . Although the exp onent is di erent from the

S LL 5

one app earing in Eq. 10, the DOS is clearly enhanced. Moreover, also in this case the

enhancement is found regardless of the distance from the junction.

In summary we considered the DOS of a Luttinger liquid in contact with a sup ercon-

ductor. We studied sp eci cally the cases of a single S-LL interface and a S-LL-S system.

Contrary to the well-known b ehavior in Luttinger liquids, the presence of the sup erconduct-

ing contact strongly enhances the lo cal DOS close to the Fermi energy, and this b ehavior

extends to large energy-dep endent distances from the interface. Our results can b e veri ed

exp erimentally [16], e.g., by means of the setup drawn in the inset of Fig. 1. We imagine

connecting the LL by means of a tunnel junction to a normal metal at a distance x from

the interface and measuring the I V characteristic of this junction. If there were no

sup erconductor the conductance of the normal metal-LL junction would go to zero as the

temp erature voltage, frequency is lowered. The presence of the sup erconductor leads to

an excess conductance at the junction.

ACKNOWLEDGMENTS

We thank C. Bruder for numerous imp ortant suggestions and W. Belzig and M. Fab-

rizio for useful discussions. The supp ort of the Deutsche Forschungsgemeinschaft, through

SFB 195, the Europ ean Community through contract ERB-CHBI-CT94-1764, and the

A.v.Humb oldt award of the Finish Academy of Sciences GS is gratefully acknowledged. 6

REFERENCES

[1] V.J. Emery,in Highly Conducting One-Dimensional , edited by J.T. Devreese,

R.P. Evrard, and V.E. van Doren Plenum, New York, 1979; J. S olyom, Adv. Phys.

28, 201 1979.

[2] Spin charge separation has b een observed in quantum wires, see A.R. Goni, ~ A. Pinczuk,

J.S. Weiner, J.M. Calleja, B.S. Dennis, L.N. Pfei er, and K.W. West, Phys. Rev. Lett.

67, 3298 1991.

[3] C.L. Kane and M.P.A. Fisher, Phys. Rev. Lett. 68, 1220 1992; K.A. Matveev and L.I.

Glazman, Phys. Rev. Lett. 70, 990 1993; M. Fabrizio, A.O. Gogolin and S. Scheidl,

Phys. Rev. Lett. 72, 2235 1994.

[4] Measurements of the density of states indicate Luttinger liquid b ehaviour in Bechgaard

salts, see B. Dardel, D. Malterre, M. Grioni, Y. Baer, J. Voit, and D. J er^ome, Europhys.

Lett. 24, 687 1993.

[5] See several articles in Mesoscopic Sup erconductivity, eds. F.W.J. Hekking, G. Schon,

and D.V. Averin, Physica B 203 1994.

[6] A. Kastalsky, A.W. Kleinsasser, L.H. Greene, R. Bhat, F.P. Milliken, and J.P. Harbison,

Phys. Rev. Lett. 67, 3026 1991.

[7] J. Nitta, T. Azaki, H. Takayanagi, and K. Arai, Phys. Rev. B 46, 14286 1992.

[8] A. Dimoulas, J.P. Heida, B.J. van Wees, T.M. Klapwijk, W. v.d. Graaf,and G. Borghs,

Phys. Rev. Lett. 74, 602 1995.

[9] R. Fazio, F.W.J. Hekking, and A.A. Odintsov, Phys. Rev. Lett. 74, 1843 1995.

[10] D.L. Maslov, M. Stone, P.M. Goldbart, and D. Loss, to b e published in Phys. Rev. B.

[11] M.P.A. Fisher, Phys. Rev. B 49, 14550 1994.

[12] G. Deutscher and P.G. de Gennes, in , edited by R.D. Parks Marcel

Dekker, NY 1965, vol. I I, p. 1005.

[13] H. Courtois, Ph. Gandit, D. Mailly, and B. Pannetier, Phys. Rev. Lett. 76, 130 1996.

[14] A similar anomalous enhancement of the lo cal DOS has b een recently found by Oreg

and Finkel'stein for a LL with a backscattering defect. Y. Oreg and A. Finkel'stein,

cond/mat 9601020 unpublished

[15] I.O. Kulik, Zh. Eksp. Teor. Fiz. 57, 1745 1969 [Sov. Phys. JETP 30, 944 1970].

[16] This setup has b een prop osed by D. Esteveet al. private communication to study the

DOS of a di usive conductor connected to a sup erconductor. A theoretical analysis has

b een p erformed by W. Belzig, C. Bruder, and G. Schon, to b e published in Phys. Rev.

B. 7

FIGURES

FIG. 1. Schematic dep endence of DOS on frequency for a pure LL dashed line and for a LL

connected to S  line. Inset: Luttinger liquid, connected adiabatically to a sup erconductor.

The shaded area indicates a tunnel junction with a normal metal used to measure the DOS in the

LL at a distance x from the interface.

FIG. 2. The lo cal DOS for a S-LL-S system for particles of sp ecies p = , plotted as a function

of the frequency ! and the distance x from one of the S-LL interfaces. Wetookg = 1 repulsive



interactions; the  -functions of Eq. 13 have b een smeared, using p eaked Lorentzians with a width

6

of the order the level spacing. Furthermore, Lk =10 ;N = =E ; =0.

F L 0 F 8 Ν(ω)

Ν LL S S-LL N

9 x

Ν LL

ω 0.25 ω Np(x, )/NL 0.2

0.15 10

0.1

0

0.01 0.0004 0.0002 x/L 0.02 ω /EF