Conical Diffraction: Complexifying Hamilton's Diabolical Legacy Mike
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Conical Diffraction: Complexifying Hamilton’s Diabolical Legacy Mike R. Jeffrey A thesis submitted to the University of Bristol in accordance with the requirements of the degree of Ph.D. in the Faculty of Science H. H. Wills Physics Laboratory September 2007 word count 32,795 Abstract The propagation of light along singular directions in anisotropic media teems with rich asymptotic phenomena that are poorly understood. We study the refraction and diffraction of light beams through crystals exhibiting biaxial birefringence, optical activity, and dichroism. The optical properties and length of the crystal are related to the beam’s width, wavenumber, and alignment, by just three parameters defined by the effect of the crystal on a paraxial plane wave. Singular axes are crystal directions in which the refractive indices are degenerate. In transparent biaxial crystals they are a pair of optic axes corresponding to conical intersections of the propagating wave surface. This gives rise to the well understood phenomenon of conical diffraction. Our interest here is in dichroic and optically active crystals. Dichroism splits each optic axis into pairs or rings of singular axes, branch points of the complex wave surface. Optical activity destroys the optic axis degeneracy but creates a ring of wave surface inflection points. We study the unknown effect of these degeneracy structures on the diffracted light field, predicting striking focusing and interference phenomena. Focusing is understood by the coalescence of real geometric rays, while geometric interference is included by endowing rays with phase to constitute complex rays. Optical activity creates a rotationally symmetric cusped caustic surface threaded by an axial focal line, which should be easy to observe experimentally. Dichroism washes out focusing effects and the field is dominated by exponential gradients crossing anti-Stokes surfaces. A duality is predicted between dichroism and beam alignment for gaussian beams: both are described by a single parameter controlling transition between conical and double refraction. For transparent crystals we predict simple optical angular momentum effects accompanied by a torque on the crystal. We also report new observations with a biaxial crystal that test the established theory of conical diffraction. For Fiona. Acknowledgments A debt of gratitude to my supervisor, Michael Berry, for presenting me with such a wonderfully old problem, the opportunity to delve into dusty volumes penned by the giants of 19th century physics, conjure phenomena with echoes through two centuries of researches on light, and dabble in the mathematical heart of physics old and new. My perspective on physics owes so much to the insightful teaching of John Hannay and Michael Berry, and I thank them for a glimpse of that curious geometric world with which physics is rendered comprehensible. For their guidance, encouragement, and nudging in new directions, I am thankful to: John Hannay, John Nye, John Alcock, Jonathan Robbins, and Jon Keating. In my work I have occasionally relied on the help of people not called Jo(h)n, among them: Matthias Schmidt, who I thank for his daring and patience in confronting a century old german tome; James Lunney and Masud Mansuripur who I thank for their collaborative contribution; Miss Turner and Mr Everitt (and his pet brick), who helped mould a young enquiring mind; and Mark Dennis, whose advice was invaluable in the transition of this unlearned undergrad into a naive but infinitesimally more learned postgrad. I would like to thank Michael and his family for their hospitality throughout my PhD research. Also, even the solitary musings of a theorist turn stale without the distractions of one’s fellow theory group inmates (listed in order of decoherence on an average Friday): Tony, Cath, Bramms, Luis, another John, Morgan, Nadav, Gary, Andy 2. Thanks also × to Steve for helping me master La τ ek$%. { } My dearest thanks to those who have made it easy for me to indulge, and even en- couraged me to continue, in endless distractions mathematical and physical, above all: my wife and her family, Fluffy, and the distinguished UH alumni. We are all students, but some of us will never learn. Authors Declaration I declare that the work in this thesis was carried out in accordance with the regulations of the University of Bristol. The work is original except where indicated by special reference in the text, and no part of the thesis has been submitted for any other academic award. Any views expressed in the thesis are those of the author. SIGNED DATE “They, that will, may suppose it an aggregate of various peripatetic qualities. Others may suppose it multitudes of unimaginable small and swift corpuscles .. springing from shining bodies at great distances one after another; but yet without any sensible interval of time, and continually urged forward .. But they, that not like this, may suppose light any other corporeal emanation, or any impulse or motion of any other medium, or aethereal spirit diffused through the main body of aether, or what else they can imagine proper for this purpose .. To avoid dispute, and make this hypothesis general, let every man here take his fancy; only whatever light be, I suppose it consists of rays differing from one another in contingent circumstances, as bigness, form or vigour.” Isaac Newton on the nature of light, Royal Society, 1675 (Whittaker 1951) This thesis includes the following content published by the author: Chapter 4.1 Berry M V, & Jeffrey M R, (2007) Progress in Optics in press Hamilton’s diabolical point at the heart of crystal optics Chapter 4.2 Berry M V, & Jeffrey M R, (2006) J.Opt.A 8 363-372 Chiral conical diffraction Chapters 3 and 4.2 Jeffrey M R, (2006) Photon06 online conference proceedings http://photon06.org/Diffractive%20optics%20Thurs%2014.15.pdf Conical diffraction in optically active crystals Chapter 4.3 Berry M V, & Jeffrey M R, (2006) J.Opt.A 8 1043-1051 Conical diffraction complexified: dichroism and the transition to double refraction Chapter 4.4 Jeffrey M R, (2007) J.Opt.A 9 634-641 The spun cusp complexified: complex ray focusing in chiral conical diffraction Chapter 4.5 Berry M V, Jeffrey M R & Mansuripur M J, (2005) J.Opt.A 7 685-690 Angular momentum in conical diffraction Chapter 4.6 Berry M V, Jeffrey M R & Lunney J G, (2006) Proc.R.Soc.A 462 1629-1642 Conical diffraction: observations and theory Contents 1 Introduction 1 1.1 HistoricalContext ............................... 4 1.2 HistoryofthePhenomenon . 7 2 Paraxial Optics and Asymptotics 17 2.1 OpticsofAnisotropicCrystals. ..... 18 2.2 Principles of Paraxial Light Propagation . ........ 23 2.3 Hamiltonian Formulation . 26 2.4 Complex Ray Directions: So Where Should We Point The Beam?...... 32 2.5 Eigenwave Representation . 35 2.6 Asymptotics of the Geometrical Optics Limit . ....... 37 2.7 ...andHamilton’sPrinciple. 41 2.8 InsidetheCrystal................................ 44 3 The Wave Surfaces 47 3.1 Fresnel’s Wave Surface and Hamilton’s Cones . ....... 48 3.2 TheParaxialPhaseSurfaces. 54 4 The Phenomena of “So-Called” Conical Diffraction 59 4.1 BiaxialCrystals................................. 61 4.1.1 So-called conical refraction . 64 4.1.2 Diffractionintherings. 66 4.1.3 Uniformisation and rings in the focal image plane . ....... 71 4.1.4 Thebrightaxialspike . .. .. .. .. .. .. .. .. 74 4.2 Biaxial Crystals with Optical Activity . ....... 77 4.2.1 The “trumpet horn” caustic of chiral conical refraction........ 80 xv xvi CONTENTS 4.2.2 Voigt’s “Trompeten Trichters”: rays inside the chiral crystal . 81 4.2.3 Diffraction and the caustic horn . 84 4.2.4 Uniformisation over the caustic . 86 4.2.5 TheStokesset .............................. 88 4.2.6 Thespuncuspandaxialspot . 90 4.2.7 Fringesnearthefocalplane . 94 4.3 DichroicBiaxialCrystals. 97 4.3.1 Conical refraction complexified . 99 4.3.2 Complex geometric interference . 101 4.3.3 Gaussian beams and the transition to double refraction .......104 4.3.4 Anoteoncirculardichroism . 111 4.3.5 Imaginary conical refraction . 112 4.4 Dichroic Biaxial Crystals with Optical Activity . ..........114 4.4.1 Chiral conical refraction complexified . 116 4.4.2 Thecomplexwhisker. .118 4.4.3 Diffraction ................................120 4.4.4 Thecomplexifiedspuncusp . .122 4.5 Angular Momentum in Conical Diffraction . 124 4.5.1 Paraxial optical angular momentum . 124 4.5.2 Nonchiral .................................125 4.5.3 Chiralitydominated . .126 4.5.4 Strongly biaxial or chiral crystals . 127 4.5.5 Torqueonthecrystal . .. .. .. .. .. .. .. .127 4.6 Observations of Biaxial Conical Diffraction . ........129 5 Concluding Remarks 137 A Solutions to the chiral quartic 145 B Spherical conical refraction 147 C Glossary of key symbols 151 Bibliography 153 List of Figures 1.1 Lloyd’s discovery of conical refraction . ........ 8 1.2 Conical diffraction of a pencil of rays . ...... 9 1.3 Theconicalrefractionlunes . 10 1.4 Photographs of chiral conical diffraction . ........ 11 1.5 Thediabolicalpoint .............................. 13 2.1 Fresnel’s wave surface and rotated coordinates . ......... 22 2.2 The parameters of paraxial conical refraction . ......... 26 2.3 ThePoincar´eSphere .............................. 31 2.4 Real and complex rays in stationary phase analysis . ......... 43 3.1 Theopticaxes .................................. 49 3.2 Duality of the wave and ray surfaces . 52 3.3 Geometry of internal and external conical refraction . ........... 53 3.4 Theparaxialwavesurfaces . 57 4.1 Evolution of the conical diffraction rings . ........ 62 4.2 Simulation of the conical diffraction ring evolution . ........... 63 4.3 The rays of internal conical refraction . ....... 65 4.4 The rays of external conical refraction . ....... 65 4.5 Asymptoticsofthesecondaryrings . ..... 69 4.6 The regimes of conical diffraction . ..... 70 4.7 Ringsinthefocalimageplane. 73 4.8 Aperture-induced oscillations in the focal plane . ........... 74 4.9 Intensityoftheaxialspike. 75 4.10 Intensity sections of the bright caustic horn . .......... 78 xvii xviii LIST OF FIGURES 4.11 The rings of chiral conical diffraction . ........ 79 4.12 Rays of chiral conical refraction . ....... 81 4.13 Ray intensity through the crystal .