2021 August Nichols Butler

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p The ACS, New York Section is pleased to announce that the Nichols Award Jury has chosen Professor Alison Butler to be the William H. Nichols Medalist for 2022. Professor Butler is DistinGuished Professor of Chemistry and Biochemistry at UC Santa Barbara. She is beinG honored for her pioneerinG contributions to marine bioinorGanic chemistry. The Nichols Medal Award will be presented at the Nichols Award Dinner that follows the DistinGuished Symposium. Professor Alison Butler was an underGraduate chemistry major at Reed ColleGe (BA 1977) and a Graduate student in Chemistry at the University of California, San DieGo (PhD 1982). FollowinG postdoctoral fellowships in the laboratories of Joan S. Valentine at UCLA and then Harry B. Gray atCaltech, she beGan her independent career in the Department of Chemistry at UC Santa Barbara in 1986. She proGressed throuGh the ranks to her current position of Distinguished Professor of Chemistry and Biochemistry at UC Santa Barbara. Professor Butler is an elected Fellow of the American Academy of Arts and Sciences (2019), the Royal Society of Chemistry (2019), the American Chemical Society (2012), and the American Association for the Advancement of Science (1997). She has also been recoGnized with the 2018 ACS Alfred Bader Award in BioorGanic or BioinorGanic Chemistry, a 2019 ACS Cope Scholar Award in orGanic chemistry, and the 2019 InorGanic Reaction Mechanisms Award of the Royal Society of Chemistry. She has served as President of the Society for BioloGical InorGanic Chemistry (2012-2014) and Chair of the Chemistry section (Section C) of the American Associate for the Advancement of Science (2012-2013). She is currently Chair of the ACS Division of InorGanic Chemistry. Further details about the Nichols Symposium for 2022 will be featured in an upcominG edition of the Indictor as well as on the New York Section website. .

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Catechol-Cation Synergy in Wet Adhesive Materials
UNIVERSITY OF CALIFORNIA Santa Barbara CATECHOL-CATION SYNERGY IN WET ADHESIVE MATERIALS A dissertation submitted in partial satisfaction of the requirements for the degree of Doctor of Philosophy in Chemistry by Gregory Peter Maier Committee in charge: Professor Alison Butler Professor J. Herbert Waite Professor R. Daniel Little Professor Song-I Han September 2017 The dissertation of Gregory Peter Maier is approved: ____________________________________________________________ J. Herbert Waite ____________________________________________________________ R. Daniel Little ____________________________________________________________ Song-I Han ____________________________________________________________ Alison Butler, Committee Chair August 2017 Catechol-Cation Synergy in Wet Adhesive Materials Copyright © 2017 By Gregory Peter Maier iii ACKNOWLEDGEMENTS My experience in graduate school has had a profound impact on me both personally and professionally. I would like to thank my advisor, Professor Alison Butler, for guiding me through this transformative process. Her support, dedication, and encouragement were unwavering and I consider myself lucky to have been a part of her research group. I would also like to thank my committee members Songi Han, Dan Little, and especially Herb Waite for their guidance in my research. I’ve been lucky to have been involved in several fulfilling collaborations. Mike Rapp from Jacob Israelachvili’s lab at UC Santa Barbara and I have been partners in research for the majority of my time in graduate school and much of this dissertation would not have been possible without him. Additionally, my current and former group members helped make a positive, fun, and engaging work environment. In particular, Robert Lewis has always been helpful with organic synthesis advise and has always been a great friend. Thank you to my family for guiding me to where I am today and to my amazing girlfriend Kate Hawley and friend Johnny Kessenich, whose willingness to move to Santa Barbara has truly made the last 5 years some of the best in my life.
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Impact of Molecular Architecture and Adsorption Density on Adhesion of Mussel-Inspired Surface Primers with Catechol-Cation Synergy † ‡ ‡ † § George D
Article Cite This: J. Am. Chem. Soc. 2019, 141, 18673−18681 pubs.acs.org/JACS Impact of Molecular Architecture and Adsorption Density on Adhesion of Mussel-Inspired Surface Primers with Catechol-Cation Synergy † ‡ ‡ † § George D. Degen, Parker R. Stow, Robert B. Lewis, Roberto C. Andresen Eguiluz, Eric Valois, † ‡ ⊥ † ∥ Kai Kristiansen, Alison Butler,*, and Jacob N. Israelachvili , , † ‡ § Department of Chemical Engineering, Department of Chemistry and Biochemistry, Biomolecular Science and Engineering, and ∥ Materials Department, University of California, Santa Barbara, California 93106, United States *S Supporting Information ABSTRACT: Marine mussels secrete proteins rich in residues containing catechols and cationic amines that displace hydration layers and adhere to charged surfaces under water via a cooperative binding eﬀect known as catechol-cation synergy. Mussel-inspired adhesives containing paired catechol and cationic functionalities are a promising class of materials for biomedical applications, but few studies address the molecular adhesion mechanism(s) of these materials. To determine whether intramolecular adjacency of these functionalities is necessary for robust adhesion, a suite of siderophore analog surface primers was synthesized with systematic variations in intramolecular spacing between catechol and cationic functionalities. Adhesion measurements conducted with a surface forces apparatus (SFA) allow adhesive failure to be distinguished from cohesive failure and show that the failure mode depends critically on the siderophore analog adsorption density. The adhesion of these molecules to muscovite mica in an aqueous electrolyte solution demonstrates that direct intramolecular adjacency of catechol and cationic functionalities is not necessary for synergistic binding. However, we show that increasing the catechol-cation spacing by incorporating nonbinding domains results in decreased adhesion, which we attribute to a decrease in the density of catechol functionalities.
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Downloaded Via UNIV of CALIFORNIA MERCED on April 28, 2020 at 20:21:08 (UTC)
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