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Generation Conditions of and Rhyodacite via the Crystallization of an Andesitic Magma. Implications for the Plumbing System at Santorini (Greece) and the Origin of Tholeiitic or Calc-alkaline Differentiation Trends in Arc Magmas Joan Andújar, Bruno Scaillet, Michel Pichavant, Timothy H. Druitt

To cite this version:

Joan Andújar, Bruno Scaillet, Michel Pichavant, Timothy H. Druitt. Generation Conditions of Dacite and Rhyodacite via the Crystallization of an Andesitic Magma. Implications for the Plumbing Sys- tem at Santorini (Greece) and the Origin of Tholeiitic or Calc-alkaline Differentiation Trends in Arc Magmas. Journal of Petrology, Oxford University Press (OUP), 2016, 57 (10), pp.1887 - 1920. ￿10.1093/petrology/egw061￿. ￿insu-01488159￿

HAL Id: insu-01488159 https://hal-insu.archives-ouvertes.fr/insu-01488159 Submitted on 14 Dec 2018

HAL is a multi-disciplinary open access L’archive ouverte pluridisciplinaire HAL, est archive for the deposit and dissemination of sci- destinée au dépôt et à la diffusion de documents entific research documents, whether they are pub- scientifiques de niveau recherche, publiés ou non, lished or not. The documents may come from émanant des établissements d’enseignement et de teaching and research institutions in France or recherche français ou étrangers, des laboratoires abroad, or from public or private research centers. publics ou privés. J OURNAL OF Journal of Petrology, 2016, Vol. 57, No. 10, 1887–1920 doi: 10.1093/petrology/egw061 P ETROLOGY Original Article

Generation Conditions of Dacite and Rhyodacite

via the Crystallization of an Andesitic Magma. Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 Implications for the Plumbing System at Santorini (Greece) and the Origin of Tholeiitic or Calc-alkaline Differentiation Trends in Arc Magmas Joan Andujar 1,2,3*, Bruno Scaillet1,2,3, Michel Pichavant1,2,3 and Timothy H. Druitt4

1Universite´ d’Orle´ans, ISTO, UMR 7327, 45071 Orle´ans, France; 2CNRS/INSU, ISTO, UMR 7327, 45071 Orle´ans, France; 3BRGM, ISTO, UMR 7327, BP 36009, 45060 Orle´ans, France; 4Laboratoire Magmas et Volcans, Universite´ Blaise Pascal–CNRS–IRD, OPGC, 5 Rue Kessler, 63038 Clermond-Ferrand, France

*Corresponding author. Telephone: (þ33) 2 38 25 54 04. Fax: (þ33) 02 38 63 64 88. E-mail: [email protected]

Received July 12, 2015; Accepted September 12, 2016

ABSTRACT Andesitic arc volcanism is the most common type of subduction-related magmatism on Earth. How these melts are generated and under which conditions they evolve towards silica-rich liquids is still a matter of discussion. We have performed crystallization experiments on a representative sample from the Upper Scoriae 1 (USC-1) eruption of Santorini (Greece) with the aim of understand- ing such processes. Experiments were performed between 1000 and 900 C, in the pressure range

100–400 MPa, at fO2 from QFM (–fayalite–magnetite) to NNO (nickel–nickel oxide) þ 15, with H2Omelt contents varying from saturation to nominally dry conditions. The results show that the USC-1 andesitic magma was generated at 1000 C and 12–15 km depth (400 MPa), migrated to shal- lower levels (8 km; 200 MPa) and intruded into a partially crystallized dacitic magma body. The magma cooled to 975 C and generated the assemblage and compositional zonations that characterize the products of this eruption. An injection of basaltic magma problably subse- quently triggered the eruption. In addition to providing the pre-eruptive conditions of the USC-1 magma, our experiments also shed light on the generation conditions of silica-rich magmas at

Santorini. Experimental of runs performed at fO2 NNO þ 1(6 05) closely mimic the compositional evolution of magmas at Santorini whereas those at reduced conditions (QFM) do not. Glasses from runs at 1000–975 C encompass the magma compositions of intermediate-dominated eruptions, whereas those at 950–900 C reproduce the silicic-dominated eruptions. Altogether, the comparison between our experimental results and natural data for major recent eruptions from Santorini shows that different magma reservoirs, located at different levels, were involved during highly energetic events. Our results suggest that fractionation in deep reservoirs may give rise to magma series with a tholeiitic signature whereas at shallow levels calc-alkaline trends are produced.

Key words: phase equilibria; andesite; liquid line of descent; experimental petrology; Santorini; tholeiitic; calc-alkaline

VC The Author 2016. Published by Oxford University Press. All rights reserved. For Permissions, please e-mail: [email protected] 1887 1888 Journal of Petrology, 2016, Vol. 57, No. 10

INTRODUCTION storage and differentiation conditions of the selected The origin of arc and their relationships with sample. We use our results to constrain the possible their silicic counterparts ( and ) is still a parent–daughter relationships between andesites and matter of debate. Various models have been discussed dacites–rhyodacites at Santorini. Overall, the results con- in the literature to explain the origin of these melts: (1) strain the architecture of the plumbing system immedi- andesites are the by-products of crystallization ately prior to large andesitic explosive eruptions and (e.g. Gill, 1981; Pichavant et al., 2002; Andujar et al., thereby improve our understanding of the ’s be- 2015); (2) andesites arise from mixing between haviour, which is critical for the assessment of future vol- canic hazards in this area. More generally, our study also Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 and basalt (i.e. Eichelberger, 1978; Ruprecht et al., provides insight into the conditions leading to the gener- 2012); (3) andesite liquids are direct melting products of ation of tholeiitic and calc-alkaline magmatic series in is- subducting oceanic crust (e.g. Green & Ringwood, land arc environments. 1968; Castro et al., 2013). Regardless of which, if any, of the above mechanisms dominates, an important ques- tion is to understand under which conditions andesitic GEOLOGICAL SETTING melts evolve towards silica-rich compositions, and in Santorini forms part of the Hellenic of the particular whether this process occurs in a single reser- Aegean Sea, which owes its origin to the subduction of voir or in multiple reservoirs located at different depths. the African plate beneath the Eurasian plate (Fig. 1; Le This is crucial for understanding the final storage depth Pichon & Angelier, 1979; Papazachos et al., 2000; of more evolved liquids and the structure of the plumb- Nocquet, 2012). The volcano lies on continental crust ing system beneath a volcano, as the generation level about 23 km thick (Tirel et al., 2004; Karagianni & of the silica-rich melts may not correspond to that of Papazachos, 2007); the boundary between the upper their pre-eruptive storage. We address this issue by and lower crust is at about 15 km depth (Konstantinou, unravelling the parent–daughter relationships between 2010). andesites and recent dacites–rhyodacites at Santorini The volcanic history of Santorini has been recon- (Greece), to understand the evolution of the plumbing structed by Druitt et al. (1999). Activity began at about system with time at this volcanic center. 650 ka with the eruption of hornblende-bearing rhyo- Santorini is one of the largest volcanoes in the lites, rhyodacites and minor andesites of calc-alkaline Aegean region of Greece, with an activity characterized affinity (Nichols, 1971a). From 550 ka onwards, the vol- by multiple, large, explosive eruptions, some of which cano emitted magmas ranging from basalt to rhyoda- caused collapse, separated in time by periods cite in composition, hornblende became scarce as a of effusive edifice construction and weaker explosive phenocryst phase, and the magmas became tholeiitic to activity (Druitt et al., 1999). The most recent caldera- transitional tholeiitic–calc-alkaline in character. Around forming eruption was the ‘Minoan’ eruption some 36 360 ka, the activity became highly explosive, with the al- kyr ago (Bond & Sparks, 1976; Heiken & McCoy, 1984; ternation of plinian eruptions and interplinian periods Druitt, 2014). Magmas at Santorini range from basalt to of constructional activity involving effusive and weakly andesite, dacite and rhyodacite, with calc-alkaline to explosive events. Direct field evidence exists for at least weakly tholeiitic affinities (Nichols, 1971a; Druitt et al., four caldera collapse events associated with the large 1999). and minor explosive events emitted all plinian eruptions. Following the Minoan eruption at types of magmas, whereas the products of large explo- about 36 ka, volcanic activity resumed within the cal- sive eruptions are restricted to andesitic, dacitic and dera at 197 BC and continued until recent times (Fig. 1; rhyodacitic compositions (Druitt et al., 1999; Vespa Pyle & Elliott, 2006). The products of this historical vol- et al., 2006). The occurrence of large explosive events canism have built up an 3km3 intracaldera edifice, the ejecting voluminous amounts of crystal-poor andesitic summit of which forms the islands of Palaea Kameni magma is a notable feature of Santorini volcanism and Nea Kameni. The last eruption of the Kameni (Druitt et al., 1989, 1999; Mellors & Sparks, 1991). Volcano took place in 1950. A period of caldera unrest, Nevertheless, previous studies of magma genesis and involving uplift and increased seismicity, took place at pre-eruptive magma storage at Santorini have focused Santorini in 2011–2012 (Parks et al., 2012). either on rhyodacitic to dacitic (Cottrell et al., 1999; The products of the <360 ka large explosive erup- Druitt et al., 1999; Gertisser et al., 2009; Cadoux et al., tions range from andesitic to rhyodacitic in composition 2014) or basaltic (Nichols, 1971a; Andujar et al., 2015) (Huijsmans et al., 1988; Huijsmans & Barton, 1989; magmas. In comparison, the conditions that lead to the Druitt et al., 1999). Large explosive eruptions of andes- generation of large volumes of andesitic liquids, and itic magma include the Upper Scoriae 1 (80 ka; Keller those involving evolution from andesite to the most et al., 2000; Vespa et al., 2006) and Upper Scoriae 2 silica-rich compositions, are still unclear. (54 6 3 ka; Druitt et al., 1999) eruptions. Large silicic In this study we investigate experimentally the phase eruptions include the Lower 1 (184 ka; Keller relationships of a representative andesite from Santorini, et al., 2000; Gertisser et al., 2009), Lower Pumice 2 and we compare these data with natural (172 ka; Keller et al., 2000; Gertisser et al., 2009), Cape and glass compositions to shed light on the pre-eruptive Riva (218 6 04 ka; Fabbro et al., 2013) and Minoan Journal of Petrology, 2016, Vol. 57, No. 10 1889

(a) (b) Eruptions

Minoan 3.6 ka Dominantly silicic

Dominantly Cape Riva intermediate 22 ka Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 Upper Scoriae 2 54 ka Upper Scoriae 1 80 ka andesitic Vourvoulos selected Middle Pumice sample 145 ka

Cape Thera

Lower Pumice 2 172 ka

Lower Pumice 1 184 ka

Cape Therma 3 196 ka Cape Therma 2

Cape Therma 1

Cape Alai

Fig. 1. (a) Simplified geological map of Santorini after Druitt et al. (1999). (b) Schematic stratigraphy of Santorini volcanic products, summarized from the data of Druitt et al. (1999). Ages are those of Druitt et al. (2016). The Upper Scoriae 1 eruption (80 ka) was the source for the andesitic sample used in this study. (c) Isopach map of pumice-fall deposits and vent location of the Upper Scoriae eruptions of Santorini. (d) TiO2 (wt %) and (e) FeO* (wt %) vs SiO2 (wt %) of Santorini magmas. The fractionation trend for Santorini magmas is shown by the grey arrow, whereas mixing models for Cape Riva and Upper Therasia andesites (grey dashed field) are shown as black lines [modified from Fabbro et al. (2013)]. It should be noted that the Upper Scoriae 1 (USC-1; Table 1) bulk-rock composition (star) plots on the fractionation trend, indicating that this composition is a true liquid and is genetically linked to more evolved magmas (see text for details).

(36 ka) eruptions (Fig. 1b). The large silicic reservoirs covering at least 60 km2 (Fig. 1; Mellors & Sparks, 1991; were dominated by rhyodacitic magma, intruded by Druitt et al., 1999). basalt to andesite magmas immediately prior to erup- Druitt et al. (1999) made a cursory petrological study tion; the latter are found as blebs or bands dis- of the USC-1 products. They showed that the dominant persed within the main silicic volume (Nichols, 1971a; (99%) juvenile component is an andesitic scoria with

Huijsmans et al., 1988; Cottrell et al., 1999; Druitt et al., 577–591 wt % SiO2; however, dacitic with 1999; Gertisser et al., 2009). 620–632 wt % SiO2 are present sparsely in the basal fallout layer and are interpreted as representing a small The Upper Scoriae 1 eruption volume of more evolved magma that was co-erupted The Upper Scoriae 1 (USC-1) eruption started with a with the andesite. They reported 3–14 wt % Plinian phase from a vent close to Nea Kameni. The first (Pl), clinopyroxene (Cpx), orthopyroxene (Opx) and phase generated a fallout deposit up to 150 cm thick, magnetite (Mt) phenocrysts in the andesite. with thin intercalated base surge layers. It subsequently With the aim of determining andesite–basalt rela- generated voluminous scoria flows that were dis- tionships at Santorini, Andujar et al. (2015) performed charged mostly towards the southern parts of the island a detailed petrographic study of the USC-1 sample that and laid down scoriaceous ignimbrite and spatter is the starting composition for the present study. 1890 Journal of Petrology, 2016, Vol. 57, No. 10

(c ) Pumice eruption; Druitt et al., 1999). This and the com- mon mantling of Cpx by an Mg-rich rim both suggest a Upper Scoriae 1 vent location and products distribution (from Druitt et al. 1999) xenocrystic origin for such Opx and Mg-poor Cpx in theandesite[seeAndujar et al. (2015)formore details]. Phase equilibrium experiments show that Santorini pond at depths of 12–14 km (400 MPa), where they fractionate to yield liquids (55–

50 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 vent 58 wt % SiO2) having up to 5 wt % dissolved H2O (H O ) at around 1000 C and at an fO QFM (603 150 2 melt 2 100 200 log units), where QFM is quartz–fayalite–magnetite buf- fer (Andujar et al., 2015). This is achieved by crystalliz- ing about 60 wt % Ol þ Cpx þ Pl þ Opx þ Mt 6 Pig 6 2 km Ilm (ilmenite). Experiments show that this phenocryst assemblage mimics physically and compositionally the 1.5 mafic xenocrystic assemblage of the USC-1 andesite, (d) USC-1 andesite Fractionation indicating that the latter probably came from the mushy trend for

% zone in which the andesite was produced. Altogether, t 1.0 Santorini magmas

w

the observations made by Andujar et al. (2015) demon-

2

O

i strate the complex and highly dynamic character of the T Santorini andesites Cape Riva plumbing system at Santorini, as already stressed by 0.5 Mixing models Upper The rasia (Fabbro et al. andesites from mixing previous studies (i.e. Cottrell et al., 1999; Druitt et al., 2013) 1999; Michaud et al., 2000; Gertisser et al., 2009; Martin 0.0 et al., 2010). 12 (e) USC-1 andesite Current thermobarometric constraints for Fractionation Santorini magmas

% t 8 trend for Gardner et al. (1996) determined a temperature of w Santorini magmas * Santorini andesites 1000 C and H2Omelt of 3 wt % for the USC-1 andesite

O

e Mixing models based on analyses of glass inclusions in plagioclase F 4 (Fabbro et al. Cape Riva 2013) Upper Therasia phenocrysts. This temperature is in the range of hom- andesites from mixing ogenization temperatures of heating stage experiments 0 (985–1005C) performed on andesitic melt inclusions by Michaud et al. (2000), although those researchers re- 45 50 55 60 65 70 75 SiO (wt%) ported higher water contents (5–6 wt %) estimated 2 using the ‘by difference method’ (Devine et al., 1995). Fig. 1. Continued. For the more silicic products (dacite to rhyodacite), pre- eruptive constraints based on a variety of geothermom- eters and experimental phase equilibria were estab- The sample is an andesitic scoria block with 28 wt % of lished by Cottrell et al. (1999) and Cadoux et al. (2014). phenocrysts set in a highly vesiculated and microcrys- Coexisting Fe–Ti oxides in dacitic to rhyodacitic prod- talline groundmass of Pl, Cpx and Mt (Table 1). The ucts yield temperatures between 825 and 1012 C phenocrysts are euhedral to subhedral Pl (16 wt %, (Barton & Huijsmans, 1986; Gardner et al., 1996; Cottrell et al., 1999; Druitt et al., 1999; Gertisser et al., 2009; An53625),Cpx[8wt%,eitherasisolated,normally Cadoux et al., 2014; Druitt, 2014). Water content esti- zoned crystals (cores of En44Fs19Wo37, Mg#70 to rims mates are in the range 3–4 wt % for post-caldera dacites of En42Fs21Wo37, Mg#67 6 1) or as overgrowths of Mg-poorer Cpx (En38Fs23Wo39, Mg#63) or pigeonite of Nea Kameni (Barton & Huijsmans, 1986), whereas for (Pig; En55Fs28Wo16, Mg#67)], Mt (3 wt %), and Opx the rhyodacitic products of the Lower Pumice 2 and (13wt%,En65Fs29Wo4). In addition, the sample has Minoan eruptions, phase equilibrium experiments gave >15 vol. % xenocrystic olivine (Ol) (Fo64), Pig, diopside H2Omelt ranging from 3 to 6 wt % (Cottrell et al., 1999; (En43–45Fs10–14Wo43–45, Mg#75–81) and An-rich Pl Gertisser et al., 2009; Cadoux et al., 2014). Pressure esti- (An91). Some xenocrysts have compositional zonations mates for the silicic reservoirs vary according to the re- suggesting partial re-equilibration with the host andes- searchers. Whereas Gertisser et al. (2009) estimated a itic melt whereas others lack such features. The Mg- pressure of 400 MPa for the Lower Pumice 2 reservoir poor augite (En38Fs23Wo39, Mg#63), low-An Pl by using the Al-in-hornblende geobarometer, Cottrell (An45–50) and resorbed Opx in the andesite have a com- et al. (1999) and Cadoux et al. (2014) determined pres- position similar to the phenocrysts of Santorini dacites sures up to 200 MPa for the Minoan, Lower Pumice 1,

(En55Fs40Wo4, Mg#58; e.g. dacite from the Middle and Lower Pumice 2 units. Although Cottrell et al. Journal of Petrology, 2016, Vol. 57, No. 10 1891

Table 1: Major element compositions of the bulk-rock natural Upper Scoriae 1 andesite sample from Andujar et al. (2015), starting material, glass and mineral phases (wt %)

Bulk- Starting SD glass* mt SD pl SD augite SD opx SD rock material (Mg#67) n:5685675

SiO2 5852 5926 017 6279 011 002 5505 144 4925 073 5205 072 TiO2 130 130 002 098 1514 229 007 013 101 012 033 006 Al2O3 1604 1560 017 1582 302 056 2661 074 354 066 109 051

MgO 284 247 006 178 264 050 008 011 1420 044 2349 077 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 CaO 655 644 025 482 007 006 1040 054 1746 081 209 019 MnO 019 022 006 019 050 022 004 005 042 012 063 010 FeO* 874 862 030 701 7145 134 062 057 1240 050 1885 069 Na2O419 432 009 470 003 004 503 031 031 005 007 010 K2O140 154 002 190 002 003 020 011 002 002 002 003 P2O5 023 023 001 Sum 100 100 100 9309 160 9827 137 9268 121 9877 132 Mg# 617 040 6712 062 6896 084 a.p.f.u. En 4183 6538 086 Fs 2050 2943 081 Wo 3698 419 041 An 5266 248 Ab 4610 250 Or 124 075 phase proportions (wt %) 321557713

*Calculated by mass balance. Bulk-rock analysed by inductively coupled plasma mass spectrometry; mt, magnetite; pl, plagioclase; opx, orthopyroxene; n, num- ber of analysis; SD, standard deviation. FeO*, total iron reported as Fe2þ. En, Fs and Wo were calculated as done by Morimoto (1989). Mg# ¼ 100Mg/(Mg þ Fe*); An ¼ 100Ca/(Ca þ Na þ K); Ab ¼ 100Na/(Ca þ Na þ K); Or ¼ 100K/(Ca þ Na þ K). End-members calculated as done by Deer et al. (1972).

(1999) inferred magma migration from 200 to 50 MPa ilmenite crystallization at 58 wt % SiO2 results in Fe–Ti before the Minoan eruption, Cadoux et al. (2014) con- depletion, silica enrichment and moderate alkali enrich- cluded that all rhyodacitic magmas from the first and ment of the melts that characterize the more evolved second explosive cycles were stored at the same pres- magmas at Santorini (dacites, rhyodacites; Fig. 1d and sure (200 MPa), and that migration of magma is not e). However, the FC process alone cannot fully explain necessary to explain the petrological attributes of the the main trends defined by the Santorini magmas. caldera-forming Minoan eruption. Pressure estimates Crustal assimilation together with repeated input of obtained for the more recent dacites of Nea Kameni mafic magma also exerts some control on magma evo- point to shallower depths (2–4 km, 80–150 MPa; Barton lution (Nichols, 1971b; Barton et al., 1983; Huijsman

& Huijsmans, 1986). Finally, fO2 values range between et al., 1988; Druitt et al., 1999; Zellmer et al., 2000). As a QFM – 05(05 log unit below the quartz–fayalite–mag- result, even if, as we argue here, the vast majority of netite buffer; Chou, 1978) and NNO þ 05(05 log unit magmas from Santorini are true fractionates, a small above the Ni–NiO buffer; Pownceby & O’Neill, 1994) for part of them fall off the main fractionation trend (Fig. 1d mafic to silicic compositions (Barton & Huijsmans, and e): such magmas are depleted in FeO* and TiO2 1986; Cottrell et al., 1999; Gertisser et al., 2009; Cadoux and have calc-alkaline affinities compared with the FC li- et al., 2014; Druitt, 2014; Andujar et al., 2015). quids. The petrology and geochemistry of these prod- ucts indicate that such magmas are hybrid products Liquid line of descent and melt evolution at from the mixing between mafic and silicic melts (e.g. Santorini Cape Riva andesite and dacite, Upper Therasia andes- Petrological and geochemical studies have already ite; Fabbro et al., 2013). shown that the main mechanism of magma evolution at Because we use the USC-1 andesite as the starting Santorini is fractional crystallization (FC; Nichols, 1971a; material for our crystallization experiments, the pres- Barton et al., 1983; Mann, 1983; Huijsmans et al., 1988; ence of 15 wt % of xenocrystic material and its effect Huijsmans & Barton, 1989; Druitt et al., 1999; Michaud on phase equilibria need to be assessed. The USC-1 et al., 2000; Zellmer et al., 2000). This process defines a bulk composition (Table 1) is shown in Fig. 1d and e liquid line of descent (LLD) for Santorini magmas that is along with a typical fractionation trend and andesites of characterized by enrichment in FeO*, TiO2 and P2O5 mixed origin. The USC-1 rock plots clearly at the TiO2 during the early stages; these elements reach peak val- and FeO* enrichment peak, far away from the field ues at 55–60 wt % SiO2 (Fig. 1d and e). This trend results defined by hybrid andesites (Fig. 1d and e; Cape Riva from the fractionation of Ol, Cpx, Pl (6 Mt), which gen- and Therasia; Fabbro et al., 2013). This observation con- erates liquids with a tholeiitic character (Miyashiro, firms that our starting material is close to a ‘true’ fractio- 1974; Druitt et al., 1999). The onset of magnetite and nated liquid, and not a hybrid andesite. 1892 Journal of Petrology, 2016, Vol. 57, No. 10

(e.g. Scaillet & Evans, 1999). The stability field of Qz is ilm loosely constrained, as this phase has been identified in pl only one experimental charge at 200 MPa; this shows that Qz crystallization is restricted to 900C and Mt H2Omelt < 5wt%. gl At 400 MPa, liquidus conditions are attained at 1000 C and 9 wt % H2Omelt (Fig. 3b). At this temperature, Mt and Cpx crystallize between 8 and 9 wt % H2Omelt, Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 whereast Pl and Opx appear at H2Omelt < 7wt %. At temperatures <985C, the Pl-in curve is shifted towards

opx higher H2Omelt (8–85 wt %), whereas Opx is not stable cpx at H2Omelt > 7wt%(Fig. 3b). The Ilm stability field has a shape similar to that observed at 200 MPa, with an 20 m upper thermal limit at 960 C, but is stable at higher H2Omelt up to 7 wt % at 400 MPa. Amph is stable at <930C, and in the H O range 7–9 wt %. At lower Fig. 2. Backscattered electron image of charge usc53 (950 C, 2 melt 200 MPa, fO2 NNO þ 15) containing 53 wt % of plagioclase H2Omelt Amph breaks down to Cpx, Opx, Mt and Ilm, (pl), clinopyroxene (cpx), orthopyroxene (opx), magnetite (Mt), being involved in a similar reaction relationship to the ilmenite (ilm) and glass (gl). The high degree of crystallization, one at 200 MPa. Qz crystallizes at 400 MPa and H O the small size of the crystals and the presence of glass pools 2 melt should be noted. < 4 wt % over the investigated temperature range (Fig. 3b; Table 2). At 100 MPa, and for the two explored temperatures EXPERIMENTAL APPROACH AND ANALYTICAL (975–1000C), Cpx, Mt and Pl co-crystallize at water-

TECHNIQUES saturated conditions (5wt%H2Omelt), whereas Opx Details concerning the starting material and capsule appears when H2Omelt is slightly decreased (Fig. 3e preparation, as well as the experimental equipment and and f). analytical conditions used in this work, are provided in the Supplementary Data (available for downloading at Phase relationships at reducing conditions http://www.petrology.oxfordjournals.org). (fO2 QFM) A decrease in fO2 does not affect the mineral assem- RESULTS blage found under more oxidizing conditions (Cpx þ Identified phases in the run products of both oxidized Opx þ Plag þ Mt þ Ilm þ Amph). Qz has not been identi- (NNO þ 15) and reduced (NNO – 05) experiments in- fied, but its presence can be anticipated in the H2O-poor clude glass (Gl), Cpx, Opx, Mt, Pl, Ilm, amphibole part of the diagram by analogy with what is observed at (Amph), apatite (Ap) and quartz (Qz) (Fig. 2). The experi- NNO þ 15. At 200 and 400 MPa, the first appearance of mental results are listed in Table 2 and displayed as a all phases occurs over a narrower H2Omelt region com- series of isobaric–polythermal (Fig. 3a–d) or isother- pared with NNO þ 15, in the water-rich part of the dia- mal–polybaric sections (Fig. 3e and f) showing the ef- gram (>6to8wt%H2Omelt depending on pressure; Fig. fects of T, P,H2O content and fO2 on phase 3c and d); the boundary curves have steeper slopes or relationships. The effects on melt compositions are are almost vertical. Mt still appears at the liquidus, but shown in Figs 4–10. We present the experimental re- Ilm stability is expanded towards higher temperatures sults depending on the prevailing fO2 (NNO þ 15or (1000 C), whereas Opx and Pl co-crystallize at 6 wt % QFM) and the range of temperatures 1000–975 C, 950– H2Omelt. Amph is unaffected by the decrease in fO2 900C. from NNO þ 15 to QFM, with an upper thermal limit at about 930 C; it appears at > 6wt% H2Omelt (Fig. 3c). At Phase relationships under oxidizing conditions 400 MPa, the decrease in fO2 decreases the liquidus (fO2 NNO 1 15) temperatures to 980 C, and the crystallization sequence At 200 MPa and 1000 C, Mt is the liquidus phase at is affected in the following ways: (1) Cpx becomes the water saturation (H2Omelt 66wt%;Table 2), and is sub- liquidus phase; (2) Ilm is shifted towards higher tem- sequently joined by Cpx, Opx and Pl (Fig. 3a). At 975C peratures and water contents, appearing with Opx at the stability of Pl and Opx moves towards higher water 7wt % H2Omelt and 1000 C(Fig. 3d); (3) Mt and Pl are contents (6 wt %). Ilm crystallizes only at temperatures displaced toward lower H2Omelt compared with NNO þ of 960 C and at H2Omelt 6 wt %. Amph crystallizes 15 conditions, Pl being the last mineral to appear in the at 930 C in the H2Omelt 6 wt % part of the sequence (Fig. 3d); (4) Amph is stable at < 950 C and diagram (Fig. 3a), being in a broad reaction relationship H2Omelt > 8 wt %, being again in a reaction relationship with Opx, as observed in other experimental studies with Opx and Pl at lower water contents. Table 2: Experimental run conditions and results Petrology of Journal

a b Run XH2Oin fH2OH2Omelt H2O log fO2 DNNO DQFM Phase assemblage P (mole %) (bar) (mole %) (mole %) (bar) Mt Ilm Cpx Opx Pl Amph Qz Ap Crystal Gl r2 Pl/Opx

Oxidized experiments 1000 C, 200 MPa; 91 h; fH2(bar): 245 –880 153 usc62 100 1940 660 764 –876 153 4 40960011 usc63 075 1446 575 725 –902 127 4357100900015 10 No. 57, Vol. 2016, , usc64 052 1007 485 –933 096 X X X usc65 036 703 410 456 –965 065 558916241401599017 151 usc66 010 194 224 360 –1076 –047 X X X X 975 C, 200 MPa; 435h;fH2(bar): 223 –915 156 usc32 100 1940 660 537 –910 158 175471929012 usc33 071 1378 562 447 –940 128 1754058 48125875003 83 usc34 058 1123 511 369 –958 110 338214167296704003 119 usc35 031 592 378 231 –1013 055 X X X X X usc36 010 194 224 231 –1110 –042 X X X X X 950 C, 200 MPa; 755h;fH2(bar): 322 –991 120 usc52 100 1940 660 660 –985 122 6510615344530470018 229 usc53 072 1391 565 445 –1014 093 63015 1231932 527474011 168 usc54 050 976 478 203 –1045 062 6 062 14819446679321037 235 usc55 030 588 377 –1089 018 X X X X X X usc56 010 194 224 –1185 –078 X X X X X X 925 C, 200 MPa; 51 h; fH2(bar): 303 –1039 113 usc42 100 1902 654 523 –1027 122 58641102 55 trace 287713009 usc43 067 1283 544 378 –1061 088 6 04119091 396588412017 435 usc44 047 901 461 –1092 057 X X X X X X usc45 030 564 370 –1132 017 X X X X X X usc46 010 190 222 –1227 –078 X X X X X X 900 C, 200 MPa; 115 h; fH2(bar): 215 –1049 120 usc57 100 1902 654 –1044 149 X X X X usc58 084 1596 602 –1059 134 X X X X usc59 069 1321 551 –1075 117 X X X X X X usc60 062 1174 522 –1086 107 X X X X X X usc61 052 989 481 –1101 092 X X X X X X X 1000 C, 400 MPa; 88 h; fH2(bar): 740 –908 124 usc67 100 4116 939 1026 –907 118 00 1000 usc68 070 2875 794 509 –938 087 012728972028 usc69 053 2198 700 546 –962 064 062733967009 usc70 029 1196 526 541 –1015 011 2 8821197326674009 94 usc71 010 412 319 377 –1107 –082 1913233335519481017 102 975 C, 400 MPa; 435h;fH2(bar): 442 –906 165 usc37 100 4051 932 855 –906 158 131398705 usc38 070 2833 788 469 –937 127 1893111889008 usc39 049 1983 667 426 –968 096 3 10431107272728015 35 usc40 029 1177 522 392 –1013 051 5 845 3925764240178 usc41 010 405 317 –1106 –042 X X X X X X 950 C, 400 MPa; 94 h; fH2(bar): 596 –977 134 usc77 100 3959 922 814 –977 127 5457111889025 usc78 047 1880 650 299 –1042 062 57081 13324391613387013 163

usc79 048 1915 656 –1040 064 X X X X X X 1893

(continued) Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 December 14 on user ISTO - CNRS by https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 from Downloaded Table 2. Continued 1894 a b Run XH2Oin fH2OH2Omelt H2O log fO2 DNNO DQFM Phase assemblage P (mole %) (bar) (mole %) (mole %) (bar) Mt Ilm Cpx Opx Pl Amph Qz Ap Crystal Gl r2 Pl/Opx usc80 029 1166 520 –1083 021 X X X X X X usc81 010 396 313 –1177 –073 X X X X X X X 925 C, 400 MPa; 50 h; fH2(bar): 733 –1039 113 usc82 100 3849 910 828 –1042 103 4708136191809023 usc83 083 3199 834 611 –1058 087 3338104154329671004 usc84 068 2626 761 597 –1076 070 524522614 463537004 usc85 054 2067 680 574 –1096 049 531112663458711289033 73 usc86 035 1329 553 –1135 010 X X X X X 1000 C, 100 MPa; 43 h; fH2(bar): 075 –837 196 usc72 100 898 460 406 –841 191 515267170830033 usc73 073 656 397 375 –868 163 55718158301699008 88 usc74 052 467 338 217 –897 134 69862532950949103132 usc75 042 375 306 217 –916 115 6511816481680320018 301 usc76 010 90 156 –1041 –009 975 C, 100 MPa; 645h;fH2(bar): 072 –875 196 usc57b 100 898 460 671 –879 191 5665811 202798013 usc58b 070 625 388 –910 159 X X X X X usc59b 041 371 304 424 –956 114 X X X X X usc60b 027 239 247 –994 076 X X X X X usc61b 010 90 156 –1079 –009 Reduced experiments 1000 C, 200 MPa; 48 h; fH2(bar): 1314 –1022 –007 062 usc27 100 1940 660 748 –1022 007 062 0909991028 usc28 070 1363 559 538 –1053 –024 032 18068 742211 231769008 usc29 051 984 480 508 –1081 –052 003 X X X X X X usc30 031 610 384 410 –1123 –094 –038 X X X X X X usc31 010 194 224 –1222 –193 –138 X X X X X X 975 C, 200 MPa; 525h;fH2(bar): 5360 –1191 129 –069 usc1 100 1940 660 665 –1186 –119 –064 020810990002 usc16 091 1758 630 –1195 –127 –072 X trace X usc17 082 1583 600 –1204 –136 –081 X trace X X X usc2 068 1325 552 342 –1219 –152 –097 22014 77323 176309691002 Petrology of Journal usc3 051 984 480 308 –1245 –178 –123 21012 6342208335665008 usc4 033 639 392 171 –1283 –215 –160 X X X X X X usc5 010 194 224 149 –1386 –319 –264 X X X X X X 925 C, 200 MPa; 49 h; fH2(bar): 1058 –1141 004 062 usc6 100 1902 654 –1135 014 067 1812124154846052 usc21b 093 1768 632 –1142 007 061 X X X X usc22b 081 1546 593 –1153 –004 049 X X X X X usc7 072 1373 561 –1164 –015 039 X X X X X X 06 o.5,N.10 No. 57, Vol. 2016, , usc8 048 915 464 –1199 –050 004 X X X X X X usc9 036 681 404 –1225 –076 –022 X X X X X X usc10 010 190 222 –1335 –186 –133 X X X X X X 1000 C, 400 MPa; 68 h; fH2(bar): 3332 –1039 –016 046 usc22 100 4116 939 720 –1038 –012 047 00 1000 usc23 070 2894 796 431 –1068 –043 016 X X usc24 053 2173 696 –1093 –068 –009 X X

(continued) Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 December 14 on user ISTO - CNRS by https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 from Downloaded ora fPetrology of Journal 06 o.5,N.10 No. 57, Vol. 2016, , Table 2. Continued a b Run XH2Oin fH2OH2Omelt H2O log fO2 DNNO DQFM Phase assemblage P (mole %) (bar) (mole %) (mole %) (bar) Mt Ilm Cpx Opx Pl Amph Qz Ap Crystal Gl r2 Pl/Opx usc25 029 1180 523 240 –1146 –121 –062 22019 74088 114221779002 usc26 010 412 319 210 –1238 –212 –153 X X X X X X 975 C, 400 MPa; 4585 h; fH2(bar): 3822 –1094 –032 029 usc11 100 4051 932 849 –1093 –029 029 00 1000 usc18 093 3765 901 –1099 –035 023 trace X usc19 082 3322 849 –1110 –046 012 X X X X X usc12 071 2871 793 613 –1123 –059 000 21017915135251749011 usc13 059 2393 728 539 –1139 –075 –016 28014 9 12237368632013 usc14 029 1194 526 –1199 –135 –077 X X X X X X usc15 010 405 317 –1293 –229 –171 X X X X X X 925 C, 400 MPa; 544h;fH2(bar): 5996 –1222 –077 –020 usc87 100 3849 910 941 –1225 –080 –022 28018 28846 142858016 usc88 085 3268 843 722 –1239 –094 –036 32078 581025 200800019 usc89 072 2769 780 600 –1254 –108 –051 4 024 1055330150149901 usc90 054 2092 684 595 –1278 –133 –075 X X X X X

XH2Oin, initial H2O/(H2O þ CO2) in the charge (in moles). H2Omelt , water content in the melt: adetermined by the solubility model of Papale et al. (2006) and using the method of Scaillet & Macdonald (2006); b determined by difference method (see text for details). fH2, hydrogen fugacity of the experiment determined by using NiPd or CoPd alloy sensors. log fO2, logarithm of the oxygen fu- gacity calculated from the experimental fH2. DNNO – DQFM is log fO2 – log fO2 of the NNO or QFM buffer calculated at P and T (NNO, Pownceby & O’Neill, 1994; QFM, Chou, 1978). Crystal, numbers indicate the phase abundance in the charge in weight per cent. Mt, magnetite; Ilm, ilmenite; Cpx, clinopyroxene; Opx, orthopyroxene; Pl, plagioclase; Amph, amphi- bole; Qz, quartz; Ap, apatite; Gl, glass; Pl/Opx, plagioclase (wt %)/orthopyroxene (wt %) in the charge. Trace, phase with a modal abundance <01 wt %. X, mineral phase identified with SEM.

1895 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 December 14 on user ISTO - CNRS by https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 from Downloaded 1896 ora fPetrology of Journal

Fig. 3. Phase relationships of the Upper Scoriae 1 andesite at (a) 200 MPa and fO2 NNO þ 15, (b) 400 MPa and fO2 NNO þ 15, (c) 200 MPa and fO2 QFM, (d) 400 MPa and fO2 QFM, (e) 1000 C and fO2 NNO þ 15, and (f) 975 C and fO2 NNO þ 15 for various temperatures, pressures and water contents in the melt. L, liquid; Pl, plagioclase; Cpx, clinopyr- oxene; Opx, orthopyroxene; Amph, amphibole; Mt, magnetite; Ilm, ilmenite; Qz, quartz. Dashed lines are estimated crystal content boundaries (in wt %). Grey field in (a) and (b)

shows the coexistence region of the natural mineral assemblage and 28 wt % of crystals in the andesite. 10 No. 57, Vol. 2016, , Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 December 14 on user ISTO - CNRS by https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 from Downloaded Journal of Petrology, 2016, Vol. 57, No. 10 1897

Crystal contents and phase proportions of agreement with previous studies on hydrous basaltic–an- experimental charges desitic compositions (Table 3; Baker & Eggler, 1987; The proportion of solid phases increases in a general Sisson & Grove, 1993; Pichavant et al., 2002; Berndt et al., way with decreasing H2Omelt (at constant pressure), 2005; Grove et al., 2005; Di Carlo et al., 2006). decreasing temperature (at constant H2Omelt) and Pl compositional changes as a function of tempera- increasing pressure (at constant temperature and ture, H2Omelt, per cent crystals and fO2 have been para- H2Omelt; Supplementary Data crystal appendix). The meterized using a linear least-squares fitting procedure. highest value that we could determine by mass-balance We have not considered adding a pressure term to this calculation (71 wt %) is reached at 925C, 400 MPa, NNO equation because of the limited range of P variation Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 þ 15 and 7 wt % H2Omelt. A decrease in fO2 from NNO covered in this work. The following empirical equation þ 15 to QFM at constant temperature, pressure and has been derived: H2Omelt decreases the crystal content (975 C, 200 MPa series; Supplementary Data crystal appendix; Table 2). Anðmol %Þ¼0 006T ð CÞ –0 7H2Omelt þ 2 72DNNO Mt and Cpx proportions increase slightly with decreas- –0 32ðwt % crystalsÞþ60 22 ing H2Omelt or temperature to a maximum of 20 wt % (1) (Table 2). Pl rapidly becomes the dominant mineral for which R2 ¼ 091 (see Supplementary Data Appendix when present (Table 2). Opx and Ilm appear in lower Equations). amounts compared with Cpx and Mt (on average <3wt Equation (1) can be used to allow back-calculation of % for Opx and <1 wt % for Ilm). Under oxidizing condi- experimental An contents to within 615 mol %. Owing tions and similar H O contents, the proportion of 2 melt to its empirical nature, we caution the use of such an Amph depends on pressure: charges annealed at equation on compositions significantly different from 200 MPa have about 5 wt % Amph compared with >13 wt % at 400 MPa (Table 2). Charges annealed at that of the USC-1 sample. Equation (1) (and those fol- lowing) is applicable in the range 1000–900 C, H2Omelt similar T, P and H2Omelt but lower fO2 crystallize less Mt and more Cpx and Opx, whereas the Pl proportion re- 10 to 1 wt % and fO2 NNO þ 15 to QFM. mains almost constant when compared with more oxi- dized runs. Clinopyroxene Mineral compositions Experimental Cpx is either augite or diopside according Plagioclase to the classification of Morimoto (1989) with compos- The compositional variation of Pl (An mol %, Or mol %) itions in the range En37–47Fs13–39Wo17–48, Mg#49–77, with TiO2 and Al2O3 contents in the range 04–17wt% as a function of H2Omelt and temperature is shown in Fig. and 13–8 wt %, respectively (Table 4, Fig. 5; 4. Pl composition is in the range An37–70Ab30–55Or04–94 (Table 3), being mostly affected by changes in tempera- Supplementary Data Appendix cpx). Cpx composition varies with changes in experimental parameters, and ture, H2Omelt, and pressure. The most calcic Pl (An70)is hence with crystal content and melt composition. At produced at 925 C, 200 MPa, 65wt%H2Omelt, whereas the least calcic Pl (An37)isproducedat950C, 400 MPa, constant temperature a decrease in H2Omelt from 6 to 5wt % H2Omelt, both under oxidizing conditions. At a 3 wt % decreases the Mg# and Wo by about 10%. given pressure, the An content decreases and Or content Similar changes are produced by an increase in pres- increases with the decrease in H2Omelt and temperature sure from 200 to 400 MPa or by an fO2 decrease from (Fig. 4), mirroring the decrease of the CaO/K2Oratioofthe NNO þ 15 to QFM. In contrast, changes in temperature coexisting melt as crystallization proceeds (see below). at constant pressure have smaller effects (<5 mol %), The effect is well illustrated by the experimental series an- except when temperature decreases from 950Cto nealed at 200–400 MPa and oxidizing conditions in which 900C(>15 mol % in series at 200 MPa, NNO þ 15). a decrease of 2 wt % H2Omelt or a change in temperature Overall, Cpx becomes progressively poorer in Al2O3 from 1000–975 C to 950–925 C decreases by 10–15 mol % and TiO2 when H2Omelt decreases (i.e. with increase in the An content of Pl (Fig. 4). At fixed temperature increas- crystallization) and with decreasing fO2 (Supplementary Fe/Mg ing either H2Omelt or fO2, or decreasing pressure, all in- Data appendix cpx). The Kd of Cpx–liquid pairs crease the An content. For example, in the series ranges between 012 and 026 (average 022 6 005), annealed under oxidizing conditions, 1000–975Candfor again in agreement with previous experimental studies H2Omelt of 4–5 wt %, the An content increases from An47 conducted on similar compositions (Table 4; Pichavant to An68 when pressure decreases from 400 to 100 MPa. et al., 2002; Berndt et al., 2005; Di Carlo et al., 2006). Changes in fO2 produce modest compositional variations The variation of Wo content with experimental condi- of Pl compared with those of pressure: a decrease in fO2 tions can be parameterized using a linear least-squares from NNO þ 15 to QFM at a given pressure and H2Omelt procedure on the entire experimental database: decreases An content by about 5 mol % (Fig. 4). The Pl–li- quid Ca–Na exchange K varies between 019 and 321 Woðmol %Þ¼–00075T ð CÞþ136H2Omeltðwt %Þþ d (2) with an average value of 178 (6 07), being in good 376DNNOþ3516 1898 Journal of Petrology, 2016, Vol. 57, No. 10 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018

Fig. 4. Compositional variation of the experimental plagio- Fig. 5. Compositional variation of experimental clinopyrox- enes. (a) Mg# and (b) Wo content of clinopyroxenes as func- clase. (a) An content (mol %) vs H2Omelt (wt %); (b) Or content (mol %) vs H O (wt %). Numbers next to symbols in the le- tions of melt H2O. Numbers next to symbols in the legend 2 melt gend indicate temperature (C) and pressure (MPa) at specified indicate temperature ( C) and pressure (MPa) at specified fO2 conditions. Grey box represents the clinopyroxene compos- fO2 conditions. Grey box indicates the plagioclase composition of the natural andesite phenocrysts and dashed grey box indi- ition of the natural andesite phenocrysts and dashed grey box cates that for the dacite xenocrysts [see text for details, and indicates that for the dacite xenocrysts [see text for details, and Andujar et al. (2015)]. Andujar et al. (2015)]. for which R2 ¼ 086 (Supplementary Data Appendix The variation of H2Omelt significantly affects Opx com- Equations). position: for instance, a decrease of 2 wt % H2Omelt de- Equation (2) can be used to back-calculate observed creases by 5–8 mol % the Mg# (and the Fs component) Wo contents to within 608 mol %. whereas the Wo content is slightly affected (Fig. 6a). Compositional changes owing to temperature variation Orthopyroxene are modest in the range 1000–950C, but more import- According to the classification of Morimoto (1989) ant below 950C: Mg# and En decrease by 5–15 mol % experimental Opx is clinoenstatite–pigeonite with com- when temperature decreases from 950 to 900 C(Fig. 6). positions in the range En51–71Fs24–44Wo35–16, Mg#49– In addition to temperature and water content effects, 75, with 1–5 wt % Al2O3 and 02–06 wt % TiO2 (Table 5). our results show that Opx composition is sensitive to Journal of Petrology, 2016, Vol. 57, No. 10 1899 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018

Fig. 6. Compositional variation of experimental orthopyrox- enes. (a) Mg# and (b) Wo content of orthopyroxenes as a func- tion of melt H2O. Numbers next to symbols in the legend indicate temperature ( C), pressure (MPa) and fO2 conditions. Grey box represents the orthopyroxene composition of the natural andesite phenocrysts and dashed grey box indicates that for the dacite xenocrysts [see text for details, and Andujar et al. (2015)]. pressure variation at oxidizing conditions; for a constant

H2Omelt and fixed temperature the increase in pressure from 100 to 400 MPa increases Mg# and the En content by about 15–20 mol %. The change in fO2 from NNO þ 15 to QFM produces compositional changes similar to those of H2Omelt, in particular at 200 MPa. The effect of Fig. 7. Compositional variation of experimental magnetites. (a) experimental parameters on Wo content (and Al2O3 and Mg# and (b) TiO2 (wt %) content as function of melt H2O. (c) TiO (wt %) content as a function of Mg# of magnetite. The TiO2, not shown) is small, with most Opx clustering in 2 grey square shows the magnetite population found in the USC- the range Wo4–6. The Opx–liquid Fe/Mg exchange Kd 1 andesite sample. varies between 011 and 029 (Table 5) and has an aver- age value of 021 6 005.

Magnetite and ilmenite do affect Mt composition. A decrease in temperature Mt has a FeO* content between 59 and 79 wt % and a and fO2 produces moderate variations of Mg# and TiO2

TiO2 content from 5 to 19 wt % (Table 6). The Mg# [cal- content (2–4%). The effect of H2Omelt is significant as culated as Mg# ¼ 100Mg/(Mg þ Fetot) on a stoichiomet- well: a decrease of 3 wt % H2Omelt at constant tempera- ric basis] varies between 35 and 9% (Table 6; Fig. 7). As ture decreases Mg# by 5% and increases TiO2 up to for other phases, changes in experimental parameters 12 wt % (e.g. series at 1000C, 200 MPa and 950C, 1900 Journal of Petrology, 2016, Vol. 57, No. 10 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018

Fig. 8. (a–i) Experimental glass compositional variations of major and minor oxides and FeO*/MgO with water content in the melt. Grey horizontal bar shows the natural USC-1 andesite calculated melt composition (Table 1).

400 MPa; Fig. 7). At fixed T,H2Omelt and fO2, a pressure Equation (3) allows back-calculation of observed increase from 100 to 400 MPa decreases the Mg# by Mg# in magnetites to within 607.

2–4%. The effect on TiO2 content is less clear compared Ilm was identified by scanning electron microscope– with that on Mg# (Fig. 7). energy-dispersive spectrometry (SEM-EDS) in several We have linearly regressed the compositional vari- charges but was often too small to obtain reliable com- ations of Mg# in magnetite with T,H2Omelt, crystal con- positions by electron microprobe. Nevertheless, we tent (wt %) and fO2, and obtained the following analysed Ilm in seven charges annealed at QFM (Table empirical equation: 7). Their FeO* and TiO2 contents are in the range 40– 45 wt % and 48–50 wt %, respectively. The limited Mg# ðmol %Þ¼0 027T þ 0 28H O ðwt %Þ magnetite 2 melt amount of data prevents quantification of the effect of –0 024 wt % crystals ð Þ experimental parameter variation on Ilm composition. þ 0 40DNNO – 20 62 (3) Amphibole for which R2 ¼ 082 (see Supplementary Data Appendix According to the classification of Leake et al. (1997), ex- Equations). perimental Amph is ferro-tschermakite to pargasitic Journal of Petrology, 2016, Vol. 57, No. 10 1901 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018

Fig. 9. (a) Compositions of clinopyroxenes and orthopyroxenes of USC-1 (Andujar et al. 2015; this work) and those from runs at fO2 NNO þ 15, 1000–975 C, and 100, 200 and 400 MPa plotted onto the classification scheme of Morimoto (1989); tie-lines for the main cpx–opx populations from the andesite are shown. (b) Compositions of plagioclase of USC-1 (Andujar et al., 2015, this work) and those from experiments plotted using the classification scheme of Deer et al. (1972). (c) Crystal content as a function of plagio- clase/orthopyroxene ratio (Pl/Opx) of experiments reproducing the crystal content and mineral assemblage (a, b) of the natural an- desite (white star).

hornblende. Its Mg# (calculated with FeO*) shows lim- boundary (e.g. charges usc30, usc34) based on the crite- ited variability with changes in H2Omelt, fO2 or pressure ria of Le Bas & Streckeisen (1991). The observed melt (Table 8; Supplementary Data Amphibole Appendix). evolution arises obviously from changes in phase as- Similarly, Amph crystallizing at 400 MPa has an Al(IV) semblages, proportions and compositions: mostly Fe– content comparable with, or slightly higher than, that at Mg minerals (Cpx–Opx mainly and Mt) and Pl, as well 200 MPa, showing that any pressure effect on Amph as the incipient crystallization of Amph or Ilm at lower composition is minor in the 200–400 MPa interval. temperatures (950–925C). The experimental trends re- produce the typical evolution of arc andesites (Table 2; Residual glass Martel et al., 1999; Pichavant et al., 2002; Almeev et al., Experimental glasses (Table 9) range from andesitic 2013). In detail, glass composition varies mostly with

(585 wt % SiO2) to dacitic (63–68 wt % SiO2) to rhyoda- H2Omelt (or increasing crystal content), and less so with citic (up to 72 wt % SiO2) compositions, with some T, P and fO2 (Fig. 8): a decrease of 3–4 wt % H2Omelt de- charges straddling the –trachydacite creases TiO2, Al2O3, FeO*, MgO and CaO content by 1902 ora fPetrology of Journal 06 o.5,N.10 No. 57, Vol. 2016, ,

Fig. 10. (a, b) FeO*/MgO and (c, d) TiO2 vs SiO2, and tholeiitic and calc-alkaline affinities of Santorini magmas (silicic- and intermediate-dominated compositions); (e, f) MgO vs SiO2

(wt %) of Santorini magmas and experimental melts at fO2 QFM and NNO þ 15. Natural rock data from Druitt et al. (1999). Errors are equal to symbol size. Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 December 14 on user ISTO - CNRS by https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 from Downloaded Journal of Petrology, 2016, Vol. 57, No. 10 1903

Table 3: Experimental plagioclase composition (wt %)

Ca–Na Run n SiO2 TiO2 Al2O3 MgO CaO MnO FeO* Na2OK2O Sum An Ab Or Kd Oxidized experiments 1000 C, 200 MPa usc65 1 5543 008 2580 016 1000 000 107 505 036 9795 5111 4670 219 019 975 C, 200 MPa usc32 usc33 1 5360 005 2842 010 1213 003 118 432 014 9995 6031 3886 083 163 usc34 1 5507 019 2638 026 1062 000 105 425 030 9811 5689 4120 191 195 950 C, 200 MPa Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 usc53 2 5749 025 2643 021 879 004 138 473 067 10000 4846 4716 438 229 SD 040 004 008 001 006 004 013 007 005 076 068 040 028 usc54 1 6137 024 2043 048 646 000 166 446 114 9625 4066 5077 857 206 925 C, 200 MPa usc42 3 5013 005 2946 018 1393 005 070 339 011 9800 6898 3038 063 322 SD 039 002 047 018 072 005 017 007 002 069 146 152 014 usc43 1 5743 021 2382 047 795 000 174 457 083 9703 4616 4807 577 279 1000 C, 400 MPa usc70 1 5604 015 2635 010 955 000 116 575 032 9943 4697 5118 185 088 975 C, 400 MPa usc39 1 5822 033 2596 013 903 057 096 456 024 10000 5142 4695 163 148 usc40 1 6035 029 2379 054 889 005 027 501 080 10000 4702 4795 504 155 950 C, 400 MPa usc78 2 5869 019 2427 025 777 006 129 569 067 9790 4117 5460 423 106 SD 042 011 089 016 028 009 019 001 001 035 097 082 015 usc79 1 6059 014 2084 027 625 003 183 492 132 9620 3737 5325 938 usc80 1 6085 032 2130 028 643 008 149 518 121 9713 3730 5435 835 925 C, 400 MPa usc83 1 5857 009 2503 010 963 000 080 486 040 9948 5095 4653 252 152 usc84 1 5861 007 2669 005 1019 000 096 524 026 10207 5100 4745 155 177 usc85 1 6102 021 2461 007 807 011 115 570 041 10135 4276 5465 259 136 1000 C, 100 MPa usc72 1 5179 003 2982 004 1318 000 102 370 006 9965 6606 3356 038 211 usc74 1 5792 004 2601 014 1094 000 097 392 022 10015 5980 3879 141 267 usc75 1 5956 029 2323 047 774 000 189 456 084 9858 4556 4854 590 277 Reduced experiments 1000 C, 200 MPa usc28 1 5324 026 2981 025 1245 017 008 338 035 10000 6558 3225 217 252 975 C, 200 MPa usc2 2 5604 002 2724 084 1085 011 005 510 030 10055 5310 4516 175 136 SD 185 000 093 003 023 002 014 025 002 208 065 061 004 usc3 3 5554 024 2515 041 989 007 181 503 046 9861 5063 4654 283 125 SD 097 013 114 007 050 004 038 027 007 079 018 036 053 1000 C, 400 MPa usc25 1 5534 029 2574 030 966 000 120 482 042 9777 5113 4620 267 135 usc26 1 5715 013 2656 033 925 004 104 553 041 10044 4685 5071 244 143 975 C, 400 MPa usc12 1 5653 016 2676 051 959 004 174 489 045 10067 5053 4665 282 137 usc13 1 5768 030 2514 041 799 001 170 462 064 9849 4667 4885 447 132 925 C, 400 MPa usc89 2 5808 021 2449 022 909 004 102 445 052 9811 5118 4535 347 257 SD 110 001 059 007 016 005 004 022 001 125 069 088 020 n, number of analysis; SD, standard deviation. FeO*, total iron reported as FeO. An ¼ 100Ca/(Ca þ Na þ K); Ab ¼ 100Na/(Ca þ Na þ Ca–Na K); Or ¼ 100K/(Ca þ Na þ K). End-members calculated as done by Deer et al. (1972). Kd ¼ (Ca/Na in plagioclase)/(Ca/Na in melt).

about 20–50% relative, whereas both SiO2 and K2O in- is related to the onset of ilmenite crystallization and the crease (Fig. 8). Na2O displays a different behaviour increase in the modal proportion of plagioclase (Fig. 3; compared with other oxides, first increasing until Table 2), which accelerates and enhances subsequent

H2Omelt reaches 6 wt %, then decreasing upon further melt evolution. An increase in pressure from 100 to reduction of H2Omelt (Fig. 8g). Glasses from charges an- 400 MPa at constant temperature produces moderate nealed either in the range 1000–975C or in the range changes in melt composition, of the order of 1–2 wt % 950–925C define two distinct trends (Fig. 8). The com- on major oxides. However, a larger pressure effect on positional differences between these two groups are melt composition is apparent when the FeO*/MgO ratio clear for SiO2, TiO2, FeO*, MgO and CaO oxides, being is considered (with an average precision of 6 05; Table less pronounced for Na2O, K2O and Al2O3 (5–10% rela- 9). Glasses at 100 MPa have the lowest ratios, and those tive). This thermal and compositional divide at 965C at 400 MPa the highest, whereas those at 200 MPa plot 1904 Journal of Petrology, 2016, Vol. 57, No. 10

Table 4: Composition of experimental clinopyroxenes (wt %)

Fe –Mg n SiO2 TiO2 Al2O3 MgO CaO MnO FeO* Na2OK2O Total En Fs Wo Mg# Kd * Oxidized experiments 1000 C, 200 MPa usc63 3 4750 143 536 1367 1995 046 884 037 004 9761 4114 1492 4315 7339 026 SD 038 005 013 005 010 004 039 011 005 027 006 058 045 079 usc64 1 4730 122 454 1424 1857 032 984 056 006 9664 4277 1658 4010 7206 usc65 1 5022 064 235 1571 1879 067 1160 002 000 10000 4352 1803 3740 7071 018 975 C, 200 MPa usc32 3 5102 066 368 1487 1950 034 938 046 012 10001 4328 1532 4084 7385 018 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 SD 052 010 116 094 060 013 046 015 010 075 068 044 078 076 usc33 4 5078 077 343 1544 1940 042 1055 036 002 10118 4344 1666 3924 7228 018 SD 010 010 021 030 060 007 025 011 003 067 075 047 108 037 usc34 3 5160 077 397 1441 1818 047 1222 063 014 10239 4165 1982 3776 6776 021 SD 039 035 075 041 035 019 038 014 007 050 052 093 012 129 950 C, 200 MPa usc52 1 5265 048 293 1524 1709 094 1027 047 006 10012 4507 1704 3632 7257 018 usc53 1 5278 044 300 1390 1923 045 1017 003 000 10000 4128 1694 4103 7091 019 usc54 2 5188 049 288 1471 1577 075 1328 024 000 10000 4338 2198 3339 6641 017 SD 039 003 033 007 178 016 087 007 000 000 079 193 301 156 925 C, 200 MPa usc43 1 5036 057 276 1505 1827 088 1217 000 000 10000 4239 1923 3698 6879 017 900 C, 200 MPa usc61 1 4880 096 130 1247 1163 073 1987 020 005 9601 3850 3441 2581 5280 1000 C, 400 MPa usc68 3 4888 111 474 1383 1851 050 1088 056 005 9905 4125 1822 3969 6937 024 SD 061 009 028 038 066 004 030 007 002 047 045 086 064 118 usc69 2 4900 090 456 1363 1863 040 1103 057 006 9879 4074 1851 4006 6877 026 SD 009 003 003 031 014 022 047 000 003 048 052 059 072 042 usc70 1 5027 079 353 1335 1562 025 1351 052 004 9788 4132 2347 3477 6377 034 usc71 2 4974 071 210 1217 1029 080 2235 027 007 9849 3738 3852 2271 4925 024 SD 042 008 023 033 046 012 028 008 001 092 076 021 118 037 975 C, 400 MPa usc38 1 4876 082 521 1301 1948 033 924 054 007 9746 4019 1600 4323 7152 018 usc39 1 5034 068 276 1386 1898 048 1290 000 000 10000 3959 2066 3896 6571 015 950 C, 400 MPa usc77 3 4899 096 422 1420 2098 020 778 046 006 9785 4207 1293 4467 7650 025 SD 045 013 011 014 017 018 050 003 006 038 027 063 068 098 usc78 3 5150 061 586 1244 1603 075 1102 122 015 9959 4068 2020 3773 6682 016 SD 076 008 258 096 082 024 118 080 004 089 002 060 097 065 925 C, 400 MPa usc82 2 5235 058 270 1331 2189 042 971 036 003 10134 3833 1568 4531 7097 020 SD 038 008 006 007 016 001 004 002 004 057 003 004 005 003 usc83 1 5230 090 506 1210 2051 026 1125 062 011 10311 3633 1895 4427 6572 012 1000 C, 100 MPa usc72 4 4735 159 541 1187 2140 025 879 039 003 9709 3671 1525 4759 7066 027 SD 020 013 033 023 019 008 048 004 005 083 055 078 042 135 usc73 3 5188 092 476 1483 1773 040 910 073 010 10044 4506 1552 3873 7439 019 SD 063 018 018 042 016 000 035 008 002 039 071 042 054 074 usc74 1 5024 092 389 1506 1411 047 1191 060 009 9729 4684 2078 3154 6927 025 usc75 2 5034 076 264 1552 1642 063 1334 032 004 10000 4414 2130 3355 6746 022 SD 047 008 136 017 119 002 024 019 001 000 065 092 156 063 975 C, 100 MPa usc57b 1 4722 169 566 1393 2016 059 819 031 005 9781 4177 1378 4345 7520 026 Reduced experiments 1000 C, 200 MPa usc28 2 5270 094 372 1434 1731 042 1288 031 013 10272 4202 2008 3716 6767 019 SD 063 009 054 010 166 009 100 001 008 047 085 065 144 026 usc29 1 5273 043 181 1602 1086 061 1940 020 004 10210 4570 3105 2227 5955 025 975 C, 200 MPa usc1 4 4888 090 296 1490 2041 038 947 025 004 9819 4244 1514 4181 7371 020 SD 121 007 067 029 012 007 017 007 002 035 044 021 039 045 usc2 2 4993 089 378 1458 1674 057 1208 045 007 9909 4325 2010 3568 6828 015 SD 021 008 005 017 079 004 062 012 003 054 060 107 160 086 925 C, 200 MPa usc6 1 5110 075 772 1005 1475 024 1103 117 039 039 3726 2294 3929 6189 025 usc7 1 4987 045 317 1365 1134 060 1786 040 007 9741 4244 3115 2535 5767 022 1000 C, 400 MPa usc25 1 5149 047 162 1599 800 060 2120 023 001 9960 4707 3501 1692 5734 030 usc26 2 5133 099 165 1379 1086 068 2079 019 003 10031 4097 3463 2325 5427 030 SD 069 047 007 055 219 001 282 003 000 150 095 413 507 238 (continued) Journal of Petrology, 2016, Vol. 57, No. 10 1905

Table 4. Continued

Fe –Mg n SiO2 TiO2 Al2O3 MgO CaO MnO FeO* Na2OK2O Total En Fs Wo Mg# Kd * 975 C, 400 MPa usc12 3 5084 076 301 1386 1750 053 1232 009 002 9894 4117 2054 3739 6672 021 SD 036 008 049 081 084 007 067 015 003 184 033 010 017 021 usc13 1 5141 061 239 1431 1587 056 1483 000 001 10000 4166 2422 3319 6324 025 usc14 1 5186 098 362 1245 1635 059 1417 000 001 10000 3832 2447 3619 6103 925 C, 400 MPa usc87 2 5111 069 318 1239 2023 030 1040 031 006 9866 3761 1772 4415 6797 020 SD 004 009 085 055 112 012 018 003 005 040 031 095 086 135 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 usc89 1 5126 065 332 1222 1606 050 1388 047 015 9850 3839 2446 3626 6108 023 usc90 1 5161 062 455 1062 1066 065 2019 047 020 9956 3542 3779 2556 4838 n, number of analysis; SD, standard deviation. FeO*, total iron reported as FeO. En, Fs and Wo were calculated as done by Fe Mg Morimoto (1989). Mg# ¼ 100Mg/(Mg þ Fe*). Kd *– ¼ (Fe*/Mg in clinopyroxene)/(Fe*/Mg in melt). between these, together defining three bands depend- andesite (at these temperatures) are best reproduced. ing on pressure. This effect is enhanced at fO2 NNO þ Pressures as low as at 100 MPa can be ruled out be- 15(Fig. 8; see below). A decrease in fO2 from NNO þ cause the compositions of the natural minerals are not 15 to QFM produces melts richer in FeO* and slightly reproduced at this pressure (see Figs 4–9). In contrast, poorer in MgO and TiO2, reflecting the overall low charges annealed at 1000–975 C, 200 MPa and 4– amounts of magnetite crystallizing in QFM charges 5H2Omelt wt % successfully reproduce the Mg# and (<20 wt %) and incoming of ilmenite (Table 2). TiO2 content of Mt, isolated augite phenocrysts (En42Fs21Wo37, Mg#67 6 1) and normally zoned Cpx crystals (cores of En Fs Wo , Mg#70 to rims of DISCUSSION 44 19 37 En42Fs21Wo37, Mg#67 6 1; see above), Opx Storage conditions of Upper Scoriae 1 andesite (En65Fs29Wo4Mg#68) and Pl (An53) from the andesite A first estimate of storage conditions of USC-1 can be (Figs 3–9). Charges annealed at 400 MPa, 1000–975C retrieved from the comparison of the natural and ex- and 5–7 wt % H2Omelt also reproduce the natural Mt, perimental phase assemblages. The lack of Ilm in the Cpx and Pl compositions, but fail to reproduce the andesite indicates that the fO2 of the USC-1 magma is Mg#70 Cpx and Opx (it should be noted that Cpx–Opx better approximated by the NNO þ 15 experiments, as crystals from these 400 MPa charges plot at 5–10 Mg#– Ilm is always present in charges at QFM (Table 2, Fig. Wo mol % lower compared with natural ones (Figs 5–9). 3). At NNO þ 15, Ilm crystallizes at 950C, which fixes In addition, when previous estimated conditions for the temperature in the range 975–1000 C. However, the iso- USC-1 andesite (T, P, fO2,H2Omelt) are used in equations thermal sections in this temperature range (Fig. 3) show (1)–(3), retrieved compositions for Mt (73 6 04), Wo a large coexistence domain for the main mineral assem- content in Cpx (38 6 06 mol %) and An content in Pl (56 blage (Pl–Cpx–Opx–Mt), precluding any fine-tuning of 6 03 mol %) match those of the natural sample (Table pre-eruptive pressure using topological arguments 1). These results support the validity of equations (1)– alone. By considering the total crystal content of the (3) for retrieving information about the ponding condi- natural andesite (28 wt %), a first estimate of H2Omelt tions of magmas having a composition similar to that of can be provided: at 975–1000C, this amount of crystals USC-1. is reproduced, together with the main mineral assem- Further insights can be gained by using the experi- blage, at 4–7 wt % H2Omelt in the pressure range 100– mental Pl/Opx ratio (wt %), which varies with crystallin-

400 MPa (grey areas in Fig. 3). ity, temperature, pressure, H2Omelt and fO2 (Table 2; Fig. This first estimate can be refined using the propor- 9c). Because natural samples commonly contain ante- tions and compositions of the minerals and glass (Figs crystic or xenocrystic minerals, the observed mineral

3–10). Considering an H2Omelt range of 4–7 wt %, the P– modal proportions are not necessarily those of the min- T–H2Omelt conditions that best approach the 28 wt % eral assemblage in equilibrium with the melt. Thus, to crystal content are 1000 C, 100 MPa, 4 H2Omelt wt % or avoid the effect produced by the presence of foreign 1000–975 C, 200–400 MPa, 5–7 H2Omelt wt %, respect- material, we use the crystal content (28 wt %) and a Pl/ ively (Supplementary Data crystal content). Tighter con- Opx ratio (12) calculated by mass balance using the straints are provided when the crystal load (28 wt %), phenocryst compositions in equilibrium with the andes-

An content in Pl (53 mol %) and Mg# (68) of coexisting itic magma (An53,En65Fs19Wo4; Table 1). In Fig. 9c the Cpx–Opx pairs are combined in isothermal–polybaric Pl/Opx ratio is plotted against the crystallinity of sections at 975–1000C(Fig. 3e and f): these parameters charges annealed at 100, 200 and 400 MPa. To achieve a define a P–H2Omelt region (dashed-line squares in Fig. given Pl/Opx ratio, charges at 200 MPa requires a lower 3e and f) in the range 200 6 40 MPa and 5 6 05wt% degree of crystallization than at 400 MPa. Thus, con- H2Omelt, in which the characteristics of the natural sidering the temperature interval 975–1000 C, charges 1906 Journal of Petrology, 2016, Vol. 57, No. 10

Table 5: Composition of experimental orthopyroxenes (wt %)

Fe*–Mg n SiO2 TiO2 Al2O3 MgO CaO MnO FeO* Na2OK2O Total En Fs Wo Mg# Kd Oxidized experiments 1000 C, 200 MPa usc65 3 5211 038 326 2165 256 072 1696 031 001 9797 6478 2848 551 6946 020 SD 054 009 074 069 006 007 053 002 002 065 014 021 024 018 975 C, 200 MPa usc33 4 5325 033 117 2488 182 058 1774 003 004 9984 6822 2728 359 7143 019 SD 108 006 041 015 007 020 051 001 001 099 010 057 016 046 usc34 1 5171 048 197 2353 199 063 2019 001 000 10050 6421 3091 390 6751 021 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 usc35 1 5272 024 109 2195 190 076 1863 007 000 10079 6418 3056 400 6775 027 950 C, 200 MPa usc52 3 5233 031 193 2439 193 079 1518 008 002 9695 7021 2450 400 7413 017 SD 091 003 012 030 019 016 068 002 003 091 020 079 045 066 usc53 3 5290 036 202 2333 166 069 1678 005 003 9782 6797 2742 347 7125 018 SD 007 008 036 015 028 008 041 006 001 008 057 052 059 051 usc54 3 5210 033 139 2204 201 077 1799 006 002 9671 6479 2968 424 6859 016 SD 014 006 017 018 030 004 029 006 004 050 033 038 059 029 925 C, 200 MPa usc43 1 5169 031 255 2352 273 070 1645 013 002 9810 6698 2629 559 7181 018 usc44 1 5062 023 131 1999 164 080 2189 007 005 9658 5896 3622 347 6195 900 C, 200 MPa usc59 1 4739 020 155 1797 210 093 2404 018 004 9440 5364 4027 451 5711 usc60 1 4686 018 175 1691 181 082 2623 026 000 5064 4405 390 5348 1000 C, 400 MPa usc70 3 5113 042 249 1941 232 067 2213 019 002 9879 5729 3664 494 6099 024 SD 071 009 059 065 038 008 077 011 002 046 089 067 091 068 975 C, 400 MPa usc39 2 5225 031 251 2108 184 085 1968 012 006 9870 6214 3255 389 6562 015 SD 032 000 046 021 041 021 036 008 004 061 093 043 086 064 usc40 1 5136 045 222 1874 239 077 2326 021 002 9943 5521 3845 506 5895 020 950 C, 400 MPa usc78 4 5143 036 259 2205 184 093 1895 017 002 9833 6386 3079 383 6747 017 SD 057 003 080 059 025 016 041 014 004 137 052 025 056 025 925 C, 400 MPa usc85 3 5305 032 308 1773 468 090 2186 030 002 10194 5233 3620 996 5911 023 SD 102 011 122 135 023 011 164 027 002 108 081 032 079 048 1000 C, 100 MPa usc73 5 5298 043 188 2584 202 090 1589 006 003 10004 7037 2428 395 7434 024 SD 041 006 022 057 020 011 033 004 004 097 046 027 043 027 usc74 2 5204 038 358 2241 253 089 1731 054 006 9973 6506 2819 528 6977 025 SD 007 004 055 055 034 001 071 014 004 013 027 059 082 035 975 C, 100 MPa usc58b 3 5314 040 191 2584 185 084 1538 007 002 9945 7123 2378 367 7497 SD 024 002 036 038 038 014 080 007 003 037 057 080 079 074 usc59b 5267 042 278 2380 238 099 1694 037 003 10038 6690 2671 481 7146 011 Reduced experiments 1000 C, 200 MPa usc28 2 5386 045 216 2104 220 063 2161 014 006 10212 5995 3454 451 6345 022 SD 138 005 008 100 013 012 097 020 008 042 027 005 047 007 usc29 1 5226 042 165 1959 271 070 2391 004 001 10129 5542 3795 551 5936 025 usc30 1 5192 060 159 1369 744 060 2567 028 007 10186 4053 4263 1583 4873 022 975 C, 200 MPa usc2 2 5032 044 122 1939 292 068 2388 000 000 9885 5498 3799 594 5914 023 SD 012 000 000 001 026 007 029 000 000 049 062 005 046 030 usc3 4 5108 041 152 1935 221 053 2284 002 002 9799 5682 3764 465 6015 020 SD 029 007 016 026 025 009 011 004 004 051 038 038 047 026 925 C, 200 MPa usc7 3 5036 038 199 1815 293 078 2292 002 004 9757 5411 3831 626 5854 022 SD 061 003 039 035 068 008 044 004 004 071 166 023 138 089 1000 C, 400 MPa usc25 3 5246 051 183 2060 273 068 2100 006 001 9989 5932 3391 566 6364 023 SD 034 001 012 058 123 008 113 003 001 046 147 174 256 109 975 C, 400 MPa usc12 2 5088 032 506 1781 278 042 1896 054 005 9683 5804 3465 653 6262 026 SD 055 010 116 065 031 006 147 034 002 017 019 131 099 096 usc13 1 5101 028 094 1921 200 057 2352 000 004 9756 5622 3862 421 5928 029 usc14 1 5047 040 180 1682 405 065 2218 007 006 9650 5169 3823 894 5749 925 C, 400 MPa usc89 2 5079 031 189 1644 195 060 2720 002 000 9919 4917 4563 418 5187 033 SD 003 006 027 015 000 020 106 001 000 078 049 092 008 075 n, number of analysis; SD, standard deviation. FeO*, total iron reported as FeO. En, Fs and Wo were calculated as done by Fe*–Mg Morimoto (1989). Mg# ¼ 100Mg/(Mg þ Fe*). Kd ¼ (Fe*/Mg in clinopyroxene)/(Fe*/Mg in melt). Journal of Petrology, 2016, Vol. 57, No. 10 1907

Table 6: Composition of experimental magnetites (wt %)

n SiO2 TiO2 Al2O3 MgO CaO MnO FeO* Na2OK2O Total Mg# Oxidized experiments 1000 C, 200 MPa usc62 2 011 451 317 411 014 062 7662 000 000 8928 905 SD 005 019 010 003 001 012 071 000 000 086 usc63 3 018 695 407 346 017 058 7380 000 003 8924 802 SD 006 012 002 010 006 008 069 000 003 101 usc64 1 015 852 374 356 016 063 7388 004 000 9068 821 usc65 2 031 1087 293 298 021 056 7134 000 001 8921 719 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 SD 016 003 006 014 002 013 079 000 002 091 usc66 1 270 1480 286 201 045 057 6910 025 008 9281 512 975 C, 200 MPa usc32 3 023 1202 370 307 015 048 7435 000 001 9403 711 SD 017 015 013 020 011 007 055 001 001 058 usc33 2 027 1408 385 313 026 028 7297 000 002 9487 738 SD 014 006 011 004 017 007 002 000 003 043 usc34 2 089 1522 340 273 012 031 7197 016 001 9481 657 SD 035 068 022 006 006 008 104 002 001 001 950 C, 200 MPa usc52 1 022 1396 335 290 020 077 7840 016 006 10002 643 usc53 3 017 1355 343 293 010 055 7924 002 001 10000 643 SD 004 022 003 006 008 040 119 000 002 097 usc54 1 004 1450 318 221 006 057 7910 034 000 10000 473 925 C, 200 MPa usc42 2 036 928 299 257 020 071 7513 005 003 9131 597 SD 000 017 029 005 006 005 011 007 004 016 usc43 1 003 1237 273 231 028 067 8155 000 006 10000 481 1000 C, 400 MPa usc70 2 027 1675 374 253 023 038 6619 004 003 9016 662 SD 003 030 007 011 002 006 078 000 003 093 950 C, 400 MPa usc77 2 015 572 313 352 011 058 7703 000 004 9029 782 SD 005 018 001 028 008 008 044 000 002 031 usc78 2 036 917 318 239 019 065 7549 000 006 9149 555 SD 012 015 014 008 005 005 029 000 002 046 usc79 1 039 1039 264 187 027 032 7450 007 005 9051 446 usc80 3 026 1065 260 193 020 049 7610 000 001 9223 449 SD 004 011 027 006 004 014 070 000 001 064 925 C, 400 MPa usc82 3 025 908 328 201 016 059 7669 001 000 9206 447 SD 008 038 027 005 006 015 074 001 001 102 usc83 3 024 996 339 169 010 061 7719 003 007 9328 375 SD 006 019 007 003 001 008 115 002 004 113 usc84 5 026 1155 331 175 019 059 7684 000 003 9452 391 SD 013 019 012 009 002 010 099 004 005 109 usc85 3 035 1226 302 156 017 046 7727 002 000 9512 347 SD 022 030 003 010 002 008 053 004 001 032 1000 C, 100 MPa usc72 2 017 690 395 404 015 064 7465 003 004 9055 913 SD 000 027 002 010 006 014 108 004 003 136 usc73 1 022 923 333 349 015 053 7465 000 000 9159 799 usc74 1 092 1053 294 290 034 049 7167 018 006 9004 698 usc75 1 065 1308 257 245 021 035 7207 009 006 9152 593 975 C, 100 MPa usc57b 2 016 684 349 416 015 066 7632 000 006 9182 919 SD 016 683 349 393 013 053 7658 000 003 9167 usc58b 1 018 986 292 336 018 075 7358 000 000 9082 781 usc59b 1 017 1107 263 304 014 062 7304 000 005 9076 718 usc60b 1 015 1156 236 258 009 072 7363 000 005 9113 610 Reduced experiments 1000 C, 200 MPa usc28 1 094 1183 629 286 015 065 5894 003 008 8177 796 usc29 2 158 1873 343 183 021 052 6466 015 007 9116 480 SD 016 245 098 034 003 011 262 006 002 395 925 C, 200 MPa usc6 3 010 1763 346 249 017 049 6250 000 004 8689 690 SD 008 045 017 015 006 009 068 000 001 081 925 C, 400 MPa usc87 1 046 1847 421 267 018 075 7306 008 012 10000 636 n, number of analyses; SD, standard deviation; FeO*, total iron reported as FeO. Mg# ¼ 100(Mg/Mg þ Fe*) in moles. 1908 Journal of Petrology, 2016, Vol. 57, No. 10

Table 7: Composition of experimental ilmenites (wt %)

n SiO2 TiO2 Al2O3 MgO CaO MnO FeO* Na2OK2O Total Reduced experiments 1000 C, 200 MPa usc28 3 014 4984 029 365 025 048 4504 004 005 9979 SD 005 014 005 010 010 009 077 002 003 092 usc29 1 085 4883 037 302 030 059 4663 006 004 10069 975 C, 200 MPa usc3 3 056 4850 044 344 038 051 4069 000 007 9458 SD 043 035 018 008 002 013 083 000 002 067 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 975 C, 400 MPa usc12 1 024 5011 023 446 046 061 3980 000 012 9602 925 C, 400 MPa usc87 2 034 4640 024 319 027 057 4194 016 000 9312 SD 012 002 006 013 002 027 002 008 000 043 usc88 1 020 4674 020 268 029 073 4286 003 004 9377 usc89 1 094 4763 065 275 039 081 4272 008 006 9603 n, number of analyses; SD, standard deviation. FeO*, total iron reported as FeO.

Table 8: Composition of experimental amphiboles (after Leake et al., 1997)

usc42(3) SD usc82(3) SD usc83(5) SD usc84(4) SD usc6(4) SD usc87(2) SD usc88(5) SD usc89(3) SD

SiO2 4145 028 4321 036 4312 037 4431 052 4173 055 4242 092 4106 040 4166 010 TiO2 301 004 239 019 268 016 297 022 328 013 255 046 316 024 344 019 Al2O3 1099 056 1172 039 1132 055 1031 048 1075 036 1050 017 1173 014 1083 028 FeO* 1134 014 1289 122 1444 043 1480 061 1324 056 1551 047 1676 052 1789 024 MnO 028 001 035 010 024 013 032 011 028 006 021 011 025 006 022 011 MgO 1447 023 1367 088 1208 016 1268 053 1274 036 1147 018 991 045 1012 035 CaO 1121 020 1117 006 1139 043 1025 020 1061 019 1083 001 1083 024 999 014 Na2O212 005 235 004 240 011 229 008 212 007 242 011 236 007 235 012 K2O109 044 046 004 046 006 039 003 035 003 032 002 049 005 046 004 Sum 9597 019 9820 115 9813 042 9831 079 9511 028 9625 020 9659 033 9706 052 atoms per formulae Si 613 622 631 638 622 634 619 621 Ti 033 026 030 032 037 029 036 039 Altot 191 199 195 175 189 185 208 190 Fe3þ 080 086 048 096 086 066 055 095 Fe2þ 060 069 128 082 079 128 157 128 Mn 004 004 003 004 004 003 003 003 Mg 319 294 264 272 283 256 223 225 Ca 178 172 179 158 169 173 175 160 Na 061 066 068 064 061 070 069 068 K021 009 009 007 007 006 009 009 AlIV 187 178 169 162 178 166 181 179 A sites 059 046 055 029 038 050 053 036 Mg# 069 065 060 060 063 057 041 051

Numbers in parentheses indicate the number of analyses. SD, standard deviation. FeO*, total iron reported as FeO. Mg# ¼ MgO/ (MgO þ FeO*) in wt %. A sites ¼ (Na þ K).

at 200 MPa and with 4–5 wt % H2Omelt successfully re- uncertainties), and higher FeO*/MgO ratios, than those produce the Pl/Opx ratio (12) and crystal content (28 wt at 200 MPa (Fig. 8). %) of the natural andesite, whereas those at 400 MPa The comparison between natural and experimental would require crystallinities of 50 wt % to achieve the phase relationships and mineral compositions therefore same ratio (Fig. 9c). constrains the pre-eruptive P–T–H2Omelt–fO2 conditions Glasses obtained at 200 MPa and NNO þ 15 also for the Upper Scoriae 1 andesite to be 200 MPa, 975– successfully reproduce the composition of the residual 1000 C, 5 6 05wt%H2Omelt and fO2 NNO þ 15 melt of the andesite (Table 1; Fig. 8). Although there (Table 2; Fig. 3). Such conditions are similar to previous are not large differences between most major oxides estimates obtained for andesitic magmas at Santorini

(i.e. SiO2,Al2O3, CaO, Na2O, K2O) of the glasses ob- (Gardner et al., 1996; Michaud et al., 2000). We note that tained at either 200 or 400 MPa and 975–1000C, coexisting Fe–Ti oxides in evolved (T < 900C) Santorini charges at 400 MPa generally have glasses with lower magmas yield fO2 between QFM – 05 and NNO þ 05 TiO2 contents (even considering analytical (Nichols, 1971a; Cottrell et al., 1999; Cadoux et al., 2014; Journal of Petrology, 2016, Vol. 57, No. 10 1909

Table 9: Composition of experimental glasses (wt %)

n SiO2 TiO2 Al2O3 FeO* MnO MgO CaO Na2OK2OP2O5 Total Sum FeO*/MgO Oxidized experiments 1000 C, 200 MPa usc62 11 6087 115 1641 585 020 277 655 445 138 037 100 92421 SD 013 008 014 006 021 008 021 014 005 007 06 usc63 3 6203 112 1715 559 008 228 579 450 147 000 100 92724 SD 018 003 032 023 013 006 017 015 008 000 07 usc65 4 6597 094 1536 508 019 127 374 472 236 038 100 95440 SD 044 007 079 040 014 007 034 006 007 011 05 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 usc66 3 7021 085 1338 462 009 063 230 424 346 022 100 96473 SD 057 011 020 011 010 007 014 012 006 008 08 975 C, 200 MPa usc32 5 6018 098 1675 758 028 220 574 446 152 032 100 94634 SD 059 015 033 021 015 006 012 027 003 002 06 usc33 5 6035 109 1639 772 022 205 556 463 160 039 100 95538 SD 030 007 013 016 012 005 019 011 013 007 03 usc34 2 6293 107 1565 670 024 166 457 487 191 040 100 96340 SD 014 004 008 022 002 000 012 003 000 011 06 usc35 4 6530 100 1474 621 015 119 373 473 248 047 100 97752 SD 022 005 016 020 011 004 016 019 005 005 05 usc36 2 6748 089 1349 571 015 070 314 452 331 060 100 97782 SD 056 004 001 001 002 003 035 004 014 036 04 950 C, 200 MPa usc52 3 6911 062 1542 336 007 078 304 476 256 028 100 93143 SD 097 011 038 001 004 004 046 021 025 010 07 usc53 5 6899 065 1477 371 019 094 287 509 257 022 100 95539 SD 015 007 004 037 008 003 013 012 004 005 04 usc54 3 7137 054 1425 337 012 064 216 441 292 021 100 97453 SD 064 004 044 024 003 010 024 010 015 011 10 925 C, 200 MPa usc42 5 6654 063 1641 388 007 109 440 508 170 019 100 94836 SD 033 006 015 016 007 008 004 041 011 005 06 usc43 3 7091 048 1427 287 007 074 255 539 258 014 100 96239 SD 025 005 031 024 005 005 008 015 009 007 04 1000 C, 400 MPa usc67 10 5845 136 1629 877 020 290 637 382 151 035 100 89730 SD 039 008 023 028 006 021 036 018 029 006 06 usc68 14 5856 132 1637 839 015 258 618 467 144 034 100 94933 SD 043 008 052 030 010 040 064 025 011 009 08 usc69 10 5898 131 1636 814 015 258 615 457 144 032 100 94532 SD 070 010 057 037 009 052 068 025 010 005 06 usc70 3 6220 130 1538 809 009 172 469 409 204 040 100 94647 SD 043 009 005 059 012 003 008 034 008 004 04 usc71 4 6521 110 1394 703 023 090 378 430 304 047 100 96278 SD 084 005 018 056 009 001 008 021 008 011 03 975 C, 400 MPa usc37 5 5969 121 1583 811 024 254 632 440 133 032 100 91432 SD 047 011 021 018 007 011 009 046 011 009 07 usc38 5 6064 102 1749 726 016 180 526 453 151 034 100 95340 SD 038 007 016 043 005 011 017 017 008 007 05 usc39 3 6208 078 1737 631 037 099 510 478 186 037 100 95764 SD 034 009 102 085 010 009 045 029 027 006 05 usc40 4 6614 084 1443 641 012 101 350 462 242 053 100 96164 SD 011 008 017 017 001 002 002 027 002 002 05 950 C, 400 MPa usc77 3 6276 111 1726 469 012 217 572 437 144 037 100 91922 SD 053 004 022 044 010 007 020 020 011 007 04 usc78 3 7059 048 1448 385 014 078 300 406 245 018 100 97050 SD 033 011 043 052 005 010 002 010 008 011 08 925 C, 400 MPa usc82 10 6462 061 1725 426 017 117 557 455 166 015 100 91737 SD 076 013 032 036 007 006 007 082 007 011 07 usc83 1 6523 078 1693 512 022 066 443 478 167 017 100 93978 usc84 9 6832 054 1538 385 011 085 352 501 227 017 100 94046 SD 042 005 024 046 009 010 012 008 012 015 07 usc85 9 7074 039 1472 330 008 059 268 442 297 010 100 94356 SD 029 009 022 011 008 004 009 037 007 008 04 1000 C, 100 MPa usc72 4 6330 108 1606 516 023 187 565 470 169 025 100 95928 SD 033 009 014 011 008 003 040 023 005 003 07 usc73 4 6528 094 1530 492 020 151 445 508 192 041 100 96333 SD 031 004 020 009 007 009 020 025 015 009 10 usc74 2 6894 081 1396 416 010 132 329 477 226 040 100 97831 SD 065 003 053 024 006 003 026 031 006 015 05 usc75 3 7191 048 1327 287 007 074 255 539 258 014 100 97739 (continued) 1910 Journal of Petrology, 2016, Vol. 57, No. 10

Table 9. Continued

n SiO2 TiO2 Al2O3 FeO* MnO MgO CaO Na2OK2OP2O5 Total Sum FeO*/MgO SD 033 009 061 047 001 001 022 009 014 001 03 usc76 975 C, 100 MPa usc57b 2 6410 105 1622 467 028 209 502 456 169 032 100 95122 SD 034 006 025 032 014 009 003 041 004 004 02 usc59b 1 7131 075 1328 363 020 077 256 420 296 034 100 95847 Reduced experiments 1000 C, 200 MPa Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 usc27 10 5919 130 1623 823 021 242 641 429 152 020 100 92534 SD 043 017 009 042 009 005 011 007 011 006 05 usc28 4 6191 094 1610 758 010 159 506 472 183 016 100 94648 SD 045 011 011 027 008 005 011 020 010 012 09 usc29 1 6444 083 1472 690 027 143 421 483 209 029 100 94948 usc30 4 6660 074 1529 548 014 065 290 514 284 021 100 95985 SD 045 016 005 016 001 004 004 023 005 003 10 975 C, 200 MPa usc1 8 5897 130 1558 876 023 278 642 434 147 017 100 93332 SD 065 012 022 016 010 004 012 040 007 010 06 usc2 2 6241 108 1565 772 020 144 466 460 203 020 100 96654 SD 093 002 052 017 007 000 013 076 024 001 01 usc3 1 6256 107 1557 795 003 136 488 450 196 010 100 96958 usc4 5 6534 097 1443 676 023 110 373 464 250 028 100 98361 SD 029 015 017 034 013 003 006 023 015 011 03 usc5 1 6985 096 1342 467 017 070 278 407 332 006 100 98567 925 C, 200 MPa usc6 3 6252 087 1672 686 005 157 545 449 148 000 100 92344 SD 057 001 012 021 005 004 002 033 005 000 usc7 1 6438 074 1622 594 031 103 399 494 225 021 100 95658 usc8 2 6795 075 1478 477 005 066 301 490 290 024 100 95472 SD 021 005 001 033 004 002 011 011 014 000 05 1000 C, 400 MPa usc22 1 5882 135 1613 877 014 254 643 419 140 025 100 92835 usc23 1 5919 130 1623 823 021 242 641 429 152 020 100 95734 usc25 3 6131 124 1632 765 018 172 488 459 185 024 100 97644 SD 026 010 037 028 000 006 010 004 003 002 04 usc26 2 6485 115 1504 602 009 118 389 497 245 036 100 97951 SD 008 013 003 004 004 006 003 005 002 001 03 975 C, 400 MPa usc11 4 5900 133 1583 880 012 265 658 408 127 035 100 91533 SD 053 010 014 011 008 013 040 038 002 008 07 usc12 3 6156 110 1606 756 001 182 514 480 161 035 100 93942 SD 019 001 006 006 001 008 008 019 008 011 01 usc13 3 6270 110 1542 719 003 170 503 467 181 035 100 94642 SD 061 007 012 028 005 013 078 037 016 009 03 925 C, 400 MPa usc87 10 6181 084 1653 674 015 163 570 487 155 018 100 90141 SD 051 009 013 022 010 003 011 036 006 012 07 usc88 3 6288 073 1703 550 019 114 507 550 174 023 100 92748 SD 057 003 009 018 006 003 002 037 006 002 05 usc89 9 6544 055 1572 536 013 093 384 566 213 024 100 94058 SD 033 009 014 025 008 005 008 036 011 010 05 usc90 3 6907 060 1547 369 005 073 285 460 281 012 100 94150 SD 008 006 015 029 008 002 009 011 013 005 05

All analyses are normalized to 100% anhydrous. Original totals are reported (Sum). n, number of analyses; SD, standard deviation. FeO*, total iron reported as FeO.

Druitt, 2014); however, there are no oxide-based esti- We now use these variations, along with the results of mates of fO2 for intermediate or mafic magmas. Our our experiments, and with data from previous experi- data show that the USC-1 andesite fractionated under ments and from the literature, to provide insights con- conditions more oxidizing than NNO, and perhaps as cerning the evolution of the USC-1 magma and the high as NNO þ 15. dynamics of the reservoir prior to the eruption. As previously pointed out, during the USC-1 eruption Evidence for magma reheating prior to eruption two different magmas were erupted: the volumetrically The textural and compositional variations observed in dominant (99%) andesite and a volumetrically subor- crystals (xenocrysts and phenocrysts) from the studied dinate dacite (620–632 wt % SiO2), which appears as andesitic sample can provide information concerning scattered and very rare pumices within the USC-1 fall- the dynamics operating within the magma reservoir. out deposit (Druitt et al., 1999). Unfortunately, there are Journal of Petrology, 2016, Vol. 57, No. 10 1911 no petrological data on the dacitic pumice. However, is worth noting that these conditions differ from those Andujar et al. (2015) reported the occurrence of felsic of andesite production, which has been inferred to minerals dispersed within the USC-1 andesite; in par- occur at 400 MPa, 1000 C and fO2 QFM, subsequent ticular, the presence of low-Mg orthopyroxene xeno- to basalt crystallization (Andujar et al., 2015). The latter crysts (En55Fs40Wo4, Mg#58), Mg-poor augite observation suggests that a decrease in pressure (En38Fs23Wo39, Mg#63) and low-An plagioclase accompanied by an increase in oxidation state may (An45–50), whose compositions mimic those of Santorini have occurred prior to and during the intrusion of the dacites (see above). Thus, as for the andesite, this infor- natural andesite. The oxidation of the magma could be mation can be used to shed light on the storage condi- due to the assimilation of shallower limestone or Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 tions of the USC-1 dacite. marble wall-rocks (Nichols, 1971b; Zellmer et al., 2000; Phenocrysts of inferred dacitic provenance [see Iacono-Marziano et al., 2008; Spandler et al., 2012) Andujar et al. (2015) for further details] provide the fol- and/or to volatile exsolution during decompression lowing constraints. The En55Fs40Wo4, Mg#58 Opx is (Burgisser & Scaillet, 2007). reproduced at 900 C, 200 MPa with 5–6 wt % H2Omelt Finally, the presence of xenocrystic phases such as (Fig. 7; Table 5). Such water contents do also reproduce olivine, An-rich Pl and high-Mg diopside, some of which the Mg-poor augite (En38Fs23Wo39, Mg#63) and the partly re-equilibrated with the andesitic magma (as indi- An45–50 from the dacite at the same pressure and fO2, cated by their compositional zoning), bears evidence of although at somewhat higher temperatures (925–950 C; an intrusion of basaltic–basaltic andesitic magma prior Figs 4 and 5). In contrast, pressures as high as 400 MPa, to the eruption, which may have provided the trigger NNO þ 15oranfO2 at QFM can be both ruled out mechanism of the USC-1 eruption (see Andujar et al., because at such conditions Pl is either less (at 400 MPa) 2015). or more (at QFM) calcic compared with Pl from the da- Based on the above, the following sequence of cite (Fig. 4). Thus, we conclude that the dacitic magma events for the late magmatic evolution of the USC-1 was probably stored at 200 MPa, at temperatures be- magma reservoir can be proposed. The andesitic tween 900 and 950 C with 5–6 H2Omelt wt %, in broad magma that was generated from basalt crystallization agreement with previous T–H O wt % constraints for 2 at 12–15 km depth rose to shallower levels and intruded dacitic magmas at Santorini (Druitt et al., 1999; Fabbro a partially crystallized dacitic body that was at 950– et al., 2013; Cadoux et al., 2014). Using these values and 925C and 8 km depth. This increased the temperature the An Pl composition as inputs in equations (1)–(3) 45–50 of the more evolved magma and generated the resorp- yields crystal contents for the USC-1 dacite between 50 tion textures of dacitic Opx entrained into the andesite. and 66 (6 14) wt %, Wo contents in clinopyroxene of 40 The subsequent cooling of the system from 1000 to 6 12 mol %, and Mg# in magnetite of 6 6 06 mol %, in 975C led to the crystallization of the andesite magma, good agreement with the compositions of the main which generated the Mg-rich rims observed on Opx and phenocrysts of the USC-1 dacite and those of Santorini the main phase assemblage and composition of the an- (this work; Druitt et al., 1999). desite. However, the cooling process did not trigger the The presence of resorbed textures on the eruption of the system by itself. The arrival of a new En Fs Wo , Mg#58 Opx of the USC-1 andesite and the 55 40 4 hotter basaltic–basaltic andesitic magma into the sys- fact that they are commonly mantled by a more Mg-rich tem may have triggered the eruption sometime later, as composition (En65Fs29Wo4, Mg#68) both suggest that the dacite experienced an episode of magma mixing evidenced by the presence of mafic xenocrysts (olivine,  with a hotter and more mafic magma; in such a scen- An-rich Pl, and high-Mg diopside; see above; Andujar ario the USC-1 andesite would be responsible for the et al., 2015). Mg-rich mantle (or higher En molar per cent) and crystal The above model for the USC-1 magma reservoir is resorption of the dacitic Opx (Andujar et al., 2015). The consistent with an open system characterized by abrupt changes in temperature and composition, as a result of fact that the andesitic Opx (En65Fs29Wo4, Mg#68) man- tling dacitic Opx is in turn overgrown by augite magma mixing–mingling processes at Santorini, which have been recorded in the eruptive products of the is- (En42–44Fs19–21Wo37, Mg#67–70) from the andesite (see Andujar et al., 2015, fig. 6), and the lack of reaction rims land (Nichols, 1971a; Huijsmans et al., 1988; Druitt et al., between them, suggests that these phases crystallized 1999; Zellmer et al., 2000; Fabbro et al., 2013). together, the sequence of Cpx En44Fs19Wo37Mg#70 ! En42Fs21Wo37Mg#67 thus representing a phase of cool- Conditions for melt evolution at Santorini: role of ing of the system from 1000C to 975C after andesite temperature and fO2 intrusion into the dacitic magma body. We infer that the Major explosive eruptions at Santorini over the last 550 main andesite and subordinate dacite magmas were kyr have been dominated by the emission of intermedi- ponding at the same depth (200 MPa), this being the in- ate (andesite–dacite; Cape Therma 1, Cape Thera, trusion level of the USC-1 andesite into the partially Upper Scoriae 1, Upper Scoriae 2; Druitt et al., 1999) crystallized dacitic magma body (50–66 wt % crystals) and silicic magmas (dacite–rhyodacite; Cape Therma 2, that then formed a compositionally and thermally Lower Pumice 1, Lower Pumice 2, Cape Riva, Minoan). zoned, highly crystallized magma reservoir or mush. It Despite their mineralogical similarities, the two groups 1912 Journal of Petrology, 2016, Vol. 57, No. 10 exhibit systematic compositional differences (Druitt observation is consistent with previous temperature et al., 1999). In particular, andesite–dacite magmas of constraints (1080–960C; Michaud et al., 2000) and with the intermediate-dominated eruptions have higher the petrology of recent eruptive products at Santorini in

FeO*/MgO ratios and TiO2 contents compared with which andesites are characterized by the lack of ilmen- their silicic counterparts, and most have tholeiitic affin- ite in their mineral assemblages (i.e. USC-1, USC-2, ities (Fig. 10a–d). In contrast, dacites (and minor andes- Cape Therma 1–3, Middle Pumice andesite, recent itic components) from the silicic-dominated eruptions Kameni products; Nichols, 1971a; Barton & Huijsmann, fall in the calc-alkaline field (Fig. 10a–d), but rhyodacites 1986; Druitt et al., 1999; Michaud et al., 2000; this work). Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 (>68 wt % SiO2) exhibit greater variability in their FeO*/ In contrast, the products of dominantly silicic eruptions

MgO ratios and straddle the calc-alkaline and tholeiitic have lower TiO2 contents, contain ilmenite and have fields (Fig. 10a and b). Such differences probably reflect pre-eruptive temperatures of 900C(Gardner et al., temporal changes in the generation, evolution and/or 1996; Cottrell et al., 1999; Gertisser et al., 2009; Cadoux storage conditions of the magmas at Santorini (Nichols, et al., 2014). This is in agreement with our experimental 1971a; Huijsman et al., 1988; Druitt et al., 1999; results. These observations imply that an fO2 NNO þ Mortazavi & Sparks, 2004). 15 to NNO þ 05 (average NNO þ 1 6 05; Tables 2 and Experimental liquids produced by the crystallization 9) prevailed for all of the Santorini evolved magmas; of the USC-1 andesite reproduce the liquid line of des- this is again consistent with our previous fO2 estimate cent defined by Santorini magmas (Fig. 10). This con- for the USC-1 magma. firms the success of our experimental approach and The above does not rule out the possibility that this gives support to models in which crystal fractionation is was not the case for the more evolved compositions the main process controlling magma evolution at (dacites–rhyodacites from the silicic group) because (1) Santorini, even if the presence of mafic material dis- these rocks contain ilmenite (see above) and (2) liquids persed within the main volume of the deposits reflects of the QFM experiments show the same relationship be- a common and recurrent process of injection of less tween temperature and melt TiO2 content (Fig. 10c and evolved magmas into a more evolved magma. d). Ilmenite also crystallizes over the range of explored However, as previously stated, the petrology and geo- temperatures (1000–925C) at QFM, but the modal chemistry of the erupted products at Santorini show abundances of magnetite and/or ilmenite are somewhat that mixing plays a subordinate role in magma evolu- lower compared with the NNO þ 15 experiments tion (Nichols, 1971a; Huijsmanns et al., 1988; Druitt (Table 2). We therefore use the plot FeO*/MgO vs SiO et al., 1999; Michaud et al., 2000; Zellmer et al., 2000), 2 to better constrain the fO prevailing in the system (Fig. yet it possibly acts as an eruption trigger. Protracted 2 10a and b). This plot shows that, except for a single run chemical mixing as a main controlling factor of magma (925C, 400 MPa), QFM glasses plot outside the field evolution requires specific conditions to occur defined by Santorini magmas. In contrast, a large num- (Laumonier et al., 2014), which are often met at many ber of NNO þ 15 to NNO þ 05 experimental glasses do calc-alkaline volcanoes, but apparently less so at fall within the Santorini field. This shows conclusively Santorini. Experimental liquids define different compos- that differentiation of an andesitic magma under reduc- itional lineages depending on P–T–fO –H O (Fig. 10). 2 2 melt ing conditions (QFM) does not produce dacitic–rhyo- On a diagram of TiO versus SiO , melts produced at 2 2 dacitic liquids that follow the lineage defined by 1000–975C fall in the intermediate-dominated (andes- Santorini melts. Thus, more oxidizing conditions (NNO ite–dacite) magma field whereas those at 950–900C fall 0 5 to NNO 1 5; Table 2) are required to explain the within the silicic-dominated region, regardless of the þ þ FeO*/MgO ratio of Santorini magmas. prevailing fO2 and pressure (Fig. 10c and d). This rela- tionship provides first-order constraints on the tem- perature of the erupted magmas, andesites and dacites Conditions required for the generation of being characterized by higher temperatures (1000– tholeiitic or calc-alkaline dacites–rhyodacites at 975C) than dacites and rhyodacites (950–850C). The Santorini experimental results also shed light on the difference in Our experimental results can shed light on the gener- the glass TiO2 content between these two groups. In ation conditions and mechanisms controlling the calc- NNO þ 15 experiments the relationship of glass TiO2 alkaline versus tholeiitic affinities of magmas at content with temperature is strongly correlated with the Santorini. Younger (<530 ka) andesitic, dacitic and rhyo- onset of ilmenite crystallization at T < 965C and the dacitic magmas at Santorini have tholeiitic to weakly increasing modal proportion of ilmenite and magnetite calc-alkaline affinities depending on their FeO*/MgO with magma evolution (Fig. 3; Table 2). Charges an- ratios (Fig. 10a and b; Druitt et al., 1999). The tholeiitic nealed at 1000–975C are characterized by the highest character has been attributed to the differentiation of a glass TiO2 content and the absence of ilmenite in the basaltic magma under reduced conditions where mag- crystallizing assemblage, whereas in those at T < 950C netite crystallization is either suppressed or occurs in ilmenite crystallizes together with significant amounts low modal proportions, allowing the Fe enrichment of magnetite, leading to an overall decrease in the TiO2 characteristic of tholeiitic series magmas (Sisson & content of the melt (Table 2; Figs 8 and 10). This Grove, 1993; Druitt et al., 1999; Andujar et al., 2015). In Journal of Petrology, 2016, Vol. 57, No. 10 1913 contrast, the calc-alkaline trend is acquired when the and 9). The decompression of such volatile-rich melts magma evolves under oxidizing conditions (>NNO), will inevitably promote fluid exsolution at around which promote a massive precipitation of magnetite. 300 MPa, which could increase the prevailing fO2,as Additionally, it may also arise by mixing an evolved shown by numerical simulations for felsic melts magma (dacite–rhyodacite) with a more mafic melt (Burgisser et al., 2008). The increase in oxidation state (basalt, basaltic andesite), resulting in a decrease in the of the system via such a process will depend on the Fe content of the mixed magmas and low FeO*/MgO final pressure reached. At 100 MPa almost half of the ratios (Sisson & Grove, 1993; Druitt et al., 1999; Fabbro amount of H2Omelt is expelled out of the magma and the Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 et al., 2013). As detailed below, our experimental results corresponding increase in fO2 will be stronger than in provide an alternative mechanism whereby the tholei- the magma stored at 200 MPa, if H2O exsolution drives itic or calc-alkaline affinities reflect the pressure of oxidation (but also see Waters & Lange, 2016). We note, magma provenance. however, that decompression may also lead to reduc- Our data show that the crystallization of USC-1 an- tion of magmas (e.g. Gaillard & Scaillet, 2014; desite at NNO þ 1 6 05 generates residual melts that Moussallam et al., 2014), so there is no unique answer have different FeO*/MgO ratios depending on the pre- to the effect of degassing on fO2. vailing temperature and/or pressure (Fig. 10). At 1000– Apart from volatile exsolution effects, which could ei- 975 C, glasses produced at 100 MPa all lie within (or in ther counteract or amplify apparent redox effects on the one case on the boundary of) the calc-alkaline field, LLD, our experimental data indicate that the FeO*/MgO whereas all 400 MPa glasses lie in the tholeiitic field; of magmas can be used to a first approximation as a glasses at 200 MPa straddle the two fields. At 950– proxy to estimate their ponding level or melt generation 925 C, both the 200 and 400 MPa data straddle the two conditions, as we illustrate below for several Santorini fields, but more of the 200 MPa melts are calc-alkaline eruptions. and more of the 400 MPa melts are tholeittic. Hence, it is apparent that the higher the pressure, the more tholei- The plumbing system of single major and minor itic the liquid line of descent. eruptions at Santorini We have therefore used the pressure–temperature Recent eruptions from Santorini are characterized by dependence of the FeO*/MgO of the melt at NNO þ 1 6 intermediate (andesite to dacite) to silicic magmas 05 to define broad domains corresponding to different (evolved dacites to rhyodacites) that volumetrically pressure and temperature intervals (1000–975C, red dominate the sequence. However, when the FeO*/MgO dashed lines or 950–850C, blue dotted lines, Fig. 11). It ratio of such magmas is considered, it is possible to ob- is worth noting that the maximum SiO content reached 2 serve that each eruption generally tapped liquids hav- by our experimental melts does not exceed 72 wt % ing mostly either tholeiitic (i.e. Vourvolous, Lower whereas the residual melts of major rhyodacitic erup- Pumice 1), or calc-alkaline (Minoan) or a mix of both tions exceed this SiO content (e.g. Druitt et al. 1999). 2 affinities (i.e. Lower Pumice 2, Cape Riva (Fig. 11a; Thus we used the data of Cadoux et al. (2014), who per- Druitt et al., 1999). In what follows, we combine the dif- formed experiments on four major rhyodacitic erup- ferent FeO*/MgO ratios of the erupted magmas with tions and at similar conditions (850C, 100–200 MPa, fO 2 our experimental results and previous geochemical and NNO þ 1), to define the shape of the curves for SiO 2 thermal constraints from the literature to provide in- >72 wt %. Figure 11a (and Fig. 10a and b) clearly shows sights on the possible origin and/or source levels of the that at temperatures of 1000–975C, shallow conditions (100 MPa) are required to generate calc-alkaline dacitic– magmas involved during single eruptions of Santorini. rhyodacitic melts whereas tholeiitic equivalents require We stress again that such an approach must be con- pressures between 200 and 400 MPa (Figs 10b and 11a). sidered as a first approximation to depth assessment, with a precision of 640 MPa. At 950–850 C and for SiO2 contents up to 72 wt %, the pressure needed to generate dacites–rhyodacites with tholeiitic affinities is 400 MPa whereas that for calc- Minoan alkaline affinity is 200 MPa. Rhyolitic melts (SiO2 >72 wt Minoan andesites, dacites and the majority of the rhyo- %) having calc-alkaline or tholeiitic affinities require dacitic products have calc-alkaline affinities with just a shallow conditions to be generated (100–200 MPa; small part of the rhyodacites and some hornblende- Fig. 11a). bearing dioritic nodules having FeO*/MgO ratios that It should be noted that, apart from the difference in fall into the tholeiitic field (Fig. 11a; Cottrell et al., 1999; temperature, pressure and oxygen fugacity, volatile ex- Druitt et al., 1999; Druitt, 2014). Pre-eruption tempera- solution during magma ascent could also control or en- tures for rhyodacitic products are 900 C(Cottrell hance the tholeiitic or calc-alkaline affinity of the et al., 1999; Druitt et al., 1999; Cadoux et al., 2014; Druitt, magma, in particular if the magma stored at deep level 2014) whereas temperatures of 990–1016C were is water rich and moderately reduced. As an example, inferred by Michaud et al. (2000) for the andesitic en- our results indicate that, at Santorini, the deep tholeiitic claves dispersed within the more evolved products. dacitic–rhyodacitic liquids generated at 400 MPa at NNO Accordingly, the majority of the andesite to rhyodacite

þ 05 could contain up to 7–8 wt % H2Omelt (Tables 2 calc-alkaline products plot in the 200 MPa field 1914 Journal of Petrology, 2016, Vol. 57, No. 10 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018

Fig. 11. FeO*/MgO vs SiO2 and tholeiitic and calc-alkaline affinities of (a–e) Santorini recent major (silicic- and intermediate-domi- nated compositions) and (f) interplinian eruptions. Natural rock data from Barton & Huijsmans (1986), Gardner et al. (1996), Cottrell et al. (1999), Druitt et al. (1999), Vespa et al. (2006), Gertisser et al. (2009), Fabbro et al. (2013) and Druitt (2014). Errors are equal to symbol size. Red dashed lines and blue dotted lines are explained in the text.

(Fig. 11a). However, the occurrence of a minor group of this work), built by multiple injections of deep-sourced tholeiitic rhyodacites and hornblende dioritic nodules (12–15 km), hot, silicic magma, which, following our re- does suggest that liquids coming from deeper levels sults, could be represented by the small tholeiitic rhyo- (400 MPa) were also involved in the eruption (Cottrell dacitic group (Fig. 11a). Andesites occur as et al., 1999; Druitt et al., 1999; Druitt, 2014). These re- disseminated blobs in the Minoan products. Such blobs sults are altogether consistent with previous depth esti- arise either from late-stage injection of hot andesitic mates for Minoan products (Cottrell et al., 1999; Cadoux magma into the main reservoir or, instead, via the et al., 2014), andesites at Santorini (this work), and vent- remobilization of a pre-existing Ba-rich andesite intru- ing models proposed by Druitt (2014) for this eruption: sion during the build-up of the reservoir (Druitt, 2014). the main calc-alkaline reservoir was lying at levels of 7– In either case, both compositions were erupted together 8 km (200 MPa; Cottrell et al., 1999; Cadoux et al., 2014; during the first phase of the eruption (Druitt, 2014), Journal of Petrology, 2016, Vol. 57, No. 10 1915 which necessarily indicates that both compositions prior to the Cape Riva eruption. In the case of Cape Riva were stored at the same depth (200 MPa) before the our estimates encompass the pressure constraints of eruption. 200 MPa obtained by Cadoux et al. (2014) based on phase equilibrium experiments. Lower Pumice 2 and 1 Lower Pumice 2 (LP2) products have an FeO*/MgO dis- Middle Pumice and Vourvoulous tribution that is similar to the Minoan one but with a We have applied the same reasoning to these domin- tholeiitic rhyodacitic group that extends towards higher antly intermediate-type eruptions. Middle Pumice ju- ratios (Fig. 11b). Because temperatures for the mafic venile products are dominated by a dacitic component Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 magmas and more evolved compositions are 1025C and a minor evolved andesite, separated by a small and <900C(Gertisser et al., 2009; Cadoux et al., 2014), compositional gap (Druitt et al., 1999). Previous tem- again similar to those of the Minoan, this indicates that perature estimates for the Middle Pumice dacites are LP2 magmas were stored between 200 and 400 MPa, about 890C(Gardner et al., 1996) whereas T > 1000C but in this case, with a higher contribution of deeper li- can be assumed for the more andesitic magma quids (Fig. 11b). The distribution of LP2 and Minoan (Michaud et al., 2000; this work). Considering these tem- products contrasts with that of Lower Pumice 1, in peratures, pressures between 400 and 200 MPa can be which all products have clear tholeiitic affinities, indicat- inferred for the dacitic and andesitic products. The ing that, in this case, liquids erupted mostly from a small compositional gap and the presence of reverse 400 MPa level according to the low temperatures esti- compositional zoning in the phenocrysts (Druitt et al., mated for LP1 rhyodacitic magmas (<900C, Cadoux 1999) suggest that a short-duration mixing episode took et al., 2014; Fig. 11c). place at levels pressures as low as 200 MPa. There are no temperature estimates for Vourvoulos magmas yet; Therasia and Cape Riva however, in view of their petrological and chemical sim- The Therasia and Cape Riva (CR) eruptions are sepa- ilarities (i.e. presence of ilmenite; Druitt et al., 1999)to rated in time by only 3000 years, and erupted similar other Santorini magmas (Druitt et al., 1999), similar dacitic magmas (879 6 15C; Fabbro et al., 2013; temperature conditions for the Vourvoulos magmas Cadoux et al., 2014). Dacitic emissions were accompa- can be inferred (<900C for dacites, 1000C for andes- nied in both cases by the co-eruption of an andesite, ites), which yield pressures of about 400 MPa for the which, according to Fabbro et al. (2013), is the product two compositions (Fig. 11e). of the mixing between the dacite and a basaltic magma. This is suggested by textural and chemical features of Interplinian pyroclastic deposits the eruptive products (i.e. presence of sawtooth plagio- Between major Plinian eruptions, smaller eruptive clase zoning, lower FeO* melt contents compared with events (known as interplinian pyroclastic eruptions, Ms their fractionated counterparts of Santorini; Fig. 1). 6 to 11; Fig. 11f ) also occurred, generating in this case However, despite their apparent similarities, the ash, scoria and pumice (Druitt et al., 1999; Vespa et al., Therasia and Cape Riva products differ in their incom- 2006). Compositionally and petrologically the interpli- patible elements (i.e. K, Zr) and rare earth elements nian eruptions are similar to major plinian eruptions. (REE), which rules out any genetic relationship between The main difference is that mafic compositions predom- the magmas (Fabbro et al., 2013). Moreover, when the inate in the interplinian volcanic record (Fig. 11f; Druitt FeO*/MgO melt ratios of both eruptions are considered, et al., 1999; Vespa et al., 2006). The FeO*/MgO ratios of the products also differ (Fig. 11d); dacitic and andesitic these eruptions spread over the 200 and 400 MPa fields: products of Therasia show mainly tholeiitic affinities, however, these estimates could be expanded towards whereas in the case of Cape Riva, two-thirds of the shallower conditions (100 MPa) if ilmenite is part of the products have a dominantly calc-alkaline character. phenocryst assemblage. According to our results the Considering the temperatures estimated for the dacitic presence of this phase constrains temperature (880C; Fabbro et al., 2013) and andesitic magmas to > 975C, which, along with the FeO*/MgO ratio of the (1000 C; this work) and the distribution of erupted prod- melts (<25) and their SiO2 contents (<65 wt %), point ucts in Fig. 11d, a pressure of 400 MPa can be inferred to pressures as low as 100 MPa for the reservoir. for the whole Therasia magma series. In contrast, the fact that Cape Riva products straddle the tholeiitic–calc- Kameni alkaline boundary line suggests that contributions from The post-caldera Kameni products are characterized by two different levels (pressures) occurred prior to the a homogeneous dacitic composition, as described by eruption: 200 MPa for calc-alkaline andesites and Barton & Huijsmans (1986). Those researchers con- 400 MPa for the tholeiitic dacites. In this case, the strained pre-eruptive temperatures at 960–1012C 200 MPa estimate can be extended towards shallower based on thermometry. Ilm was not found in levels as the Cape Riva andesite group straddles the any of the studied samples, in agreement with our re- 200–100 MPa fields (Fig. 11d), suggesting that this was sults concerning the temperature dependence of Ilm probably the depth of mixing and hybrid generation crystallization in Santorini magmas. The distribution of 1916 Journal of Petrology, 2016, Vol. 57, No. 10

FeO*/MgO for Kameni products combined with avail- CONCLUSIONS able temperature estimates constrain pressures to be- The structure of the recent Thera plumbing tween 100 and 200 MPa for the Kameni dacites (Fig. system 11c). This is in general agreement with the estimates of The combination of information concerning the melt Barton & Huijsmans (1986), who used the Cpx–Pl geo- generation and storage conditions of different eruptions barometer to constrain pressures between 80 and over the historical record allows us to reconstruct the 150 MPa for Kameni dacites. These results point to- structure and temporal evolution of the volcanic plumb- wards shallow ponding conditions for the Kameni mag- ing system. Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018 mas (3–6 km), at depths that are similar to those Following Andujar et al. (2015), Santorini basalts calculated for the recent unrest episode in 2011–2012 migrating from the mantle stagnate at depths of 12– (4 km; Newman et al., 2012; Parks et al., 2012; 15 km from where they can either erupt directly (Fig. 12, Foumelis et al., 2013; Papoutsis et al., 2013). arrow 1) or fractionate to generate andesitic liquids. However, the recent study of Druitt (2014) on the These can in turn move towards shallower levels (6– products of the AD 726 eruption found ilmenite and con- 8 km, 200 MPa), pond and create reservoirs feeding strained pre-eruptive temperatures by using Fe–Ti oxy- major intermediate eruptions such as USC-1 and USC-2 thermometers to be between 900 and 930C. This lower (Fig. 12, arrow 2; this work). The subsequent fraction- temperature increases pressure estimates to higher val- ation of these shallow andesites yields calc-alkaline da- ues (400 MPa) for the AD 726 event (Fig. 11). Altogether cite and rhyodacite derivatives such as those of the the Barton & Huijsmans (1986) and Druitt (2014) data Minoan and Lower Pumice 2 eruptions (Figs 10 and 11; are consistent with the hypothesis proposed by Martin Fig. 12, arrows 3). In contrast, when the andesites gen- et al. (2008) and Parks et al. (2012) in which Kameni erated at a depth of 12–15 km keep fractionating there, magmas could evolve at high pressures (400 MPa) and the process produces dacitic to rhyodacitic liquids of then be injected upwards to 100–200 MPa for a short tholeiitic affinity, similar to those feeding Lower Pumice period of time (Martin et al., 2008). 1, Therasia and Ms11 interplinian eruptions (Figs 10 and We conclude that intermediate eruptions of tholeiitic 11; Fig. 12, arrows 4). However, during the ascent from affinity probably tapped andesite and dacite magma depth towards the surface, these evolved tholeiitic li- reservoirs located at depths equivalent to pressures of quids can intercept shallow calc-alkaline andesitic to 200 MPa and temperatures of 1000–975C (i.e. USC-1 rhyodacitic reservoirs, as suggested previously for the and USC-2 eruptions). In contrast, silicic-dominated (da- Lower Pumice 2, Cape Riva and Minoan eruptions (Fig. cite–rhyodacite) eruptions could originate from some- 12, arrow 5). The difference in depth between major what cooler (950–900C) and deeper reservoirs eruptions separated by a short time interval could thus (400 MPa) if tholeiitic, or from shallower ones (200 to explain why eruptions having similar mineral assem- blages, compositions and volumes may or may not 100 MPa) if calc-alkaline. These results reinforce previ- generate (i.e. Lower Pumice 1 and 2; Cape Riva ous observations concerning the complexity of the and Therasia eruptions). This suggests a plumbing sys- plumbing system at Santorini volcano (Martin et al., tem in which magmatic reservoirs at different structural 2008; Druitt et al., 2012; Fabbro et al., 2013; Druitt, 2014) levels can coexist in time (Fabbro et al., 2013). and can be used to understand the different compos- The fact that melts from different depths were itional signatures of magmas involved during single involved in single eruptions could explain the presence eruptions at Santorini. of rare amphibole in recent pyroclastic products We stress here that the intensive conditions (T, P, (Minoan; Lower Pumice 2; Cottrell et al., 1999; Gertisser fO ) inferred for dacitic to rhyodacitic eruptions mostly 2 et al., 2009), as, according to our results, the generation reflect those of melt generation occurring from a USC-1 of dacitic–rhyodacitic melts requires T < 925C and type andesite by crystal fractionation processes. In fact, amphibole fractionation (Fig. 3). This would explain in our estimates largely overlap with previous storage turn the variability observed in H2Omelt contents in melt constraints inferred for these eruptions (i.e. Minoan; inclusions from Minoan products (Druitt et al., 2016) Lower Pumice 2; Cape Riva; see above) so the liquid and the complex zonation patterns recorded in plagio- composition, in some instances, does also mimic those clase phenocrysts from this eruption (Druitt et al., 2012). of equilibration prior to eruption. Nevertheless, we are Melt extraction from different depths prior to or during aware of the limitations of our working procedure: in caldera-forming eruptions is not an uncommon process some cases liquids can record deeper source conditions in large silicic eruptions (e.g. Bishop ; Wallace et al., that could be different from those registered by mag- 1995). mas, phenocrysts or melt inclusions (e.g. Lower Pumice The presence of basaltic andesites carrying a mafic 1; Cadoux et al., 2014; this work). In contrast, pheno- fingerprint (i.e. USC-1) or the occurrence of basaltic en- crysts or melt inclusions could potentially record shal- claves dispersed within the more felsic products indi- lower conditions or short periods of storage than those cates that mafic magmas generated at 12–15 km can of liquids (e.g. Kameni; interplinian eruptions; Druitt intercept the shallower silicic reservoirs and trigger the et al., 2016). eruption, mix and generate hybrid magmas such as Journal of Petrology, 2016, Vol. 57, No. 10 1917 Downloaded from https://academic.oup.com/petrology/article-abstract/57/10/1887/2770690 by CNRS - ISTO user on 14 December 2018

Fig. 12. Schematic view of the plumbing system of the recent Therassia volcanism (see text for details). Eruptions: USC-1,-2, Upper Scoriae 1 and 2; CR, Cape Riva; LP1 and LP2, Lower Pumice 1 and 2. Continuous-line arrows indicate direct magma supply and eruption (1–4). Dashed-line arrows show magma ascent, storage and fractionation (1, 2) and/or interaction with shallower reser- voirs (5).

Therasia–Cape Riva or, instead, pass through the shal- ACKNOWLEDGEMENTS low reservoirs and produce mafic eruptions (Fabbro J.A., B.S. and M.P. thank Dr I. Di Carlo for technical sup- et al., 2013; Andujar et al., 2015). port with SEM–electron microprobe analysis. We thank The depths inferred for the recent Kameni magmas Duncan Muir, Gerhard Worner and an anonymous re- (4–6 km) are slightly shallower than those inferred for viewer for their insightful reviews, which improved the most of the major silicic eruptions (i.e. 7–8 km for paper. Minoan and Lower Pumice 2 magmas). The fact that re- cent magmas could be stored at shallower levels (4 km) after a caldera-forming process suggests that, following each collapse, the volcanic edifice is mostly destroyed FUNDING and major restructuring of the plumbing system takes This work was partly funded by the ANR STOMIXSAN, place, as suggested, for instance, for Vesuvius (Scaillet contract no. ANR08CEAO80, by the INSITU project of et al., 2008) or Mt St Helens (Gardner et al., 1996). re´ gion Centre, and equipex PLANEX (ANR-11-EQPX36), Magmas can then reach shallow depths during the first and LABEX VOLTAIRE. This is Laboratory of Excellence stages of the reactivation of the volcano. However, the ClerVolc contribution number 136. subsequent surface accumulation of erupted material builds a new edifice, leading to an increase of the verti- cal compressive stress field, which would prevent silicic magmas from reaching shallow depths, forcing them to SUPPLEMENTARY DATA pond at increasing pressures as the edifice grows (Pinel Supplementary data for this paper are available at & Jaupart, 2000; Scaillet et al., 2008). Journal of Petrology online. 1918 Journal of Petrology, 2016, Vol. 57, No. 10

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