The NIST Cold Neutron Research Facility

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The NIST Cold Neutron Research Facility Volume 98, Number 1, January-February 1993 Journal of Research of the National Institute of Standards and Technology [J. Res. Natl. Inst. Stand. Technol. 98, 1 (1993)] The NIST Cold Neutron Research Facility Volume 98 Number 1 January-February 1993 H. J. Prask, J. M. Rowe, J. J. The Cold Neutron Research Facility more details on some of the research Rush, and I. G. Schroder (CNRF) at the National Institute of opportunities that the facility will bring standards and Technology (NIST) Re- to NIST. National Institute of Standards search Reactor (NBSR) is now coming on line, with the first seven experimen- Key words: cold neutrons; guide hall; and Technology, tal stations operational, and more sta- neutron facilities; neutron guides; neu- Gaithersburg, MD 20899 tions scheduled to be installed during tron instrumentation; neutron proper- 1992. The present article provides an ties; neutrons; research reactors. introduction to the facility, and to other articles in the current issue that give Accepted: July 8, 1992 1. Introduction Since the advent of nuclear reactors with reason- • the nondestructive nature of low energy neutrons ably high fluence rates (fluxes) in the 1950s, the • the fact that neutrons with wavelengths compara- use of the thermal neutrons produced by these ble to interatomic spacings in condensed matter sources to study a wide range of problems has have energies comparable to the energies of grown rapidly. This growth has resulted from the atomic vibrations. properties of neutrons as probes, which include: The potential of this research was realized early, • absorption with subsequent radioactive decay and the Atomic Energy Commission built a succes- (used as an analytical tool) sion of research reactors with increasing fluence • high penetration as a result of the lack of an elec- rates throughout the 1950s and 1960s. trical charge This potential was also perceived by three physi- • scattering by nuclear interactions (which leads to cists at the National Bureau of Standards (NBS, a nonmonotonic variation of scattering with now NIST)-R. S. Carter, H. Landon, and C. atomic number) Muelhause—who proposed, designed, and built the • special sensitivity to hydrogen and hydrogenous 20 MW research reactor, NBSR, on the new NBS materials along with strong difference in scatter- site in Gaithersburg. The original proposal was jus- ing by hydrogen and deuterium tified on the importance of the contributions that • scattering by magnetic interactions (as a result of the NBSR would provide to the NBS mission in the magnetic dipole of the neutron) analytic chemistry, standards, solid state physics, • simple interpretation of results (as a result of the and nuclear physics, and was intended to serve weak interaction) NBS and other government agencies in the Volume 98, Number 1, January-February 1993 Journal of Research of the National Institute of Standards and Technology Washington area. The reactor design emphasized and the use of large radial penetrations into the versatility, incorporating a large number of experi- high flux regions to maximize intensity for beam mental facilities with different capabilities, rather research. than concentrating on any one specific area of re- Since the reactor first achieved continuous oper- search. The success of this philosophy can be seen ation in 1969, the use of the facilities has grown both in the increasing utilization of the reactor by steadily in both the number of researchers served NIST and other researchers, and in the changing (over 450 research participants the last year before emphasis in programs over the years. The design the CNRF was operational) and in the breadth of also included many advanced features that have the community served (the 450 participants came since been incorporated into other designs, includ- from 15 NIST divisions or offices, 25 other govern- ing a completely passive emergency cooling system, ment agencies, 50 universities and 25 industrial lab- a novel split core fuel design (recently adopted into oratories). The NBSR has gone from a local designs for the Advanced Neutron Source and the resource to a truly national facility, with re- spallation source at Los Alamos National Labora- searchers from all over the country. A diagram of tory), helium and carbon dioxide blankets around the current layout of facilities around the reactor is high flux regions to reduce radioactive emissions. shown in Fig. 1. Polarized Beam Triple-Axis Spectrometer Dlffractometer^ Single Crystal Dlffractometer Triple-Axis Spectrometer Thermal Column Radiography Facility BT-5 To Be Developed High Resolution Powder Dlffractometer Triple-Axis Spectrometer Polarized Beam I Spectrometer Fig. 1. Principal experimental facilities in the reactor hall. Volume 98, Number 1, January-February 1993 Journal of Research of the National Institute of Standards and Technology One of the features incorporated into the design from the MeV energies typical of nuclear reactions was the large penetration for a "cold neutron down to the meV energies typical of atomic mo- source" shown in Fig. 1. From the beginning, the tions in thermal equilibrium at approximately room designers intended that this penetration would one temperature. The energy spectrum produced by day be used to provide an intense source of neu- such moderators is a Maxwellian distribution with trons with lower energies than those typical of a characteristic temperature close to that of the other ports by installation of a cryogenically cooled moderator itself—hence the name thermal neu- block of neutron moderator. A moderator for neu- trons. An example of such a spectrum is shown in trons is a material which scatters the neutrons pro- Fig. 2, with temperature chosen to represent the duced by fission so that their energy is reduced spectrum seen by the thermal beam tubes at the 10^3 B—I—I—I—r 10^2 ca 10" 0,0 Ice (40 K) 03 10»° 10» 108 107 0,0 Ice (300 K) 10« I , I , , I _, L 0.00 0.50 1.00 1.50 2.00 Wavelength (nm) ^ 15.0 —J I J I I J l— -i—I—!—;—I—I—I—I—r o o I °c, 10.0 Q \ o o 5.0 CM 1=1 as 0.0 0.00 0.50 1.00 1.50 2.00 Wavelength (nm) b Fig. 2. (a) Neutron fluxes for the cold moderator cavity filled with liquid D2O and D2O ice. (b) Flux gain, D20(ice)/D20(liquid), from the data of (a). The moderator temperature of 40 K produces a Maxwellian distribution with an "effective" tempera- ture of 60 K. Volume 98, Number 1, January-February 1993 Journal of Research of the National Institute of Standards and Technology NBSR. Cold neutrons are defined as those with en- trons lO's of meters away from the reactor into ergies less than 5 meV, corresponding to 60 K and large experimental halls (generally called guide velocities less than 1000 m/s. However, this cold halls). These guides are based on the total internal neutron port was not utilized at the beginning, and reflection of neutrons below a critical angle that is the development concentrated on the thermal neu- a function of the reflecting material and neutron tron beams and facilities. In 1985, the development energy. This reflection is exactly analogous to opti- of the cryogenic port began in earnest with funding cal reflection, and the critical angle depends on the of a cold neutron initiative (made possible by pre- deBroglie wavelength of the neutron, which is in- liminary funding from the NBS director in 1984). versely proportional to neutron velocity and equal As discussed below, events have shown that the to 0.4 nm at 1000 m/s. Thus, guides work best at large area allowed for a. cold source in the NBSR long wavelengths and therefore for cold neutrons. design and the very wide range of angular access The guides themselves consist of pipes which are (over 30°) was a key to providing a unique opportu- made of optically flat glass coated with materials of nity to create the only fully internationally competi- high scattering power (generally an isotope of tive cold neutron research capability in the United nickel) and which are evacuated in order to reduce States. losses due to air scattering. Using these devices, it The interest in applications of cold neutron tech- is possible to transport intense beams of cold neu- niques was stimulated by the success of the West- trons out of the reactor building with losses of less ern European research reactors, most notably the than 1%/m, thus opening up the possibility of cre- Institut Laue Langevin (ILL) in Grenoble, France. ating many new types of measurement capability in Among the many successes of these facilities was a large new experimental hall. the demonstration of the power of a technique Based on these considerations, NBS proposed a called Small Angle Neutron Scattering (SANS) as cold neutron facility for the FY1985 budget, and it applied to a wide variety of problems in polymers, was included in the budget submission to the De- biology, metallurgy, and other areas in which struc- partment of Commerce and 0MB for that year. tures with distance scales in the 1-100 nm range However, many proposals for new facilities were were critical. The United States was highly compet- submitted at that time from different agencies, so itive in atomic and molecular scale measurements the Office of Science and Technology Policy re- with thermal neutrons, but was far behind in uti- quested a national study to set priorities for these lization of longer wavelength neutrons, and the facilities. As a result, the National Academy of Sci- SANS technique was the area addressed first. In ences commissioned a study by a panel of the Na- 1979 one of the first competence proposals funded tional Research Council on "Major Facilities for by the NBS director was to develop a SANS spec- Materials Sciences and Related Disciplines" trometer and research program at the NBSR, chaired by Professor F.
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