Nucleosynthesis
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Subterranean Production of Neutrons, $^{39} $ Ar and $^{21} $ Ne: Rates
Subterranean production of neutrons, 39Ar and 21Ne: Rates and uncertainties Ondrejˇ Srˇ amek´ a,∗, Lauren Stevensb, William F. McDonoughb,c,∗∗, Sujoy Mukhopadhyayd, R. J. Petersone aDepartment of Geophysics, Faculty of Mathematics and Physics, Charles University, V Holeˇsoviˇck´ach 2, 18000 Praha 8, Czech Republic bDepartment of Chemistry and Biochemistry, University of Maryland, College Park, MD 20742, United States cDepartment of Geology, University of Maryland, College Park, MD 20742, United States dDepartment of Earth and Planetary Sciences, University of California Davis, Davis, CA 95616, United States eDepartment of Physics, University of Colorado Boulder, Boulder, CO 80309-0390, United States Abstract Accurate understanding of the subsurface production rate of the radionuclide 39Ar is necessary for argon dating tech- niques and noble gas geochemistry of the shallow and the deep Earth, and is also of interest to the WIMP dark matter experimental particle physics community. Our new calculations of subsurface production of neutrons, 21Ne, and 39Ar take advantage of the state-of-the-art reliable tools of nuclear physics to obtain reaction cross sections and spectra (TALYS) and to evaluate neutron propagation in rock (MCNP6). We discuss our method and results in relation to pre- vious studies and show the relative importance of various neutron, 21Ne, and 39Ar nucleogenic production channels. Uncertainty in nuclear reaction cross sections, which is the major contributor to overall calculation uncertainty, is estimated from variability in existing experimental and library data. Depending on selected rock composition, on the order of 107–1010 α particles are produced in one kilogram of rock per year (order of 1–103 kg−1 s−1); the number of produced neutrons is lower by ∼ 6 orders of magnitude, 21Ne production rate drops by an additional factor of 15–20, and another one order of magnitude or more is dropped in production of 39Ar. -
Monitored Natural Attenuation of Inorganic Contaminants in Ground
Monitored Natural Attenuation of Inorganic Contaminants in Ground Water Volume 3 Assessment for Radionuclides Including Tritium, Radon, Strontium, Technetium, Uranium, Iodine, Radium, Thorium, Cesium, and Plutonium-Americium EPA/600/R-10/093 September 2010 Monitored Natural Attenuation of Inorganic Contaminants in Ground Water Volume 3 Assessment for Radionuclides Including Tritium, Radon, Strontium, Technetium, Uranium, Iodine, Radium, Thorium, Cesium, and Plutonium-Americium Edited by Robert G. Ford Land Remediation and Pollution Control Division Cincinnati, Ohio 45268 and Richard T. Wilkin Ground Water and Ecosystems Restoration Division Ada, Oklahoma 74820 Project Officer Robert G. Ford Land Remediation and Pollution Control Division Cincinnati, Ohio 45268 National Risk Management Research Laboratory Office of Research and Development U.S. Environmental Protection Agency Cincinnati, Ohio 45268 Notice The U.S. Environmental Protection Agency through its Office of Research and Development managed portions of the technical work described here under EPA Contract No. 68-C-02-092 to Dynamac Corporation, Ada, Oklahoma (David Burden, Project Officer) through funds provided by the U.S. Environmental Protection Agency’s Office of Air and Radiation and Office of Solid Waste and Emergency Response. It has been subjected to the Agency’s peer and administrative review and has been approved for publication as an EPA document. Mention of trade names or commercial products does not constitute endorsement or recommendation for use. All research projects making conclusions or recommendations based on environmental data and funded by the U.S. Environmental Protection Agency are required to participate in the Agency Quality Assurance Program. This project did not involve the collection or use of environmental data and, as such, did not require a Quality Assurance Plan. -
Tracer Applications of Noble Gas Radionuclides in the Geosciences
To be published in Earth-Science Reviews Tracer Applications of Noble Gas Radionuclides in the Geosciences (August 20, 2013) Z.-T. Lua,b, P. Schlosserc,d, W.M. Smethie Jr.c, N.C. Sturchioe, T.P. Fischerf, B.M. Kennedyg, R. Purtscherth, J.P. Severinghausi, D.K. Solomonj, T. Tanhuak, R. Yokochie,l a Physics Division, Argonne National Laboratory, Argonne, Illinois, USA b Department of Physics and Enrico Fermi Institute, University of Chicago, Chicago, USA c Lamont-Doherty Earth Observatory, Columbia University, Palisades, New York, USA d Department of Earth and Environmental Sciences and Department of Earth and Environmental Engineering, Columbia University, New York, USA e Department of Earth and Environmental Sciences, University of Illinois at Chicago, Chicago, IL, USA f Department of Earth and Planetary Sciences, University of New Mexico, Albuquerque, USA g Center for Isotope Geochemistry, Lawrence Berkeley National Laboratory, Berkeley, USA h Climate and Environmental Physics, Physics Institute, University of Bern, Bern, Switzerland i Scripps Institution of Oceanography, University of California, San Diego, USA j Department of Geology and Geophysics, University of Utah, Salt Lake City, USA k GEOMAR Helmholtz Center for Ocean Research Kiel, Marine Biogeochemistry, Kiel, Germany l Department of Geophysical Sciences, University of Chicago, Chicago, USA Abstract 81 85 39 Noble gas radionuclides, including Kr (t1/2 = 229,000 yr), Kr (t1/2 = 10.8 yr), and Ar (t1/2 = 269 yr), possess nearly ideal chemical and physical properties for studies of earth and environmental processes. Recent advances in Atom Trap Trace Analysis (ATTA), a laser-based atom counting method, have enabled routine measurements of the radiokrypton isotopes, as well as the demonstration of the ability to measure 39Ar in environmental samples. -
The R-Process Nucleosynthesis and Related Challenges
EPJ Web of Conferences 165, 01025 (2017) DOI: 10.1051/epjconf/201716501025 NPA8 2017 The r-process nucleosynthesis and related challenges Stephane Goriely1,, Andreas Bauswein2, Hans-Thomas Janka3, Oliver Just4, and Else Pllumbi3 1Institut d’Astronomie et d’Astrophysique, Université Libre de Bruxelles, CP 226, 1050 Brussels, Belgium 2Heidelberger Institut fr¨ Theoretische Studien, Schloss-Wolfsbrunnenweg 35, 69118 Heidelberg, Germany 3Max-Planck-Institut für Astrophysik, Postfach 1317, 85741 Garching, Germany 4Astrophysical Big Bang Laboratory, RIKEN, 2-1 Hirosawa, Wako, Saitama, 351-0198, Japan Abstract. The rapid neutron-capture process, or r-process, is known to be of fundamental importance for explaining the origin of approximately half of the A > 60 stable nuclei observed in nature. Recently, special attention has been paid to neutron star (NS) mergers following the confirmation by hydrodynamic simulations that a non-negligible amount of matter can be ejected and by nucleosynthesis calculations combined with the predicted astrophysical event rate that such a site can account for the majority of r-material in our Galaxy. We show here that the combined contribution of both the dynamical (prompt) ejecta expelled during binary NS or NS-black hole (BH) mergers and the neutrino and viscously driven outflows generated during the post-merger remnant evolution of relic BH-torus systems can lead to the production of r-process elements from mass number A > 90 up to actinides. The corresponding abundance distribution is found to reproduce the∼ solar distribution extremely well. It can also account for the elemental distributions observed in low-metallicity stars. However, major uncertainties still affect our under- standing of the composition of the ejected matter. -
OLLI: the Birth, Life, and Death Of
The Birth, Life, and Death of Stars The Osher Lifelong Learning Institute Florida State University Jorge Piekarewicz Department of Physics [email protected] Schedule: September 29 – November 3 Time: 11:30am – 1:30pm Location: Pepper Center, Broad Auditorium J. Piekarewicz (FSU-Physics) The Birth, Life, and Death of Stars Fall 2014 1 / 12 Ten Compelling Questions What is the raw material for making stars and where did it come from? What forces of nature contribute to energy generation in stars? How and where did the chemical elements form? ? How long do stars live? How will our Sun die? How do massive stars explode? ? What are the remnants of such stellar explosions? What prevents all stars from dying as black holes? What is the minimum mass of a black hole? ? What is role of FSU researchers in answering these questions? J. Piekarewicz (FSU-Physics) The Birth, Life, and Death of Stars Fall 2014 2 / 12 The Birth of Carbon: The Triple-Alpha Reaction The A=5 and A=8 Bottle-Neck 5 −22 p + α ! Li ! p + α (t1=2 ≈10 s) 8 −16 α + α ! Be ! α + α (t1=2 ≈10 s) BBN does not generate any heavy elements! He-ashes fuse in the hot( T ≈108 K) and dense( n≈1028 cm−3) core 8 −8 Physics demands a tiny concentration of Be (n8=n4 ≈10 ) Carbon is formed: α + α ! 8Be + α ! 12C + γ (7:367 MeV) Every atom in our body has been formed in stellar cores! J. Piekarewicz (FSU-Physics) The Birth, Life, and Death of Stars Fall 2014 3 / 12 Stellar Nucleosynthesis: From Carbon to Iron Stars are incredibly efficient thermonuclear furnaces Heavier He-ashes fuse to produce: C,N,O,F,Ne,Na,Mg,.. -
Electron Capture in Stars
Electron capture in stars K Langanke1;2, G Mart´ınez-Pinedo1;2;3 and R.G.T. Zegers4;5;6 1GSI Helmholtzzentrum f¨urSchwerionenforschung, D-64291 Darmstadt, Germany 2Institut f¨urKernphysik (Theoriezentrum), Department of Physics, Technische Universit¨atDarmstadt, D-64298 Darmstadt, Germany 3Helmholtz Forschungsakademie Hessen f¨urFAIR, GSI Helmholtzzentrum f¨ur Schwerionenforschung, D-64291 Darmstadt, Germany 4 National Superconducting Cyclotron Laboratory, Michigan State University, East Lansing, Michigan 48824, USA 5 Joint Institute for Nuclear Astrophysics: Center for the Evolution of the Elements, Michigan State University, East Lansing, Michigan 48824, USA 6 Department of Physics and Astronomy, Michigan State University, East Lansing, Michigan 48824, USA E-mail: [email protected], [email protected], [email protected] Abstract. Electron captures on nuclei play an essential role for the dynamics of several astrophysical objects, including core-collapse and thermonuclear supernovae, the crust of accreting neutron stars in binary systems and the final core evolution of intermediate mass stars. In these astrophysical objects, the capture occurs at finite temperatures and at densities at which the electrons form a degenerate relativistic electron gas. The capture rates can be derived in perturbation theory where allowed nuclear transitions (Gamow-Teller transitions) dominate, except at the higher temperatures achieved in core-collapse supernovae where also forbidden transitions contribute significantly to the rates. There has been decisive progress in recent years in measuring Gamow-Teller (GT) strength distributions using novel experimental techniques based on charge-exchange reactions. These measurements provide not only data for the GT distributions of ground states for many relevant nuclei, but also serve as valuable constraints for nuclear models which are needed to derive the capture rates for the arXiv:2009.01750v1 [nucl-th] 3 Sep 2020 many nuclei, for which no data exist yet. -
Star Factories: Nuclear Fusion and the Creation of the Elements
Star Factories: Nuclear Fusion and the Creation of the Elements Science In the River City workshop 3/22/11 Chris Taylor Department of Physics and Astronomy Sacramento State Introductions! Science Content Standards, Grades 9 - 12 Earth Sciences: Earth's Place in the Universe 1.e ''Students know the Sun is a typical star and is powered by nuclear reactions, primarily the fusion of hydrogen to form helium.'' 2.c '' Students know the evidence indicating that all elements with an atomic number greater than that of lithium have been formed by nuclear fusion in stars.'' Three topics tonight: 1) how do we know all the heavier elements are made in stars? (Big Bang theory) 2) How do stars make elements as heavy as or less heavy than iron? (Stellar nucleosynthesis) 3) How do stars make elements heavier than iron? (Supernovae) Big Bang Nucleosynthesis The Big Bang theory predicts that when the universe first formed, the only matter that existed was hydrogen, helium, and very tiny amounts of lithium. If this is true, then all other elements must have been created in stars. Astronomers use spectroscopy to examine the light emitted by distant stars to determine what kinds of atoms are in them. We've learned that most stars contain nearly every element in the periodic table. The spectrum of the Sun In order to measure measure what kinds of atoms were around in the earliest days of the Universe, we look for stars that were made out of fresh, primordial gas. The closest we can get to this is looking at dwarf galaxies, which show extremely low levels of elements heavier than helium. -
Arxiv:1901.01410V3 [Astro-Ph.HE] 1 Feb 2021 Mental Information Is Available, and One Has to Rely Strongly on Theoretical Predictions for Nuclear Properties
Origin of the heaviest elements: The rapid neutron-capture process John J. Cowan∗ HLD Department of Physics and Astronomy, University of Oklahoma, 440 W. Brooks St., Norman, OK 73019, USA Christopher Snedeny Department of Astronomy, University of Texas, 2515 Speedway, Austin, TX 78712-1205, USA James E. Lawlerz Physics Department, University of Wisconsin-Madison, 1150 University Avenue, Madison, WI 53706-1390, USA Ani Aprahamianx and Michael Wiescher{ Department of Physics and Joint Institute for Nuclear Astrophysics, University of Notre Dame, 225 Nieuwland Science Hall, Notre Dame, IN 46556, USA Karlheinz Langanke∗∗ GSI Helmholtzzentrum f¨urSchwerionenforschung, Planckstraße 1, 64291 Darmstadt, Germany and Institut f¨urKernphysik (Theoriezentrum), Fachbereich Physik, Technische Universit¨atDarmstadt, Schlossgartenstraße 2, 64298 Darmstadt, Germany Gabriel Mart´ınez-Pinedoyy GSI Helmholtzzentrum f¨urSchwerionenforschung, Planckstraße 1, 64291 Darmstadt, Germany; Institut f¨urKernphysik (Theoriezentrum), Fachbereich Physik, Technische Universit¨atDarmstadt, Schlossgartenstraße 2, 64298 Darmstadt, Germany; and Helmholtz Forschungsakademie Hessen f¨urFAIR, GSI Helmholtzzentrum f¨urSchwerionenforschung, Planckstraße 1, 64291 Darmstadt, Germany Friedrich-Karl Thielemannzz Department of Physics, University of Basel, Klingelbergstrasse 82, 4056 Basel, Switzerland and GSI Helmholtzzentrum f¨urSchwerionenforschung, Planckstraße 1, 64291 Darmstadt, Germany (Dated: February 2, 2021) The production of about half of the heavy elements found in nature is assigned to a spe- cific astrophysical nucleosynthesis process: the rapid neutron capture process (r-process). Although this idea has been postulated more than six decades ago, the full understand- ing faces two types of uncertainties/open questions: (a) The nucleosynthesis path in the nuclear chart runs close to the neutron-drip line, where presently only limited experi- arXiv:1901.01410v3 [astro-ph.HE] 1 Feb 2021 mental information is available, and one has to rely strongly on theoretical predictions for nuclear properties. -
Heavy Element Nucleosynthesis
Heavy Element Nucleosynthesis A summary of the nucleosynthesis of light elements is as follows 4He Hydrogen burning 3He Incomplete PP chain (H burning) 2H, Li, Be, B Non-thermal processes (spallation) 14N, 13C, 15N, 17O CNO processing 12C, 16O Helium burning 18O, 22Ne α captures on 14N (He burning) 20Ne, Na, Mg, Al, 28Si Partly from carbon burning Mg, Al, Si, P, S Partly from oxygen burning Ar, Ca, Ti, Cr, Fe, Ni Partly from silicon burning Isotopes heavier than iron (as well as some intermediate weight iso- topes) are made through neutron captures. Recall that the prob- ability for a non-resonant reaction contained two components: an exponential reflective of the quantum tunneling needed to overcome electrostatic repulsion, and an inverse energy dependence arising from the de Broglie wavelength of the particles. For neutron cap- tures, there is no electrostatic repulsion, and, in complex nuclei, virtually all particle encounters involve resonances. As a result, neutron capture cross-sections are large, and are very nearly inde- pendent of energy. To appreciate how heavy elements can be built up, we must first consider the lifetime of an isotope against neutron capture. If the cross-section for neutron capture is independent of energy, then the lifetime of the species will be ( )1=2 1 1 1 µn τn = ≈ = Nnhσvi NnhσivT Nnhσi 2kT For a typical neutron cross-section of hσi ∼ 10−25 cm2 and a tem- 8 9 perature of 5 × 10 K, τn ∼ 10 =Nn years. Next consider the stability of a neutron rich isotope. If the ratio of of neutrons to protons in an atomic nucleus becomes too large, the nucleus becomes unstable to beta-decay, and a neutron is changed into a proton via − (Z; A+1) −! (Z+1;A+1) + e +ν ¯e (27:1) The timescale for this decay is typically on the order of hours, or ∼ 10−3 years (with a factor of ∼ 103 scatter). -
Appendix A: Scientific Notation
Appendix A: Scientific Notation Since in astronomy we often have to deal with large numbers, writing a lot of zeros is not only cumbersome, but also inefficient and difficult to count. Scientists use the system of scientific notation, where the number of zeros is short handed to a superscript. For example, 10 has one zero and is written as 101 in scientific notation. Similarly, 100 is 102, 100 is 103. So we have: 103 equals a thousand, 106 equals a million, 109 is called a billion (U.S. usage), and 1012 a trillion. Now the U.S. federal government budget is in the trillions of dollars, ordinary people really cannot grasp the magnitude of the number. In the metric system, the prefix kilo- stands for 1,000, e.g., a kilogram. For a million, the prefix mega- is used, e.g. megaton (1,000,000 or 106 ton). A billion hertz (a unit of frequency) is gigahertz, although I have not heard of the use of a giga-meter. More rarely still is the use of tera (1012). For small numbers, the practice is similar. 0.1 is 10À1, 0.01 is 10À2, and 0.001 is 10À3. The prefix of milli- refers to 10À3, e.g. as in millimeter, whereas a micro- second is 10À6 ¼ 0.000001 s. It is now trendy to talk about nano-technology, which refers to solid-state device with sizes on the scale of 10À9 m, or about 10 times the size of an atom. With this kind of shorthand convenience, one can really go overboard. -
Radiogenic Isotope Geochemistry
W. M. White Geochemistry Chapter 8: Radiogenic Isotope Geochemistry CHAPTER 8: RADIOGENIC ISOTOPE GEOCHEMISTRY 8.1 INTRODUCTION adiogenic isotope geochemistry had an enormous influence on geologic thinking in the twentieth century. The story begins, however, in the late nineteenth century. At that time Lord Kelvin (born William Thomson, and who profoundly influenced the development of physics and ther- R th modynamics in the 19 century), estimated the age of the solar system to be about 100 million years, based on the assumption that the Sun’s energy was derived from gravitational collapse. In 1897 he re- vised this estimate downward to the range of 20 to 40 million years. A year earlier, another Eng- lishman, John Jolly, estimated the age of the Earth to be about 100 million years based on the assump- tion that salts in the ocean had built up through geologic time at a rate proportional their delivery by rivers. Geologists were particularly skeptical of Kelvin’s revised estimate, feeling the Earth must be older than this, but had no quantitative means of supporting their arguments. They did not realize it, but the key to the ultimate solution of the dilemma, radioactivity, had been discovered about the same time (1896) by Frenchman Henri Becquerel. Only eleven years elapsed before Bertram Boltwood, an American chemist, published the first ‘radiometric age’. He determined the lead concentrations in three samples of pitchblende, a uranium ore, and concluded they ranged in age from 410 to 535 million years. In the meantime, Jolly also had been busy exploring the uses of radioactivity in geology and published what we might call the first book on isotope geochemistry in 1908. -
Sensitivity of Type Ia Supernovae to Electron Capture Rates E
A&A 624, A139 (2019) Astronomy https://doi.org/10.1051/0004-6361/201935095 & c ESO 2019 Astrophysics Sensitivity of Type Ia supernovae to electron capture rates E. Bravo E.T.S. Arquitectura del Vallès, Universitat Politècnica de Catalunya, Carrer Pere Serra 1-15, 08173 Sant Cugat del Vallès, Spain e-mail: [email protected] Received 22 January 2019 / Accepted 8 March 2019 ABSTRACT The thermonuclear explosion of massive white dwarfs is believed to explain at least a fraction of Type Ia supernovae (SNIa). After thermal runaway, electron captures on the ashes left behind by the burning front determine a loss of pressure, which impacts the dynamics of the explosion and the neutron excess of matter. Indeed, overproduction of neutron-rich species such as 54Cr has been deemed a problem of Chandrasekhar-mass models of SNIa for a long time. I present the results of a sensitivity study of SNIa models to the rates of weak interactions, which have been incorporated directly into the hydrodynamic explosion code. The weak rates have been scaled up or down by a factor ten, either globally for a common bibliographical source, or individually for selected isotopes. In line with previous works, the impact of weak rates uncertainties on sub-Chandrasekhar models of SNIa is almost negligible. The impact on the dynamics of Chandrasekhar-mass models and on the yield of 56Ni is also scarce. The strongest effect is found on the nucleosynthesis of neutron-rich nuclei, such as 48Ca, 54Cr, 58Fe, and 64Ni. The species with the highest influence on nucleosynthesis do not coincide with the isotopes that contribute most to the neutronization of matter.