Landfill Mining: Prospecting metal in Gärstad landfill
Ariana Tanha Daniel Zarate Division of Environmental Technology and Management
Master Thesis Department of Management and Engineering LIU-IEI-TEK-A- -12/01454- -SE
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Landfill Mining: Prospecting metal in Gärstad landfill
Master Thesis in Landfill Mining Department of Management and Engineering Division of Environmental Technology and Management Linköping University by
Ariana Tanha Daniel Zarate
LIU-IEI-TEK-A- -12/01454- -SE
Supervisors: NILS JOHANSSON
IEI, Linköping University
MAGNUS HAMMAR
Tekniska Verken i Linköping
Examiner: JOAKIM KROOK
IEI, Linköping University
Linköping, 19 September, 2012
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Linköping University Electronic Press
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© Ariana Tanha, Daniel Zarate.
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Abstract All processes in society produce waste. In nature, the waste is normally used as a resource for another process, but in human societies waste is often discarded. These discarded materials end up in places for depositing waste known as landfills. The increase in population, and humans’ tendency to improve their quality of life, has led to an increase in consumption of material. More material consumption means generating more waste, and more waste means bigger landfills. The increasing size of landfills has brought some other issues, such as increased land use and higher environmental impact. However in these landfills a lot of valuable materials are discarded and the concept of landfill mining (LFM) has been proposed in order to solve these issues and use landfills as a possible source of materials. Landfill mining is not yet a common practice, and the first barrier for this is the uncertainty of the amount and value of materials within landfills.
The purpose of this study is to prospect the amount of metals in one specific landfill, in this case Gärstad landfill in Linköping, Sweden. This is a first step to show the feasibility of landfill mining as an alternative way of extracting materials. The study is limited only to metals because they are one of the most important resources in today’s society.
The theoretical background of the study is based on material flow analysis (MFA). Two approaches are used to study the materials in the landfill. The first is top‐down which studies the flows of materials and the second is bottom‐up which studies the stocks of material in the landfill. Based on these approaches the method was developed. First the system boundaries in time and space were defined. Then the amount of waste in landfill was estimated from the two mentioned approaches. In the end the metal content of the waste was estimated. Some criteria are also defined to compare the accessibility of the metals in the landfill.
The results of this study show that there is a considerable amount of metals in the landfill, and that ash deposits resulting from incineration are the most interesting source of metals; with iron, aluminium, copper and zinc being the most abundant. The results are presented by type of waste, area of the landfill and accessibility in order to identify the hotspots.
Later it is discussed that the method is cheap and fast but highly depends on previous data and available information. Also the metal content of the landfill is compared with natural ores. In the end the metal content of the landfill is evaluated and estimated to be around 3 billion SEK. It shows that aluminium, titanium and copper have the highest value money wise.
As conclusion it was shown material flow analysis is a valid way to prospect landfills. But further cost‐ benefit analysis must be carried out to determine if landfill mining is justifiable. Also some recommendations are proposed to Tekniska Verken in order to facilitate future studies. The first is to develop a systematic way for landfilling different kind of waste and document them. Second is to include metals which have economic potential in the regular sampling from landfill.
Keywords waste, landfill, landfill mining, material flow analysis, metals, metal stocks, ashes.
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Acknowledgements We would like to thank Nisse, our supervisor, who despite of being on parental leave met with us regularly to provide guidance and feedback, and his son Mio, who brought joy to our supervisory meetings.
We would like to thank Magnus Hammar from Tekniska Verken, our contact person, who always provided us with necessary data, information and amusing comment in his emails, even though he was very busy at work.
We would like to thank Joakim Krook, our examiner, for his guidance and help during writing the thesis.
Finally we would like to thank all the people who in some way or another where involved and helped in this process.
Linköping, September, 2012 Ariana Tanha Daniel Zarate
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Table of Contents 1 Introduction ...... 15 1.1 Aim ...... 15 1.2 Limitation ...... 16 1.3 Background ...... 16 2 Theoretical Framework ...... 19 2.1 Industrial Ecology ...... 19 2.2 Landfill Mining ...... 20 2.3 MFA (Material Flow Analysis) ...... 21 3 Method ...... 23 3.1 Assumptions ...... 25 4 Collected Data and Estimations ...... 27 4.1 Gärstad Landfill History ...... 28 4.1.1 The old Incinerator ...... 28 4.1.2 KV1 ...... 28 4.1.3 Gärstad Verket ...... 28 4.1.4 FUDD ...... 29 4.1.5 Landfill Tax ...... 29 4.2 Flows and stocks of waste ...... 29 4.2.1 Estimation of flows between 1974‐1990 and outflows ...... 32 4.2.2 Waste flow history...... 33 4.3 Concentrations ...... 33 4.3.1 Ashes ...... 33 4.3.2 Construction and demolition waste ...... 35 4.3.3 Me‐OH Sludge...... 36 4.3.4 Household Waste ...... 36 4.3.5 Mixed Waste ...... 37 4.3.6 Others ...... 37 4.4 Accessibility Criteria ...... 37 5 Results ...... 39 5.1 Scrap metal ...... 40 5.2 Metal content in ashes ...... 40 5.3 Metal content in C&D waste ...... 41 5.4 Metal content in Metal hydroxide sludge ...... 42
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5.5 Metal Content in Household Waste ...... 42 5.6 Metal Content by Areas ...... 43 5.7 Accessibility and Hotspots ...... 44 6 Discussion ...... 47 6.1 Method ...... 47 6.2 Data ...... 47 6.3 Comparing concentrations with mining ...... 48 6.4 Comparing LFM with modern mining ...... 48 6.5 Value ...... 50 6.6 National Numbers ...... 50 6.6.1 Gärstad landfill as a source of material ...... 51 7 Conclusion ...... 53 7.1 Recommendations for the company ...... 53 8 Bibliography ...... 55 Appendix A: Inflows of the landfill per year ...... 59 Appendix B: Metal amounts in different types of ash ...... 65
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List of Figures Figure 1: Location of Gärstad landfill, 3 Km northeast of Linköping, Sweden...... 18 Figure 2: The life cycle of a product; the disposal stage includes all the material inside a landfill...... 19 Figure 3: Closing the loop; instead of disposing of material, they are reinserted into the life cycle. Own illustration based on Frosch & Gallopoulos (1989) ...... 19 Figure 4: Diagram of the two methods used in the study. The left one was used for estimating amounts of landfilled waste and metal and the right for verifying the amount of waste and allocating the metal...... 24 Figure 5: The different areas of Gärstad landfill, each area used for different purposes, except for E which is a lake...... 27 Figure 6: Ashes in all forms (BA, FA and sludge) sent from each power plant for landfilling in Gärstad. The old incinerator was decommissioned in 1980 and thus no more ash was sent from there. Own illustration, based on data from all Gärstad landfill environmental reports and county administration permissions...... 29 Figure 7: Schematic view of the waste flows to and from the landfill (the oval shape) currently. The two circles are power plants that send their incineration residue to landfill which makes up around 85% of the total incoming waste...... 31 Figure 8: The landfilled amount of main types of wastes since landfill started operating, 1974 until now, 2011...... 33 Figure 9: Estimated amount of landfilled metals in all forms calculated from flows of waste...... 39 Figure 10: Estimated amount of different metals in all types of landfilled ash...... 41
List of Tables Table 1: generated and treated waste in Sweden in years 2004, 2006 and 2008 (dry weight) (Naturvårdverket, 2012). The landfilled mining waste is the landfilled waste generated from the mining industry and should not be confused with LFM...... 17 Table 2: Usage description of the landfill areas...... 27 Table 3: All identified waste flows of Gärstad; from which the interesting waste flows were selected for calculating metal amount in the landfill ...... 30 Table 4: Area, volume and waste content of each area until 2009 (Hammar, 2012)...... 32 Table 5: Identified outflows of ash from Gärstad landfill...... 33 Table 6: Estimated metal concentrations in bottom ash generated from different fuels (waste, coal and wood)...... 34 Table 7: Estimated metal concentrations in fly ash, generated from different fuels; and for wood from different filters...... 34 Table 8: Conversion factor used to obtain the amount of metals from their oxide form...... 35 Table 9: Estimated metal concentrations in C&D waste based on (Boverket, 1998)...... 35 Table 10: Concentrations of metal in me‐OH sludge from different studies (weight %)...... 36 Table 11: Estimated metal concentrations in household waste ...... 36 Table 12: Accessibility criteria applied to different areas of the landfill...... 38 Table 13: Estimated total amount of waste based on flows approach; and estimated amount of landfilled metals in all forms calculated from flows of waste and its ratio compared to total amount of waste...... 39
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Table 14: Estimated total amount of waste based on volume approach; and estimated amount of metals using the rate from the flows approach...... 40 Table 15: Estimated total amount of scrap metal in the landfill, and its rate compared to the total amount of waste...... 40 Table 16: Estimated total amount of landfilled ash and the estimated amount of metals within...... 40 Table 17 : Iron and Aluminium in scrap form in bottom ash from waste incineration...... 41 Table 18: Total amount of landfilled C&D waste and the estimated amount of metals within...... 42 Table 19: Total amount of me‐OH waste and the estimated amount of metals within...... 42 Table 20: Total amount of Household waste and the estimated amount of metals within...... 43 Table 21: Estimated amount of metals in A0 ...... 43 Table 22: Estimated amount of metals in A1, underground ...... 43 Table 23: Estimated amount of metals in A1, above ground ...... 43 Table 24: Estimated amount of metals in A2, underground ...... 43 Table 25: Estimated amount of metals in A2 aboveground ...... 44 Table 26: Estimated amount of metals in FUDD cell ...... 44 Table 27: Estimated amount of metals in B ...... 44 Table 28: Estimated amount of metals in C ...... 44 Table 29: Estimated amount of metals in D ...... 44 Table 30: Estimated amount of metals in F ...... 44 Table 31: Estimated amount of metals in me‐OH cell...... 44 Table 32: Concentration of different metals in ores compared to those in ashes...... 48 Table 33: Concentrations of metals in ores compared to those in the landfill...... 48 Table 34: Estimated economic value of some metals in the landfill...... 50 Table 35: Deposited ashes in Sweden compared to those in Gärstad and the ratio between them. .. 50 Table 36: Total amount of metal in landfilled bottom ash in Sweden; then downscaled to Gärstad landfill and compared with results of this study. All units are in tonne...... 51 Table 37: Domestic material consumption of some metals in Sweden downscaled to Östergötland and compared with landfilled amount of metals in Gärstad landfill...... 51
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Terms Anthropogenic stocks: Refers to the material in the technosphere that already has been extracted, processed, used, or discarded.
Ash: Is the non‐combustible residues of an incineration process.
Bottom Ash: Is the ash which is taken out from the bottom of an incinerator after burning the fuel.
Flue gas: Is the gas emitted to the atmosphere from an incineration process; which usually goes through a smokestack.
Fly ash: Is the ash that follows the flue gas.
Metal‐Hydroxide: Is any metal element which has formed a compound with hydroxide anion (OH‐), and thus shown with Me‐OH.
Metal‐Oxide: Is any metal element which has formed a chemical compound with oxygen anion (0‐‐).
Mixed Waste: Mixed waste is a mixture of household, industrial, ash and all other waste which used to be landfilled.
Natural Stock: Refers to the material available in natural sources (e.g. ores), where the elements have been gathered through geological processes.
Sludge: Refers to the fluid residue from cleaning flue gas and bottom ash with water.
Wastes: “are substances or objects which are disposed of or are intended to be disposed of or are required to be disposed of by the provisions of national law” (EIONET, 2009).
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Abbreviation BA: Bottom Ash CHP: Combined Heat and Power CY: Cyclone Filter C&D: Construction and Demolition EL: Electrostatic Filter EPA: Environmental Protection Agency FA: Fly Ash FUDD: Funktionsanpassad Deponidesign [Landfill designed for specific function] KV: Kraftvärmeverket [CHP Plant] LFM: Landfill Mining Me‐OH: Metal Hydroxide MSW: Municipal Solid Waste MSWI: Municipal Solid Waste Incinerator WEEE: Waste from Electrical and Electronic Equipment
Number system Comma (,) is used as decimal separator and space ( ) is used as thousands separator. All the units are based on the International System of Units (SI).
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1 Introduction All processes in society produce waste. In nature, the waste is normally used as a resource for another process, but in human societies waste is often discarded. These discarded materials end up in places for depositing waste known as landfills. The increase in population, and humans’ tendency to improve their quality of life, has led to an increase in consumption of material. More material consumption means generating more waste, and more waste means bigger landfills.
This thesis focuses on the valuable materials that are deposited in landfills. Since landfills are the most common way for waste disposal and exist all over the world (UNSD, 2011) . The landfills are becoming bigger, and represent different threats to society and the environment; for example numerous hazardous substances reside inside them which can pollute the water and the land (Baas, et al., 2011).
In order to tackle the waste problem, The EU Commission on environment has defined a waste hierarchy which sets priority on how the waste should be treated. From the highest priority to the lowest they are: prevention, re‐use, recycling, recovery and disposal (EU, 2008). Based on this definition, landfilling falls under the disposal step. Disposal of waste has the lowest priority and thus needs to be avoided as much as possible. A solution to this problem could be the emerging LFM (Landfill Mining) concept, which makes it possible to shift landfill from a disposal stage to a recycling or recovery stage. LFM means recovering the landfilled waste, and use the buried material for other purposes. There are many barriers for doing so, including economical, technical, legal, and health and safety (Baas, et al., 2011).
Just like a normal mining project, before you can extract material from a landfill you need to know what resides inside it and what kind of waste has been deposited; thus it could be argued that the first barrier is prospecting. After searching for other studies about waste composition inside landfills, we found out that most of them focus on the environmental impact of heavy metals and leachate (Cossu, et al., 1995; Rettenberger, 1995). A few pilot studies (Hogland, 2002; Hogland, et al., 2004) which prospect landfills in Sweden classify metals as a single category without any more details. This can also be seen in the review made by Krook et al (2012) where no papers about prospecting metals in landfills were identified. Previous research (Cossu, et al., 1995; Hogland, 2002) shows that the waste composition of landfills has large variations in physical and chemical characteristics. This makes the estimation of the content and thus determination of valuable resources or hazardous substances difficult.
Hence prospecting is a key challenge. Earlier studies have used sampling method for prospecting (Hogland, et al., 2004) which is expensive, time consuming and reflects only a fraction of the landfill and thus leads to an isolated understanding. In this study we will use another method called MFA (Material Flow Analysis) which maps all the waste that has entered and left the landfilled through time. By this means, we will be able to give a better picture of landfill and its content. The main objective of this thesis is to prospect for metals, not because of its environmental impacts but for its economic value; so it is intended to serve as a base for future feasibility studies.
1.1 Aim The main goal of the project is to prospect Gärstad landfill. Thereby the occurrence of different metals will be estimated, their location and distribution will be shown and the accessibility of these
15 metal stocks will be assessed. The secondary goal is to develop a generic method for prospecting landfills. The research questions that we try to answer are as follows:
1. How much different metals have been landfilled in Gärstad landfill over time? 2. Where is the metal located? 3. In what forms are the metal found? 4. What are the advantages and disadvantages of MFA compared to direct measurements when applied to prospecting landfills?
1.2 Limitation In this study we included the metals that we could find data for. For this decade more data was available, and twenty different kinds of metals were included: (Iron (Fe), Aluminium (Al), Arsenic (As), Boron (B), Barium (Ba), Cadmium (Cd), Cobalt (Co), Chromium (Cr), Copper (Cu), Mercury (Hg), Manganese (Mn), Molybdenum (Mo), Nickel (Ni), Lead (Pb), Antimony (Sb), Selenium (Se), Tin (Sn), Titanium (Ti), Vanadium (V), and Zinc (Zn)). For previous decades, where data couldn’t be found, we limited the metal types to ferrous and non‐ferrous. Also the study only considers the metals within the underground and above ground waste in Gärstad landfill area. None of the structures such as office buildings, processing facilities and transportation equipment are included in the prospecting. Also temporary flammable waste deposits which are stored for a short time are not included in the calculations, since they will be eventually used as fuel for the incinerators, and thus converted into ash in the future. Temporary non‐flammable waste will be considered as landfill by law only if it is stored more than 3 years (Hammar, 2012), and the same concept was applied in the calculations.
1.3 Background Sweden’s waste management history starts in 1969 when the Environment Protection Act came in force and put new environmental obligations on waste treatment facilities. In the 1970s, the government emphasized that waste has to be seen as a resource. In the 1980s, the phase‐out or substitution of hazardous substances started. In 1992 the concept of “producer responsibility” was introduced which obliged certain producers to collect and dispose their products after being used. After Sweden joined EU in 1995, the waste management got greatly influenced by EU policies and regulatory frameworks like the Framework Directive on Waste, the Landfill Directive, and the Waste Incineration Directive. In 1997 the landfill bans were imposed which prohibited landfilling of flammable and organic waste; later in 2000, tax on landfilled waste started. These steps in waste management go on to this date (Swedish Environmental Protection Agency, 2005).
In 2008 about 98 million tonne of waste was generated in Sweden. Out of this, more than 70 million tonnes (72%) of waste was generated by the mining industry. Household waste was about 5 million tonnes (5%) and the rest belongs to other sectors. In table 1, the generated and treated waste in Sweden in years 2004, 2006, and 2008 can be seen. It is important to consider that the figures represent the dry weight (without water) of waste; thus the mining industry waste becomes 59 million tonnes instead of 70 million tonnes.
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Table 1: generated and treated waste in Sweden in years 2004, 2006 and 2008 (dry weight) (Naturvårdverket, 2012). The landfilled mining waste is the landfilled waste generated from the mining industry and should not be confused with LFM.
hazardous waste non‐hazardous waste kton 2004 2006 2008 2004 2006 2008 household waste 373 489 349 4 459 4 643 4 044 industrial waste 981 2 288 1 715 113 482 116 093 80 061 mining industry waste 58 400 61 800 58 699 recycled waste 292 339 108 17 544 26 059 2 853 incinerated waste 382 312 187 10 773 18 598 8 311 landfilled waste 494 378 384 3 937 3 765 3 837 landfilled mining waste 58 400 61 800 58 699
Currently the Swedish waste management system tries to achieve maximum environmental and social benefits from the waste. This has been possible through the cooperation of different actors, business, municipality and people. The producers are responsible for some products in their end of life stage, municipalities are responsible for household waste and people are responsible for separating their waste. Actually as of 2011, 99% of the household waste was recycled for energy or material (Avfall Sverige, 2011).
The most important methods for waste treatment in Sweden include material recycling for packaging, paper, scrap, and WEEE (Waste Electrical and Electronic Equipment), biological treatment through digestion or composting of green and food (organic) waste, waste‐to‐energy of combustible waste (household), and finally landfilling for waste that cannot be recycled (Avfall Sverige, 2011).
Since this study is about landfills, we chose Tekniska Verken i Linköping AB (publ), a company which itself belongs to Linköping Municipality. This company is involved in different areas like electricity production, district heating, water and sewage treatment, waste treatment and biogas. The company also owns the Gärstad Landfill where waste is deposited. The Gärstad landfill falls under the energy division in the company (Tekniska Verken i Linköping AB (publ), 2010).
Currently the Landfill receives all kinds of waste from more than 30 municipalities in Östergötland County. Household waste and other flammable waste are incinerated for energy recovery. Other waste like C&D is deposited and some other like WEEE is sent to other facilities for treatment.
Gärstad landfill is located about 3 Km northeast of Linköping, Sweden. The map of the facility can be seen in figure 1.
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Figure 1: Location of Gärstad landfill, 3 Km northeast of Linköping, Sweden.
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2 Theoretical Framework All products that we use are made out of different materials like metals, plastics and etc. These materials are extracted from different sources that lay in the rigid outer part of the earth known as lithosphere. After being processed into different products they enter the anthroposphere, which is the regions of the surface of earth affected by humans, like cities and villages. Then the products start to be used in everyday applications. Materials inside different products that are in this phase are known as “stock in use”. Then the product is thrown away after being used. The life cycle of a product can be seen in figure 2.
Material Manufacture Distribution Usage Disposal Extraction
Figure 2: The life cycle of a product; the disposal stage includes all the material inside a landfill.
2.1 Industrial Ecology With the raise in awareness of environmental and economic issues such as mineral depletion and scarcity of mineral resources, it has been proposed (Frosch & Gallopoulos, 1989) that the material life cycle should be a closed loop, meaning that all the material that goes to waste should be reused or recycled, and that material in stock which is no longer used but not thrown away should be recovered to replace natural sources. For this purposes all the waste that normally goes to disposal should be instead send to one of the previous phases. It is even suggested that all the material that has been deposited already in the landfill should be extracted and reinserted into the cycle as shown in figure 3 (Frosch & Gallopoulos, 1989).
Material Extraction/ Recovery
Disposal / Manufacture Recolection
Usage Distribution
Figure 3: Closing the loop; instead of disposing of material, they are reinserted into the life cycle. Own illustration based on Frosch & Gallopoulos (1989)
The concept of closing the cycle is, however, much more complex to achieve in practice; because the different phases of one product are not independent from other products or materials, meaning each life cycle stage of a product may interact with a life cycle stage of another product or material
19 and the efficiency of these interactions will determine the amount of waste of the whole system. To optimize these interactions it is necessary to have a system approach in which the industry emulates the natural processes to maximize the efficiency of energy and resources use and to minimize waste. This concept was first introduced by Frosch and Gallopoulos (1989) and is known as Industrial Ecology.
To minimize the waste it is necessary that different industries interact with each other in the way that the waste of one process can be used as raw materials for another. The practice of this industrial symbiosis leads to reduced needs for extraction of virgin materials, reduced costs for companies, and less discarded waste. The success of this approach depends on the correlation between government, manufacturers and consumers; normally the interactions between industries appear naturally, but then the challenge appears when the materials leave the industrial level and are scattered in the rest of the society, and the recollection and recovery processes become much harder. Here the role of governments and consumers gains importance as it is their duty to facilitate the ways in which waste is treated and where the materials will reach their end of life (Frosch & Gallopoulos, 1989).
When materials reach their end of life stage, two things can happen: either they persist without being used or they are discarded in the form of waste. The first case is called material hibernation, where a material stays in the anthroposphere for years without being collected by any waste management process (UNEP, 2010). In the latter case, where materials are thrown away, they can be managed in several ways in order to return to the material cycle, but when it is not possible, they are discarded and generally end up in landfills.
2.2 Landfill Mining One of the biggest challenges for industrial ecology is how to deal with these growing hibernating stocks in the anthroposphere, and is has been suggested (UNEP, 2010) that mining them can be a solution to reintroduce material into the cycle and as a replacement for natural resource extraction. The process of extracting these materials and bring them back in the material cycle is called urban mining (UNEP, 2011). And more specifically if the extraction comes from a landfill the associated term is landfill mining. Landfill mining is defined by Krook et al (2011) as “a process for extracting minerals or other solid natural resources from waste materials that previously have been disposed of by burying them in the ground”.
According to previous studies (Hogland, 2002; Krook, et al., 2011), there are many additional benefits from landfill mining, which includes: conservation of landfill space, reduction of landfill area, expanding landfill lifetime, prevention and remediation of pollution and other sources of contamination like leachate1, material and energy recovery, reduction in management system costs, site redevelopment, and reclamation of land.
Landfill mining was first carried out in 1953 in order to obtain fertilizer for orchards (Krook, et al., 2011). Historically the attempts on landfill mining have been done for land reclamation and recovery of the soil, but not for material recovery.
1 A liquid material that drains from stockpiled material and contains environmentally harmful substances (wiki).
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2.3 MFA (Material Flow Analysis) One of the tools used in industrial ecology is MFA. It allows the user to quantify the flows or stocks of certain material that goes into, through and, out of a system of interest. To make a MFA it is necessary to define a system boundary and a time scale. The system boundary is spatial boundary that confines a specific area (i.e. a factory, city or county). Defining a system boundary facilitates the data collection phase in a study. The time scale chosen is normally one year, because most of the data from governments, organizations and agencies are reported annually.
After defining the system boundary and time scale, the estimating method is defined. The standard methods for estimating a material stock are the bottom‐up, and top‐down (UNEP, 2010).
Bottom‐up: in this method the data about the level of stock is collected and used for estimating the amount of material stock. This can be shown with the below formula: