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Comitato Nazionale Energia Nucleare

HEAVY PRODUCTION. INDUSTRIAL PROCESS AND PLANTS

(A Bibliography - 2nd Rev, Edition)

D. LAVRENCIC Comitato Nazionale Energia Nucleare

H~AVY WATER PRODUCTION. INDUSTRIAL PROCESS AND PLANTS

(A Bibliography - "nel Rei'. Edition)

D. LAVRENCIC Testo pervenuto nel febbraio 1974

Edito dai Comitato Nazionale Energia Nucieare, Divisione Affari Internazionali e Studi Economici, Ufficio Edizioni Scientifiche - Viale Regina Margherita, 125 Roma. Stampato in formato UNI presso la Tipolitografia RANCOS - Roma INDEX

I. General pag. 1 II. Bibliographies II 31 III. Determination and Analyses of It 41 IV. Heavy Water Production II 73 A - Reviews of Production Processes II 75 B - Patents Review (Brévatome, Paris) II 97 C - Actual II 137 D - Production Plants and Equipment II 195 E - Technical and Economic Aspects II 227 F - Potential Production Processes II 237 V. Heavy Water Reactors " 279 VI. Main Conferences Held on Heavy Water

and HWRs • "299

Subject Index " 307

Authors Index "311

Societies Index " 377 Annex Introduction

This work aims at outlining a status of the heavy water production processes and fabrica'!^-1 plants.

The bibliography contains references from the scientific and technical literature on analysis and production of heavy water and on the role of irWIl in programs. It does not include refe rene us to survey biological effects oi' and heavy water.

The material is arranged under the following main items:

I. General: general information on the principal subject of the bibliography and on related ones.

II. Bibliographies: bibliographies on deuterium and heavy water and on related arguments. ill. Determination and analyses of deuterium and heavy water: various methods for the following analysis of and for water production are reported.

IV. Heavy Water Production

A: Reviews of various production processes ; B: Review of patents on heavy water production (Patents selected by Brévatome, Paris); Addendum with patents reported on Nuclear Science Abstracts (1972 - 1973, Oct. 15th); C: Actual industrial processes: chemical exchange (bithermal exchange between hydrogen sulphide and water; single temperature -hydrogen exchange; hydrogen-water exchange); ID: Production plants and equipment: conceptual studies on designs; description, operation and equipment of fabrication plants and projects. A sheet of plants and projects ordered by country is also included; E: Reviews on technical and economic aspects of industrial heavy water production; consumption and demand of D20; IT

F. : Potential production processo«: chemical exchange processes between other substances than those mentioned above; physical separation processes (, absortive fractionation, absorbtion, diffusion etc. ) and others.

V. Heavy water reactors A. : A table of research, test and power heavy-water-moderated reactors is included. For the bibliography on this reading, reference is made to heavy water x-eactors bibliography, .edited by IAEA, Vienna, in January, 1970. (ST1/PUB/21/37) 13.: HWlts in Nuclear Power Programmes: nuclear strategy studies with HW/ls performed in different countries; heavy water and fuel requirements for HWlt.

VI. Main Conferences on Heavy Water and Heavy Water Reactors are also listed. Under each subject, references are listed from the first to the most recent one. The magazines where the year, only'is "indicateti are listed in alphabetical order. In cases where the exact title is not known, a title containing the subject of reference is given in brack test. Works are given in English language, unless otherwise marked. Author index is included. Authors of the patents listed in the Addendum are not included in this index. The main sources of information are the Nuclear Science Abstracts from 1946 to 1973; the Chemical Abstracts, as well as the available bibliographies and status report from USA, USSR, France, Canada, India, , Italy and Romania are also been examined. Ill

Refere 11cos

Nuclear Science Abstracts 194G-19r/:>. (Oct. 15, 197:-!)

Bibliography of Research on Heavy Water Compounds. A. II. Kimball Comp, H. C. Urey, 1. Kirshenbaum eds, 1st ed. McGraw-Hill Book Co. , lnc 1949, ( N"NES-ri[~4C).

Isotope Separation and Exchange. G. M. Begun, R.E. Allen Comps. TID-3 036 (Revised). June 1954.

Production of Heavy Water. G. M. Murphy, II, C. Urey, 1. Kirshenbaum eds. 1st ed. McGraw-Hill Book Co. , Inc. New York - Toronto - London. 1955. (NNES-4F)

Heavy Water Production. J, J, Jacobs comp. TID-3091 (Suppl. .1) June 1964.

Deuterium and Heavy Water. A Selected Bibliography. G. I-I. Vasaru, A. Mihaila, P. Szentgyorgyi. May 1970. I- GENERAL 3

I - G E N l'I II A T,

1. THE HYDROGEN ISOTOPE OF 2. Kallmann H. , Easarcfi' W. Naturwisscnseh. 20, 472, 1932.

2. A HYDROGEN ISOTOPE OF MASS 2. Urey U.C., Bviekwoi.Ule F. G. , Murphy G. M. I'Jiya.' Jiev. 39, 164-5, 1032.

3. ISOTOPE OF HYDROGEN OF MASS 2. A Review. Landsberg G. S. Uspekhi Fiz. Nauk 12, 343-50, 1932. (In Russian)

4. HEAVY WATER. Boahouffer K. F. Angew. Chcm. 46, 776-9, 1933.

5. ISOTOPE OF HYDROGEN AM) ITS 1 'JlOPURTiES. Mikolic S.S. Bull. Soc. Chini. Roy. Yougoslave 4, 227-35, 1933.

6. . A Review. Kaptein A.J. G. Gliom, vveekblad 30, 695-701.. 1933. 7. ISO'J.'OPLOS OF HYDROGEN. Lewis G.N. ,J. Amur. Chem.Süe. 55, 1207-8,1933.

8. THEORETICAL CONSIDERATIONS CONCERNING THE SEPARA­ TION OF ISOTOPES. Eyving II., Sherman A. J. Clicm. Phys. 1, 345-0, 1933.

9. HEAVY HYDROGEN AND HEAVY WATER.. A Review. Naturo 132, 5:3GJO:}:j.

10. SEPARATION OF Til LO . Collie C.ll. Nature 132, 5G8-9,1033.

11. EXPERIMENTS ON HEAVY HYDROGEN. Parkas A. , Farkas L. Nature 132, 894,1033.

12. HEAVY HYDROGEN. Rutherford E. Nature 132, 955-G, 1933.

13. THE RELATIVE ABUNDANCE OF HYDROGEN ISOTOPES. Bleakney W., Gould A.J. Phys. Rev. 44, 2G5-8, 1933.

14. THEORETICAL AND PRATICAL STUDIES OF ATOMIC AND MOLECULAR FORMS OF THE HYDROGEN ISOTOPES. Taylor H.S.,Eyring II. Proc. Am .Phil. Soc. 72, 255-64, 1933. 5

15. CHEMICAL PROPERTIES OF THE HYDROGEN ISOTOPES. Urey U.C. Rev. Sci. Instr. 4, 423-5, 1933.

16. SEPARATION AND PROPERTIES OF THE ISOTOPES OF HYDRO­ GEN. Urey U.C. Science 78,506-71, 1933.

17. RECENT ADVANCES IN SCIENCE;PHYSICAL . A Re­ view. Wanribrough-Jones O.II. Science Progress 28,107-15,1933.

18. HEAVY WATER. A Review. Domange L. Ann. pharm, franc. 41, 144-8,1934.

19, HEAVY HYDROGEN AND THE WORK OF HAROLD C. UREY. A Review. Harkins W.D. Chem.'Bull.'(Chicago) 21, 83-7, 1934.

20. HEAVY HYDROGEN OR DEUTERIUM, AND HEAVY WATER. A Review. Boutàric A. Genie civil. 104,444-6, 1934.

21. HEAVY WATER. A Review. Lindner J. Scientia Farm. 5, 24-9, 1934.

22. HEAVY HYDROGEN AND HEAVY WATER. A Review. Ouellet C. Naturaliste canadj.en 61, 205-11, 1934.

23. HEAVY HYDROGEN AND HEAVY WATER. A Review. Nature 133, 197,1934.

24. PHYSICAL AND CHEMICAL PROPERTIES OF HEAVY WATER. A Review. Ilideal E.K. Nature 134,504, 1934. ft

THE HYDROGEN ISOTOPE AND HEAVY WATER. A Review. Frerichs R. Naturwissenschalten 22, 113-8, 1934.

THE HEAVY HYDROGEN ISOTOPE. Farkas L. Naturwissenschaften 22, G14-23;640-G;G58-G2, 1934.

THE HYDROGEN ISOTOPE OF MASS 2. A Review. Haantjes J. Nede.rl. Tijdschr. Natuurk. 1, 33-4 0,1934.

HEAVY WATER. Dominik W. Polish Ayr. Forest. Ann. 33, 359-70, 1934.

METHODS AND RESULTS OF RESEARCH ON ISOTOPES. Mattauch J. Physik. Z.35,507-021, 1934.

EXPERIMENTS ON HEAVY HYDROGEN. Farkas A,, Farkas L. Proc. Roy. Soc. (London) A144, 467-80, 1934.

ISOTOPES OF HYDROGEN AND THEIR SEPARATION. A Review. VeilS. Rev. Sci. 72, 174-7, 1934.

THE NEW HYDROGEN. Science 80,21-5, 1934.

THE NEW HYDROGEN. An Adrcss. Rutherford E. Scientia Milan 55,341-9,1934.

HEAVY HYDROGEN. Chittock C. School Sci. Rev. 16, 132, 1934. 7

35. HEAVY WATER. A Review. Cignoli F. Semana méd. (Buenos Aires) 1,2008-71, 1934.

3ß. ISOTOl'Y OF HYDROGEN. HliJAVY WATER. A Review. Hamann E. Süddeutsche Apotli. Ztg. 74, 1,15-G, 1934.

37. HYDROGEN ISOTOPE AND HEAVY WATER. Vasil'ov A. M. Trans. Kirov Inst. Chcm. Tcchnol. (Kazan) No. 2, 129-49, 1934. (In Russian)

38. ISOTOPE OF HYDROGEN AND HEAVY WATER. Tcmkin M. Uspekhi Khini. 3, 217-35, 1934. (In Russian)

3 9. 1SOTOPY OF HYDROGEN, HEAVY WATER. A Review. Bochme J. Z. physik. c hem. Unterricht 47, 216-23, 1934. (In German)

40. STUDY ON PROBLEMS: HEAVY WATER, HEAVY HYDROGEN AND GRAVITATION. Hartmann J. U. 1934. (In German)

41. HEAVY WATER. Mark H. Ed. F. Dcuticke, Leipzig.

42. SOME THERMODYNAMIC PROPERTIES OF HYDROGEN AMD DEUTERIUM. Nobel Lecture. Urey II. C. Angew. Chem. 48, 315-20, 1935.

43. DEUTERIUM AND ITS COMPOUNDS. A Review. Darmois F. Bull. Soc. Chini. (France) (5) 2, 1513-44, 1935.

44. HEAVY HYDROGEN AND HEAVY WATER. A Review. Malan-Nelson A. M.Giorn. farm. chim. 84, 108-17, 1935. 3

il RA VT HYDROGEN Alvi.) HEAVY WATER. A liuviow. Ciay ,]. Ingenieur (Utrecht) 50A,220-3, J935.

ISOTOiTC EXCHANGE EQUILIBRIA. Urey li. C. , Croi IT L, Y. ,J. Aia.. CliOJn.Soc. 57, 321-7, HJo'5.

HYDROGEN ISOTOPES AND DEUTERIUM OXIDE OH HEAVY WATER, Prosovits P. Keemiu Touted 2, 50-liO, 1Ü35.

HEAVY WATER IN CHEMISTRY, Pulanyi M, Naturo 135, 19-26, 1JJ35.

ISOTOPES. A Review. Aston E. W. Nature 135,080-7,11)35.

DEUTERIUM, A NEW TOOL POR. CHEMISTS. A Review. Greene CIL NUCIOUK 12, J7Ü-2, 1.935.

HEAVY HYDROGEN AND 20th CENTURY CHEMISTRY. A Lecture. Pharm. J .1:54,88, 1935.

OUR PRESENT KiX'OWLEDCE OP HEAVY HYDROGEN AND HEAVY WATER. Mark II., Wuld IVI. Pi-utuplasinu 20, 109-27, 1935.

HYDROGEN AND ISOTOPES AND HEAVY WATER. A Review. I.unelund H. Tek. Poei-en.i Pinkuid Pocrh. 55, 35-ÌÌ, 11)35. 9

54., ISOTOPY OF THE ELEMENTS. A Review. Mattauch J. Z.VDI 79, 1140-4,1935. -

&5. DATA ON HEAVY WATER. Reitz O.Junk. , The Hague 1935. (In German)

56. ORTOHYDROGEN, PARX AHYDROGEN, AND HEAVY HYDROGEN. Farkas A. Cambridge University Press, London 1935. (The McMillan Co. New York 1935)

57. THE SEPARATION OF ISOTOPES. Champetier G. Bull. soc. c him. (France) 3 (5) 1701-27,1936.

58. HEAVY HYDROGEN, THE ISOTOPE OF HYDROGEN'AND HEAVY WATER. Champetier G. Bull, soc, encour. ind. nati. 135, 237-49, 1936.

59. HEAVY HYDROGEN - HEAVY WATER. A Review. Stoeckl K. 'Med. Klim.32, 1105-9, 1936.

60. HEAVY WATER. A Review. Bueno O. G. Politecnica, (Quito, Ecua­ dor) 1,306-12,1936.

61. RECENT ADVANCES IN SCIENCE:GENERAL AND ORGANIC CHEMISTRY. ISOTOPES. Brady O. L. Science Progress 31, 100-3,1936.

62. THE HEAVY HYDROGEN ISOTOPE. A Review:Wirtz K. Z.physik. ehem. Unterricht 49, 14-28, 1936.

63. PRESSURE AND HEAT OF VAPORIZATION OF HEAVY WATER. Riesenfeld E. H., Chang T. L. Z. physik. Chem. B 33, 120-6,1936. to

THE PHYSICAL CHEMICAL AND BIOLOGICAL QUALITIES OF HEAVY WATER. A Review. Indovina R.,Citarda A. Bipchim. e Terap.sper.24,236-47,1937.

RECENT RESEARCH ON HEAVY WATER AND ITS OCCURRENCE IN NATURE. Riesenfeld E. II. Sveiisfckem. TM. 49, 113-23, 1937.

HEAVY WATER. Seijo E. Rev. centro estud. farm, y biochim. 27, 92-107,1937.

DEUTERIUM AND HEAVY WATER. A Review. Borocco A. L. Rev. chim. ind. (Paris) 46, 322-9, 1937.

REACTIONS IN HEAVY WATER. A Review. Suess H. Österr. Chem. Ztg.(Wien) 40,239-43,1937.

GENERAL AND INORGANIC CHEMISTRY OF DEUTERIUM. A Review.Einecke.E. Chem. Ztg. (Wien) 41, 331-40;355-9;371-6; 395-400,1938.

CONCENTRATION OF THE HEAVY ISOTOPES OF OXYGEN AND THE ISOTOPIC ANALYSIS OF WATER.Skarre O.K., Brodskii AjI.Dokl. AkacT. Nauk. SSR 20, 565-8, 1938. (Rept. L. V.' Pisarzhevskii Inst.' Phys. Chem. Sci. Acad. Sci. Ukr. SSR 11, 75-98,1938)

ISOTOPES. A Review. Souza-Reis F. de, Moggi S. Rev.quim. e farm. Rio de Janeiro 3, 34-40, 1938..

NEWS ABOUT HEAVY HYDROGEN. A Review. Royen P. Umschau 42,207-9, 1938.

DEUTERIUM AND ITS COMPOUNDS. (Deuterium and composes de deuterium. Tables annuelles de constantes. No. 1) Hermann Cie, Paris 1938. (In French) 11

74, HEAVY WATER, A Review. Kilde G. Dansk. Tids. Farm. 13, 69-92, 1939.

75. SEPARATION OF ISOTOPES. Walcher W. Ergeb. exakt. Naturwiss. IB', 155-228, 1939.

76. HEAVY WATER. A Review, Steinert B. Wallerstein Labs. Com.- muns. 2,21-4, 1939.

77. THE SEPARATION OF ISOTOPES. Urey II. C. Pub. Am. Assoc. Advance. Sci. No. 7, Recent Advances in Surface Chemistry and Chem. Phys. 73-87, 1939. (Reports on Progress in Physics VI, 48-87,1939)

78. SEPARATION OF ISOTOPES .Urey H.C. Phys. Soc. Reports on Progress in Physics 6,48-77, 1940.

79. SEPARATION AND USE OF STABLE ISOTOPES. Uréy H.C. J. Appi. Phys. 12, 270-7, 1941.

80. 'IEAVY WATER. A Review. Selwood P. W. J. Chem. Education 18, 515-20, 1941.

81. ISOTOPE REVIEW FOR 1940. Flu egge S. , Mattauch J. Physik. Z. 42,1-5, 1941.

82." PROPtBAlS FOR CONCENTRATION OF DEUTERIUM. Cohen K. Columbia Serial No. 4R-133, Aug. 194.1.

83.' PROPOSALS FOR CONCENTRATION OF DEUTERIUM. Cohen K. SAM Rep. A-118, June 1941.' 84. THE THEORY OF RATE PROCESS. Glasstonc S. , Laidlor K. J. , Eyring J-I. McGraw-Hill, Now York, 1941,

85; CHEMICAL ENGINEERS' HANDBOOK, J, II, Perry Ed. McGraw Hill Book Co. Inc. New York 1941. (pp.'2542, 2550-G2)

8G. REPORT ON ISOTOPES, 1941. Flügge S,, Mattauch J, Physik. Z. 43, 1-5, 1942.

87. SEPARATION FACTOR. Cohen K., Mayer H. L, SAM Rep, 4M-11, ' Jan, 13, 1942,

88. THE HYDROGEN ISOTOPES;THERMODYNAMIC PROPERTIES OF THEIR COMPOUNDS. MDDC-149(>. Sept. 1942. Deci. Nov. 25, 1947.

89. MATERIALS OF CONSTRUCTION. Hiskey C. F. SAM Rop, 100XR-lC52.Nov.-10, 1942.

90. THE THEORY OF BY EXCHANGE REACTIONS. Waldmann L. Naturwiss. 31, 205-6, 1943.(In German) (AEC-tr-1911)

91. THE PHENOMENA OF SEPARATION PROCESSES. Klemm A. Z. Physik 123, Nos. 1-2,10-27,1944.

92. METALLURGICAL PROJECT REPORT. Fermi E., Zinn W. H. , Wattenberg A. CP-1827. June 1944.

93. HEAVY WATER. Kirshenbaum I., Graff J., Forstat H. SAM Rep. A-2193.Aug.T7, 1945. 13

94. APPLICATIONS OF ISOTOPES IN CATALYTIC REACTIONS AT SURFACES. Taylor PI. S. Frontiers in Chemistry 3, 19-42,1945.

95. SYMPOSIUM ON ATOMIC ENERGY AND ITS IMPLICATIONS. 50 YEARS OF ATOMIC PHYSICS. METHODS AND OBJECTIVES IN THE SEPARATION OF ISOTOPES. Urey II. C. Proc. Am. Phil. Soc.90, No. 1, 30-5, 1946.

96. THE THERMODYNAMIC PROPERTIES OF ISOTOPIC SUBSTAN­ CES. A Review. Urcy U.C. J. Chora. Soc. 502-31,.1947.

97. ISOTOPE SEPARATION FOR THE PURPOSE OF PRODUCTION OF NUCLEAR ENERGY. Groot S.'lt. de.Nedcrland Tijdsch. Naturk. 13,113-20, 1947.

98. SEPARATION OF STABLE ISOTOPES. Steward D..W. Nucleonics 1, 18-26, 1947.

99. ; SEPARATION AND PHYSICS OF ISOTOPES. A Review. Paemel O. van. Tech. Wetenschap. Tijdsch. 10, 56-9, 1947.

100. THE SCIENCE AND ENGINEERING OF INfUCLEAR POWER. Goodman C. Ed Addison Wesley, Cambridge Mass. 1947-4 8.

101. THE SEPARATION OF STABLE ISOTOPES. Parravano G. Chi­ mica e Industria 30,296-301,1948.

102. SEPARATION OF ISOTOPES. Dunlap G. W., Lichtenstein R. M. Elee. Eng. N. Y. 65, 469-74, 1948. 14

FIAT Rev. German Science 1939-46: \ 103. SEPARATION OF UNWEIGHTABLE AMOUNTS OF SUBSTANCES (ISOTOPES) AND USE OF THE PRODUCT OBTAINED. Inorg. Chem.Pt. 1.113-20, 1948;

104. SEPARATION OF ISOTOPES. Dickel G. Inorg. Chem. Pt.I. 121-3,1948;

105. SEPARATION OF ISOTOPES IN SMALL QUANTITIES. Walcher W. Nuclear Physics and Cosmic Rays. Pt.II, 94-107, 1948;

106. INACTIVE ISOTOPES, THEIR SEPARATION AND APPLICATIONS. Dickel G. Phys. Chem. 7-17, 1948;

107. ISOTOPE EXCHANGE EQUILIBRIA; Suess H. Phys. Chem. 19-24, 1948.

108. ISOTOPE SEPARATION BY UREY'S METHOD. Muylle R. L'indu­ strie Chemique Beige 13,17-23, 1948.

109. SOME RECENT WORK ON THE SEPARATION AND USE OF STA­ BLE ISOTOPES. Lauder I. J. Proc. Roy. Soc. N. S. Wales 82, 183-95, 1948.

110. COMPILATION OF THERMAL PROPERTIES OF HYDROGEN IN ITS VARIOUS ISOTOPE AND ORTO-PARA MODIFICATIONS. Wooley H. W. , Scott R. B., Brickwedde F. G. J. Res. Natl. Bur. Stds. 41, 379-475, 1948. 15

111. FUNDAMENTALS OF ISOTOPE SEPARATION. A Review. Cohen K. Nucleonics 6,2,3-9,1948.

112. ATOMIC ENERGY FOR MILITARY PURPOSES. Smythe H.D. Princeton University Press, Princeton N, J. 1948.

113. ON THE SEPARABILITY OF ISOTOPES IN . Martin H. Proc. of the German Buns en Soc. for Applied Phys. Chemistry Meeting, Stuttgart. Oct. 7-10, 1948. Angew.'Chem. 61, 297-305, 1949. (In German)

114. HEAVY WATER. Barr F. T. AECD-2871, Nov. 23,1949. Deci. Jan. 20, 1950.

115. THERMODYNAMICS. Guggenheim E. A. North-Holland Publishing Co. Amsterdam. 1949.

116. ISOTOPE ENRICHMENT THROUGH EXCHANGE REACTIONS. Clusius K. Chimia . () 4,275-84, 1950.

117. ISOTOPE EXCHANGES. RECENT PROGRESS. Haissinsky M. J. chim. phys. 47, 957-82,1950.

118. ISOTOPES IN THE STUDY OF CHEMICAL REACTIONS. Arnstein H. R. V., Bently R. Nucleonics 6, No. 6, 11-27, 1950.

119. THE SEPARATION OF ISOTOPES. A Review. Hoang T. F. Rev. questions sci. 1.1/378-88, 1950. 16

120. SEPARATION OF ISOTOPES. Groth W. Umschau 50, 402-4, 1950. (In German)

121. SEPARATION OF ISOTOPES AND THEIR USE IN EXPERIMEN­ TATION. Clusius K. Verhandl. Schweiz. Naturforsch. Ges. 33-52, 1950.

122. SEPARATION TUBE METHOD AND CHEMICAL EXCHANGE PROCESS FOR THE SEPARATION OF ISOTOPES. Becker E. W, Angew. Chem. 62,121-5, 1950. (In German)

123. CHEMICAL EXCHANGE AS A VERSATILE ISOTOPE SEPARA TION PROCESS. Clcwctt G. H. Y-683, Nov. 7, 1950.

124. SEPARATION OF ISOTOPES. Langer A., Stephens W. E. Official Gazette 64, 305, 1951.

125. UTILIZATION OF HEAVY WATER. Kirshenbaum I., Murphy G. M., Urcy II. C. (Columbia Univ. New York. Substitute Alloy Materials Labs. USA). TID-5226. 1951. Deci. Feb. 27, 1957. (NNES-III-4B).

12G. THE THEORY OF ISOTOPE SEPARATION. Cohen K. National Nuclear Energy Serics-III, McGraw-Hill Book Co. Inc. New York 1951.

127. PHYSICAL PROPERTIES AND ANALYSIS OF HEAVY WATER. Kirshenbaum I. ed. G. M. Murphy, H. C. Urey. McGraw-Hill Book Co., Inc., New York 1.951. National Nuclear Energy Series III, Vol. 4A. (NNES-III-4A) falso Ch. HI) 17

128. ISOTOPES. Bigeleisen J. Ann. Rev, Phys. Chem. 3, 39-5G, 1952.

129. MEASUREMENT OF THE DEUTERIUM CONCENTRATION IN CONDENSED OF BORACIFERUS SOFFIONE AT LARDERELLO. Cerrai E., Marchetti C., Silvestri M. Nuovo Cimento(.9), 9, 511-6, June 1952. (In Italian) (also Ch III)

130. THE CONTINUOUS ISOTOPIC ENRICHMENT BY CASCADES. Walen R. Ree, trav. inst. recherches structure matiére (Belgrade) 1-, 35-67,1952.

131. ISOTOPES. Bigeleiscri J. Ann. Rev. of Nuclear Science Vol.2, Annual Rev. Inc. Stanford, Calif. (USA). 1953. (p. 221-39)

132.. CHEMICAL SEPARATION OF STABLE ISOTOPES. Clèwett G. H. Ann.. Rev. of Nuclear Science Vol. 1. Annual Rev.Intì. Stanford Calif. (USA) 1953. (p. 293-300) iSS.. CHEMICAL ENGINEERING ASPECTS OF NUCLEAR POWER. Benedict M. Industr. and Engng. Chem. 45, No. 11, 2372, 1953.

134. THERMAL CONDUCTIVITY OF HEAVY WATER. Meyer F., Eigen M. Z. Naturforsch. 8a, 500-1, 1953. (In German)

135. A COMPILATION OF DATA OF DEUTERIUM COMPOUNDS. Armstrong G. T. NBS-2306. Feb. 24,1953.

136, HEAVY WATER. Augood D. R. Industrial Chemist 30, No. 359, 585,1954. 18

137. REPORT FROM GENEVA. REACTOR MATERIALS. Nucleonics 13, No. 9, G4-7.1, Sept. 1955.

138. LAWS ül<* EQUILIBRIUM DEUTERIUM DISTRIBUTION IN HYDRO­ GEN-ISOTOPE EXCHANGE REACTIONS. Varshavskii Ya. M.,

Vaisberg S. E. Dokl. AN SSSR 100, 97-100, 1955 . ([n Russian)

139. • ALTERATIONS OF HEAVY WATER IN . Germagnoli E., Mongini L. Energia Nucleare (Milan) 2, No. 15, 323-31, 1954-1955.(In Italian)

140. CHEMICAL ENGINEERING COST ESTIMATION. Aries and . McGraw-Hill Book Co. New York. 1955.

"ATOMRUNDSCHAU". A Review. IGLefoth W. Atomkernenergie 1, No. 9, 328, 1956.'(In German)

142. THE ANALYSIS AND PRODUCTION OF STABLE ISOTOPES. Roth E. CEA Rep. No. 536. 1956. (Chimic Analytiquc No. 1, 3-14, 1956)

143. PROGRESS IN NUCLEAR ENERGY. SERIES IV. TECHNOLOGY AND ENGINEERING. R. Hurst, S. McLain Eds. McGraw-Hill Book Co. Inc. , New York, 1956.

144. THEORY OF SEPARATION OF STABLE ISOTOPES. Türkin V. K. Trudy Moskov. Khim. Technol. Inst. im.D.I. Mendeleeva No. 22 247-51,1956. 19

145, HEAVY WATER (Schweres Wasser). Kruse E. Orion-ßUcher, Murnau 105G. (In German)

14G. CHEMISTRY AND SEPARATION OF ISOTOPES. Panchenkov G. M., Semiokhin I.A., Akishin P.A. Vestnik Moskov. Univ.Ser. Mat. Mec. Astron. Fiz.Khim. 12, 190-214, 1957.

147. TABLES OF PROPERTIES OF HEAVY WATER AT SATURATION TEMPERATURES. Howieson J. Nei-77, 1957. (AECL-1055)

148. ISOTOPIC ANALYSIS OF WATER. Shatenstein A. I., Yakovleva E. A. , Zvyagintseva E. N. , Varshavskii Ya. M., Izrailevich E. A. , Dykhno N...M. lad. AN SSSR. 1957. (German Transl. VEB Deutsch.Verlag Wiss. Berlin 1960;AEC-tr-4136,1957) (In Russian)

149. INDUSTRY TOWARDS NUCLEAR ENERGY (L'industrie devant l'energie nucléaire). Baumgartner R., Bishop A.S. et al. Paris 1957. (p. 237-47) (In French) OECE Paris. Vol. I 1957;Vol. II 1958.

150. NUCLEAR CHEMICAL ENGINEERING. Benedict M., Pigford R. McGraw-Hill Co., Inc., New York, 1957.

151« SEPARATION OF ISOTOPES.Klemm A. Atomwirtschaft 12, No.8/9, 341-2, 1958. (In German)

152. NEW HORIZONTS FOR STABLE ISOTOPES. Ruder man I. W. 20, P/801(USA) 2nd Geneva Conf. 1958.

153. CONCEPTIONS OF THE MODERN PHYSICS:ISOTOPES, HEAVY WATER. Purcaru C.I. Bucharest 1958.

154. SOME PROBLEMS OF ISOTOPE SEPARATION THEORY. Rozen A. M. Trv.dy Vses.Konf. Prim. Izotopov. Moscow 1958. (In Ruffian/ 20

155, PROCEEDINGS OF THE INTERNATIONAL SYMPOSIUM ON ISOTOPE SEPARATION, Amsterdam, Apr. 1957. J. Kistemaker J. Bigeloisen, A. 0. C. Nier Eds,-North-Holland Pubi. Co. Amsterdam 1058.

156. HEAVY WATER. Suslov B.' N. Gosud. Izd. Teklmiko-Tcoret. Lit. Moscov 1958. (In Russian)

157. NUCLEAR FUSION. Kurchatov I.V. Atomizdat, Moscow 1958. (In Russian)

158. CHEMICAL ENGINEERING AROUND THE WORLD. E. L. Piret ed. New York, 1958.

159. ISOTOPIC SEPARATION FACTOR OF SLOW DISCHARGE MECHANISM OF HYDROGEN ELECTRODE REACTION. II. Kodera T. (Hokkaido Univ. Sapporo, JAPAN) J. Research Inst. , Hokkaido Univ. 7, 75-6, Sept. 1959.

160. CISE - Centro Informazioni Studi Esperienze. Isotope Separation- Heavy Water. Milano, Jan 1959. (p. 87-90) (In Italian)

161, HEAVY WATER, lladulcscu C. Ed. Technica, Bucharest, 1959.

A RESEARCH ON ISOTOPIC COMPOSITION OF EVOLVED HYDROGEN WITH SPECIAL REFERENCE TO THE MECHANISM OF NICKEL CATHODE, llirota K., I-Iisano T. (Osaka Univ. JAPAN) Bull. Chcm. Soe. Japan 33, 1019-20, July 1960. 21

1.G3, HEAVY WATER. Sekowski S. Chemik (Gliwice) 13,306-8,1960.

164. KINETICS OF ELECTROLYTIC KYDROGEN AND DEUTERIUM EVOLUTION. Conway B. E. (Univ. of Ottawa, CANADA) Proc. Roy. Soc. (London) A256, 128-44, May 31,1960.

1G5. REACTOR HANDBOOK. EDITION REVISED AND EN­ LARGED. VOLUME I. MATERIALS. Tipton C. R. Jr. New York, Interscience Publishers, Inc. 1960.

16G. DESIGN AND CALCULATION IN THE . (Projektirung und Vorkalkulation in der chemischen Industrie) Springer Verlag, Heidelberg 19G0. (In German)

167.. THE THEORY OF ISOTOPE ENRICHMENT BY HOT-COLD METHODS. Priebsch J. Acta Phys. Austriaca 14,347-57,1961.

168. OVERVOLTAGE DEPENDENCE OF DEUTERIUM SEPARATION FACTOR ON PLATINUM. Horiuti J., Fukuda M. (Hokkaido Univ. Sapporo, JAPAN) Shokubay (Tokyo) 3, No. 2, 115-7,1961,

169. ISOTOPE PRODUCTION AND DEVELOPMENT. Peisach M., Walter A. Israel AEC, 685, G3-G, 1961. 22

170. HEAVY WATER. Pratt H. R. C. AERE, CE/R 735, 1961.

171. NUCLEAR FUELS AND MATERLALS DEVELOPMENT. (Division of Reactor'Development, USAEC). TID-11295. Feb. 1961.

172. THERMAL FEEDBACK IN COUNTER-CURRENT PROCESSES. Pohl H. A. (Du Pont'do Nemours E. I. & Co. At. En. Div. Wilmington, Del. and Princeton Univ. N. J, Plastics Lab. ) Part. I. Technical Rep. 61 A. TID-12452. Apr. 1, 1961. Part. II. Technical Rep. 61 B. TID-12453. Apr. 1, 1961.

173. PROGRESS IN NUCLEAR ENERGY. SER. IV. ENGINEERING AND SAFETY. C. M. Nicholas Ed. Pcrgamon Press, London 1961.

174. SEPARATION OF STAPT ,E ISOTOPES. Johnson F. A. Encyclopaedic Dictionary of Physics. J. Thcwlis Ed. Vol. 4. Pergamon Press, London 19G1.

175. SEPARATION OF ISOTOPES. London H. Ed. Newness, London 1961.

176. ISOTOPE SEPARATION. De Michelis B. , Villani S. Politecnico di Milano. Istituto di Fisica. CISE-Segrate (Milano). Milano 1961. (In Italian)

177. ATOMIC ENGINEERING. TOME. IV.'NUCLEAR MATERIALS. (Inst. Nat. des Sci. et Tech, Nucl. and Paris Presses Universitaires de France) Vol. 1 and 2. 1961. (In French)

178. THE PRESENT STATE OF THE RESEARCH IN THE FIELD OF ISOTOPE SEPARATION IN EUROPE AND USA. Kakihana H.' J.At.En.Soc. Japan 4, 716-9,19.62. 23

179, SEPARATION FAC TOR OF DEUTERIUM ON PLATINUM HYDRO­ GEN ELECTRODE IN AQUEOUS SULPHURIC . Fulcuda M.', Horiuti J. J. Res. Inst. Catalysis, Hokkaido Univ. 10, 43-72, July 1962.

180. POWER REACTOR TECHNOLOGY. Zinn. W. H. Vol. 5. No. 4, Sept. 1962.

181. ISOTOPE SEPARATION METHODS. Gazith M. USAEC. LS-101. 1962.

182, THEORETICAL BASIS OF THE ISOTOPE CHEMISTRY. Roginskii S.S.,VEB Deutsch. Verlag Wiss. Berlin 1962. (In German)

183. HEAVY WATER ENRICHMENT IN SEA SALT MANUFACTURE. Weingaertner E. ,Datta R. L. Dechema Monograph. 47, 317-32, 1962.

184. NEW RESEARCH ON HEAVY ISOTOPES OF HYDROGEN. At. Energ. (USSR) 14, No. 6, 593-4, 196.3. (In Russian)

185. SEPARATION OF STABLE ISOTOPES. Chen W. Hua Hsueh Tung Pao. No. 8, 10-20,1963.

186. SEPARATION METHODS FOR STABLE ISOTOPES. Vasaru G. Rev. Chim. (Bucharest):

I.' CHARACTERISTICS OF THE SEPARATION INSTALLATIONS. Terminology. 14(4) 223-8,1963;

II. METHODS BASED ON REVERSIBLE PROCESSES:DISTILLA- TION, ISOTOPIC EXCHANGE, CENTRIFUGATION.'14(5) 285-9, 1963; III. METHODS BASED ON IRREVERSIBLE.PROCESSES:THERMAL DIFFUSION. 14(8) 474-8, 1963; 24

IV. METHODS BASED ON IRREVERSIBLE PROCESSES:GASEOUS DIFFUSION, MASS DIFFUSION, SEPARATION JET, MOLECULAR DISTILLATION. 14,605-9,1963. (Trans. MLM-1296 Miamisburg, Ohio. Sept. 1965)

187. BASIC TRENDS IN THE DEVELOPMENT OF METHODS FOR THE SEPARATION OF STABLE ISOTOPES. Sakodynskii K. I., Zhavoronkow N. M. Zhur. Prikl. Khim. 36(12), 2564-79, 1963. (In Russian)

183. HEAVY WATER. TIIERMOPHYSICAL PROPERTIES. Kazavchinskii Ya. Z., Kcssolman P. M., Kirillin V. A. , Rivkin S. L., SychGV V. V., Timrot D. L., Sheinlin A. E., Shpilrain E. E. V. A. Kirillin Ed. State Power Press, Moscow-Leningrad 1963. (In Russian)

189. ON HEAVY ISOTOPE OF HYDROGEN AND . Vlasov N. A. ,Samoilov L. N. At. Energ. (USSR) 17(1) 3, 1964. (In Russian)

190. ISOTOPE SEPARATION, THE FINAL STEP IN RAW MATERIAL PRODUCTION FOR NUCLEAR TECHNOLOGY. Murrenhoff A. P. Kerntechnik 6(12), 553-4, 1964.

METHODS FOR.THE SEPARATION OF STABLE ISOTOPES. Vasaru G. Rev. Chim. (Bucharest): V. METHODS BASED ON IRREVERSIBLE PROCESSES: MIGRATION, , BIOLOGICAL PROCESSES. 15(3) 156-9, 1964; VI. METHODS BASED ON SPECIFIC PROCESSES:ELECTRO- MAGNETIC AND PHOTOCHEMICAL SEPARATIONS. 15(5) 291-5, 1964. (Trans. MLM-1296. Miamisburg, Ohio, Sept. 1965) 25

192. ANALYSIS OF ESSENTIAL NUCLEAR REACTOR MATERIALS. C.J.Rodclen cd. 19G4.

193. STABLE ISOTOPE SEPARATION. Bottcr F. , Molinari Ph., Dirian G., Grünspan S. , Moncs F., Saito E. , Lerat J. M. , Roth E. CEA Saclay Rep. No. 2047. 1964.

194. SEPARATION OF ISOTOPES. Annual Progress Report. NYO-755-1. Sept. 1, 1964.

195. WATER AND IN NUCLEAR POWER PLANTS. Kot A. A. Atomizdat, Moscow 1964. (In Russian. Israel Transl. 1966)

19G. A RKVIEW OF NUCLEAR. INDUSTRY CHEMICAL TECHNOLOGY. Neumann L. Rypar V. SNTL Prague 1964. (In Czech)

197. CHEMICAL PROCESSING IN THE ATOMIC ENERGY INDUSTRY. A. It. London, Ilii'fo Books Ltd. 1964.

198. THERMODYNAMIC PROPERTIES OF HEAVY WATER. A Compi­ lation of Available Data. Lundkvist B., Persson T. Brcnnstoff- Wärme-Kraft 17(7) 356-G2, 1965.

199. HEAVY HYDROGEN ISOTOPES AND THEIR PREPARATION. Kiss I. (HUNGARY) Fiz.Szemle 15(10) 311-5, 1965.

200. SPECIAL METHODS OF STABLE ISOTOPE ANALYSIS.-Müller G. Kernenergie 8(5) 265-83, 19G5.(In German)

201. SEPARATION OF ISOTOPES:INTRODUCTION AND SUMMARY. Taylor T. I. Separation of Isotopes. Annual Progress Report 1905. NYO-755-2. Paper 1. 26

202. ISOTOPE ANALYSIS.DETERMINATION OF.HEAVY WATER AND OF URANIUM. Roth E. , Bir R. Gonio Atomique Vol. V. 1965, (p. 395-435) (also Ch. Ill)

203. SEPARATION OF ISOTOPES. Senvar C. B. Turk. At. En. Comm,. Sci. Pubi. Sor. B, Vol. VI. 1965.

204. SEPARATION OF NATURAL ISOTOPES. Selecki A. Panstwowe Wyclawn. Nauk., Warsaw 1965. (iti.Polish)

205» INTERACTIONS BETWEEN THE HYDROGEN ISOTOPES AND THEIR ORTHO- AND PARA-MODIFICATIONS. Knaap II. F. P. ot al. Disc. Faraday Soc. 40, 135-9, 1965.

206. ATOMIC ENGINEERING. VOLUME V. PRODUCTION OF BASIC NUCLEAR MATERIALS. PRODUCTION AND UTILIZATION OF ARTIFICIAL ELEMENTS. Second Edition Review and Addenda to Part of Volume IV; (Inst. Nat. des Sci. et Tech. Nucl. Saclay). Paris Presses Universitäres, 1965. (In French)

207. TECHNICAL DEVELOPMENT IN EQUIPMENT CONSTRUCTION FOR HEAVY-CHE MIC AL INDUSTRY. Plaskura W. Chom. (Gliwice) Wkladka No. 2, 1-8, 1965;No. 1, 1-6, 1966.

208. SEPARATION OF ISOTOPES. Blum J. M. Energ. Nucl. 8, 207-11, 1966.

209. THE INSTITUTE OF STABLE ISOTOPES AT LEIPZIG. MUhlenpfordt J. Isotopenpraxis 2, 113-6,1966. (in German) 27

210. PROGRESS IN PRODUCING STABLE ISOTOPES. Wetzel K. Isotopenpraxis 2,277-84, 1966. (In German)

211. HEAVY WATER. Gryson H. Rev. Ind. Minerale 48, No. 3, 182-91, 1966.

212. SEPARATION OF THE ISOTOPES OF URANIUM BY THE SEPARATION NOZZLE PROCESS. Becker E.W., Bier K., Bier W., Schnette R., Seidel D. Angew. Chem. Inst. Ed. 6, 507-18, 1967.

213.. TEN YEARS OF ISOTOPE TECHNIQUE IN ROMANIA. Mercea V. Isotopenpraxis 3,239-40,1967. (In German)

214. ISOTOPE SEPARATION. Holmberg K. E. (Aktiebolaget Atomenergi, Stockholm, SWEDEN) Svensk.Kem. Tidskr. 79, No. 2, 89-93, 1967. (In Svedish)

215. IMPROVED GAS-LIQUID CONTACTING IN CO-CURRENT FLOW. Voyer R. D. /Miller A. I. AECL-2765. 1967.

216. PRODUCTION OF BASIC MATERIALS FOR THE NUCLEAR INDUSTRY. Annual Report 1967. CEA. (CEA, Paris, FRANCE). (In French) (NP-17597. 1967. p. 109-35)

217. PRODUCTION OF DEUTERIUM. Jül-Bibl. -7. May 1967. Inf. No. 262

218. PROGRESS REPORT (on Deuterium Separation). Jan. 1, 1967-Oct. 1, 1967.NYO-3783-3.

HERMETICALLY SEALED WATER PUMPS IN NUCLEAR POWER PLANT INSTALLATIONS. Sinev N. M., Udovichenko P. M. Atomizdat, Moscow 1967. (In Russian) 28

220. OPTIMIZATION OF SEPARATION PROCESS. Dickol G. Isotopenpraxis 4,419-214, 1968. (In German)

221. THE COMING AGE OF NUCLEAR ENERGY. Weinberg A. M. Nuclear News 11, No. 7, 30-4, July 1968.

222. A LYMAN'S GUIDE TO HEAVY WATER. AECL-3034. 1968.

223. STANDARDIZATION OF THE DEUTERIUM CONTENT OF HEAVY WATER. Baertschi P., Rosatzin H. (Eidgenossisches Inst, fuer Reaktorforschung, Wuerelingen, SWITZERLAND). EIR-142. Oct. 1968. (In German)

224. PHYSICAL PROPERTIES OF HYDROGEN ISOTOPES. Shtukkenberg Yu. M. Yu.I. Moskalev Ed. Atomizdat, Moscow 1968. (In Russian)

225. ISOTOPES IN CHE MS TRY. Duncan J. F., Cook G. B. Clarendon Press, Oxford, 1968.

226. MODERATORS. Gauthron M. (Inst. Nat. des Sci. et Tech. Nucl. Saclay;Paris Presses Universitaires, Paris, FRANCE). Genie Atomique 27-43, Tome II. 1968. (In French)

227. STABLE ISOTOPES. Väsaru Gh. Ed. Technica, Bucharest 1968.

22 8. STANDARDS FOR A PRATICAL SCALE OF pD IN HEAVY WATER. Paabo M., Bates R. G. (NBS, Washington, D. C. USA). Anal. Chem. 41, 283-5, Feb. 1969. 29

WESTERN DEPOSITS: A NATIONAL SOURCE OF POWER. Steinberg M.,.Powell J., Manowitz B. (Brookhaven National Lab., Upton, N. Y. ).'BNL-50187. NOV. 1969.

ANNUAL REPORT, 1968-1969. (Atomic Energy of Canada Ltd. , Ottawa, Ont. CANADA). AECL-3326.'1969.

CHEMISTRY AND MATERIALS DIVISION. Progress Report, Oct. 1-Dec. 31, 1969. AECL. (CRNL. Chalk River, Ont. CANADA) AECL-3521 (PR-CMa-11)

REACTOR DAY 1969 OF THE GERMAN ATOMFORUM. Winnacker K. (Deutsches Atomforum e. V., Dusseldorf, W. GERMANY)NP- 17899. Apr. 16, 1969. (In German)

REVIEW OF FUEL PROCESSING TECHNOLOGY PRESENTED AT THE 1964 GENEVA CONFERENCE. Gresky A. T.(ORNL, Tenn. USA) .Progr.Nucl. Energy Ser. Ill, 4, 3-34, 1970.

HEAVY WATER AND ORGANIC FLUIDS AS AND REFLECTOR MATERIALS. Ayres J. A. (Battelle Northwest, Richland, Wash. USA). Trilling C.A. Nucl. Eng. Des. 14, 363-89, Feb. 1971.

SPECIFIC HEAT AND ENTHALPY OF LIQUID HEAVY WATER. Rosta P.Z. (Atomic Energy of Canada Ltd., Sheridan Park ()). AECL-3689. May 1971. (TDAI-43). 4 ì I i II - B113 LIOGRA IMIIES

a

ti 33

BIBLIOGRAPHIES

DEUTERIUM. A Bibliography. Chem. Eng. News 12, 11, 1934.

BIBLIOGRAPHY OF DEUTERIUM (as of Aug. 1, 1934). Young A.R. Perm. State Coll. (USA)

THE HYDROGEN ISOTOPE OF ATOMIC WEIGHT TWO. UreyH. C., Teal O.K. I nv. Mod. Ph.ys, 7, 34-94, 1935.

FIAT REVIEW OF GERMAN SCIENCE 1939-194G.

HEAVY WATER. Vol. I. Part C. Bibliography. Chapter II. Bibliogra­ phy of Published Literature, compiled by Kimball A. II. AECD-1975. June 30, 1946. Deci. May 19, 1948.

BIBLIOGRAPHY OF RESEARCH ON HEAVY HYDROGEN COM POUNDS. Kimball A. 11. comp. Urey H. C. , Kirshenbaum I. Eds. New York, McGraw-Hill, 1949. (NNES-HI-4C)

THERMAL DIFFUSION. A Bibliography. AERE-Inf/Bib-59. Feb. 1950.

DEUTERIUM AND HEAVY WATER-PHYSIOLOGICAL AND BIOLOGICAL ACTION. Bibliography of Published Literature. CAERE, Harwell Berks, UK). AERE -Inf /Bib -60. Feb. 1950. 34

9. SELECTED BIBLIOGRAPHY ON ISOTOPE .SEPARATION METHODS. Morphew A.T. TID-457.Feb. 1951. (UCRL-Bibl-5116)

10. ISOTOPE SEPARATION. A Bibliography of Separation Methods. Whetsel II. B., Mills G.F. K- 814. Oct. 1951. (UCRL-Bib-5116. Pt. II)

11. BIBLIOGRAPHY ON DISTILLATION. Lawrence S. J., Givens E. j KAPL-588. Aug. 1951. ! I I 12. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: | ANNUAL BIBLIOGRAPHY-1946. Brown L. M. , Beckett C. W. | NBS-1527. May 1, 1952. J

13. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPHY-1947. Brown L. M., Beckett C. W. NBS-1631. June 1, 1952.

14. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPIIY-1948. Brown L.M., Beckett C. W. NBS-1685. July 21, 1952.

15. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPHY-1949. Brown L. M., Goldstein J. M., Beckett C.W. NBS-1721. Aug. 1, 1952.

16. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPHY-1950. Brown L. M., Goldstein J. M. Park J. L. , Beckett C.W. NBS-1777. Sept. 1, 1952.

; ,- ' r/l-r. 35

THE BIOLOGICAL EFFECTS OF DEUTERIUM COMPOUNDS. Morowitz H.J.., Brown L.' M.(NBS, USA).NBS-2179. Jan. 14, 1953.

BIBLIOGRAPHY OF RESEARCH ON THE PROPERTIES OF THE ISOTOPES OF MOLECULAR HYDROGEN; Friedman A.S., Beckett C. W. NBS-2266. Mar.'15, 195 3.

A CRITICAL REVIEW OF THE LITERATURE RELATING TO THE VAPOR PRESSURE OF AMMONIA AND TRIDEUTEROAM- MONIA. Armstrong G.'T. (Nat. Bur. of Stand. , USA) NBS-2626. June 30, 1953.

A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPHY-1951. Brown L. M„Friedman A.S. (NBS,USA)NBS-2529. Aug. 1,1953.'

A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS. BIBLIOGRAPHY OF UNCLASSIFIED GOVERNMENT REPORTS: 1947-1952. Brown L. M. , FriedmanA. S. NBS-2492. Sept. 1, 1953.

BIBLIOGRAPHY ON DEUTERIUM SEPARATION METHODS. Drews W:'P.NYO^6084. Dec. 4, 1953. Deci. Oct. 28, 1955;(SöA-159)

A .REVIEW OF THE REACTION KINETICS OF DEUTERIUM COMPOUNDS. I. REACTION OF INORGANIC COMPOUNDS. Brown L.M., Friedman A.S; NBS-3091.March 15, 1954. 36

24. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPHY-1952. Brown L. M., Friedman A.S. NBS-3144. March 1954.

25. ISOTOPE SEPARATION AND ISOTOPE EXCHANGE. Bibliography of Unclassified Literature. Begun G. M. (ORNL), Allen R. E. (Techn. Inf. Service USA) comps. TID-3036 (Rev.) June 1954. (TID-3036, Jan. 23, 1953)

26. NUCLEAR SCIENCE:A Bibliography of Selected Unclassified Literature. TID-3070. Apr. 1955.

27. A REVIEW OF THE PROPERTIES OF DEUTERIUM COMPOUNDS: ANNUAL BIBLIOGRAPHY-1953. Brown L. M., Friedman A. S. NES-3985.Sept. 1,1955.

28. BIBLIOGRAPHY OF RESEARCH ON DEUTERIUM AND COMPOUNDS 1945 TO 1952. Brown L. M., Friedman A.S., Beckett C.W. (NBS, USA).NBS-C-5G2.Jan.27, 1956.

29. HEAVY WATER. Bibliography of British,Canadian and American Reports etc, and a Selected References to the Published Litera­ ture. Clarke R. AERE-Inf/Bib-87. (Suppl. 5). June 1957.

30. BIBLIOGRAPHY OF RESEARCH ON DEUTERIUM AND TRITIUM COMPOUNDS 1953-54. Johnson V. R., Brown'L. M., Friedman A.S. NBS-C-562(Suppl. D.July 1957. 37

A REVIEW OF THE PROPERTIES OF DEUTERIUM AND TRI­ TIUM COMPOUNDS. ANNUAL BIBLIOGRAPIIY-1955. Johnson V.R. NBS-5446,Oct. 30, 1957.

GASEOUS THERMAL DIFFUSION. I. Bibliography of Open Litera­ ture 1940-57.11. A Bibliography of the Report Literature, 1941-57. (Frost F.E.) McFadden C. UCRL-511G. Jan. 1958.

AN ANNOTATED BIBLIOGRAPHY ON HEAVY WATER AND HEAVY WATER REACTORS. Curran A. T. (Babcock and Wilcox Co. Atomic Energy Div., Lynchburg, Va. USA). BAW-47. Feb. 1958.

A REVIEW OF THE PROPERTIES OF DEUTERIUM AND TRI­ TIUM COMPOUNDS. ANNUAL BIBLIOGRAPHY-1956. Johnson V.R., Oppenheim I. NBS-5092.May 1958.

LITERATURE SURVEY ON ISOTOPE SEPARATION. LS-2 3. Nov. 1958.

THERMAL DIFFUSION. A Bibliography. Grove G.R. MLM-1088. June 1959.

ISOTOPE SEPARATION AND ISOTOPE EXCHANGE. A Bibliogra­ phy with Abstracts. Begun G. M. ORNL-2 852,Oct. 2 8, 1959.

THE HYDROGEN SULPHIDE-DUAL-TEMPERATURE PROCESS. A Bibliography of Selected Report Literature. Jacobs J.M. TID-3091. Oct. 1959. 38

BIBLIOGRAPHY ON GAS SEPARATION BY CENTRIFUGE. Thomas J.R.,Maughan G.I. DEGIS-48(R). Nov. 1959.

ISOTOPIC EXCHANGE REACTIONS BETWEEN AMMONIA AND HYDROGEN OR SOME HYDROGEN COMPOUNDS. Houberger M.', Botter F. CEA-Saclay-Bib. No. 3. 1959.

ISOTOPE SEPARATION BY GASEOUS DIFFUSION AND CENTRI- FUGATION.A Literature Search. Jacobs J.J. T1D-3554. May 1960.

NEUTRON AGE MEASUREMENTS IN WATER, D2O, WATER-ME­ TAL MIXTURES, , VARIOUS ORGANICS AND ORGANIC- ' METAL MIXTURES AND SLOWING DOWN PROPERTIES OF VA­ RIOUS MEDIA FOR . UNCLASSIFIED BIBLIOGRAPHY. Chapman M.J. (Atomic International Div. Of North American Avia­ tion, Inc., Canoga Park, Calif. USA). NAA-SR-Memo-5546. Aug. 1, 1960.

HEAVY WATER REACTORS AND TIIK PROPERTIES, ANALYSIS, HANDLING, AND EFFECTS OF HEAVY WATER. A BIBLIOGRA­ PHY. Duke D. M. (Bab'cock and Wilcnx Co. Atomic Energy Div,, Lynchburg, Va. USA). BAW-1209. Dec. 1960.

A BIBLIOGRAPHY SEARCH ON RADIOACTIVATION ANALYSIS. Gada F. CISE Rep. No. 83. Jan. 1961.

APPLICATION OF CHEMICAL EXCHANGE METHODS TO ISO- TOPIC SEPARATIONS. Drury J. S. (ORNL, Tenn. USA). Progr. in Nucl. Energy, Ser. IV, 4, 308-4.8, 1961.

ISOTOPE SEPARATION METHODS. Annotated Bibliography. Gazith M. (Israel AEC) LS/101.Juno 1962. 39

47. PHYSICAL CONSTANTS OF ISOTOPIC SUBSTITUTIONS IN WATER (Ol7-Ol8-D-T).DirianG.(CEA, Centre d'Etudes Nucl., Saclay, FRANCE). CEA-Bib-15. 1962.

48. HEAVY WATER PRODUCTION. An Annotated Bibliography of Selected Literature. Jacobs J. M., comp. (Division of Technical Information Extension, USAEC). TID-3091,(Suppl. 1) June 1964.

49. ABSTRACTS OF CANADIAN PATENTS ON THE PRODUCTION OF HEAVY WATER, Armstrong F. i; (AECL, Chalk River. Ont. CANADA). AECL-2279. July 1965.

50. BIBLIOGRAPHY OF REFERENCES FOR THE THERMOPHYSICAL 4 PROPERTIES OF IIe, H, D, HD, Ne, Ar, N, O, C02, CII4, C2H6, Kr AND REFRIGERANTS 13, 14, AND 23.Dimiduk P. W. AFML-65-338. 196 5.

51. PHYSICAL AND CHEMICAL PROPERTIES OF AMMONIA. Bibliographic Compilation, Jacolin O. CEA-Bib. No. 57. 19G5.

52. BIBLIOGRAPHY OF HEAVY WATER PRODUCTION. Shah P.G.S. (Pakistan AEC). AECL-CHEM-103. 1966.

53. LIST OF UNCLASSIFIED REPORTS AND PAPERS PUBLISHED BY STAFF OF THE ISOTOPE RESEARCH DIVISION. 1950-1965. AERE-Bib. 127(Rev. 1). 1966.

54. MOLECULAR PHYSICAL PROPERTIES OF THE HYDROGEN ISOTOPES AND THEIR ISOTOPIC COMBINATIONS. Biblio- graphycal Compilation. Guizouarn L. CEA-Bib-87. 1967.

55. .METHODS FOR HEAVY WATER PRODUCTIONS.(Foreign Patents). Bakin V.O. Moscow TNIIPI, 1967. 40

56. THERMAL DIFFUSION. A Bibliography. Vasaru Gh. Räp. I. IAEA, Vienna, STI/PUB/21/28.1968.

57. LIST OF PATENTS OF I-I2S-ri20 EXCHANGE, OF DUAL TEMPE­ RATURE SYSTEMS AND ABSTRACTS OF H2S-H20 PATENTS. Vasaru Gh. IFA-AG-4.May 1970. (Unpublished Report)

58. HEAVY WATER REACTORS. Bibliographical Series No. 37. STI/PUB/21/37.IAEA, Vienna, 1970.

59. DEUTERIUM AND HEAVY WATER. A Selected Bibliography. Vasaru Gh., Ursu D., Szentgyórgyi P., Mihaila A. (Academia R.S.R. Cluj,Inst.de Fizica Atomica, ROMANIA) Cluj 1970.

6u. STABLE ISOTOPES. Vasaru Gh. (Academia R.S.R. Cluj, Institululde Fizicä Atomica) CEA-Bib-136.Sept. 1970.

61. BIBLIOGRAPHY ON PRODUCTION OP HEAVY WATER. Nagrathna R. A. (comp). Bhabha Atomic Research Center, Bombay (India) . BARC-BIB-3. 1970 Ill - DETERMINATION AND ANALYSIS OF DEUTERIUM AND HEAVY WATER 43

III - DETERMINATION AND ANALYSIS OF DEUTERIUM AND HEAVY WATER

1. ADDITIONAL EVIDENCE FOR AN ISOTOPE OF HYDROGEN OF MASS 2.Bleakney W. Phys.'Rev.'39, 536, 1932.

2. MASS SPECTROSCOPHIC RESEARCH ON HYDROGEN AND HELIUM. Kallmann H. , Lasareff W. Naturwissenschaften 20, 206,1932.

3. ISOTOPIC ANALYSIS OF WATER. Crist R. H. , Murphy G. M. , UreyH-.C. J. Am. Chem. Soc. 55, 5060-1, 1933.

4, MICROPYCNOMETER, FOR THE DETERMINATION OF DIF­ FERENCES IN THE ISOTOPIC RATIO OF WATER. GÜfülan E. S. Jr. ,-PoIanyi M. Z. Physik. Chem. A 166,254-6,1933.

5. THE USE OF THE INTERFEROMETER IN THE ISOTOPIC ANA­ LYSIS OF WATER. Crist R. H., Murphy G. M. , Urey H. C. J. Chem. Phys. 2, 112-5, 1934.

6. AN EXAMINATION OF WATER FROM VARIOUS NATURAL SOURCES FOR VARIATIONS IN ISOTOPIC COMPOSITION. Washburn E. W., Smith E.R. Bur. Standards J. Research 12, 305-11,1934. 44

PREPARATION OF PROTIUM OXIDE AND THE DETERMINATION OF THE PROPORTION OF DEUTERIUM IN THE HYDROGEN OF NORMAL WATER. Ingold E. II., Ingoici C. K. , Whitaker H. , Whytlawgray R. Nature 134,661,1934.

MICRO-METHOD FOR THE DETERMINATION OF HEAVY WATER. Goldfinger P., Scheepers L. Compt. Rendu. 198, 1916-8, 1934.

THE DETERMINATION OF THE DEUTERIUM CONTENT OF THE DILUTE HEAVY WATER BY FLOATING METHOD. Harada M. J. Chem.Soc. Japan 5G, 811-8, 1935.

INTERFEROMETRIC ANALYSIS OF HEAVY WATER. Filippova N.S. ,Slutskaya M. M. Acta Physicochim. USSR 5, 131-6, 1936.

INTERFEROMETRIC ANALYSIS OF HEAVY WATER. Filippova N. S. , Slutskaya M. M. J. Phys. Chem. USSR 8, 468-71,1936.

PRODUCTION OF LIGHT WATER AND THE DETERMINATION OF THE DEUTERIUM CONCENTRATION OF ORDINARY WATER. Morita N., Titani T. Bull. Chem.Soc. Japan 11,403-13,1936.

A MICRO METHOD FOR THE ACCURATE DETERMINATION OF D20 IN WATER. Feuger-Eriksen K., Krogh A., Ussing II. Biochem. J. 30, 1264-9, 1936.'

A METHOD OF ANALYSIS OF HEAVY WATER. Farkas A. Trans. Faraday Soc. 32,413-5, 1936. 45

A SIMPLE METHOD FOR THE DETERMINATION OF D20 CONTENT OF- SMALL QUANTITIES OF WATER. Fromherz H. , Sonderhoff R. , Thomas H. Ber. 70B, 1219-23, 1937.

A METHOD FOR THE ANALYSIS OF HEAVY WATER. Filippova N. S., Slutskaya M, M. Trudy Dnepropetrovsk. Khim. -Tekh. Inst. 14-24, 1938. (Khim, Referat. Zhur. 2, No. X, 9, 1939)

MEASUREMENT OF THE DEUTERIUM CONTENT IN MIXTURES OF H2O AND D2O.Lindersti'oem-L)ng K., Jacobsen O. ', JohansenG. Compt. Rend. Trav. Lab. Carlsberg, Sér. chim. 23, 17-25, 1938.

PRECISION DETERMINATIONS OF THE OF DEU­ TERIUM OXIDE AND WATER.ELECTROLYTIC SEPARATION OF THE OXYGEN ISOTOPES. Tronstad L., Brun J. Trans, Faraday Soc. 34, 766-73, 1938.

DETERMINATION OF HEAVY HYDROGEN. Harteck P. Z.Electro- chem. 44, 3-8, 1938.

A MODIFIED MICROPIPET FOR DETERMINATIONS IN HEAVY WATER ANALYSIS. Rosebury F. , van Heyningen W.E. Anal, Chem. 14, 363-4, 1942.

A MASS SPECTROMETER FOR ROUTINE HYDROGEN ISOTOPE ANALYSES:SUPPL. No.l. Nier A.O.C.,Stevens C.'M.', Rustad B. AECD-2767. Mar, 17, 1943. Deci. Jan, 3, 1950. 46

MODIFICATION OF APPARATUS FOR DEUTERIUM OXIDE DETERMINATION BY THE FALLING DROP. Fetcher Jr.F.S. Ind.Eng.Chem.Anal.Ed.TG,^, 1944.

CHEMICAL RESEARCH-ANALYTICAL REPORT FOR MONTH ENDING JULY 1, 1944. (Chicago Univ, Metallurgical Lab. USA). CC-1915. Aug; 11, 1944.'Deci. Jan. 30, 195G.'(A-2803)

METALLURGICAL PROJECT REPORT. Fischer R.B., Potter R.À.,VoskuylR. J. MUC-DHT-103.

THE SPECTROGRAPHIC ASSAY OF HEAVY WATER. (Based on CC-24G7).Tomkins F. S., Fred M. (ANL^ 111. USA). AECD-3100; ANL-HDY-577. Deci. Mar. 21,1951.

METALLURGICAL PROJECT REPORT. Brayson J. A, M-CP-1928, July 1944.

ANALYSIS OF HEAVY WATER BY EQUILIBRATION. Fischer R.B. , Potter R.A.,Voskuyl R.J. (Univ. Metallurgical Lab. Chicago, USA). CC-2994. May 15, 1945. Deci. Dec. 15, 1955.

STANDARDIZATION OF THE pD SCALE.'Fischer R. B., Potter R. A.CC-3271.Sept. 12, 1945. 47

29. DETERMINATION OF DEUTERIUM IN WATER; A MASS SPECTRO­ METRY METHOD. Fischer R. B., Potter R. A. , Voskuyl R. J. Anal. Chem. 20/571, June 1948. (MDDC-1208, deci. Aug. 8, 1947).

30, DETERMINATION OF DEUTERIUM IN WATER. CONVERSION TO METHYL DEUTERIDE AND AND MEASUREMENT BY MASS SPECTROMETER. Orchin M., Wender I. ; Friedel R. A. Anal. Chem. 21, 1072, 1949.

31. THE DETERMINATION OF HEAVY WATER. Puddington I. E. Can. J.Res.27B, 1-5, Jan. 1949.

32. ANALYTICAL CHEMISTRY AND STANDARDS FOR NUCLEAR PU­ RITY. Gueron J.Atomes 4, 53-6, Feb. 1949.

33. THE RELATION OF APPARENT TO TRUE pH IN DEUTERIUM . Hart R. G.(Nat. Res. Council of Canada). CRE-423. June 1949.

34. ANALYSIS OF HEAVY WATER WITH A HIGH DEUTERIUM OXIDE CONTENT BY GRAVIMETRIC METHODS. Viallard R. Bull. Soc. Chim. France, Nos. 5-6, 265-71, May-June 1949. (AERE- Trans-ll/3/5/211;AEC-tr-1299)

35, DETERMINATION OF HEAVY WATER. Thomas B. W. Anal. Chem. 22,1476,1950.

36. HEAVY WATER PICNOMRTllY. Corrai -E., Orsoni L. , Sii vostri M.CISE-10. 1950. (In Italian) 48

DETERMINATION OF ISOTOPE RATIOS OF KNOWN DEUTERIUM- HYDROGEN SAMPLES USING A MASS SPECTROMETER. Alfin Slater R.B.,Rock S. M., Swislochi M. Anal. Chem. 22, 421-3, Mar. 1950.

A SIMPLE METHOD FOR THE DENSIOMETRIC DETERMINA­ TION OF HEAVY WATER. Sapir stein L. A. J. Lab, Clin; Med. 35, 793-4, May 1950.

INFRARED SPECTROMETRIC DETERMINATION OF DEUTERIUM OXIDE IN WATER. Thornton V., Condon F. E. Anal. Chem. 2? 690-1, May 1950.

DETERMINATION OF THE ABSORBED WATER BY EXCHANGE WITH DEUTERIUM OXIDE. EXTENSION OF THE EXCHANGE METHOD TO STUDY OF MACROMOLECULAR STRUCTURES. Villani R. J.Chim. Phys. 48, 372, 1951. (AEC-tr-1887)

ANALYSIS OF HYDROGEN-DEUTERIUM MIXTURES AND OF MIXTURES OF HEAVY-WATER AND LIGHT-WATER BY MEANS OF A MASS SPECTROMETER. Chenouard J., Gueron J., Roth E. (Commissariat à l'Energie Atomique, FRANCE). CEA-87. July, 1951.

CONTROL OF THE PURITY OF HEAVY WATER BY ELECTRIC CONDUCTIVITY MEASUREMENTS. Selmi L. (CISE, Milan, ITALY). CISE-28, 1952. (In Italian) (CEA-tr-X-405)

MEASURING THE CONCENTRATION OF DgO IN AQUEOUS SOLUTIONS OF HEAVY WATER. Cerrai E., Marchetti C., Silve­ stri M. CISE-31, 1 952. /

44. THE COLORIMETRIC DETERMINATION OF TRACES OF BORON IN HEAVY WATER. Fizzotti C. ,Selmi L. (Chimica e Industria, Milan,-Italy). 34,265-6,1052. (In Italian) (AEC-tr-1960)

45, ON THE CONCENTRATION OF HEAVY WATER IN GLACIER . SandstrBem A.E.Arkiv.Fysik, 3/549-56,1952.

46. DETERMINATION OF DEUTERIUM IN LIQUID WATER. Trenner N.R., Walker R.W.The Perkin-Elmer Instrument News 4, No. 1, 1, 1952.

47. APPLICATION OF A FLOAT METHOD TO RAPID MEASURE­ MENT OF D2O CONCENTRATION IN AN OF HEAVY WATER. Cerrai E. , Marchetti C. , Silvestri M. , Nuovo Cimento (9), 9, 530-4, June 1952. (In Italian)

48# THE ISOTOPIC ANALYSIS OF HYDROGEN IN VARIOUS COMPOUNDS. Bigeleisen J. , Perlman M. L. , Prosscr H. C. Anal. Chem. 24, 135G-7, 1952. (BNL-1058)

49. MASS SPECTROMETRIC DETERMINATION OF DEUTERIUM IN WATER. Goodall C. A. , Alkire G.'J. HW-25258. Aug. 20, 1952.'

50. CONVERSION OF HYDROGENIC MATERIALS TO HYDROGEN FOR ISOTOPIC ANALYSIS. Bigeleisen J., Perlman M. L. Prosser U.C. Anal. Chem. 24, 135G,Aug. 1952.

51.'PRECISION DETERMINATION OF DEUTERIUM IN H20-D20 'MIXTURES BY A PICNOMETER METHOD. Silverman L... Gossen W.NAA-SR-236, 1953. 50

52. MEASUREMENT OF DEUTERIUM OXIDE CONCENTRATION IN WATER SAMPLES BY THE MASS SPECTROMETER. Washburn H.W., Berry C.E.,IIall L. O. Anal. Chem. 25, 130-4, Jan. 1953.

5(3. INFRARED Sl'ECTRA OF HEAVY WATER ADSORBED ON SILICA GEL. P it tu; il lui Ci. C. , Garland C. W., Jura G. J. Am. Chem. Soc. 75, 803-5, Feb. 20,1953.

54. ISOTOPIC PROPORTION OF WATER BY MEASUREMENT OF ABSORPTION IN THE INFRARED. Lecomte J., Ceccaldi M., Roth E. J. Chini. Phys. 50, 1G6, Mar. 1953.

55. USE OF HEAVY WATER AS SOLVENT FOR SPECTROSCOPIC INVESTIGATION IN NEAR INFRARED.Evstigneev V. B.Doklady Akad.Nauk.S.S.S. R. 89,105-8,Mar. 1,1953.

56. DETERMINATION OF HEAVY WATER WITH THE HOT WIRE GAGE, llaldeman 11. G. Anal. Chem. 25, 787-90, May 1953.

57. INFRARED SPECTRA .AND MOLECULAR STRUCTURE OF SOME GROUPS VI 11EXAFLUORIDES. Canni J. AERK-C/U- 1264, Oct. 22, 1953.

58. THE DETERMINATION OF THE. DgO CONTENT OF HEAVY WATER BY A MASS SPECTROMETER. Reynolds P., Loveridye B. A. (AERE, Harwell, Berks, UK). AERE-GP/R-1282. Oct.. 26, 1953.

59. FINAL REPORT COVERING THE PERIOD JUNE 15, 1948 TO DECEMBER 31,1953. Carpenter R. B., McDonough R., Patterson W. A. (Bairtl Associates, Inc. USA). NP-501 5. 51

GO. THE DETERMINATION OF THE D2O CONTENT OF HEAVY WATER BY INFRARED SPECTROMETRY. Stevens W. II., Thurston W. M. (AECL, Chalk River, Ont. CANADA). AECL-295. 1954.

61. DENSITY OF HEAVY WATER ENRICHED IN OXYGEN ISOTOPES DETERMINED BY ELECTROLYTIC METHOD. Isberg P., Luiidberg L. Z. Naturforsch. 9,472-3, 1954.(In German) (CEA-tr-A-955)

62. A METHOD FOR THE ANALYSIS OF MICROSCOPIC QUANTITIES OF HEAVY WATER. Mardaleishvili R. E. , Lavrovskaya G. K., Voovodskii V. V. Zhur. Fiz. Khim. 28, 2195-8, 1954. (In Russian)

63. RECORDING DIFFERENTIAL HEFRACTOMETER. Campbell D. N., Fellows C.G., Spraklen S.B.et al. Ind. Eng. Chem.46, 1409, 1954.

64. A SIMPLE INFRARED GRATING SPECTROMETER FOR USE IN ANALYSIS. Gaunt J. AERE-C/R-13D8. Apr. 9, 1954. .

65; A MASS SPECTROMETER FOR THE ISOTOPIC ANALYSIS OF HYDROGEN CONTAINING A LOW CONCENTRATION OF DEUTERIUM. Reynolds P.-AERE-CP/R-1449, Aug. 1954.

66. THE DETERMINATION OF DEUTERIUM OXIDE BY INFRA-RED SPECTROMETRY.Gaunt J. (Atomic Energy Res. Establ., Harwell, Berks, UK). Analyst 79, 580-5, Sept. 1954.

07. A DIFFUSION-EQUILIBRATION METHOD AS A STAGE IN THE DETERMINATION OF THE DEUTERIUM OXIDE CONTENT IN 1-2 MICROLITRES OF FLUID. Lars Garby (Univ. of Uppsala, SWEDEN). Acta Chem.Scand. 9, ,\... 2, 339-41, 1955. 52

68. DETERMINATION OF SMALL QUANTITIES OF AND OXYGEN OCCURRING AS IMPURITIES IN tJYDROGEN AND HELIUM. Zinovyeva N. P. Zavodskaya Lab. 1, 1955. (In JUissian)

69. CONTINUOUS ANALYSIS OF ORTHO-PARA-HYDROGEN MIX­ TURES. Woitzcl D. II., Wlüte L. E. Rcv. Sci. Instr. 26, 290, Mar. 1955..

Proceedings of the International Conference on tlie Peaceful Uses of Atomic Energy, Geneva 1955.

70. INFRA-RED METHODS FOR ANALYSIS OF HEAVY WATER. Gaunt J. 8, P/410(UK).

71. ON METHODS OF ISOTOPIC ANALYSIS OF HEAVY WATER. Vladimirskii K. V., Kats M. Ya., Stasevich B. M. 8, P/63KUSSR).

72. ISOTOPIC ANALYSIS OK WATER EY NEAR INFRA-RED SPECTRO­ PHOTOMETRY. SillM-rnuiii K.8, P/1010().

73. DETERMINATION OK SMALL AMOUNTS OF DEUTERIUM OXIDE IN-WATER BY INFRA-RED . Berglund- Larsson U. (Nobel Inst, of Chemistry, Stockholm, SWEDEN). Acta Chem.Scand. 10, No. 4, 701-2, 1956.

74. THE ANALYSIS OF HEAVY WATER BY INFRA-RED SPEC­ TROMETRY. Gaunt J. (Atom*« Energy Res. Establ. .Harwell, Didcot, Berks, UK). Spect.rochim. Acta 8, 57-65, 1956. (AERE- C/lt- IfiSti. Apr. 25, l!)5fi). 53

75. AN APPARATUS FOR CONTINUOUS ISOTOPIC ANALYSIS OF HYDROGEN-DEUTERIUM MIXTURES. Silvestri M., Adorni N. Nuovo Cimento X-4, 1610, .1956.

INVESTIGATION OF "BITTERNS" AS A SOURCE FOR HEAVY WATER. Weingaertncr E., Datta R. L. (Indian Inst, of Sci., Ban­ galore, INDIA). J.Indian Inst. Sci. 38, 73-86, Jan. 195G.'

77_ THE ANALYSIS OF HEAVY WATER. Bryant F. J. (United King­ dom Atomic Energy Authority. Res. Group. Chem. Div., Woolwich Outstation, UK). Mar. 1956.

78. ISOTOPE SPECTRAL ANALYSIS. Stziganov A. R. Uspekhi Fiz. Nauk 58, 365-414, Mar. 1956. (In Russian)

79. A MICROFLOTATION METHOD OF ANALYZING HEAVY WATER. Gragcrov I. P. (L. V. Pisarzhevsky Inst, of Phys. Chem. USSR). Zhur Anal.Khim. 11, No. 3, 264-8, May-June 1956. (In Russian) (English translation)

80. CONTINUOUS MEASUREMENT OF DEUTERIUM CONCENTRA­ TION BY MEANS OF TI1KRMAL CONDUCTIVITY. Silvestri M., Adorni N. Rev. Sci. [n.str. 27, 388, June 1956.

81. THE-DETERMINATION OF DEUTERIUM BY THE MASS-SPEC- TROMETRIC METHOD. MnrDonald A.., Reed R. I. (Univ. of Glasgow,•UK). Analyst 81, -I0I- 3,July 1956. 54

82. APPLICATION OF FLOAT METHOD FOR PRECISION MEASU­ REMENT OF DENSITY OF WATER BETWEEN 3, 7 AND 4, 2PC AND FOR DENSITY MEASUREMENTS OF VERY SMALL SAMPLES OF SOLID SUBSTANCES. Spaepen J. Mededcl Konikl. Vlaam. Akad. Wetenschap.Belg.Kl. Wetenschap, 19, No. 5, 1957. (AEC-tr-3847).

83. ANALYSIS OF D20/H20 BY THE INTERFEROMETER. Namba S. (Sei. Res. Inst., Ltd., Tokyo, JAPAN). Rev. Sci. Instr. 27, 872-3, Oct. 1956.

84. METHODS FOR ISOTOPIC ANALYSIS OF WATER. I. NEW AP­ PARATUS FOR THE FALLING DROP METHOD OF ISOTOPIC ANALYSIS OF WATER. Shatenstein A. Y. , Varshav skii' Y;i. AI. (Karpov Moscow Physico-Chemical Inst. ). Zhur Anal. Khim. 11, No. 6, 746-8, Nov. -Dec. 1956.(In Russian)

85. MEASUREMENT OF LOW DEUTERIUM CONCENTRATION IN WATER BY-MEANS OF FLOAT METHOD. Brigoli B., Cerrai E., Silvestri M. (CISE Labs., Milan, ITALY). Energia Nucleare 4, 43-9, Feb. 1957.

86. MEASUREMENT OF DEUTERIUM CONTENT IN HIGHLY ENRICH ED SAMPLES OF HEAVY WATER BY MEANS OF A FLOAT METHOD. Adorni'N., Brigoli B., Silvestri M. Energia Nucleare, (Mili.ui)4, 31.5-8, Aug , 1957.

87. ISOTOPIC ANALYSIS OF HEAVY WATER BY NUCLEAR RESO­ NANCE. Goldman M. (Savannah River Lab., Aiken, S. C. USA). Arch. Sci. ,(Geneva) 10,247-0, 1957. (AEC-tr-5328)

88. APPARATUS FOR STANDARD MEASURING OF DEUTERIUM ISOTOPIC EXCHANGE RATE BETWEEN HYDROGEN AND AT ATMOSPHERIC PRESSIIUK AND 100°C. Silvestri M., Adorni N. Nuovo Cime-ilio V. (Serie X)-2fi(i, 1957. (In Italian) 55

89. THE DEUTERIUM OXIDE CONTENT OF WATER SAMPLES FROM OIL-FIELDS. Cziké K./Fodor P. Acta geol.-Acad.Sci. Hung. 4, 331-9, 1957. ' 90. DETERMINATION OF THE CONTENT OF HEAVY WATER IN A MIXTURE OF HEAVY AND NORMAL WATER. Fort A. (Karlovy Univ., Prague, CZECHOSLOVAKIA). Czcchoslov. J. Phys. 7, 740-4, 1957. (In Czech)

91. THE DETERMINATION OF DEUTERIUM OXIDE IN WATER BY FREEZING POINT MEASUREMENTS. Fodor P.,Czike K. Magyar Kein. Folyci.-.-ut (;;}, No. 2-3, 95-6, 1957. (In Hungarian)

92. A STUDY ON THE FALLING-DROP METHOD OF ANALYSIS OF HEAVY WATER. Ching-Lien Chang, Chih-Hsiang Cheng, Hui- Pillsu. Sci. Record (Peking) 1,417-19, 1957.

93. A METHOD FOR THE SPECTRAL QUANTITATIVE ANALYSIS OF THE ISOTOPIC COMPOSITION OF IlHAVY WATER. Dontsov P. Yu. , Striganov A.R. Zhur. Analit. Khim. 12, 6-9, Jan. -Feb. 1957. (In Russian)

94. METHODS FOR ISOTOPIC ANALYSIS OF WATER. II. NEW LIQUIDS FOR THE DROPPING METHOD OF THE ISOTOPIC ANALYSIS OF WATER WITH A DEUTERIUM CONCENTRATION UP TO 100%. Shatenstein A. I., Yakovleva E. A., GP.adkova E. N. , Suzdaltseva S. F., Antipova N.P. Zhur Anal. Khim. 12, No. 1, 115-7, Jan.-Feb. 1957. (In Russian) 9S\ ANALYSIS OF MIXTURES OF LIGHT AND HEAVY WATER BY MEANS OF A SIMPLE INFRARED PHOTOMETER. Berton A. , Ceccaldi M. Chini. Anal. No. 3, 102-3, Mar; 1957. (In French)

96. METHODS FOR ISOTOPIC ANALYSIS OF WATER. III. THE COMPLETE ISOTOPIC ANALYSIS OF WATER BY DECOMPOS­ ING WITH IRON. SJiatenshtein A. I., Varshavskii Ya. M. (Karpov Moscow Physico-Chemical Inst. USSR). Zhur. Annlit. Khim. 12, 236-9, Mar. -Apr. 1957. (In Russian) 56

97. • METHODS FOR ISOTOPIC ANALYSIS OF WATER. IV. METHOD FOR COMPLETE ANALYSIS OF WATER. Shatenstein A. I. , Yako- vleva E. A., Suzdallscva S. F., Antipova N. P. Zhur. Anal. Khim. 12, No. 3, 398-401, May-June 1957. (In Russian)

08. METHODS FOR ISOTOPIC ANALYSIS OF WATER. V. A FLOAT METHOD FOR MEASURING DENSITY DIFFERENCE WITH AN ACCURACY WITHIN +0, 2 . Shatenstein A. I. , Zvyagintseva E. I. Zhur. Anal. Khim. 12, No.4. 5.16-22, July-Aug. 1957.

99. IN THE ISOTOPIC ANALYSIS OF DEU­ TERIUM. Brigoli B.Energ.Nucl. (Milan) 4, No 5, 4 11-9, Oct. 1 957. (In Italian)

100 A NEW BALANCING DROP METHOD FOR THE DETERMINA­ TION OF THE DENSITY OF HEAVY WATER. Yoshihide Naito (Tokyo Metropolitan Univ., Sctagaya, JAPAN). Bull. Chem. Soc. Japan 30, 939-40, Dec. 1957.

101. DENSIMETRIC METHODS FOR ISOTOPIC ANALYSIS OF DEUTE­ RIUM. Brigoli B.Encrg. Nucl. (Milan) 4,483-91, Dec. 1957. (In Italian)

102. APPARATUS FOR THE CONTINUOUS ANALYSIS OF MIXTURES OF ORTHO-PARA HYDROGEN AND DEUTERIUM. Vasilyev D.I. , Shalnikov A. I. Pribory i tekh. eksp.4, 1958. (In Russian)

103. MASS Sl'K( TROMETRIC ANALYSIS OF SOME HYDROGEN OX­ IDES. Kei-win I. L. , Col tin M. Can. J. Phys. 3(i, 184-91, Feb. ] 958. 57

Proceedings of the 2nd United International Conference on the peaceful Uses of Atomic Energy, Geneva 1958: 104. HEAVY WATER MONITORING BY . Stevens W. H. Bayly I. G. 28, P/188 (CANADA);

105. QUANTITATIVE DETERMINATION BY NUCLEAR MAGNETIC RESONANCE. Ionel Solomon. (CEA, Paris). 28, P/l 154 (FRANCE);

106. THE NUCLEAR AS A TOOL FOR DETEC­ TION, ANA LYSIS AND STRUCTURE OF CHEMICAL COMPOUNDS. Dharmatti S. S. , Kanekar C.R.,Mathur S.C.(Tata Inst, of Funda­ mental Res., Bombay,

107. NON DISPERSIVE INFRA-RED ANALYSIS MIXTURES OF WATER AND HEAVY WATER. Bosselaar C. A. (Stichting voor Fundamen- teel Ondcrzock dor Materie, Utrecht). 28, P/2250. (NETHERLAND)

108. DETERMINATION OF DEUTERIUM OXIDE IN WATER BY MEASUREMENT OF FREEZING POINT. Reaser P. B., Burch G.E, (Tulane Univ. and Charity Hospital of Luisiana, New Orleans USA). Science 128, 415-6, Aug. 22, 1958.

109. MEASUREMENT OF SMALL AMOUNTS OF H2O IN D?0 BY NEAR-INFRARED ABSORPTION SPECTROSCOPY. Biggers R.E. (Oak Ridge Nat. Lab. , Term. USA). CF-58-12-143. Dec. 8, 1958. 58

HO. DETECTION OF THE LEAKS OF HEAVY WATER FROM A REAC­ TOR INTO THE LIGHT WATER OF ITS EXCIIANGFRS. Julliot C. , Lousiart A., Nordemann D. (CEN, Saclay, FRANCE). "Nuclear Electronics I. "p. 435-40. Proc. Int.Symp. Paris 1958. IAEA 1959.

111. ANALYSIS OF HEAVY WATEu. IN CONCENTRATIONS AP­ PROXIMATE TO THAT EXISTING IN NATURAL WATER. Otero de la Gandnrn J. L. ,Gispert M.G. Anales Real Soc.Espan. Fis. y Qium. (Madrid) Ser.B 55B, 73-82, 1959. (In Spanish)

112. SIMPLIFIED FLOAT METHOD FOR THE DETERMINATION OF THE D20 CONTENT OF WATER. Baertschi P. , Thllrkauf M. (Univ. of Basel, SWITZ. ). Hclv. Chim. Acta 42, 282-93, 1959. (CEA-tr-A-GGG)

113. TEMPERATURE-FLOAT METHOD FOR ISOTOPIC ANALYSIS OF HEAVY WATER WITHIN LOW CONCENTRATION RANGES Weingaertncr E., Datta R. L. , Kumar R., MJiacbvan E..G. Indian Inst. of. Sci. Golden Jubilee Res. Volume 1909-1959, p. 170-80,1959.

114. SEMI-MICROMÉTHOD FOR ISOTOPIC ANALYSIS OF SUB­ STANCES CONTAINING ABOUT 100% OF DEUTERIUM. Shatcnshtcin A. I., Antnnchik Yu.I. (Karpov Physico-Chemical Inst., Moscow, USSR). Zhur. Anal. Khim. 14, 100-3, Jan.-Feb.11959. (In Russian)

115. MEASUREMENT OF THE PURITY OF GRAPHITE AND HEAVY WATER. Hering H. (Commissariat à l'Energie Atomique, Paris, FRANCE). CEA-1094. Feb. 1959.

HB# ANALYTICAL CHEMISTRY DIVISION ANNUAL PROGRESS REPORT FOR PERIOD ENDING DECEMBER 31, 1958. (Oak Ridge Nat. Lab. , Term. USA). ORNL-2662. Mar. 3, 1959. 59

n,7( AN EXPERIMENTAL DETERMINATION OF SPECIFIC VOLUMES OF HEAVY-WATER. Kirillin V. A. , Oulibin S. A.Teploenerge- tikaNo. 4, 67-72, Apr. 1959. (In Russian) (CEA-tr-R-1579)

Proc.oi the 6th Tripar'ite Instrumentation Conf., Chalk River, Ontario, Canada, Apr. 1959. AECL-801: 118. RECENT DEVELOPMENTS IN THE INFRA-RED ANALYSIS OF HEAVY WATER. Bayly J., Stevens W. H. (Atomic Energy of Canada Ltd. , Chalk River, Out. CANADA). AECL-801;. p. 39-41;

119. DETECTION OF D20 LEAKAGE IN HEAT EXCHANGERS. Gruber G. 1-1. (Du Pont de rumours E.I. tv Co.Savannah River Plant, Aiken S.C. USA). AEC. 301,: p. 73-6.

120. THE SPECTROGRAPHIC DETERMINATION OF IMPURITIES IN HEAVY WATER. Webb R. J. (United Kingdom Energy Autho­ rity. Res. Group Chemistry Div., Woolwich Outstation, UK). AERE-AM-8. Apr. 1959.

121. ISOTOPIC ANALYSIS OF WATER. Kats M. Ya., Lapteva F. S. Zhur. Anal.Khim. 14, No. 2,227-33, Mar. -Apr. 1959. (In Russian)

122. ANALYSIS OF HgO AND D20 MIXTURES BY INFRA-RED SPECTROSCOPY. DETERMINATION OF MOLECULAR EX­ TINCTION COEFFICIENTS. Ceccaldi M. (Centre d'Etudes Nuel., Saclay, FRANCE). Rev. Universelle Mines(9)15,May 1959. (CEA-1285; AEC-tr-5270)

123. TRITIUM GENERATION IN D20 SYSTEMS OF PRTR. Regimbal J. J., Hayward W. H. (General Electric Co. Hanford Atomic Prod­ ucts Operation,. Richland, Wash. USA).HW-61151. July20, 1959.

124. DETERMINATION OF LOW CONCENTRATION OF DgO IN WATER BY THE FLOTATION METHOD. Report No. 27. Canna vale L. (Comisìon Nacional de Energia Atòmica,. Buenos Aires, AR­ GENTINA). I960. 60

125., DEUTERIUM CONTENT OF THE U. S. NATIONAL BUREAU OF STANDARDS ISOTOPE REFERENCE SAMPLES. Yoshio Horibe, Mituko Kobayakawa, (Tokyo Metropolitan Univ., Tokyo, JAPAN). Bull.Chem. Soc. Japan 33, 116-7, Jan. 1960.

12G. THE ANALYTICAL PROBLEMS AND THE PRODUCTION OF HEAVY WATER. Niof G. Bull. Inform. Sci. et Tech. (Paris) No. 40, 19-23, May 19G0. (In French)

127. ISOTOPIC ANALYSIS OF HEAVY WATER OF THE REACTOR. Sandroni S. (CNRN, Ispra, ITALY). CNI-33. May 1960.

128. ANALYSIS OF HEAVY WATER BY DENSITOMETRIC METHODS Ching-Lien Chang (Univ. of Peking, CHINA). Kernenergie 3, 892-7, Sept. I960.

129. DETERMINATION OF THE CONCENTRATION OF HEAVY WATER IN THE NATURAL OF CHILE. la. WATERS OF THE REGION OF CONCEPCION. Fighetti C.,Schenkel G. et al. (Univ. de Concepcion, CHILE). Boi. Soc. Chilena Quim., 10, 1-5, Dec. 1960. (In Spanish)

130. ANALYSIS BY MASS SPECTROMETRY OF SAMPLES OF LIGHT WATERS ENRICHED WITH D20 UP TO 1%. Barbieri W., Chiesa A. et al. (CNRN, Ispra, ITALY). CNI-42. (In Italian)

131. ANALYSIS OF D20/H20 INTERFEROMETER. Versino B. (CNRN CSN, Ispra, ITALY). CNI-46. (In Italian)

132. ISOTOPIC ANALYSIS OF LIGHT WATER. Sandroni S., Barbieri W. (CNRN;CSN, Ispra, ITALY). CNI-46. (In Italian) 61

133; THE SPECTROGRAPHS ANALYSIS OF INORGANIC IMPURITIES IN HEAVY WATER. Artaud J.,Normand J., Vie R. (Commissa­ riat a l'Energie Atomique. Contro d'Etudes Nucl. ,Saclay, FRAN­ CE). CEA-1027. 19G1.

134. A NON-DISPERSIVE INFRARED ANALYZER AND ITS USE­ FULNESS FOR THE ANALYSIS OF MIXTURES OF WATER AND HEAVY WATER. Bosselaar C. G. A. Thesis, Utrecht, Rijksuniversiteit, 10G1. (In Dutch)

135. PROGRESS REPORT FOR 1961. Stichtag voor Fundamental Onderzoek, Utrecht;Stiching Institut voor Kernphysisch Onderzoek, Amsterdam. NP-12208, 1961.

136. THE COULOMETRIC DETERMINATION OF BORIC OXIDE IN HEAVY WATER. Parker A. , Terry E. A. (UK Atomic Energy Authority.Res. Group Chemistry Div. , Woolwich Outstation, UK). AERE-AM-72. Jan. 1961.

137. ANNUAL.REPORT OF ICPP ANALYTICAL SECTION FOR 1960, Shank R. C. (Phillips Co. Atomic Energy Div. Idaho Falls, Idaho, USA). IDO-14547. Apr. 14, 1961.

138. HEAVY WATER ANALYSIS IN THE 1% TO 99% D20 RANGE BY INFRARED SPECTROPHOTOMETRY. Stevens W. H., Bayly J. G. et al, (Atomic Energy of Canada Ltd. , Chalk River, Ont., CANADA). AECL-1391. Sept. 1961. (CRDC-1051)

139. ON THE EXPERIMENT ON THE ANALYSIS OF THE HEAVY WATER BY INFRA-RED SPECTROMETRY. Okabe T. ,Denki Shikensho Iho25, 679-86, Sept. 1961. (In Japanese) 62

140.. DETERMINATION OF DEUTERIUM CONCENTRATION UM HEAVY WATER BY THE REACTION 0*6(d, n)FJ'INDUCED BY REACTOR NEUTRONS; Amiel S. , Peisach M. (Atomic Energy Commission, Tel Aviv, ISRAEL). IA- 692. Oct. 1961.

141. HEAVY WATER ANALYZER WITH INTERFERENCE FILTER. CeccaJdi M,, Goujon P. (CEA, CEN, Saclay, FRANCE),TID-7629 : p. 91-109.(ÖRNL, USA). Analytical Chemistry in Nuclear Reactor Technology. 5th Conf. Gatlinburg Term. USA. Oct. 1961.

142. ANALYSIS OF HEAVY WATER AT NEAR NATURAL WATER CONCENTRATIONS. PART II. Otero de la Gandara J.L.,Gispert M. (.'<. Anales Real Soc. Espan. Fis. y Quim. (Madrid)Ser. B, 57, 827 :?2,Dec. 1961.

14 3, A SIMPLIFIED WAY OF DETERMINING DEUTERIUM IN WATER BY THE FALLING UHOP METHOD. Zlotowaki J., Wroblewska M. (Univ. of Warsaw, POLAND). Nukleonika 7, 775-88, 1962. (In Polish)

144, RECORDING HYDROMETER FOR LIQUIDS ESPECIALLY ADAPT­ ED TO THE CONTINUOUS MEASUREMENTOF HEAVY WATER. Chatel S.,Nief G. (CEN, Saclay, FRANCE). CEA-2184. 1962. (In French)

145. EXPERIMENTAL DETERMINATION OF HEAVY WATER DEN­ SITY AT HIGH PRESSURES AND TEMPERATURES. Rivkin S. L., Akhundov T. S. (All-Union Inst, of Thermal Tech., USSR). Teploenergetika, No. 5,62-5, 1962. (In Russian).

146, THE DETERMINATION OF THE D20 CONCENTRATION IN HEAVY WATER BY THE FLOAT METHOD. Kummerer K. (Kern- forschiingszentrumn, Karlsruhe, GERMANY). Z. Physik 169, 166-77, 1962. (In German) 63

147. DETERMINATION OP HEAVY WATER PURITY BY INFRARED ABSORPTION. Abernathey R. M., Morgan T. D. (Phillips Petroleum Co. Atoivu: Energy Div. , Idaho Falls, Idaho, USA). IDO-14576. •l.-m. 16, 1962.

148. \\ AUTOMATIC TIMER FOR DETERMINATIONS OF D20 CONCENTRATIONS IN WATER BY MEASUREMENTS ON DROPS FALLING IN O-FLUOROTOLUENE. Jason A.C., Lees A. (Ücpt.of Sclent, and Ind. Res., Aberdeen, Scotland, UK). J. Sci. Instr. 39, 1G2-4, Apr. 1962.

149. AN IMPROVED INFRA-RED METHOD OF MONITORING I1FAVY WATER. Bayly J. G., Booth R. J. , Stevens W. H. (Atomic Energy of Canada Ltd., Chalk River, Ont. CANADA). CRRP-1099. July 1962.

t (.lloquium on Heavy Water. Madrid, Dec. 1962. (JEN Madrid and EAES Paris). NP-13766:

150. THE "TWO-IMAGE" FLOAT METHOD AT TEMPERATURE BELOW 25°C. Otero J. L. , Gispert M. , Rojas J. L. NP-13766, p,155-66.

151. A DOUBLE SLOW NEUTRON SPECTROMETER. Bondarenko I. I. , Liforov V. G. , Nikolaev M. N. , Orlov V„ V., Parfenov V. A. , Semenov V.A. , Smirnov B. I. Turchin V. F. Inelastic Scattering of Neutrons in Solids and Liquids. Vol. I. 127-37. IAEA 1963. (In Russian)

152. A RAPID INFRARED METHOD FOR THE QUANTITATIVE

DETERMINATION OF D20-H20 MIXTURES. Fochler H.S. . (Standard Oil Co. of Ohio, Cleveland, USA). Appi. Spectry. 17, 105-6; 1963. : 64

153. USE OF MEASUREMENTS OF DEUTERIUM CONTENT IN THE STUDY OF METEOROLOGICAL AND GEOLOGICAL PHENOMENA, Roth E. J. Chirrt;Phys. GO, 339-50,1963. (In French)

154, DETERMINATION OF DEUTERIUM OXIDE BY THE FALLING DROP METHOD, Te-Chiu Chin,ChingV Lien Chang (Peking Univ. GHINA).Acta Chim. Sinica 29,266-76, 1963.

155. NON-DISPERSIVE INFRA.-RED ANALYSIS OF MIXTURES OF WATER AND HEAVY WATER. Bosselaar C. A. (Philips' Gloeüampenfabricken, Nijmegen, NETHERLANDS). Appi. Sci. Res. , Sect. B, 10, 137-56, 1963.

156. SPECTROCHEMICAL ANALYSIS OF H20-D20 MIXTURES BY MEANS OF BAND SPECTRA. Dunken H. , Mikkeleit W. Haucke G. Glas. Hem. Drus. (Beograd)28, No-8-9, 429-38, 1963. (NP-tr-1309, p.21-8.)

157, NEW MEDIUM FOR THE FALLING DROP METHOD OF ANALYSIS OF DILUTE HEAVY WATER. Te-Chiu Chin,Chircg-LienChang (Peking Univ. CHINA). Sci. Sinica, (Peking) 12, 147-8, Jan. 1963. (In English)

158. THE EXPERIMENTAL DETERMINATION OF THE SPECIFIC VO­ LUME OF HEAVY WATER AT HIGH TEMPERATURES AND PRES­ SURES. Rivkin S. L. , Akhundov T. S. At. Energy(USSR) 14, 581-2, June 1963. (In Russian)

159. DETERMINATION OF THE ABSOLUTE CONCENTRATIONS OF

I-I20-D20 MIXTURES USING THE INCREASE IN SENSITIVITY OF INFRARED ABSORPTION MEASUREMENTS. Ceccalcli M. (CBA,-CEN.'Saclay, FRANCE). CEA-R-2441. 1964. 65

160, INVESTIGATION OF TA-' ACCURACY OF THE DROP METHOD ANALYSIS OF HEAVY WATER HAVING A LOW CONCENTRA­ TION OF DEUTERIUM. Wei Chung-Wu, Liu Tien-Ch'iu. Ch'ing Hua Ta Hsueh Hsueh Paoli, 61-71, 1964.

161. INVESTIGATION OF THE ACCURACY OF DROP-METHOD ASSAY OF HEAVY WATER WITH A LOW CONCENTRATION OF DEUTERIUM. II. INVESTIGATION OF THE MOVEMENT OF LARGE DROPS. Lo Ch'i-Fang, Liu Tien-Ch'iu Xh'ing Hua Ta Hsueh Hsueh Pao 11, 73-80, 1964.

162. IMPROVEMENT OF THE OF THE FALL­ ING-DROP METHOD BY INCLINATION OF THE TUBE. Proksch E., Bildstein II. et al. (Osterreichische Studiengesellschaft i'llr Atomenergie G. m. b. II. Inst. für Chemie, Seibersdorf,. AUSTRIA). SGAE-CH-6/1964. (In German)

16 3. AN'INFRARED METHOD FOR DETERMINING VARIATIONS IN THE DEUTERIUM CONTENT OF NATURAL WATER. Bayly J. G., Stevens W. II., Thurston W. M. (Atomic Energy of Canada Ltd., Chalk River, Ont., CANADA). AECL-2076, Jan. 1964. (CRDC-1141)

1G4. DETERMINATION OF THE DEUTERIUM CONTENT OF A SAMPLE OF DEUTERIUM OXIDE BY THREE METHODS. Goldblatt M., Jones W,M. (Los Alamos Seien. Lab., N. Me's. USA) Anal. Chem. 36, 431-2, Feb. 19C4. (LADC-5874)

165. SEQUENTIAL ANALYSIS OF RADIO- IN HEAVY WATER MODERATOR. Holcomb II. P. (Du Pont de Nemours E. I. &Co.Savannah River Lab., Aiken, S.C. USA).DP-886. May 1964. * 66

166. CONTINUOUS INFRA-RED MEASUREMENT USING AN INTER­ FERENCE FILTER. ANALYSIS OF H20-D20 MIXTURES. Ceccal- di M., Coujon P. (Commissariat a l'En'ergie Atomique; Centre d'Etudes Nucleaires, Saclay, FRANCE). CEA-R-2440. May 1964.

157. ANNUAL REPORT OF DIVISION ANALYTICAL BRANCH FOR 19G3. Shank R.C.et al. (Phillips Petroleum Co. Atomic Energy Div. .Idaho Falls, Idaho, USA). IDO-14636. June 1964.

168. SPECTROPIIOTOMETRIC DETERMINATION OF HYDROGEN CONTENT IN HEAVY WATER. Gordon G. , Yamatera H. (Univ. of Maryland College Park; USA). Anal. Chem. 36, 1866-7, Aug. 1964.

169 RAPID DETERMINATION OF D20 CONTENT IN WATER USING A VAPOUR PRESSURE OSMOMETER. Lazzarini E. (CSN, E. Fermi, Politec., Milano, ITALY). Nature 204, 87 5-6, Nov. 28, 1964.

17°. HEAVY WATER. Anderson C. E., Ebeiihack.D. G. (Du Pont de Nemours E.I. & Co. Savannah River Plant, Aiken, S. C. USA). Analysis of Essential Nuclear Reactors Materials(C. J. Rodden Ed. 1964) (p. 629-57)

171. ANALYSIS OF HEAVY WATER IN CONCENTRATIONS NEAR TO(THAT IN) NATURAL WATER. III. Otero de la Gandara J.L., Gispert M., Rojas J. L. An. Real Soc; Espan. Fis. yQuim (Madrid) Ser.B,61, 1155-62, 1965. (In Spanish)

172. DETERMINATION OF THE ISOTOPIC COMPOSITION OF WATER BY FALLING-DROPLETS METHOD. Blaga L.", Blaga L., Chifu A. (Inst, of Atomic Phys. ,'Cluj, ROMANIA). Stud. Cer- cet. Fiz. 17, 765-7-3, 1965. 67

173. THE HANDLING OF DEUTERATED WATER AND SPECIFIC PROBLEMS OF DEUTERIUM ANALYSES. Chifu A. (Inst,of Atomic Phys., Cluj, ROMANIA). Acad. Repub. Pop. Rom. Stud. Cercet. Fix. 17, 574-610, 19G5. (In Rumanian)

174. A SIMPLE METHOD FOR DETERMINATION OF THE H/D RATIOS FROM FIELD ION-MASS SPECTRA OF 1I20/D20 OR NII3/ND3 MIXTURES.Richter E. L., Schmidt W. A. (Max-Planck- GeseUschaft, Berlin, GERMANY). Z. Naturforsch. 20a, 317-19, Feb. 1965. (In German)

175. GAS-CHROMATOGRAPHIC DETERMINATION OF THE DEUTE­ RIUM CONTENT (99 to 100 at. percent) IN HEAVY WATER. Jaeger K. (Gesellschaft i'uer Linde's Eismaschinen AG, Hoellriegels- kreuth, W. GERMANY). Kerntechnik 7, 221-4, May 1965. (In German)

176. APPLICATIONS OF ATOMIC ABSORPTION SPECTROSCOPY. Wheat'.J. A. (Du Pont de Nemours E.I. &Go. Savannah River Lab., Aiken S.C. USA).DP-980. July 1965.

177. STUDIES ON THE PRODUCTION OF HEAVY WATER. IH. ANALYTICAL CONTROL OF THE PRODUCTION INSTALLA­ TIONS. Olero"de;'la Ganclara J.L., Gispert M., Rojas de Diego J.L. (J-.E.N., Madrid, SPAIN). Energia Nu ci. (Madrid) 9, 248-55, July-Aug. 1965. (In Spanish)

173. AUTOMATED ANALYSES FOR THE CHARACTERIZATION OF HEAVY WATER MODERATOR. Gaddy R. H. (Du Pont de Nemours E. Ì. &Co. Savannah River Lab., Aiken, S. C. USA). Technicon'Analytical.Symposium Aug. 3, 1965. (CONF-650919-2)

179. A IIIGHSENSITTVÌTY HEAVY WATER LEAK DETECTOR. Bayly ' J. G. (Atomic. Kiuu-g.y or Cannda Ltd., Chalk River, Ont. CANADA). A KCl.-22!) I. OH..' I !)(i.r>.' 68

180. ANALYSIS OF DEUTERIUM" OXIDE-WATER MIXTURES AND MEASUREMENT OF THE DEUTERIUM ISOTOPE EF­ FECT ON THE ACID- EQUILIBRIUM OF N, N-DIME- THYLBENZYLAMINE USING NUCLEAR MAGNETIC RESON­ ANCE. Leyden D.E., Reilley C. N. (Univ. of N. C., Chapel Hill, USA). Anal. Chem. 37, 1333-8, Oct. 1965.

181. DETERMINATION OF THE D2O CONTENT IN WATER BY INFRARED SPECTROMETRY. Knezevic Z.V. (Boris Kidrich Inst, of Nucl. Sci., Belgrade, YUGOSLAVIA). Isotopenpraxis 1, 69-71, Nov. 1965.

18?. ISOTOPIC ANALYSIS OF HEAVY WATER BY INFRARED SPECTROMETRY. Rojas J. L. Energ. Nucl. (Madrid.)9, 453-8 , Nov.-Dec. 1965, (In Spanish)

183. AUTOMATIC SPECTROPHOTOMETRY ANALYSIS OF DEUTE­ RIUM OXIDE FOR VARIOUS PRESENT IN CONCENTRATIONS OF THE ORDER OF PARTS PER 109. Britt R. D. Jr. (E. I. Du Pont de Nemours & Co., Aiken, S. C. USA). Tech. Eau (Brussels) No. 238, 29-33, 1966. (In French)

184. THE DETERMINATION OF HEAVY WATER WITH THE UR-10 •. SPECTROPHOTOMETER. Kocent A-, ,Vasatkova J.(Cancur Res. Inst. /Brno, CSSR). Jena Rev., No/4, 228-9, 1966.

185. SIMPLE METHOD FOR DETERMINATION OF THE D2O CON­ CENTRATION. Cabicar J. , Einhorn F. fTechnische Hochschule, Pray ue, £sSR). Z. Naturforsch. 21a, 504, Apr. 1966. (In.German)

186. METHOD OF ISOTOPIC ANALYSIS OF OXYGEN IN MICROQUANTI- TIES OF WATER. DETERMINATION'OF. EQUILIBRIUM DISTRIBU­ 18 TION COEFFICIENTS OF 0 BETWEEN H20 AND CO2 AND D20 AND CO2. Majzoub M. (CEN Saclay, FRANCE). J. Chem. Phys. 63, 563-8, Apr. 1966. (In French) ri 9,

1'87. ANALYTICAL PROCEDURES (1966) FOR THE HEAVY WATER AND HELIUM SYSTEMS OF THE NRX AND NRU REACTORS. PART I, II, AND III. (Atomic Energy of Canada Ltd. , Chalk River, Ont. CANADA). AECL-2596. June 1966.

188. ISOTOPE DILUTION ANALYSIS WITH STABLE ISOTOPES. PART I. EXPERIENCES IN DETERMINATION OF WATER CONTENT BY ISOTOPE DILUTION ANALYSIS WITH D20. Krumbiegel P. , Huebner H., Rolle W. (Inst, fuer Stabile Isotope, Leipzig. Deutschen Akad. der Wissenschaften, Berlin, GERMANY). Isotopenpraxis 2, 220-4, June 19G6. (In German)

189. INFRARED DETERMINATION OF RESIDUAL HYDROGEN IN DE-UTERATED INORGANIC COMPOUNDS. Whateley T. L., Whittem R.N. (Australian-Atomic Energy Commission Res. Establ., Lucas Heights,AUSTRALIA). AAEC-TM-326. May 1966.

190. DETERMINATION OF DEUTERIUM ION CONCENTRATION IN DILUTE UNBUFFERED DEUTERIUM OXIDE SOLUTIONS. Bau­ mann E.W. (Du Pont de Nemours E.I. &Co., Aiken, S. C. USA). Anal. Chem. 38, 1255-7, Aug. 1966.

191. USE OF DIMETHYL SULPHOXIDE AS A SOLVENT FOR THE RAPID ISOTOPIC ANALYSIS'OF WATER BY INFRARED SPEC­ TROMETRY. Mahadevan E.'G. (Columbia Univ., New York, USA). Analyst, 92, 717-8, 1967. ,

192; ANALYSIS OF HEAVY WATER BY THE FLOAT METHOD OVER THE ENTIRE CONCENTRATION RANGE. Gispert M., Rojas J. L., Otero de la Gandara J. L. (J. E.N., Madrid, SPAIN). An.Real.Soc.Espan.Fis.y Quim. (Madrid) Sor. B, 63,479-84, •Apr. 1967. (In Spanish) 70

193. FUNDAMENTAL CALCULATION OF ACCURACY IN HEAVY WATER STANDARDS..Rowland P. R. (Atomic Energy Establ., Winfrith, Eng. UK). AEEW-M-745. May 1967.

194.PHOTOMETRIC DETERMINATION OF THE 1SOTOPIC CON­ TENT OF HEAVY WATER. Feuerstein II. (Kernforschungszentrum, Karlsruhe, W. GERMANY). KFK-570. May 1067. (In German)

195 WATER QUALITY CONTROL IN THE HFBR. Protter S.R. (Brook- haven Nat. Lab. , Upton, N. Y. USA). P.N.L- II 56.1. June 196 7.

196. METHOD FOR THE DETERMINATION OF OXYGEN ISOTOPIC RATIOS IN HEAVY WATER. Robinson B. K. , Symons W. J. (Atomic Energy Establ. , Winfrith, UK). AEEW-R-550. Sept. 1967.

197. RAPID WIDE-RANGE DETERMINATION OF HEAVY WATER BY CUT-OFF PYCONOMETER. Rowland P. R. t Wright C. R., Knott A.R. AAEW-M746.19G7.

198. MtCllOCHEMICAL ANALYSIS SECTION: SUMMARY OF AC­ TIVITIES, JULY 196G-.IUN13 1937. Taylor J. K. (Nat. Bur. of Stand. , Washington, D.C. USA). NBS-TN-425. Out. 1967.

199. DETERMINATION OF WATER-HEAVY WATER MIXTURES BY 19F NUCLEAR MAGNETIC RESONANCE. Devcrell C., Schaumburg K. (Nat. Res. Council, Ottawa, CANADA). Anal. Cliem. •39, 1879-80, Dec. 1967.

200. FUNDAMENTAL PROBLEMS OF HEAVY WATER'DOSIMETRY IN NUCLEAR I IE ACTORS. David L., Tomaskova LÙUstav Jadcrncho Vy/Jumui, Prague, CZECHOSLOVAKIA). Jad. Energ.14, 11 -20, Jan. 1968. (In Czech) 71

201. STANDARDIZATION OF THE DEUTERIUM CONTENT OF HEAVY WATER. Baertschi P., Rosatzin H. (Eidgenössisches Inst, fuer Reaktorforschung, Wuerelingen,SWITZERLAND). Oct. 1968. (In German)

2 02. STANDARDS FOR A PRATICAL SCALE OF pD IN HEAVY WATER. Paabo M., Bates R. G. (NBS. Washington, D. C. USA). Anal. Chem. 41, 283-5, Feb. 1969.

2 03. DENSIMETRIC ISOTOPIC ANALYSIS OF LIGHT AND HEAVY WATER BY USE OF OXYGEN EXCHANGE BETWEEN DIOXIDE AND WATER. Staschewski D. (Kernforschungszentrum Karlsruhe, GERMANY). Ber. Bunsenges, Phys. Chem. 73, No. 1, 59-65. Mar. 1969. (In German)

2J4. INTERFEROMETRIC DETERMINATION OF SMALL AMOUNTS OF D20 AND H20. Mercea J. (Inst. Atomphysik, Cluj, ROMANIA). Chem. - Ing. -Tech. 41, 508-10, Apr. 1969. (In German)

205. A CALORIMETER APPARATUS TO MEASURE THE ENTIIAL- PIIY DIFFERENCE OF HEAVY WATER. Nowak E. S., Chan. J. (Univ. of West.Ont., London, CANADA). J. Heat Transfer 91, 235-40, May 19S9.

206. INFRARED ANALYSIS OF HEAVY WATER-WATER MIXTURES OF INTERMEDIATE (3 TO 97 PERCENT) CONCENTRATION. Kimbrough D. Jr., Askins R. W. (Georgia Inst, of Tech., Atlanta, USA). A;ud, Chem. 41, 1147-8, July 1969.

207. DEUTERIUM ANALYSIS BY PHOTONEUTRON DETECTION. George K. D. , Kramer H. (Sterling Forest Res. Center, Tuxedo, N.Y.USA).Nucl. Appi.Technol. 7, 385-8, Oct. 1969. 72

208. IN-LINE D20 ANALYSIS. Stutheit J. S., Rampey W. P. (Du Pont de Nemours E. I. & Co., Aiken, S. C. USA). Nucl. Instrum. Methods 75,43-4,1969.

209, CHEMISTRY AND MATERIALS DIVISION; Progr. Rep. Oct. 1 - Dec. 31, 1969. (AECL, CNRL, Chalk River,"Ont. CANADA).

210. DETERMINATION OF DEUTERIUM IN HEAVY WATER BY SECON­ DARY DEUTERON ACTIVATION. Pretorius R., Wainerdi E. R. (Texas A and M Univ. College Station, USA).Talanta 17, 51 -9, Jan. 1970.

211. A COMPARISON OF ANALYSES OF HIGH-PERCENTAGE HEAVY WATER SAMPLES BY DENSITY MEASUREMENTS AND BY IN­ FRARED SPECTROSCOPY. Moravec J.,Sara V., Vagner J,, Kysela J. (Inst. Nucl. Res. of CSAV-Re2-CSSR) Jaderna energie 17, No. 1,28-30, 1971; f1

IV ' HEAVY WATER PRODUCTION 75

REVIEWS OF PRODUCTION PROCESSES

THE NEED OF ADEGUATE PROVISION FOR THE QUANTITY PRODUCTION OF DEUTERIUM WATER. Washburn E. W. Science 78, 555-6,IÖ33.

THE MANUFACTURE OF DEUTERIUM AND ITS COMPOUNDS. Webb W.A. Ind. Eng.Chem. News Ed. 12, 63, 1934.

COMMERCIAL PRODUCTION OF HEAVY WATER. An Edito­ rial. Nature 133, G04, 1934.

THE PREPARATION OF HEAVY WATER. Schachert F. Priroda 28, 226-34,1935.

THE ELECTROLYTIC SEPARATION OF HYDROGEN AND DEUTERIUM AND THE CATALYZED EXCHANGE REACTION HD+H2O-H2+HDO. Butler J .'A. V. Z. Elektrochem. 44, 55-G2, 1938.

EXCHANGE REACTIONS BETWEEN LIGHT AND HEAVY HYDROGEN. A, Review. Ingolfi O.K., Wilson C, L. Z. Elcktro- •chem. 44, 62-72, 1938. 76

INDUSTRIAL MANUFACTURE AND APPI-ICATIONS OF HEAVY WATER AND OF DEUTE.RIUM DERIVATES. A Review. Darmois E. Tccli. Ind. Chi-n. ;\jo. 284 bis, 16-8, 1939.

(On DuaL Temperature Exchange).Edmonds S. M., ßix-baum N. Ind. Eng. Gliom. Anal. Ed. 12, GO, 1940.

(On Dual Temperature Process). Shaw A.J. Ind. Eng. Chem. Anal. Ed. 12, 668, 1940.

SEPARATION OF ISOTOPES BY CHEMICAL MEANS. Urey II. C. J. Wash. Acad. Sci. 30,277-94, 1940.

A COMPARISON OF THE METHODS OF PREPARING HEAVY WATER. Brodskii A. I. Zhur. Priklad Khim. 13, 6 70-5, 1940. (In Russian)

ON PRODUCTION OF HEAVY WATER. Farkas A. SAM Re­ port. A-84. Jan. 11, 1942.

(On Dual Temperature Process). Kimball G. E., Stockmayer W.U. Col. Univ. Rep. A-144. Apr. 7, 1942.

(On Dual Temperature Processes).Spevack J. S. Col. Univ. Rep. A-393.DCC. 3, 1942.

(On Dual Temperature Process). Kimball G. E., Stockmayer W. II. Col. Univ. Rep. 100XR-1G57. Oct. 14, 1942. 77

IG. (On Dual Temperature Processes). Spevack J. S. Col. Univ. Monthly Report. Nov. 11, 1942.

17. (ON Deuterium Separation by Means or Exchange Reactions). Mayer II. Col. Univ. Memo. Nov. 21 and 26, 1942.

18. (On Dual Temperature Process). Kirshcnbaum I. Col. Univ. Thesis. 1942.

19. (On D2O Production). Webb G. M.A Letter to J. E. Ahlberg Col. Univ. Sept. 3, 1942.

2 0. REPORT ON PRELIMINARY ANALYSIS OF THE EXCHANGE PLANT. Chopin J. H., Urey U.C. SAM Report 3R-23 (A-501) Jan. 5, 1943.

21. (On Dual Temperature Processes). Brown F. B. Col. Univ. Rep, A-566. Mar. 12, 1943.

22. (On Dual Temperature Processes). Brown F. B. Col. Univ. Rep.A-591. Apr. 14, 1943.

23. (On D20 Production). Ahlbcrg J. E. , Blair T. S. , Bcthuno A. J. de, Koracli JVI., Urban J., Vona J. Col. Univ. Rep. A-1214. Nov. 5, 1943.

24. (On Separation Processes). Cohen K., Mayer H. L. SAM Memo. 4M-10. Jan. 2, 1943.

25. OPTIMUM DESIGN OF CATALYTIC TOWERS. Mayer H. L. SAM Rep. 4R-34. Mar. 12, 1943. 78

THE PHENOMENOLOGY OF TWO PROCEDURES FOR SE­ PARATING ISOTOPES. Klemm. A. Z. Naturforsch. 1,252-7, 194G.

SURVEY ON HEAVY WATER AND ITS PRODUCTION. Silvestri M. CISE-2.1946. (In Italian)

MULTISTAGE SEPARATION PROCESSES. Benedict M. Am. Inst.Chcm. Engrs.43, No. 2,41-60, 1947.

CALCULATION OF EQUILIBRIUM CONSTANTS FOR ISO- TOPIC EXCHANGE REACTIONS. Bigeleisen J., Mayer M. G. J. Chem. Phys. 15, 261-7, 1947.

SEPARATION OF ISOTOPES BY THERMAL DIFFUSION. A Review. Wolczek O. Widomosci- Chem. 7/9, 1, 21-5, 1947. (In Polish)

THE DUAL TEMPERATURE PROCESS FOR ISOTOPE SE­ PARATION. MDDC-89. ADD, 1, 547.Deci. Feb. 26, 1947.

CHEMICAL METHODS OF ISOTOPE SEPARATION. Reid A. F. U. S. Naval Med. Bull. SuppL205-8, 1948.

PRELIMINARY STUDY OF POSSIBLE PROCESS TO PREPARE HEAVY WATER. Perpérot II. Mem. Poudres 32,429-36, 1950.

REVIEW OF THE PRESENT STATUS OF ISOTOPIC SEPARA­ TION METHODS. Grotli W. (Bunsenges. fUr physik. Chemie, GERMANY).ZtGchr.Elektfochem. 54, 5-12, 1950. (In German)

LABORATORY STUDIES FOR SEPARATION PROCESSES.. Gidinoff M. L., Joris G. G., Taylor E. H., Taylor H. S., Urey H.C. NNES4II-4D. 1951. 79

3G. CHEMICAL EXCHANGE REACTIONS FOR THE PRODUCTION OF HEAVY WATER. Bigclcisen J. et al. BNL-107. 1951.

37. DEUTERIUM CONCENTRATION BY CHEMICAL EXCHANGE. Bigeleisen J. et al. BNL-118. 1951.

38 SEPARATION OF STABLE ISOTOPES. THE ROLE OF ENGI­ NEERING IN NUCLEAR ENERGY DEVELOPMENT. Benedict M. 3rd Ann. Oak Ridge Summer Symp. Aug. 27 to Sept. 7, 1951. TlD-5031.Dec.lD51.

HEAVY WATER. Brim J. Tidsskr. Kjemi, Borgvson. Mot. 13, 156-G1,1953.

HEAVY WATER. Cerrai E.Energia Nucleare (Milan) No. 5, 96 9G-103, Dec.20, 1952.

41. STATUS OF HEAVY WATER PROCESSES. Thayer V. R. TID-2008. Mar. 1953. (Reactor Sci.Technol, 3,(1), 9-22)

42. STATUS OF HEAVY WATER PROCESSES.Thayer V.R. (Du Pont de Nemours E. I. &Co, Atomic Energy Div. , Wil- minghton.Del. USA). TID-2504. (Del. )(Suppl. 1) (DPW-G6G2. Del.)

43. HEAVY WATER. A REVIEW OF PROCESSES AND PLANTS FOR LARGE-SCALE PRODUCTION. Selak P.J./Finke J. Chem. Eng. Progr. 50, 221-9, May 1954.

44. ON PROPERTIES AND PREPARATION OF HEAVY WATER. Baertschi P., Kuhn W. Techn. Rundschau 52, 1954. (In German) 80

ON DEUTERIUM DISTRIBUTION IN HYDROGEN ISOTOPIC EXCHANGE. Varshavskii Ya. M., Vaisberg S. E. ZhürvFiz. Khim.-22, No. 3, 52 3-32, Mar. 1955.

REPORT FROM GENEVA. REACTOR MATERIALS. Nuc leonics 13,No. 9,G4-71.Scpt. 1955.

SURVEY OF HEAVY WATER PRODUCTION PROCESSES. Benedict M. 8, P/819. (USA). 1st Geneva Coni". 1955.

SOME ASPECTS OF THE HEAVY WATER PREPARATION DESIGNED FOR A SWITZERLAND REACTOR, dc Haller P. P/923. ( SWITZERLAND). 1st Geneva Conf. 1955. (Abstract only)

GENERAL ASPECTS ON INDUSTRIAL SEPARATION OF ISOTOPES. Gueron J. CEA-Saclay Rep. 456. 1955.

THE THEORY OF ISOTOPE SEPARATION BY COUNTER- CURRENT CHEMICAL EXCHANGE. Marcus W.C. De, Halle E. von. K-1190. Jan. 19,1955.

DEUTERIUM SEPARATION STTJDYProgrcss Report No. 2. Drews W. P. (Esso Res. and Eng. Co., Linden, N. J. USA). NYO-G085.Aug. 1, 1955. Deci. Mar. 4, 1957.

DEUTERIUM SEPARATION STUDY. Progress Report No. 4. (Final Report on HEAVY WATER MANUFACTURE SURVEY). Barr. F. T., Drews W. P. (Esso Res. and Eng. Co., Linden, N. J. USA). NYO-7523. Oct. 14, 1955. Deci. Mar. 25, 1957. (SOA-188) 81

53. PRODUCTION OF HEAVY WATER. NATIONAL NUCLEAR ENERGY SERIES, DIVISION III, VOLUME 4F. G. M. Murphy, I-I. C. Urey, I. Kirshenbaum, eds. New York, McGraw-Hill Book Co., Inc. 1955. (NNES-III-4F)

54, THE PRODUCTION OF HEAVY WATER. Becker E. W. Angew. Chem. 68, 6-13,1956. (In German)(AERE-Lib/Transr734; AEC-tr-2808)

55. OPTIMUM CONDITIONS FOR THE ENRICHMENT OF HEAVY WATER IN HOT-COLD COLUMNS. I. THE SINGLE HOT-COLD SYSTEM. Bier K. Chem. Ing. Tech. 28, 265-88, 1956. (In Ger­ man) (AEC-tr-2887)

56. PRODUCTION OF HEAVY WATER. Sojka, J. Chem. Prumysl. 6, No. 4, 170-2, 1956, (In Czech)

57. THE ANALOGY BETWEEN ISOTOPE 'XCHANGE IN COUNTER- CURRENT COLUMNS AND ADSORPTION PROCESSES. Rozen A. M. Doklady Akad/Nauk SSSR 108, 122,1956. (In Russian)

58. HEAVY WATER PRODUCTION. D2O BEHAVIOUR IN REACTORS. Roth E. Chim. &Ind., Suppl. Energie Nucléaire 75, No. 2,42-52, 1956.

59. ISOTOPIC EFFECT IN THE LIQUID-VAPOR EQUILIBRIUM OF BINARY SYSTEMS CONTAINING DEUTERIUM COMPOUNDS. Rabinovich I. B., Nikolaev P. N., Gochaliev Z. E., Tretyakova N. N. ( Lobachevskii' Gorkii State Univ. USSR). Doklady Akad. Nauk SSSR, 110, 241-4, Sept. 11, 1956. (InRussian) 82

PREPARATION OF HEAVY WATER. Fellner-Felldeg H. Gas und Wasserfach 97, No. 24, 1017-9, 1956. (In German)

PILOT-PLANT-SCALE MANUFACTURE OF HEAVY WATER.' Cziko K» , Fodor P. Magyar Tudomanyos Akad.Központi Fiz. Kulat(!) Intezetcnek Közlcmenyei 4, 68-75, 195G.(In Hungarian)

HYDROGEN ISOTOPE EXCHANGE. Augood D. R. Nature 178, 754-5,1956.

HEAVY WATER PRODUCTION METHODS. Nucl.'Power 1, 9-15,May 195G.

HEAVY WATER PROJECT. II. Brown C.J. July 1956.

HEAVY WATER PRODUCTION. Benedict M. (MIT, Cambridge, Mass. USA). NP-6975. Lecture delivered at Reykjavik, Iceland. Sept.G, 195G.

Proceedings of the Scientific Congress, Nuclear Sessions, Rome, July 195G.CNRN 1956: PROBLEMS CONNECTED WITH THE PRODUCTION OF HEAVY WATER IN ITALY. Silvestri M.p. 315-34; (In Italian)

PROBLEMS CONNECTED WITH THE PRODUCTION OF HEAVY WATER IN THE UNITED KINGDOM. Pratt H.R.C, p.315-34;

PROBLEMS CONNECTED WITH THE PRODUCTION OF HEAVY WATER IN FRANCE. Roth E. p. 335-52. (In French) 83

69. SURVEY OF HEAVY WATER PRODUCTION PROCESSES. Benedict. M. (MIT, Cambridge, Mass. USA). Progress in Nuclear Energy. Series IV. Technology and Engineering. R. I-Iusrt, S. McLain eds. New York, McGraw-Hill Book Co. , Inc., 195G. (p.3-56)

70. HEAVY WATER IN GERMANY. Atomics 8, No. 11, 428-30, Nov. 1957.

71. THE PREPARATION OF GRAPHITE AND HEAVY WATER. Beckmann R. Atompraxis 3, (2), 60, 1957.

72. METHODS OF OBTAINING HEAVY WATER. Otero de la Gandara J. L. Energia Nuclear (Madrid) 1, No. 2,45-58, Apr.-June 1957. (In Spanish)

73. SPECIAL MATERIALS FOR NUCLEAR INDUSTRY. Cerrai E. Energia Nucleare (Milan) Suppl.Vol. 3, 82-92, 1957.

74. NEW RESEARCH DEVELOPMENTS FOR INDUSTRIAL SCALE ISOTOPE SEPARATION. Villani S. Energia Nucleare (Milan) 4,187-95,1957.

75. METHODS OF PRODUCTION OF HEAVY WATER. Nuklconika 2,No.l, 111-30, 1957. (In Polish) 84

ISOTOPE SEPARATION BY MULTISTAGE METHODS. Johns T.F. Progr. Nucl. Phys.6, 1-25, 1957.

THE PRODUCTION OF DEUTERIUM OXIDE AND THE DETERMINATION OF ITS DENSITY. Shatenstein A. I., Yakimenko L. M., Kalinachonko V. R., Yakovleva E. A.. Zhur. Neorg. Khim. 2, 985-94, 1957. (In-Russian) (CEA-R-367; JPRS-2499)

AN INVESTIGATION OF TECHNIQUES FOR THE SEPARATION OF HYDROGEN AND DEUTERIUM. PART I.ZONE REFINING OF MIXTURES OF ORDINARY AND HEAVY WATER. PART II. THE REACTION OF IRON WITH MIXTURES OF ORDINARY AND HEAVY WATER. PART III. GAS CHROMATOGRAPHY WITH HYDROGEN AND DEUTERIUM SAMPLES. Thomas C. O. Thesis, Univ. of Tennessee, Knoxvillo, 1957.

Proceedings of the Int. Symp. on Isotopie Separation, Amster­ dam, Apr. 1957. North Holland Pubi. Co. Amsterdam 1958.

EVALUATION OF ISOTOPE SEPARATION PROCESSES. Garret G. A. ,Shacter J. (p. 17-32);

THE SIGNIFICANCE OF THE PRODUCT AND SUM RULES TO ISOTOPE FRACTIONATION PROCESSES. Bigeleisen.J. (BNL, Dept. Chem., Upton L. I., N. Y. USA), p. 121-57;

ENRICHMENT OF ISOTOPES BY THE DIFFERENCE IN RATES OF ISOTOPIC REACTIONS. Bernstein R. B. (Univ. Mich., Ann Arbor, USA), p. 313-15;

ISOTOPE SEPARATION BY FRACTIONAL DISTILLATION. London H.. p. 319. 85

METHODS OF HEAVY WATER PRODUCTION. Stouls L. , Enex-gie Nucléaire 2,4, 397-407, 1958.

CHEMICAL EXCHANGE. Augood D. R. Ind. Chem. 34, No. 404, 533, 1958.

PRODUCTION OF HEAVY WATER. White A. S. Industr. Chemist. 34, No. 406, G71,1958.

PRODUCTION OF HEAVY WATER IN FRANCE. Roth E. ; Stouls L. ,Dirian G. , Lazax-d B. , Nie! G. (CEA, Paris). 4, P/1261. (FRANCE). 2nd Geneva Coni". 1958.

METHODS FOR THE SEPARATION OF STABLE ISOTOPES. Blanc D. A cero y onci-gia, Barcelona IG, 92, 54-6 0, 1959. (In Spanish)

INDUSTRIAL PRODUCTION OF HEAVY WATER. Sakodynskii K. I, Atomnaya Encrg. 6, 14-20, Jan. 1959. (In Russian)

INDUSTRIAL PRODUCTION OF HEAVY WATER. Malkov M. P. Atomnaya Energ. 7, 101-9, Aug. 1959. (In Russian)

PRODUCTION OF HEAVY WATER. Bebbington W., Thayer V. R. Chcm. Eng. Progr. 55, No. 9, 70-78, Sept. 1959.

OPTIMUM CONDITIONS FOR THE ENRICHMENT OF HEAVY WATER IN HOT-COLD COLUMNS. II. THE ENRICHING SYSTEM, THE STRIPPING SYSTEM AND THE TRANSFER COLUMN.'Bier K. Chem. Ing. Tech. 31, 22-30, 1959.'(In Ger­ man) (NP-tr-400) K6

PERFORMANCE CHARACTERISTICS OF DEUTERIUM EXCHANGE PROCESSES. Dietze M., Pilz S.' Chem.Tech. (Berlin) 11,544-6,1959.

PRODUCTION OF HEAVY WATER.'Santos Maccdo C. M. Eng. Nuclear (Port. ), No. 5, 80-3,1959.'(CEA-tr-X-369)

OPTIMUM CONDITIONS FOR THE DUAL-TEMPERATURE EXCHANGE PROCESS OF PRODUCING HEAVY WATER. Mizushina T., Takainatsu T, , Yoshida A., Nakanishi A., Kono M., Sayama H. Kagaku Kogaku 23, 71-80,1959.'(In Japanese)

INDUSTRIAL METHODS FOR THE PRODUCTION OP HEAVY WATER. Zhavoronkov N. M., Sakodynskii K. I. Khiiri; Prom. No. 3, 35-48, 1959. (In Russian) ( JPRS-50G4)

HEAVY WATER PRODUCTION METHODS. Varshavskti Ya. M., Vaisberg S. E. Khim.Nauka i Prom. 4, 498-509, 1959. (In Russian) (JPRS-12G74)

PREPARATION OF HEAVY WATER. K'o-shueh- Hsin-wen No. 39, 10-12, Dec. 7, 1959. (JPRS-7462 p. 13-23)

PRODUCTION OF HEAVY WATER. Hannerz K. Tekn. Tidskr. 89, No. 7, 151-6, 1959.

HEAVY WATER PRODUCTION IN ROMANIA. Mercea V., Peculea M. , Grecu E. Rep.IFA (Bucharest) A4, 1959.

HEAVY WATER. Kllchler L. (Farbwerke Hoechst A. G. Frankfurt am Main. W. GERMANY). Atom. u. Strom 6,35-40, Apr. 1960. (In German)

HEAVY WATER PRODUCTION. Roth E. Bull. Inform. Sci. et Tech. (Paris) No. 40, 2-3, May 1960. (In French) 87

102, METHODS OF THE PRODUCTION OF HEAVY WATER. Giona A. R. Ingegnere (Milan) 34, No. 3, 217-23, 1960.

103. TWO-TEMPERATURE METHODS OF PRODUCING HEAVY WATER. Sakodynskii K. I., Zhavoronkov N. M. (Karpov Inst, of Physic and Chemistry, Aoadcmyof Sciences, USSR). Uspekhi Khini. 29,112-37, Sept. 19G0. (In Russian)

Proc.of the Joint Symposium on Instrumentation & Computa­ tion in Process Development and Plant Design, London, ICE, 19G0. 104. DESIGN METHODS FOR DUAL-TEMPERATURE CHEMICAL EXCHANGE PROCESSES FOR PRODUCTION OF DEUTERIUM. Lyon C. J. (AERE, Harwell, Berks. UK).

105. THE SEPARATION AND THE ROLE OF ISOTOPES. Hellmuth D. VDI Nachr. 15, 50, 6,19G1.

106. DESIGN CONSIDERATIONS FOR A REACTOR FOR CHE MICAL EXCHANGE METHOD OF PRODUCING HEAVY WATER. Kalyanasundaram C. V., Kumar R., Datta R. L. Chem. Process. Design, Symp. Bangalore India 32-5, 19Gl.(Publ. 19G3)

107. INDUSTRIAL MANUFACTURE OF HEAVY WATER. Zhavoronkov N. M., Sakodynskii K. I. (Karpov Inst, of Physic and Chemistry, Moscow, USSR). Kernenergie 4, No. 12, 893-904, Dec. 19G1. (In German) (JPRS-42164)

108. APPLICATION OF CHEMICAL EXCHANGE METHODS TO 1SOTOPIC SEPARATIONS. Drury J. S. (ORNL) Progr. in Nucl. Energy, Ser.. IV, 4, 308-48, 1961. H8

109. THEORY OF ISOTOPE SEFARATIONIN COLUMNS. llozon A.M. Atomizdat, Moscow 19G0. (In Russian)

110. GENERALITIES ON THE OF THE PROCESSES FOR HEAVY WATER PRODUCTION. Dirian G. Bull. Inform. Sci. et Tech. (Paris) No. 40, 24-35, May 1960. (In French)

111. SEPARATION AND USE OF STABLE ISOTOPES. I. SEPARA­ TION OF STABLE ISOTOPES BY CHEMICAL EXCHANGE. Wetzel K., Krctzchmann G. Chem. Tech. 12, 26 3-6, 196 0. (In German)

112. PRODUCTION OF HEAVY WATER FOR REACTORS. Bolhar- Nordonkampf F. Electroteeh. u. Maschinenbau, 77, 387-90, Sept. 1, 19C0. (In Gentian)

113. HEAVY WATER PRODUCTION. Favre I. Energie nucléaire 2,108,1960.

114. PRODUCTION OF HEAVY WATER IN THE . Walker P. T. Ind. Chemist 36, 373-6, 1960.

115. HEAVY WATER PRODUCTION IN THE .U. S.A. Thayer .V. Nucl. Power 5, No. 46, lOOrll, 1960.

11G. PRACTICAL USABLE METHODS FOR ISOTOPE SEPARATION. Walker W. Physik. BlHtter 16,61-72, 19G0. 89

11Y. CONTROL OF THE DUAL TEMPERATURE EXCHANGE PROCESS FOR THE MANUFACTURE OF HEAVY WATER. Morris J. "W., Scotten W. C. Chem. Eng. Progr. , Symp. Ser. 58(39), 26-38, 19G2.

118. STABLE ISOTOPE SEPARATION. II. PRODUCTION PROCES­ SES. Linderstroem-Lang C. U, (Atomenergikommissiones Forsogsanlaeg, Riso, DENMARK). Dansk. Kemi 43, 165-71, 1962. (In Danish)

119. SEPARATION OF HEAVY WATER BY ISOTOPIC EXCHANGE. Roth E. Energia Nucleare 4, 332-42,1962.

120. THE SEPARATION OF HEAVY WATER. Brancker A. V. Ind. Chem. 38, 14-22,1962.

121. APPLICATION OF CHEMICAL EXCHANGE METHODS TO ISOTOPE SEPARATION.DruryJ.S. J. Nucl. Energy Pt. B., Reactor Technol. 3, 120-GO, 1962.

\12.. DEVELOPMENT DIRECTIONS IN THE PERFECTION OF METHODS FOR THE SEPARATION OF STABLE ISOTOPES. Zhavoronkov N. M., Sakodynskii K.I. Kernenergie 5,211-9, 1962. (In German)

123. HEAVY WATER PRODUCTION. Becker E. W.A. (Inst. fUr Kernverfahrenstechnik, Karlsruhe, W. GERMANY). STI/PUB/ 15/21. IAEA, Mar. 1962.

124. ISOTOPE SEPARATION BY MEANS OF ION TRANSPORT, DISTILLATION AND THERMAL DIFFUSION. Clusius K; • Cheni. Ing. Tcchn. 35, 422-8, 1963. 90

125. THE HYDROGEN ELEMENT AND THE PREPARATION OF HEAVY WATER. Jcnn J. T., Akar P. Energie Nucl. 5, 98-114, Mar. rApr. 1963. (In French)

126.. THE PRESENT STATE AND THE PROBLEMS OF HEAVY WATER MANUFACTURING. Kurihara Y. Genshiryoku Kogyo 9, No. 8, 57-62;Aug. 1963. (In Japanese)

127. THE PRESENT STATE AND PROBLEMS OF TECHNOLOGY FOR HEAVY WATER PRODUCTION. (PART)2. Kurihara Y. Genshiryoku Kogyo 9, No. 9, 17-20, Sept. 196 3. (In Japanese)

128. SOME FEATURES OF THE DUAL TEMPERATURE METHOD OF SEPARATION OF HYDROGEN ISOTOPES. Vaisberg S. E., Varshavskii Ya. M. (Inst, of Radiation Physics, Chemistry and Biology, Academy of Sciences, USSR). Zhur. Fiz. Khim. 6 0, 115-23, Janr Feb. 1963. (In Russian)

129, SEPARATION OF ISOTOPES, ANNUAL PROGRESS REPORT. Taylor T.I. TID-19592, Sept. 1, 19G3.

130. ENRICHMENT AND USE OF STABLE ISOTOPES. Groth W. 2nd Wiss. Tag. Deut. Atomforums Munich 1963. (p. 239-51; pubi. 19G4)

131. ISOTOPE SEPARATION BY DISTILLATION AND CHEMICAL EXCHANGE. Murrenhoff 'A. P. Kerntechnik 6(12), 554-7, 1964.

132. INDUSTRIAL PRODUCTION OF DEUTERIUM. Murrenhoff A.P. 'Kerntechnik 6(12), 558-60, 1964.

133. PRODUCTION OF DEUTERIUM AND OF HEAVY WATER BY ISOTOPIC EXCHANGE. Meriel Y. Sci. progr. Nat. (Paris) No. 3352,305-10, 1964. 91

3rd International Conference on Peaceful Uses of Atomic Energy. Geneva 1Ì3G4:

134. STUDY OF THE PRODUCTION OF HEAVY WATER IN FRANCE. Lefrancois II., Lerat J.'M., Roth E. P/91. (FRANCE). 3rd Geneva Conf. 1964. (CEA-R-2G46)

135. STUDIES ON THE PRODUCTION OF HEAVY WATER AT J. E. N. P/49G. Alvarez J., Gispert M. , Maria A. Otero J. L., Rojas J. L. 3rd UN Geneva Conf. 1964.

136. . PRODUCTION OF HEAVY WATER. Roth E., Rostaing M. Genie Atomiquc Vol. V. 1965. (p. 317-49)

137. CALCULATIONS OF THE DUAL TEMPERATURE SEPARA­ TION OF ISOTOPES BY EFFECTIVE CONCENTRATION METHOD. Filippov G. G. ,Sakodynskii K. I., Zelvenskii Ya. D. Khim. Prom. 1, 10-14, 1965. (In Russian)

138. A REVIEW OF HEAVY WATER PRODUCTION PROCESSES. Rae H.K. (AECL, Chalk River, Ont. CANADA). AECL-2503, 1965.

139. PRODUCTION OF HEAVY WATER. Ice C. PI. Research Materials Coordination and Planning Meeting, Nov. 14-J 5, 19G3. ORNL-TM-1047. 1965. 92

j.40. METHODS OF SEPARATING STABLE ISOTOPES. I. -VI. Vasari! Gli. MLM-129G. Sept. 1965. (English translation)

141. MULTISTAGE SEPARATION PROCESSES. I. IDEAL AND SQUARED OFF CASCADES. II. THERMODYNAMIC EF­ FICIENCY OF SEPARATION PROCESSES. Pratt I-I.' R. Univ. of Madras 1966.Indian Chem. Eng. 8, 6 0-82, 19GG.

142. CHEMICAL EXCHANGE PROCESSES FOR HEAVY WATER. Rao IF. K. AECL-2555. 19G6.

143. INFORMATION ON HEAVY WATER PRODUCTION. Pcculea M., Sampalcanu L. IFA Report, Bucharest, Jan. 19GG. (Unpublished)

144. THE PRODUCTION AND THE APPLICATIONS OF STABLE ISOTOPES. Vasaru Gli. IFA Report, Bucharest, 15-3G, 19GG.

145. A REVIEW OF THE SEPARATION OF STABLE ISOTOPES. Gverdisiteli I. G. Abh. Deut. Akad. Wiss. Berlin, Kl. Math. Phys. Tech. 1, 79-85, 19G7.

146. THE HEAVY WATER PRODUCTION IN CANADA. Energie Nuclóairc 9, 343, 1967.

147. ADVANCES IN THE FIELD OF SEPARATING STABLE ISOTOPES BY CHEMICAL EXCHANGE. Ciric M. ,Krell E., Kulicke P. , Missbach D., Mühle K. ,Schuetze H., Stiehl G., Thiel S., Weise G., Wetzel K. Isotopenpraxis 3,21-6,1967. (In German) 93

148. CONSIDERATION OF PROCESSES IN SEPARATION COLUMNS FROM THE POINT OF VIEW OF THE APPROACH TO EQUILI­ BRIUM. Mercca V., Palibroda N., Grecu E. Kernenergie 10, 54-9, 1967. (In German)

149. THE SEPARATION OF ISOTOPES IN DUAL-TEMPERATURE SYSTEM WITH OPEN CIRCUITS. Mercca V., Grecu E., Olariu A. Rev. Roura. Pliys. 12, 29-42, 19C7.

150. CHEMICAL RESEARCH AT THE SWEDISH ATOMIC ENERGY COMPANY. Svenke E. (Aktiebolaget Atomenergi, Stockholm, SWEDEN). Svcnsk Kern. Tidskr. 79, No. 2, 89-93, 19G7. (In Swedish)

151. A BRIEF SURVEY OF PROCESSES FOR HEAVY WATER PRODUCTION. Ryan R. K. (Australian Atomic Energy Com­ mission Res. Establ., Lucas Heights, AUSTRALIA). AEC/TM-3G8. Feb. 19G7.

152. SEPARATION OF ISOTOPES. Summary of the Results of the Dual-Temperature Process for Concentrating Deuterium by the Methyl- and the PI2S Exchange Reactions with Water. Goldfrank J. C. CU-755-4, Paper III C. 1967.

153.. COMPARISON OF ME TI IY LAC ET Y LENE AND I-I2S EXCHANGE WITH H20 FOR CONCENTRATING DEUTERIUM*IN A DUAL TEMPERATURE SYSTEM. Goldfrank J.C. CU-755-5, Sect. III. Sept. 20, 19G8.

154. ON HEAVY WATER PRODUCTION IN ROMANIA. IFA Report, Bucharest, 19G7. (Unpublished) 94

155. PRESENT PROBLEMS OF HEAVY WATER PRODUCTION. Mihaila A., Vasaru G. IFA Report, Bucharest, 1967. (Unpublished)

156. CONTINUOUS TECHNIQUES FOR THE SEPARATION OF STABLE ISOTOPES. Selcclri A. Isotoponpraxis, 4, 293-7, 1968. (In German)

157. HEAVY WATER PRODUCTION. Law C.A. Nuclear Eng. 13, 145, 510-2,1968.

158. PHYSICAL METHODS FOR THE SEPARATION OF ISOTOPES. Kokoh A. Rev. Chini. Miner. 5, 645-82,1968.

159. ORIENTATIVE STUDIES ON PROFILE AND EMPLACEMENT OF A HEAVY WATER PLANT. Manciulescu A. IPRAN Report IFA, Bucharest, 1968.

160. HEAVY WATER PRODUCTION IN ROMANIA. Mercea V. IFA Report, Bucharest, Oct. 1968. (Unpublished)

161. ISOTOPE SEPARATION PRACTICE. Bigeleisen J. Advan. Chem. Ser.No. 89, 1-24, 1969.

162. HEAVY WATER. Malleroy A. Atomes 24, 265, 322-5,1969.

1G3. HEAVY WATER EXPERIENCE AT HALDEN. Wood J.' I., Wullum T. Nucl. Eng. Int. 14, 338-42, 1969.

164. PRODUCTION OF HEAVY WATER. Status Report. Ayres J. A. (Batelle-Northwest, Richland, Nash. Pacific Northwest Lab. USA) BNL-884. Mar. 1969. 95

Ì65. REVIEW OF HEAVY WATER PRODUCTION PROCESSES. Rae II. K. (Atomic Energy of Canada Ltd. .Chalk River (Ontario)). AECL-2503. Aug. 1969.

1G6. REVIEW OF FUEL PROCESSING TECHNOLOGY PRESENTED AT THE 1964 GENEVA CONFERENCE. Gresky A. T. (ORNL) Progr. Nuc'l. Energy Sur. Ill 4, 3-34.1970.

1G7. HEAVY WATER PRODUCTION. A REVIEW OF PROCESSES. Lewins D. M. (Australian Atomic Energy Commission^ Research Establishment, Lucas Heights). AAEC/TM-562. Sept. 1970.

16&. STUDIES OF HEAVY WATER PRODUCTION IN FRANCE. Roth E.. Rostaing M. (CEA. FRANCE). CNEN Symp. on the Technical and Economic Aspects of Heavy Water Production. Turin. Italy. Sept. 30 - Oct. 1. 1970.

169. STRUCTURAL ACTION OF CHROM1A FOR INCREASING THE CATALYTIC PROPERTIES OF NIKEL IN THE HYDROGEN-HEAVY WATER ISOTOPIC EXCHANGE. Olariu A. (Inst, of Nuclear Physics, Bucharest). Stud. Cercet. Fiz. 22, 953-85. 1970. (In Rumanian)

170. VERSATILE HEAVY WATER. Swaroop J. (Bhabha Atomic Research Centre, Bombay). Vaigyanik 3, No. 1.8-12. Mar. 1971. (In Hindi)

171. STUDIES OF PRODUCTION PROCESSES AND HEAVY WATER PLANTS USING THE FRENCH PROCESS. Roth E. ,Traourouder R., Viratene J., Lefrancois B. P/607 (FRANCE) 4th Geneva Conf.1971.

172. INDUSTRIAL PRODUCTION OF HEAVY WATER. Kortus J., Zoch O. (Czech Atomic Energy Commission, Prague). Jad. Energ. 17, No. 9, 291-6. Sep. 1971. (In Czech) 96

173. HEAVY WATER PRODUCTION.Lewins D. M., Alfredson P. G. (Australian Atomic Energy Commission, Coogee). At. Energy Aust. 15, No. 3, 2-11, Jul. 1972.

174. CHEMICAL PROCESS ENGINEERING. PROCESS AS AN ADVANTAGEOUS PROCESS IN FUEL REPROCESSING. 7. CHEMICAL PROCESSES IN THE DEVELOPMENT OF NUCLEAR TECHNOLOGY. Lanius E. II. VDJ, Nachr". 2G, No. 14, 14, 1972. (In German)

175. PLANTS AND PROCESSES FOR THE PRODUCTION OF HEAVY WATER. Nitschkc E. Atomwirtschaft 18, No. 6, 274-80, June 1973. (In German) 97

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98

Open to public inspection DA Germany F. R. Patents granted DB At public disposal OS South Africa SAD Sweden SP Switzerland BS Patents BR U. S.S.R, Author Certificates CA

(Information received as of .January 22,1971)

if i 99

BREVATOME/ DOCUMENTATION' R 1910

Heavy water Production by Chemical Exchange H2S-HDO B.l Fabrication d'eou lourdo par óchango chiciique H-S - HDG

1 - US 2 787 526 du 9.11.1943 U.S.A.E.C. "r-lethod of isotope concentration"

BP 845 501 4.10.1944 S.P.E.V.A.C.K. CP 574 293 7.10.1944 A.E.C.

2- US 2 776 263 du 16.04.1945 U.S.A.E.C. "Corrosion inhibitors for deuterium exchange process"

.1- US 2 741 543 du 22.05.1945 U.S.A.E.C. "Process for the production of deuterium oxide"

CP 558 985 26.04.1946 A.E.C. BP 837 730 25.04.1946 U.K.A.E.A.

4- US 2 895 803 du 29.09.1950 J.S. 5PEVACK "Procède et instalhtion de concentration d'isotopes"

BF 1 232 316 2B.05.1957 DA 1 235 272 28.05.1957 BP 865 705 23.04.1957 CP 612 087 14.08.1957 BP 865 706 23.04.1957 CP 763 347 9.01.1961 BJ 36-13 808 9.05.1957 CP 780 298 9.01.1961 BJ 37-11 655 9.05.1957

5- US 2 954 279 du 23.02.1954 RENSSELAER POLYTECHNIC INSTITUTE "Method of manufacturing heavy water"

BP 81 e 777 18.06.1956 DA 1 047 753 20.06.1956

6- US 2 952 525 du 20.10.1955 RENSSELAER POLYTECHNIC INSTITUTE "Procède de fabrication d'eau lourde"

BF 1 157 971 11.09.1956 DA 1 050 319 21.06.1956 BP 818 421 18.07.1956

7- BF 1 164 729 du 12.01.1957 CE.A. "• Perfectionnement aux procédés d1 enrichissement isotopique par échange bitherme ".

BS 347 172 24.12.1957 BB 563 817 9.01.1958 CP 592 261 30.12.1957 US 3 007 777 3.01.1958 BP 870 036 1.01.1958 BI 582 359 31.12.1957 DA 1 080 073 11.01 1958 NP 126 702 10.01.1958 BJ 35 B488 10.O1.195e BE 239 310 27.12.1957 BLUX . 35 683 6.01.1958 IP 10974 27.11.195B 100

BREVATÜME / DOCUMENTAT I UN lì 1910

PF 1 164 750 du 15.01.1957 CE.A. "Perf ectionneiiten t nux procèder, d'enrichisscment isotopique por échange bithenne".

BS 3/17 5Ue 30 12 1957 BJ 35-R4B9 14.Ol.1950 CP 600 Ü05 10 01 1950 DE 239 461 B.Ol.1950 BB 563 fllO 2 01 .1950 IP 11 005 12.01.1950 BI 503 602 1 1 01 .1950

BF 165 257 du 23.01.1957 C.E A. "Perfectiünnetiien t aux procédés d ' enrichissemen t isotopique par échange bitherme".

CP 600 007 16.01.1958 BI 583 609 16.01.1958 BS 34B 956 14.01.1958 BJ 35-0490 22.01.195B BP 079 467 21.01.1950 SP 200 527 23.01.1950 BB 564 177 22.01.1950 IP 11 025 17.Ü1.195B MP 126 776 21.01.1950 BLux 35 704 11.01.1950 DA 1 206 390 22.01.1950 BE 239 639 10.01.1950 in - BF 1 169 140 du 5.03.1957 L'AIR LIQUIDE "Procède d'enrichissement d'un compose chimique en un element". DA 1 055 507 1 .03.1950 BI 5Ü8 027 4.03.1950 1 1 - BF 1 175 094 du 6.06.1957 C.E.A. "Perfectiunnement aux procédés d'cnrichissement isotopique par échange bitherme"•

19. - BF 1 170 661 du 5.07.1957 Sté D'ETUÜES POUR L'OBTENTIOtJ DU DEUTERIUM "Perfectionnement au procede de refroidissement d'un gaz dans un échange isotopique bitherme".

BI 591 579 19.06.195D IP 11 450 15.06.1950 5P 219 562 4.07.1950 DA 1 260111 2.07.1950

13 - DA 1 064 919 du ?.10.1957 PINTSCH DAI1AG A.G. "Verfahren zur Iso topenanreicherunq d^rch zwei temperatur - Stoffaustausche

14 - 5PD 1 169 du 7.02.1950 ALLMANNA SVENSKA ELEKTRISKA A.D. "Method and means for heat exchange of gases".

CP 630 951 31.01.1959 DA 1 137 421 4.02.1959

15- BP 067 840 du 10.03.1950 CONSTRUCTORS JOHN BROWN Ltd. &. N.W. R0BERT5 "Improvements in or relating tD the concentration of deuterium". 101

BREVATOME / DOCUMENTATION R 1910

16- 5PD 3 665 du 16.I LMANNA 5VEN5KA ELEKTRISKA A.B. "Procède pour le refroiu d'un gaz en circulation dans une installation .pour l'enricl .cement de l'oau en eau lourde".

BF'1 221 479 6.04.1959 CP 616 04B 1.04.1959 DA 1 255 096 14.04.1959 17- BF 1 207 117 du 1.0B.1958 -ELEKTRISK KVAELSTOF AKTIESELSKAB "Procède et installation pour la fabrication d'oxyde de deuterium".

18- US 3 142 540 du 25.06.1959 J.5. SPEVACK "Apparatus for dual temperature exchange". 19- DA 1 193 4B0 du 26.0e. 1959 K. SCHOE.NEHANN J. CONNEMANN '"Verfahren zum Isotopenaustauach nach dem Heiss-Ka^lt-Verfahren". 20- DA 1 193 4B1 du 5.03.1960 K. SCHOENEMANN J. CONNEMANN "Procède d'échange thernique pour la separation d'isotopes selon le procède d'échange chaud-froid". BF'1 2B3 48C 4.03.1961 BB 61B 750 B.06.1962 BP 979 320 20.05.1962 2i- CP 727 029 du 11.03.1963 DOW CHEhlCAL Co. "Process for istope concentration". BF 1 463 916 15.10.1965 22- CP 7E5 690 di. 31.08.1963 CANADIAN GENERAL ELECTRIC Co. "Dual temperature isotope concentration process". 23- BF 1 3S4 692 du 15.11.1963 CE.A. "Installation perfectionnée pour la production d'eau lourde".

BB 654 957 2B.10.1964 CP 766 15B 14.11.1964 BP 1 050 125 13.11.1964 BS 423 730 26.10.1964 US 3 431 0e0 13.11.1964 24- BF 1 409 660 du 22.07.1964 CE.A. "Systeme de recuperation de chalélir pour installation de production d'eau lourde par le procède d'échange isotopique bitherme".

CP 738 B67 B.07.1965 BB 665 147 9.06.1965 B5 433 209 B.06.1965 US 3 3B6 502 B.07.1965 BP 1 IIB 966 13.07.1965 DA 1 542 650 9.07.1965

25- USD 457 359 du 20.05.1965 ESSO RESEARCH L ENG.-Co. "Deuterium concentration process and apparatus". CP e03 445 6.05.1966 102

BREVATOME / DOCUMENTATION'

R 1910

9R- U5 3 437 567 du 2B. 12.1965 LUIit.US Co. "Procède perfectionné pour récupérer l'hydrogène sulfuré dans la production d'eau lourde".

BF 1 52B 639 20.12-1966 CP 796 OBé 27.12.1966 37- U5 3 411 884 du 11.04.1967 U.5.A.E.C. "Process for concentrating heavy water". CP 812 696 21.06.1967 28- USD 721 674 du 16.04.196B U.S.A.E.C. "Perf ectionnen.ents aux procédéc d'échange d'isotopes à deux .ter.-.pératures". BF 2 010 461 15.04.1969 OS 1 916 574 1.04.196t 29- USD 721 675 du 16.Ü4.1968 U.S.A.E.C. "Perfectionnemünts aux procédés d'échange d'isotopes à deux temperatures". BF 2 007 461 15.04.1969 C5 1 916 573 1.04.1969

3(1- U5D 721 676 du 16.U4.196E U.S.A.E.C. "Perf ectionnemen ts aux procédés d'échange d'isotopes à deux tei.-.pératurcs". BF 2 00: 459 14.04.1569 Do 1 916 570 1.04.1569' 31- CPD 31 19B du 30.09.1568 CANADIAN GENERAL ELECTRIC Cy Ltd. "Echangeur à tour étagée notamnicnt destine à lu production d'eau lourde". BF 2 019 256 30.09.1969 OS 1 949 3E7 30.C9.1569 103

BREVATOME / DOCUMENTATION

R 191Ü Heavy water Production by Chemical Exchange NH3-HD B.2 Fabrication d'eau lourde par échange chimique NU- - HD

1 - US 2 676 E75 du 16.06.1942 U.S.A.E.C. "Catalytic apparatus for isotope exchange"

CP 519 Oil 12.06.1943

ü -U5 2 650 379 du 21.11.1 942 I1.5.A.E.C. "Proceus for production of d .utc oxide a3 a source of deuterium".

BP PGü 73Ü 11 .11 .1943 I'.K.A. CP. 53Ü 34 3 9.11 .154 3 U.ii.A. .C. 3 - US 2 787 526 du. 5. 11.1943 U.S.A.E.C. "tfethod of isotope concentration", BP C45 501 4.1c'. 1944 S. P.E.V. A .C. K. CP 574 293 7.10.154.1 A.E.'C.

4 - BP L07 SÜ3 du 4.C5.1956 COSTAR'- JCHfo BRUV.'N Ltd. "PerfectionnEraunts relatifs ä un procède d'cxtrcction du deuterium de gaz renf eri;,^nt de l'hydrogàne". BF 1 174 545 3.05.1557 DA 1 051 092 4.U5.1957 CP 619 092 4.C5.1957 5 - DA 1 030 E1C du 16.06.1556 F. U.H.D.E. Gnbh. "Verfahren zur Gewinnung von nn Deuterium angereicherter,) VJassEX zw. Wasserstoff • aiy 'jzazcr". 6 - BP G69 413 du 4.07.1956 U.K.A.E.A. "Procède de production d' csu luurde".

BF 1 178 627 3.07.1957 DP B9 558 3 07 1957 BI 574 307 3.07.1957 MP 92 998 28 06 1957 CP 592 366 27.06.1957 BJ 39-11 753 4 07 1957 BB 550 926 3.07.1957 BP 864 768 du 2.06 1956 U.K.A.E.A. "Perfectionnements concernant la pxoduction d'eau lourde". BF 1 1P0 420 31.07.1957 BB 55'J 165 1 .08.1957 BE 236 899 31 07 1957 i 50J 42P 29.07.1957 BN 110 418 31 .07 1957 D 1 129 13L 29.07.1957 NP 93 075 31 .07 1957

.../... 104

BREVATOHE / DOCUMENTATION

a 1910

R. DA 1 036 223 du 17.00.1956 F. UHDE Grnbh "Procède d'enrichiscement ou d'obtcntion d'eau lourde ou cours de la aynthèsa de l'ammoniac ovec échange d'isotopcs entre l'anmoniac et 1'hydrogène".

3F 1 100 973 G.06.1957 BD 560 102 16 OQ 1957 BP B70 452 7.06.1557 CP 585 614 10 CG 1957 US 2 997 365 13.Oe.1957 BI 576 227 31 07 1557 EJ 39-5 912 12.00.1957

a- 3F 1 169 140 du 5.03.1957 L'AIR LIQUIDE "Procède d' enrichissement d*un compose chimique en un element".

DA 1 055 507 1.03.1950 BI 568 027 4.03.195B

10 - BP G67 846 du 10.03/1958 CONSTRUCTORS JOHN BROWN Ltd. & N.W.ROBERTS. "Improvements in or relating to the concentration of Deuterium". 11 - ÜP_ du 14.G3.1958 OSTERREICHISCHE STICKSTOFFWERKE A.G. "Procede de concentration du deuterium dans l'hydxogène ou 1'ammoniac".

3F 1 224 376 12.03.1559 BP 847 504 16.03.1959 DA 1 155 228 5.03.1959 LENTIA.

12 - DA 1 120 431 du 13.00.1956 F. UHDE Gobh "Procède d'enrichissement d'eau ou d'h^drogène en deuterium, dans la synthèse de 1'ammoniac".

BF 1 237 972 13.06.1959 BP 092 067 13.08.1959 BB 561 674 13.06.1959

13 - BF 1 209 633 du 22.OB.1958 C.E.A. "Perfectionnement aux méthodes de soutirage dans les procédés d'enri­ chissement isotopique pax échange bitherr.ie".

BS 359 120 18.08.1959 BP 920 227 10.08.1959 BB 581 756 17.08.1959 BLux 37 561 18.00.1959 CP 630 236 18.06.1959 IP 12 886 18.08.1959 BI 614 303 7.08.1959

14- BF 1 219 270 du 13.12.1958 HOUILLERES DU BASSIN DU NORD ET DU PAS-de- CALAIS "Perfectionnements aux cetalyseuxs de polyméxisation et d'échange".

BP 925 923 11.12.1959 BJ 37-7 735 14.12.1959 CP 637 770 11.12.1959 US 3 133 793 10.12.1959 BB 585 501 9.12.1959 BI 621 772 12.12.1959 DA 1 124 694 11.12.1959 B5 411 356 11.12.1959 BND 246 367 12.12.1959 105

BREVATOME / DOCUMENTATION R 1910

15- B5 3B3 939 du 13.03.1959 5UL2ER "Fabrication d'hydrogène enrichi en deuterium, et pr'oduction consecutive d'eau lourde". BF 1 249 06B 23.02.1960 BP 903 367 9.03.1960 BND 237 B67 7.04.1959 in- BF 1 237 166 du B.06.1959 CE.A. "Perfectionnement aux procédés de preparation d'eeu lourdc par échange isotopique monotherme ammoniac et hydrogène". CP 644 705 31.05.1960 NP 105 454 30.05'.196O BB 591 019 9.05.1960 BS 400 385 16.05.1960 05 1 417 759 3.06.1960 IP 13 933 25.05.1960 BP 952 335 25.05.1960 US 3 233 971 6.06.1960 17- BF 1 241 260 du 6.08.1959 CE.A.fi. H0UILLERE S DU BASSIN DU NORD ET DU PA5-DE-CALAIS "Perfectionnements aux procédés de recuperation des catalyseurs dans les processus d'enrichiaseraent en deuterium d'un compose hydrogéné". BLux 39 032 1.0E.1960 BND 254 625 6.08.1960 DA 1 142 344 3.0E.1960 B5 397 610 30.07.1960 BJ 37-9 690 5.0B.196D BI . 636 9B4 6.0B.1960 CP 656 471 5.08.I960 US 3 163 589 2.0B.1960 BB 593 655 1.0B.I960 DP 96 640 6.OB.1960 BP 950 200 4.OB.1960 18- BF 1 351 353 du 2B.OB.1959 C.E.A. 1 HOUILLERES DU BASSIN DU NORD ET DU PA5-DE-CALAI5 "Procède de saturation par contact direct d'une phase gazeuse par de la v/apeur d'un liquide charge en adjuvant non non v/olatif". CP 656 855 14.09.1960 US 3 098 020 11 OB.1960 BB 593 857 5.0B.1960 NP 104 396 12 OB.1960 BE . 260 836 13.08.1960 OS 1 417 782 29 OB.1960 ILux -' 39 063 6. OB.1960 B5 405 244 6 08.1960 BP 951 791 25.OB.1960 US 3 214 243 11 OB.1960 BJ 38-18 650 29.OB.1960 BI 636 154 17 OB.1960 DP 96 109 25.08.1960 BND 255 253 27 OB.1960 19 BF 1 243 843 du 5.09. 1959 C.E.A. "Perfectionnement aux p rocédés d'enrichissement isotopi par échanc e bitherme NH3-H2». BE 260 791 3.09.1960 BLux 39 119 .31 .08.1960 BI 626 119 2.09.1960 BB 594 323 '29 .OB.1960 20 BF 1 243 945 du 11.09 1959 CE.A. "Perfectionnement aux procédés d'enrichissement isotopique par échange bitherme à Systeme de contact d"épuisement". BE 260 827 6.09.1960- BLux 39 132 2.09.1960 BI 626 119 2.09.1960 BB 594 524 29.OB.1960 106

BREVATOME / DOCUMENTATION R 1910

21 - US. °u 1.10.1959 NORSK HYDRO-ELEKTRISK KVAELSTOFAKTIESELSK'A "Process for the concentration of heavy water". BP 867 736 3.12.1959 22 - BPD 33 906 du 6.10.1959 U.K.A.E.A. "Procède d'échange thermiquc". BF 1 268 977 4.10.1960 23 - DA 1 145 5e5 du 18.11.1959 BADISCHE ANILIN &. SODA-FABRIK A.G. "Procède pour la production d'hydrogène lourd". BF 1 273 612 14.11.1960 US 3 100 138 15.11.1960 BND 258 003 16.11.1960 BS 40,7 963 21.10.1960 24 - BP 896 269 des 4.02. et 22.09.1960 U.K.A.E.A. "Procède de concentration du deutériun". DA 1 152 999 4.02.1961 CP 653 188 4.02.1961 SP 192 252 3.02.1961 BF 1 281 601 4.02.1961 BI 632 580 3.01.1961 US 3 377 135 6-02.1961 BS 401 931 4.02.1961 NP 100 74e 3.02-1961 25 - DA 1 171 398 du 11.03.1960 F. UHDE Gmbh "Method of recycling a catalyst used for isotope exchange". CP 672 392 22.01.1962 26 - DA 1 171 399 du 11.03.1960 F. UHDE Gmbh "Method of recycling a catalyst used for isotope exchange". CP 672 s'91 22.1.1962 27 - BF 1 269 472 du 14.12.1960 C.E.A..HOUILLERES DU BASSIN DU NORD ET DU PAS-de-CALAIS., Cie de CONSTRUCTION HECA- NIQUE, PROCEDE SULZER ET L'AIR LIQUIDE " Perfectionnement aux procédès de preparation d'eau lourde par échange isotopique monotherme NH3 - H_". BLux 40 923 7.12.1961 BB 611 155 5.12.1961 DA 1 168 395 12.12.1961 US 3 239 310 7.12.1961 BND 272 357 8.12.1961 NP 105 455 5.12.1961 OP 231 958 13.12.1961 BS 412 825 5.12.1961 CP 701 779 8.12.1961 BI 660 563 13.12.1961 BP 9G5 782 6.12.1961 28 - DA 1 200 789 du 2X01.1961 F. UHDE Gmbh "Procède pour l'obtention d'isotopes, à deux ou plusieurs Stades". BF 1 314 170 24.01.1962 OP 230 329 23.01.1962 BP 999 618 .24.01.1962 BI 663 166 23.01.1962 US 3 503 710 17.01.1962 107

BREVATOME / DOCUMENTATION

R 1910

29 - I5P 15 941 du 25.08.1vul F. KLEIN et K. BAR-ELI "Precedes d'enrichissement du deuterium".

BF 1 331 779 17.08.1962 BP 994 303 10.08.1962 CP 719 200 8.08.1962 US 3 457 041 11.U5.1967

30 - DA 1 198 799 du 16.02.1963 F.UHDE Gmbh "Verfahren zur Verminderung der Deuterium - veri iste beim Isotopen ouBtausch mit Flüssigkeitskreislauf".

31 - BF 1 3B3 743 du 13.03.1963 C.E.A., HOUILEERE'J DU BASSIM DU NORD ET DU PA5-DE-CALAIS, CUMPANIE DU CONSTRUCT ION MECANiqUE - PRUCEDEb 5ULZER ET L'AIR LIGUIH "Perfectionnements au procède d'échange isotopique ammoniac -hydrogèi «_•" .

DA 1 253 683 6.03.1964 0P 245 532 12.03.19 64 BB 645 204 13.03.1964 BLux 45 65U 13.03.1964 CP 780 2B8 13.03.1964 US 3 342 550 26.03.1964 BP 1 023 859 12.03.1964 IP 20 940 9.03.1964 BS 426 750 12.03.1964 BND 6 402 667 13.03.1964 NP 107 115 7.03.1564

32 - BF 1 373 686 du 1U.U6.1963 C.E.A., HOUILLERE . DU BAbSlN DU MORD ET !)U PAS-DE-CALM'i, Ci" le CUN5TRUCTIUN f-ECAIII- ÜUE - PR0CEDE5 SULZ'JR et 1 «AIR LIQUIDE " Plateau perfectionné pour colcnnes de contact rjdz-liquide" .

OS 1 442 718 9.06.1964 OP 254 140 ' 1Ü.U6.1964 BB 648 900 5.06.1964 BP 1 063 443 9.G6.1964 CP 778 760 '10.06.1964 US 3 394 927 1U.06.1964 BND 6 406 508 9.06.1964 NP 111 900 8.06.1964 BS • 426 729 9.06.1964

33 - PAP U 10 B3B du 24.06.1964 F. UHDE Gmbh S. Ges, für KERNFORSCHUNG mbh "Procède pour l'épuration de l'hydrogène ou du mélange d'azote et d'hydrogène av/ant son introduction dans une installation destinée à la concentration du deu+érium".

BF 1 44B 234 23.06.1965 BP 1 105 498 23.06.1965 CP 773 480 23.06.1965

34 BF 1 4Q9 860 du 22.07.1964. C.E.A. "Systeme de recuperation de chaleur pour installation de productiun d'eau lourde par le procède d'échange isotopique bitherriiu".

CP 73B 867 9.07.1965 BB 665 147 9.06.1965 BS 433 209 8.06.1965 US 3 386 502 B.07.1965 BP 1 118 966 13.07.196 5 DA 1 542 650 9.07.1965

35 BF 1 433 444 . du 15.02.1965 F. UHDE Gmbh "Procède permettant de diminuer les pertes de deuterium lore de la production de D_0".

.../... 108

BREVATOME / DOCUMENTATION

R 1910

36 - BP 1 066 470 du 10.03. et 10.12.1965 U.K.A.E.A. "Procède pour la fabrication de matières enrichies en deuterium".

BF 1 476 887 9.03.1966 US 3 437 442 7.03.1966 CP 782 9B7 7.03.1966 05 1 567 871 9.03.1966

37 - BF 1 450 643 du 30.06.1965 CE.A. "Procède d'enrichissoment isotopique par échange bitherme iinuiuninr - hydrogène".

BP 1-084 940 27.06.1966 BB 681 121 16.05.1966 SP 225 302 29.06.1966 US 3 464 789 28.06.1966 OP 262 233 13.06.1966 CP 813 262 24.06.1966 BS 454 811 18.05.1966 DA 1 567 417 15.06.1966

38 - BF 1 462 290 du 24.09.1965 CE.A. "Procède d'enrichissement isotopique de 1'hydrogène".

BP 1 125 670 21.09.1966 BS 455 720 24.00.1966 BB 685 905 24.08.1966

39 - BP 1 100 991 du 7.01.1966 U.K.A.E.A. "Procède et appareil de production de matières enrichies en deuterium".

BF 1 507 428 3.01.1967 U5 3 505 016 4.01.1967

40 - BF 1 494 264 du 27.07.1966 C.E.A., H0UILLERES DU BASSIN DU l'URD ET DU PA5- de - CALAIS, L'AIR LIQUIDE t= t Cid dt. CONSTRUCTION MECANIQÜE, PROCEDES5ÙLZER "Procède amélioré d'échange isotopique pour 1'utilisation d'un cycle d'échange monothern.e ammoniac-hydrogène" .

BB 700 925 5.07.1967 BLux 54 176 26.07.1967 BS 464 866 26.07.1967 US 3 479 140 21.07.1967 BND 6 709 695 17.07.1967 NP 116 905 6.07.1967 BP 1 149 729 27.07.1967 CP 820 786 26.07.1967 41 - BF 1 515 B90 du 16.08.1966 CE.A., HOUILLERES DU BASSIN DU NORD ET DU PAS-DE-CALAIS, L'AIR LIQUIDE et Cie DE CONSTRUCTION liECANIQUE, PROCEDES 5ULZER "Procède amélioré pour la realisation d';s échsnges isotopiques suivent le procède monotherme". BB 700 892 4.07.1967 US 3 471 257 28.07.1967 DP 1 150 405 18.07.1967 NP 116 904 6.07.1967 BLux 54 046 6.07.1967

42 - BF 1 509 0B9 du 17.10.1966 CE.A., HOUILLERES DU BASSIN DU NORD ET DU PAS-DE-CALAIS, L'AIR LIQUIDE et tie DE CONSTRUCTION MECANIQUE, PROCEDES SULZER "Amelioration du procède monotherme d'échange isotopique entro ammoniac et deuterium".

BLux 54 046 6.07.1967 US 3 471 257 28.07.1967

.../... 109

BREVATOME / DOCUMENTATION

R 1910

43- BF 1 522 400 du 14.03.1967 C.E.A. "Plateau a plaques perforéos pour colonnes u'uchanges".

44- BF 1 523 472 du 24.03.1967 C.E.A. "Procède et dispositif d'échantillonnage d'une solution liquide sous prsasion".

45-Bf ft 92 590 / 1 494 264 du 15.06.1967 CiE.A,, H0UILLERES DU BASSIN DU NuRD ET PA5-DE-CALAIS, L'AIR LIQUIDE et Cie DE CONSTRUCTION t'ECANIQUE, PRUCEDES SULZE "Procède amélioró d'échange isotopique pour 1'utilisatiun d'un cycle d'échange monotherme ammoniac-hydrogène".

IR- CP D 1 5B6 du 3.10.1967 A.E.C. Ltd. "Colonne à plateaux à courants paralleles pcur échanije entre liquide^ et gaz".

BF 1 5B7 797 3.10.196B 0b 1 B00 990 3.10.196B BND 6 B14 162 3.10.1968

4"? - B5D 6 671 du B.05.1968 SULZER "Procède et appareil de traiteraent d'ammoniac deutérié".

BF 2 008 061 7.05.1969 BB 732 350 30.04.1969 110

BREVATOME / DOCUMENTATION

R 1910 Heavy water Production by Chemical.Exchange H2O-HD

Bt3 Production d'eau lourde pBr/échange chirnique H_0 - HD

1 - Ql du 6.12.1934 F. HANSGIRG "Improvements in or relating to a process for the production of water enriched with heavy water".

BP 462 191 4.11.1935 DA 674 965 12.03.1935 US 2 134 249 3.12.1935

2 - Of? du 23.12.1935 F. HANSGIRG "Improvements in or relating to the production of heavy water".

BP 4B7 066 22.12.1936 US 2 156 851 10.11.1936

3 - US 2 6B9 7B2 du 27.02.1942 U.S.A.E.C. "Production of heavy water".

BP '795 920 13.03.1943 U.K.A.E.A. CP 539 823 19.02.1943 A.E.C.

4 - US 2 676 875 du 16.06.1942 U.S.A.E.C. "Catalytic apparatus for isotope exchange".

CP 519 811 12.06.1943

5 - US 2 690 379 du 21.11.1942 U.S.A.E.C. "Process for production uT deuterium oxide as a source of deuterium".

BP 800 730 11.11.1943 U.K.A.E.A. CP 530 343 9.11.1943 fi - US 2 787 526 U.S.A.E.C. du 9.11.1943 "Method of isotope concentration".

BP 845 501 4.10.1944 S.P.E.V.A.C.K. CP 574 293 7.10.1944 A.E.C.

7 - US 2 690 380 du 4.05.1944 U.S.A.E.C. "Production of deuterium oxide".

CP 520 374 4.05.1945 BP 748 991 3.05.1945

8 - US 2 677 668 du 11.01.1945 U.S.A.CC. "Stabilization of reduced metal catnl st".

CP 514 229 11A01.1946 Ill

BREVATOME / DOCUMENTATION

R 1910

q - US 2 677 6P9 du 11.01.1945 U.S.A.E.C. "Stepwise stabilization of raduced metal catalysts",

CP 514 230 11.01.1946

10 - »5 2 851 427 du 22.03.1945 U.S.A.E.C. "Method of purifying catslysts".

11 - BI 493 492 du 31 :07.1952 C.I.S.E. "Procède pour enrichir l'eau en deuterium".

BF 1 0B6 502 30.07.1953 BB 521 B32 30.07.1953

12 - DA 1 003 690 du 8.09.1954 E.W.A. BECKER "Procède d'obtention d'eau ou d'hydrogène enrichis en deuterium".

BF 1 138 776 26.08.1955 US 3 087 791 1.09.1955 BP 803 274 25.06.1955 BS 341 481 3.08.1955 BN 108 803 17.OB.1955 CP 616 561 6.09.1955

13 - B_S du 3.08.1955 E.W.A. BECKER "Verfahren zur Gewinnung von mit Dauterium angereichertem Wasser oder WasBarstoff".

DA 1 052 960 29.10.1955

u- JJ£ du 18.11.1955 N0R5K HYDRO-ELEKTRISK KVAELSTOFAKTIESELSKAB "Procède d'extraction du deuterium è partir d'hydrogène mélange à d'autree gaz".

BF 1 179 985 19.11.1956

15 - US 2 967 0B9 du 25.11.1955 'H0UDRY PROCESS CORP. "Process for making heavy wator".

is - DA 1 032 233 du 30.04.1956 E.W.A. BECKER "Procède d'obtention d'eau ou d1hydrogens enrichis en deuterium".

BFA 71 295/1 138 776 26.4.1V57 US 2 927 003 29.04.1957 BP 834 306 30.04.1957

17 - DA 1 131 191 du 16.06.1956 F. UHDE Gmbh PA 1 135 S65 23.01.1957 DA 1 147 203 .9.08.1956

" Procèdi de fabrication d'eau,ou d'hydrogène,anrichia en deutèri um BF 1 179 427 14.06.1957 CP 585 604 21.06.1957 BP B64 026 17.06.1957 BB 558 414 15.06.1957 .../. 112

BREVATDME / DOCUMENTATION

R 1910

18- DP 869 413 du 4.07.1956 U.K.A.E.A. "Procède de production d'eau lourde"

BF 1 17B 627 3.07.1957 BB 550 926 3.07.TJ57 BI 574 307 3.07.1957 CP 592 366 27.06. TJ57 NP 92 998 26.06.1957 DP H9 558 3.07.1957 BJ 39 11 753 4.07.1957

19- BP C69 414 du 4.07.1956 U.K.A.E.A, "Appareil de production d'eau lourde".

BF 1 182 332 3.07.1957 BB 558 927 3.07.1957 BE 236 348 3.07.1957 DP 1 121 593 3.07.1957 NP 105 935 4.07.1957

20- DA 1 066 555 du 20.10.1956 RUHRCHEMIE A.G. 8. 5TEINBDHLEN-ELEKTRIZITAET "Process for the production of heavy water".

BP B65 411 8.10.1957 CP 583 841 16.10.1957 B5 401 932 2.10.1957

?1- BP B81 941 du 9.11.1956 U.K.A.E.A. "Procédés d'hydratation et de deshydratation de gaz".

BF 1 105 920 8.11.1957 CP 574 226 4.11.1957 U5 3 019 61.0 6.11.1957 BB 562 184 6.11.1957 DP 1 056 634 D.11.1957

99- DA 1 038 542 du B.12.1956 E.W.A. BECKER "Process for the production of water or hydrogen having an increa -.ed deuterium content".

US 3 036-891 4.12.1957 BP 824 820 4.12.1957 BI 602 461 29.11.1957

23- BF 1 169 140 du 5.03.1957 AIR LIQUIDE "Procède d1enrichissement d'un compose chimique en un element".

BP 1 055 507 1.03.1958 BI 588 027 4.03.1958

24- BP 877 089 du 24.04.1957 .U.K.A.E.A. "Appareil d'échonge catalytique".

BF 1 195 063 24.04.1958 CP 5BB 262 18.04.1958 BI 588 531 22.04.1958 BB 566 990 21.04.1958

.../... I1J

BREVATOHE / DOCUMENTATION

R 1910

25- BP B69 415 du 24.04.1957 U.K.A.E.A. •"Procède de production d'eou lourde".

BFA 73 511 / 1 178 627 24.D4.195B CP 592 367 1B.04.195B BB 567 DB2 24.04.1958 US 3 336 113 24.04.195B NP 97 607 24.04.195B

26 - DA 1 046 590 du 7.06.1957 DEGUSSA "Procède de traitcment de catalysours dans des dispositifs d'échange pour 1•enrichissement de deuterium".

BF 1 196 731 7.06.195B BI 591 7B3 4.06.195B BP 889 B2B 9.06.1958

'il- DA D U 4 471 du 19.OB.1957 F. UHDE Gmbh "Procède et dispositif pour la reduction de la concentration de deuterium dans l'humidité résiduairo imprégnant un catalyseur pulwérulent après filtration d'une suspension du catalyseur sur le g3teau de filtration".

BF 1 201 757 19.OB.1958 US 2 980 420 19.08.1958 BI 593 604 1B.OB.1958

28- DA 1 074 555 du 20.01.1958 V. BAYERL "Procède de production de deuterium".

BF 1 213 247 du 9.DI.1959 CP 619 681 13.01.1959 BP B96 021 13.01.1959 BI 605 202 9.01.1959 DWP 19 225 22.12.1957

90- DA 1 0B2 BB4 du 11.10.195B RUHRCHEMIE A.G. "Process for the production of heavy water".

BP 930 606 30.09.1959 BB 503 407 9.10.1959

30- DA 1 076 093 du 11.10.195B DEGUSSA "Verfahren zur Anreicherung von Deuterium in Wasser oder Wasserstoff". 31 - DA 1 200 261 du 22.11.195B METALLGESELLSCHAFT A.G. "Verfahren zur Anreicherung von .Deuterium".

32- PAP 30 525 du 24.04 &. 1.1.06 1?" PEGUSSA "Procède pour 1'enrichissement de 1 Vau ou de l'hydrogène en deuterium, e installation pour sa mise en oeuvre'

BF 1 255 667 25.04.1960 BB 509 902 19.04.1960 CP 223 170 22.04.1960 BI 617 405 23.04.1960 BN 250 700 22.04.1960

.../... 114

BREVATOME / DOCUMENTATION

R 1910

33- BF 1 245 589 du 25.07.1959 OFFICE NATIONAL INDU5TRIEL DE L'AZOTE "Catalyseurs destines à l'échange isotopique entr.e l'eau et l'hydrogène à haute temperature".

BP 929 653 13.07.1960 DB 593 203 22.07.1960 BN 253 147 22.06.1960

3d- DA 1 171 390 du 11.03.19ri3 F.UHDE Gmbh "Method of recycling a catalyst used for isotope exchange".

CP 672 392 22.01.1962

•» 35- DA 1 171 399 du 11.03.1960 F. UHDE Gmbh "Method of recycling a catalyst used for isotope exchange".

CP 672 391 22.01.1962

3P, - BF 1 278 246 du 6.12.1960 Veb Vakutronitk "Procède de concentration de deuterium et de fabrication d'eau lourde".

DA 1 145 145 21.10.1960 DP 23 705 20.04.1960 CA 148 246 6.1-2.1960 BN 25B 064 17.11.1960 DP 98 686 1.11.196D

37- US 3 206 365 du 8.02.1963 50C0NY MOBIL OIL "Production of heavy water".

38" DAD U 10 549 du 3.03.1964 F. UHDE Gmbh Ges.für Kernforschung m.b.H. "Procède de regeneration de catalyseurs à base de métaux nobles empoison- nés par des oxydes inetalliques".

BF 1 425 833 1.03.1965 115

BREVATOME/ DOCUMENTATION

R 1910

Heavy water Production by Chemical Exchange: Equipment and other Processes j; 4 Fabrication d'eau lourde par échange chimique : appareillage et autres procédés.

oLhcr processes: autres procédés :

1 - US 2 690 3B1 du 15.05.1945 U.S.A.E.C. "Isotope exchange process for concentrating deuterium".

2 - US 2 690 3e2 du 28.05.1945 U.S.A.E.C. "Dual temperature isotope exchange process".

CP 522 983 2.05.1946 BP 800 851 10.05.1946 equipment appareillaqe

3 - BSD 76 064 Ju 22.07.1959 SULZER "Colonne de tranfert de rnatière perfectionnée".

BF 1 264 235 21.07.1960

4 - BSD 76 065 du 22.07.1959 SULZER "Perfectionnements aux colonnes de transfert de matière". BF 1 264 236 21.07.1960 BN 243 011 4.09.1959

5 - BS 372 645 du 29.10.1959 SULZER "Separating devices and separating plant incorporating such devices".

BP 908 917 20.10.1960 DA 1 174 706 12.11.1959

6 - BSD 6 832 . du 15.06.1960 SULZER "Apparatus for mass transfer between two phases".

BP 973 748 29.05.1961 BF 1 266 913 6.09.1960

7 - BSD 4 341 du 12.04.1961 SULZER "Substance exchange columns".

BP 1 005 586 12.03.1962 BE 1 318 149 21.03.1962

8 - BSD 13 437 17.11.1961 SULZER "Appareillage pour l'extraction des produits d'une colonne d'échange". BF 1 '334 800 28.09.1962 BJ 39/18 003 4.10.1962

.../... 116

BREVATOME / DOCUMENTATION R 1910

9 - BSD 9 1BB/62 du 31.07.1962 SULZER "Colonne pour l'échange de substances".

BF 1 362 274 4.07.1963

10 - USD 241 494 du 3.12.1962 UNION CARBID&CORP. "Catalyseurs de reaction chimique et son procède de preparation".

BF 1 413 872 2.12.1963 BB 640 629 20.11.1963 BP 1 074 129 25.11.1963

11 - BSD 15 547 du 19.12.1963 SULZER "Colonne pour l'échange de produits".

BF 1 438 259 15.12.1964 DA 1 237 067 7.01.1964 BP 1 069 770 21.12.1964 CP 770 028 15.12.1964

12 - BSD 11 527 du 16.OB.1967 SULZER BSD 9 362/6B 24.06.1968 SULZER

"Garniture pour colonne d'échange de produits".

BF 1 575 344 2.08.1968 BB 719 499 14.08.1968 BP 1 186 647 16.08.1968 117

BREVATOME/ DOCUMENTATION R 1910 Heavy water Production by Hydrogen Distillation ]3_5 Fabrication d'eau lourde par distillation d'hydrogène

! -BN du 1.10.1954 STAMICARBON N.V. "Procède pour réfrigérer de l'hydrogène technique"

BF 1 130 015 1.10.1955

2 -BN des 22.10., 13.11.1954 8. 28.02.1955 STAMICARBON N.V. "Procède pour 1'extraction d'hydrogène lourd et d'eau lourde". BB 542 107 20.10.1955 BF 1 139 652 22.10.1955 DA 1 018 848 2tl.10.1955 CP 561 840 22.10.1955 US 2 098 554 17.10.1955 BP 815 098 29.10.1955

3 - BN du 4.02.1955 STAI-1ICARB0N N.V. '.'Procède pour la production ou la recuperation de froid par vaporation d'un liquide s'éveporant à très basse temperature". BF 1 14e 002 4.02.1956 CP 587 974 2.02.1956 BP 795 270 31.01.1956

4 - B5 332 465 du 10.Ü2.1955 0ERLIKON "Verfahren zur Gewinnung von Deuter.ùi^moxyd".

5 " B5 332 466 du 12.02.1955 OERLIKON "Procède de production de l'oxyde de deuterium". BF 1 141 241 1C.02.1956

(i - BS 332 467 du 1.03.1955 OERLIKON "Verfahren zur Gewinnung von Deuter.t>imoxyd".

7 - IN ' du 12.03.1955 STAMICARBON "Procede pour l'extraction de deuterium".

DA 1 066 554 12.03.1956 BP 826 962 12.03.1956 BF 1 152 631 12.03.1956 BB 545 933 10.03.1956 CP 575 762 12.03.1956

8 - BS 340 492 du 1.03.1956 LONZA "Verfahren zur Gewinnung von Deuter/Oj(m (D_)".

.../... 118

BREVATOME / DOCUMENTATION

R 1910

9- BP B69 412 du 19.06.1956 U.K.A.E.A. "Installation de distillation de 1•hydrogàne".

BF 1 177 343 18.06.1957 DA 1 144 30B 19.06.1957 CP 596 586 19.06.1957 US 2 960 838 19.06.1957 BS 3 700 /59 ' 19.06.1957 NP 97 806 19.06.1957

10" DA 1 026 284 du 7.07.1956 HOECHST "Procède pour concentrer l'hydrogène lourd".

BF 1 178 228 5.07.1957 CP 613 201 5.07.1957 BI 577 546 6.07.1957

] ! - BN 99 069 du 11.07.1956 5TAMICARBON N.V. "Improvements in the low temperature separation of gas mixtures".

BP 823 754 4.07.1957

12- BF 1 157 917 du 7.09.1956 L'AIR LIQUIDE "Procède de liquidation d'un gaz".

US 2 954 677 12.00.1957 CP 605 896 22.08.1957 BP 842 471 20.08.1957

13- U5 3 004 628 du 17.07.1957 U.S.A.E.C. • " Rectified absorption method for the separation of hydrogen isotopes"

H - BP 893 057 du 25.11.1957 U.K.A.E.A. "Improvements in or relating to low temperature gas mixture separation processes".

BF 1 215 376 24.11.1958 BI 599 214 20.11.1958 CP 612 ODD 14.11.1958

15- DA du 11.12.1957 Ges. für LINDE'S,. EISMASCHINEN A.G. "Improvements in low temperature purificetion of gases".

BP 894 558 10.12.1958

16- BS du 1.02.1958 SULZER "Purification of gases".

BP 865 870 20.01.1959 n

119

BREVATOME / DOCUMENTATION

R 1910

17- DA 1 066 187 du 4.07.1958 DEGUSSA "Procède pour 1'enrichissement de l'hydxogène lourd et dispositif pour aa mise en oeuvre".

BF 1 229 332 3.07.1959 NP 101 221 1.12.1959 18- DAD G25 088 ig- DAD G25 052 des 6 t 11.0B.195B Ges. für LINDE'S EISMASCHINEN A.G.

"A process of and an apparatus for low temperature gas separation".

BP 904 007 6.0B.1959 NP 102 742 5.0B.1959

20- DAD G25 003 du 6.0B.1958 Ges. für LINDE'S EISMASCHINEN A.G. "A method of and an apparatus for gas treatment".

BP 907 477 6.08.1959

21 - US 3 126 267 du 24.07.1959 AIR PRODUCTS 8. CHEMICALS "Separating isotopes of hydrogen".

22- BF 1 271 501 du 2.05.1960 CE.A. "Nouvelle installation de distillation d'hydrogène".

BL 40 059 25.04.1961 BN 264 254 2.05.1961 BB 602 994 25.04.1961 OP 232 958 28.04.1961 CP 660 349 27.04.1961 DP 101 579 15.01.1961 BP 932 178 1.05.1961

23- BF A 78 64B/ 1 271 501 9.11.1960 CE.A. "Nouvelle installation de distillation d'hydrogène".

OP 232 958 28.04.1961 US 3 216 800 1.05.1961

tv ti 120

BREVATOME / DOCUMENTATION R 1910 Heavy water Production by Water Distillation B.6 Fabrication d'eau lourde par distillation d'eau

1 - BB 490 239 du 19.07.1949 Mykola R0MANIW "Separation dB l'eau lourde".

2 - BB 490 900 du 31.06.1949 Mykola ROMANIW "Separation de l'eau lourde".

3 - BJ du 3.12.1954 S. YAGI, Y URAGUCHI "Method and apparatus for the purification of heavy water".

US 2 999 795 21.11.1955

4 - DW 14 311 du 9.07.1955 V. BAYERL "Verfahren und Vorrichtung zur Gewinnung von DeutentSi^Tioxyd".

5 - US 2 79B 359 du 1.0B.1955 U.S.A.E.C. "Steam power plant with means for heavy water concentration".

CP 567 92B 5.06.1956 BP B24 954 31.07.1956

6 - BP B06 975 du 27.10.1955 U.K.A.E.A. "Garniture pour colonnes de distillation".

BF 1 163 919 26.10.1956 A.E.C. CP 575 971 9.10.1956 A.E.H. .BS 34B 955 26.10.1956 A.E.C.

7 - BF 1 152 915 du 5.04.1956 o. GRANER "Procède et appareil de distillation"

8 - BFA70 19B/1 152 915 du B.12.1956 J. GRANER "Procède et appareil de distillation".

9 - BF 1 1B9 393 du 31.12.1957 Sté INDUSTRIELLE L COMMERCIALE DE LA Cie DES SALINS DU MIDI "Procède de separation des variétés isotopiquas de l'eau".

10 - BSD 76 063 du 22.07.1959 SULZER "Colonne de transfert de matière".

BF 1 264 234 21.07.1960

•••/«•• 121

HREVATOME / DOCUMENTATION

R 1910

11 - B5D 76 064 du 22.07.1959 5ULZER "Colonne de transfert de matière perfectionnée".

BF 1 264 235 ' 21.07.1960

12 - BSD • 76 065 du 22.07.1959 SULZER "Perfectionnements aux colonnes de transfert de matière".

BF 1 264 236 21.07.1960

13 - B5D 77 752 du 3.09.1959 5UL2ER "Distillation columns".

BP 933 281 24.OB.1960 DA 1 123 293 21.09.1959

14 - DW 25 046 du 21.12.1959 K. WETZEL "Process for obtaining Deuterium-enriched hydrogen compounds".

BF 1 253 501 18.03.1960 BP 950 627 14.03.1960 OP 227 235 21.01.1960 CA 148 793 31.03.1960 DA 1 144 697 22.12.1959 BN 249 395 14.03.1960 CP 679 138 1.04.1961

.15 - BF 1 262 640 du 19.04.1960 5té COMMERCIALE DE5 SALINS DU MIDI "Perfectionnement aux procédés pour la separation des veriétés isotopiques de l'eau".

DA 1 274 564 19.04.1961

in - BFA' 78 919/1 152 915 du 17.12.1960 J. GRANER "Procède et appareii de distillation".

Add 70 196

17 - BFA 79 520/ 1 262 640 du 7.4.1961 Sté COMMERCIALE DE5 SALINS DU MIDI "Perfectionnement aux procédés pour la separation des variétée isotopiques de l'eau".

DA 1 274 564 19.04.1961

18 - USD 679 916 du 1.11.1967 PACTIDECORP. "Appareii pour augmentar le concentration d'une fraction liquide moine volatile dans un mélange de liquides".

BF 1 590 459 31.10.1968 BND 6 815 610 31.10.1968 BP 1 189 608 31.10.1968 122

BREVATCME / DOCUMENTATION

R 1910

19 - BSD 6 B71 du B.05.1966 SULZER "Procède et appareil de traitement d'ammoniac deutéré".

BF 2 OOB 061 7.05.1969 E3 732 39C 30.04.1969

20 - DA 1 767 700 du 6.06.1968 STEINKOHLEN-ELEKTRIZITÄT A.G. "Application de la chaleur perdue dans des centrales à l'obtsntion d'eau lourde".

BF 2 010 2B5 6.06.1969

Kai

$&• 123

BREVATOME / DOCUMENTATION

R 1910

Heavy water Production by Ammonia Distillation B, 7'. Fabrication d'nau lourde par distillation d1ammoniaqua"

1 - BP 807 B03 des 4.S.1956 £ 29.04.1957 COSTAIN-JOHN BROWN Ltd. "Perfactionnements relatif 6 un procède d'extraction du deuterium de gaz renferment de l1hydrogene*. BF 1 174 545 3.05.1957 BP 1 091 092 4.05.1957 CP 619 092 4.05.1957 2 - BF 1 164 BB2 du 19.01.1957 Sta des Pioduita Azotes "Procèdo da fabrication da l'eau lourde".

3 - BP 867 B4B du 10.03.1958 CONSTRUCTORS JOHN BROWN Ltd. i. N.W.ROBERTS "Improvements in or relating to the concentration of deuterium". 124

BREVATOME / DOCUMENTATION

R • 1910 Heavy water Production by Methane Distillation 3'g Fabrication d'ssu lourde par distillation du i:

1 - BF 1 444 991 du . 14.06.1965 BRITISH AMERICAN OIL Cy Lt.i "Procède de production ds methanes deulérés et d'sau lourdu

CP 711 45B 14.12.1963 BB CS 2B9 11.06.1965

Heavy water Production by Distillation of Other Compounds Q g Fabrication d'eau lourde par distillation d'autxes composes

1 - BF 1 191 413 du 10.02.1958. K.E. (OLMBERG "Procède pour la separation des isot.-'^s.dB l'hydrogène".

BI 604 651 30.01.1959

2 - BF 1 207 143 du 25.08.1958 K.E. ÌI0LMBERG "Procède pour la séparstion dea isotc-oss dB l'hydrogène1'.

3 - U5 3 101 256 du 28.OB.1958 qUARTZ £ SILICE "Separation of hydrogan isotopes". 125 BREVATOME / DOCUMENTATION R 1 91 G

Heavy water Production by Electrolysis B,10 Fabrication d'eau laurda par électrol;

1- US 2 108 570 du 27.06.1933 AMERICAN SECURITY 4. TRb. LO. "Kinds of WBtar and method of producing them".

2 - US 2 137 430 du 15.05.1934 W.A. WEBB "ProcesB for the concentration of isotopes".

3 - DA 623 336 du 2.06.1934 I.G. FARBENINDUSTRIE A.G. "Verfahren zur Gewinnung von Schwerem Wasser und Schwerem Wasserstoff".

4 - BF 7B9 B22 -du 25.03.1935 .A.E. KN0WLES "Perfectionnements apportés à 1'electrolyse de l'eau". BP 435 450 21.02.1934 US 2 044 704 29,Ü3.1935 BN 42 704 19.03.1935 DA 666 393 26.03.1935

5 - DA 915 690 des IB.10.1941, 8.05.1945 & 7.05.1950 A. KLEMM "Verfahren zur Anreicherung von Isotopen".

6 - HP du 21.12.1942 N0RSK-HYDR0-ELEKTRISK KVAEL5T0FAKTIESELS- KAB "Procède pour élever la concentration de l'eau lourde". BF 922 529 18.02.1946 BP 620 837 10.01.1946 7 - BP 726 532 du 15.02.1943 U.K.A.E.A. "Improvements in and relating to the production of heavy water".

B - BP 726 771 du 10.08.1943 U.K.A.E.A. "Improvements in ond relating to the production of heavy, water",

CP 531 807 24.07.1944

fl - BP 581 908 du 16.11.1943 L. TR0NSTAD "A method and apparatus for the combined preparation of hydrogen, heavy water and metals or alloys'with low carbon content". in - US 2 695 26B du 27.01.1945 U.S.A.E.C. •"Process for the concentration of isotopes". CP 509 231 28.11.1944 126

BREVATGME / DOCUMENTATION

R 1910

11 - B5 328 414 du 16.08.1954 OERLIKON "Verfahren zur Gewinnung von Deuterium oxyd".

12 - BS J32 465 du 10.02.1955 OERLIKON "Verfahren zur Gewinnung von Deuterium oxyd".

13 - BS 332 467 du 1.03.1955 OERLIKON "Verfahren zur Gewinnung von Deuterium oxyd".

14 - DA 1 057 585 du 31.05.1955 K. DIEBNER "Procède relat'f à 1'enrichissement du deuterium".

15-BE du 1.06.1955 JUNTA DE ENERGIA NUCLEAR "Procède et dispositif pour obtenir de l'eau lourde à des degrés de puraté differente".

BF 1 150 242 25.05.1956 BP 837 894 25.05.1956 BB 548 230 30.05.1956 CP 566 101 26.05.1956

16 - DA 1 058 479 du 13.08.1955 F. UHDE Gmbh "Mit elektrolytisher kaskada arbeitendes Verfahren zur Herstellung von schwerem Wasser".

17- NP du 6.10.1955 N0R5K HYDRO-ELEKTRISK KVAELSTOFAKTIE- SELSKAB "Procède de concentretion de l'eau lourde".

BF 1 158 105 4.10.1956 BS 357 379 2.10.1956 CP 566 397 3.10.1956

18- DA 1 051 820 du 11.11.1955 RUHRCHEMIE A.G. i. STEINKOHLEN-ELEKTRIZI TAT A.G. "Verfahren zur Anreicherung von schwerem Wasser".

CP 575 018 8.11 .1956

m- DA 1 023 017 du 18.07.1956 W. VIELSTICH "Verfahren zur Anreicherung von schwerem WBSser in elektrochemischen Zellun".

20- BF 1 166 831 du. 1.02.1957 J.C. SEAILLES "Procède électrolytiqua da separation d'éléments épurés notamment da l'eau lourde".

BP 882 607 30.01.1958 127

BREVATOME / DOCUMENTATION

R 1910

21- BJ du 24.08.1957 ZAIDAN-HOJIN NOGUCHI KENKYU - JO "Process of carrying out electrochemically electrolysis".

US 3 111 472 8.04.1958

22 - BF 1 203 110 du 21.07.1958 J.C. 5EAILLE5 "Procède de fabrication das isotopes de l'hydrogène et de l'eau".

93 - BF 1 207 117 du 1.08.1958 NORSK HYDRO-ELEKTRISK KVAELSTOFAKTIESELS- KAB "Procède et installation pour la fabrication d'oxyde de deuterium".

24 - DA 1 088 932 du ' 5.03.1959 RUHRCHEMIE A.G. "Verfahren zur Gewinnung von schewerem Wasser in elektrochemiechen Zellen".

25 - DA 1 154 443 du 12.05.1959 A. KOSSNER &. E. WICKE "Verfahren zur Steigerung der Permeabilität von Metallen gegenüber Wasserstoff".

26 - DA 1 109 653 du 22.05.1959 RUHRCHEMIE A.G. i. STEINKOHLEN-ELEKTRIZITRT "Procède et diepositif pour l'obtention continue d'eau riche en deuterium et electrolyse de l'eau". BF 1 256 969 17.05.1960 CP 641 333 13.05.1960 SIEMENS BB 591 026 19.05.1960

27 - BF 1 322 116 du 2B.08.1959 MQUILLERES DU BASSIN DU NORD ET DU PAS-de- CALAIS L C.E.A. "Nouveau procède pour 1*enrichiesement ou le fractionnement isotopique de l'hydrogène".

BP 926 488 25.08.1960 BB 593 858 5.08.1960 DA 1 155 425 29.08.1960 BI b26 113 19.08.1960 US 3 098 020 11.08.1960 SP 219 359 29.08.1960 BN 255 292 27.08.1960

28 - BJD 3 460 du 6.02.1960 I. 0BINATA "Method of separating and concentrating isotopes and difficult-to-separate elements by electrolysis".

BP 913 336 du 30.01.1961

29 - DA 1 183 892 du 14.06.1961 L. KANDLER "Cellule d*electrolyse pour la dècompoeition de l'eau".

BF 1 329 797 14.06.1962 128

BREVATOME / DOCUMENTATION

R 1910 w - BF 1 31B 703 du 9.01.1962 C.F.T.U. "Perfectionnementa aux procédéa de fabrication d'eou lourde".

31 - OA 1 245 337 du 26.10.1962 SIEMENS A.G. &. VARTA A.G. "Verfahren zur elektrochemischen Deuterium 8nreicherungn.

32 - BP 973 B20 du 30.11.1962 JOHNSON,MATTHEY L Cy Ltd. "An improved method of 8aparating hydrogen isotopes".

33 - BJD 31 166 du 21.06.1963 ASAHI KASEI KOGYO K.K. 8. H. KAKIHANA i. ATOMIC FUEL CORP. "Procède pouz separer et anrichir des isotopes".

U5 3 425 924 17.01.1964 BF 1 403 196 19.06.1964 DA 1 232 926 19.D6.1964 BP 1 066 374 19.06.1964

34 - BJD 40 311 du 2.OB.1963 ASAHI KASEI KOGYO K.K. Ä. H. KAKIHANA "Perfectionnements apportéa aux procédéa pour la separation d'isotopea",

BF 1 402 626 30.07.1964 BP 1 067 367 4.OB.1964 05 I 442 362 31.07.1964 US 3 414 500 27.07.1964

35 - CPD 952 421 du 16.02.1966 A.E.C. Ltd. "Procède electrolytique pour la preparation da l'eau lourda".

BF 1 510 31B 27.01.1967 BP 1 152 094 27.01.1967 US 3 514 382 31.01.1967 129

BREVATOME / DOCUMENTATION

R 1910

Heavy water Production by Other Processes 3 n Fabrication d'eau lourde par autraa procédés

1 - BE 485 904 du 19.11.1946 M. ROMANI« "Separation de l'eau lourde par sa refrigeration et le décontage et l'évaporisation de l'eau légère".

2 - US 2 780 526 du 12.04.1951 UNION OIL Co. "Isotope separation process",

3 - BI 518 551 du 10.06.1954 L. BARN0CCHI "Procedimento per la produzione di acqua pesante".

4 - DA 1 091 541 des. 26.03. &. 14.06.1955 DEGUSSA "Procède de separation de matières soua forme de gaz ou de vapeur, an particulier dea isotopes et dispositif pour sa realisation". BF 1 230 416 18.07.1955 E.W.A. BECKER BP 794 834 7.07.1955 BB 539 578 5.07.1955 5 - BF 1 129 214 25.07.1955 CE.A. "Perfectionnement à la separation des isotopea et des composes de mesaee moléculaires trèa voisines".

6 - BP 826 128 du 8.09.1955 U.K.A.E.A. "Improvements in or relating to tha saparation of isotopes".

7 - DA 1.0B3 768 du 2.12.1955 SIEMENS "Verfahren zum trennen von Isotopen".

8 - BP 825 934 du 4.02.1956 U.K.A.E.A. "Improvements in or relating to the separation of the isotopos of hydrogen". CP 615 400 1.02.1957

9 - DA du 9.03.1956 CASSELLA FARBWERKE "Procède de separation de melanges liquidas". BF 1 169 182 7.03.1957 BP 823 297 7.03.1957 BJ 35 308 8.03.1957 130

BREVATOME / DOCUMENTATION R 1910

10- SAJJ du 2.07.1956 8. 3.04.1957 SOUTH AFRICAN COAL OIL AND GAS CORP. Ltd. "(ìocédé de concentration ou d'isolsment du deuterium ou d'eutres isotopes ou de leurs composes". BB 558 556 20.06.1957

11 - DA 1 096 675 du 5.09.1956. DEGUSSA "Procède de eéperation de metières sous forme de gaz ou de vapeur, en particuliex dee isotopes et dispositif pour sa realisation".

BF A 74 040 / 1 230 416 3.09.1957 E.W.A. BECKER BB 559 713 30.07.1957 BP B25 798 30.08.1957 BI 600 721 19.07.1957 US 2 951 554 3.09.1957

12 « US 2 863 526 du 17.10.1956 U.S.A.E.C. "Method of separating hydrogen isotopes".

13-DA dee 12.06. 8. 20.08.1957 CASSELLA FARBWERKE 14.08.1957 8. 6.05. 1958 "Procède de eéperation de melanges de carps". BF 1 211 398 11.06.1958 BP 836 857 10.06.1958 u - BP 907 657 du 26.06.1957 R.J. CROSS "Improvements in the separation of light and heevy components of a fluid mixture".

15 - DA du' 12.11.1957 RfltJlRCHEMIE A.G. "Process for producing heavy water".

US 3 019 088 10.11.1958 BP 901 713 12.11.1958

16 - U5 3 197 402 du 20.11.1957 S.L. RUSKIN "Methode for the rapid recovery of heavy weter end other products".

17- DAD 22 349 du 14.12.1957 RUHRCHEMIE A.G. "Process for the production of heavy water", BP 903 257 27.11.1958

18- BF 1 188 904 du 21.12.1957 Sto INDUSTRIELLE 8. COMMERCIALE DE LA Ci( DES SALINS DU MIDI "Procède de separation de variétés ieotopiques en phess liquide". 131

BREVATOME / DOCUMENTATION R 1910

ID - USD 745 374 du 30.06.195B WESTERN ELECTRIC Co. "Procèda at apparali d'axtraction da 1'helium". BF 1 227 030 11.06.1959 BP 869 047 25.06.1959 BB 579 767 17.06.1959

?.0 - BI 593 750 du 12.07.1958 G. PAOLUZI "Parati eamiparmaabili adatta alla aaparaziona rapida dal deuterio dal comune idrogeno, o dal tritio dal deuterio".

21 -BLux D 36 315 du 4.08.1958 P. MALDAGUE "Procèdi da production da deuterium et de ses composes eins! que d'eutres isotopee logore". BF 1 231 593 4.08.1959 BP 923 852 29.07.1959 BB 561 198 30.07.1959 BN 241 448 21.07.1959 BI 614 914 3.08.1959

22 - DA 1 143 792 du 10.11.1959 U. SCHMIESCHEK "Verfahren zur Anreicherung von Deuterium in Deutorium-Wasserstoff-Gomischen durch Adsorption und Dosorption an "Palladium".

?? - BI 635 056 du 1.03.1960 G. PAOLUZI "Perfezionamento nelle pareti samipsrmeabili destinata alla separazione del Deuterio del comune idrogeno".

24 - US 3 PB1 156 du B.04.1960 FLUOR CORP. "Separation of deutariui from hydrogen*.

E6 - US 3 05B 811 du 25.04.1960 ATLANTIC REFINING Co. "Method for the enrichment of D-0 in solutions of 0,0 in HjO".

gB - DAD 574 558 du 29.06.19 61 SIEMENS "Procède et installation pour la separation masaiqus da gaz rèactifs". BF 1 375 681 27.06.1962 US 3 230 693 22.06.1962

•xi - BF 1 330 152 du 15.02.1962 G.A. RUBISS0W "Methode da double contrifugation simultanee moyens employes st produits ainsi obtenus". 132

BREVATOME / DOCUMENTATION R 1 91 0

28 - I5P 17 6B7 du 22.07.1962 FERTILIZERS Ä. CHEMICALS LTD L H. AHARONI "Procède perfectionné de preparation de fractions d'hydrogène enrichies en deuterium". /

BF 1 363 0B1 17.07.1963 CHEMICALS 8. PHOSPHATES Ltd.

29 - DA 1 241 416 du 30.05.1964 Gos. für KERNFORSCHUNG mbh. "Einrichtung zum trennen von Isotopen".

30 - BF 1 414 B59 du 28.00.1964 C.E.A. "Perfectionnements au remplissage dea colonnea de aéperation ieotopique par Chromatographie, et procède de preparation".

BB 668 377 17.08.1965 BS 449 583 27.-8.1965 OS 1 519 978 26.08.1965 BP 1 123 044 27.0R. 1965

31 - US D 357 687 du 21.09.1964 GENERAL ELECTRIC Co. "Improvements in process for the separation of gases by permeetion through a polyarylene oxide film".

BP 1 115 413 10.09.1965 BF 1 458 476 17.09.1965 BB 669 917 21.09.965

32 - US 3 368 968 du . 3.03.1965 A.M.F. "Method for the deselinization of water".

33 - SA_D__2_5J12 du 11.05.1965 V. PRETORIUS, H. H. HAHN "Improvements relating to chromatography".

BP 1 148 661 9.05.1966 BP 1 148 662 9.05.1966 US 3 493 497 10.05.1966

3^ - BF 1 478 542 du 14.03.1966 S. R.T.I. "Procède de separation continue des isotopes de l'hydrogène d'un mélange gezeux par odsorption à contre-courant".

35 - BF 1 478 569 du 15.03.1966 S.R.T.I. "Procède d1enrichiasement isotopique d'un mélange gazeux contenant en particulier das isotopes de l'hydrogène".

36 - BF 1 492 087 du 19.04.1966 S.N.P.A. "Disposäif de recyclage utilissble en Chromatographie".

17 - US 3 460 318 du 14.12.1966 GULF GENERAL ATOMIC Inc. "Centrifugal molecula separator". 133

BnEVATOME / DOCUMENTATION R 1910

38- BF 1 583 714/ du 14.04.1967 CE.A. "Procédés et dispositifs de separation des molecules'1,

OS 1 90B 792 21 .02.1969 BE 364 225 26.02.1969 IP 31 632 16.02.1969 BL 57 986 12.02.1969 BND 69/02 586 19.02.1969

i» 134

ADDENDUM:

List of Patents Reported on Nuclear Science Abstract from 1972 till Oct. 15; 197.3

U.S. Patents

METHOD AND APPARATUS FOR TREATING PRE-ENRICHED AMMONIA. Hartmann F., Gisler H. R. (to Sulzer Brothers. Ltd). U.S.Patent 3, 644, 093. 22 Feb. 1972. Priority date 8 May 1968. Switzerland.

PRODUCTION OF HEAVY WATER EMPLOYING A GROUP VIII CATALYST. Mikovsky R.J. (to Mobil Oil Corp. ). U.S. Patent 3,681,021. 1 Aug. 1972. Field 31 Mar. 1970.

PRODUCTION OF HEAVY WATER. Thayer V. R. U.S.Patent 3,685,966. 22 Aug. 1972. Field 4 Aug. 1969.

DEUTERIUM SULFIDE SEPARATION AND ITS CONVERSION TO DEUTERIUM OXIDE. Glew D. N., Clarke E. C. (to Dow Chemical Co.). U.S. Patent 3,690,829. 12 Sep. 1972. Field 22 May 1970.

ISOTOPE SEPARATION WITH HEAT BALANCING. Nazzer D. B. (to Canadian General Electric Co. Ltd. ). U.S. Patent 3, 690, 830. 12 Sep. 1972. Priority date 30 Nov. 1968. Canada.

PROCESS FOR ENRICHMENT BY COUNTER-CURRENT MASS TRANSFER. Thayer V. R. U.S. Patent 3, 692,477. 19 Sep. 1972. Fiald 4 Aug. 1969.

DUAL TEMPERATURE FIXED CARBON BED HEAVY WATER CONCENTRATION PROCESS. Broughton D. B. (to Universal Oil Products Co. ). U. S. Patent 3, 700, 417. 24 Oct. 1972. Field 4 Nov. 1968. 135

8, INCREASED RECOVERY IN DUAL TEMPERATURE ISOTOPE EXCHANGE PROCESS. Babcock D.F., Neill J.S. (to United States Atomic Energy Commission). U.S.Patent 3,711,598. 16 Jan. 1973. Field date 11 May 1971.

9. METHOD OF DECONTAMINATING HEAVY WATER COOLED AND MODERATED REACTOR. Motojima K., Sakurai H., Onishi H,, Sasaki Y. , Koike M., Ueno K. (to Japan Atomic Energy Research Inst.). U.S. Patent 3, 737, 373. 5 Jan. 1973. Priority date 2 July 1970. Japan,

French Patents

1. IMPROVED PROCESS FOR PREPARING HEAVY WATER BY ISOTOPIC EXCHANGE (MONOTHERMIC TYPE) BETWEEN GAS-AND SINTHESIS GASES. Lesur P., Viratelle J. (to Socicte Chimique des Charbcmnages. Commissariat à l'Energie Atomiquc. l'Air Liquide. 1'Exploitation des'Procedes Georges Claude. Compagnie de Construction Mecanique. Procedes Sulzcr). French Patent 2, 056, 050. 19 Apr. 1971. Filed 25 Aug. 1969. (In French)

2. IMPROVED METHOD FOR PREPARING HEAVY WATER USING MONOTHERMAL ISOTOPIC EXCHANGE BETWEEN AMMONIA AND A SYNTHESIS GAS. Lesur P., Viratelle J; (to Societe Chi­ mique des Charbonnages. Commissariat à l'Energie Atomique. l'Air Liquide. Socicte Anonyme pour l'Exploitation des Procedes Georges Claude. Compagnie de Construction Mecanique. Procedes Sulzcr). French Patent 2, 074, 737. 8 Oct. 1971. Filed 22 Jan. 1970. (In French)

3. ISOTOPIC ENRICHMENT OF HYDROGEN FOR HEAVY WATER PRODUCTION. Lambert I., Ravoire J., Roth E. (to Commissariat à l'Energie Atomique). French Patent 2, 079, 708. 18 Oct. 1971. Filed 10 Feb. 1970, (In French) 136

British Patent

RECOVERY OF HYDROGEN SULPHIDE FROM WATER. Nazzer D.B. B. , Thayer V. R. (to Canadian General Electric Co. Ltd. ). British Patent 1, 285, 077. 9Aug. 1972. Filed 27 Oct. 1969.

Germany F.R. Patents

PLANT FOR THE PRODUCTION OF DEUTERIUM-ENRICHED WATER. Kluge H. (to Steinkohlen-Elektrizitaets AG). German Patent 2. 048, 117. 20 Anr. 1972. (In German)

UTILIZATION OF WASTE HEAT FROM POWER PLANTS FOR THE PRODUCTION OF HEAVY WATER. Kluge H. (to Steinlcohlen- Elektrizitaets AG). German Patent 1,767,7001 18 May 1972. (In German) 137

C - ACTUAL INDUSTRIAL PROCESSES 1 - Chemical Exchange 1 - Bithermal Exchange between Hydrogen Sulphide and Water (H2S - HDO)

1. THE CONCENTRATION OF.DEUTERIUM BY THE S-PROCESS. Spevack J.'S.' Columbia SAM Report A-393.Dec. 3,1942. Deci. 1957.

2. THE TEMPERATURE COEFFICIENT OF EXCHANGE CONSTANT FOR THE HYDROGEN SULPHIDE-WATER SYSTEM.' McClure D. C.', Herrick C.'E. Columbia SAM Report A-582.'Apr. 8,1943.

3. THE EFFECT OF TEMPERATURE AND PRESSURE ON THE MURPHREE PLATE EFFICIENCY FOR THE DEUTERIUM EX­ CHANGE BETWEEN WATER AND HYDROGEN SULPHIDE. Spevack J.S.', Grabow ski E.J. (Columbia Univ.', New York.Div. of War Research, USA). A-597.Apr.'17,1943.'Deci. Mar.' 14, 1957.

4. THE DUAL TEMPERATURE PROCESS FOR ISOTOPIC SEPARA­ TION, Spevack J.S.. MDDC-891. Deci. Feb.'26', 1947.'

5. THE IMPROVED DUAL-TEMPERATURE PROCESS FOR THE PRODUCTION OF HEAVY WATER(INCLUDING COST ANALYSIS AND PILOT PLANT PROGRAM).'Spevack J.S. NYOO-85.'Oct.'25, 1949.Decl.July 27, 1959.':

6. THE IMPROVED DUAL-TEMPERATURE PROCESS FpR THE PRODUCTION OF HEAVY WATER. REVIEW OF REPORT NYOO-85. Benedict M. , Golden S., Norton W. J, ( Res. Inc., New York,USA);NYO-180.'Jan.'6,1950.'Decl..Feb.'27, 1957. : 1.18

TUE DEVELOPMENT OF TUE ".DUAL-TEMPERATURE" PROCESS FOR TUR PRODUCTION OF HRAVY WATER. New York Operation Office. Div. of Technical Advisers AEC. iNTYOO-799. Sept. 11, 1050. Deci. Apr. P.. 15157.

CALCULATION OF REACTION EQUILIBRIUM FOR ISOTOPE EXCHANGE. Talcvskii. V. 1Y1. Zluir. Fiz.Kliim. 25, 2(N -73, 1051. (hi Russian)

S-PROCESS PILOT PIANT-FIKST RESULTS AND PROCESS PRINCIPLES. Eabcock D. F. , Biii'orrl C. B. Ji\ , Morris J. W. (Du Poni; de Nemours E. I. &Co. Savannah River Lab. , Augusta, Ga. USA). DP-3. Nov. 23, .1 951. Deci. Feb. .10, 1957.

EXCHANGE REACTIONS BETWEEN HEAVY WATER AND SULFUR COMPOUNDS AND THE ASSOCIATED ISOT01TC ANA­ LYSES. Kirshcnbaum I. (Columbia Univ., New York, USA). TJD-5028. May 25, 1.051. Deci. Mar. 7, 1957,

PHASE BEHAVIOUR IN THE I12S-WATER SYSTEM. Scllcck F. T. , Carmichael L. T. , Sage P.. 11. Ind. Eng. Choi». 44, 2219-2G, 1952.

CORROSION IN H2S-TI2O SYSTEM. Snyder .I.A. , Warren D. DP-9G. Oct. 1.95:"..

THE EQUILIBRIUM BETWEEN HYDROGEN SULPHIDE AND HEAVY WATER. Small P. A. Trans.-Faraday Soc. 33, 820-3, 1957.

HEAVY WATER PRODUCTION THROUGH THE Ir^S/l^O DUAL TEMPERATURE EXCHANGE PROCESS. Weiss G. Chain. Ing. Tech. 30,433-40, 1950. (In German) (AEC-tr-3365) 139

15. A TWO TEMPERATURE PROCESS FOR THE SEPARATION OF BINARY MIXTURES. Sakodynslcii K. I., Babkov S. I., Zhavoronkov N. M. Dokl. Vyssh. Shkoly, Khim. Tcchnologiya 1, 598,1950.

16. MEASUREMENT OF EQUILIBRIUM CONSTANTS FOR THE D2 EXCHANGE BETWEEN HYDROGEN SULPHIDE AND WATER. Haul R.A. W.,BohnkccH. , Dietrich II. Angcw. Chemie 71,30, .1.959.

17. PRODUCTION OF HEAVY WATER. Bcbbington W. P. (Du Pont dc Nemours E. I. &Co., Wilmington, Del. USA), Thayer V. R. Chum. Eng. Progr. 55, No. 9, 70-fi, Sept. 1959.

18. HEAVY WATER PRODUCTION THROUGH TWO TEMPERATURE EXCHANGE PROCESSES, PARTICULARS THE H2S HOT-COLD EXCHANGE PROCESS. Weiss G. Declicma Monograph. 34, 148-65, 1959.

19. A K.WETIC STUDY O.F THE EXCHANGE OF DEUTERIUM BE­ TWEEN LIQUID WATER AND GASEOUS HYDROGEN SULPHIDE. Garancl J. , Amanrich R. J. Chini. Phys. 56, 532-47, 1959. (NP-tr-44G)

20. SEPARATION OF HEAVY WATER BY MEANS OF A 1I2S-H20 ISOTOPIC EXCHANGE DUAL TEMPERATURE PROCESS. Alvarez Gonzales J. R., Maria Arcocha A. M., Otero tic la Ganclara J. L., Rojas de Diego J. L. (JEN, Madrid, SPAIN). Anales real soc. ospan. fis.y qui in. (Madrid) Sor. B5G, 547-58, May I960. (In Spanish) (CEA-tr-X-410)

21. CHEMICAL AND BIOLOGICAL STUDIES WITH DEUTERIUM. Katz.T.J. Am. Scientist 48, 544-80, Dec. 1960.

22. INDUSTRIAL' TESTS ON HEAVY WATER PRODUCTION BY H2S-H20 EXCHANGE. Lazartl B. (CEA), Tillol A.(SOD). Bull. Inform. Sci. et" Teclin. (Paris) No. 40, 14-18, May 1960. (In French) 140

SWEDISH HEAVY WATET! PROCESS. Eriksson B.J.(AlImüima Svcnska Elcktriska A. D., Vllstorüs, SWEDEN). Chum. &• Process Eng.41, f»-7, ,T:ui. l.iXiO.

SWEDISH HEAVY WATER PROCESS-2. Eriksson B.J. (Ailina'n- na Svonska E'iokt,.viska A. B,, SWEDEN). Cliom. fc.Proces s Eng. 41, 0:5-7, Feb. 1.9(ill.

HEAVY WATER PRODUCTION IN SWEDEN. Eriksson B.J. Nuclear Eny. r>, 400-12, Sopì. IfJfiO.

1SOTOPIC EQUILIBRIUM CONSTANTS OF THE DEUTERIUM EXCHANGE DETWEEN HBO AND HuS, UoSc, AND ll2Te. Marx D. CEA-R-i:5,')2. DK;«, (in French)

REMARKS ON TTIE ARTICLE BY I?.. Haul, H. Bohnke, II. Dietrich, Measurement of the Equilibrium Constants of the Deuterium Exchange between IT2S and HoO. Grantlcoilof. P., Roth E. CEA-Kop. .1.4 0Q. 19(50.

THERMODYNAMICS OF THE HYDROGEN SULPHIDE-WATER SYSTEM RELEVANT TO THE DUAL TEMPERATURE PROCESS FOR THE PRODUCTION OF HEAVY WATER. Tcehn. Rep. 58 ß. Pohl 11. A. T til-(>(><)(>. July 1, .1.9(50. (.1. Gliom. Eng. Data G, 515-21, 10(j.l)

APPLICATIONS OF CHEMICAL EXCHANGE METHODS TO ISO- TOPrC SEPARATION. Drnry J.S. (ORNL Tenn. USA). Progr. in Nuelear Energy 3e.r. IV 4, 308-43,10G1. Ml

SOLUBILITY OF IRON SULL'llllMù'à. Todi. rep. No. (HC. Polii H.A. (Du Poilt tie Nemours E. 1, fc Co.,Atomic Energy Div., Wilmington Del., Princeton Univ. N. J. Plastics Lab.. USA). TID-124 51, Apr .'1,1001.'

THERMAL FEEDBACK IN COUNTER-CURRENT PROCESSES. PART I. Polii H.A. (Du Pont do Nemours E. I. & Co., Atomic Energy Div. Wilmington, Del. and Princeton Univ. N.J. Plastics Lab. USA). T[D-.l2452.'Apr.' !., 1061.'

THERMAL FEEDBACK IN COUNTER-CURRENT PROCESSES. PART II. Pohl II. A. (Du Pont do Nemours E. I. & Co. , Atomic Energy Div. Wilmington., Del. and Princeton Univ. N. J. Plastics Lai). USA). Tip-12453. Apr. 1, 1961.

SWEDISH HEAVY WATER PROCESS. Eriksson B.J. ASEA Res. J. (Sweden) 7,280-304,1962.

CONTROL OF THE DUAL TEMPERATURE EXCHANGE PROCESS POH THE MANUFACTURE OF HEAVY WATER. Morris J. W., Scottoli W. C. (Du Pont do Nemours E. I, & Co., Aiken, S. C. USA). Chcm. Eng. Progr., Symp. Sor. 53, 26-38,19G2. (Presented at A. I. Ch. E.Meeting, Ran Francisco, Cai. USA, Dec. 1059)

MATERIALS OF CONSTRUCTION FOR THE DUAL-TEMPERA­ TURE EXCHANGE PROCESS FOR PRODUCING HEAVY WATER. Thayer V. R., DcLong W. B. Chom. Eng. Progr., Symp. Sor. 58, 86-93,1962. (Prosontod at A. I, Ch. E. Meeting, San Francisco, Cai. USA, Dec. 1959)

CATALYTIC EXCHANGE OF HYDROGEN SULPHIDE AND OF HYDROGEN WITH DEUTERIUM ON DISULPHIDE OF MOLY­ BDENUM AND TUNGSTEN. Wilson R. L., Kcmball C. , Galwey A. K. Trans. Faraday Soc. 58, No. 3, 583-92, 1962. 142

37. CALCULATION OF THE EQUILIBRIUM CONSTANTS OF ISOTOPE EXCHANGE BETWEEN WATER AND II2S; Katoluikov S. G., Shlypnikov S. V. Zhur. Fiz. Kirim. 3G, No. 4, 853-4, 1962. (In Russian)

3«. EXAMINATION OF RECENT IMPROVEMENTS PROPOSED BY THE AMERICANS IN HEAVY WATER PRODUCTION BY THE IT2S PROCESS. Uostning M. Report of the Colloquium on Heavy Water. (JEN, Spain and EAES Paris), Madrid Deo. 1,902. (NP-13766 P.7-2G)

30. WHY THE GS PROCESS STILL TOPS COMPETITORS. Law C. A. Can. Nucl. Tcclmol. 3, 30-40, 1904.

40. HEAVY WATER-OUR STAKE IN THE FUTURE. Con. Chem. Process. 50, No. 5, 00, 7G, May 10GG.

41. CANSO, N. S., SITE FOR HEAVY WATER PLANT. Can. Nucl. Tccluinl. 5, No. 4, 30, .Tuly-Aug. .1 .!)GG.

42. PERFORMANCE OF SIEVE TRAYS UNDER GS HEAVY WATER PROCESS CONDITIONS. PART 1. LOW PRESSURE OPERATION. Burgoss M. P., Garvin R. G., Scotteli W.C. (Du Pont de Nemours E.I. & Co., Aiken, S.'C.'Savannah River Lab. USA). DP-1025. June 1,966.

43. SEA-WATER TO FEED HEAVY WATER PLANT..Can. Chem. Process. 51, No. 6,41-2;45-6, June 1967.

44. HEAVY WATER PROCESS DEVELOPMENT AT CHALK RIVER. Rae II. K. (Atomic Energy of Canada, Ltd. Chalk River, Ont. CA­ NADA). Chem. Can. 19, No. 44-G, Oct. 18,1967. (AECL-2895) 143

45. HEAVY WATER COMES TO . Chem. Eng. Progr. 63, No. 6, 44, June 1967.

4G. PERFORMANCE OF SIEVE TRAYS UNDER GS HEAVY WATER PROCESS CONDITIONS .PART II. HIGH PRESSURE OPERATION. Garvin 11. G.', Norton E. R. (Du Pont de Nemours E. I. &. Co., Aiken, S.C. Savannah River Lab. USA). DP-1025-II. Apr. 1967.

47. SIEVE-TRAY PERFORMANCE UNDER GS-PROCESS CON­ DITIONS. Garvin R.' G.', Norton E. R., Chem. Eng. Progr. 64, 99-106, 1968.

48. ISOTOPE EXCHANGE RATES. V. HOMOGENEOUS REACTION BETWEEN H2S AND D2. Burcat A., Lifshitz A., Lewis D. , Bauer S.II. J. Chom. Phys. 49, 1449-57, 1968.

49. PHYSICAL PROPERTIES OF H2S-H20 MIXTURES. Aicro J. 15, 272-5, 1969.

50. EQUILIBRIUM CONSTANTS FOR GS PROCESS REACTIONS IN­ VOLVING TRITIUM COMPOUNDS. Jackson D. P. (AECL, CRNL, Chalk River, Ont.' CANADA). AECL-3382. Aug. 19G9.

51. COMPARISON OF METHYL ACETYLENE AND HYDROGEN SULPHIDE EXCHANGE WITH WATER FOR CONCENTRATING DEUTERIUM IN A DUAL TEMPERATURE SYSTEM. Goldfrank J. C.. New York, Columbia Univ. 1969.

52. PREDICTED PERFORMANCE OF GS PROCESS WITH SUPPLE­ MENTARY FEED TO THE HOT TOWER. Burgess M. P. (Du Pont de Nemours E.I. and Co., Aiken, S. C. Savannah River Lab.). Apr. • 1970. 144

53. DEVELOPMENT OP THE HYDROGEN SULPHIDE-WATER DUAL TEMPERATURE TECHNOLOGY. Spcvack J. S. CNEN Symposium on Technical and Economic Aspects of Heavy Water Production, Turin, Italy. Sept. 30-Oct. .1, 1970.

54. OBTAINING OF HEAVY WATER BY THE DUAL TEMPERATURE H2S PROCESS. Agostini J. P. (Commissariat à l'Energie Atomique, Sa clay, France .Centre d'Etudcs Nucleaires). CEA-R-4217. Oct. 1971. (In French) 143

45. HEAVY WATER COMES TO NOVA SCOTIA. Chem. Eng. Progr. 63, No. 6, 44, June 1967.'

46. PERFORMANCE OF SIEVE TRAYS UNDER GS HEAVY WATER PROCESS CONDITIONS.'PART II. HIGH PRESSURE OPERATION. Garvin R. G., Norton E. R. (Du Pont de Nemours E. I. &• Co., Aiken, S.'C. Savannah River Lab. USA).DP-1025-II. Apr. 1067.

47. SIEVE-TRAY PERFORMANCE UNDER GS-PROCESS CON­ DITIONS. Garvin R.' G.', Norton E. R., Chem. Eng. Progr. 64, 99-106,19G8.

48. ISOTOPE EXCHANGE RATES. V. HOMOGENEOUS REACTION BETWEEN I-I2S AND D2. Burcat A., Lifshitz A. , Lewis D. , Bauer S.'H." J. Chom. Phys. 49,1449-57,1968.

49. PHYSICAL PROPERTIES OF H2S-H2O MIXTURES. Aicre J. 15,272-5,1969.'

50. EQUILIBRIUM CONSTANTS FOR GS PROCESS REACTIONS IN­ VOLVING TRITIUM COMPOUNDS. Jackson D. P. (AECL, CRNL, Chalk River, Ont.'CANADA). AECL-3382. Aug. 1969.

51. COMPARISON OF METHYL ACETYLENE AND HYDROGEN SULPHIDE EXCHANGE WITH WATER FOR CONCENTRATING DEUTERIUM IN A DUAL TEMPERATURE SYSTEM. Goldfrank J. C. . New York, Columbia Univ. 1969.

52. PREDICTED PERFORMANCE OF GS PROCESS WITH SUPPLE­ MENTARY FEED TO THE HOT TOWER. Burgess M. P. (Du Pont de Nemours E. I. and Co., Aiken, S. C. Savannah River Lab. ). Apr. 1970. 144

DEVELOPMENT OF THE HYDROGEN SULPHIDE-WATER DUAL TEMPERATURE TECHNOLOGY.'Spovack J. S. CNEN Symposium on Technical and Economic Aspects of Heavy Water Production. Turin, Italy. Sept. 30-Oct.' 1,1970.

OBTAINING OF HEAVY WATER BY THE DUAL TEMPERATURE H2S PROCESS. Agostini J, P. (Commissariat a l'Energie Atomique, Saclay, France .Centre d'Etudes Nucleaires). CEA-R-4217. Oct. 1971. (In French) 145

ACTUAL INDUSTRIAL PROCESSES 1 - Chemical Exchange 2 - Chemical Exchange between Ammonia and Hydrogen

(Nil3 - HD)

AMMONIA - HYDROGEN EXCHANGE; Arnold H. R. Columbia Memorandum Nov. IG, 1942.

N PROCESS DESIGN. Chapin J. II., Quinn P. G., Reynolds T. G. SAM Report A-402. Doc. 5, 1942.

(On Deuterium Separation by Means of Exchange Reactions). Columbia University Memorandum Nov. 21 and 2G, 1942.

PROGRESS REPORT ON ISOTOPIC SEPARATION. Urey H. C. SAM Report A-170. Apr. 25, 1942.

CATALYSTS POR WATER-HYDROGEN AND AMMONIA HYDROGEN SYSTEMS. Urey II. C., Arnold H. R. SAM Report A-330. Oct. 20,1942.

CATALYSTS FOR AMMONIA-HYDROGEN EXCHANGE. Arnold II. R. SAM report 2 AR-4 (A-105). Jan. 9, 1943.

EQUILIBRIUM TIME. Mayer H. L. SAM Memorandum 4 M-4. Jan. 5, 1943. 146

B. HIGH CONCENTRATION PROCESS.' Mayer H.', Bonner R. SAM Report 4 R-19. fob. 2, 1943.'

9. TPIE N PROCESS.Quinn G.F.SAM Report 3 R-16 (A-510). Jan. 4, 1943.

10. PRELIMINARY REPORT ON HIGH CONCENTRATION OF DEUTERIUM BY CATALYTIC EXCHANGE REACTIONS. Mayer H. .Bonner R. AECD-3754.' Feb.'4, 1943.Deci. Aug. 14,1956.

11. COMPLEMENT SEARCH OF INTERCEPTION OF HYDROGEN ATOMS BY AMMONIA MOLECULES.'Mund W.', Huyskens P., Lories R. Bull. Classe Sci. Acad. Roy.'Belg.'35, 995, 1949.

12. SLOW EXCHANGE OF HYDROGEN IN AMMONIA SALT SOLUTIONS. Brodski A. I., Sulima L. V. Dokl. Akad. Nauk. SSSR 74,513-5, 1950.

13, BNL-Document C-4027. Bigcleiscn J. 1950. (Classified)

14. REACTION BETWEEN DEUTERIUM AND AMMONIA ON EVAPORATED METAL CATALYSTS.'Singleton J. II. , Roberts E. R., Winter E.R. S.' Trans. Farad.'Soc.'47, 131Ü-31, 1951. 147

CHEMICAL EXCHANGE REACTIONS FOR THE PRODUCTION OF HEAVY WATER. Interim Progress Report. Chemistry Dept. Bige leisen J., Elliot N., Irsa A. P., Kant A. et al. (BNL, Upton, N.Y. USA).BNL-107.Apr. 15, 1951. Deci. Nov. 14, 1956.

PROGRESS REPORT OF IH E CHEMISTRY DEPARTMENT. CON­ CENTRATION OF DEUTERIUM BY CHEMICAL EXCHANGE PROCESSES. Interim Report for Apr. 15-July 1,1951. Biegeleisen J., Elliot N. , Friedman L., Irsa A. P., Kant A. , Perlman M. L., Prosser H. C. (BNL, Upton N.Y. USA) BNL-118. Aug. 1951. Deci. Jan. 5, 1956.

AMMONIA PROCESS FOR DEUTEJIIUM.CONCENTRATION. Thompson W. I. (Ferguson I-I. K. Co. Atomic Energy Div. /New York, USA). HKF-113. Sept. 4, 1951. Deci. Feb. 20, 1957.

PLATE EFFICIENCY IN THE EXCHANGE OF DEUTERIUM BETWEEN AMMONIA AND HYDROGEN. Perlman M. L., Biegeleisen J. (BNL, Upton N. Y. USA) BNL-143. Dec. 3, 1951. Deci. Dec. 3, 1955.

THE CONCENTRATION OF DEUTERIUM BY CHEMICAL EX­ CHANGE BETWEEN HYDROGEN AND AMMONJA. Bigeleisen J., Perlman M. L. BNL«.1.4(i. I)tic. J.5, 1051. Deci. Dec. 5,1955. 148

DISPROPORTIONATION IN DEUTERATED AMMONIA. Bigeleisen J. J. Cham. Phys. 20,1945-6, 1952.

HYDROGEN-EXCHANGE REACTIONS OVER IRON SYNTHETIC AMMONIA CATALYSTS AT -1950C. Kummer J. T., Emmett P.H. J. Phys. Chem. 56, 258-61, 1952.

DISPROPORTIONATION IN DEUTERIATED AMMONIA. Stedman D.F. J. Chem. Phys. 20, 718-21,1952.

CATALYSIS ON EVAPORATED FILMS. I.'THE EFFICIENCY OF DIFFERENT METALS FOR THE REACTION BETWEEN AMMONIA AND DEUTERIUM. Kemball C. Proc. Roy. Soc. (London) A 2.14, 413-26, 1952.

KINETIC STUDIES ON IRON UTILIZED AS CATALYST FOR AMMONIA SYNTHESIS. I. TEMPERATURE EFFECT ON EXCHANGE REACTION RATE BETWEEN DEUTERATED . AMMONIA AND HYDROGEN. Enomoto S. Shokubai 8, 47, 1952.

REACTION OF AMMONIA AND DEUTERIUM ON EVAPORATED NICKEL CATALYST. Kemball C. Trans. Farad. Soc. 48, 254-8, • 1952.

THE MECHANISM OF THE EXCHANGE OF HYDROGEN GAS WITH SOLUTIONS OF IN LIQUID AMMO­ NIA. Wilmarth W. K., Dayton J. C. J. Am. Chem. Soc. 75, 4553-6, 1953. (NP-4339;U-23788)

EQUILIBRIUM IN THE EXCHANGE OF DEUTERIUM BETWEEN AMMONIA AND HYDROGEN.' Perlman M., Bigeleisen J., Elliot N. J. Chem. Phys. 21, 70-2,1953. . 149

28. THE EXCHANGE REACTION BETWEEN DEUTERIUM AND AMMONIA ON THE SURFACE OF METAL POWDERS. Gutmann J. R. J. Phys.Chem. 57, 309-12,1953.

29. REVIEW OF THE AMMONIA-HYDROGEN DUAL-TEMPERA­ TURE SYSTEM FOR HEAVY WATER MANUFACTURE. Final Report. Mar. 26,1952. Deci. Mar. 4, 1957. (SOA-69). SUPPLEMENT 1. Martin . H. Z., Barr F. T. Mar. 28, 1952. SUPPLEMENT 2. ELIMINA­ TION OF EQUILIBRATOR IN AMMONIA PROCESS FOR-HEAVY WATER MANUFACTURE. Barr F. T. (Standard Oil Development Co.Esso Labs., Linden, N.J. USA).NYO-6055. Feb. 1953.

30- THE NICKEL COVERED BY SELENIUM AS CATALYST. II. MECHANISM OF EXCHANGE REACTION BETWEEN DEU- TERATED AMMONIA AND HYDROGEN IN THE PRESENCE OF NICKEL COVERED BY SELENIUM. Kaneko J. Shokubai 10,20, 1954.

31. EXCHANGE REACTION BETWEEN AMMONIA AND DEUTE­ RIUM. Miyahara K. J. Res. Jnst. Catalysis, Hokkaido Univ. 4, 193-8,1957.

32. HEAVY WATER AS AMMONIA PLANT "BY-PRODUCT". Chem. Engng. Progr. 54, 9,13 0,1958. li

SOLUBILITY OF GASEOUS MIXTURE (N2+3H2) IN THE LIQUID AMMONIA. LefrahgòiV'ÌB., Vaniscotte C. Genie Chimique 83, 5/ 139-45; 1960.

SATURATION OF A GASEOUS MIXTURE (N2+3H2). WITH AMMO­ NIA IN THE PRESENCE OF LIQUID AMMONIA AT. 300 AND ' 500 kg/cm%ETWEEN-70°C AND +60°C. Lefrancois B., Vaniscof- tè C.Chaleur Ind.419, 183-6, 1960. (In French)

HEAVY WATER, FRENCH RESEARCH AND PROCESSING. Paulsen F.R.Nucl. Energy, 471-3, Oct. 1960.

DEUTERIUM EXCHANGE BETWEEN HYDROGEN AND LIQUID' AMMONIA WITH POTASSIUM AMIDE AS CATALYST. Haul R.A.W.: Ihle H., Schierholz H. Chem. Ing. Tech. 3-3, No. 11, 713'-8,1961.' (In German) I

EXCHANGE OF DEUTERIUM BETWEEN HYDROGEN AND LIQUID AMMONIA. Bourke P. J., Lee J. L. Trans. Inst j, Chem., :. Engrs.39, No. 156, 280, 1961.

THE ISOTOPIC EXCHANGE BETWEEN GASEOUS HYDROGEN AND LIQUID AMMONIA. PART I: THE KINETICS OF THE EX­ CHANGE INA BUBBLING CONTACTOR. Rebora P. L. (L. R. S. R,, Milan, ITALY). Energia Nucleare 9, 388-96, July 1962. (In English)

A NEW PROCEDURE FOR THE PREPARATION OF HEAVY WATER BY ISOTOPIC EXCHANGE. Roth E. (CEN, Saclay, FRANCE) Energie Nucl.4, 332-42,_Sept. -Oct. 1962. (In French) ... .151

KINETICS OF ISOTOPE EXCHANGE BETWEEN HYDROGEN , AND LIQUID AMMONIA ON HETEROGENEOUS CATALYSTS. ' Haul R., Blenheman D. J.' Catalysis 1(5), 432-42,1962.

ISOTOPE EXCHANGE BETWEEN GASEOUS HYDROGEN AND LIQUID AMMONIA. Bar-Eli K., Klein F. S. J. Chem. Soc. London 1378-88, 1962.

ISOTOPE EXCHANGE BETWEEN HYDROGEN AND LIQUID AMMONIA IN THE PRESENCE OF HETEROGENEOUS CATALYSTS. Haul R., Blennemann D. KFA jlllich Rep. No. 31-PC. 1962.

SOLID-LIQUID EQUILIBRIA IN THE NHg-KNHg SYSTEM. Moreau C.Lepoutre G. Bull. Soc. Chcm. (France)No. 8, 1721-3, 1963. (In French)

DETERMINATION OF THE SEPARATION FACTOR OF DEU­ TERIUM BETWEEN AMMONIA AND HYDROGEN. Ravoire J., Grandcollot P., Dirian G. (CEN, Saclay, FRANCE). J. Chini. Phys. 60, 130-8, Jan.-Feb. 1963. (CEA-R-2244. 1963)

KINETICS AND MECHANISMS OF THE EXCHANGE BETWEEN LIQUID AMMONIA AND HYDROGEN IN THE PRESENCE OF POTASSIUM AMIDE. Dirian G.yBotter F. /Ravoire J., Grand­ collot P. J. Chim. Phys. GO, 139-47, 1963 (In French) (CEA-TP-1560)

HYDROGEN EXCHANGE BETWEEN D2 AND NH3 CATALYZED BY EVAPORATED Ni FILM. Mjyahara K. J.' Res. Inst ; Catalysis, Hokkaido Univ. 11(2), 129-31, 1963.' 1SZ

GAS ABSORPTION PERFORMANCE OF BUBBLE COLUMN- (with Special Reference to the NH3-H2 process for Deute­ rium Separation).'Bourke P.'J.', Pepper D. Trans. Inst. Chem. Engrs. (London) 4.1(1), 40-50, 1963,

THE AMMONIA HYDROGEN EXCHANGE SYSTEM FOR THE ENRICHMENT OF HEAVY WATER.'Schindewolf U., Walter S. Abt. Deut. Akad. Wiss.Berlin, Kl. Chem.', Gcol. Biol. 7, 163, 1964.

CONTRIBUTION TOWARDS THE STUDY OF DEUTERIUM SEPA RATING FACTORS BETWEEN AMMONIA AND HYDROGEN. Lei'rancois B., Bourgeois Y. Genie Chim. 91, No. 5, 138-49, May 1964.

NEW CATALYSTS FOR THE EXCHANGE OF DEUTERIUM BETWEEN HYDROGEN GAS AND LIQUID AMMONIA. Kenyon A.R., Pepper'D. J. Appi. Chem. London 14, 399-405,1964.

PRODUCTION OF HEAVY WATER FROM NITROGEN-HYDRO­ GEN MIXTURES. Gel'pcrin 1.1., Kalioiina S. E,, Rapoport L. L. . Khim. Prom. No. 6, 475-6,1964.(In Russian)

ISOTOPE EXCHANGE BETWEEN AMMONIA AND HYDROGEN . Neth.Appl.6, 402,667, Sept. 14, 1964.

ACCUMULATION OF DEUTERIUM BY COUNTERCURRENT ISOTOPE EXCHANGE BETWEEN HYDROGEN AND AMMONIA IN THE HOT-COLD PROCESS. Schindewolf U., Walter S. Ber. Bunsenges. Phys. Chem. 69, 907, 1965.

CATALYSIS BY ALKALINE OF THE ISOTOPE EX­ CHANGE BETWEEN HYDROGEN AND LIQUID AMMONIA. Delmas R., Courvoisier P., Ravoire J. J. Chim. Phys. 62, 1423-5, Nov. - Dec. 1965. (In-French) 153.

PRODUCTION OF HEAVY WATER FROM NITROGEN-HYDRO­ GEN MIXTURES BY ISOTOPIC EXCHANGE IN THE SYSTEM HYDROGEN-AMMONIA. Kalinina S. E., Trubitsyn B. A., Gel'pcrin I.I. Khim Prom.'41(ll), 861-8, 1965,(In Russian).

DECOMPOSITION OF AMMONIA ON A NICKEL CATALYST. Tamaru K., Tanaka K., Fukasalai S., Ishida S. Trans. Faraday Soc. 61, No. 4, 765-72, 1965.

(On Heavy Water Production). Can. Chem. Processing P-56. June 1966.

PRODUCTION OF HEAVY WATER AT THE NATURAL GAS FERTILIZER FACTORY FENCHUGANJ. A Feasibility Study. AEpD/CH-8. Feb. 1966. (Pakistan AEC Accession Nc-25464)

ISOTOPIC EQUILIBRIUM IN THE HYDROGEN-AMMONIA SYSTEM. Barb D., Moraru N. Stud. Cercet. Fiz. Bucharest 19,131-9,1967.

FRENCH PROCESS FOR MAKING HEAVY WATER.Bauche P., Lefrancois B.Ann. Mines No. 5, 17-30,-May 1968. (In French)

REPARATION FACTOR IN THE ISOTOPE EXCHANGE REACTION BETWEEN LIQUID AMMONIA AND HYDROGEN. Sakharovski Yu. A. ,Zel'vensid Ya.D. At.Encrg. (USSR) 25,499-503,1968.

ISOTOPIC EXCHANGE OF DEUTERIUM BETWEEN AMMONIA AND HYDROGEN: A NEW PROCESS FOR THE PREPARATION ; OF HEAVY WATER. Roth E. Bull. Inform. Sci. Tech. (Paris) No. 123, 3-10fFeb. 1968. (In French) UM.

63. ..DjjO'FROM SYNTHESIS GAS LOOKS PROMISING. Can. Chem.' Process.52:71-4,Sept; 1968.

64. ISOTOPIC EXCHANGE BETWEEN MOLECULAR HYDROGEN AND AND LIQUID AMMONIA CATALYZED BY ALKALI AMIDES. Delmas R. CEA-R-3377.' 1968.

65. ISOTOPIC EXCHANGE BETWEEN HYDROGEN AND LIQUID AMMONIA CATALYZED BY ALKALI AMIDES.'Delmas II., Courvoisier P.,Ravoir J.' Advan. Chem. Ser. 25-39,1969.

D20 SUPPLY ACCORDING TO THE H2/NH3 DUAL TEMPERA­ TURE PROCESS. Becker E. W., Lang G., Schindewolf U. (Univ. Karlsruhe; Kernforschungszentrum, Karlsruhe, W, GERMANY) Atomwirt., Atomtech. 14, 257-60, May 1969. (In German)

67. PURIFICATION OF HYDROGEN AND SYNTHESIS GAS BY SCRUBBING WITH LIQUID AMMONIA AND SOLUTIONS OF ALKALI-METAL AMIDES IN AMMONIA.'Schindewolf. U.", Horrike J. Chem. Ing.'Tech.'41,11, 645-8, 1969.'

68. AMMONIA-HYDROGEN EXCHANGE: WATER DECOMPOSITION , ON IRON; "REGONFLAGE".' Vasaru G." (ROMANIA).'Status.Report IFA-AG-1.'Sept; 27, 1969.'(Unpublished) 155

ACTUAL INDUSTRIAL PROCESSES 1 - Chemical Exchange' '.'•• 3 - Hydrogen - Water Exchange (H2Ò - HD)

CATALYTIC ACTIVITY OF ALKALI LYE FOR H2O-HD ISOTOPIC EXCHANGE. Wirtz K., Bonhoeffer K. F. Z. physik. Chemie 117A, 1, 1936. (In German)

THE KYDROGEN-WATER VAPOR EXCHANGE REACTION ON METAL CATALYSTS. Progress Report. A-149. March 10, 1942. Deci. Dec. 6, 1955.

PROGRESS REPORT ON ISOTOPIC SEPARATION. Urey H. C. SAM Report 143. Mar. 19, 1942.

CATALYSTS FOR WATER-HYDROGEN AND AMMONIA-HYDRO­ GEN EXCHANGE. Urey H.C., Arnold H. R. SAM Report A-330, Oct. 20/1943.

CALCULATION OF CONVERSION EFFICIENCY. Joris G. G., Hiskey C. F., SAM Report A-36 3. Nov. 5,1942.

THE EQUILIBRIUM H2+HDO=HD+H20 AND FURTHER EX­ CHANGE EQUILIBRIA IN THE SYSTEM H2, D2, AND H20. , Suess II. E.' Z. Naturforsch. 4a, 328-32, Aug. 1949. (In German)

HEAD LOSSES OF HYDROGEN AND STEAM MIXTURES THROUGH A CATALYST BED SUPPORTED BY ACTIVE CARBON.'CerraiE.',Roseo L.' La Chimica e l'Industria 36; 603,1954.' • _l\; - 156

8. A THERMAL METHOD FOR CONCENTRATING.HEAVY,WATER... Cerrai E., Marchetti C., Renzoni R., Roseo L.', Silvestri M.', Vil­ lani S. (Laboratori CISE, Milan, ITALY). NUCLEAR ENGINEERING; PART I. Chem. Eng. Progr.' Symposium Ser.'No. 11, 271-80.1954. (Energia Nucleare(Milan) 2, No. 14, 257-71;, 1955)- (In Italian)

9,' EFFICIENCY OF SOME CATALYSTS IN THE EXCHANGE REAC- ' TIONS BETWEEN HEAVY WATER AND HYDROGEN. Savie P., Ribnikar S., Pavlovic B. 8, P/958. ( YUGOSLAVIA).'.lst UN Geneva Conf. 1955. . 10. CATALYSTS FOR DEUTERIUM EXCHANGE BETWEEN HYDROGEN AND WATER. Brigoli B. , Cerrai E, Presented at Symposium on Heavy Water, Rome, Italy, Mar.' 31 -Apr.' 2, 1955.

11. THE ISOTOPIC EXCHANGE BETWEEN HYDROGEN AND WATER ON PLATINUM. RELATIVE RATES OF EXCHANGE OF ISOTOPIC HYDROGEN MOLECULES. Hannerz K. (Royal Inst, of Tech., Stock­ holm, SWEDEN). Acta Chem. Scand. 10, No. 4, 655-66, 1956.

13.'.. PREPARATION AND BEHAVIOR OF SOME CATALYSTS FOR DEUTERIUM ISOTOPIC EXCHANGE REACTION BETWEEN HYDROGEN AND WATER VAPOR. Brigoli B., Cerrai E., Renzo- ni R., Silvestri M. Nuovo Cimento No. 3, Suppl. Vol. 5, Ser. X, 478, 1957. (In Italian)

13. THERMODYNAMIC AND KINETIC PECULIARITIES OF ISOTOPE- EXCHANGE REACTIONS OF HYDROGEN..Varshavskiy Ya. M., Vaisberg S. E. Usp. Khim. 27, 1434-68, 1957. (In Russian)

,:;.A,' RADIATION-INDUCED EXCHANGE OF DEUTERIUM BETWEEN HEAVY WATER AND DISSOLVED HYDROGEN. Bardwell J., Dyne P.J. Can. J. Chem. 35, 82-8, Jan. 1957. 157

Proc. Int. Symp.' on Isotope Separation, Apr, 1957.' North Holland Pubi.'Co.'Amsterdam 1958:

STUDY OF CHEMICAL EXCHANGE BETWEEN HYDROGEN AND ,' WATER IN PRESENCE OF LIQUID PHASE-CATALYST.'.Montarmi, R#, Balaceànu J,'C.', Dirian G. (Inst.'Francais du Petrole, Rueil; CEN Saclay, FRANCE) p."247-71.'.(IFP-1554.'Apr.' 1957);

MASS AND PIEAT TRANSFER IN CONCURRENT. LIQUID-GAS FLOW. POSSIBLE APPLICATION TO SOME SEPARATING PROCES-. SES AND TO SOME SEPARATING UNITS. Finzi S., Renzoni R., .' Silvestri M., Villani S. (CISE, Milan, ITALY).P- 44-61; (Energia Nucl., Milan, 4, 211-21, June 1957).

ENRICHMENT OF HEAVY WATER IN HIGH PRESSURE EX­ CHANGE BETWEEN HYDROGEN AND AN AQUEOUS CATALYST SUSPENSION. PART I. Becker E. W., HÜbener R. P., Kessler R.W.'. Chem.Ing.Tech. 30, 2 88-96, 1958. (In German) (AERE-Lib/trans-799. 1958)

THE CATALYSIS OF THE H2-D20 EXCHANGE BY AQUEOUS BUFFER SOLUTIONS. Miller S. L., Rittenberg D: (Columbia Univ. NY, USA). J. Am. Chem. Soc. 80, 64-5, Jan. 1958.

EXCHANGE REACTIONS BETWEEN HYDROGEN GAS AND HYDR03ÖTL GROUPS. A CONVENIENT PREPARATION OF TRITIUM-LABE LED WATER. Swain C. G., Kresge A. J. (Massachusetts Inst, of Tech. .Cambridge, USA). J, Am. Chem. Soc. 80, 5281-3, Oct. 5, 1958.

ENRICHMENT OF HEAVY WATER BY HIGH PRESSURE EX­ CHANGE BETWEEN HYDROGEN AND AN AQUEOUS SUSPENSION OF A CATALYST. Becker E.W., Bier K.,Hllbener R. P., Kessler R.W. (Univ. of Marburg). 4, P/1000. (GERMANY). 2nd UN Geneva Conf, 1958.

.' EXCHANGE OF DEUTERIUM AND HEAVY OXYGEN AMONG HYDROGEN, WATER VAPOR AND OXIDE CATALYSIS OF SPINEL TYPE.Yukio Yoneda,Akio Fujimoto, Shoji Makishima.' , (Univ. of Tokyo, JAPAN). J. Phys. Chem.' 63, 1987-90, Dec. 1959.' 158

KINETICS OF CATALYZED GAS-LIQUID. REACTION IN A • STIRRED REACTOR. DEUTERIUM EXCHANGE BETWEEN', GASEOUS HYDROGEN AND LIQUID WATER. SaitoH.', Moritd N. ,SatakaO. Kagaku Kogaku 23, 45078, 1959;

THE EFFECT OF SOME HYDRODYNAMIC FACTORS ON THE CATALYTIC DEUTERIUM EXCHANGE BETWEEN HYDROGEN AND WATER VAPOR. Selecki A. Nukleonik a 5, 513-30, 1960.

DEUTERIUM-EXCHANGE REACTION BETWEEN WATER AND HYDROGEN. Selecki A. Wiadomosci Chem. 14, 741-58; 1960.

PLATINUM CATALYSTS FOR THE HYDROGEN-WATER VA­ POR ISOTOPIC EXCHANGE REACTION. Margineanu P., Piringer O., Szentgyb'rgy P. IFA Report, Bucharest, 1960. (Unpublished))

ISOTOPIC EXCHANGE OF DEUTERIUM BETWEEN HYDROGEN . AND WATER IN THE VAPOR PHASE. Baran W. J. , Cretella R.F. Arg. Com. Natl. Energia At. Informe No. 57, 1961.

INFLUENCE OF H2-D2O ISOTOPIC EXCHANGE OCCURING ON . TPIE SURFACE ON Pd-H ELECTRODES ON THEIR POTENTIAL. Bucur R.V. Rev. Physique (Bucharest) 6,269, 1961.

CATALYSTS ON THE ENRICHMENT OF HEAVY WATER BY MEANS OF EXCHANGE REACTION. Saburo Enomoto, Hiroaki Ugajin (Utsunomiya Univ. JAPAN). Shokubai (Tokyo) 3, No. 2, 126-30, 1961. (In Japanese) 159

THE ISOTOPIC EQUILIBRIUM OF A HYDROGEN-WATER SYSTEM.' Barb D., Mercea V.' IFA-IDF 13, Bucharest, 1961.

THE EQUILIBRIUM OF THE H2-H2Ó ISOTOPIC.EXCHANGE REACTION. Ciobotaru T., Szcntgyörgy P., Margineanu-P. IFA Report, Bucharest, 1961. (Unpublished)

ENRICHMENT OF HEAVY WATER BY HIGH PRESSURE EX­ CHANGE EETWEEN HYDROGEN AND AN AQUEOUS CATALYST SUSPENSION. PART III. EFFECTS ON SPECIFIC EXCHANGE PERFORMANCE OF ADDITIVES. Becker E.W., Kessler R.W., HÜbener R. P. (Technische Hochschule, GERMANY). Chem.Ing. Tech. 34, 105-8, 1962. (KFK-92) (In German)

DUAL TEMPERATURE SEPARATION SYSTEM FOR THE ISOTOPIC EXCHANGE COMBINED WITH VAPOR DIFFUSION. Margineanu P., Mercea J.', Mercea V., Olariu A. IFA Report, Bucharest, 1962. (Unpublished)

KINETICS OF THE CATALYTIC EXCHANGE REACTION OF DEUTERIUM BETWEEN WATER VAPOR AND HYDROGEN ON VARIOUS SURFACES. Nakhmanovich M.L., Morozov N.M., Buadze L.G., Temkin M.I. (Karpov Inst, of Physics and Chemistry, Acad., of Sciences, USSR). Dokl. Akad.Nauk SSSR148, 1346-9, Feb. 21, 1963. (In Russian)

THE HOMOGENEOUS CATALYSTS OF THE ISOTOPE EXCHANGE BETWEEN HYDROGEN AND LIQUID WATER. Schindewolf U.' J. Chim. Phys. 60/124-9, 1963. 160

DUAL-TEMPERATURE HYDROGEN ISOTOPE EXCHANGE BETWEEN A GAS VAPOR MKTURES AND A SOLUTION OF GAS. Vaisberg S. E., Varshavskii Ya. M. Zh. Fiz. Khim. 37;. 87-93,1963. (In Russian)

HEAVY WATER PRODUCTION BY H2-H2O ISOTOPIC EX­ CHANGE. Mercea V., Peculea M., Grecu E., PalibrodaN.- IFA Report, Bucharest, 1963. (Unpublished)

THE INFLUENCE OF CAPILLARY CONDENSATION ON THE. ACTIVITY OF Ni-Cr203 CATALYSTS FOR THE ISOTOPE EX-. CHANGE REACTION BETWEEN HYDROGEN AND WATER. Barb D., Margineanu P., Mercea V., Olariu A. Abh. Deut. Wiss. Berlin, Kl. Chem., Geol., Biol. 7, 793-9, 1964.

KINETICS OF THE ISOTOPE EXCHANGE BETWEEN HYDROGEN AND WATER. (Compensation Effects). Marazan N., Margineanu P., Olariu A. Abh. Deut. Akad. Wiss. Berlin, Kl. Chem., Geol. Biol. 7, 811-9, 1964.

THE ISOTOPE EXCHANGE BETWEEN HYDROGEN AND WATER. Mahadevan E.G. Indian J.Chem. 2(1), 1-5,1964.

DEUTERIUM ENRICHMENT BY DUAL TEMPERATURE EX­ CHANGE REACTION BETWEEN HYDROGEN AND WATER. Sawayanagi S., Kurihara Y. Koatsu Gasu Kyokaishi,27, 626-32,1964.(In Japanese)

NOMOGRAM FOR SOME CALCULUS FOR THE HYDROGEN- WATER ISOTOPE EXCHANGE REACTION. Szentgyörgy P.' Stud. Cercet. Fiz. (Bucharest) I16, 729,1964. 161

ISOTOPIC EXCHANGE BETWEEN HYDROGEN AND WATER IN A-STREAM REGIME OVER A POROUS .CATALYST LAYER. Palibroda E., Palibroda N., .IFA Report, Bucharest 19G4. (Unpublished)

LIQUID PHASE CATALYSIS OF DEUTERIUM EXCHANGE REAC­ TION BETWEEN WATER AND DISSOLVED HYDROGEN. (S.M. Thesis). Barthelemy R. (MIT, Mass. USA). Feb. 1964.

RATE OF EXCHANGE OF DEUTERIUM BETWEEN WATER AND DISSOLVED HYDROGEN IN PRESENCE OF DIMETIIYLAMINE. Ishida T. , Benedict M. (MIT, Mass., USA). MIT-2249-1, Feb. 1964.

HOW D2O MAY BE MADE IN SASKATCHEWAN. Can. Chem. Process.49,71-5,1965.

KINETICS OF ISOTOPE EXCHANGE BETWEEN HYDROGEN AND WATER VAPOR OVER NICKEL CATALYSTS. I. EFFECT OF TRANSPORT PROCESSES ON THE REACTION RATE.' Nedumova E. S., Boreskov G.K. , Slin'ko M.'G." Kinetika i kataliz 6, 65-73, 1965. (In Russian)

INFLUENCE OF THE PRESSURE ON THE ACTIVITY OF Ni- „r203 CATALYST IN THE HYDROGEN-WATER ISOTO- PLC EXCHANGE REACTION. Margineanu P., Mercea V., Olariu A. IFA Report, Bucharest, 1965. (Unpublished) 162

PRODUCTION OF HIGH ACTIVITY Ni-Cr203 CATALYST, FOR THE HYDROGEN-WATER ISOTOPIC EXCHANGE. ' ,.. ; REACTION • Bolojga- M; ,:Szentgy.örgyi P.' IFA .Reppr t; Buchare• -x, ," 1965. (Unpublished) .

THE TRITIUM BETA-RAY INDUCED REACTIONS IN DEU­ TERIUM OXIDE VAPOR AND HYDROGEN OR CAREON MONOXIDE AND THE EXCHANGE OF.H-ATOMS WITH WATER MOLECULES. Bibler N. E. Columbus, Ohio, Ohio State University, 1965.

CATALYTIC EXCHANGE OF DEUTERIUM GAS WITH WATER AND WITH AND THE EFFECT OF OF THESE REACTIONS. Jones M. L. Thesis. KnoxviUe, Term., University of Tenn. 1965.

DEUTERIUM SEPARATION BY AMMONIA DISTILLATION AND HYDROGEN-WATER EXCHANGE. Benedict M. MIT-2249-2. 1965. ' . '

HOMOGENEOUS CATALYSIS OF D2/H20 EXCHANGE BY .Ru(III)Cl3. EVIDENCE FOR HETEROLYTIC SPLITTING OF H2.Halpern J., James B. J. Can. J. Chem. 44, 671-5,1966.

DEPENDENCE ON pH OF THE RATE OF DEUTERIUM EX­ CHANGE BETWEEN HYDROGEN AND WATER ON NICKEL CATALYST. Enyo M., Matsushima T. J. Res.'lnst. Catal. Hokkaido Univ. 14, 248-56, 1966. 163

.DETERMINATION OF THE TRANSPORT CONSTANTS FOR CATALYZED HYDROGEN-WATER VAPOR-WATER'ISOTOPIC EXCHANGE REACTION. Hodor'I. ', Moraru. N., Peculqa M. Sampaleanu L. IFA Report,Bucharest, 1966. (Unpublished)

COMPARATIVE TREATMENT OF HYDROGEN POISSONING OF THE Pt-ACTIVE CARBON AND Pd-ACTIVE CARBON CATALYSTS IN THE ISOTOPIC EXCHANGE- REACTION BETWEEN HYDROGEN AND WATER. Strugaru D., :Paladi '• M., Piringer O. Stud. Cercet. Fiz. (Bucharest) 18, 1081, 1966.

ISOTOPE EXCHANGE AND EQUILIBRATION REACTION ON NICKEL IN THE SYSTEM DEUTERIUM-LIGHT WATER. Enyo M. J. Res.'lnst. Catal.'Hokkaido Univ.' 15,1-20,1967.

ISOTOPIC EXCHANGE OF DEUTERIUM BETWEEN HYDRO­ GEN AND WATER VAPOR ON ALUMINA PROMOTED NICKEL.- Olariu A., Margineanu P,' Preprint IFA (Bucharest) 15-48. Sept. 11, 1967.'

HYDROGEN ISOTOPE EQUILIBRIA IN THE SYSTEM HYDROGEN-WATER.' Bottinga Y.' J.' Phys.' Chem. 72, 4338-40, 1968.

ISOTOPE EXCHANGE OF DEUTERIUM BETWEEN HYDRO­ GEN AND WATER" VAPOR ON ALUMINA-PROMOTED NICKEL. Olariu A.', Margineanu P. Rev.'Roum.' Phys. 13, 823-8,1968.. 164

SEPARATION OF DEUTERIUM BY' CONTINUOUS COLUMNS, USING THE HYDROGEN-WATER.ISOTOPE EXCHANGE );. ' REACTION. Mei\cea V.v.IFA Report/Bucharest, 15-52; 1968. (Energie Nucleäire 10, 367-75,1968)

STUDIES OF SOME CHEMICAL PROPERTIES OF THE Ni-Cr203 CATALYST USED IN THE HYDROGEN-WATER ISOTOPE EXCHANGE REACTIONS. A New' Preparation Method. Szentgyorgy P. Thesis. Univ. of Cluj, Romania. 1968;

CONSIDERATIONS ON A DUAL PURPOSE DUAL TEMPE­ RATURE PROCESS FOR PRODUCING D20. Marchetti C. , Simon R. CNEN Symp. on Heavy Water Production. Turin/ Italy. Sept. 30-Oct. 1, 1970. .1*5

- ACTUAL INDUSTRIAL PROCESSES \ 2 - Distillation 1 - Distillation of Hydrogen

SEPARATION AND PROPERTIES OF THE ISOTOPES OF HYDROGEN. Urey H.C. Science 78, 566-71,1933.

THE HYDROGEN ISOTOPE OF MASS 2 AND ITS CONCENTRATION. Urey H. C., Brickwcdde F. G., Murphy G. M. Phys. Rev. 40, 1-15,1932

INCREASE OF CONCENTRATION OF H1!!2 BY FRACTIONAL EVAPORATION AND RECTIFICATION. Keesom W. H., van Dijk H., Haantjes j. Proc. Acad. Sci. Amsterdam 36, 248-52,1933. Comm. Leiden 224, 1933.

THÈ'VAPOR PRESSURE OF . Scott R. B., Brickweddc F. G. Phys. Rev. 48,1935.

PRELIMINARY STUDY OF THE FRACTIONATION OF ISOTOPIC ISOMERS BY DISTILLATION. Stedman D. F. Can. J. Research 13B, 114-21,1935.

THE SEPARATION OF DEUTERIUM BY THE DISTILLATION OF LIQUID HYDROGEN. Thiele E.W. Columbia Memorandum to H.C. Urey. Apr. 15, 1942. UiG

DISTILLATION OF HYDROGEN. Thiele E. W. Columbia Memorarf- dum.Sept.2, 1942.

DU PONT STUDIES. Huffman J. R. SAM Report A-330. Oct. 20, 1942.

FRACTIONATION OF LIQUID HYDROGEN. Huffman J. R. Columbia... Memorandum. Nov. 11, 1942.

VIBRATIONAL FREQUENCIES OF THE ISOTOPIC WATER MOLECULES;EQUILIBRIA WITH THE ISOTOPIC . Lib by W. F. J.Chcm. Phys. 11, 101-9,1943.

(On Hydrogen Distillation Process). Johnston II. L. Ohio State University Progress Report. SAM Reporl A-533. Feb. 13, 1943.

(On Hydrogen Distillation Process). Johnston H. L. Ohio State University Progress Report.SAM Report A-593.Apr. 10,1943.

CONSTRUCTION, OPERATION AND MAINTENANCE OF A 'POLIMER FRACTIONATION UNIT. Eichna J. R., Carpenter G. K., Manus C.J. Mc., Tuck R. ,Risher C. A-2370. July 23, 1946. Deci. Feb. 12, 1957.

HANDBOOK OF LOW TEMPERATURE TECHNIQUES. Malkov M. P., Pavlov F. K. Moscow 1947. (In Russian)

RESULTS OF LOW-TEMPERATURE RESEARCH. VIII. RECTIFI­ CATION OF H2-HD-D2 MIXTURES TO OBTAIN DEUTERIUM , DEUTERIUM, AND HEAVY WATER. Clusius K., Starke K. Z. Naturforsch. 4a, 549-59, Oct. 1949. (In German) ><57

6» SOME FRACTIONATION EFFECTS INVOLVING THE ISOTOPES OF HYDROGEN. A Review.- Eidinoff M. L. Trans. N.Y. Acad. Sci. IG, 70-82,1053.'

17. TECHNIQUES AND MATERIALS FOR USE AT LIQUID HYDROGEN TEMPERATURE. Benedict M., Graff O. (TJSAEC,Oak Ridge, Teiin. USA). Report M-151.

18. LOW TEMPERATURE DISTILLATION OF HYDROGEN ISOTOPES. Abraham B.' M., Flotow II. E. ANL-5204. Dec. 1953. Deci. Dec. 1955.

19. HYDROGEN DISTILLATION PROCESS FOR THE ISOLATION OF HEAVY WATER. .Maloney J: O. , Quinn G. F. , Ray II. S.NNES-I.II-4F, 83-98,1955.

20. PRODUCTION OF HEAVY WATER BY THE DISTILLATION OF LIQUID HYDROGEN. Hall L. G. Proc. Symp. on Heavy Water. Rome Mar. 31rApr. 2,1955. Rome, Italy. CNRN Roma 1956.

2.1. UNSTATIONARY MASS TRANSPORT IN RECTIFICATION COLUMNS. Rozen A. M. Dokl. Akad. Nauk. SSSR 107, 295-8, 195G. (In Russian)

22. THE DISTILLATION CHARACTERISTICS OF LIQUID HYDROGEN. Sellers E. S. , Augood D. R. Trans. Inst. Chem. Engrs. 34, 53-78, . 1956.

23. THE FINAL CONCENTRATION OF HEAVY WATER BY RECTIFI­ CATION. Progress in Nuclear Energy. Series 4:Technology and Engineering (Editors R. Hurst, S. McLain). McGraw Hill Book Co. 1956.P. 57-61. 1 ri

16g

24. DISTILLATION OF HYDROGEN-DEUTERIUM. MKTURES. l-'lyan T. M. et al. Proc. of the 1956 Cryogenic Engineering Coin". Ed. K, D, Timmcrhaus, Chem. Eng. Dept., Univ. of Colorado, .Boulder,, Colo. USA. Feb. 1957. V' h 25. PRODUCTIONOF DEUTERIUM BY THE DISTILLATION OF LIQUID HYDROGEN. Maloncy J. O., Hughes II. E., Adclington N. G. COO-1.9. 1057.

2G. PURIFICATION OF HYDROGEN FOR DISTILLATION. Denton W. II., Shaw B., Ward D. E. Paper presented at the Joint Symposium on Industrial Low Temperature Gas Separation, London, Nov. 26, 1957.

27. PRODUCTION OF DEUTERIUM BY DISTILLATION OF HYDROGEN. Denton W.U. Proc. Int. Symp. oh Isotope Separation, Amsterdam 1957. North Holland Publishing Co. Amsterdam 1958. (p. 383-4)

28. LOW-TEMPERATURE DISTILLATION OF HYDROGEN ISOTOPES. Timmerhaus K. D., Weitzel D. H., Flynn T. M. (NBS Cryogenic Lab., Boulder, Colo. USA). Chem. Eng. Progr. 54, No. G, 35, June 1958.

Proceedings of the 2nd United Nations International Conference on the Peaceful Uses of the Atomic Energy: Geneva 1958: 29. SOME ASPECTS OF HEAVY-WATER PRODUCTION BY DISTIL­ LATION OF HYDROGEN. Bailey B. M. (Little A.D. Inc., Cambridge, Mass.) 4, P/10G3.(USA);

30. EXPERIMENTAL RESEARCH ON THE RECTIFICATION OF LIQUID HYDROGEN TO OBTAIN DEUTERIUM. Kanda E., Sato S. , Sato T., Monna G., Tashiro T., Kubota M., Matsugashita. T. 4, P/13G2. (JAPAN);

è 169

31. PRODUCTION OF HEAVY WATER IN INDIA. Gami D. C., Gupta D., Prasad N. B., Sharma K. C. (Atomic Energy Establ. Trombay) 4, P/1G49. (INDIA);

32. INDUSTRIAL SEPARATION OF DEUTERIUM BY LOW-TEMPERA r. TURE DISTILLATION. Malkov M. P., Zcldovitch A. G., Fradkov A. B. ,Danilov LB. 4, P/2323. (USSR) - (.lad. Energia 4,344-51,' 1958);

33. INDUSTRIAL PRODUCTION OF HEAVY WATER BY DISTIL­ LATION OF LIQUID HYDROGEN. Akar P., Simonet G. 4, P/2538. (FRANCE).

34. PROGRESS IN FRACTIONAL DISTILLATION. Goldos R. L. Chom. Eng. Progr. Symp. Sor. 55, 25, 87-93,1959.

35. PROGRESS IN THE HEAVY WATER PRODUCTION BY THE HYDROGEN DISTILLATION METHOD. Ruzicka J. (USIHV jaclcrneho vyzkumi CSAV, Prague, CSSR) . Jaderna Enor^ie. 5, 340-4, 1959. (In Czech)

36. PRODUCTION OF DEUTERIUM BY HYDROGEN DISTILLATION. Schlattercr R., LehmerW., Baklus W. Kältetechnik 11, 250-4, 1959. (In German)

37. PROGRESS IN DISTILLATION TECHNOLOGY. Aerov M. E., Malyusov V.A. Khim. .Nauka i Prom. 3, 73G-45, Jan. 1959. (In Russian)

38. LOW TEMPERATURE DISTILLATION OF HYDROGEN ISOTO­ PES. NBS (USA). Tech. News Bull. 43, 116-8, June 1959. 170

39. STUDIES OF THE LOW-TEMPERATURE DISTILLATION OF HYDROGEN ISOTOPES.' Flynn T.' M.' (NBS, Boulder, Colo.' USA). Cryogenics 1, 96-100, Sept.'I960.'

40. THE SEPARATION OF DEUTERIUM ON AN INDUSTRIAL SCALE • BY LOW TEMPERATURE DISTILLATION.' Malkov M.' P., ZeldoVich A. G., Fradkov A.' B., Danilov I. B. (Inst, of Physical Problems, Acad of Sci.', Moscow, USSR).' Progress in Cryogenics.Vol. 2, G9-8G,K. Mcndelssolin ed.' Now York, Acad. Press, inc. 1960.

41. HANDBOOK OF LABORATORY DISTILLATION. Krell E. VEB Deut.'Vcrlag dor Wiss.'Berlin 1960.

42. STUDIES OF THE LOW TEMPERATURE DISTILLATION OF HYDROGEN ISOTOPES. Flynn T. M. (NBS, Boulder, Colo. USA) Advances in Cryogenic Engineering. Vol. 6. K. D. Timmerhaus ed. New York, Plenum Press. Inc. 1961. (p. 236-44)

43. INDUSTRIAL SCALE RECTIFICATION OF HYDROGEN. Scholz W.Kältetechnik 13,184-8,1961.

44. DISTILLATION OF HYDROGEN ISOTOPE MIXTURES. INDUS­ TRIAL MANUFACTURE OF DEUTERIUM WITH LOW TRITIUM CONTENT. Coulon A., Simonct G. A., Stouls L. (CEA, Paris, FRANCE). Problems of Low Temperature Physics and Thermo-- dynamics. New York, Macmillan Co. Vol. 3, 1962. p. 45-63. (In French). (Rev. Gen. Froid 39, No. 11, 1305-15, 1962) 171

45. PRODUCTION OF HEAVY WATER BY THE LOW TEMPERA - ' TURE DISTILLATION OF HYDROGEN. Banikiotes G. C., Cimler E., Sze M. C. Chem. Eng. Progr., Symp. Sor. 58, 17-25, 1962.

46. INDUSTRIAL PRODUCTION OF DEUTERIUM POOR IN TRITIUM. Coulon A. (Office Nat. Industrial de l'Azote, Toulouse, FRANCE). Stouls L. .Simonet G. Ind. At. 6, 81-93, 19G2. (In French)

47. HEAVY WATER AS A BY-PRODUCT OF LIQUID HYDROGEN PRODUCTION. Vandcr Arene! P.C. Chcm. Eng. Progr. 59, No. 8, Aug. 19G3.

48. THE SEPARATION OF DEUTERIUM BY THE DISTILLATION OF LIQUID HYDROGEN ON A LARGE SCALE. Lchmev W. Technology and Uses of Liquid Hydrogen. Porgamon Press 1964. (p.341-58)

49.. INDUSTRIAL ACHIEVEMENTS OF LIQUID HYDROGEN DISTIL­ LATION. Lehmer W. Inst. Int. du Froid.Cours sur l'Hydrogéne Liquide, Grenoble 1965. (p. 283-93) (Pure Appl.Cryog. 5, 283-93, 1966)

50. HYDROGEN PRODUCTION AND LIQUEFACTION. Newton C. L. Cliem. Process. Eng. 48, No. 12, 51-8, 1967.

•r'l. EXPOSE ON TECHNICAL DEVELOPMENTS OF THE LOW TEMPERATURE PROCESS FOR HEAVY WATER RECOVERY AND ITS ECONOMIC RESULTS. Gutonsky E. T. K. (Linde A. II., Munich, W. GERMANY).CNEN Synip. on Tech. and Econ. Aspects of Heavy Water Production,'Turin, Italy, Sept.. 30-Oct. 1, 1970. 173

ACTUAL INDUSTRIAL PROCESSES 2 - Distillation 2 - Distillation of Water

SEPARATION OF THE ISOTOPIC FORMS OF WATER EY FRACTIONAL DISTILLATION. Lewis G. N., Cornish R. E. J.Am.Chem.Soc. 55, 2616-7, 1933.

THE ISOTOPIC FRACTIONATION OF WATER BY DISTIL­ LATION AND BY ABSORPTION."Washburn B.W..,Smith E. R. J. Chom. Phys. 1, 426, 1933.

THE ISOTOPIC FRACTIONATION OF WATER(Rcsearch Paper No. 601). Washburn E. W., Smith E. R., FrandÉen M. J. Res. NBS 11,453-62,1933.

ISOTOPIC FRACTIONATION OF WATER BY DISTILLATION. H&ll N. F., Jones T. O. J. Am. Chem. Soc. 56, 749-50, 1934,

INCREASE OF THE PERCENTAGE OF DEUTERIUM IN WATER DURING VERY SLOW EVAPORATION. Tucholski T. Nature 134,29, 1934. 174

CONCENTRATION OF HEAVY WATER BY SPONTANEOUS EVAPORATION. Hughes E. D., Ingoici C. K., Wilson C. L. Nature 134, 142, 1934.

THE ISOTOPIC FRACTIONATION OF WATER DUE TO EVA­ PORATION AND DISTILLATION. I-Iarada M., Titani T. BuU. Chem. Soc, Japan 10, 41-2,1935.

ISOTOPIC SHIFT OF WATER BY DISTILLATION. Horiuchi J., Oka moto G.' Bull. Chom. Soc. Japan 10, 503-5, 1935.

DISTILLATION AND RECTIFICATION OF DILUTE SOLUTIONS OF VOLATILE COMPOUNDS. I. THEORETICAL STUDY AND ..• APPLICATION TO THE CASE OF HEAVY WATER. Jaulmes P. Chimie et Industrie 33, 1045-52,1935.

VAPOR PRESSURES OF THE ISOTOPIC FORMS OF WATER. Wahl M. H., Urey II. C. J. Chem. Pliys. 3, 411-4, 1935.

THE CONCENTRATION OF HEAVY WATER IN A STEAM BOILER. Stumper R. Vom Wasser 10, 207-8, 1935.

THE EFFECT OF ISOTOPES IN ION AND THE HEAT OF SOLUTION. Largo E.,Martin W. .Sattler H. Z. Ges.Naturw. 1., 441-2, 1930. (In German)

CAN THE DIFFERENCE IN DENSITY BETWEEN SEA WATER AND FRESH WATER BE EXPLAINED BY THE FRACTIONAL DISTILLATION OF THE .WATER ISOTOPES. Neumann K. , Toh m lor G. Z. physik. Chem. A 176, 226-3, 1936. (In German) 175

14. THE SEPARATION OF ISOTOPES BY RECTIFICATION AND RECTIFICATION AS A METHOD OF PURIFYING GASES. 7th Congr. Int.'.. Froid. 1st Comm. Int. Rapports ot Communic. June 1936.(p. 103-11)

15. ON CALCULATION OF THE NUMBER OF STAGES, REFLUX RATIO AND RATIO OF SEPARATING AGENT TO FEED. VerterssianK.A.,Fenskc M.,11. Incl.Eng. Chem. 29, 270, 1937..

Ig. (On D2O Separation by Distillation). Guinot II., Clark F. W.. Trans. Inst. Chem. Engrs (London) 16,189-99,1938.

17, SEPARATION PROCESSES. SEPARATION OF ISOTOPES BY FRACTIONAL DISTILLATION OF WATER. Randall M., Webb W. A. Ind. Eng. Chem. 31, 227-30, 1939.

18; (On D2O Separation by Distillation). Smith D. M. , Bryant W. M. D. , Mitchell J. Jr. J. Am. Chem. Soc. 61, 2407,1939.

19< (On Heavy Water Separation by Distillation). Wentworth T. Q. Othmer D. F. Irans. Am. Inst. Chem. Engrs. 3G, 785-99, 1940. ' ' (Ind. Eng; Chem. 32,1588-93, 1940)

2 0 : (On D2O Separation by Distillation). Othmer D. F. Chem. and Met. Eng. 48, 91-4,1941. 1.76

21, (On D2O Separation by Distillation). Keyes D. B. Ind. Eng. Chem. 33, 1019-21,1941.'

22. (On D2O Separation by Distillation). Natta G., Matter G. I. ehem. To elm. Berlin, Ver. Chem. App. 16,201-4,1943.

23, (On D2O Separation by Distillation). Wentworth T. O., Othmer D. F., Pohler G. M.' Trans. Am.'Inst. Chem. Engrs. 39, 565-78, 1943.

24. APPLICATION OF DIFFERENTIAL, SOLUBILITY TO WATER •SEPARATION. Huffman J. R. SAM Report 3 R-60. Feb. 1, 1943.

25, (On D2O Separation by Distillation) Scatchard G., Bridgforth R. M. Jr., Sheffield.E. L. Columbia University Reports: A-588,Apr.'l3,1943;A-598, May 12, 1943;A-733, June 14,1943; A-759, July 27,1943.'(Final Report from MIT Group).

26. (On D2O Separation by Distillation). Hutchison C. A., Lyon A, M. .Columbia Univ. Report A-745. July 1,1943.

27. {On D20 Separation by Distillation). Ewell 11, II,, Harrison J, M., Berg L. Ind. Eng. Chem..36, 871-5, 1944. 177

(On D2O Separation by Distillation). Francis A. W. Ind. Eng. Chem. 3G, 1096-104, 1944.

(On D2O Separation by Distillation). Colburn A. P., Phillips J. C. Trans. Am. Inst.Chem. Engrs. 40, 333-59, 1944.

(On D2O Separation by Distillation). Berg. L., Harrison J. M., Montgomery.G. W. Ind. Eng. Cherh. 37, 585-7,1945.

(On D20 Separation by Distillation). Ewell R. II., Welch L. M. Ind.Eng. Chom. 37,1224-31, 1945.

(On D2O Separation by Distillation). Lake G. R. Trans. Am. Inst. Chem. Engrs. 4.1, 327-52,1945.

(On D2O Separation by Distillation). Benedict M., Rubin L. C. Trans. Am. Inst. Chem. Engrs.41, 353-70, 1945.

(On D2O Separation by Distillation). Benedict M., Johnson C. A. , SolomoivE., Rubin L. C. Trans. Am. Inst. Chcm. Engrs. 41, 371-92,1945.

(On D2O Separation by Distillation). Colburn A. P., Shoenborn E. M. Trans. Am. Inst. Chem. Engrs. 41,421-43, 1945.

(On D20 Separation by Distillation). White R. R, Trans. Am.. Inst. Chem. Engrs. 41, 539-41, 1945. 178

(On D2O Separation by Distillation). Drickamer H. G., Brown G. G., White It. R. Trans. Am. Inst. Chom. Engrs. 4.1, 555-629, 1945.

(On D2O Separation by Distillation)Dunn C. L., Miller R. W., Picrotti G. J., Shires R. N., Souclors M. Jr. Trans. Am. Inst, Chem. Engrs. 41, G31-44,1945.

(On D2O Separation by Distillation). Updike O. L. Jr., Langdon W. M.,Keycs B.D. Trans. Am. Inst. Chom. Engrs. 41, 717-36, 1945.

(On D20 Separation by Distillation). Dicks R. S., Carlson C. S, Trans. Am. Inst. Chom. Engrs. 41, 788-803, 1945.

(On D2O Separation by Distillation). Wohl K. Trans. Am. Inst. Chom. Engrs. 42, 215-49, 194G.

THE PREPARATION OF HIGH-PURITY HYDROGEN DEU- TERIDE. Fookson A., Pomcrantz P., Rich E.H. Science 112, 748-9,1950.

SEPARATION OF ISOTOPES BY FRACTIONAL DISTILLA­ TION. Dostrovsky I., Gillis J., Llewellyn D. R. Bull. Research Council Israel 1,120-1, 1951. (L. Parkas'Mem. Vol. G2-94, 1952)

STUDIES ON ISOTOPES. I. THE ISOTOPIC COMPOSITION OF WATER WHICH HAS BEEN ENRICHED IN HEAVY ISOTOPES BY FRACTIONATION. Mackenzie II. A. E., Milnor A. M. J. S. African Chom. Inst. 4, 57-62, Juno 1951. 179

45. STUDIES ON ISOTOPES. II. THE APPROACH TO ISOTOPIC EQUILIBRIUM DURING FRACTIONAL DISTILLATION WITH APPRECIABLE HOLD-UP IN THE STILLPOT. Mackenzie I-I.A.E,, Malherbe P.N. J. S.African Chem. Inst. 4, 63-8, 1951.

46.' SEPARATION OF D2O/H2O BY HIGH TEMPERATURE DISTIL­ LATION. Mills G. F. (Carbide and Carbon Chemicals Co. K-25 • Plant, Oak Ridge, Tenn. USA). KLI-1098. Sept. 26, 1951. Deci. Oct. 17,1955.

47. THE SEPARATION OF ISOTOPES BY FRACTIONAL DISTIL­ LATION. II. DETERMINATION OF PARAMETERS FROM PRO­ DUCTION DATA. VALUE OF THE UNIT PROCESS SEPARATION 1G 18 FACTOR FOR THE H2 0-Il2 0 SYSTEM. Dostrovski I., Gillis J., Llewellyn D. R., Vromen B.H. J. Chom. Soc. 3517-24, 1952.

48. THE CHEMICAL METHOD OF ISOTOPE SEPARATION AS A RECTIFICATION PROBLEM. Becker E. W., Bier K. Z. Naturforsch 7a, G51-64, 1952. (In German) (AEC-tr-5527)

49. PREPARATION OF LIGHT WATER BY DISTILLATION. ITS COMPOSITION AND THE DENSITIES AND FRACTIONATION FACTORS OF ITS ISOTOPES. Watson H.E. J. Appi. Chem. (London) 3,556-63,1953.

50j THE ENRICHMENT • OF HEAVY WATER BY FRACTIONAL DISTILLATION. Ehrcnbcrg W., Jaffkc H. Z. angew. Phys. 5, 375-6, 1953. (In German) (AERE-Lib/Trans-49G) 180.

51. VAPOR PRESSURE STUDIES INVOLVING SOLUTIONS IN LIGHT AND HEAVY WATERS. I.'THE APPARATUS AND DE­ TERMINATION OF VAPOR PRESSURES AT 30°C OF SOLU­ TIONS OF SODIUM AND POTASSIUM CHLORIDES IN ORDI­ NARY WATER. II. THE VAPOR PRESSURE OF HEAVY WATER AND THE SEPARATION FACTOR OF THE MIXED WATERS. Combs R. L. , Googin J. M. , Smith I-I. A. J. Chem. Phys, 58, 997-1001, Nov. 1954.

52. HEAVY WATER PRODUCTION BY NATURAL WATER DISTIL­ LATION. I. GENERAL CONSIDERATIONS. Rac II. K. (Atomic ' Energy of Canada Ltd. Chalk River Project, Chalk River, Ont. CANADA). CEI-73, Oct. 1, 1954. (AECL-322)

53. HEAVY WATER PRODUCTION BY NATURAL WATER DISTIL­ LATION. II. Preliminary Cost Estimate. Rae K. H. , Stenning A.H. AECL-323.1954.

54. THE PRODUCTION OF HEAVY WATER BY DISTILLATION OF ORDINARY WATER. Pratt.II. R. C. Proc.Symp. on Heavy Water. Rome, Mar. 31-Apr. 2, 1955. CNRN Roma, 1955.

55.' HEAVY WATER PRODUCTION BY NATURAL WATER DISTIL­ LATION. III. WETTED-WALL COLUMN DEVELOPMENT. Bancroft A. R., Rae II. K. (AECL, Chalk River Project, Chalk River, Ont.'CANADA). CRCE-G08.' July 1955.'(AECL-230)

Proceedings of the International Conference on the Peaceful Uses of Atomic Energy, Geneva 1955: 56. FINAL CONCENTRATION OF HEAVY WATER BY RECTIFI­ CATION, Baertschi P. , Kuhn W. 8, P/927. (SWITZERLAND)

57,' TEMPERATURE DEPENDENCE OF THE DEUTERIUM DISTRIBUTION IN THE REACTION LiAlH4+4HDO. Savie P., Dogramadzi N. , Novakovic M. 8, P/960. (YUGOSLAVIA) 181

58. ISOTOPIC ENRICHMENT BY SLOW EVAPORATION OF WATER. Knop L., Stern F. J. Stefan Inst, Ropts. (Ljubljana) 3,149-50,1956.

59. THE FINAL CONCENTRATION OF HEAVY WATER BY RECTIFICATION. Progress in Nuclear Energy - Series 4: Technology and Engineering. McGraw Hill Co. New York 195G.(p.57-Gl)

6 0. VAPOR PRESSURE STUDIES INVOLVING SOLUTIONS IN LIGHT AND HEAVY WATERS. III. THE SEPARATION FACTOR FOR THE ISOTOPES OF HYDROGEN DURING DISTILLATION FROM SALT SOLUTIONS IN THE MDCED WATERS AT ROOM TEMPERATURE. Googin J. M., Smith II. A. (Univ. of Tennessee, Knoxville, USA). J. Phys. Chem. 61,345-50, Mar. 1D57.

61. SEPARATION OF HYDROGEN ISOTOPES BY MULTI- COMPONENT DISTILLATION. Flynn T. M., Timmerhaus K. D., Weitzel D. II., Draper J. W. Proc. 2nd Cryogenic Eng.Conf., Boulder Col. USA.56-63, 1957.

62. CONCENTRATION OF HEAVY WATER BY DISTILLATION AND ELECTROLYSIS. Bebbington W. P., Thayer V.'R. (Du Pont de Nemours E.I. &Co. ).4, P/1065. (USA). 2nd UN Geneva Conf. 1958.

63. APPLICATION OF THE ISOTOPIC EFFECT AT THE SEPAT RATION OF.IGO AND 180 ISOTOPES DURING RECTIFICA­ TION OF HEAVY AND LIGHT WATER. Baertschi P., Thllrkauf M. Helv. Chim. Acta 43, 80-9,1960.

64. SEPARATION OF HYDROGEN ISOTOPES BY DISTILLING AZEOTROPE'MIXTURES OF STRONG BY MEANS OF WATER. I. THEORY OF SEPARATION METHOD. Wetzel K. Isotopentechnik .1, .1.5-8, lOfiO. • 182

THE SEPARATION OF MIXTURES OF ORDINARY AND HEAVY WATER BY ZONE REFINING. Smith II. A., Thomas CO. J. Phys. Chem. 63, 445-7, 1959.

THE SEPARATION OF HYDROGEN ISOTOPES BY DISTIL­ LATION OF AZEOTROPIC ACID-WATER MIXTURES. Wetzel K.,Schlitze II., Kretzchmann G., Mllhle K.' (Inst, für physikalische Stofftrennung, Leipzig, E. GERMANY). Naturwissenschaften 47, 374, 19G0. (In German)

DISTILLATION OF ISOTOPIC MIXTURES IN A PROFILED REGIME. Barb D., Bucur R. , Olai^iu A. Stud. Cercet. Fiz. (Bucharest) 12,879-91,1961.

THE BEHAVIOUR OF FILLING MATERIAL INTERFACES IN ISOTOPE SEPARATION BY DISTILLATION. Krcll E. Kernenergie 5, 242-5, 19G2. (In German)

COMPARISON OF DIFFERENT METHODS FOR THE DE­ TERMINATION OF THE SINGLE STAGE SEPARATION FACTOR IN SEPARATION OF HYDROGEN ISOTOPES BY EXCHANGE DISTILLATION. Kretzchmann G., Wetzel K., Schlitze li., Mllhle K., Habedank M. Kernenergie 5, 258-61, 1962. (In German)

D20 PRODUCTION BY LOW PRESSURE, PERIODIC RECTI­ FICATION. Dorabialska A., Swiatknwski W. (Lodz Tech. Univ.. POLAND). Zeszyty Nauk Politech. Lodz. , Chem. 12,61-7, 1962. (In Polish)

LOW TEMPERATURE STILL FOR SEPARATION OF HYDRO­ GEN ISOTOPES. Johnson B. S., Rust F. G. D. DP-73C. Sept. 1962. 183

.72. ISOTOPIC FRACTIONATION DURING THE DISTILLATION OF WATER. Merlivat L., Botter F. , Nief G. J. Chim. Phys. GO, 56-9,1963. (In French)

.73. ENRICHMENT OF DEUTERIUM DURING DISTILLATION. Petersen G. I., Benedict M. Nucl. Sei. Eng. 15, 90-7,19G3.

74. A DISTILLATION METHOD WITH LIMITING CONDITIONS FOR THE DETERMINATION OF THE ISOTOPE SEPARA­ TION PARAMETER. Kroll E., Thiol S. Abh. Deut. Wiss. Berlin, Kl. Chem., Geol. Biol. 7, 89-91,19G4.

75. INVESTIGATION OF VACUUM RECTIFICATION WITH THE SPIRAL-TYPE EXCHANGE ELEMENTS OF THE KLOSS DESIGN. Bcvcrs K. Chcm.Ing. Tech. 3(5, No. 3, 217-21,19G4. (In German)

7G. THEORETICAL CONSIDERATIONS ON THE PRODUCTION OF HEAVY WATER BY RECTIFICATION. Otero de la Gan- dara J. L., Alvarez Gonzalez J. R. Energia Nucl. (Madrid) .8, 2G-37, Jan. -Mar. 1.9G4. (In Spanish)

77. A NEW DISTILLATION TECHNIQUE FOR ISOTOPE CON­ CENTRATION. Silvestri M., Angelino G. C., Brigoli B. (CISE, Milan) 12, P/557. (ITALY). 3rd UN Geneva Conf. 19G4.

78. DETERMINATION OF THE SEPARATION COEFFICIENT OF HDO AND D20 BY DISTILLATION. Ceccaldi M., Riedinger M. CEA. March 29, 19GG. (DPC. SIS. SSM/GG-43/MC/FP) 184

79. FINAL RECTIFICATION OF HEAVY WATER IN THE BATCH PRODUCTION METHOD. Gispert Bennach M., Rojas de Diego J. L. , Echavarri T., Ortcgo J. M. An.Quim. 64, 869-78, 1968.

80.' PREPARATION OF HEAVY WATER. IV. FINAL CASCADE RECTIFICATION. Gispert M., Rojas J. L. Encrg. Nucl. ' (Madrid) 12,27-39, 1968.

81. STUDIES ON HEAVY WATER PRODUCTION CASCADE. FINAL RECTIFICATION. Gispert M., Rojas J.L. Encrg. Nucl. (Madrid) 12, 51, 1968.

82. PROPOSED ANALYSIS-D20 DISTILLATION USING LOW COST STKAM. Young J. R. Pac. Northwest Lab. 1967. Unpublished data.

83. SUITABILITY OF WATER-HEAVY WATER SYSTEM AS TEST MIXTURES IN DISTILLATION COLUMNS. Lentz H., Wagner H. G. Ber. Bunsenges. Phys. Chcm. 73, 66-8, 1969.

84. LOW-COST HEAVY WATER PRODUCTION BY WATER DISTILLATION. Böhme D. W., Young J. R. (Battelle North­ west, Rich. Wash. USA) Trans. Am. Nucl. Soc. 12, 496-7, Nov. 1969: 185

C - ACTUAL INDUSTRIAL PROCESSES 3 - Electrolysis of Water

CONCENTRATION OF THE H2 ISOTOPE OF HYDROGEN BY THE FRACTIONAL ELECTROLYSIS OF WATER. Washburn E. W. ,Urey H. C. Proc. Nat. Acad. Sci. 18,496-8, 1932.

ISOTOPES OF HYDROGEN. Lewis G. N. J. Am. Chem. Soc. 55, 1297-8,1933.

CONCENTRATION OF THE HEAVY HYDROGEN ISOTOPE. Newell J. L., Ficklen J. B. Jl Am. Chem. Soc. 55, 2167, 1933.

ELECTROLYTIC SEPARATION OF HYDROGEN ISOTOPES AND THE MECHANISM OF THE CATHODE PROCESS. Topley B., EyringH. J. Am. Chem. Soc. 55, 5058-9, 1933.

THE ISOTOPIC FRACTIONATION OF WATER. Washburn E.W., Smith E. R., Frandsen M. J. Chem. Phys. 1, 288, 1933. (J. Res. NBS 11,453-62, 1933. Res..Paper No. GOO)

CONCENTRATION OF THE H2 ISOTOPE. Lewis G. N. , McDonald R.T. J. Chem. Phys. 1,341-4, 1933.

THE CONCENTRATION OF DEUTERIUM BY ELECTROLYSIS. Rank D.H. J. Chem. Phys. 1, 750-1, 1933.

TECHNIQUE FOR THE ELECTROLYTIC PRODUCTION OF D2O. Taylor H.S.,Eyring H. , Frost A. A. J. Chem. Phys. 1, 186

9. THE ELECTROLYTIC ISOLATION OF THE HEAVIER HYDROGEN ISOTOPE BY G. II. LEWIS. Polanyi M. Naturwiss. 21, 316-7, 1933.

10. A CASCADE ELECTROLYTIC PROCESS FOR SEPARATING THE HYDROGEN ISOTOPES. Urey H. C. , Wahl M. II. Phys. Rev. 43, 566,1933.

11. ZERO-POINT ENERGY AND THE SEPARATION OF ISOTOPES. Eyring H. Proc. Nat. Acad. Sci. U.S. 19, 78-81, 1933.

12. CONCENTRATING HEAVY WATER. Brodskii A. I., Alcksandrovich V. A, ,Slutskaya M. M,, Shelud'ko M. K. Compt. Rend. Acad. Sci. URSS 3, 615-7, 1934.

13. CONCENTRATION OF THE HEAVY HYDROGEN ISOTOPE BY ELECTROLYSIS. Erleinnayer IJ., Gartner H. Hciv. Chun. Acta 17, 30-1,1934.

14. THE MANUFACTURE OF DEUTERIUM AND ITS COMPOUNDS. Webb W.A. Chem.Eng. 12,63, 1934.

15. ISOTOPIC FRACTIONATION OF HYDROGEN. Hunt H. J.Chem. Phys. 2 Phys. 2, 106, 1934.

16. THEORY OF THE ELECTROLYTIC SEPARATION OF ISOTOPES. Bell R. P. J.Chem. Phys. 2, 164-6, 1934.

17. SEPARATION OF-THE HYDROGEN-ISOTOPES BY ELECTRO­ LYSIS. Topley B., Eyring H. J. Chem. Phys. 2, 217-30, 1934.

18. THE SYSTEMATIC CALCULATION AND THE TECHNIC OF SEPARATION OF HEAVY WATER. Goldfinger P.,Scheepers L. J. Chim. Phys. 31, 628-46, 1934.

19. THE ELECTROLYTIC PRODUCTION OF HEAVY WATER. Hori Y. Elektrochem. Assoc. Japan 2, 290-7, 1934.

20. FRACTIONATION OF ISOTOPES OF HYDROGEN AND OXYGEN IN A COMMERCIAL ELECTROLYSER. Washburn E. W. , Smith E.R., Smith F.A. J. Res NBS 13, 599-608,1934. (Res. Paper No. 72.9) 187

21-, CONCENTRATION OF DEUTERIUM BY THE ELECTROLYSIS OF WATER. I. Ota Y, Mem. Faculty Sci. Agr. Tailioku Imp. Univ. 10, 71-9,1934.

22. ELECTROLYTIC CONCENTRATION OF DEUTERIUM. Dell R. p., Wollenden J. II. Nature 133, 25-G, 1934.

23. ELECTROLYTIC CONCENTRATION OF THE HEAVY HYDROGEN ISOTOPES. Topley B., Eyring II. Nature 133, 292, 1934.

24i ENRICHMENT OF THE HEAVY HYDROGEN ISOTOPE. Uhlmann W. Naturwiss. 22, 199-20, 1934.'

25, A CASCADE ELECTROLYTIC PROCESS FOR SEPARATING THE HYDROGEN ISOTOPES. An Abstract. Urey H. C. , Wahl M. II. Pliys. Rev.45,56G,1934.

2G PREPARATION OF HEAVY HYDROGEN. Harteck P. Proc.Phys. Soc. (London) 46,277-80,1934.

27. GENERAL CONSIDERATION ON THE THEORY OF THE SEPARA­

TION OF Hi AND H2 BY ELECTROLYSIS OF WATER. Fowler R. H. Proc, Roy, Soc. (London) A 144,452-66,1934.

28. EXPERIMENTS ON HEAVY HYDROGEN. III. ELECTROLYTIC SEPARATION OF HYDROGEN ISOTOPES. FarkasA.., Parkas L. Proc. Roy.Soc. (London)A 146,623-9,1934.

29. ATTEMPTS TO INCREASE THE HEAVY HYDROGEN ISOTOPE WATER. Gllnterschulze A,. Keller F. Z.Elektrochem. 40, 182-3, 1934.

30. THEORETICAL AND'EXPERIMENTAL STUDIES ON THE METHOD ON OBTAINING HEAVY WATER. Kami enski B. Roczniki Chem 14, 401-5,1934.

31; METHOD OF OBTAINING DEUTERIUM OXIDE FROM WATER BY ELECTROLYSIS. Schwartz K., KÜchler L., Steiner H. Z. Elektrochem. 40, 298-9, 1934. IB«

32.. ELECTROLYTIC ENRICHMENT OF THE HEAVY HYDROGEN ISOTOPE IN WATER. Tronstad L. , Brim J. Z. Elektischem. 40, 556-8, 1934.

33. EFFECT OF ON THE CONCENTRATION OF HEAVY WATER. Brodskii A. I., Skrinnikova II. P. Acta Physico- chim. URSS 2, B0n-10, 1935.

34. (On D2O Separation) SclwoocI P. W. , Taylor H. S., Hippie J. A. Jr. , Bleakney W. J. Am. Chcni. Soc. 57, 642, 1935.

35. ELECTROLYTIC SEPARATION OF THE HYDROGEN ISOTOPES. Halporn O. .Gross Ph. J. Cheni. Phys. 3, 452-G, 1935.

36. ELECTROLYTIC PRODUCTION OF HEAVY WATER. RELATION BETWEEN CURRENT DENSITY AND ISOTOPE SEPARATION COEFFICIENT. Noguchi T. J. Elcktroclicm. Assoc. , .Japan 3, 505-10, 1935.

37. CONCENTRATING THE HYDROGEN ISOTOPE, D, BY E LECTRO- LYSIS OF WATER. H. PRODUCTION OF HEAVY WATER AND AP­ PARATUS. Ota Y. Mem. Faculty Sci. Agr. Taihoku Imp. Univ. 15, 165-70, 1935.

38. EFFICIENCY OF SEPARATION OF HYDROGEN AND DEUTERIUM BY ELECTROLYSIS. Oddie T. H. Proc. Pliys. Soc. (London) 47, 1060-7, 1935.

39. THE ELECTROLYTIC SEPARATION FACTOR OF THE HYDRO­ GEN ISOTOPES UNDER VARIOUS EXPERIMENTAL CONDITIONS. Eucken A. .Bratzlcr I-I. Z. phys, Chem, A 174,273-90, 1935.

40. CONCENTRATING HEAVY WATER. Brodskii A. I., Aleksandrovich V. A. , Slutskaya M. M., Shol-'d'ko M. K. Ber. Inst. Physik. Chem. Akad. Wife's. Ukr. SSR 5, 151-4, 1936.

41. THE ELECTROLYTIC SEPARATION OP DEUTERIUM. Edwards A. J. , Walton II. F. , Boll R. P. , Wollenden J. H. J. Chem. Soc. 286-7,1936 ' 189

42. THERMAL CONDUCTIVITY METHOD FOR FOLLOWING THE ELECTROLYTIC SEPARATION OF HYDROGEN ISOTOPES. Newell W. C., Purccll R. I-I., Gregory H. S., Ellingham H. J. T. Nature, 3 37, 6.9-70, 1936.

^3. TEMPERATURE COEFFICIENT OF ELECTROLYTIC SEPARA­ TION OP THE HYDROGEN ISOTOPES. Walton H, F., Wolfenden J. I-I. Nature 138,468,1935.

44. THE RELATIVE EFFICIENCIES OF THE MULTISTAGE AND ONE-STAGE PROCESS IN THE ELECTROLYTIC PREPARATION OF HEAVY WATER. Chiplonkar T. Proc. Indian Acad. Sci. 4 A, 463-7,1936.

45. THE NATURE OF OVERVOLTAGE AND THE ELECTROLYTIC SEPARATION OF HYDROGEN ISOTOPES.Horiuchi J. ,Okamoto G. Papers Inst. Phys. Chem. Res. (Tokyo) 28, 231-42, 1936.

46. THE ELECTROLYTIC SEPARATION FACTOR OF DEUTERIUM AT VERY LOW CONCENTRATIONS. Walton II. F. .Wollenden J. A. J.Chem.Soc. 1677-9,1937.

47. POLAROGRAPHIC STUDIES WITH THE DROPPING-MERCURY CATHODE. LXX.-HYDROGEN OVERVOLTAGE IN MIXTURES OF LIGHT AND HEAVY WATER AND THE SEPARATION COEF­ FICIENT. Heyrovsky J. Collection Czechoslov. Chem. Communs. 9,345-59,1937.

45. AN EFFECT OF RECTIFIED CURRENT FROM A TUNGAR VALVE UPON THE ELECTROLYTIC SEPARATION OF HEAVY WATER. Asada T. , Honde E. Nature 139, 885-6, 1937.

49. SIMPLE EQUIPMENT FOR ELECTROLYZING HEAVY WATER. Slack C. M. ,Ehrke L. F. Rev.Sci. Instr. 8, 39, 1937.

50. THE ELECTROLYTIC SEPARATION OF THE HYDROGEN ISO­ TOPES ON A PALLADIUM CATHODE.'Farkas A. Trans. Faraday Soc.33,552-9,1937. 1 yo

51. ELECTROLYTIC WINNING OF HEAVY WATER. IV. Noguchl T. J.Electrochom.Ass. Japan 6, 299-303, 1938, (Rov. PhyB. Chom. Japan 13,50, 1930)

52. THE ELECTROLYTIC SEPARATION OF DEUTERIUM: THE INFLUENCE OF TEMPERATURE AND CURRENT DENSITY AT VARIOUS CATHODE METALS. Walton II. F., Wolfendon J. II. Trans. Faraday Soc.34,436-49,1938.

53. PREPARATION OF HEAVY WATER. Al.cksiinclrovi.ch V. A. , Sliclud'ko M. K. Zliur. Priklad. Khim. 13,483-9«, 1940.4(In Russian)

54. PRODUCTION OF D20 FOR USE IN THE FISSION OF URANIUM. Urcy II. C. .Grosse A. V., Waiden G. A-94.Junu 23, 1941. Deci. May 21, 195G.

55. ELECTROLYSIS AT CONSTANT VOLUME OF A MIXTURE OF LIGHT AND HEAVY WATER. Savard J. J. Phys. Radium {Gì 5, 85-9, 1944.

5ß. KINETICS OF IONIC DISCHARGE AND IONIZATION OF ADSORBED DEUTERIUM ATOMS ON A PLATINUM ELECTRODE. Jtozental K.I., Dolin P.I., Ershlcr B. V.' J. Phys. Chom. URSS 19, 601-14, 1945;

57.. KINETICS OF THE DISCHARGE OF DEUTERIUM IONS AND IONIZATION OF ADSORBED DEUTERIUM ATOMS ON PLATINUM ELECTRODE. Rozental K. I., Dolin P. I., Ershlor B.V. Acta Physi- cochim.URSS 21,213-34, 194G.

58. CONCENTRATION OF ISOTOPES THROUGH ELECTROLYTIC TRANSFER IN AQUEOUS SOLUTIONS.Klomm A. Z.Naturforsch. 3a, 127-8, 1918.

59. ELECTROLYTIC CONCENTRATION OF HEAVY WATER. I. THEORY. Orsoni L., Silvestri M. (Milan, ITALY). CJSE-16. 1950. (In Italian)

GO. ACCUMULATION OF HEAVY WATER BY COUNTER-CURRENT ELECTROLYSIS. Martin II., Ruhtz E. Z. Elektrochem. 54, 5G0-G, 1950. (In Gorman) (AEC-tr-lG87) 191

61.. THE SIGNIFICANCE OF. ISOTOPIC REACTIONS IN RATE THEORY. Eyriug II., Cagle F. VV. M. Jr. J. Phya. Chcm. 5.G, B.89-1'2, 1952.

62.. THE EFFECT Ol' NITRATE-ION AND AMMONIA ON THE ELECTROLYTICAL SEPARATION OF HYDROGEN-DEUTERIUM ISOTOPES. Hojman J. M. Bull. Inst. Nucl.Sci. Boris lüdrieh (Belgrade) 3,121-G, 1953.

G3 INFLUENCE OF THE TEMPERATURE ON THE ELECTROLYTIC SEPARATION OF HYDROGEN ISOTOPES. Brun J., Varbcrg Tli. Kgl. Norske Videnskab.'. Selskabs., Forh. 26,19-21, 1953.

G4. THEORETICAL ASPECTS OF THE ELECTROLYTIC METHOD OF PREPARING HEAVY WATER. Subramanian G.S. Bull. Contrai EIcctrochem. Res. Inst. Karaikudi 2, No. 2,65-U, 1Ü55.

G5. INFLUENCE OF OXYGEN ON THE ELECTROLYTIC SEPARATION OF HYDROGEN ISOTOPES. Brun J., Andreassen K. Kgl. Norsko Videnskab. Solskabs. Fori). 28, No. 1, 1-4, 1955.

66. ELECTROLYTIC CONCENTRATION OF HEAVY WATER. Okajinia Y., Yoshikawa Y., Doug Zwig llan. Nip-ion Kcgaku Zasshi 7G, 1370-4, 1955.

.67.. MODIFICATION IN THE ELECTROLYTIC AND EXCHANGE REACTION PROCESS FOR THE PRODUCTION OF HEAVY WATER. Otero de la Gandara J. L., Giapert J. 8, P/1120. (SPAIN). 1st Geneva Conf. 1955.

68. INFLUENCE OF THE CATHODE METAL ON THE SEPARATION OF HYDROGEN ISOTOPES. Brun J., Varberg Th., Gunderson W., Solli It. Kgl. Norste Videnskab. Selskabs. Forh. 29, 5-9,1956.

69. INFLUMCIS OF IMPURITIES ON THE ELECTROLYTICAL CONCEN­ TRATION OF HEAVY WATER. Brun J., Gundorson W., Varberg Th. (Technical Univ. of Norway, Oslo, NORWAY)'. Kgl. Norske Videnskab. Selskabs. Forh. 30, No. 5, 29-34, 1957. 192

70. PRODUCTION OF HEAVY WATER UNDER SEMI-INDUSTRIAL CONDITIONS. Czike K., Pod or P.'(State Ros. Inst, of Phys. ). Energia es Atomtech. 11, 503-G, 1958. (In Hungarian)

71. THE ELECTROLYTIC HYDROGEN DEUTERIUM SEPARATION FACTOR AND REACTION MECHANISM. Conway B.E. Proc. Roy. Soc. (London) A 247-, 400-19, 1958.

72. CORRELATION BETWEEN CATIIODIC OVERVOLTAGE AND THE SEPARATION EFFICIENCY FOR HYDROGEN ISOTOPES. Brun J., Gunclorscn W., Lnsson A.T. Kgl.Norskc. Videnskabs. Forh. 32, 68-73,1959.

73. MODIFICATION IN THE PROCESS FOR THE PRODUCTION OF. HEAVY WATER BY ELECTROLYSIS AND THE EXCHANGE- . REACTION. DECREASE IN THE STEAM CONSUMPTION. Gispert M., Otero J. L. (JEN, Madrid, SPAIN). An.Real. Soc. Espan. Fis. y Quim. (Madrid) Sor. B56, 559-G8, 19G0.(In Spanish) (CEA-tr-X-411)

74. THE SEPARATION OF HYDROGEN ISOTOPES BY ELECTROCHE­ MICAL EXCHANGE. Wetzel K., Schumann K.D. J. Prakt." Chem. 12, 140-5,1961.

75. HEAVY WATER. THE NORSK HYDRO PROCESS. Myhre K. Tidssk;. Kjemi, Bergvesen Met. 21, 204-8, 1961. 76. IMPROVEMENTS RELATING TO POWER CONSUMPTION IN THE ELECTROLYTIC PRODUCTION OF HEAVY WATER. Raman M.S.';,.' Datta R. L. .Chem. Age India 13, 343-5, 1962.

77.' ON THE INDUSTRIALIZATION OF THE ELECTROLYTIC CON­ CENTRATION METHOD OF HIGHLY ENRICHED HEAVY WATER. I. ELECTROLYTIC CONCENTRATION CASCADE AND . Masami Shimizu, Saburo Nito, Akishige Harada. Nippon Genshiryoku Gakkaishi 4, 180-7, Mar. 1962. (In Japanese)

78. ON THE INDUSTRIALIZATION OF THE ELECTROLYTIC CON­ CENTRATION METHOD OF HIGHLY ENRICHED HEAVY WATER. II. RECOMBINATION AND REMOVAL OF ALKALI. Masami Shimizu, Saburo Nilo, Akishige Harada.Nippon Gakkaishi 4, 211-7, Apr. 1962. (In Japanese) 193

NATURAL ISOTOPES. IV. SEPARATION BY THE METHOD OF ELECTROLYSIS. Selecki A. Przemysl Chem. 41, 293-G, 19G2. (In Polish)

THE ISOTOPE EFFECT ON HYDROGEN ELECTRODES. Lewis G. P. Thesis, Brooklyn, Polytechnic Inst. 1062.

PHYSICAL AND TECHNICAL ASPECTS OF REDUCING THE ENERGY REQUIRED FOR THE ELECTROCHEMICAL PRODUC­ TION OF DEUTERIUM. Winsel A.'(TH Brunswick, W. GERMANY). Chem. Ingr. Tech. 35, 379-85,.May 19G3.(In German)

THE .FRACTIONATION OF HYDROGEN ISOTOPES BETWEEN HYDROGEN IONS AND WATER. Gold V. Proc. Chem.Soc. 141-3, 19G3.

ISOTOPE ENRICHMENTS BY COUNTER-CURRENT ELECTRO­ LYSIS IN AQUEOUS SOLUTIONS. Theimann W., Wagener K. Z. Naturforsch. 18a, 228-35, 1963.

ELECTROLYTIC SEPARATION OF DEUTERIUM. EFFECT OF TEMPERATURE. Raman M.S., Kumar R., Datta R. L. (Indian Inst, of Science, Bangalore, INDIA). Z. Naturfosch. 18a, 347-50, Mar. 196 3.

ELECTROCHEMICAL OF WATER VAPOR IN . SOLID OXIDE ELECTROLYTE CELLS, III.'SYSTEM FOR ECONOMICAL HYDROGEN PRODUCTION. White D.W.,Spacil H. S. Electrochem. Society Meeting, Montreal, (CANADA), Nov. 9, 1968.

ELECTROLYSIS AD A METHOD FOR THE PRODUCTION OF HEAVY WATER. Vasaru G.,Bucur R.V. IFA-AG-2 (Cluj) Oct. 10, 1969 (Unpublished)

ISOTOPIC FRACTIONATION OF HYDROGEN IN THE WATER- ION SYSTEM. Znamirovschi V. Rev.Roum. Phys. 14, 175-81,1969.

LABORATORY ENRICHMENT OF HEAVY WATER BY ELECTRO­ LYSIS.'PART I.'DESIGN OF ELECTROLYTIC CELLS AND CAL- CULATIONOF THE MEAN CURRENT DENSITY. Hallaba E., illy A.I. M. (Atomic Energy Establishment, Cairo).'Isotopenpraxis 7, No. 10, 427-30, Oct. 1971. 194

89. LABORATORY ENRICHMENT OF HEAVY WATER BY ELECTRO­ LYSIS. PART II. EFFECT OF CURRENT DENSITY, CATHODE MATERIAL, AND TEMPERATURE ON THE SEPARATION FACTOR. Hallaba E., A.ly A. I. M. (Atomic Energy Establishment, Cairo). Isotopenpraxis 7, No. 11-12, 456-9, Nov.-Dec. 1971. i liyyi Ulli II Ì)!!i iii III IlIll-III 1 31 ilil i .! . III! II il i iiiji . 1! 1 i n n ili !I ini II |i • tfii in ij ml i jl-uii ;'ii HI! ititi. }i UJÜU Uè pilo t plan

„•al l pilo t plan ecal l pilo t plan il. planne d pilo t plan larg a pilo t plan unse r sonatruei l o n nip hi i 1 ii3.!»li! l'i I Il i lli.lhihm.8 L II i j s :• • :• * nil- i % • 1,.« ..; c.,, » S i - • ;. « « - 5 ;. - , , , » , , „ , . , J ; 5 li.s- I § ||g?|l|B|£|l£|| i ,||?S Si? E ES £ 1 ..»1 E|,| mi, ,ie \%n%%%n sllH I ] i 1 i!I iiMrllllli s ? lim ni ir" ni ì .miiiir.'ij.iiii-'ii filili I i1,= ! nil li i ! ! li ù HI \ h imi• K!ilih i'• itili (f. S= .5. s = s 3 . S R K SS S IV. D. 1. 1 - INDUSTRIAL HEAVY WATER PLANTS AS OF FEBRUARY 1974

N. C ountry Location Capacity Constructor o'r owner Remarks t/year Plants based on H2S/HDO Process

1. USA Savannah River 180 Gir ller-Lummus/Dupont In operation since 1952 Final enrichment: H20 distillation

2. Canada Glace Bay 360 Spevack-Burns & Roe/Deuterium In trasformation of Canada Ltd. Final enrichment: H2O distillation Start-up: 1975

3. Port Hawkesbury 360 Lummus/Can. G. E. Ltd. In operation since 1970 Final enrichment: ^OdistUlation (Sulzer)

4. Bruce 2x365 Lummus /Can. G. E. Ltd. In operation since 1973

5. India Kota 100 Dept. Of Atomic Energy Engineering. Start-up: 1975 Plants based on NHs/HD Process

6. India Baroda 67 Group. Eau Lourde Proced. One temperature process Ammoniac /Dept. of At.E nergy Start-up: 1974

7. Tuticorin 71 Group. Eau Lourde Proced. One temperature process Ammoniac/Dept. of At. Energy Start-up:1974

8. Talcher 63 Uhde/Dept. of Atomic Energy Dual temperature process Final enrichment: H2O distillation (Sulzer) Start-up: 1975

Plants based on Hi distillation

S. India Nangal 14 Linde/Dept. of Atomic Energy In operation since 1962

Plants based on Electrolysis

10. Norway 20 Norsk Hydro In operation since 1934 Final enrichment: H2O distillation

(IV.A-175) 199

PRODUCTION PI-ANTS 2 - Plants based on HgS / TIPO Process

THE OPERATION OF A DUAL-TEMPERATURE SINGLE STAGE TOWER FOR DEUTERIUM CONCENTRATION. Eidinoff M.L. , Hiskey C. F. (Columbia Univ., New York. Div. of War Research; USA). A-718. May28, 1943. Deci. Nov. 1, 195G.

DUAL TEMPERATURE HEAVY WATER PROCESS EVALUATION OF PROPOSED TESTING AND PRODUCTION PROGRAM AT WABASH ORDNANCE WORKS. (Girdler Corp. Gas Processes Div. Louisville, Ky. USA). NYO-681. Apr. 21, 1950. Deci. Feb. 27, 1957.

DANA PLANT TECHNICAL MANUAL. Part. I. Bebbington W. P., Keller W. R. (E. I. du Pont do Nemours ^v Co. USA). DPTM-1. Dec. 15, 1951.

THERMAL BEHAVIOUR OF COUNTER-CURRENT EQUIPMENT. Hull H.A., Pohl H.A. (Du Pont Co.AED, Wilmington, Del. USA). DP-97.Dec. 1954. Deci. Apr. 15, 1957.

INDIANA D20 PLANT OFF STREAM. Nucleonics 15, No. 1, R 12, Jan.1957.

AMERICAN HEAVY WATER PLANT TO SHUT DOWN. Atomics 8, No. 2, 39, Feb. 1957. 200

OECD D20 PLANT IN ICELAND? Atomwirtschaft 3, No. 1, 294,July 1958.

HEAVY WATER. Pari; 6. FLOWSHEETS, DESIGN AND COST ESTIMATION FOR 22 AND 3G t/year PRODUCTION PLANTS USING II2S PROCESS. Walker P. T., Lyon C. J., Handley D. , Hcnsley J. D. C., Pratt II. R. C. AERE-CE/R-2343. 1958.

SECOND D2O PLANT. Atomwirtschaft 4, No. 5, 222-3, May 1959.

A PRELIMINARY APPROACH TO THE CALCULATION OF A WATER-HYDROGEN SULPHIDE DUAL TEMPERATURE DEUTERIUM SEPARATING PLANT. Brigoli B., Villani S. (CISE, Milan, ITALY) Energia Nucleare (Milan) G, 784-92, Dec. 1959.

PRODUCTION.OF HEAVY WATER. SAVANNAH RIVER AND DANA PLANTS. Technical Manual. Bebbington W. P. , Thayer V. R. eds.(Du Pont de Nemours E.I. &Co. Savannah River Lab., Aiken, S. C. USA). DP-400J.F. Proctor comp. July 1959. (TID-4500)

HEAVY WATER PRODUCTION IN THE USA. Thayer V. R. Nucl. Power 5, No. 4G, 103-11, Feb. 19G0.

FLOWSHEETS AND SUPPLEMENTARY DATA FOR THE HEAVY WATER PLANT DESCRIBED IN Chem. Eng. Progr. 58, 53-61,' No. 4, April 19G2. Proctor J. F., Thayer V. R. (Du Pont de Ne­ mours E. I. & Co. Savannah River Lab., Aiken S. C. Wilmington, Del. USA) TID-15733. 19G2.

HEAVY WATER POWER REACTOR PROGRAM MONTHLY PROGRESS REPORT, FEBBRUARY 1SG3. (Savannah River Opera- tions Office, AEC, USA). SRO-80. 1963.

•K^^fjr^-^it-J^J^wt»» Jinr--T**-T rv,"rr~-Ty^u'-rTiW*^TiT-7^»* V- \-V 201

15, USAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS REPORT, JANUARY 1964. Ililborn II. S. comp. (Du Pont de Nemours E.l. & Co. Savannali River Lab. Aiken, S. C. USA),DPST-04-33-l. lf>. USAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS REPORT, FEBRUARY 1964. Ililborn H. S., comp. (Du Pont de Nemours E. I. &. Co. Savannah River Lab., Aiken, S. C. USA). DPST-G4-33-2. Mar. ID, 1964.

17. IISAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS REPORT, MARCII.UHM. Hilborn U.S. comp. (Du Pont de Nemours E. [. & Co. .Savannah River Lab., Aiken, S. C. USA). DPST-64-83-3. Apr. 17, 19(54.

18. USAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS REPORT, APRIL 1964. Beach J. E., comp. (Du Pont de Nemours E.I. & Co. Savannah River Lab., Aiken, S. C.USA). DPST-G4-83- 4. May 15, 1964.

19. USAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS REPORT, MAY 1904. Hilborn II. S., comp. (Du Pont de Nemours E.I. & Co. Savannah River Lab. , Aiken, S. C. USA). DPST-64-83-5. June 18, 1964.

20. USAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS REPORT, JUNE 1964. Hilborn H. S., comp. (Du Pont de Nemours E.'l. & Co. Savannah River Lab., Aiken, S. C. USA). DPST-64-83-6. July 15, 1964.

21. USAEC-AECL COOPERATIVE PROGRAM MONTHLY PROGRESS REPORT, JULY 1964. Hilborn II. S. (Du Pont de Nemours E.I. &Co. Savannah River Lab., Aiken, S. C. USA). DPST-64-83-7. Aug. 24,1964. 202

22. HEAVY WATER PLANT. Prospect, T!ie Lunumis Co. Canada LUI. 1968.

23. THE STATUS OF CANADIAN CONSTRUCTION PROJECTS. PART II. HEAVY WATERAND OTHER.NUCLEAR PROJECTS. Can. Nucl. Assn. Annual Conf. June 19G9.

24. MAJOR CHANGES RECOMMENDED BEFORE DEUTERIUM'S PLANT OPERATIONAL. Chem.Can. 21, 33-4, Nov. 1969.

25. BRUCE HEAVY WATER PLANT. Robinson R. D. (Lurnmus Co. Cauda, Ltd. Don Mills, Ontario). Progress Report. 70-CNA-423. May 1970.

CNEN Symposium on Technical und Economic Aspects of Heavy Water Production. Turin, Italy, Sept. 30-Ocl. 1, 1970: 20. FABBRICATION AND CONSTRUCTION EXPERIENCE. BRUCE AND PORT IIAWKESBURY HEAVY WATER PLANTS.Spray P. II.G. ( A EC L.CANADA);

27. DESIGN CRITERIA FOR HEAVY WATER PLANT BASED ON H2S-H20 EXCHANGE PROCESS. Bhargawa R. K., Sadhukhan H. K., Scligal I. J.S., Deslipande P. G. (Bhabha Atomic Research Center Trombuy-Bombay, INDIA).

28. BRUCE AUXILIARY STEAM SUPPLY.Kolisnyk Z. (Montreal Engineering Co. Ltd. ), Spray P. H. G. Eng. J. (Montreal) 55,No.4, 22-G,Apr. 1972.

29. SINGLE UTILITY ELECTRIFIES NOVA SCOTIA. Mod. Power Eng. GG,No. 8, 56-7, Aug. 1972. 203

D - PRODUCTION PLANTS 3 - Plants Based on NII3/HD Exchange Process

1. HEAVY WATER PRODUCTION. Constructors John Brown Ltd. (UK). Brochure presented at the 2nd UN Geneva Conf.1958.'

2. ENRICHMENT OF DEUTERIUM THROUGH HIGH PRESSURE ISOTOPIC EXCHANGE BETWEEN HYDROGEN AND LIQUID AMMONIA IN A HOT-COLD PLANT. Walter S., Schindewolf U. Chcm.Ing. Tocli. 37, No. 12,1185-91, 1965,(Angew. Chemie.'77, No. 14, 620,19G5,Angew.Chcm.Inst.Ed. Eng.4,597, 1965)

HEAVY WATER FROM COAL?. Colliery Guardian 208, 212, Feb. 14, 1964.

HEAVY WATER PLANT AT MAZINGARBE. Lefrancois B.Bull. Inform. Sci. Tech. (Paris) No. 123, 11-20, Feb. 1968. (In French)

HEAVY WATER PLANT. Le Chatolier J. Bull. Inform. Sci. Tech. (Paris) No. 123, 21-5, Feb. 19G8.(In French) ?.0

A PILOT PLANT FOR DUAL TEMPERATURE EXCHANGE FOR STUDIES TO DEVELOP NII3- IJ2 PROCESSES. Kostaing M. Bull. Inform. Sci. Tech. (Paris) No. 12 3, 27-30, Fob. 1Ö6Ö.

THE HEAVY WATER, PLANT OF MAZ1NGARBE. Roth E.(CEN, Sac-Jay, FRANCE), l.'.edhome A., Lefrancois B., Le Chalolicr J. Tillol A. Enorg. Nucl. (Paris) 10, 2.1.4-1.9, May 11H>1}. (In French)

MAZ1.NCAUBE HEAVY WATER PLANT. Nu el. Eng. Int. 14, 578-80, .iLily IDfii).

THE MAZINGARBE HEAVY WATER PLANT. Société Chimique des Charbonuages. CEA. Nuolc.x 19G9.

INDIA'S AEC PROPOSES A $.1. ß-BILLION, 10-YEAR. NUCLEAR POWPIR PROGRAM. Nucleonics Week 11, No. 30, fi, Aug. G, 1070.

CNEN Symposium on Technical and Economic: Aspects of Heavy Watc 1- Production. Turin, Italy. Sept. 30-Oct. 1, 1970:.

OPTIMIZATION OF DEUTERIUM PRODUCTION PLANT WITH THE AMMONIA-HYDROGEN SYSTEM. SchtndcwolJ' U., Lang G. (Inst. fUr Kernverl'alnonstochnik, K.FK Karlsruhe W. GERMANY);

PROBLEMS OF DESIGN AND CONSTJÌUCTION OF A PLANT FOR THE PRODUCTION OF HEAVY WATER BASED ON THE DUAL- TEMPERATURE AMMONIA-HYDROGEN EXCHANGE SYSTEM. Waller S., Nttschke E. (Friedrich Ulule G. ni. b. II. Dortmund, W. GEH MANY): 205

13. PROBLEMS ON A CONCEPTUAL DESIGN OF A JJEAVY WATERÌ PRODUCTION PLANT.-CONTRIBUTION OF AG1P NUCLEARE. Bracci l'orli L. , Cnbclla A., Duranti Vnlenìiiii P. (AGTP Nucleare, Jlaly) ;(ln f-.i'liaii)

14.. OPERATING EXPERIENCE OP* MAZINGARBE HEAVY WATER PLANT. i_,e!'rancni,s Jl. (Sor.. Chiiniquc clc Cliurbonnago,FRANCE) (fn P'vench).

15. CRITERIA FOR THE DESIGN OF NII3-H3 TWO-TEMPERATURE PLANT FOR HEAVY WATER PRODUCTION. Folli E. (CISE), Polastri F., Vaccaro G. Energia Nucleare (JVIilaii) 17, 721-32, Doc. 1970

16. OPTIMIZATION OF HEAVY-WATER ENRICHMENT PLANT BASED ON LI2/NH3'EXCHANGE AND OPERATING BY THE HOT/COLD PRINCIPLE. Lang G. , SchindcwoH' U. Chcm. Ing. - Tech. 43, No. 14, 004-10, July 1971. (in German) 207

D - PRODUCTION PLANTS 4 - Plants Based on I-Ip.O/lID Exchange Process

1. TRAIL REPORT. Weight M.M. Aug. 28, 1944.

2. THE PRODUCTION OF HEAVY WATER AT TRAIL B. C. Barlow E. A. (AECL, Chalk River, Ont. CANADA). CRE-374. Mar. 8, 1948. Deci. Feb. 22, 1955. (AECL-163)

CALCULATION OF THE PERFORMANCE OF EXCHANGE IN THE PRODUCTION OF HEAVY WATER. Carlson II. C., Maloncy J. O^ A-327. Oct. 7, 1942. Deci. May 14, 1954.

4. CATALYTIC EXCHANGE ELECTROLYTIC PROCESS FOR THE ISOLATION OF HEAVY WATER AT TRAIL B. C. Maloney J. O., Quinn G. F., Ray II. S. Production of Heavy Water. G. M. Murphy, H. C. Urcy, I. Kirshenbaum eds. McGraw Hill 1955. (NNES-III-4F) p.9-52)

5. A METHOD FOR THE GRAPHICAL CALCULATION OF THE NUMBER OF THEORETICAL PLATES IN AN ELECTROLYTIC PLANT AITH EXCHANGE TOWERS FOR THE PRODUCTION OF HEAVY WATER. DinelJi D. Energia Nucleare (Milan) 2, 426-33, Aug, 15, 1955. (In Ita.lian)(AERE-Lib/trans-G06) 208

6. .CALCULATION METHODS FOR TRANSFER COLUMNS. Villani S. Energia Nucleare (Milan) 2, 504-18, 1955.

7. DEUTERIUM SEPARATION COLUMNS AND HEAVY WATER. Silvestri M., Villani S', Presented at Symposium on Heavy Water . Rome, Italy, March 31-Apr. 2, 1955.

8. RECENT EXPERIMENTS ON THE PRODUCTION OF HEAVY WATER BY ELECTROLYSIS AND ISOTOPIC EXCHANGE REACTIONS.Finzi S.', Ronzoni R., Silvestri M. Energia Nuclea­ re (Milan) 3, No. 4, 294-308, Aug. 195G.(In Italian)

9. HYDROGEN-WATER VAPOR CONDENSERS DESIGN. Finzi S., Ronzoni R., Silvestri M., Zavattarelli R. (CISE, Milan, ITALY). Energia Nucleare (Milan) 4, 199-210, June 1957.

10. A NEW PROCESS FOR THE MANUFACTURE OF HW WAS SHOWN. ACTIVITIES INCLUDING THE PRODUCTION OF U, Th, Zr, REACTOR FUEL ELEMENTS, CONTROL RODS & RE­ FRACTORIES. Degussa (Germany). Atomics and Nuclear Energy 9, No. 10, 341, Oct. 1958.

11. DEGUSSA UHDE LARGE PILOT PLANT CONSTRUCTION. Atomkernenergie 3, 362, 1958.

12, DEGUSSA PLANT. Nuclear Engineering 3, No. 29, 352, 1958.

13. ENRICHMENT OF HEAVY WATER BY HIGH PRESSURE EX­ CHANGE BETWEEN HYDROGEN AND AN AQUEOUS CATALYST SUSPENSION.PART II. CONSTRUCTION AND OPERATION OF A PILOT PL-ANT. Walter S., Nitschke E., Bode C. (Friedrich Uhde GmbH, Dortmund, GERMANY). Becker E. W., Huebener R. P., Kessler R.'A., Schindewolf U. Chem. Ing. Tech. 34,7-10,1962. 209

14. LABORATORY PILOT PLANT FOR THE EXPERIMENTATION OF ISOTOPIC PROCESS AT HYDROGEN-WATER EXCHANGE REACTION IN A BITHERM SYSTEM. Fcculca M,, Boian M., Fatu C., Potior T. IFA Ilcpoi't, Bucharest, 030/19G5. (Unpublished)

15. INSTALLATION FOR HEAVY WATER PRODUCTION BY THE HYDROGEN-WATER ISOTOPIC EXCHANGE REACTION OC­ CURRING IN A COLUMN AND WITH PHASE CONVERSION BY ELECTROLYSIS, IN THE RANGE OF 5-99, 8% DEUTERIUM. Boian M., Mcrcea V. , Palibroda N., Pcculea M. IFA Report, Bucharest, G9G/19G7. (Unpublished)

1C. CAUSTIC SODA SOLU'TlON AS CATALYST FOR ISOTOPIC EXCHANGE BETWEEN HYDROGEN AND WATER IN A TRANSFER COLUMN FOR TECHNICAL CONCENTRATION OF DEUTERIUM. SchindewoLl' U., Hornke J. Chem. Ing. Tech. 40, 29-30, 1968. (In German)

17. ENRICHING COLUMN FOR THE SEPARATION OF LIGHT WATER BY ISOTOPE EXCHANGE REACTION BETWEEN HYDROGEN AND WATER. Mcrcca V., Palibroda N., Fodor T., Stoicovici L. Isotopenpraxis 4, 328-30, 19G8. (In German)

18. EFFICIENCY OF THE EXCHANGE SPACE WITH DIFFERENT STRUCTURES IN A CATALYZED HYDROGEN-WATER VAPOR- WATER ISOTOPIC EXCHANGE REACTION COLUMN. Boian M., Hodor I.', Pcculea M., Straulca R.S. IFA Report (Bucharest) IS-50-.1DG8. 211

D - PRODUCTION PLANTS 5 - Distillation Plants

1. CONCENTRATION OF THE OXYGEN ISOTOPES. Urey H. C., Pegram G. B., Huffman J. R. J. Chem. Phys. 4, 623, 1936.

2. DISTILLING APPARATUS FOR THE SEPARATION OF ISO­ TOPES. Pegram G. B. , Urey II. C., Huffman J. R.- Phys. Rev. 49,883, 1936.

3. SEPARATION OF OXYGEN ISOTOPES BY A FRACTIONATING COLUMN. Huffman J. R., Urey H. C. Ind. Eng. Chem. 29, 531-5,1937.

4. PACKED FRACTIONATION COLUMNS AND THE CONCENTRA­ TION OF ISOTOPES. Cohen K. J. Chem. Phys. 8, 588-97, 1940.

5. OPERATING MANUAL OF WATER-DISTILLATION UNITS. Monier J. A. 1941.

6. PRODUCTION OF HDO WATER BY DIRECT METHOD. Amick M. G. SAM Report A-394. Dec. 4, 1942. 212

7. PRELIMINARY PLANT DESIGN. Huffman J. R. SAM Report A-402. Dec. 1, 1942.

8. FRACTIONATION OF LIQUID HYDROGEN. Huffman J. R. Columbia Memo. Nov. 11, 1942.

0. (On Hydrogen Distillation). Johnston II. L. Ohio State Uni­ versity. Progress Report. SAM Report A-501. Jan. 9,1943.

10. SEMIWORKS DISTILLATION TESTS. Carlson R. C. Du Pont Engng. Dopt. Report Mar. 8, 1043.

11. THE SE PARATION OF ISOTOPES BY THE DISTILLATION OF WATER. Thode H. G., Smith S. R., Walking F. O. Can. J. Res. 22 3,127-36,1944.

12. A CONVENIENT AND EFFICIENT FRACTIONATING COLUMN AND ITS USE IN THE SEPARATION OF THE HEAVY ISOTOPES OF HYDROGEN. Dostrovsky I., Hughes E.D. Nature 153, 164-5, 194G.

13. FRACTIONAL DISTILLATION AND ITS APPLICATION IN THE CONCENTRATION OF HEAVY ISOTOPES OF OXYGEN' AND HYDROGEN. Dostrovsky I., Hughes E. D. , LleweUyn D. R. Nature 161,858-9,1948. 213

INDUSTRIAL FRACTIONATING-TOWER PACKING. Scottele! R. C. Cliem. Eng, Progress

STATUS REPORT ON HEAVY WATER PRODUCTION PROGRAM. DESIGN OF PRODUCTION PLANT-HYDROGEN DISTILLATION PROCESSES, HYDRO-CARBON RESEARCH, INC., CONTRACT AT (3.0-1) -810, DESIGN OF PILOT AND PRODUCTION PLANT AND CONSTRUCTION OF PILOT PLANT-DUAL-TEMPERA­ TURE PROCESSES, THE GIRDLER CORPORATION, CONTRACT AT(30-l)-947.NYO-699. June 19, 1950, Deci. Jan. 15, 1959.

SOME CHARACTERISTICS OF STEDMAN PACKING IN THE DISTILLATION OF HYDROGEN AND ITS ISOTOPES.'Fooicson A., Pomerantz, P., Rothberg.S. J. Research Nat. Bur. Stds. 47, 449-55, Doc. 1951.

STUDIES ON ISOTOPES. III. THE PERFORMANCE OF STAINLESS STEEL GAUZE RING PACKING IN THE . ISOTOPIC FRACTIONATION OF WATER. Mackenzie II. A. E. Malherbe P. N. J,S. African Chem, Inst. 4,69-78,1951.

LOW TEMPERATURE HEAVY WATER PLANT. (Hydrocarbon Research Inc. USA), NYO-889. Mar. 15, 1951. .

OPTIMAL FLOW IN FRACTIONATING COLUMNS FOR ISO­ TOPE SEPARATION.'DostrovskyI.',Gillis J., Vromen B.H. Bull. Research Council Israel 2, 68-9,1952. 214

HYDROGEN - LIQUIFYING PLANT FOR SCIENTIFIC RESEARCH INSTITUTES. Malkov M. P., Fradkov A.B. Zhur. Tekh. Fiz. 22, 6, 1952. (In Russian)

ANALYTICAL METHODS FOR THE CALCULATION OF CASCA­ DE SYSTEM OF RECTIFICATION COLUMNS. Zliavoronkov N. M., Zelvenskii Ya. D. Sbornik Protsess.i i Apparati Khimicheskoi-' Tcklmologn. Goskhimizdat, Moscow 1953. (In Russian)

THE STEAM VENTS OF TUSCANY AND THE LARDERELLO PLANTS. Mazzoni A. 2nd. Ed. Calderini, .Bologna, 1954.(In Italian)

DW PLANT OPERATING CHARACTERISTICS. Blair J. A. (Du Pont do Nemours E.I. & Co.Savannah River Lab.-, Augusta Ga. USA).TID-5337.Junel8, 1954. Deci. Mar. G, 1957.

TILE KUHN PRECISION RECTIFYING COLUMN. Sulsser Tech.. Rev. (Switz. )No. 2, 36-47, 1955.

A PRELIMINARY STUDY OF SOME ASPECTS OF A HEAVY WATER PLANT. Tech. Memo. No. 30. Vander Arend P. C. (NBS- AEC Eng. Lab., Boulder, Colo. USA). NBS-3519. Feb. 11, 1955.

THE DESIGN OF ISOTOPE SEPARATION PLANTS. SOME DE­ SIGN EQUATIONS FOR THE DISTILLATION PROCESS. Dostrovsky I. Presented at Symposium on Heavy Water. Rome, Italy, Mar. 31-Apr. 2, 1955. (CNRN Rome 1956)

THE DESIGN OF ISOTOPE SEPARATION PLANTS:SOME BASIC. DESIGN EQUATIONS FOR THE DISTILLATION PROCESS. Dosirovsky I., Lehrer Y. 8,.P/774 (ISRAEL). 1st Geneva Conf. 1955 215

28. WATER DISTILLATION PROCESS FOR THE ISOLATION OF HEAVY WATER AS EMPLOYED BY E. I. DU PONT DE NEMOURS & CO. Inc. AT MORGANTOWN. Maloney-J. O.\ Quinn G. F., Ray II. S. NNES-III-4 F,'55-83,1955.

29. SPRAY-PACK: A NEW INDUSTRIAL DISTILLATION AND AB- SORBPTION TOWER PACKING. McWilliams J. A., Pratt U.R. G., Dell F.R.Trans.Inst. Chem.Engrs. (London) 34, No. 1, 18-43,3 956.

30. THE CASCADING PROBLEM IN A WATER DISTILLATION PLANT FOR HEAVY WATER PRODUCTION. Cerrai E., Silve­ stri M., Villani S. Z. Naturforsch. Ila, G94-7Ü1, 1956.

31. PRELIMINARY PROJECT REPORT FOR THE NANGAL FERTI­ LIZER HEAVY WATER PROJECT. Saint Gobain, Paris, France. Apr. 195G.

32. PRELIMINARY PROJECT REPORT FOR THE NANGAL FERTI­ LIZER HEAVY-WATER PLANT. Part II. VLtro Engineering Div. New York. Aug. 195G.

33. FURTHER DEVELOPMENTS OF SPRAY-PACK : DISTILLATION COLUMN PACKINGS. McWilliams J. A., Pratt II. R. G. AERE. CE/R 1941. Nov. 15, 1956.

34. A DYNAMIC PROGRAMMING SOLUTION TO A PROBLEM IN HEAVY WATER PRODUCTION. Bellman R. (RAND Corp., Santa 'Monica, Calif. USA). Nuclear Sci. and Eng, 2, 523-5, July 1957.

35. DESIGN ASPECTS OF PLANT FOR PRODUCTION OF HEAVY WATER BY DISTILLATION OF HYDROGEN. (Arthur D. Little Inc., Cambridge, Mass. USA).NYO-2134.Dec. 11, 1957. 216

30. DESIGN CRITERION FOR WATER DISTILLATION PLANT FOR HEAVY WATER PRODUCTION. Canini R. Proc. Int. Syinp, on Isotopes Separation 1957, North Holland Pubi, Co. Amsterdam 1958. (p. 360-82)

37, THE PILOT PLANT AT BOULDER. Timmerhaus K. D., Wcitzel D. II. , Flynn rr. M. Cliem, Eng. Progr. 54, No, G, 36-4G, June 1958.

38. INDUSTRIAL SCALE HYDROGEN-DEUTERIUM DISTILLATION SEPARATION IN FRANCE. Chem. Engineering Progr. 54, No. 11, 12G, 128, 1958.

39. ON DISTILLATION COLUMNS FOR ISOTOPE SEPARATION, I-Iavlicek F. I. (J, Stephan Inst. Ljubljana, YUGOSLAVIA). Energ. Nucl. (Milan) 5, No. 8, 527-30, Aug. 1958.

40. A LABORATORY APPARATUS FOR DEUTERIUM ENRICHMENT BY THE RECTIFICATION OF LIQUID HYDROGEN, Weisser R. H. Sulzer Tcch.il. Rev. (Switzerland) 40, No. 3, 71-4,1958.

41. DESIGN OF THE FINAL STAGES OF. DEUTERIUM PRODUCING FLANTS. Lehrer Y., Woissnian Y. (Israel Atomic Energy Com­ mission)^, P/lull. (ISRAEL). 2nd UN Geneva Conf. 1958.

PRODUCTION OF HEAVY HYDROGEN IN A LARGE-SCALE RECTIFICATION PLANT. Lehmer W., Sellmaier A., Baldus W. Linde Ber. Tech. u. Wiss. 5, 3-14, 1959. (In German) (NP-tr-417)

HOW LINDE MAKES HEAVY WATER FROM HYDROGEN. Chem. Eng. GG, No. 4, 68, 70, 72, Feb. 23, 1959. 217

THE PILOT PLANT FOR LIQUID HYDROGEN DISTILLATION AT TOULOUSE;StoulsE.Bulirinf;Sci. et Tech. (Paris) No. 40, 4-10, May 1960. (In French) • '"'

WATER DISTILLATION. THE PILOT PLANT OF SOULOM. Lazard B. Bull. Inf. Sei. et.Tech. (Paris) No. 40, 11-13, May 1960. (In French)

PILOT PLANT DATA FOR HYDROGEN ISOTOPE DISTILLA­ TION. Flynn T. M. (NBS, Boulder .Colo. USA). Chem. Eng. Progr. 56, No. 3, 37-42, Mar. I960.- •

. THE McCABE-THIELE DIAGRAM FOR ISOTOPE SEPARATION AND A GENERAL FORMULA FOR CALCULATING THE NUM-: ; BER OF THEORETICAL PLATES IN A MASS EXCHANGE COLUMN. Dietze M., Pilz S. Chem. Techn.' 12, No. 2, 81-7, 1960. (In German)

McCABE-THIELE DIAGRAM .FOR THE IDEAL CASCADE. , Slirowiec A. J.. Ind. Eng. Chem.' 52, 789, 1960.

INDUSTRIAL INSTALLATION FOR PRODUCTION OF HEAVY- WATER AT LOW TEMPERATURES. Hanny J. Schweiz. Arch., Angew.Wiss.u.Tech. 26', 115-28, 1960. (CEA-tr-A-943)

A LOW-TEMPERATURE PLANT FOR THE PRODUCTION OF HEAVY WATER. Hanny/J. Sulzer,Tech. Rev. (Switz; ) 42, No. 2,. 9-24, 1960.

INDUSTRIAL INSTALLATION/FOR THE SEPARATION OF DEÙr.' TERIUM FROM LIQUID HYDROGEN BY RECTIFICATION. : Haenny J. Problems of Low Temperature Physics and Thermo>v dynamics.New York, McMillan Co.'Vol. 2.1960. (p. 29-45) '. !

218

52. ISOTOPIC DESIGN OF A PLANT FOR PRE-CONCENTRATION, OF HEAVY WATER BY DISTILLATION OF WATER, STARTING WITH NATURAL WATER. Ceri-ai E., Silvestri M., Villani S. j (CISE, Milan, ITALY). CISE-81. Sept. 1960. (In Italian) j

53. RECENT ADVANCES OF DISTILLATION TECHNICS. Brigoli j B., Energia Nucleare;(Milan): Part I, 7, No. 9, 590-G, Sept. 1960; ] Part II. 7, No. 11, 7G1-8, Nov. 1960. j * 54. CALCULATION METHODS FOR FRACTIONATING COLUMNS. Brigoli B. Energia Nucleare (Milan) 7, No. 12, 845-8, Dec. I96 0.

55# ' HEAVY WATER PLANT MELDS NEW FEATURES. Chopey N. P. Chem. Eng. G8, No. 4, 118-21, Feb. 20,1961.

56 A DISTILLATION PLANT FOR H2OI8 ENRICHMENT. Adorni N., Angelino G., Brigoli B.Chem. Age; of India 12, No. 4, 333-7, July - Aug.19G1.

57. PREDICTING TRAY EFFICIENCY IN DISTILLATION COLUMNS. Coates J., Pressung B. S.Chcm. Engr. 68, 8,187-90,1961.

58. OPTIMUM REFLUX CONDITIONS FOR COLUMNS OF ISOTOPE SEPARATION. Olariu A. Stud. Cercet. Fiz. (Bucharest) 13, No. 6, 939-45,19G2.

59. KOCH-SULZER RECTIFICATION COLUMNS. Koch Engineering Co. New York, (USA). Bulletin KS-1.

§p•.•;• 60. HIGH PRECISION DISTILLATION COLUMNS. Kuhn W. Bull. Mp, ; Assoc. Franc. Techniciens Petrole 154, 559-91,1962.. t]

'& t • fl

I II m 219

CI. ON THE INDUSTRIAL ADAPTABILITY OF THE PACKINGS .OF THE HEAVY WATER DISTILLATION TOWER. Masami S. (Showa Dcnko K. K,, JAPAN), Shimizu M., Matsumoto S. Nippon Genshiryoku Gakkaishi 4(2), 85-94, Feb. 1962. (In Japanese)

G2. SOME ANALYSES ON • THE OPERATION OF WATER RECTIFICA­ TION TOWER. Masami S., Shinichi H. (Keio Univ., Tokyo, JAPAN). Nippon Genshiryoku Gakkaishi 4, 313-21, May 1962. (In Japanese)

G3. FINAL-AND RECONCENTRATION OF HEAVY WATER BY MEANS OF KUHN-SULZER COLUMNS. ThUrkauf M. (JEN, Madricl;EAES, Paris). ColloquLum on Heavy Water, Madrid. Dec. 13-14, 1962. NP-1376G (p. 77-83)

G4. PERFORMANCE OF A COCURRENT DISTILLATION CONTACTING DEVICE. Angelino G., Brigoli B. »Silvestri M. Energia Nucleare (Milan) 10,85,1963.

65. SULZER RECTIFICATION PLANTS FOR SEPARATING D20 FROM H2O. Huber M., Sperandio A. Sulzer Tech. Rev. (Switz. ) 46,177-88,1964.

66. ANALYSIS OF OPERATING EXPERIENCE OF A HYDROGEN DISTILLATION PLANT; Gami D. C., Rapial A. S. 12, P/754. (INDIA). 3rd UN Geneva Conf. 1964.

67. CHARACTERISTICS AND DESIGN OF A CO-CURRENT DISTILLA­ TION COLUMN. Angelino G., Brigoli B., Silvestri M. Energia Nucleare (Milan) 12, 353, 1965. ..

68. INSTALLATION FOR HEAVY WATER PRODUCTION BY DISTILLATION IN THE CONCENTRATION RANGE OF 5-ütf, 8% DEUTERIUM. IFA (Bucharest). Rep. 1667/1967. (Unpublished) ••""••••»--'-•-• 'I -1

220

69. STAINLESS MEETS STRINGENT TEST ON HEAVY WATER PLANT. Can. Mach. Mctalwòrk. 79, 6G-7, May 1968.

70, RECTIFICATION OF HEAVY WATER IN COLUMNS IN PARALLEL., >; Gispert M. , Rojas J. L. (JEN Madrid, SPAIN).An.'Quim. 64, 7G5-74, i July- Aug. 1968.

71. HEAVY WATER RECOVERY PLANT. Prospect.Linde A. G. 567/2E.1968/

72. NATURAL WATER DISTILLATION PLANT. Selecki A. (Warsaw Technical Univ., POLAND).Nuclear-Eng... Int. 15, No. 172, 717-9, Sept. 1970.(CNEN Symp. Turin, Itali. Sept. 30-Oct. 1, 1970)

73 EFFICIENCY OF AN EXCHANGE PLATE IN CONCURRENT. Brigoli B. (CISE, Milan, ITALY) CNEN Symp. on Technical ed. Economic Aspects of Heavy Water Production. Turin, Italy Sept. 30-Oct.l, 1970.

i

m & I:

IM |fli

II '4 221

D - PRODUCTION PLANTS 6 -Plants based on Electrolysis df Water

1. APPARATUS FOR THE SEPARATION OF ISOHYDROGEN (DEUTERIUM) OXIDE BY ELECTROLYSIS. Harkins W. D., Doede C. J. Am. Chem. Soc. 55,4330-1, 1933.

CONTINUOUS-FLOW METHODS OF CONCENTRATING DE.U- TERIUM. Anderson L. C., Halford J. O., Bates J. R. J. Chem. Phys.2, 342-4, 1934.

3. PRODUCTION OF LARGE QUANTITIES OF HEAVY WATER. Tronstadt L. Nature 1.33, 872, 1934.

4. A LABORATORY SET-UP FOR THE ELECTROLYTIC FRACTIO­ NATION OF HYDROGEN ISOTOPES. Erlenmayer H., Gartner H'. II. Helv. Chim. Acta 17, 1226-31,1934. III. Helv. Chim. Acta '1TB, 419-20, 1935.

5. LABORATORY APPARATUS FOR THE ELECTROLYTIC CON­ CENTRATION OF THE ISOTOPE 2 OF HYDROGEN. Champetier G. Bull. Soc. Chim. France (5) 2; 162-7, 1935.

PLANT. O FOR THE PRODUCTION OF HEAVY WATER. Brown ; Wj. G., Daggett A. F. J. Chem. Phys.,3, 216-8, 1935. Sì AIP LE EQUIPMENT FOR ELECTROLYSING HEAVY WATER., Slack C. M. , Ehrke L. F. Rev. Sci. Insti-, 8, 39, 1937.

PRODUCTION OF HEAVY WATER. Alcksandrovich V. A. Novosti Teknniki No. 26-7, 50-1, 1939.

INEXPENSIVE EQUIPMENT FOR THE PREPARATION AND CONCENTRATION OF PURE D2O DEUTERIUM RICH WATER. DESCRIPTION OF CONSTRUCTION AND OPERATION OF THE FORMER OHIO STATE UNIV. HEAVY-WATER PLANT. Johnston II. L., Hall W.H.Ohio J. Sci. 41, 357-65, 1941.

OPERATING MANUAL OF THE ELECTROLYTIC PLANT AT MORGANTOWN. Monier J. A. 1941

SECONDARY PLANT EVAPORATION. Cavers S.D. CMS Rep. 3, Sect. 953, May 18, 1944.

(On Deuterium and Heavy Water Analysis). Wright M. M. Trail Rep. 63, Aug. 2Q, 1944.

ELECTROLYTIC P-9 PRODUCTION OPERATING MANUAL. Ilarty W.'M.'(Du Pont de Nemours E.I. & Co. Morgantown Ordnance Works, Morgantown, W..Va. USA) M-3132.Sept. 1, 1945. Deci. Jan. 12, 1956.

PRE CON CENTRATION OF HEAVY WATER IN ELECTROLYSIS PLANT. Orsoni B. Proc.XI Inst. Congr. Pure and Applied Chem. (London) 5, 1057-63, 1947. (Chim. e Industr. 30, 232-4,1948)

184 " CYCLOTRON DEUTERIUM ELECTROLYZER TESTS. Report No. ll.Stephan W.'J.(Univ.'Berkeley, California,Radia­ tion Lab. USA).M-37l2.Mar.20, 1947.Deci.Nov. 29, 1955. 223

IG. AUTOMATIC EQUIPMENT FOR ÉLECTROLYZING HEAVY WATER. Wanick R.W. Rev.'Sci. Instr. 21, 2G2, 1950.

17. ELECTROLYTIC CONCENTRATION OF HEAVY WATER.II CONTINUOUS OPERATION PLANTS. Or soni L.", Silvestri M." CISE-17.1050.'(In Italian)

18. AN AUTOMATIC HEAVY WATER'ELECTROLYSIS APPARATUS, Rabinovich E.S.,Douglas J.'E. Rev. Sci.Instr. 22 Z 9.Nov. 1951.

19. THE CONTINUOUS ISOTOPIC ENRICHMENT BY CASCADES. Walen R.Rec. Tx-av. Inst.'Rech. Structure Matiére (Belgrade) 1,35-G7,1952.

20. A DEUTERIUM ELECTROLYSIS PLANT Lloyd J. T. J. Sci. Instr.29, No.5, 1G4-5, 1952.

21. OUTLINES OF SMALL-SIZED ELECTROLYTIC PLANT FOR D20 AT HYGII DEGREE OF CONCENTRATION. Cerrai E„ Orsoni L., Silvestri M.CISE-32, 1952. (In Italian)

22. II20-D20 SOLUTIONS NEUTRALIZATION AND DISTILLATION PLANT. Cerrai E., Silvestri M, CISE-33.1952. (In Italian)

23. ELECTROLYTIC SYSTEMS WITH COLUMNS FOR THE RECO­ VERY OF DEUTERIUM BY THE EXCHANGE REACTION. Cerrai E. /Marchetti C., Silvestri M., Villani S. Part i;CISE ReP;61 (AERE-Trans-834). Partii; CISE-62.:July 30, 1954. (AERE-Trans- 835) Part IIlJ STUDY OF FOUR-STAGE SYSTEMS WITH COLUMNS CONSISTING OF CONDENSATION PLATES, WITH PARTICULAR REFERENCE TO THE YIELD AND OTHER CHARACTERISTIC PARAMETERS.'ECONOMIC CONSIDERATION CONCERNING THE RECOVERY OF DEUTERIUM; CISÉ-63. July 1954. (AERE- Trans-836) 224

A METHOD FOR THE GRAPHICAL CALCULATION OF THE NUMBER OF THEORETICAL PLATES IN AN ELECTROLYTIC PLANT WITH EXCHANGE TOWERS FOR THE PRODUCTION Oli' HEAVY WATERpinclli D. Energia Nucleare (Milan) 2,426-33, Aug. 15, 1055.(1» Italian) (AERE-Lib/Trans-GOfi)

CALCULATION METHODS FOR TRANSFER COLUMNS. Villani S. Energ. Nucl. (Milan) 2, 5.04-18, 1955.

A MERCURY SAFETY VALVE FOR ELECTROLYSIS OF HEAVY WATER. Chauclliri II,' M.'{Government Coll., Lahore, PAKISTAN) Proe.Phys.Soc. (London) B-G'8, 1157-8, Dec. 1, 1955.

REPORT ON RECENT ITALIAN EXPERIENCES IN THE PROD­ UCTION ON HEAVY WATER USING PROCESS ELECTROLYSIS AND PLATE TOWERS. Finzi S., Ronzoni R., Silvestri M. Proce­ edings of the Scientific Congress, Nuclear Session, July 2-6, 1956, 3rd Electronic-Nuclear International Review. (Roma, National Committee for Nuclear Research). 1956.

DESIGN OF AN ELECTROLYTIC PLANT FOR THE CONCEN- ' TRATION OF HEAVY WATER. Deshp ancle P.O., Gami D.C." 4, P/1G69. (INDIA). 2nd UN Geneva Conf. 1958.

THE ELECTROLYTIC CELL FOR HEAVY WATER PRODUCTION. Kawashima N. Kogyo Kogaku Zasshi 62, 487-98, 1959.

DESIGN OF A PLANT FOR FINAL ENRICHMENT OF AQUEOUS SOLUTIONS OF D20 UP TO CONCENTRATIONS OF 99, 8%; Finzi S., Marchetti C. , Ronaoni R., Silvestri M'. Part I.'CHEMICAL DESIGN-PHYSICS OF THE PLANT. CISE-76.' Juno 1960. Part II-A. DESIGN AND CONSTRUCTION OF THE TYPE ELE­ MENTS. OPERATING EXPERIMENTS. CISE-77; June I960. Part II-B. CONSTRUCTION DESIGN OF TYPE ELEMENTS.! CISE-78.June I960. " Part. III. TECHNICAL DESIGN, CISE-79. July 19G0.' 225

31. PRODUCTION OF '.HEAVY WATER BY THE ELECTROLYTIC METHOD. Tai Y. K., Hsu Y.' C. (Taiwan Univ.' CHINA) Ho Tsu K'o I-Isueh 2, 10-8, 1960.

32. PRODUCTION OF LOW-TRITIUM DEUTERIUM. Drury J.'S., Guymon R. H., Joseph E." Fj (ORNL, Tenn. USA). Chem.' & Pro­ cess Eng.'42, 220-4, May 1961.

33. ON THE OPTIMUM CASCADE OP MANUFACTURING OP HEAVY WATER AS A BY-PRODUCT IN THE WATER-ELECTROLYSIS PLANT.ELECTROLYSIS-EXCHANGE REACTION+WATER RECTIFICATION+RECOVERY ELECTROLYSIS. Shimizu Ml (3rd Tech. Div., Showa Denkó KjK,, JAPAN), Kawashima K' Nito S., Matsumoto'S. J. At.Energy Soc. Japan 3, 770-8, Oct,! 1961. (In Japanese)

34. THE INDUSTRIALIZATION'OF THE ELECTROLYTIC CONCEN­ TRATION METHOD OF HIGHLY' ENRICHED HEAVY WATER. Shimizii M.', Nito S.', Harada A. (In Japanese) Part I. ELECTROLYTIC CONCENTRATION CASCADE AND CELL. Nippon Genshiryoku Gakkaishi 4, No. 3, 180-7, 19G2. Part II. RECOMBINATION AND REMOVAL OF ALKALI. Nippon Gerehirypku Gakkaishi 4, No.' 4, 211-7, Apr. 1962.

Report of the Colloquium on Heavy Water.' J.' E.'N.' Madrid Dec'1962 (JEN and EASES). NP-13766: 35. A THEORETICAL STUDY ON THE UTILIZATION OF GAS SCRUBBERS IN A CASCADE OF ELECTROLYSERS AND ISO- TOPIC EXCHANGE. Otero de la Gandara J.' L., Maria Arcoclia A.M. NP-13.766'(p.' 37-52);

36. A STUDY OF THE OPTIMUM HANDLING PROCEDURES OF A CASCADE OF ELECTROLYSERS AND ISOTOPIC EXCHANGE REACTORS BY MEANS OF AN ELECTRONIC COMPUTER. Otero de la'Gandara J.'L., Maria Arcocha A. M.NP-13766 (p.'53-76); 226

37. HEAVY WATER PRODUCTION. IN SPAIN.' DESCRIPTION OF THE. JEN-EIA PLANT AT SABINANIGO.'Gispert Bennach M.'(JEN, MadridjEAES, Paris).NP-l3766.(p.'27-36).

38. STUDY ON THE PRODUCTION OF HEAVY WATER.'I.DESCRI­ PTION OF THE JEN-EIA INSTALLATION AT SABINANIGO.' Otero de.la Gandara J.'L.', Gispert Bennach M.(JEN, Madrid, SPAIN). Energia Nu ci. (Madrid) 8, No. 32, 4-11, Oct,-Dec. 1964. (In Spanish)

39. STUDIES. ON THE PRODUCTION OF HEAVY WATER. II. PILOT PLANT FOR ELECTROLYSIS AND BURNERS.'Otero de la' Gandara J. L., Gispert Bennach Mi',Rojas J.'L.'Energia Nucl. (Madrid) 9, 90-4, Mar.-Apr. 1965. (In Spanish)

40. LABORATORY ELECTROLYZER WITH HIGH CURRENT CHARGE. Palibroda E., Fodor T.' Rev. Chim. (Bucharest) 16, 94, 1965. 227

E - TECHNICAL AND EC ONO MIC-AS PEC TS

1. DUAL-TEMPERATURE HEAVY WATER PROCESS EVALUATION OF PROPOSED TESTING AND PRODUCTION PROGRAM AT WA­ BASH RIVER ORDINANCE WORKS. (Girdler Corp. Gas Processes Div., Luisville,, USA), NYO-G81. Apr. .21, 1950, Deci. Feb. 27, 1957.

2. EVALUATION OF HEAVY WATER PRODUCTION AT GASEOUS DIFFUSION PLANT SITES. Blumkin S., Dehoney R. W., Shacter J. (Carbide and Carbon Chemicals Co. K-25 Plant, Oak Ridge, Tenn. USA). K-843. Nov. 26, 1951. Deci. 27, 1955.

3. REPORT ON THE FEASIBILITY OF HEAVY WATER PRODUC­ TION IN INDIA. Brun J. June 1954.

4. DENSITY AND COST RELATIONS FOR D20 AND SOLUTIONS OF UO2SO4 IN D2O. TBR Memorandum No. 2, Gaines A. L. (ORNL, Tenn. USA). CF-54-10-86.'Oct. 14, 1954.

5. CHEAP HEAVY WATER. Rae II. K. Chemistry in Can. 7, No. 10, 27-32, 1955.

G. ECONOMIC PROBLEMS IN THE PRODUCTION OF HEAVY WATER ' BY DISTILLATION OF NATURAL WATER, USING THERMOELECTRIC CENTER. Casini R. Energia nucl. (Milan) 3, 188-203,195G.

7. CHEAPER WAYS TO MAKE,D20. Harteck.P. Nucleonics 14, No. 9,. 97^9,1956.. '•--. .'•'•''. 228

CUTTING THE COST OF HEAVY WATER. Atomic World 9, No. 11, 382-5, Nov. 19.58. ...

CALCULATION OF D20' COST. Atòmwirtschart 3, 36, Jan. 1958.

LESS D9O. Atòmwirtschart 4, No. 5, 224,' May 1959.

SAVANNAH D20 PLANT COSTS. Atomwirtschaft 4, No. 10, 455, Oct. 1959.

SECRETS OF LOW COST HEAVY WATER. Labine R. A. Chem. Eng. G6,No.21, 170-3, Oct. 19","i~959.

EUROPEAN ATOMICS. FUEL GROWTH:U CONCENTRATES AND ENRICHED FUELS PRODUCTION IN INCREASING;MODERATORS AND OTHER AUXILIARIES ALSO GET ATTENTION. Chem.Engng. News 37, No. 30, 64;1959.

TECHNICAL-ECONOMICAL STUDIES OF A PRIMARY UNIT FOR HEAVY WATER SEPARATION BASED ON 1SOTOP1C EXCHANGE REACTION AT HIGH PRESSURE AND SUSPENDED CATALYST. IFA-Report (Bucarest), F5, 1959. (Unpublished)

STUDIES OF THE MARKET FOR NUCLEAR MATERIALS. II. MODERATORS. B,HEAVY WATER. Paris, OEEC, 1959.

CHEMICAL AND BIOLOGICAL STUDIES WITH DEUTERIUM. Katz J.J. Am. Scientist 48, 544-80, Dec. 1960. 229

17. MODIFICATION IN THE PROCESS FOR THE PRODUCTION OF HEAVY WATER BY ELECTROLYSIS AND THE EXCHANGE REACTION. DECREASE IN THE STEAM CONSUMPRION. Gispert M., Otero J. L. (JEN, Madrid, SPAIN). An. Real. Soc. Espan. Fìs. y Quim. (Madrid) Ser. E56, 559-68, I960. (In Spanish) (CEA-tr-X-411)

18. HEAVY WATER STAKES LURE NEW ENTRY. Chem. Eng. G7, No. 19, 92-4, Sept. 19,1960.

19. THE FUTURE FOR CHEAP HEAVY WATER. Barr F. T., Drews W. P. (Esso Res. and Eng. Co., Linden, N. J. USA). Chem. Eng. Progr.5G,No. 3,49-56, Mar. 196 0.

20. PRODUCTION AND APPLICATION OF HEAVY WATER. Kllchler L. (Farbwerke Hoechst AG, Frankfurt am Main, W. GERMANY). Chem. Ingr. Tech. 32, 773-81, Dec. I960. (NP-tr-647)

21. NATURAL ISOTOPES. II. SEPARATION CASCADES SOME PRO­ BLEMS OF ECONOMICS AND ENGINEERING. Sclecki A. Przemysl. Chem. Polska 40, No. 11,626-31, 19Gl.(In Polish)

22. THE ECONOMICS OF HEAVY WATER PRODUCTION. Proctor J. F., Thayer V. R. (E. I. du Pont de Nemours & Co. Savannah River Laboratory) TID-139G4. Dec. 6, 1961.

23. THE PRODUCTION OF HEAVY WATER. Ruzicka J. Technika Hlubokych Teplot. CSAV Pubi. House, Prague 1961. (p. 43-108)

24. CHEAPER HEAVY'WATER A BONUS FOR AECL. Can. Chem. Process. 46, 76-8,June 1962.

25. ECONOMICS OF HEAVY WATER PRODUCTION. Proctor J. F'. Thayer V. R. Chem. Eng. Progr. 58, No. 4, 53,-61, Apr. 1962. (TID-15733) > 230

2G. PRESENT STATE OF THE PRODUCTION AND OF THE MARKET OF URANIUM-235 AND HEAVY WATER. Villani S. (CISE, Milan,' ITALY). Energia Nucleare' ( Milan) 9, 212-25, Apr. 19G2. (In Italian) (AEC-tr-5200)

27. HEAVY WATER COST AND AVAILABILITY OF HEAVY WATER IN THE UK. Johnson K. D., Walker P. T. AERE-R-3905. 19G2.

28. NUCLEAR MATERLALSrWHAT'S OUR FUTURE?Can. Chem. Process. 47, G3, 65-G,Apr. 19G3.

29. POSSIBILITIES OF THE PRODUCTION OF HEAVY WATER IN ARGENTINA. Silber man E,, Crotella R. F. Commission National de Energia Atomica Rep. No. 90. 19G3. (NP-13340)

30. WHY THE GS PROCESS STILL TOPS COMPETITORS. Law C. A. Can. NucLTeclmol. 3, 36-40, 19G4.

31. TECHNICAL-ECONOMICAL STUDIES ON INDUSTRIAL PILOT PLANT CONSTRUCTION FOR HEAVY WATER PRODUCTION AT U. F. S. Savinesti (Romania). Grecu E., Mercea V., Moraru N., Olariu A., Palibroda N., Peculoa M. IFA Report (Bucharest) 033/ 13G4. (Unpublished)

Proceedings of the Third International Conference on the Peaceful Uses of Atomic Energy. Geneva Aug. 31-Sept. 9, 19G4:

32. PRODUCTION OF HEAVY WATER IN THE USA. Bebbington W. P., Proctor J.F.,Scotten W.C., Thayer V. R. 12, P/290(USA); 23 JL

33. TECHNICAL AND ECONOMICAL CONSIDERATIONS FORPRODUr CING200 t/year OF HEAVY WATER IN INDIA. Deshpande P. G.',. Gami D, C.', Nagaraya Rao S. 12, P/753(INDIA).

34. ECONOMIC OPTIMUM OF A SATURATOR-SEPARATING COLUMN CONDENSER ASSEMBLY IN.AN ISOTOPE SEPARATION PROCESS. ' Peculea M. Rev. Roum.Phys; 10, No.'4, 393-402,1965.

35. HEAVY WATER-OUR STAKES IN THE FUTURE. Can. Chem. Process. 50, 60;76, 1966.

36. COST OF HEAVY WATER PRODUCTION BY USING BITTERNS WATER. Kumar R., Datta R. L. (Indian Inst, of Science, Bangalore, INDIA). Indian Chem. Eng. 8/No. 1,2-5, 1966.

3.7. ECONOMIC ASPECTS OF INDUSTRIAL PRODUCTION OF HEAVY . WATER. Malasek E., &och O. Jad Energ. 12, 166-71, 1966. (In Czech)

•3.8. STUDIES ON THE ENERGETICAL OPTIMUM OF A ISOTOPIC SE­ PARATION COLUMN. Peculea M. Kernenergie 9, 351-5, 1966.

3.9. PRODUCTION OF HEAVY WATER AT THE NATURAL GAS FERTILIZER FACTORY, FENCHUGANJ. Shamsul A. K. M. (At. Energy Centre Dacca, Chemistry Div. PAKISTAN) AECD/CH-8. Feb.1966.

40. HEAVY WATER PRODUCTION.Report of an American Industrial Forum (A. I..F. ) Ad Hoc Committee. April 1966. 232

4.1. EXPERIMENTAL STUDY 'OF THE'.THERMOENERGETIC BEHAVIOUR OF AN ISOTOPIC SEPARATION INSTALLATION. Peculea M.'vBoiari' M.',' Fatu C.:Rev.Chim. (Bucharest) .'19, 524-9,1967.

42. A PRECISE ESTIMATION OF . PLANT AND' PRODUCTION COSTS FOR A HEAVY WATER PLANT(36, 2 t/yr) ADDED TO A 545 t/day (600 sh. t/day) AMMONIA PLANT. Linde Aktiengesellschaft Werksgruppe, Munich:19&7.

43; THE OPTIMIZATION OF A CHEMICAL PROCESS WITH GREAT. ENERGY CONSUMPTION BY ENERGETICAL METHODS. Peculea M. 5th Coni. Ind. Power Economy, Prague 1967. (II/1-22)

44. D2Ò FROM SYNTHESIS GAS LOOKS PROMISING. Can. Chem. Process.52, 71-4; 1968.

,'45. NEW LOW ENERGY PROCESS MAKES IMPACT ON HEAVY WATER PRODUCTION. Ellwood P. Chem Eng. (N.Y. ) 75, 56, 1968.

46. FLOODING BEHAVIOUR, OPTIMUM WORKING POINT, AND EF­ FICIENCY OF SEPARATION OF PACKED COLUMNS. Lentz H. Chem.-Ing.-Tech.41, 855-61,1968

47'. NELSON REFINERY COST INDEX. Nelson W.-L. (comp. )'Eri'g. ' News-Record 180, No. 12, 93, Mar. 21, 1968.

.48. AECL WANTS A 400 t/year ADDITION TO D20 CAPACITY IN CANADA. Nucleonics Week 9, No. 12, 7, Mar. 21,1968.

•49. WORLD'S HEAVY WATER PINCH CREATES POLITICAL PROBLEMS. FOR AEC. Nucleonics Week 9, No. 18, 1-4, May 2,1968. ''

50: DESALTER'CUTS COST IN HALF. Water Newsletter, Water Inf. Center, Inc. Port .Washington New'York (USA). Apr.' 22, 1968. . . 233

51. THE CANADIAN APPROACH TO CHEAPER HEAVY WATER '(1967,). Bancroft A. R. AECL-3044. Feb. 1968.

52. THE ECONOMICS OF HYDROGEN AND OXIGEN PRODUCTION BY WATER ELECTROLYSIS AND COMPETITIVE PROCESSES. Mrochck J. E. Conf. Abound. Nucl. Energy, Gatlinburg, Tenn. USA. Aug. 1068.

53. HEAVY WATER PRODUCTION IN CANADA. Law C. A. Nucl. Eng. 13; 510-2, Juno .1968.

54. HEAVY WATER. (Australian Atomic Energy Commission, research Establishment Lucas Heights) Jan. 1970.

55. TECHNICAL STATUS OF THE LOW-TEMPERATURE PROCESS FOR HEAVY-WATER RECOVERY. ON THE ECONOMY OF THE LOW- TEMPERATURE PROCESS FOR HEAVY-WATER RECOVERY. Gutowski H. Kerntechnik 12, No. 516, 233-41, 1970.

CNEN Symp.on Tech. and Economic Aspects of Heavy Water Production^ Turin, Italy 1970:

56. ECONOMICS- OF HEAVY MANAGEMENT. Rüssel S. H. (AECL, Canada);

57. OPERATIONAL AND ECONOMIC ASPECTS OF HEAVY WATER PRODUCTION AT NANGAL BASED ON LIQUID HYDROGEN DI­ STILLATION. Bimbhat K. S. (India).

58. STUDIES AND TECHNICAL RESEARCH CONNECTED WITH DEUTERIUM AND NITROGEN-15 SEPARATION. Peculea M. Bull. St. Techn. Inst. Politechnic Timisoara, Romania. (In Press)

59. OPTIMIZATION OF A HEAVY WATER ENRICHMENT PLANT WITH A HOT/COLD OPERATING H2/NH3-EXCHANGE SYSTEM. Lang G.:, Schindewolf U. (Kernforschungszentrum, Karlsruhe(West Germany). (KFK-1483; p. 804-9). July 1971. (In German) 234

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes • 1 - Chemical Exchange between Hydrogtn and Deuterium

THE KINETICS OF THE a-PARTICLE INDUCED EX­ CHANGE REACTION BETWEEN HYDROGEN AND DEUTERIUM. Mund W., van Meersche M. Bull, classe sci. Acad. roy. belg. 36, 47-G2, 1950.

HYDROGEN-DEUTERIUM EXCHANGE ACTIVITY OF CATA­ LYSTS. Holm V.C.F. ,Blue R.W. Ind. Eng. Chem. 44,107-13, 1952.

THE EFFECT OF INHIBITORS ON THE HYDROGEN-DEUTERIUM EXCHANGE REACTION. Stephan M. J., Danby C.J. (Univ. of Oxford, UK). Proc. Roy. Soc. (London) A232, 271-7, Oct. 25, 1955.

THE OXYGEN-INDUCED HYDROGEN-DEUTERIUM EXCHANGE. Klein R., Scheer M.D.', Schoen L. J. (Bureau of Mines, Pittsburg, USA) J.Am.Chem.Soc.78,47-9, Jan. 5, 195G.'

HOMOGENEOUS EXCHANGE REACTION BETWEEN HYDROGEN AND DEUTERIUM.'Boato G., Careri G.'(1st.'di Fisica, Univ. di . Roma), Cimino A., Molinari E., Volpi G.G. (Ist.di Chimica Gene­ rale ed Inorganica, Univ.'di Roma, Centro per la Chimica del CNR Roma) J,'.Chem.Phys.'24, 783-91, Apr.'1956.'

THE ROLE OF IONS IN THE RADIATION INDUCED EXCHANGE OF HYDROGEN AND DEUTERIUM.'Thompson S.O.', Schaeffer Ö..: A.'(BNL, Upton, N.'Y.'USA)J.'Am.'Chem.'Soc.'80, 553-8, Feb;5, 1958* 235

7, . THE CATALYTIC ACTIVITY OF GERMANIUM IN RELATION TQ THE ISOTOPIC EXCHANGE INACTION BETWEEN HYDROGEN AND DEUTERIUM. Boreskov G.K., Kuchaev V. L. (Karpov Physico- Chemical Research Inst. USSR).Doklady Akad. Nauk SSSR 119, 302-4, Mar. 11, 1958, (In Russian) :

8. HYDROGEN-DEUTERIUM EXCHANGE REACTIONS CATALYZED BY . Kelly M. Biochem. J. 109, 322-4,19G8. 237

F - POTENTIAL PRODUCTION PROCESSES 1.- Chemical Exchange Processes 2 - Chemical Exchange between and Water 1 - Aromatics/Water

1. THE DEUTERIUM EXCHANGE REACTION BETWEEN p-XYLENE AND DEUTERIUM OXIDE CATALYZED BY SULPHURIC ACID. Tomiko Ueda (Osaka Univ., Tokyo, JA PAN). Shokubay l,No..l, 1-7, 1959.

2. AROMATIC TRITIUM EXCHANGE IN WATER AND DEUTERIUM OXIDE. Gold V. , Lambert R. W., Satchell D. P. N. (King's Coll., •' London, UK). Chem. & Ind. No. 42, 1312-3, Oct. 17, 1959.

3. THE CATALYTIC DEUTERIUM EXCHANGE REACTION OF AND ITS DERIVATIVES WITH DEUTERIUM OXIDE BY-Ni POWDERS. Kozo Hirota, Tomiko Ueda, Kciji Kuwata, Motoyosi Hata da. (Osaka Univ. JAPAN). Shokubai 2, 181-8, 19G0,

4. THE CATALYTIC DEUTERIUM EXCHANGE REACTION OF p-XYLENE AND ANISOLE WITH DEUTERIUM OXIDE ON- METALLIC CATALYST. Tomiko Ueda, Kozo Hirota. (Osaka Univ., JAPAN). Shokubai(Tokyo) 3, No.'2, 122-6, 1961.

5# DEUTERIUM EXCHANGE REACTIONS WITH SUBSTITUTED AROMATICS. III. HETEROCYCLICS AND POLYCYCLIC HYDRO­ . Garnet). J. J,. . Sollicli W. A. (Univ. of Now South Wales Sidney, AUSTRALIA). Australian .!. Chcin. IB, No. 1, 56-04, Feb. 1962. 238

6. LABELLING OF HYDROCARBONS BY EXCI-IANGE CONDITIONS FOR HIGH YIELD. Gordon B.'E., Madison J.J. (Shell Co. Emeryville, Calif. USA) Symp. on Advances in Tracer Methodo­ logy, Los Angeles, Calif. USA). Mar. 1963. (CONF-398-1)

7, THE SELECTIVITY OF CATALYSTS IN THE HYDROGEN EXCHANGE REACTION OF p-KYLENE WITH DEUTERIUM OXIDE. Tomiko Ueda, Kozo Hirota. (Osaka Univ. JAPAN). Nip­ pon Kagaku Zasshi 84,882-6, Nov.1963. (In Japanese) 239

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes

2 - Chemical Exchange between Hydrocarbons and Water 2 - Unsaturated Aliphatics/Water

EQUILIBRIUM STUDIES ON THE EXCHANGE REACTION BETWEEN ACETYLENE AND HEAVY WATER.' Reyerson L. H.'', Gillespie B. J. Am. Chem. Soc. 57, 2250-1,1935.

EXCHANGE OF METHYL ACETYLENE WITH WATER-CATALYSIS' OF THE EXCHANGE, BY BASE OR BY ION.EXCHANGE RESINS. Stacey I.'{Columbia Univ., N. Y. USA). Ph.D. Thesis. 1956.

CATALYTIC ISOTOPIC EXCHANGE REACTION BETWEEN AND DEUTERIUM OXIDE ON NICKEL CATALYSTS. Hirota K., Hironaka Y. {Osaka Univ. JAPAN). Shokubai (Tokyo) 4/ No. 1,41-6,.1962. {In Japanese) .

THE ISOTOPIC HYDROGEN EXCHANGE BETWEEN PROPENE AND DEUTERIUM OXIDE CATALYZED BY NICKEL POWDER. Hirota K., Hironaka Y. (Osaka Univ. JAPAN). Bull. Chem, Soc. Japan 37,535-42, Apr.1964.

INVESTIGATION OF THE EXCHANGE BETWEEN METHYL ACETYLENE AND WATER FOR CONCENTRATION OF DEUTE­ RIUM. Mahadevan E.G., Taylor T. I. {Columbia Univ. USA). NYO- 755-1,Sept. 1964.

EQUILIBRIUM IN THE DEUTERIUM EXCHANGE OF ACETYLENE AND WATER. Pyper J.W. ..Long F. A. (Cornell Univ., Ithaca, N. Y;j USA). J. Chem. Phys. 41, 1890-6, Oct. 1, 1964. 240

7. ON THE MECHANISM OF H-D EXCHANGE IN ACETYLENE AT INTERMEDIATE TEMPERATURE: A RESPONSE. Bauer S. IL', Jeffers P.„Zevos N.' J.'Phys.Chem. 71,4412-G, 19G7.

8. RESEARCH PROPOSAL:SEPARATION OP HEAVY WATER UTILIZING THE ISOTOPE EXCHANGE REACTION BETWEEN METHYL-ACETYLENE AND WATER. Goldfrank J. C. Separa­ tion of Isotopes. CU-755-4, Paper HI B. 1967. 241

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 2 - Chemical Exchange between Hydrocarbons and Water 3 - Saturated Aliphatic s/Water

EXCHANGE OF DEUTERIUM OXIDE WITH BROMODICHLORO- METHANE AND CHLORODIBROMOMETHANE.ShermanR.il., Bernstein R. B. J. Am. Chem. Soc. 73,1376-7. Mar. 1951.'

SEPARATION FACTOR FOR THE H/D EXCHANGE REACTION BETWEEN WATER AND -DITHIOL-1, 2.'Haul R. A.'W.', Bienemann D. Z. Physik. Chem.' (Frankfurt) 23, 300-2, I960.' (In German) (CEA-tr-A-1381)

HYDROCARBONS FROM THE LOW-TEMPERATURE HEATING OF . Hoering T. C., Abelson. P. H. (Carnegie Inst., Washing­ ton, D. C. USA). Carnegie Inst. Wash., Pap. Geophys. Lab. No. 1440, 256-8,Dec. 19G4. 242

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 2 - Chemical Exchange between Hydrocarbons and Water 4 - Heterocyclic Hydrocarbons/Water

ISOTOPIC EXCHANGE OF ACTIVE METHYL HYDROGENS. II. DEUTERATION OF DIPHENYL-METHYLPYRYI.IUM AND METIIYLTROPYLIUM SALTS. Card E., Bally I., Vasilescu A. et al. (Inst, of Atomic Physics, Bucharest, ROMANIA). J. Label. Compounds 1, 1H2- 8, July-Sept. 19G5.

DEUTERIUM EXCHANGE OF 4-PYRIMIDONES AND 4-PYRI- MIDTHIONES. 1. Wright G. E., Bauer L., Bell C. h. (Univ. of Illinois, Cliicago, USA). J. Hclerocycl. Cheni. 3, 440-3, Dec. 19GG.

ISOTOPI 0 EXCHANGE OF ACTIVE METHYL HYDROGENS. V. REACTIVITY OF Ot-AND y -METHYL GROUPS AND ß- . HYDROGENS IN PYRYLIUM SALTS. Gard E., Vasilescu A. ; Mateescu G. D., Balaban A. T. (Inst, of Atomic Physics, Bucharest, ROMANIA). J. Label. Compounds 3, 19G-2Ü5, July-Sept. 19G7.

STUDIES ON HYDROGEN EXCHANGE. VIII. THE BASE- CATALYSED HYDROGEN EXCHANGE OF METHYL HYDROGENS OF METIIYLPYRIDAZINES AND THEIR N-OXIDES. Kawazoe Yutaka, Yoshioka Yuko, Yamada Mutsumi, lgeta Hiroshi. Chem. Pharm. Bull. (Tokyo), IH, 2000-2, Doc. 19G7. 243

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 2 - Chemical Exchange between Hydrocarbons and Water 5 - Alicyclic Hydrocarbons/Water

1# HYDROGEN-DEUTERIUM EXCHANGE IN SOME POLYAZAINDENES. Paudler W. W.', Helmick L. S. (Ohio Univ., Athens, USA). Chem. Commuti. No. 8, 377-8, 1967. 244

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 3 - Chemical Exchange between Hydrocarbons and Hydrogen 1 - Aromatics/liyclrogcn

CATALYTIC DEUTERIUM EXCHANGE REACTIONS WITH ORGA- N1CS.X1V. DISTINCTION BETWEEN ASSOCIATIVE AND DIS­ SOCIATIVE fT-COMPLEX SUBSTITUTION MECHANISMS. Garnelt J. L., W. A. Sollich-Bauingarlncr (Univ. o! NSW, Sydney, AUSTRALIA). J. PJiys. Chcin. 0(3, 3.1.77-83, Nov. 19G4.

CATALYTIC DEUTERIUM-EXCHANGE REACTIONS WITH ORGANICS. XIX. Pi-COMPLEX ADSORPTION IN THE EX­ CHANGE OP THE .Garnctt J. L., Sollich- Baumgartner W. A. (Univ. of NSW, Kensington, AUSTRALIA). J.Pliys.Chein.G'9, 1950-8, June .1 9G5.

NICKEL-CATALYSED HYDROGEN EXCHANGE OF ALKYLA- ROMATIC HYDROCARBONS AND TOLUIC ACID DERIVATIVES WITH DEUTERIUM OXIDE. MacDonalcl C. G. , Shannon J. S. (Commonwealth Scicnt. and Indus.Res. Organ., Chatswood, NSW, AUSTRALIA). Australian J. Chem.18, 1009-21, July 19G5.

RADIATION-INDUCED ISOTOPE EXCHANGE IN SOME CG- HYDROCARBONS. Kroh J., Ilankiewicz E. (Technical Univ., Lodz, POLAND). Bull. Acad. Pol. Sci. Ser. Sci. Chirn. 14, 243-4, 19G6. 2-1 ft

CATALYTIC DEUTERIUM EXCHANGE REACTIONS WITH ORGANICS. XXVII. THE ALKYLBENZENES ON SELF-ACTIVAT­ ED GROUP VIII TRANSITION METALS.Fisher B.D.,Garnett J. L. (Univ. of NSW, Kensington, AUSTRALIA ). Au&lral. J. Chem. 19,2293-2310.000.196(5.

CATALYSIS OF HYDROGEN EXCHANGE IN in-DINITROBEN- ZENE. Bunccl E., Zabel A. W. (Queen's Univ., Kingston, Ont,, CANADA). J. Amer. Chem. Soc. 09, 3082-4, June 7, 1967.

KINETICS OF HYDROGEN ISOTOPE EXCHANGE IN BENZENE USING A HOMOGENEOUS PLATINUM CATALYST. Hodges R. J., Gamctt J. L. (Univ. of NSW, Kensington, AUSTRALIA). J. Phys. Chum. 72, 1073-82, May 1068. 246

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 3 - Chemical Exchange between Hydrocarbons and Hydrogen 2 - Unsaturated Aliphatics/Hydrogen

THE EXCHANGE MECHANISM OF HYDROCARBON RADICALS WITH MOLECULAR DEUTERIUM. Voevodskii V. V., Lavrovskaya G. K. , Mardaleishvili P. E. Doklady Akad. Nauk SSSR 81, 1951. (In Russian) (AEC-tr-1538;Tcch. Trans TT-358)

HYDROGEN EXCHANGE AND ISOMERIZATION OF SATURED HYDROCARBONS WITH SULPHURIC ACID. Stevenson D. P.', . Wagner C. D. , Bccck O., Otwos J. W. J. Am. Chem.'Soc.'74, 32G9-B2, July 5, 1952.

ISOTOPE EXCHANGE OF HYDROGEN IN FREE ALKYL RADICALS. Lavrovskaya G. L., Mardaleishvili R. E., Voevodskü V.V.ydsprosy Khim. Kinetiki, Kataliza i Reaktsiónnoi Sposobnosti-Akad-. Nauk. SSSR, Otdel. Khim. Nauk 40-53, 1955. (TT-701) (In Russian)' "'

ISOTOPIC EXCHANGE BETWEEN DEUTERIUM AND HYDRO­ CARBONS ON NICKEL-SILICA CATALYSTS.Burwell H.'.L.\ Tuxworth R.H. (Northwestern Univ.'Evanston.'Ill.USA) J. Phys.: Chem. 60,1043-9, Aug.'1956. . ' ,

ON TWO MECHANISMS OF IIYDROGENATION AND EXCHANGE BETWEEN AND DEUTERIUM ON PALLADIUM. Kazanskii V. B., Voevodskii V. V. (Lomonosov Moscow State . Univ. USSR). Doklady Akad. Nauk SSSR 111, 125-8,;Nov. 1, 1956. . (In Russian) 247

ON THE ISOTOPIC EXCHANGE BETWEEN GASEOUS HYDROGEN AND SOLID POLYMERS UNDER THE ACTION OF NUCLEAR RADIATION.' Vnrslinvsku Ya. M. , Vasiliev G.' Ya, ', Karpov V. L,, Lnmrkin Yu.'S.', Poti-ov J.' Ya. Doklucly Akad, Nauk SSSR 11 ti, 315-5, Jan.' 11, 1058. (Tn Russian)

REACTION BETWEEN DEUTERIUM AND METHYL RADICALS OBTAINED ACCORDING TO POLONYI METHOD.'Ivanov O.A.', Fok N.V"., Vocvodskii V.'V.'(Lomonosov State Univ.'Moscov, USSR) Doklady Akad. Nauk SSSR 11 8, 1142-5, Feb. 21, 1 958. (In Russian) 248

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 3 - Chemical Exchange between Hydrocarbons and Hydrogen 3 - Saturated Aliphatics/l-Iydrogen

1. HEAVY WATER PRODUCTION - DESCRIPTION OF PROCESS FOR THE PRODUCTION OF HYDROGEN AND WATER ENRICHED IN HEAVY WATER. Chrones J. (Nat. Res. Council of Canada. Atomic Energy Project, Chalk River, Ont. CANADA). XM-65. May 29,1951.

2. ON THE CHEMICAL, EXCHANGE BETWEEN HYDROGEN AND SATURATED HYDROCARBONS. Varshavskii Ya. M., Vaisberg- S.E., Lozhkina M, G. Zhur. Fiz. Khim. 29, No. 4, 750-1, Apr. 1955.

KINETICS OF METHANE-DEUTERIUM EXCHANGE OVER NOBLE METAL, ALLOYS. McKee D. W., Trans. Faraday Soc. 61,2273-83,1965. 249

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 4 - Chemical Exchange between Amides, Aminoacids and Water 1 - Amines/Water

THE ISOTOPIC EXCHANGES EFFECTED, FROM A MIXTURE IN THE LIQUID OR VAPOR PHASE OF ALIPHATIC AMINES Ol OF DIMETHYLIIYDRAZTNE WITH HEAVY WATER. Pannetier G., Gucncbaut H., Marsigny L., Deschamps P.- J. Chim. Phys. 58, 790-G, Sept. 1961. (In French)

A THERMODYNAMIC STUDY OF THE TERNARY SYSTEM, TRIETHYLAMINE, WATER AND.HEAVY WATER, WITH SPECIAL REFERENCE TO ISOTOPE SEPARATION PROBLEMS. Linderstroem-Lang C. U. (Danish Atomic Energy Commission, Riso, DENMARK). Acta Chem. Scand. , 16,1730-50, 1962.

ISOTOPIC EXCHANGE OF DJ.FLUORAMINE WITH DEUTERIUM OXIDE AND TRIFLUOROACETIC ACID. Becker W. E., Impastato F. J. (Ethyl Corp., Baton Rouge, La. USA). Jan. 4, 19G5. (CONF- 650401) 250

- POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 4 - Chemical Exchange between Amines, Aminoacids and Water 2 - Aniinoacicls/Water

EXCHANGE OF DEUTERIUM AND l80 BETWEEN WATER AND OTHER SUBSTANCES. 2. ALTERNATIVE METHODS. Krause I. M., Lindcrstrjim-Lang K.' 3. DEUTERIUM EXCHANGE OF SHORT PEPTIDES, SANGER'S A-CHAIN AND INSULIN.' Ilvidt A., Linderstr^m-Lang.Compt. rend. trav. lab. Carlsberg Ser.'Chim.'29JNo.'22-23, 367-402, 1955.

DEUTERATION OF PROTEINS AND POLYAMIDES IN DEUTERIUM OXIDE VAPOR. Jeffries R. {ShirleyInst.'; Manchester, Eng. UK). J. Polymer. Sci. Pt. A2, 5161-70, Dec. 1964..

DEUTERIUM-HYDROGEN EXCHANGE BETWEEN WATER AND SILK FIBROIN. Morrison J. L. (Ontario Res. Foundation, Toronto, CANADA). Can. J. Chem. 42, 1009-15, May 1964.

COMPARISON OF WATER SORPTION AND DEUTERIUM- HYDROGEN EXCHANGE SITE IN POLY- L- VA LINE. Brandt W., Budrys R.S. (Univ. of Chicago, USA). J. Phys. Chcm.69, 1432-4, • Apr. 1965.

DEUTERIUM-HYDROGEN EXCHANGE IN AMIDE N-H GROUPS. Klotz I. M., Frank B. II. (Northwestern Univ., Evanston, 111. USA). J.Am.Chem.Soc. 87, 2721-8, June 20, 1965.

HYDROGEN-DEUTERIUM EXCHANGE OF POLYPEPTIDES. (Thesis). Leichtling B. II. (Northwestern Univ., Evanstonj 111. LISA). 1966. 251

-POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 5 - Chemical Exchange between Amines, Amides and Hydrog 1 - Amines/Hydrogen

THE ISOTOPIC EXCHANGE OF GASEOUS HYDROGEN WITH LIQUID AMINES. Bar-Eli K., Klein F. S. J. Chem. Sóc. London 3083-88, 19G2;

CATALYTIC HYDROGEN EXCHANGE- OF ANILINE ON SUP­ PORTED METAL CATALYSTS. Hagiwara Hiroshi, Echigoya Etsuro (Tokyo Inst, or Tech. JAPAN). Bull. Chem. Soc. Jap. 39, 1G83-9, Aug. 1966.

HEAVY WATER PRODUCTION BY A MINE-HYDROGEN EXCHANGE.'Bancroft A.R., Rae H. K. (AECL, CANADA) CNEN Symposium on Technical and Economic Aspects of Heavy Water Production. Turin, Italy, Sept. 30 - Oct. 1, 1970.'

AECL'RESEARCH IN ENGINEERING.'(Atomic Energy of Canada Ltd.,Chalk River, Ontario). 1971. (AECL-3787)

HEAVY WATER PRODUCTION USING AMINE-HYDROGEN ISOTOPIC EXCHANGE. Holtslander W.J. AECL Research in Engineering 5-7, Sept. 1971. (AECL-3990)

CHEMICAL ENGINEERING RESEARCH AND DEVELOPMENT FOR FUEL REPROCESSING AND HEAVY WATER PRODUCTION. Rae H. K. (Atomic Energy of Canada Ltd., Chalk River, Ontario. ' Chalk River Nuclear Labs.). Nov. 1971. (AECL-3911) lù&lil. iAl.r.^iiU.'Aì;;*

252

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes - 5 - Chemical Exchange between Aminos, Arnims and Hydrogen 2 - Amides/Hydrogen

1.. THE HYDROGEN EXCHANGE OF ALKALI AMIDES AND HYDRO­ XIDE WITH DEUTERIUM GAS. Claeys Y. M., Dayton J. C., Wilmarth W.K. J.Chem.Phys. 18, 759, 1950. 253

F. - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 6 - Chemical Exchange between Organic Aci'cls and Water' or Hydrogen 1 - Organic Acids/Water

1. ; DEUTERIOXIDE-CATALYZED EXCHANGE REACTIONS.OF iviETHYLENECYCLOPROPANECARBOXYLIC ACIDS WITH DEUTERIUM OXIDE. Bottini A. T., Davidson A. J, (Univ.-of Calif., • Davis, USA). J. Org. Chem. 30, 3302-8, Oct. 1965. •

BASE-CATALYZED HYDROGEN-DEUTERIUM EXCHANGE IN BIVALENT METAL-EDTA CHELATES. Terrill J,_B. , R'eilley' C.N.'(Univ. of North Carolina, Chapel Hill USA). Anal'chem. 38, 187G-81, Dec-, 19G6. • ' ' ' . V

• \ : '• • 254

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes * •. 6 - Chemical Exchange between Organic Acids and Water or Hydrogen 2 - Organic Acids/Hydrogen

1. THE EFFECTS OF CERTAIN NITRO AND RELATED COMPOUNDS UPON THE RATE OF EXCHANGE OF DEUTERIUM GAS WITH ACETIC ACID OVER ADAMS PLATINUM CATALYST. Smith N. A. McDaniel E. L. (Univ. of Tenn; Knoxville, USA) J. Am. Chem. Soc. 77, 533-5;Feb. 5,1955. .255

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 7 - Chemical Exchange between , and • Water 1 - Hydrides, Hydrates/Water

PROPOSAL OF A NEW METHOD FOR THE SEPARATION OF HYDROGEN AND DEUTERIUM BY CHEMICAL EXCHANGE BETWEEN SIMPLE HYDROGEN COMPOUNDS AND PALLADIUM HYDRIDE AND PALLADIUM DEUTERIDE. Salmon O.N. (KAPL,. Schenectady, N. Y. USA). KAPL-M-ONS-2(Del..). Feb. 9, 1953. Deci. del. Feb. 25, 1957.

EXCHANGE BETWEEN HEAVY WATER AND CLAY MINERALS

Faucher-J.A., Thomas H.'C.'(Yale Univ.',New Haven, Conn. USA)r J.Phys.Chem. 59, 189-91, Feb. 1955.

HYDROGEN AND. OXYGEN ISOTOPES APPLIED TO THE STUD"fr 18 OF WATER-METAL REACTIONS.EXCHANGE OF D20 WITH ALPHA ALUMINA MONOHYDRATE. Bernstein R. B."(Àrgonrie Nat. Lab., Lemont, Illinois, USAhANL-^Sg. Aug. 1958.

ISOTOPIC EXCHANGE OF A HYDRIDOPLATINUM (II) COMPLEX WITH DEUTERIUM OXIDE. Falk C.'D., Halpern J. (Univ. of.Chi­ cago, USAK J.Am. Chem.Soc.87, 3523-4, Aug. 5, 1965. 256

F- POTENTIAL PRODUCTION PROCESSES 1 - Chemical 'Exchange Processes 7 - Chemical Exchange between Hydrides, Hydrates and Water 2 -r /Water

EQUILIBRIUM IN THE EXCHANGE OF HYDROGEN BETWEEN PHOSPHENE AND WATER. Weston R.E., Bigeleisen J. J. Chem. Phys. 20, No. 9, 1.400, 1.052.

AN EVALUATION OF THE FEASIBILITY OF UTILIZING THE EXCHANGE OF HYDROGEN BETWEEN PI [OSPITINE AND WATER FOR-THE PRODUCTION .OF DgO. Bigeleisen J., Weston R.E. Jr. (Brookhavcn Nat. Lab., Upton, N. Y. USA). BNL- 156. Feb. 1952. Deci. Dec. 2, .1.955.

KINETICS OF THE EXCHANGE OF HYDROGEN BETWEEN PHOSPHINE AND WATER: A KINETIC ESTIMATE OF THE .ACID AND BASE STRENGHTS OF PHOSPUINE. Weston R.E. Jr., Bigciciscn ,1. (BroukhavcMi Nat. Lab., Upton, N. Y. USA). BNL-1655. 1953.

KINETICS OF THE EXCHANGE OF HYDROGEN,BETWEEN PHOSPHINE AND WATER : A KINETIC ESTIMATE OF THE ACID AND BASE STRENGHTS OF PIIOSPHINF^ Weston R.E., Bigeleisen J. J. Am. Chem. Soc. 7C, 3074-8, 1954.

JSOTOPIC EXCHANGE REACTIONS OF TRANS-HYDRID O- Gl 1LOROBIS (TI'METU YLPIIOS PHI.NE) PLATIN UM (II) . Falk CD., IUilpern J. (Univ. of Chicago, USA). IAEA Symposium on Exchange K

DEUTERIUM EXCHANGE BETWEEN PHENYLPHOSPHONOUS ; ACID AND WATER. Reuben J., Samuel D^Sllver B. L. (Weizmanri Inst.of Science, Rehovoth; ISRAEL). J.Äm. Chem.Soc. 85, . 3093-6, Oct. 20, 196a 258

F - POTENTIAL PRODUCTION PROCESSES 1 " Chemical Exchange Processes 7 - Chemical Exchange between Hydrides, Hydrates and Water 3 - /Water

], EQUILIBRIUM IN THE EXCHANGE OF HYDROGEN BETWEEN AUSINE AND WATER. Zcltman A. H., Gerhold G. (Los Alamos Sci, Lai)., N, Mexico, USA), J. Chcm, Phys. 31, 889-91, Oct, 1959. 259

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes •8 - Chemical Exchange between Ilydi-ogen UnlirJes and Difrorcnt.Substanccs 1 - Hydrogen Ualidos/Water

A METHOD FOR INVESTIGATING THE ISOTOPIC EXCHANGE REACTION INA LIQUID DEUTERIUM FLUORIDE MEDIUM. Varshavskii Ya. M., Lozhkina M. G. (Karpov Moscow. Pnysico- Chemical Insl. USSR). Zhur. Fi/. Khiin. 31," Oil -4, Apr. 1957. (hi Russian).

TIIPM3XC11ANGE OF DEUTERIUM BETWEEN HYDROGEN CULO RIDE AND WATER. Pugh O. , Labaton V. Y. (Gt. Brit. Capenhurst Works, Capcnliursl, Chcs. , Eng. UK). IGR-TN/CA-G52. Aug. 1957.

TWO-TEMPERATURE EXCHANGE OF DEUTERIUM IN THE SYSTEM WATER-. Vaishcrg S. E., VarshavKkii Ya. M. Zhur. Fiz. Kirim. 37, 307-9, 19G3. F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processus 8 - Chemical Exchange between Hydrogen Halides ar:d Different Substances 2 - Hydrogen Halidos/llydrogen

1. . METHODS AND TECHNIQUES OF PHYSICOCHEMICAL INVE­ STIGATIONS. A METHOD OF STUDYING THE REACTION OF ISOTOPIC EXCHANGE OF HYDROGEN IN LIQUID DEU'I'ERIUM BROMIDE, Kaliuachenko V, R., Varshavskiy Ya. M. , Shatenstein A.'I. Zhur.'Flz.'Khim,'30, 1140-3,195G. (In Russian) (AEC-tr-2976) 261

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 8 - Chomical Exchange between Hydrogen Halides and Different Substances 3 - Hydrogen Ilalides/Hydrocarbons

1. HYDROGEN ISOTOPE EXCHANGE IN HYDROCARBONS IN LIQUID DEUTERIUM FLUORIDE. Varshavskii'Ya. M. , Shatenstein A. I. Doklady Akacl. Nauk SSSR 95, 297-9, 1954. (In Russian)

2. DETERMINATION OF THE COEFFICIENT FOR THE DISTRIBUÌ TION OF DEUTERIUM IN THE ISOTOPIC EXCHANGE OF HYDRO­ GEN BETWEEN NAPHTALENE AND DEUTERIUM BROMIDE. Varshavskii. Ya. M. , Kalinaclienko V*. R. , Vaisberg S. E., Shatenstein A.I. Zhur. Fiz. Khim. 30, 1647-51, 1956.

3. HYDROGEN EXCHANGE BETWEEN AROMATIC HYDRO ~- CARBONS AND LIQUID DEUTERIUM BROMIDE. Shatenstein A. I., Kalinachenko V. R., Varshavskii Ya. M. (Karpov Moscow, Inst, of Phys.Chem. USSR). Zhur. Fiz. Khim..30, 2093-7, Sept. '1956.

4. HYDROGEN EXCHANGE BETWEEN BENZENE AND NAPHTALENE DERIVATES AND LIQUID DEUTERIUM BROMIDE. Shatenstein A. I., Kalinachcnko V. R., Varshavskii Ya. M. (Karpov Moscow Inst, of Physical Chemistry, USSR). Zhur. E.iz! Khim. 30, 2098-2105, Sept. 1&5C. 262

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 8 - Chemical Exchange between Hydrogen Ilalicles and Different Substances 4 - Hydrogen Ilalicles/Organic Acids

HYDROGEN-DEUTERIUM EXCHANGE IN AQUEOUS SOLUTIONS OF GLYCOLIC:. ACID AND OF SODIUM FORMATE. Bok L.D.C., PeUcrs L. B. J.Chem.Soc. 1524-5, Apr. 1952. 263

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 9 - Chemical Exchange between Ion Exchange Resins and Water

PURIFICATION OF HOMOGENEUS CHAIN REACTING SOLUTIONS PROTIUM-DEUTERIUM EXCHANGE .WITH AMBER UTE IR-L Adamson A. W. , Boyd G. E'. (Clinton Labs. , Oak Ridge, Tenn. USA). MonC-77.Apr.'2, 194G. Deci. Jan. 11/195C.

^2tP

ON THE REACTION OF DEUTERIUM OXIDES WITH CATION RESINS. Meleshko V. P., Myagkoi O. N., Bogatyrev K. S. (Voronezh State Univ. , USSR). Zliur, Neorg. Khim. 6, 9-14, Jan. 19G1. (In Russian) .

SEPARATION OF STAHLE ISOTOPES BY CHEMICAL AND ION EXCHANGE METHODS. Panchenkov G. M. J. Chem. Phys. 60, 107-13,1963. 264

F - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 10 - Chemical Exchange between Mercaptans and Water

EXCHANGE OF DEUTERIUM BETWEEN MERCAPTANS AND WATER. Hutchison C. , Gillies D. (Columbia Univ., New York. Div. of War Research.-USA). A-754. July 9, 1943. Deci. Dec. 8, 1955.

SEPARATION FACTOR FOR THE Il/D EXCHANGE REACTION BETWEEN WATER AND ETHANE-DITHIOL-1, 2. Haul R. W.A., Blcnneman D. Z. Physik. Chem. 23, 300-2, 1960. (CEA-tr-A-1381) 265

P - POTENTIAL PRODUCTION PROCESSES 1 - Chemical Exchange Processes 11 - Chemical Exchange between and Water

ACID-AND BASE-CATALYZED HYDROGEN-DEUTERIUM EX­ CHANGE BETWEEN DEUTERIUM OXIDE AND SIMPLE KETONES. Bothner-By A.A., C. (Mellon Inst., Pittsburgh, USA)..J. Org. Chcm.'32, 402-3, Feb. 1S61. 266

F - POTENTIAL PRODUCTION PRODUCTION 2 - Physical Separation Processes 1 - Absorptive Fractionation •

1. PRELIMINARY STUDIES FOR THE SEPARATION OF HD FROM H2 BY RECTIFIED ABSORPTION. Hanson D.N.,IIunt C.d'A;, Cook M.W., Fiele J. L. (California. Univ., Berkeley. Radiation ., . Lab. USA). UCRL-1723. Mar. 17,1952. Deci. Apr. 6, 1956.

THE SEPARATION OF HD AND H2 BY ABSORTIVE FRACTIONA­ TION. Augood D.R. Trans, Inst. Chem. Eng. 35,394-408, 1957. 267

F - POTENTIAL PRODUCTION PROCESSES 2 - Physical Separation Processes 2 - Adsorption

THE SEPARATION OP HYDROGEN ISOTOPES BY FRACTIONAL DESORPTION. Taylor H.S. ,-Gould A.J., Bleakney Wr. Phys.:Rev.,43, 496-7,1933.

QUANTITATIVE SEPARATION OF HYDROGEN ISOTOPES 3Y FRACTIONATED DESORPTION. Peters K. , LohmarW. Z. physik. Chem.'(Leipzig) 180A, 51-7, 1937. (In German) ( CEA-tr-577)

THE ADSORPTION OF DEUTERIUM BY A PLATINUM CATALYST.'Bond G. C. (Princeton Univ. N. Y. USA). J.'Phys. Chem.'60, 702-3, May 1956.

GAS CHROMATOGRAPHIC SEPARATION OF HYDROGEN ISO­ TOPES'. Glueckauf E., Kitt G. P. Proc.pf • the.Intern. Symposium on Isotope' Separation. Amsterdam 1957. North Holland Pubi. Co. Amsterdam 1958. (p. 210-2G)

THE SEPARATION OF ISOTOPES AND'ORTHO-PARA HYDRO­ GEN AND DEUTERIUM-BY PREFERENTIAL ADSORPTION AT LOW TEMPERATURE.THE THERMODYNAMIC PROPERTIES OF ORTHO-HYDROGEN AND PARA DE UTERIUM. White D.(Ohio State Univ. Research Foundation, Columbus, USA). TID-11621.' Dec.1960. r „jJJ^lIMI'Ù" ' , " V' "". ' 'SI, - /-?".' ~.- »... . • -.1': .!->I«-Ì K-^ji'^'-iö^ji^ tifassi

208

• ISOTOPE SEPARATION BY CHROMATOGRAPHIC METHODS. . Gliieckaiif" É. Separation of Isotopes.' ..H.London ed, George Newness Ltd. London, 1^61.

ORTHO-PARA AND ISOTOPE SEPARATIONS BY PREFEREN­ TIAL ADSORPTION AT LOW TEMPERATURES. White D., Haubaeh W. J., Lasscttre E. N. (Ohio State Univ. Columbus, USA). Pure and Appi. Chem. 2, Nos. 1-2, 323-4, 1961.

8. SEPARATION OF THE ISOTOPES HT AND ORTIIO-D2 BY AD­ SORPTION AT LOW TEMPERATURES. Kalorski A. , Ebcrhart J. G. , White D. (Ohio State Univ., Columbus, USA). J. Phys. Chem. 34,2189-90, June 1961.

9,i *:• THEORY OF ISOTOPE SEPARATION OF HOMO- AND HETEROr NUCLEAR DIATOMIC MOLECULES BY ADSORPTION AT LOW TEMPERATURES. Katorsld A., White D. J. Chem. Phys. CO, "29-31, Jan. -Feb. 1903.

10. . SEPARATION OF ISOTOPES BY GAS AND ION EXCHANGE CHROMATOGRAPHY. Glucckauf E. J. Chem. Phys. CO, 73-80, Jan.-Feb. .I 9G3.

11- ON THE HYDROGEN-DEUTERIUM EXCHANGE ACTIVITY OF SILICA GEL: ALUMINUM IMPURITY AND RADIATION EFFECT. Kohh H.W. Catalysis 2, 208-10, June 1963.

12. THE CHROMATOGRAPHIC SEPARATION OF THE HYDROGEN ISOTOPES INCLUDING TRITIUM. King. J. Jr. J. Phys. Chem. 67, 1337, June 1963.

13. THE SEPARATION OF H2 AND D2 BY MOVING-BED ADSORP-. TION : CORROBORATION OF ADSORBER DESING EQUATIONS. Basmadjian D. (Univ. of Ottawa, CANADA). Can. J. Chem. Eng. 41;, 2G9-72, Dec. 1963.

«•• »>'••• v-Vif. - • '. ili • 269

14. PHYSICO-CHEMICAL SEPARATION OF ISOTOPES. Hotter F., Molinari P., Dirian G. 12, P/90. (FRANCE) 3rd "UN Geneva Ccmf. 19G4.

15. THE LOW TEMPERATURE'CHROMATOGRAPHIC SEPARATION OF THE ISOTOP.IC HYDROGENS AT 25 AND 77°K. Haubach W. J., Knobler C. M., Katorski A., While D. J. Phys. Chem. 71, .1.393-402, 19(57. ri

270

F - POTENTIAL PRODUCTION PROCESSES 2 - Physical Separation Processes 3 - Cent ri fugati on

1. B-A PROPOSES D2O FROM METHANE. Can. Chem. Process 49, No. 8,47-8. 56, Aùg,Ì965.

THE REACTION OF. METHANE AND DEUTERIUM ON EVAPORAT­ ED NICKEL CATALYSTS. Kemball C. Proc.Roy. Soc. (London) 207A, '539-54/July 23, 1951.

EXPERIMENTS WITH A CENTRIFUGAL FORCE WITH SIMULTA­ NEOUS PRODUCTION OF COLD AND HOT AIR. Ranque G.I. J. Phys. Radium 4, No. 7, 1125-55, July 1933.

THE EXPANSION OF GASES IN A CENTRIFUGAL FIELD. Ililsch R. Z. Naturforsch 1, 208-14, 1946. (In German)

i 1 i, j '

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•f. • ! Ii r 271

F- POTENTIAL PRODUCTION PROCESSES 2 - Physical Separation Processes 4 - Distillation of Ammonia and Methane !

POSSIBLE DISTILLATION OR SIMILAR METHODS FOR THE RECOVERY OF D2O.Stedman D. C. (Nat.Res. Lab. CANADA). Report No. C50-49S, June 8/1949.

2. DISPROPORTIONATION IN DEUTERATED AMMONIA. Bigeleisen J. J.Chcm.Phys.20, 1495-6,1952.

3^ DEUTERIUM SEPARATION STUDY.DISTILLATION OF AMMO- . NIA AND OF METHANE. Progress Report No. 3 (on HEAVY WATER MANUFACTURE SURVEY). Drews W. P. (Esso Res. and Engineeririg'Có.|Linden,.N;.J.USA).NYO-7522.0ct. 4, 1955.Decl. Jan.12,195G. •

AMMONIA DISTILLATION FOR DEUTERIUM SEPARATION. Petersen G. T., Benedict'M. (Mass. Inst.'of Tech. ^Cambridge, Mass.;USA).NYO-2347.MaylG, I960..' •"'

5; DEUTERIUM ENRICHMENT IN THE DISTILLATION OF AMMO­ NIA. Petersen G. T., Benedict M. (MIT, Cambridge, Mass. USA). Nucl.Sci.Eng. 15,90-7, Jan. 1963. •

VAPOR.PRESSURE OF SATURATED LIQUID METHANE. Physica 32,1890-900,1964. . ' ^^^

1,< I Ml

272

11 ,1 i F - POTENTIAL PRODUCTION PROCESSES 2 - Physical Separation Processes 5 - Distillation of Other Compounds

FRACTIONATION OF THE HYDROGEN ISOTOPES IN THE DISTILLATION OF ETHYL ALCOHOL.'Widiger A.' H.', Brown W. G.' J.' Am.'Chem.'Soc.'ßl, 2453-4,1939.'

2. ' RECOVERY OF D20 AND-U02F2 BY DISTILLATION.Fischer R., Wattcnberg A. (Chicago Univ. Metallurgical Lab. USA). CC-3302. : Oct. 10, 1945. Deci. Dec. 22, 1955.

3; ENRICHMENT OF DEUTERIUM BY DISTILLATION OF DIS­ SOCIARLE COMPOUNDS. Holimberg K. .R. (Atomenergy AB., Stock­ holm).^" P/180. (SWEDEN)' 1st UN Geneve Coni'. 1955.

THE SEPARATION OF HYDROGEN ISOTOPES BY DISTILLA­ TION OF ÀZEOTROPIC ACID-WATER MIXTURES. We'txclK.., Schlitze H., Kretzschman G:', Mtihle K. (Inst, i'ilr Physikalische . Stofftrennung, Leipzig , GERMANY). Naturwissenschaften 47, 374, 1960. (In German) '. ;

M

111;''} 273

F - POTENTIAL PRODUCTION PROCESSES 2 - Physical Separation Processes 6 - Diffusion

SEPARATION OF HYDROGEN ISOTOPES BY DIFFUSION THROUGH PALLADIUM.'Harris L., Jost W., Pearse R. W. B. Proc.Natl. Acàd. Sci. U.S. 19, 991-4, 1933.

PURIFICATION OF THE HYDROGEN ISOTOPES BY DIFFUSION. Hertz G.L.Naturwissenschaften 21, 884- 5 , 1933. (In German)

A DIFFUSION METHOD OF SEPARATION OF ISOTOPES. Urey H.C. Phys.Rev.44, 314,1933.

ADDITIONAL EXPERIMENTS FOR THE SEPARATION OF ISOTOPES.'PRODUCTION OF PURE HEAVY HYDROGEN BY DIFFUSION .'ilarmsen H.', Hertz G.'L.', Schlitze W.' Z.'Physik 90, 703-11, .1934. (In German) (AEC-tr-4395) «ssMsa^^ ^1

274

F - POTENTIAL PRODUCTION PROCESSES 2 - Physical Separation Processes 7 - Thermal Diffusion

1. RESEARCH ON THERMppiFFUSION IN THE LIQUID PHASE; THERM OD IFFUSION IN HEAVY WATER. Prigogine I. ,De Brouckère L. ,Buess R.Physica..18, 015-20, Nov. 1952.

2. THE SEPARATION OF HYDROGEN AND TRITIUM BY THERMAL DIFFUSION. Boorman C., KronbergerH. (UKAEA Ind. Group. Risley UK) Proc.Int. Symp. on Isotope Separation. Amsterdam 1957. North Holland Pubi. Co. Amsterdam 1958. (p.471-7)

3. THERMAL DIFFUSION FACTOR FOR HYDROGEN AND WATER MIXTURES. Saxena S. C. (Atomic Energy Establish.', Trombay, INDIA). Indian J. Phys. 34, 449-55, Oct. I960;:' '

4/ THE THERMAL DIFFUSION COLUMN. Vasaru Gh., MMer. G., Reinhold G., Fodor; T. VEB Deutscher. Verlag der Wissenschaften, Berlin 1969.

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\ / V»i . ^ K ~f^A -•'aj 1 ,& j 1 vV* k »^ .i *ift' i: l 275

F - POTENTIAL PRODUCTION PROCESSES 2 - Physical Separation Processes 8 - Solvent Extraction

FINAL REPORT ON LABORATORY SEMIWORKS TESTS OF TRIETHY-LAMINE IN SOLVENT EXTRACTION. Bebbington W. P. SAMReport A-1916.Sept. 1943. '

LIGHT WATER SEPARATION WITH TRIETHYLAMINE. Hahn H. T.; Street E; B. (General Electric Co.Hanford Atomic Products Operation, Richland, Wash. USA). HW-48735. Feb. 22, 1957. 276

F - POTENTIAL PRODUCTION PROCESSES 2 - Physical Separation Processes I 9 - Others

SEPARATION OF ISOTOPE MIXTURE BY NOZZLE PROCESS. Mikami 11., Oyama Y. Bull. Tokyo Inst. Technol. Spec. 49, 167-80, 1962.

SEPARATION OF GASES AND ISOTOPES IN A WHIRLING TUBE. Bornlccsscl 1C, Pilot J. Z. Physik. Clicm. 221, 177-84, 19G2.

CHARACTERISTICS OF A VORTEX TUBE. SokoloyJE.Y. Thermal Eng. 13, No. 7, 84-91, 1 966. *>»•;"' 277

F - POTENTIAL PRODUCTION PROCESSES 3 - Others

1. ENRICHMENT OF HEAVY WATER BY BIOLOGICAL METHOD. Webb J. (Coll.' of Technology, Belfast, UK). Nature 177, 988-9, May 26,1956.'

2. PHOTOCHEMICAL SEPARATION OF ISOTOPES.'Rozenberg J. Isotop.' Radiat.' Technol.' 3, 200-5, Spring 1966. V - HEAVY WATER REACTORS V,A - HBAVY-WATER-KODERATED REACTORS IB THE WORLD

Location Power Type Fuel Pirnt criti­ Sezarks cal ity data

ABCCT7rMA

Central nuclear «a Atucha Atucha (Buenos AyreB) 319 We PWH UQ2 197 4 Centra"* Nuclear en Rio Tercero Jtto Tercero (Cordoba) SOD Itffa PHSH Bat V0\ 1960 ccesitted AUSTRALIA HlPAR Lucas Heighta, Sydney 10 «t RR highly enr. O-Al alloy Jan.. 195S eiallar to DIDO (UK)

BELGIWI z VEBÜ3 *ol <0,5 kwt CE U02 (7* 350) Apr. 1964 2 BH-E/Vuleain Power Plant Hol 10,£ «e SSO tJ02 (7)1 3&0) Dec. 1966 1964-66 P#R; 1966-59 S5H; fro« July 1969 CABADA rwji 2EEP '-'' Chalk Elver, Ontario . 0,1 kWt CE Bat U metal or oxide. Fu, Sept.1945 235o BRI Chalk River, Ontario 40 ir#t TR Bat ti natal July 1947 original 20 Wt TOO . Ctalk River, Ontario 110 KWt TR Bat 0 retai Nov. 1957 original 200 SWt ZED-2 - Chalk River, Ontario 0,1 k»e CE Bat U netsl or oxide Sept.1950 2l5 WR-t . «hiteahell 40 ¥*t PE 002(2,4* U) Nov. 1965 BPD power Plan Rolphton 22 Ff«e BHWR Nat D02 Apr. 1962 eo&vertea froa PHWR to BH*H In i$6B; operating fron Peb. 1969 Douglas Point (CATOU) Power PI. Tiverton, Ontario 203 We PHWfi flat UOa Nov. 1966 CentIlly power Plant Centllly, Quebec 250 **e H*BLWR Nat U02 Hov. 1970 Piekering-1 Pickering, Ontario 508 X*e PHWR Nat U02 Feb. 1971 MeVering-2 Pickering, Ontario 508 We FJflTH Bat 0D2 Sept.1971 Pickering-3, -4 Pickering, Ontario 2x508 K#e PHWR Bat U02 1972,1973 Bruca-1, -2, -3» -4 Power Plant Oouglaa Potat-LaVa Huron 4x750 KWe P«*R Wat no% 1976-1979 under construction

CHIBA P.H. TVH-S Peking 7/10 KWt RR 195B TVR-S (USSR)

CZECHOSLOVAKIA TR-0 HBZ, Prague 3 kwt max CE Kat U 1970 A-1 Power Plant Jaalovake Bohuni.ee, Slov. 110 We H*GCR fiat 0 Oct. 1972

DEMARK DR-3 RtflS 10 H*t TR highly enr. U-Al alloy San. 1960 einilBr to PLUTO (UK)

PRABCE

EL-1 (ZOE) Fon t enay-aux-Ro sag 150 k*t RR Bat 002 Dee. 1948 original 3 k*t EL-2 Saclay 2500 Wt TR Bat U setal Oct. 1952 shut down in Sept. 1965 Aquilon Saelay ne gl. CE Nat ti metal Aug. 1956 shut down in Key 1967 BL-3 Saclay 20 Ifft TR U03O.35< &*UÌ July 1957 EOLE - Cadsracha 1 kVt max CE Nat + enr. II Dec. 1965 EL-4 Power plant Brennilis 70 We HeGCR O02(1,65* 235u) Dec. 1966 HPH Grenobl* 57 J«t TR highly ear. U-Al alloy Aug. 1971 Prench-Oersan collaboration

GERKASY P. 71. 44 Kwt in PR-2 Karlaruhe 44 KU TR Bat 0 metal Sar. 1961 power lncreaaet! fro» 12 to July 1966 PfiJ-2 ::' Jalieh 15 tf*t TB highly enr. U-Al alloy HOY. 1962 als.ilar to DIM(UK); po-er increased rroa original 10 to 15 Wt in Dec.1967 KZPR ' .: Karlaruh« 52,5 *#a PHWH Sept.1Q65 235 KKN-Karnkraftwerk Niedaratchbach Siedereichbach 100 Me K*CCH U02(1,151C 0) 1972 under construction

IBDIA CIRUS Troabay . 40 Mft TR Sat U setal July i960 ZERLINA !" Trombay 0,4 Wit CE variable Jan. 1961 Hsjasian-), Power Plant Rana Pratap Secar 200 »Yt PH*R Bat Ü02 1972 Hajastan-2 Power Plant Bann Prntap Sag&r 200 XI a PHWR Wat U02 1974 under cosstraccion Kalnakkaa- Power Plant KalpaWeaai, Eadraa 2x200 me PHVR flat U02 1976 -1979 Karlsruhe 52,5 KKB PHWR Hat U02 _ Sept-1965 KXK-Kertlcrafftwerk Ntedaretehbaeh Riedereichbach 100 KM* Ma^.15* 235Ui WI4 unfier construction

IlfDIA CJHbS Troabay 40 Wt ' TH 5at Ü metal July 1960 ZERLIHA Trombay 0,4 Ht CE variable Jan. 1961 Rejaatan-I, power Plant Rana. Pro tap Setar 200 ttHt PHWR Hat U02 1972 Tiijagtan-a Power Plant flann Pratap Cagur '200 »We PH#R »st U02 1974 under eoaatrjetion Kalpakkan- Powar Plant Kalpakkoa, Vadras 3x200 ne PH*R JTat IM J 1976 -1979 under construction

ISRAEL IRR-2 Disona 25 mrt TR Rat V Sec. 1963

ITALY 2 Ieprs-1 lepra 5000 kit TR U-Al alloy (20jC ^\J) Bar. 1959 •latilar to UTB ECO lepra 1 Wt sax RR Hat U metal Dec. 1965 ESSOH lepra 40 Wt PE Hat nc+hitfhly enr.U-Al all *er. 1967 -, RB-i Bologna negl. CE Rat U aetal Aug..1S7l French "Aquilon* CIRENE Power Plant Latin« 40 KV«' ItwPCR flat UOj 197 7 JAP AIT JBR-2 Tokai Mura, io wt TB highly enr U-Al alloy Oct. i960 .. - * LICJk (ftHGP; AHB) Toltai. Iura 0,05 Ht CE uranS- oulphate (20]l **5U) Juna 1961 «nut down Sac- 19&7 in D20 ."' J HB-3 Total Mura ', io nt TH Hat ti metal Sept.1962 - OCA aagl. CE puora Tauruga 165 «a HWBL"3 UOjO.W ?35U> 1975 tfWH prototype under construe t tan V HORWAY JEEF-1 Kjeller 450 Wt RR Kat ü metal June 1951 original lOO kWt HIBH HaldATL 20 nt PE U02(l,5* *l'ö> Juno 1959 NORA Kjeller 0,1 kWt CE Hat 0 metal or U02 sl.enr. June 1961 JEEP-2 Kieller 2000 JcWt RR VOgO,?* W5«) Sec. 1965

PAXISTAK ' >- KATDPP-Xarschi Huclear power Pinot Paradise Point, Karachi 125 We PH*R 5at UO2 Aug. 1971 10UTH AFRICA '*•

Pelinduna Zero r P»llndaba, Pretoria negl. CE Ifov. 1967

SWEDEN - r ' V * R-1 Stockholm 0,6-1 OTt HB Ras Ü* metal July 1954 R-0 Studavik 0,05 kvt CE {Tat 0 metal Sept.1959 B-3/Adan Power Plant Agesta 12 We PHWS Bat UU2 July 1963 62 ywt (dual purpose reactor) R-4/EVB Power Plant «nrviken 135 We BCTR - - the tranaforaatica in BWS stopped in *70 • SWITZERLAND DIORIT W&rnlIngen 30 »rt TR Hat 0 metal Aug. I960 original 20 Wt Lucana power Plant' Lucena 5,8 We HVGCR 0,96^ enr. U Dee. 1966 shut down in Jan. 1969

' OTI03 OF SOVIET SOCIALIST HEP. TVR XOBCB 2500 k*t RR 80* enr. U Apr. 1949 original 500 k*t

s TVR-S 20 Wt max RR for export tmiTRft KTNQDOH DIM Karwell 15 Wt TI highly enr. U-Al allay Bov. 1556 original IO avt PLUTO Harwell 22,5 Wt TR highly enr. U-Al alloy Oct. 1957 original 10 Wt HAZEL Harwell 0 CE uxanyl fluoride (45.5J«- Peb. 1958 shut down in July 1958 ,.* 235u) in D20 DHTR Dounraay 22,5 Mft TR highly anr. U-Al alley Kay 1958 similar to PLUTO; shut do*n in May 1969 DAPKSE Harwell 0,1 kWt CE highly enr. U-Al alloy Peb. 1962 • DIKPLE Vlnfrttb Heath 0,1 Wt CE variable June .1962 . originally in Harwell; critical at fin- triti Heath In July >954 JUHO VinXrith Heath. 0,1 knt mt ünrPn Apr. 1964 SOKWB Power Plant •"ioJrith Heath 100 We HW3LWR UOj (2,28)C Z35a) Sept.1967 * ÜMTED STATFS Or ATTICA Kay 1944 «hut dtnm in Kay 1954 - CP-3 Argonne, 111. 300 Wt HS Mat U aetal 1 PDP Aiken, S.C. 1 kit BR Hat or ear. U Sept.1953 CP-5 Argonne. 111. 5 Wt RR highly ear. U-Al alloy Peb. 1954 • 1IRE-2 Oak Bidga, Tens. 5200 Wt RR highly e^^. Uranyl sul- Dec. 1957 abut down 1B Apr. 19&1 phate in D2O I «TTR Cambridge, ansa. 5 mrt RR highly enr. U-Al alloy July 1958 P3E SUL, Aiken, S.C' negl. CE Hat U -lov. 195Ö 5PEM II Idaho Palla, Idrho transient RR highly enr. U-Al alloy Mar. I960 shut down. to. 1365 * PRTR Richland, Wash. 85 Wt TH Pu-Al alloy *- nat. or de­ Nov. 1960 ' pleted UO2 HWCTS Alken» S.C. 61 Wt TH highly enr. U-2r alloy Nar. 1962 shut do«n In Dec. 1964 4 f CVTH Power Plant Parr Saoala, S.C. 17 We pHwa -i,6i enr. U Kar. 1963 with oil fired superheater; ah« down m UTK* Atlanta, Ca. 1000 Wt RR highly enr. U-Al alloy Dec. 1964 1907 ALHT Ases, Xo-a 5000 Lift RS highly «nr. U-Al alloy 1965 HPBR Upton, R.Y. 40 l»t TH highly enr. U-Al alloy Oct. 1965 K_.* RTR Aiion, S.C. 1 k*t RS 1967 JBSÄ Gaithersburg, Uà. 10 K>t TR Highly enr. U-Al alloy Sec. 1967 - YUGOSLAVIA RH Vinca, Belgrade nasi. CS Nat. or 2jC ear. U Apr. 195Q RA Vinca, Belgrade 6,5/10 Wt RH 2* enr. U Dec. 1959 TYri-S (USSR)

CE • Critical experiment PKVR • Fr*3Burixed heavy water moderated and cooled reactor 33C • Spectral «hi« controlled reactor BHWR * Boiling heavy water cooled, heavy water soderated reactor R8 - HBaaarca reactor KVCCR * Heavy water moderated, gas cooled reactor 18 - Teat reactor tfrpCEt • Heavy water fog cooled reactor PE « Power experiment H*BI*B « Heavy water colling light water reactor 2H3

B - HEAVY WATER REACTORS IN NUCLEAR POWER PROGRAMS

1. NORVEGIAN ATOMIC RESEARCH. Gliom, and Eng. News 2G, 3780,Dec. 20, 1948.

2. AUSTRALIAN A.E.C. RESEARCH PROGRAMME. Walson-Munro C. N. (Australian Al.omic Energy Commission, AUSTRALIA). Nuclear Eng. 1, 183-5, Aug. 195G.

3, REPORT FROM SPAIN: SENSE OF URGENCY GRIPS MADRID ON NUCLEAR POWER; CONVENTIONAL SOURCES TO BE FULLY EXPLOITED IN 10 YEARS. Nucleonics 15, No. 7, 2G, July 1 957.

4. NATURAL OR ENRICH KD URANIUM FOR POWER REACTORS?. Lewis \V. B. (Chalk River, Out., CANADA). AtomwirlschaR 2, No. 9, 285, Ì957. (In Cprman)

5. ANALYTICAL CONTROL OF HEAVY WATER IN REACTOR. MODERATOR SYSTEM. Zcmyan E. M. (Du Pont de Nemours E. I. & Co.. Savannah River Lab., Augusta, Ga. USA). Analytical Chemistry in Nuclear Reactor Rechnology Nov. 1957. Gatlinburg Tonn. USA. TID-7555. (p. 175-83) !J.'ÌLJ£Z,±ÌU**&Ì'>*~<'^ÀVJ.

2M4

Proceedings Di'Ilio Second United .Nations International ConJ'oren- cc on tlio Poacci'uJ l;s"K ol'Alomk: Energy, Geneva IDS!!: G. HEAVY WATER MODERATED AND COOLED POWER REACTORS. Eabeovk I). !•'. », P/fill) (USA):

7. TI!!1: NUCLEAR ENERGY PROGRAM AND ELECTRIC POWER PROBLEMS IN SPAIN. Oloro Navascues .1. i\l. J, P/2U3G. (SPAIN)

8. NUCLEAR. POWER PLANTS. Pelrov. P. A. Gosenergor/rlat, Moscow 1953. (In Russian)

9. FINANCING NUCLEAR ENERGY PROGRAMS AND RELATIONS BETWEEN THE STATE AND JNDIJSTRY. OECE, Paris, 1 959.

10. ESTIMATES OE NUCLEAR* ENERGY PRODUCTION IN EUROPE 1958- L'Jfif). NATIONAL PROGRAMMES. BASIS FOR CALCULATING CAPITAL COSTS-COSTS FACTORS. OECE Paris, 1959.

USAEC Symposium on l>2(-)- moderated reactors. Germantown, My. USA. Alar. 1.959. TtD-7575:

11. ACCOUNTING PARTICLES FOR. D20 IN POWER - REACTOR OPERATION. Shepherd 1:3. Ü/SAEC)TTJ.D-757Ö p. 11-1.4;

1.2. FUTURE REQUIREMENTS POR. D.,0. Lane J. A. (ORNL, Temi. I/SA):T!I>-7!V75 p. 15 WW; 285

r l J. CAPABILITY OF ARC TO SUPPLY D20 FOR FUTURE NEEDS. lUiUcrv/orlh A.-V. (UÖARC, Wash. I). C. ).TI.D-7r>7r> p. 23-7.

14. ADVANCED COURSE OW HEAT EXTRACTION FROM BOILING WATER POWEII REACTORS AND ASSOCIATED DYNAMIC PROBLEMS, (PL II). Nethcrlantls'-Norwoginn Reactor School. KjclJcr, Norway.'Aug. 195)9. (NP-928G) .

15. HEAVY WATER IN HEAVY-WATER BASED NUCLEAR POWER PROGRAMMES. Ortiz Fornagucrn R. («TEN, Madrid, SPAIN). EAES Enlarged Symposium on Heterogeneous Heavy Water Power Reactors, Majorca, Spain, Oct. 19G0. (CONF-4 J 0-1)

16. A CANADIAN APPROACH TO NUCLEAR POWER. Gray J. L. AECL-lt55.Dcc.19G0.'

17. AN Il20-D20 MODERATED REACTOR. HebbinglonW..P. (Du Pont dc Nemours E, I. & Co., Aiken, S.C. USA). Nuclear Sci.and Eng. 8, '720,'Doc. 1960.

18. REACTOR HANDBOOK. .2nd Ed. Revised and Enlarged. Vol. I. Materials. Tipton Jr. C. R. N'3W York, Intorscicncc Publishers •I960.

19. ECONOMIC POTENTIAL FOR D20 POWER REACTORS. Isakoff 1. (Du Pont Co. Aiken, S. C. USA) DP-570. Feb. 1 961.

20. SPKCIALPHYSICO CHEMICAL PROBLEMS RELATED TO THE USE OF HEAVY WATER IN REACTORS.Dirian G. Bull. Inform. Sci. Tech. (Paris) No. 87, 55-G7, Oct. 19G4.(In French) 2H0

21. ANALYSTS OF HEAVY WATER IN VIEW OF ITS I'REPARATION AND USF, IN NUCLEAR REACTORS. Rolli E. Colloquium on Heavy Water. Madrid, Doc. 1962. (JEN Madrid and EAES Paris). NP-.1.37GG. p. 135-54. (In French)

22. HEAVY WATHIR POWFR REACTOR PROGRAM MONTHLY PROGRESS REPORT, .IANI/ARY 1364. (Savannah River Opera­ tions Office, IJSAEC). SRO- 98.,Ian. 19G4.

23j THE CSVTS 3rd CONFERENCE ON NUCLEAR ENERGETICS. Maiasek E. Prague. 19(54. (in Czech)

24. ACCOUNTING SYSTEMS FOR HEAVY WATER AND FISSIONABLE MATERIALS. Fletcher G. W., Reid II. R., Jenkinson W. G. (AECL, • Chalk River, Out. CANADA). AECL-2202. IAEA Symposium on Nuclear Materials Management, Vienna,Aug. 30-Sepl. 3,19G5. (CONF-6 50803)

25. THtRD REPORT ON THE COMPETITIVITY OF NUCLEAR ENERGY. Serie Studi Economici. CNEN 1 965. (In Italian)

2G. THE CHANGING PATTERN OF PROBLEMS IN THE USE OF HEAVY WATER IN NUCLEAR REACTORS.Dole. L. (CEN, Saclay, FRANCE). Ind. At. 9, No. 7-8;57-G9, 1065. (In French)

27.. A COMPARATIVE EVALUATION OF. ADVANCED CONVERTERS. Rosenthal M. W. et al. ORNL-308(5. Jan. 1 9(55. . ,

28. DEMANDS FOR NUCLEAR FUELS AND .COSTS OF DIFFERENT; r REACTOR TYPES IN GERMANY. Grümm 11.,.Gupta D., HhTelp W. et al. KFK-3G(>. Soni. 19(55. :,, ..;• .:-.,.-:

29. WORLD FORECASTS OF NUCLEAR CAPACITY TO .1 985. Merlin. n.'H.et al. Canadian Nuclear Association Report (55-CNA-200. 1 9(55. ANALYSIS OF THE STUDIES ON THE ECONOMY" OF U-Th CYCLE. Scui'icim CI. D., Lav reticle D., LIUTKHU A. , VendLUi P.EUR 2537Ì, 19GG.(In UnlLan)

ACHIEVEMENTS AND PROSPECTS OF HEAVY WATER REACTORS. Lewis W. B. (AECL, CANADA) DL-73. 1966.

THE ROLE AND REQUIREMENTS OF HEAVY WATER IN CANADA AND THE WOULD. Cochrane Ò. R. (Canadian Nuclear Association, Toronto, Onl. CANADA)6G-CNA Paporr301. Annual Conference on Organic and Heavy Water Reactors, Winnipeg, Canada June 1966. (CONF-GGOolG-lü)

UTILIZATION OF DISCHARGED URANIUM IN HEAVY WATER REACTOUS. Grllmm [I. Nuldeonik I), No. 8, 1 f)GG. (In German)

THOniÜM'BREEDERS AND CONVERTERS THEIR INFLUENCE ON FUEL CYC LE'ECONOMICS AND FUEL UTILIZATION. Kasten P.R. AEC Symposium on Thorium Cycle Gatlinburg, Tenn., USA. Feb. 19GG.

SUPPLEMENT TO KFK-3GG:DEMANDS FOR NUCLEAR FUELS AND COSTS OF DIFFERENT REACTOR TYPES IN GERMANY. Grllmm It.,.Gupta D., IlHfelc W. et al. KFK-466, Sept. 1966. (In German)

,CANDU REACTORS TO 1980 AND IN THE LONG TERM. Gray J. L., Lewis W. B., Haywood L. R. 15 th" Sectional Meeting of the World Power Conf. Transactions. Tokyo Oct. 15-20, 1966. Vol. Ill p. 1487-97. 2HH

37. 11 RAW WATER POWER REACTORS. Millar C. IT.. (AEC, Chalk River, Out. CANADA). AEOL-2Ü27. Nov, 19CÌCJ.

38. FOURTH REPORT ON THE COMPETITIVITY OF NUCLEAR ENERGY. Serie Studi Economici. CNEN 1907. (In Kalian)

39. DEVELOPMENT OF HEAVY WATER POWER. REACTORS IN THE FEDERAL REI'UDLIC OK GERMA NY. Keller W.FAES Symp.on .the Kufure of Advanced Converters Portugal. Apr. 1 9G7.

40. REVIEW Ol«' LOKS FORECAST OE INSTALLED NUCLEAR CA­ PACITY (I i)70 - I 9Bi>). Merlin II. B. AKCL-2H75, Apr. 1 9G7.

4J. A PROGRAM TO SURVEY CANADIAN DEUTERIUM SOURCES. Bancroft A. R. , Drown R. M. (AECL, CRNL, Chalk River, Out. CANADA) AECL-2573. July 19G7.

Heavy Water Power Reactors. IAEA Symposium, Vienna, Sept;1967. 1AEA19GU. 42. PROGRESS IN THE DEVELOPMENT OE HEAVY WATER MODE­ RATED AND COOLED THORIUM-1 IRANI UM-233 CONVERTER. Steiner! C. (W.GERMANY) (SM-90/7) p. 44 3-50;

43. COSTS AND ECONOMICS OF IIEAVY-WATER-MODERATED NUCLEAR PLANTS. Haywood L. R. , Aikin A.M. (AECL, Chalk RivCM-, Onl. CANADA).p^ififi.jjo.(AFCI,-2!).|fi. li)f;7): :w>

•I-I. OUTLOOK l-'Oli IIEAVY-WAT.KU. HNACTOHS. LRWJK W. 13. p. 545-1).

45. TUR USE Ol"' THORIUM IN HEAVY WATER MODERATED REAC- TOUS. Cra'/.inni Ci., Rinaldini C., Zananloiii C. Kneryia Nucleare (Milan).15, No. (>. .»%».

4«. IIKAVY WAT 1.1 R REACTOR PROGRAM PLAN. Ilarl.y 11. BNLW-B56, Mur.'l, 19G8.

47. ILLUSTRATIVE POWER RTOACTOll PROGRAMMES. OF-CD-ENEA. Mayl9(i8.

Economics of . IAEA Symposium, GoUwaldov (GSSR) Mayl9G3. IAEA 19(Ì8. 40. AVAH.IATHLI1TY.1TS INFLUENCE ON LONG-TERM REACTOR PROGRAMMI«. ScurJoi'ni G. P.., Lavrencic D., Valnnt P.

49. E VALUATION OF VARIOUS FUEL CYCLES IN HEAVY-WATER - MODERA TEH ClRENti-TYPE REACTORS. Cardosi G., Vcndilti P. (SlVI-i()r>/.'i2)

50. REVIEW OF HEAVY WATER REACTOR PHYSICS. Uotincn V. O., Schmid L. C. (BaUcUc-Northwesl, Richland, Wash. Pacific North - . ;\vcsl Lab. USA). RNWL-1119. May 196«.

Utilization or Thorium in Power Reactors. IAEA Panel, Vienna, June 1.9 Ci 8; 51. THORIUM UTILIZATION ACTIVITIES IN ITALY. Ambrosini G. C., Ncpi O., Baldctti S;

52. A TWO TYPK STRATEGY OF DaO-NATUHAL URANIUM REAC­ TORS AND ADVANCED HIGH- POTENTIAL CONVERTERS OF STKMI'INS AG.SIeinerl C. •»M

53. TIIIS KCONOM1C POTENTIAL OK DI FFKR10 NT ADVANCED RKACTOR COÌVCKPTS IN A FUTURE POWIOH. GENERATING SYSTKMS. Hoolluhur A.,Kr!lmer II,, Wagcmaiin K . (W. GKRMANY) ANS Winter Meeting Int. Washington D.C. Nov. Jf)(i».

54. NUCLKAR. ENERGY IN CANADA : Pit KSK NT CONDITIONS AND PROSPECTS. Casa A. I-1., Pcrilli M. L., Sansone M. Notiziario CNHN l'l, No. 12, «5-01, liner. 1«)fifi.(lii Italian)

CAN THORIUM COMPETE WITH URANIUM? AN ASSESSMENT OF HEAVY WATER AND GRAPHITE MODERATED REAC.TORS. Oraziani G. , Rinaklini C., Znnanluni C., Devos J. J., Paruccini M. EUR 424G ol 969.

5G. ANNUAL REPORT, 1 9GS-19G9. (Atomic: Energy of Canada Ltd., Ottawa, Olii. CANADA). AECL-332G. 19G9.

57. SOME FA (.)NOi\l!C ASPECTS OF BREEDING IN THE THORIUM (••(JELLED IIEAVY-WA'1'ER REACTORS. (LE VALUBREEDER). Charpeniier M. Energie NucJéaire 11, May 1969. (In French) _,

5». TIPS ECONOMIC PROSPECTS OF HEAVY WATER REACTORS. Mandel H. Atomwirlsehal't, Atomledi. 14, No. 7, 347-53, July 1969. (In German) (Notiziario CNKN I 5, No. 12, 87-93, Dec. 19G9. In Italian)

59. HEAVY WATER IN CANADA'S POWER REACTORS. Rae H.K., Charlcsworth D.H., Bancroft A. II. (AECE, Chalk River, Onl:., CANADA). Rug. J. (Montreal) 52, 1.7-2.1, Dec. 19G9. •

GO. HEAVY WATER. (Australian Atomic Energy Commission Research Establishment, Lucas Heights). Jan, 1970. (INIS-ml-23) 2'H

.STATUS OF HEAVY WATER REACTORS IN Till*] WORLD. Paulieka I. (Boluinico Atomic Power Station, Czech. ). (Jn Slovak) (CONF-7012J4, Paper No. 13. 5th conference on nuclear power; Piostany, Czechoslovakia, Doe. I 970)

FlF'Hl REPORT ON THE COMPETITIVIT/Y OF NUCLEAR ENERGY. Serie Sludi Economici. C NEN 1970. (In Italian)

POWER AND RESEARCH REACTORS IN MEMBER STATES. 1971 Edition. IAEA, Vienna 1971. STI/PUB/194/4.

DIRECTORY Ol*1 NUCLEAR .REACTORS. IAEA, Vienna. Power Ueaclprs. Vol.I-STl/PUB/4(1950);Vol.lV-STl/PUB/53(19G2); Vol. VK-STI/PUI3/174(19(i8);Vol..IX-STJ/PUB/29ü(1971).

DATA FOR CALCULATING VALUES ON NUCLEAR FUEL CYCLES, pp. 51-75 ol'Coneeplion on Nu e.I ear Energy Till 2000. A.D.Tokyo, Japan Atomic Industrial Forum, Ine. 197.1. (In Japanese)

OPTIMUM SEKING METHODS APPLIED TO NUCLEAR REACTOR DESIGN! "CASE STUDY OF.'MINIMIZING FUEL AND HEAVY WAT Kit COSTS. Suda N. (Osaka Univ. ), Oyo K. Nippon Gonshiryoku Gakkaishi 14, No. 8, 422-9, Aui<. 1972. (In Japanese)

ADVANCED IIWR POWEJt PLANTS. Lewis W.B. (Atomic Energy oi' Canada Ltd., Clialk River, Ontario. Chalk River Nuclear Labs.). Nov. 1972. (AKCL-4^04.CONF-720817;DL-] 10. Conference on Nuclear Power for Tomorrow. Atlantic City, New Jersey, USA. Aug. 1972)

ADVANCED NUCLEAR REACTORS. Caprioglio P.(CCR Euratom, Ispra, Italy). Knor«. Nuci. (MiJan) 20, No. 2, 75+80. Fol>. 1973. (In Italian)

GENTILLY-CANDTJ-BLW PLANT: INITIAL OPERATING EXPERIENCE. Com. Naz. Euer»-. Nucl. Noli'/. 19, No. 2, 85-88. Pel;. 1973. (In Italian) 292

70. CIRENE PROTOTYPE. Bromato A. (CNEN, Milan), Casagrande I., Podretlt A. Com.Naz. Gncrg.Nucl. Notiz. 19, No. 3,28-42. Mar. 1973. (In Italian)

71. CIRENE RESEARCH AND DEVELOPMENT PROGRAM. Mancini C. (CNEN, Milan), Villani S. Com. Naz. Eiiorg. Nucl. Noti. 19, No. 3, 43-82. Mar. 1973. (In Italian)

72. PROSPECTS OF UTILIZATION OF THE CIRENE REACTORS. Barabaselii S. (CNEN, Milan), Cawtollt G., Silvestri M.Com.Naz. Enui-K. Nucl. Noti-/.. 19, No. 3, «3-90. Mar, 1973. (In Italian)

73. APPROXIMATE CALCULATION METHOD FOR DESIGNING THE CORE SUPPORT STRUCTURE OF A PRESSURE TUBE REACTOR. Cravarolo L. , Zeiger P. (CISE, Segrato, Italy). Energ. nucl. (Milan) 20, No. 5, 280-292. May 1973.

74. SOURCE MATERIALS FOR NUCLEAR ENERGY. 1972 Atomic Energy Programs:Operating and Development Functions;. (TID-26277, pp. 29-44) 293

C - TREATMENT OF DEGRADED HEAVY WATER

PURIFICATION OF D2O MODERATOR BY ION EXCHANGE. Hcston W. M,, BanicK- C, .1,, Wilson T. II. (E. I. du Pont de Nemrjiirs & Co.Savannah Riven- Lal>. Aiken S. C. USA). DP-73. .Tune 1954.

APPLICATION OF MIXED-BED ION-EYCHANGE TO WATER PURIFICATION IN NUCLEAR REACTORS. SLvotz N., Scheibelhut C.IJ. In<.I.Eiitf.Chem.47,No. I), 1020, 1955. (Part I);Ind. Eng. Chem. 47/No. 10, 2140, 1955. (l'art If.)

RE-USE OF COOLING WATER IN AN AEC INSTALLATION. . Rilmloau A. L. Ind. Eng. Clicm.48, No. 12, 2159, 195G.

BEHAVIOUR OF HEAVY WATER IN PILES OF CEA, Chenouard J., Dirian G., Roth E. 9/P/348 (FRANCE) 1st Geneva Conf. 1955.

PURIFICATION OF'THE HEAVY WATER OF REACTORS ELI AND EL2 BY ION EXCHANGE RESINS. Clienouard J., Roth E. CEA-G73A. Sect. IV-VIII, p. 10-22, 1957. (AEC-tr-4G32)

DISTILLATION OF LIGHT WATER FROM HEAVY WATER MODERA TOR.Bertschc E. C. (Du Pont do Nemours E. I. &Co. Savannah River Lab. Augusta, Ga. USA). DP-325. Dec.1958. 294

7. (On Heavy Water Epuraliou). Natcr K.A. Jener Pubi. No. 17, .1959.

9. RECOVERY OF DgO FROM D.ET.ONIZERS. Bertschc E. C. (Du Pont de Nemours E. I. fcCo. Savannah River Lab., Augusta, Ga. USA). DP-381. Apr. .1959.

1 0. WATER TREATMENT PRO.iBLEMS IN NUCLEAR POWER PLANTS. Ellki G. (Budapest .Technical Univ., 1IUNGARIA). Energia és Atnmtedi. 13, 220-32, Apr, - May 19G0,(ln Hungarian)

3 1. THE USE OF HEAVY WATER IN NUCLEAR REACTORS. Chenouard J. Bull. Inforni. Sei. et Tedi. (Paris) No. 40, 3f>-47, May 19G 0. (In French)

12. RECOVERY OF DEGRADED HEAVY WATER AT THE SAVANNAH RIVER PLANT. Seotten W.C.(Du Pont tic • Nemours E. I. &. Co. Savannah River Lab., Aiken, S. C. USA USA). DP-470. July 19G0. il . I 13. THE HEAVY WATER SYSTEM OF THE PROCESS DEVE­ i'l LOP MEN'I' PILE. Dunldoe A. E. (Du Poni eie Nemours 13.1. & Co.Savannah River Lab. , Aiken, S. C. USA). DP-5G7. June 1.961. ì 14. CHEMICAL AND RADIOCHEMICAL ANALYSIS AND PURI­ FICATION OF THE HEAVY WATER TAKEN FROM THE RA REACTOR. Maksimovie Z. P., Ceranic T., Marinkovic M. Bull. Inst. Nuel.Sei. "Tim-is Kidric:", Belgrade 13, J, 19G2. 295

MWtATU UE PURIFLCATI.ON l'UOGItl'ISS REPORT. I. DESCRIP­ TION OF EQUIPMENT, TESTS J.a, Hi, AND 1L. lir.nmuinnE. W. (I')u I'out di! Ni'inoiii'H K. I, to Co. Savuiiiinli Rivi-r Lnh,, Alki.-n; S.C. USA). DI'-fiYfl. Foli. JfUia.

TREATMENT ANT) ANALYSTS Ol-' 'ITIE WATER ANT) CAS IN •Jlllt-2. (,1'apan At. KIHMVHUH, TUHL, Tokyo, ,TA PAN) J AERI-1024. Apr. 1 Wi'2. (In Jiipani'su)

SEPARATiVE WORK AS A PERFORMANCE CRITERION FOR A HEAVY WATER llECONCEN'rRATION UNIT, Scotton W. C. (Du PoiiL .du .No mourn. E.I. &Co, Savannah Hi vol Lab. /Aiken, S.C. USA). DÌ'-ti.Vi. May 19CÌ2.

CALCULATIONS FOR DISTILLATION OF DEGRADED HEAVY WATER..Svendsas P. (JEN, Madrid, SPATN;Europoan Atomic Energy Society, Par-is, FRANCE). NP-137GG (p. 85-93). Dec. 19G2.

PURIFICA'WON OF REACTOR. MODERATOR . Propoli E.At. Energy Rcv..l,No. 1, 5-42, J 9G3. (In English)

TREATMENT OF WATER'.IN THE EXPERIMENTAL REAC­ TORS OF TI IE C. E. A. Dolle L. ,Conan D. La Chimica dell'Ac­ qua noi Reattori Nucleari, p.' 1 CI- 05. Symp. on Water Chemistry in Reactors, Rome, CNJWN, J SCI«. (Ln French) (CONF-213)

HEAVY WATER CLEANUP BY ELECTROPHORESIS. Boyd.D. C. (Genoral Electric Co., Jlanl'ord Atomic Products Operation, Richland, Wash: USA);HW-77Ö50. Aug. 1, 1 9G3.

••PitOB LE MS OF HEAVY WATER. PURI FTC ATJON BY ION EX- CIIANG'E METHOD. Tin Shw->uiitf, T'uny Ticn-c-lien, Ling- Fon- \i:\ni\ (Chincso Ai-adi-my '>r Srioiu-os, IVI.inj;. Iiisl. or Atomic Kniiff-y, c:111NA). NP-l(;(ii:t. I

23. HEAVY WATER HANDLING .EXPERIENCE IN THE SPERT II REACTOR FACrUTY, Montgomery C. Jl. (Phillips Petroleum Co. Atomic Energy Div., Idaho Falls, Idaho, USA). JDO-J «997. July 1 9fi4.

24. D20 EXPERIENCE AT PU.C.F. Fishbaugor J. R. (General Electric Co. Ilnnford Atomic Product« Operation, Richland, Wash. USA). HW-8M7:». July24, 19(i4.

Proceeding« of Ilio Third International Conference on the Peace­ ful Usus of Atomic Energy, Geneva 1 9G4: 20. THE MANAGEMENT Ol-' HEAVY WATER .1<"OR RESEARCH AND POWER REACTORS. Morrison J. A. (Alomit: Energy of Canada Ltd. Chalk Rivor Nuclear Labs. , Chalk River, Out. ), Thomas M. II., Watson L. C., Woodhoad L. W. 12. P/29 (CANADA); (AECL-2029. 1964)

2G. COMMERCIAL TECHNICAL METHODS FOR RECONCENTRA- TION AND PURIFICATION OF DEGRADED AND CONTAMCNED . HEAVY WATER FOR NUCLEAR REACTORS.Saito T. (Sliowa Denko K. K., Tokyo), Sonoda S., Kurihara Y., Takaniatsu T., Morita T. 12, P/433. (JAPAN).

27. STUDIES ON TTIK RECONCENTRATJON OF DEGRADED HEAVY WATER. 11 a rada A., Kurlhara Y. (Showa Dunko Co., Ltd., JAPAN). Nippon Gcnshiryoku Gakkaishi (i, «28-32, Nov. 19G4. (In Japanese)

28.PURIFICATION OF HEAVY WATER BY ION EXCHANGE RESIN. Akishigc Harada, Yasuo Kurihara (Showa Denko Co., Ltd., JAPAN). Nippon Gcnshiryoku Gakkuishi G. G90-4, Dee. 19G4. (In Japanese)

2a.P(/R[FfCATION OF HEAVY WATER CONTAMINATED WITH : OIL. Paul S. D. , GaiH'san M. el a'l. (Alomic Kriorify Kstahl. , Trombay, INDIA). Indian .1. 'IVHuiul. W, 2IÌ2-M, July 19(15. V)l

A HIGH SENSITIVITY HEAVY WATER LEAK DETECTOR. Bayly J. G. (AECL, Chalk River, Out. CANADA). AKCL-2201. Oct.] 0(55.

DECONTAMINATION OF TI 115 HEAVY WATER SYSTEM OF Till'; HA REACTOIl. MiiUaimovit' Z. H., Nussonov P. M., Nikolié li. M., Miiviiìkuvii: JVI.J)./Elie L. IVI. Bull. Boris Kiclriu Inst. Nuc.1. Sei. IG, 251-63, Oct. 19G5. (In Russian)

PURIFICATION OF HEAVY WATER. 6th Ann. Rep. OECD, Halden Reactor Project 1064/65. .1065. (p. 151-7)

CHEMICAL ELIMINATION OF ALUMINA IN SUSPENSION IN HEAVY WATER OF NUCLEAR REACTORS. Lecloux A. CEA-R-2990. Feb. 1967.

CHEMICAL PROBLEMS POSED BY THE OPERATION OF REACTORS. Symposium on the Chemistry of Reactors, JÜLICH. Oct. 1966. Villard R. (CEA, Paris, FRANCE). Ratlio- chim. Acta, C, 1-6, Sept. 19G7. (In French)

PROCEDURES FOR HEAVY WATER RECONCENTRATION. Milosevic It., Kosaric .N. Nuld. Encrg. 5, No. 3-5, 53-4, 1000-69. (In Serbocroatian) (CONF-G81079)

FURTHER DEVELOPMENT OF SULZER HEAVY WATER COLUMNS. WarlcriwciLl.Gr M. Sul'/.er Tech. Rev. 53, 84-G, 1970

SULZER RECTIFYING PLANTS FOR ENRICHING HEAVY WATER. Zmasek R. (Wintcrthur Engineering Works Div., Switzerland). Sulzer Tech. Rev. 54, No. 3, 199-20.1972.

TRITIUM AND HYDROGEN EXTRACTION PLANTS FOR ATOMIC POWER REACTORS. Damiani M. (Snlzer Brothers Ltd. /Winterthur, Switzerland), Getraitd II., Sonn A.Sulzcr Tech. Rev. 54, No.4, 283-7. 1972. VI - LIST OF MAIN CONFERENCES ON HEAVY WATER

AND HEAVY WATER REACTORS 301

VI - LIST OF MAIN CONFERENCES ON HEAVY WATER AND IIBAVY .WATER UJSACTOHS

Simposium on Heavy Water Production oi-ganizcd by European Society of Atomic Energy. Rome Marcii 31-April 2, 1955.

International Conference on the Peaceful Uses of Atomic Energy (United Nations). Geneva, Aug. »-2 0, J 955. (1st Geneva Coni'. 1955). A/CONF 8/l'/3,4, 5,G,7, 34», 357,361,387,410,495,605,023,631, 744, 790, 791, »19, H23,'839, Mil, 879, 8HG, 920, 923,927, 934, 958, 988, 1010, 1120.

Third ElecLronic-Nucleal International Review. Scientific Congress- Nuclear Session: Colloquium on Heavy Water. Home, Italy, July 6,1956.

International Symposium on Isotope Separation. Amsterdam, Nether­ lands. Apr. 23-27, 1957.

Second United Nations International Conference on the Peaceful Uses of Atomic Energy. Geneva, Sept. .1-13, 1958. (2nd Geneva Conf. 1958). A/CONF 15/P/135,.136, 151, 160, 180, 181, 188,208, 209, 210, 212, 231,24 5,246,255,259,334, 335, 336, 340,423,424,491,559,572,575, 500, UÓ0, 610, 723, 745, 703, 1000, 1063, 1065, .1150, 1154,'1.1 97, 1261, 1336, 1362, 1383, 1400, 1475,' 1476, 1524, lull, 1628, 1630, 1649, 1669, 1929, 1949, 2036, 2053,2094, 2105, 2250, 2323, 2336, 2424, 2471, 2495, 2538. 302

USAEC. Symposium on Heavy Water Moderated Reactors. German- town, My. USA. March 3-4, 1959. (TID-7575)

American Institution of Chemical Engineers (A. I. Ch, E. ) Meeting. San Francisco,-Calif. USA. Dec. 1959

EAES Enlarged Symposium on Heavy Water Power Reactors. Majorca, Spain. Oct. I960. (CONF-410)

[AEA Symposium on Programming and Utilization of Research Renclm-s. Vienna, Oct. 1G-21, 1961.

The Canadian Nuclear Association Conference on Heavy Water Reactors. Ottawa, Canada. May 1962.

Gth World Power Conference. Melbourne, Australia. Oct. 20--'27, 1962.

Colloquium on Heavy Water, (Junta de Energia Nuclear Madrid and European Atomic Energy Society, Paris) Madrid, Spain. Dec. 13-14,1962.

IAEA Panel on Heavy Water Lattices.Vienna, Feb. 1963. (CONF-116)

The C'SVS Third Conference on Nuclear Energetics. Prague 1964.

Third International Conference'on the Peaceful Uses of Atomic Energy. Geneva, Aug. 3.1-Sept. 9, 19G4. (3rd Geneva Conf. 1964) A/CONF 2Ö/P/2,' G, 7, 8, 9, 10, 11, 12, 29, 39, 40, 51, 69, 70, 76, 78, 90, 91, 116,129, 174, 17G, 209, 268,^290, 417, 433, 496, 522, 523, 525, 532, 557, 594, 595, 602, 603, G05, 608, 625, 630, 669, 673, 682, 683, 691, 692, 697, 709, 711, 743, 744, 753, 754, 76-3, 777,778, 779, 808, 809, 810, 833, 859,8G0,877. 303

Canadian Nuclear Association Annual Conference on Organic and Heavy Water Reactors. Winnipeg, Canada. May 30-Juno 1/196G. (CONF 6R051G-5)"

IAEA Symposium on Heavy Water Power Reactors. Vienna, Sept. 11- 15, 106 7. (SM-99)

British Nuclear Society Conference on Steam Generating Heavy Water Reactors. London, UK. May 14-16, 1968.

IAEA Symposium on Economics of Nuclear Fuel. Gottwaldov, CSSR. May 27-31, 1968. (SM-Ì.05/8, 31, 32)

IAEA Panel on Utilization of Thorium in Power Reactors. Vienna, June 4-8, 19G8.

7th World Power Conference. Moscow, USSR. Aug. 20-25, 1968.

Reactor day 1969 of the German Atomforum. Frankfurt, F. R. G. Apr. 16.19G9:

Canadian Nuclear Association Annual Conference on the Status of Canadian Construction Projects. June 19G9.

Nuclex 69. International Nuclear Industries Fair and Technical Meetings. Basel, Switzerland. Oct. 6-11, 1969.

CNEN Symposium on the Technical and Economic Aspects of the Heavy Water Production. Turin, Italy. Sc-pt. 30-Oct, I, 1970. 304 k Ite là I! • I 26. Fourt.li Intornntiotml Conference on the Peaceful Uses oj" AlomLc % Eucsvyy. (Teneva, Sept. (>-J(>, 1071. (4th Gonevu Coni'. 15)04) 8 A/CIONF. 4Ü/I,/:I4G,0()7. , | 4

li

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3 i I N DE X E S

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13

I I

I I 307

Subject Index

I.. General II. Bibliographies III. Determination and Analyses of Deuterium and Heavy Water IV. Heavy Water Production A - Reviews of reparation processes B - Patent .Review - Patents selected from the files of Brevatomc, Paris.- Addendum 1- Heavy Water Production by Chemical Exchange II2S-HDO 2- Heavy Water Production by Chemical Exchange NII3-IID 3- Heavy Water Production by Chemical.Exchange H2O-HD 4- Heavy Water Production by Chemical Exchange: Equipment and Other Processes 5- Heavy Water Production by Hydrogen Distillation G- Heavy Water Production by Water Distillation 7- Heavy Water Production by Ammonia Distillation 8- Heavy Water Production by Methane Distillation 9- Heavy Water Production by Distillation of Other Compounds 10- Heavy Water Production by Electrolysis 11- Heavy Water Production by Other Processes C - Actual Industrial Processes 1 - Chemical Exchange 1 - Bithcrmal Exchange between Hydrogen Sulphide and Water (HoS-IIDO) 2 - Chemical Exchange bci.wecn Ammonia and Hydrogen (NII3-HD) 3 - Hydrogen - Water Exchange (H20-HD) 2 - Distillation 1 - Distillation of Hydrogen 2 - Distillation of Water 3 - Electrolysis of Water D - Production Plants 1 - Table (Summary) 2- Plants based on H2S-HDO Process 3 - Plants based on NII3-HD Process 4 - Plants based on II2O-HD 'Process 5 - Distillation Plants . G - Plants based on Electrolysis of Water 308

IC - Technical and economical aspects F - Potential Production Processes 1 - Chemical Exchange Processes 1 - Between Hydrogen and Deuterium 2 - Between Hydrocarbons and Water 1 - Aromatic:« - II2O

2 - Unsafcurated Aliphatic» - 1I20 3 - .Saturatoci Aliplm.ti.es - II2O 4 - Heterocyclic: Hydrocarbons - H2O f) - Alicyclie Hydrocarbons - IT2O 3 - Between Hydrocarbons and Hydrogen 1 - Aroma tics - Hydrogen 2 - Unsaturated AliphaU.cs - Hydrogen 3 - Saturated Alipliatj.es - Hydrogen 4 - Between Aminos, Aminoacids and Water 1 - Aminos - H2O 2 - Aminoaeicls - H20 !5 - Between Amines, A111i.noaci.ds and Hydrogen 1. - Amines - Hydrogen 2 - Amides - Hydrogen 6 - 'Between Organic Acids and Water or Hydrogen 1 - Organic Acids - H2O 2 - Organic Acids - Hydrogen , 7 - 'Between Hydrides, Hydrates and Water .1. - Hydrides, Hydrates - HoO 2 - Phosphine - II2O 3 - Arsine - II2O ft - Between Hydrogen Halides and Different Substances 1 - Hydrogen Haliden - II2O 2 - Hydrogen Halides - Hydrogen 3 - Hydrogen Tlalidcs - Hydrocarbons 4 - Hydrogen HaJides - Organic Acids 0 - Between Jon Exchange Uesins and Water 10 - Between Mercaptans and Water ] I - Between Kolons and Water 2 - Physical Separation Processes 1 - Ahsorlive 1'Vaclioiial.ion 2 - Adsorption 3 - Ceni ri fugai 4 - Instillation of Ammonia and Methane 5 - Instillation of Other Compounds (i - Diffusion 309

7 - Thermal Diffusion 3 - Solvent Extraction 0 - Others 3 - Other Polcntial Processes Heavy Water Reactors A - Table (Summary) B - Heavy Water Tfaactors in nuclear power programs C- Treatment of Degraded Heavy Water Main Conferences on Heavy Water and Heavy Water Reactors 310

1 ?, IV. F. 2. 243 II 33 IV. F. 3. 244 III 43 IV. F. 3. 246 IV. A 75 IV. F. 3. 248 IV. 13 97 IV. F. 4. 249 IV. B. 1 sra IV. F. 4. 250 IV. B. 2 103 IV. F. 5. 251 IV. B. 3 110 IV. F. 5. 252 IV . 1.3. 4 115 IV. F. 5. 253 IV. B. 5 117 IV. F. G. 254 IV. E. 6 120 IV. F. 7. 255 TV. B. 7 123 IV. F. 7. 256 IV. B. 8 124 IV. F. 7. 258 I.V. 13. 0 124 IV. F. 8. .1 259 IV. 13. IC) 125 IV. F. 8. 2 20 0 IV. 13. 1.1 1.2 H IV. F.1.8 . 3 261 Addendi m to 1?R 134 1V.F. 1.8.4 262 IV. C. .1. 1 137 IV. F.1 . 9 26 3 IV. C. 1. 2 145 IV. F.1 . 10 264 IV. C. 1. 3 155 TV.F. 1. 1 1 205 IV. C. 2_ I 105 IV. F.2 . 1 266 IV. C. 2, 2 173 IV. F.2. 2 267 IV. C. 3 185 I.V. F.2 . 3 270 IV. D. 1 105-6 IV. F. 2.4 271 IV. D. 1. 1 197-fì IV. F. 2.5 272 IV. 1"). 2 ton IV. F. 2.G 273 iv. n. 3 203 IV. 2.7 274 IV. "1"). 4 207 IV. 2.0 275 IV. D. 5 211 IV. F, 2. 9 276 IV. D. 6 221 IV. F, 3 277 IV. E 227 V.A 281 IV. F. 1. 1 234 V. 13 283 IV. F. 1. 2..1 237 V.C 293 IV. F. 1. 2. 2 239 VI 301 IV. F. 1. 2.3 241 IV. F. 1. 2.4 242 311

Authors Index A -

Abolson P. II. IV (P. 1.2.3-3) Abernathoy lt. M. III (147) Abraham B. M. IV (C. 2.1.-18) Aclamson A. W. IV (P. 1.9-1) Addington N. G. IV (C. 2.1.-25) Adorni N. III (75, 80, 86, 88);IV (D. 5-56) Aerov M. E. IV (C. 2.1-37) Agostini ,1. P. IV (CI. 1.-54) . Aharoni II. IV (P.. 11-28) Ahlbcrg «I.E. IV (Ar23) Aie re J. IV (C. 1.1-49) Ailcin A.M. V (B-43) Akar P. IV (A-125; C. 2. 1-33) Akhundov T.S. 111(145,158) Akishin P.A. I (146) Aleksandrovich Y. A. IV (C. 3-12,40,53; D.6-8) AlKii-Slatot' R. 13. III (37) Alfreds on P. G. IV (173)

Alkire G.J. ITI (49) Allen R. E. II (25) Alvrtroz-Oonaal.fi.s J. R. IV (A-135; CI. 1-20; C.2.2.-76)

Aly A. [. M. IV (C. 3-88,89)

Aiunnridi II. IV (CI. 1-19) Ambrosi ni G.C. V (13-51) Ainiek M.G. IV (D.5-(!) .11.

Amici S. 111(14 0) Anderson C.E. 111(170) Anderson L.C. IV (D. G-2) Andreassen K. IV (C. 3-65) Angelino G. C. IV (C. 2. 2-77; D. 5-5G, G4, G7) Antipova N. P. Ili (94,97) Antoncliik Yu.I. IH (114) Armstrong F.S. II (40) Armstrong G. T. I (135); II (19) Arnold H. Ti. IV (C. 1. 2-1, 5, G; C. 1. 3-4) Arn.stein TI. II. I (.11 fi) Artaud J. 111(133) Asada T. IV (C. 3-48) Askins II. W. Ill (20G) Aston F.W. I (49) AugoodD.R. I (13G); IV (A-G2, 84; C.2.1-22; F.2.1-2) AyrosJ.A. I (234); IV (A-1G4) •313

- B

Babcock D.F. IV (C. 1.1-9); V (B-G) Babkov S. I, IV (C. 1.1-15) Baortschi P. I (223); III (112,201); IV (A-44; C. 2. 2-56, 63) Bailey B. M. IV (C. 2.1-29) Hakin V. O. II (55) Balaban A. T. IV (F.1.2.4-1,3) Balacoanu T.'C, IV (C.1.3-15) Baldctli S. V (B-51) Bald us W. IV (C.2.1-3G;D.5-42) Bully I. IV (F. 1.2.4-1) Bamann E. I (36) Bancroft A. R. IV (C.2.2-55; E-51; F. 1.5. 1-3); V (B-41, 59) Banick C.J. V (C-.l) Banikiofco« G. C IV (C.2.1-45) Marabaschi. S. V ( I1-72) HiU'aiiW.,1. IV (C. 1.3-26) Barb D. IV (C. 1.2-59; C.1.3-29,37; C.2.2-G7) Barbieri W. III (130,132) Bardwoll .1. IV (C.1.3-14) : j Bar-Eli K.- nr(B. 2-21); C. 1.2-41; F. 1.5.1-1) Barlow E. À. IV (D. 4-2) ßarnocchi L. IV (li. 11-3) Barr F. T. 1 (114); IV (A-52; C. 1.2-29; E-19) Bar I hole my R. [V (C. 1.3-43) Basmailjan 1). IV (P. 2.2-13) Bales J. R. lV(D.(i-2) Bate« R. G. I (228); III (202) Bauche P. IV (C.'l.2-G0) 314

Bauer L. IV (F. 1. 2. 4-2) Bauer S.U. IV (C. 1. 1-48; F. .1. 2. 2-7) Baumann E. W. III (190); V (C-15) Baumgartner R. 1(149). BayerlV. IV (B.3-28; B.6-4) Bayly J. G. III (104, 118, 138, 149, 1G3, 170); V (C-30) Beach J. E. IV (D. 2-18) 13 ebbing ton W. I\ IV (A-90; C. 1. 1-17; C. 2. 2-G2; D. 2-3, 11; E-32; F. 2. 8-1); V (B-17) Becker E. W.A. I (122,212); IV (A-54, 123; B.3-12, 13,16, 22; C. 1. 2-G6; C. 1. 3-17, 20, 31; C. 2. 2-48; D.4-13) Becker W. E. .IV (F. 1. 4. 1-3) Beckett C.W. 11(12,13,14,15,16,18,28) Beckmann R. IV (A-71) Bedhome A. IV (D.3-7) Beeck O. IV (F.1. 3. 2-2) Begun G. M. .11(25,37) Behnke II. IV (C. .1. 1-lß, 27) ; Bell CT,. IV, (F. .1.2.4-2) Bell IL I'. IV (0.3-16,22,41) Bcllmann R. IV (D. 5-34) Benedict M. I (133,150); IV (A-28, 38, 47, G5, G9; • C. 1. 1-6; C. 1.3-44, 51; C. 2. 1-17; C. 2. 2-33, 34, 73; F. 2. 4-4, 5) Bonthly R. I (118) .•' Berg L. IV (C. 2. 2-27, 30) Borglurid-Lars son U. HI (73) Bernstein R. H. IV (A-flJ; F. 1. 2. 3-1; F. 1. 7. 1-3) Berry C.E. 111(52) Borion A. 111(00) - 315

Bertsche E. C. V(C-6,9) Bethune A.J.de ' IV (A-23) BeversK. IV (C. 2. 2-75) BhargawaR.K. . IV (D.'2-27) Bibler N. E. ' IV (C. 1.3-49) Bier K. I (212); IV (A-55, 91; C. 1. 3-20; C. 2. 2-48; P. 2. 9-4) Bier W. I (212) Bigeleisen J. I (128, 131,455); III (48, 50); IV (A-29, 36, 37, 80, 161; C. 1. 2-13, 15,16,18, 19, 20, 27; F.1.7. 2-1, 2, 3, 4; F.2.4-2) Biggers R.E.. Ill (109) Bildeau A.'L. V (C-3)

Bildstein H.' HI (162) ;

Bir R. ' «;> I (202) : : Birbaum N. '' ''' *"-^ts;sJV (A-8)'' . •• ' Bishop A.S. I (149) Blair J.A. IV (D..5-23) Blair T.S. IV (A-23) • • Blaga li. ta (172) Blaga Lu HI (172) Blanc D. IV (A-87) ' BleakneyW. I (13); III (1); IV (C. 3-34; F. 2. 2-1) BlennemanD. IV (C.l. 2-40,42; F. 1. 2. 3-2, F. 1.10-2) Bluer R.W. IV(F.l.l-2) BlumJ.M. 1 (208) Blumkin S. IV (E-2) Boato G. IV (F. 1.1-5) ' Bochme J., I (39) Bode C. " IV (D.4-13) 316

Boettchor A. V (B-53) Bogatyrev K,S. IV (F. 1.9-2) Böhme D.W. IV (C 2.'2-84) Boian M. IV (D.'4-14,15,18; E-41) .Bok L.D.C. IV (F.'i;8.4-1) Bolhar-Nordcnlcampf F.' IV (A-112) Bologa M. IV (C. 1.3-48) BondG.C. IV (F.'2.'2-3) Botulai-en.Wl.1. ,111(151) Bonhoelfcr K. F. I (4); IV (C. 1. 3-1); C. 3-15) Bonner R. IV (C. 1.2-8, 10) Boorman C. IV (F. 2. 7-2) Booth R.J. 111(149) Boreskov G. K.' IV (C. 1. 3-46; F. 1.1.-7) Bornlcessel K. IV (F. 2. 9-2) BoroccoA.L. I (67) Bosselaai-C.A. 111(107,134,155) Botlmer-by A, A. IV (F. 1.11-1) Botter F. I (193); II (40;'IV (C. 1. 2-45; C. 2. 2-72;;, F.2.2-14) .. ; Bottinga Y. IV (C. 1.3-58) Bottini A. T. IV (F.l.6.1-1) Boui-gcois Y. IV (C. 1. 2-49) BourJce P.J. IV (C. 1. 2-37, 47) Boutaric A. I (20) BoydD.C, V (C-21) BoydG.E. IV (F. 1.9-1) Bracciforti L. IV (D. 3-13) 317

Brady O. L. I (61) BrankcrA.V. ' IV (A-120) Brandt W. IV (F. 1.4. 2-4) . Bratzlcr II. IV (C. 3-39) Brayson J. A. ITI (26) Brickwcddo F.G. I 2,110); IV (C. 2.1-2, 4) Bridg forth Jr. 11. !M. IV (C. 2. 2»2.r>) Brigoli B. I (162); ". (65," 86, 89, 99, 101); IV (C. 1. 3-10, 12; C. 2. 2-17; D. 2-10; D. 5-53, 54, 56, 64, 67, 73) Britt R.D.Jr. Ill (183) Broclskii A. I. I (70); IV (A-11; C. 1. 2-12; C. 3-12, 33, 40) Brogliato A. V (B-70) Brown C.J. IV (A-64) Brown F. B.. IV (A-21, 22) Brown G.G. '" ,,, IV (C.2.2-37) Brown G. W. " IV (C. 3-15; D. 6-6)

Brown L. M. 11(12,13,14,15,16,17,20,21,23,24,27,28,30) Brown R. M. V (B-41) Brown W, G. IV (F. 2.5-1) BrunJ. HI (18); IV (A-39; C. 3-32, 63,65,68,69, 72; E-3) Bryant F.J..- 111(7.7) BryantW.M.D. IV (C.2.2-18) • Buadze.L.G. IV (C. 1.3-33) Bucurll. V. IV (C. 1.3-27; C. 2. 2-67; C.3-8G) Budris R.S. ' IV (F. 1.4.2-4) Euclci G. V (C-10) Buono O. G. I (6 0) 318

Buess R. IV (F.2.7-1) Buford.Tv.C.B. IV (C. 1.1-9) BUki G. V (C-10) Bunccl E. IV (F. 1.3.1-G) Burcat A. IV (C. 1.1-48) Burch G. E. III (108) Burgess M. P. IV (C. 1.1-42) Burwcll R. L. IV (F. 1.3.2-4) Butler J. A. V. IV (A-5) Butterworth A. V. V (B-13) 319

Gabella A. IV (D. 3-13) Cabioar J, 111(185) Caglc F.W. M. IV (C. 3-01) Campbell D. N. III (63).- Cannavate L. Ili (124) Caprioli io P. V (n-68) Cat'dosi G. V (B-49) •>•' Carori G. TV (F. 1.1-5) l Carlson C.S. IV (C. 2. 2-40) Carlson U.C. IV (D.4-3)' Carlson I?.. C. IV (D/5-10V Carnnchaol L.. T. IV (C. l.;l-rl); Carpenter G. K. IV (C. 2: 1-13); Carpenter R. B. III (59) .•••••<•.

Casa A. F. V (B-54) Casagranctc I. ' V (13-70) Casini R. IV (D. 5-36; E-G) Castelli G.' V (B-72)

Cavers S. D. TV (D.G-11) CoccalcÜ M. III (54,95,122,141, 3 59,106); IV (C. 2. 2-78) C cranio T. V (Cr 14) • Cerrai E. I (129); III (3G, 43, 47, 85); IV (A-40, 73; C. 1. 3-7, 8, 10, 12; D. 5-30,.52; D. G-21, 22, 23) Champctier G. I (57, 58); IV (D. 6-5) Chan J. III (205) Chang C. L. III (92,128,154,157) :>?.()

Chang T. L. 1 (G3) C hap in J. II. IV (C. 1.2-2) Chapman M.J. II (42) CharloRwoi-th D.H. V (R-50) Char p enti c:r M. V (B-57) Cliatcl S. m (144) Chnucli-i 11. M. IV (D.G-2G) Chen W. i (.185) Cheng C. II. in (92). Chonouartl J. in (41); V(C-4,5, 11)

Chiusa A. in (130). Chifu A. in (172,173) Chin T.C. in (154,157 Chiplonkar T. IV (C. 3-44)' Chittock C. I (34) Chopey N. P. IV (D.5-55) Choppin J. II. IV (A-20) Chroncs J. IV (F. 1.3.3-1) C ig noli F. I (35). Cimino A. IV (F. 1.1-5) Cimler E. IV (C.2.1-45) Ciobotaru T. IV (C. 1.3-30) Ciric M. IV (A-147) Citarcla A. I (G4) Clacys Y. M.. IV (F. 1.5. 2-1) Clark F.W. IV (C.2.2-1G) Clark-ll. 11 (29)' 321

Clay ,1. 1 (45) Clcwutt CS. II. I. (.133,132) Clusius K. 1 (110,121); IV (A-124; C, 2. 1-15) Conte« ,f. IV (I). ß-D7) Cue I a* an (• T). R. V (H-32) Culi un IC. I (112, BH, 07, 111, 120): IV (A-34; I). 5-4) Culbm-n A. P. IV (C. 2. 2-2!], 36) Collie C. TL J. (JO)-. Combs R. U ,1'V (C. 2,2-51) Conan I.). V (C-20) Condon F.K III (HO) Conneman J. IV (15. 1-10, 20) Conway P.. E. I (104); IV (C.3-71) Cook G. 13. I .(225) Cook M. W. IV(F.2.1-1) Copper A. II. I (197) Cornish R. E. IV (C.2.2-1 Cottili M. III (103) Coulon A. IV (C.2.1-44,46) Couvvölsior P. IV (C. 1.2-54,65) Cravarnlo L,. V (B-73) Crutulla .11. F. IV (C. 1.3-26; B-29) Crist R. H. III (3, 5)...-';. Cross R.J. IV (B. 11-14)

Curran A. T. II (33) : Cziko K. III (89, 91); IV (A-61; C. 3-70) ,'-.'':';'-- 5- * r H

- D - 11 ! ; ! ? Uatftjol A. ]•'. IV (a 0-fi) Damiani M. V(C-31) [j Dnnhyn.J. ^ (F. 1. 1.-3) Danilov I.B. IV (C 2.1-32, 40) [^ DarmoisF. I (43); IV (A-7) j] DattaR.L.' 1(1 83); III (76, 113); IV (A-10G;C. 3-76, 84;E-3G) H

David L. HI (200) Davidson A..T. IV (F. 1. 1. 1-1)

Daylon ,1. C. IV (C. 1.2-20; I'M. 5. 2-1) Do Bvouekci-c L. IV (F. 2. 7-1)

Dulioncy 11. W. IV (F-2) Delmas R. .IV (C. 1. 2-54, G4, Kf,)

Do Long W. B. iV > Do Michclis B. I (176) Denton W.U. IV (C. 2. 1-26, 27)

Deschamps IV IV (F. 1. 4. 1-1) •• Deshpamlo l\G. IV (D. 2-27; D. 6-28; E-33)

DcvcrcllC. 111(109) Devos J.J. V (B-55) Dharmatti S. S. 111(106) Dickol G. I (220) Dicks U.S. LV(C.2.2-40) Di ebne rK. IV (B. 10-14) Dietrich 11. IV (C. 1.1-16) Diolzo M. TV (A-Ü2; D.5-47) Dijk H. van IV (C. 2. 1-3) Diinicluk P. W. II (50) Dinolll D. IV (D. 4-5; D. 6-24) Dirian G. I (193); II (47); IV (A-86; 110; C. 1. 2-44, 45; C.1.3-15; F. 2. 2-14); V (B-20; C-4)

Doede C. iv (D. 6-1) Dogramadzi N. iv (C. 2. 2-57) DolinP.I. IV (C. 3-56, 57) Dolle L. v (B-26; C-20) Domangc L. I; (18) Dominik W. j (28) Douglas J. E. IV (D. 6-18) Doutsov P. Yu. Ill (93) DorabiaLska A. IV (C. 2. 2-70) Dostrovsky I. IV (C. 2. 2-43, 47; D. 5-12, 13, 19, 26, 27) Doug Z.H. IV (C.3-66) Dx-apex*. J.-W. IV (C. 2. 2-61) . Drews W. P. II (22);;IV (A-51, 52; E-19; F. 2.4-3)

Drickanicr H. G. IV (C. 2. 2-37) ; ; DmryJ.S. II (45); IV (A-108, 121; C. 1.1-29; D. 6-32) Duke D. M. H (43) Duncan J. F. I (225) Dunkln II.. HI (156) Dmikluo A. la. V (C-13) Dunlap G. W. I (102) DunnC.L. IV (C. 2. 2-38) Duranti-Valcntini P. • IV (D. 3-13) Dykhnq N. M. I (148) Dyne P. IV (C.1.3-14) Bf P 324 II I Is

JI: - I I !(% Ebenliack D. G. Ill (170) Si Eborhart ,T. G. IV (F.2. 2-8) Hchavarri 'V. IV (C.2.2-7Ì3) Kchiyoy.'i K. tv (I'M. f>. .1-2) Edmonds ß. M. IV (A-8) i Edwards A. J, IV (C. 3-41) p Ehrcnbt!!'^ \V. IV (C. 2.2-50) Ehi-kG L. F. IV (C. 3-49; D. 6-7) II Eichna J. R. IV (C. 2. 1-13) EklinolT M. L. IV (C. 2. 1-16; D.2-1) Eiyon M. I (134) Eineckc E. I (09) Einhorn F. III (185) ' m Elich L. M. V (C-31) El.lingliam II. J. T. TV (C.3-42) Elliot N. IV (C. 1.2-15, IG, 27) ili Ellwood P. IV (E-45) Emmet P.H. IV (C/l.2-21) Enomoto S. IV (C. 1.2-24;C. 1.3-28) Enyo Ivr. IV (C. 1.3-53, 5G) Eriksson B. J. IV (C. 1.1-23, 24, 25, 33; .13-22) Erlcnmaycr II. IV (C. 3-13; D.G-4) Er.slücr B. V. IV (C. 3-56,57) Euckon A. IV (C.3-3Ö) I Evstigiiccv V. B. JII (55) li

$ 325 I'if, :I? 3 ;£ «a Ewc.ll R. TI IV (C. 2. 2-27, 31) -, i Eyrlng 11. va 1(8,14; 84); 17(0.3-4,8,11,17,23,01) I 1TO I m Li I

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Falk CD. IV (F. 1.7.1-4; F. 1.7. 2-5) Parkas A. I (11, 30, 56); III (14); IV (A-12; C. 3-28, 50) Parkas L. I (H* 2G> 30): IV (C. 3-28) PatuC. IV (D. 4-14; E-41) Faucher J.A. IV (F. 1. 7. 1-2) Favre I. IV (A-113) Fellner-Felldeg H. IV (A-60) Fellows CG. m (ß3) Fenske M. R. IV (C 2. 2-15) Fermi E. I (92) Fetchcr Jr.F.S. 111(22) Feugcr-Erikson K. 111(13) Feuerstein II. III (104) FickJ.L. IV (F. 2. 1-1) Ficklen J.B. IV (C. 3-3) Figlictti C. HI (129) - Filippov G.G. IV (A-137) Filippova N. S. 111(10,11,16) Finke J. IV (A-43) / Finzi S. IV (C 1.3-16, 20; D. 4-8; D. 6-27, 30) FishbaugcjrJ.il. V (C-24) FishcrB.D. IV (F. 1. 3. 1-5) Fisher R. IV (F. 2.5-2) ' FishevR.B. 111(24,27,28,29) FizzoltL C. III (44) Fletcher G.W. V (B-24) 327

Flotov H. E. IV (C. 2.1-18) Flu egge S. I (81,86) Flynn T..M. IV (C. 2.1-24, 28, 39, 42; C. 2. 2 -61; D. 5-37, 46) Fochler S. III (152) Fodor P. III (89, 91); IV. (A-61; C. 3-70) Fodor T. IV (D. 4-14, 17; D. 6-40; F. 2. 7- 4) Fok N.V. IV (F. 1.3. 2-7) Folli E. IV (D. 3-15) Fookson A IV (C. 2.2-42; D.5-16) Forstat H. I (93) Fort A. III (90) Fowler R. H. IV (C. 3-27) Fradkov A. B. IV (C. 2. 1-32,40; D. 5-20) Francis A. W. IV (C. 2.2-28) Frandsen M. IV (C. 2. 2-3; C. 3-5) Frank B. H. IV (F. 1.4.2-5) Fred M. •, III (25)

Frerichs R. I (25) "•• Friedel R.A. 111(30) Friedman A. S. II (18, 20, 21, 23, 24, 27, 28, 30) Friedman L. IV (C. 1.2-16) Fromherz H. HI (15) ' Frost A. A. IV (C. 3-8) ' Frost F. E. II (32) Fujimoto A. IV (C.l. 3-21) Fukasalai S. IV (C.l. 2-56) Fukuda M. I (168, 179) 328

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Gada F. II (44) GaddyR.H. 111(178) Gacrtner II. IV (C. 3-13; D. 6-4) Gaincs A. L. IV (E-4) GalweyA.K. IV (C. 1. 1-36) GamiD.C. IV (C. 2. 1-31; D. 5-66; D. G-28; E-33) Ganesan M. V (C-29) Garaud J. IV (C. 1.1-19) Garby L. HI (67) GardE. IV (F. 1.2. 4-1, 3) Garland C.W. HI (53) Garnett J. L. IV (F. 1.2.1-5; F. 1. 3.1-1, 2, 5, 7) Garret G.A. IV (A-79) Garvin R. G. IV (C.1.1-42, 46, 47) Gaunt J. 111(57,64,66,70,74) Gauthron M. I (226) Gazith M. I (181); II (46) Geldes R. L. IV (C. 2.1-34) Gel'perin 1.1. IV (C.1.2-51,55) George K.D. III (207) Gcrhold G. IV (F. 1. 7.3-1) Germagnoli E. I (139)

Gertraud R. V (C:38) GidLnofXM. L, . IV (A-35) Güfillan E..S. Jr. Ill (4) Gillespie B. IV (F. 1. 2. 2-1) .Gillies'D. IV (F. 1.10-1) 329

GillisJ. IV (C. 2. 2-43,47; D. 5-19) Giona A.R. ' IV (A-102) GisperùBennach M. G. Ill (111, 142, 150,171,177, 192); IV (A-135; C. 2. 2-79, 80, 81; C. 3-67, 73; D. 5-70; D. 6-37,38, 39; E-17)

Givenc E. Il (11) Gladkova E. N. 111(94) .Glasstone S. I (f>4) GlueckaufE. IV (F. 2. 2-4, 6,10) Gochaliev Z. E. IV (A-59)' Gold V. IV (C. 3-82; F. 1.2. 1-2) Goldblatt M. Ill (164) Golden S. IV (C. 1.1-6) Goldfinger P. Ill (8); IV (C 3-18) Goldfrank J. C. " IV (A-152, 153; C. 1. 1-51; F. 1. 2. 2-8) Goldman M. Ill (87) Goldstein J. M. II (15, 16) GoodallC.A. •.,.,.. HI (49) Goodman C. I (100) '•'•.. Googin J! M. IV (C. 2. 2-51, 60) Gordon B. E. IV (F. 1. 2. 1-6) Gordon G. Ill (168) Gossen W. Ill (51) !, Goujon P. .Ill (141, 166) Gould A. J. I (13); IV (F. 2. 2-1)

Grabowski E.J. IV (C. 1.1-3) Graff J. I (93) Graffo. ' IV (C. 2.1-17) 330

Gragerov I. P. Ill (79) Grandcollot P. IV (C. 1. 2-44, 45) Graner J. IV (B. 6-7, 8, 16) Gray J. L. V (B-13,36) Graziarli G. V (B-45,55) Grecu E. IV (A-99; 148,149; C. 1. 3-3G; E-31) Green C.H. I (50) Gregory II. S. IV (C. 3-42) GreiffL. Y. 1(46) GreskyA.T. I (233); IV (A-166) Grooth S.R. de I (97) Gross P. IV (C.3-35) Grosse A. V. IV (C. 3-54). Groth W. I (120); IV (A-34,130) Grove G. R. II (36) Grauber G. H. 111(119) Gruemm H. V (B-28,33, 35) Grünspan S. I (193) Gryson H. I (211) Guenebaut H. IV (F. 1.4. 1-1) Guenterschulzo A. IV (C. 3-29) GueronJ. Ill (32, 41); IV (A-49) Guggenlieim E. A. I (115) ' Guinot H. IV (C. 2. 2-16) Guizoarn L. II (54) . Gunderscn W. IV (C.3-68,69,72) Gupta D. IV (C.2.1-31); V (B-28, 35) 331

Gutman J. R. IV (C. 1.2-28) Gutovsky E. T. K. IV (C. 2.1-51) Guymon R,H. IV.(D;6-32) Gverdisiteli I. G. IV(A-145)

m 1 m M 332

- II -

Haantjes J. I (27); IV (C.-2.1-3) Habedank M. IV (C. 2.2-69) Haeffele W. V (B-28, 35) HaennyJ. IV (D. 5-49, 50, 51) Hagiwara H. IV (F. 1. 5.1-2) Hahn H.H. IV (B. 11-33) HahnH. T. IV (F. 2. 8-2) Haissinsky M. 1(117) HaldemanR. G. 111(56) HalfordJ.O. IV (D. 6-2) Hall L. G. Ill (52); IV (C. 2. 1-20) HallN.F. IV (C. 2. 2-4) HallW.H. IV(D.6-9) Hallaba E. IV (C. 3-88, 89) Halle E.van IV (A-50) Haller P. de IV (A-4 8) Halpern J. IV (C. 1.3-52; F. 1.7.1-4; F. 1.7. 2-5) HalpernO. IV (C.3-35) Handley D. IV (D. 2-8) Hankiewicz E. IV (F. 1. 3.1-4) Hannerz K. IV (A-98; C. 1.3-11) Hanson D. N. IV (F. 2.1-1) Hansgirg F. IV (B. 3-1,2) I-Iarada A. .,.' IV (C. 3-77, 78; D. 6-34); V (C.-27, 28) Harada M. Ill (9); IV (C. 2. 2-7) Harkins W. D. I (19); IV (D. 6-1) 333

Harmsen H. IV (P. 2. 6-4) Harris L. IV (P. 2.6-1) Harrison J. M. IV (C. 2. 2-27, 30) Hart R. G. 111(33) Harteck P. Ill (19); IV (C.3-26; £-7) Hartmann J. U. I (40) Harty'H. V (B-46) HartyW. M. IV (D. 6-13) I-Iatada M. IV (P. 1. 2. 1-3) Haubach W.J. IV (P. 2. 2-1, 15) Haucke G. Ill (156) HaulR.A.'W." IV (C. 1.1-16,27; C. 1. 2-36, 40, 42; F. 1.2. 3-2; P. 1.1.0-2) Havliqek F. IV (D. 5-39) HaywarclW.H. Ill (123) Haywood L. R. V(B-3G,43) Hellmuth'D. IV (A-105) HelmickL.S. IV (F. 1.2. 5-1) Henslejv J.D.C.' IV (D. 2-8) Hering H. . 111(115) Herrick-C.B. IV (C. 1.1-2) Hertz G.L. •;.'. • '• IV (F. 2. 6-2,4) HestonW.M. V (C-l) .

Heuberger M. t • II (40) Heyningen W.E.von' 111(20) Heyrovsky J. IV (C.3-47) HilbornH.S. ' "• IV,(D. 2-15, 16, 17, 19,20, 21) 334

Hllsch R. IV (P..2. 3-4). Hippie J.A.Jr. IV (C.3-34)

HironakaY. IV (P. 1. 2. 2r3, 4) Hlrota K. I (102); IV (F. 1. 2. 1-3, 4, 7; P. 1.2. 2-3,4) His ano T. I (162) Hiskcy C. F. I (89); IV (C. 1. 3-5; D. 2-1) I-IoangT.F. 1(119) Hodges R.J. IV (I'M. 3. 1-7) llodor I. IV (C. 1.3-54; D. 4-18) Hoc ring T. C. IV (F. 1. 2.3- 3) Hojman .T.M. IV (0.3-02) Itolcomb H..P. Ill (105) HolmV.C.F. IV (F. 1.1-2) Ilolmbcrg K. E. I (214); IV (B. 9-1 2; P. 2. 5-3) Holtslandur W.J. IV (F.'l. 5. 1-6) ' -:/-n Hondo E. TV (C. 3-4«) ,y". Hori Y. IV (r:. 3-K!) ^ Horibe Y. Ill (125) 7j" Horiuti J. I (108,179); IV (C. 2.2-3; C. 3-45) . Ilurnkc J. IV (C. 1;2-67; D.4-1G) Howies on J. I (147) Hsu H.P. III (92) " Hsu Y. P. IV (D. 6-31) Huber M. IV (D. 5-65) Hucbener R. P. IV (C.1.3-17,20, 31; D. 4-13) Huebner H.. Ili'(188) • Huffman J. R. IV (C. 2; 1-8, 9; C. 2. 2. -24; D. 5-1, 2, 3, 7, 8); Hughes E.D. IV (C. 2.2-6; D. 5-12,13) Hughes H. E. 335

Hughes H. E. IV (C. 2,1-25) Hull ILA. IV (D. 2-4) Hunt C.d'A. IV (F. 2.1-1) limit II. IV (C.3-15) Hurst Jl. 1(143); IV (A-G9) Hutchinson C. IV (F. 1,1.0-1) Hutchinson CA, IV (C.2.2-2G) Iluyskcns P. IV (C.1.2-11) Hvidt A. IV (F. 1,4.2-1) 336

- I

Ica C. II. IV (A-130) potali. IV (F. 1.2.4-4) IhIeH« IV(C.1.2-3G) Impastato F. J. IV (F. 1. 4.1-3)

Indovina R, j (G4)

Ingoici C. K. HI (7);'lV (A-G); C. 2. 2-G)

Ingoici E. li m (Y)

IrsaA-P- IV (C.l. 2-15, 16)

Isakofr t. v (B-19) 'snida S. IV (CI. 2-56) Ishida T- IV (CI. 3-44)

Isberg P. In (61) IvanovO.A. IV (F. 1. 3. 2-7) Izrailevich E. A. \ (34g) 337

- J

Jackson D. P. IV (C.1.1-50) Jacobs J. J. II (41) • Jacobs J. AT. n (38,40) Jacobson 0. HI(17) Jacolin O. II (51) Jaeger K. in (175) Jafrkc IT. IV (C. 2. 2-50) James B.J. IV (C.1.3-52) Jason A.C. 111(148) Jaulmos P. IV (C. 2. 2-9) Jerfcrs P. IV (P. 1.2. 3-7) Jeffries R. IV (F. 1.4. 2-2) -lenkinson W. G. V (B-24) Jcnn J. T. IV (A-125) Johanscn CI. Ill (17) Johns T.F. IV (A-7G) JohnsonB.S. IV (C. 2. 2-71) JohnsonC.A. IV (C. 2. 2-34) Johnson F. A. 1(174) Johnson K. D, IV (22-27) Johnson V. II.' II (30, 31, 34) Johnston I-I.L. IV (C. 2.1-11, 12; D. 5-9; D.G-9) Jones M. L. IV (C. 1. 3-50) Jones T. O. IV (C.2.2-4) Jones W. AT. HI (164)-' Joris G.G. IV (A-35; C. 1.3-5) Joseph E. F. IV (D.G-32) Jost W. IV (F. 2. 6-1) Julliot C. II (110) Jura G. III (53)

>>*'. 339

Kakihana II. 1(178); IV (B. 10-3; Kalinachenko V. R. IV(A-77; F. 1.8.'2- Kalinina S. E. IV (C.1.2-51,55) Kallmann H. I (1); III (2) Kalyanasundaram C. V. IV (A-106) Kamienski B. IV (C.3-30) Kanda E. IV (C. 2.1-30) Kandier L. IV (B. 10-29) Kanekar C. R. 111(106) Kaneko J. IV (C. 1.2-30) Kant A. IV (C. 1.2-15,16)

Kaplein A. K6)

Kasten P. R. V(B-34) Katclnikov S. G. IV (C. 1.1-37) Katorski' A. IV (F. 2. 2-8, 9,15) Kats M.ya. III (71,121) KatzJ.J. IV (C. 1.1-21; E-lß) Kawashimn K. IV (D. 6-20, 33) Kawazoo Y. IV (P. 1.2.4-4) Kazanskii V. B. :IV(F.r.3.2-5) Ka'/avchinskii Yrx. 7,. 1(188) KecsomW.II. IV (C.2.1-3) Kokoh A. IV (A-158) 340

Keller F. IV (C.'3-20) Keller W. 11. • IV (D.2-3); V (B-3?) Kelly M. IV (F. 1.1-8) Rombali C. IV (C.1.1-36; C.1.2-23,25; F. 2. 3-1) Kcnyon A. R. IV (C. 1.2-50) Kcrwinl. L. 111(103) Kesselraum P. M. 1(188) Kessler R.W. IV (C. 1.3-17, 20, 31; D.4-13) KeycsD. B. IV (C. 2. 2-21, 39) Kilcle G. I (74) ' Kimball A. H. II (5, 6) Kimball G. E. IV (A-13,15) Kimbrough D. Jr. 111(206) King. J. Jr. IV (F.'2. 2-12) KirillinV.A. I (188);'III (117)

Kirshenbaum I. I (93,125,127); II (6); IV (A-18J53;-,C'.l;lr10) Kiss I. 1(199)' 'S; Kistemakcr J. 1(155) Kitt G. P. IV (F. 2. 2-4) Klein F. S. IV (B. 2-29; C. 1. 2-41; F. 1. 5.1-1) Klein R. IV (F. 1.1-4) Klomm A. I (01,151); IV (A-26; B. 10-5; C. 3-58) Kliefoth W. I (141) Klotz I.M. IV (F. 1.4.2-5) Knaap II. F. P. I (205) , Knezevic Z.V. III (181) KnoblerC.M. ., IV (F.2.2-15) KnottA;R. 111(197) 341

KnopL. . IV (C. 2.2-58) KnowlesA.E. IV (B.'10-4) Kobayakawa M. 111(125), Kocent A. HI (184) Kodera T. l (159) KohnH.W. IV (F. 2. 2-11) KoltsnyUZ. IV (D.2-28) Kono M.' IV (A-94) Kosaric N. v (C-35) Kot A.A. 1(195) Kramer H. HI (207); V (B-53) Krause I. M. IV (F. 1.4. 2-1) KrellE. IV (A-147; C. 2.'1--41; C. 2. 2-68, 74) KresgeA.J. IV (C. 1.3-19) KretzchmanG. IV (A-111; ci 2. 2-66, 69; F. 2. 5-4) Krogh A. m (13) ; Kroh J. -, IV (F. 1.3.1-4) Kronbergor II. IV (F. 2.7-2) Krumbicgel P. Ill (188) Kruse E. * (145) • Kubota M. , IV (C. 2.1-30) KuchaevV.L. IV (F. 1.1-7) Kuechler L. !V (A-10Ó; C.3-31; E-20) KuessncrA. ,'.'.IV (B. 10-25) Kuhn W. IV (A-44; C. 2. 2-5G; D. 5-GO) Kulicke P. IV (A-147) Kumar R. Ill (113); IV (A-106; C. 3-84; E-36) Kummer J. T. IV (C. 1.' 2-21) 342

Kummerer K. III (14G) Kurchatov I. V. 1(157) Kurihara Y. IV (A-12G, 127; C.'l.'3-40); V (C-26, 27, 28) Kuwata K. IV (F. 1 -2.1-3) Kysela J. III (211) "• •

• I

ni'«*!.', 343

LabatonV.Y. IV (P."l." 8.1-2) Labine R.A. IV (E-12) Laidler K.J. I (84) Lake G. R. IV (C. 2. 2-32) Lambert R. W. IV (F. 1.'2. 1-2) Landsberg G. S. 1(3) Lane J. A. V (B-12) Lang G. IV (C. 1. 2-66; D. 3-11,16; E-59) LangdonW.M. ;; IV (C. 2. 2-39) Langer A. I(124) Lantus E.H. - IV(A-174).

Lapteva F. S. Ill (121) :, Large E. • ••'_•, IV (C. 2. 2-12) Lasareff W. I (1); HI (2)/

Lassettre E. N. ; IV (F. 2.2-7) Las son A. T. IV (C. 3-72) Lauder I. J. I (109) . ; Lavrencic D. jV. IB-30,48) Lavrovskaya G.K. ; •; III,(G2); IV (F. 1. 3. 2-1, 3) LawC.A. ; : IV (A-157; C. 1.1-39; E-30, 53) Lawrence S. J. 11(11) Lazard B. IV (A-86; C. 1.1-22; D. 5-45) Lazurkin Yu.S. IV (F. 1.3.2-6) Lazzarini E. Ill (169) Le Chatelier J. IV (D. 3-5, 7) Leconte J. Ill (54) 344

Ledoux A. V (C-33) Leo J. L. IV (C. 1.2-37) Lees A. 111(148) Lefrancois B, IV (A-134, 171; C. 1. 2-33, 34, 49, 60; D. 3-4, 7,14) Lehmcr W. IV (C. 2. 1-36,48,49; D. 5-42) Lehrer Y. IV (D. 5-27, 41) Leichtling B,H. IV (F. 1.4. 2-6) Lentz H. IV (C. 2. 2-83; E-46) Lepoutre G. IV (C. 1.2-43) Lerat J. M. I (193);.IV (A-134) Lewins D. M. ,IV(A-1G7, 173) Lewis D. IV (C. 1.1-48) Lewis G. N. I (7); IV(C.2.2-1; C.3-2,6) Lewis G. P. IV (C. 3-80) Lewis W. B. V(B-4,31,36,44,67) Leyden D. E, III (180) Libby W. F. IV (C. 2.1-10) Lichtenstein R. M. I (102)" Liforov V. G. 111(151) Lifshitz A. IV (C.1.1-48) Linderstroem-Lang C.U. IV (A-Ì18; F. 1.4.1-2; F. 1.4. 2-1) Linderströem-Lang K. III (17) Lindner J. 1(21) Ling F. L. V (C-22) ••"•••• ^ •Liu.wT.C, HI (160," 161) / r' Llewcllin.D. R. IV (C.'2. "2-43, 47; D.5-13)

/ 345

Lloyd J. T. IV (D. 6-20) LoC.F. ' III (161) Lohmar W. IV (F. 2. 2-2) London H. I (175) Long F. A. IV (F. 1.2. 2-6) Lories R. IV (C.1.2-11) Lousiart A. 111(110) Loveridge B.A. 111(58) Lozhkina M. G. IV (F. 1. 3. 3-2; F. 1. 8. 1-1) Lumetti A. V (B-30) Lundberg L. Ill (61) Lundkvist B. . I (198) Lunelund H. 1.(53) Lyon A.M. IV (C. 2. 2-26) LyonC.J. IV (A-104; D. 2-8) 346

M -

Mac Donald A. Ill (81) Mac Donald C. G. IV (F. 1. 3. 1-3) Mackenzie H.A.E. IV (C. 2. 2-44, 45; D. 5-17) Madison J. J. IV (F. 1. 2. 1-6) Mahadevan E. G. Ill (113, 191); IV (C. 1. 3-39; F. 1. 2. 2-5) Mjzovb M. Ill (186) MakishimaS. IV (C. 1.3-21) Maksimovic Z. B. V (C-14, 31) Malan-Nelson A. M. I (44) Malasek E. IV (E-37); V (B-23) Malherbe P.N. IV (C. 2. 2-45; D. 5-17) MalkovM.P. IV (A-89; C. 2. 1-14, 32,40; D. 5-20)

Malleroy A. IV (A-162) MaloneyJ.O. IV (C. 2. 1-19, 25; D. 4-3,4; D. 5-28) MalyusovV.A. IV (C. 2. 1-37) • ,. Mancini C. V (B-71) Manciulescu A. 'IV'(A-159) Mandel H. V (B-58) Manowitz B. 1(229) MarazanN. IV (C. 1.3-38) MarchettiC. I (29); III (43, 47); IV (C. 1. 3-8; D. 6-23,30)

MarcusW.C.de IV (A-50) Mardaleishvili 11. E. IH (G2); IV (F. 1. 3. 2-1, 3) Margincanu P. IV (C. 1. 3-25, 30, 32, 37, 38, 47, 57, 59) Maria-Arcocha A. M. IV (A-135; C. 1. 1-20; D. 6-35, 36) Marinkovic M. D. V (C-14, 31) Mark II. 1(41,52) 347

Marsigny L. IV (F. 1. 4. 1-1) . Martin TI. . I (113); IV (C. 3-60) Martin IT. Z. IV C. 1. 2-29) Martin W. IV (C. 2. 2-12) Marcinola F. V (C-8) Marx R. IV (C. 1.1-26) Masami S. • IV (D. 5-61, 62) Mateescu F. IV (F. 1.2. 4-3) MathurS.C. HI (106) Matsugashita T. IV (C. 2. 1-30) Matsumoto S. IV (D. 5-61; D. 6-33) Matsushima T. IV (C. 1.3-53) MattauchJ. 1(29,54,81,86) Matter'G.L IV(C.2.2-22) MaughanG.L ' II (39) Mayer ILL. I (87); IV (A-17, 24, 25; C. 1. 2-7, 8, 10) Mayer M.'G. • IV (A-29) Mazzoni A.' IV (D. 5-22) McClureD.C. IV (C. 1.1-2) Mc Daniel E.L. IV (F. 1. G. 2-1) Mc Donald R. T. IV (C. 3-6) Mc Donough R. Ill (59) Me Fadden C. II (32) McKeeD.W. IV (F. 1. 3. 3-3) Mc Lain S. I (143): IV (A-69) Mc Manus C. J. IV (C.'2. i-13) Mc Williams J. A. • IV (D. 5-29, 33) Meersche M. van ' IV (F.1.1-1) 348

IVIeleshko V. P. IV (F. 1. 9-2) Mcnes F. I (193) Mcrcca J. Ill (204); IV (C. 1. 3-32) Mercca V. I (213); IV (A-99, 148, 149, 1G0; C. 1. 3-29, 32, 3G, 37, 47, GO; D.4-15, 17; E-31) MerielY. IV (A-133) Merlivat L. IV (C. 2. 2-72) Meyer F. I (134) Mikami II. IV (F. 2. 9-1) Miliaila A. II (59); IV (A-155) Mikkelcit W. Ill (15G) Mikolic S. S. I (5) MillarC.H. V (13-37) Miller A. I. I (215) Miller R. W. IV (C. 2. 2-38) .MillcrS. L. IV (C. 1.3-1.8) Mills G. F." II (10); IV (C.2.2-4G) MilhcrA. M. • IV (C. 2. 2-44) Milosevic R. V (C-35) Missbach D. IV (À-U.7) . • Mitchell J. Jr. IV(C:2.-2-.18) '. Miyahara K. IV (C. 1.2-31, 4G) Mizusliina T. - IV (A-94) Moggi S. ' I (71) Molinari Ph. I (193); IV (F. 2. 2-14) Mongini L. 1 (139) Monier .I.A. IV (D. 5-5; D.6-10) Monna G. IV (C. 2. 1-30) Montarnal R. IV (C. 1. 3-15) 349

Montgomery CR. V (C-23) Montgomery G. W. IV (C 2. 2-30) Moraru N. IV (C. 1. 2-53; C. 1. 3-54; E-31) Moravec J. Ili (211) Morcau C. IV (C. 1.2-43) Morgan T. D. Ili (147) MorLta N. Ili (12): IV (C. 1.3-22) Morlta T. V (C-26) \ Morowitz I-I. J. II (17) •.'••:••• MorozovN. M. IV (C. 1.3-33) Morphcw A. T. II (9) Morris J.W. IV (A-117; C. •]. 1-9, 34) Morrison J. A. V (C-25) : Morrison J. U IV (F. 1. 4. 2-3) MrochekJ. È. IV (E-52) Muhele K. IV (A-147; C. 2. 2-66, 69; F. 2. 5-4) Mueller G. I (200); IV (F. 2. 7-4) Mucllcnpfordt J. I (209) Mund W. IV (CI. 2-11; F. 1. 1-1) Murphy C. M. I (2, 125, 127); III (3, 5); IV (A-53; C. 2. 2-2) MiirronhoffA. P. T (1 90); TV (A-1 31, 132) * Muyllo R. 1. ( I 08) MyagkoiO.N. IV (F. 1. 9-2) Myhrc K. IV (C. 3-713) 350

N -

Naclimanovich M.L. IV (C. 1. 3-33) Nagaraja-Rao S. IV (E-33) Nagrathna R. A. II (Gl) Naito Y. Ill (100) Nakanishi A. IV (A-94) Namba S. Ill (83) NassonovP.M. V (C-31) NalcrK.A. V (C-7) Natta G. IV (C. 2. 2-22) NedumovaE.S. TV (C. 1.3-46) Nelson W. L. IV (E-47) Nepi 0. V (B-5.1) Neumann K. . IV (C. 2. 2-13) Neumann L. I (196)

Newell J.L. IV(C.3-3)/;: Newell W.C. IV (C.3-42) . - ,, Newton C. L. IV (C. 2,1-50) Nicholas CM. .• ; 1(173) ':./:•••;

NiefG. ••• .: III (126,144); IV (A-86, 121; C. 2. 2-72) Nicr A.O.C. I (155); III'(21)' Nikolaev M. N. 111(151) Mkolacv P. N. IV (A-59) NikoUcR.M. V (C-31) Nito S. IV (C. 3-77, 78; D. G-33, 34) Mtschke E. IV (A-175; JJ.3-12; D.4-13) Noguclii T. IV (C. 3-36,51) Nordemann. D. Ill (110) I

? 351

I Normand J. I11 <133) I Norton E.R. IV (C.1.1-46, 47) I Norton W.J. IV (C. 1.1-6) I Novakovic M. IV (C. 2.2-57) ! Nowak E.S. 111(205) 352

O -

Obi nata I. IV(B:10-28) Oddio T. II. IV (C.3-38) Ugo K. VIB-GG) Okahc: T. HI (.1.39) Okajima Y. IV (C.3-GC) Okajnoto CI. IV (C.2.2-8; C.3-45) Olariu A. IV (A-149, 1G9; C. 1. 3-32, 37, 38, 47, 57, 59; C,2. 2-G7; D. 5-58; E-31) Oppenheim I, il (34) Orchin M. 111(3 0) Orlov V.V. III (151) ursoni B. IV (D.G-14) Orsoni L. III (3G); IV (C. 3-59; D. 6-17, 21) Ortego J. M. IV (C. 2. 2-79) Ortiz-Fornaguera R. V (B-15) Ota Y. IV (C. 3-21, 37) Otero de la Gamlara J. L. III (1.11, 142, 150, 171,177, 192); IV (A-72, 135; C. 1. 1-20; C.2.2-76; C. 3-67, 73; D.6-35,3G,38,39; E-17) Otero Navascues J. M. V (B-7) Othmcr D. F. IV (C.2.2-19, 20, 23) Otwos J.W. IV (F. 1.3. 2-2) Ou eilet C. 1(22) Oulibin S. A. 111(117) Oyama Y. IV (F. 2. 9-1) 353

- P -

Paabo M. 1(228); 111(202) Paemel O. van I (99) Paladi M. IV (C. 1. 3-55) Palibroda N. . IV (A-148; C. 1. 3-36, 42; D. 4-15,17; E-31) Panchcnkov. G. M. I (14G); IV (F. 1. 9-3) Pannetier G. IV (F. 1. 4.1-1) PaoluziG. IV(F.1.4.1-D ParfenovV.A. 111(151) Park J. L. II (16) Parker A. 111(136) Parravano G. I (101) Parrucini M. Ill (59) Patterson W. A. 111(59) PaudlerW.W. IV (F.'l. 2. 5-1) Paul S.D. V (C-29) Paulicka I. V (B-6J) Paulsen F. R. IV (C. 1.2-35) Pavlov K.F. IV (C. 1.2-14) Pavlovic B. IV (C. 1.3-9) Pearse R. W. B. IV (F. 2.6-1) Peculea M. IV(A-99,143 C. 1.3-36, 54 D.4-14,15, 18 E-31, 34,38,41,43,50) Pedretti A. V (B-70) Pegram G. B. IV (D. 5-1, 2) Peisach M. I (169) III (140) Pepper D. IV (C. 1.2-47,50) ' Perilli M. L. V (B-54) .354

Perlman M. L. Ill (48, 50); IV (C. 1. 2-15, 16, 18, 19, 27) Pcrperol H. IV (A-3 3) Perry J. II. ' 1(85) Pcrsson T. I (198) Peters K. IV (F. 2. 2-2) PotlersenG.T. IV (C. 2. 2-73; F. 2. 4-4, 5) Pctrov I.Ya. IV (F. 1. 3. 2-6) Pctrov P.A. V (B-8) PettersL. B. IV (F. 1. 8. 4-1) Phillips J. C. IV (C. 2. 2-29) Pierotti G.J. IV (C. 2. 2-38) Pigford R. 1.(15 0) Pilot J. IV (F. 2. 9-2) Pilz S. IV(A-92; D. 5-47) Pimentel G. C. 111(53) PiretE.L. 1(158) Piringer O. IV (C..1. 3-25, 55) PlaskuraW. I (207) Pohl I-I. A. I &72); IV (C. 1.1-28, 30, 31,32; D. 2-4) Pohler G.M. IV (C. 2. 2-23) Polanyi'M. I (48); II (4); IV (C. 3-9) Polastri F. IV (D. 3-15) Pomerantz P. IV (C. 2. 2-42; D. 5-16) Potter R. A. Ill (24, 27, 28, 29) Powell'J. I (229) Prasad N.B. IV (C.2.1-31)

Pratt H.R.C. I (170); IV. (A-67f141; C. 2. 2-54; D. 2-8; D.5-29,33) Pressung B. 3 IV (D. 5-57) Pretorius R. m (210) Pretorius V. IV (B. 11-33) 355

Prigogine I. IV (F. 2. 7-1) Proctor J. P. IV (D. 2-13; E-22, 25, 32) Proksch E. Ill (162); V (C-19) Prosovits P. I (47) Prosser II. C. Ill (48, 50); IV (C. 1. 2-16) ProtterS.R. 111(195) Puddington I.E. Ill (31) Pugh 0. IV (F..1.8. 1-2) Purcaru C.I. I (153) Purcell R.I-I. IV (C. 3-42) Pyper.T.W. IV (F. 1. 2. 2-6) 35fi

Q

Qu inn F.G. I.V (C. 1. 2-2, 9; C. 2. 1-19; D. 4.-4; D. 5-28) 357

- R -

Rabinovich I. B. IV (A-59) Rabinovitch B. S. IV (D. 6-18) RadulescuC. 1(161) Rae II. K. IV (A-138, 142,165; C. 1. 1-44: C. 2. 2-52, 53, 55; E-5; F. 1. 5. 1-3,6); V (B-59) Raman M.S. IV (C. 3-76, 84) Rampey W. P. Ill (208) Randall M. IV (C. 2. 2-17) Rank D.H. IV (C. 3-7) Ranque G.I. IV (F.2.3-3) RapLalA. S. IV (D. 5-66) Rapoport L. L. IV (C. 1.2-51) RavoireJ. IV (C. 1. 2-44, 45, 54, 65) RayH.S. IV (D. 4-4; D. 5-28) ReaserP. B. 111(108) Rebora P. L. IV (C. 1. 2-38) Reed R.I. 111(81) RegimbalJ.J. Ill (123) Reid A.F. IV (A-32) ReidPI. B. V (B-24) ReilleyC.N. Ill (180); IV (F. 1. 6. 1-2) Reinhold G. .IV (F. 2. 7-4) Reitz O. • .1.(55) RenzoniR. IV (C. 1. 3-8, 12, 16, 20; D. 4-8, 9;D. 6-27, 30) Reuben J. IV (F. 1. 7. 2-6) Reyerson L. H. ' IV (F. 1. 2. 2-1) 358

Reynolds P. Ill (58,65) Reynolds T. G. IV (C. 1. 2. -2) Ribnikar S. IV (C. 1.3-9) Rich E.H. IV (C. 2. 2-42) Richter E. L. Ill (174) Ridoal E. K. I (24) Riedinger M. IV (C. 2. 2-78) Riosenfeld E.H. I (G5) Riualclini C. V (B-45, 55) Rishcr C. IV (C. 2.1-13) Rittenbcrg D. IV (C. 1. 3-18) Rivldn S. L. I (.1.88); III (145,158) Roberts E. R. TV (C.1;2-14) Robinson II. K: 111(196) Robinson R.D. IV (D. 2-25) Rock S. M. Ill (37) RoddenC. J. I (192) Rogiinski S.S. • I (182) Rojas de Diego J. L. Ill (150,171,177, 182, 192); IV (A-135; C. 1. 1-20; C. 2. 2-79, 80, 81; D. 5-70; D.6-39) Rolle W. Ill (188) Romaniw M. IV (B. 6-1, 2; B. 11-1) Rosatzin II. I (223); III (201) Rosebury F. 111(20) Rosenthal M. W. V (B-27) Roseo L; iy--(C.l. 3-7,8) Rosta P.Z. I (235) Rostaing M. IV (A-136, 168;C. 1. 1-38;D. 3-6)w .; Roth E. 1(142, 193;202);III (41,54, 153);IV(A-58, 68, 86, 101, 119, 134, 136, 166, 168, 171;C. 1.2-39, 62); V (B-21;C-4, 5) 359

Rothberg S. . IV (D. 5-16) Rowland P. R. 111(193,197) Royen P. I (72) Rozen A.'M. I (154); IV (A-57, 109; C. 2. 1.-21) Rozenborg J. IV (F.3-2) Rozental K. I. IV (C. 3-5G, 57) Rubin L. C. IV (C. 2. 2-33,34) Rubissow G. A. IV (B. 11-27) Ruderman I. W. I (152) Ruhtz E. IV (C. 3-60) RuskinS. L. IV (B. 11-16) Rüssel S. II. IV (E-55) RustF.G.D. IV (C. 2. 2-71) Rustad B. 1X1(21) Rutherford E. 1(12,33) Ruzicka J. IV (C. 2.1-35; E-23) RyanR.-K.'"' IV (A-151) Rypar V. I(196) 360

Saclhukhan H. K. IV (D. 2-27) Sage B. II. IV (C.l.1-11) Saito E. I(193) Sa ito II. IV (C.l. 3-22) Saito T. V (C-26) Sakharovskii Yu. A. IV (CI. 2-61) Sakodynskii K. I. I (187); IV (A-88, 95,103, C 1. 1-15). Salmon O. N. IV (F. 1.7.1-1) Samoilov L. N. I (189) Sampaleanu L. IV (A-143; C. 1.3-54) Samuel F; IV (F.1.7.2-6) Sandroni S. III (127, 132) Sandstrocm A. E. III (45) Sansone M. V (B-54) Santos-Macedo C. M. IV (A-93) Sapirstcin L. A. II (38) Sara V. III (211) Sataka O. IV (CI. 3-22) Satchel'l D. P. N. IV (F. 1.2.1-2) Sato S. IV (C. 2.1-30) Sato T. IV (C 2. 1-30) Sattler H. IV (C. 2. 2-12) Savard J. IV (C.3-55) Savie P. IV (C. 1.3-9; C 2. 2-57) Sawayanagi S. IV (CI. 3-40) 361

SaxenaS'.C. IV (F. 2. 7-3) Sayama H. IV (A-94) Scatchard G. IV (C. 2, 2-25) Schacherl F. IV (A-4) Schaeffer O. A. IV (F. 1.1-6) Schaumburg K. 111(199) Scheepors L. Ill (8); IV (C. 3-18) Scheer M.D. IV (F. 1.1-4) Scheibelhut C.H. V (C-2) Schenkel G. • HI(129) Schierholz H. IV (C. 1.2-36) Schindcwolf U. IV (C. 1. 2-48, 53, 66, 67;C. 1. 3-34; D. 3-2, 11, 16;.D.4-13, 16; E-59) Sclatterer R. IV (C. 2.1-36) Schmid L.C. V (B-50) Schmidt W. A. 111(174) Schmieschek U. IV (B. 11-22) Schnette R. I (212) SchoenL.J. IV (F. 1.1-4) Schoenborn E. M. ... IV (C. 2. 2-35) Schoenemann K. IV (B. 1-19, 20) Scholz.W. IV (C. 2.1-43) Schuetze II. IV (A-147; C. 2. 2-66, 69; F. 2. 5-4) Schuetze W. , IV (F. 2.6-4) Schumann K. D. ,-..IV (C.-3-74) ., , Schwartz K. ' = IV (C. 3-31) Scoüeld R. .:;.;:,.;• iy(D.5-14) ScottR.B. : ' 1(110); IV (C. 2.1-4) ,. 362

Scottcn W.C. IV (A-117, 157; C. 1.1-34, 42; E-32); V(C-12,17) Scuricini G. B. V(B-30,48) Seattles J. C. IV (B. 10-20, 22) Sehgal I.J.S. IV (D. 2-27) Seidel D. I (212) Seito E. I (66) Sekowski S. I (163) SclakP.J. IV (A-43) Selecki A. I (204); IV (A-156; C. 1. 3-23, 24; C. 3-79; D.5-72; E-21) Selleck F. T. IV (C. 1. 1-11) Sellers E. S. IV (C. 2.1-22) Sellmaicr A. IV (D. 5-42) Selmi L. Ill (42,44) SelwoodP.W. I (80); IV (C. 3-34) SemenovV.A. 111(151) Semiokhin I.A. I (146) Senn A. V(C-38) Senvar C.E. I (203) Shacter J. IV (A-79; E-2) Shah P. G.S. II (52) Shalnikov A. I. Ill (102) Shamsul A. K. M. IV (E-39) Shank R.C. Ill (137,167) ShannovJ.S. IV (F. 1.3. 1-3) ' SharmaK.C. IV (C.2. 1-31) Shatenstein A. I. I (148); III (84, 94, 96, 97, 98, 114); IV (A-77; F.l. 8.2-1; F. 1.8. 3-1, 2, 3,4) Shaw A.J. IV (A-9) 363

Shaw B. IV (C. 2. 2-26) Sheffield E. L. IV (C. 2. 2-25) Sheinlin A. E. : I (188) Shelud'ko M. K. IV (C. 3-12, 40, 53) Shepherd E. V (B-ll) Sherman A. I (8) Sherman lt. H. IV. (F. 1. 2. 3-1)

Shimizu M. IV (C. 3-77, 78; D. 5-61; D. 6-33, 34) Shinichi H. IV (D. 5-62) Shires R.N. .. iy (C. 2.2-38) Shlypnilcov S. V. TV (C.1.1-37) Shpilrain E, E. 1(188) Shtukkenberg Yu:M. . . 1(224);: SilbermanE. -Ill (72); IV (E-29) B. I-,. IV (F. 1. 7. 2-6) Silverman L. Ill (51) , Silvestri M. I (129); III (36, 43, 47, 75, 80, 85, 86, 88); : .';.•; . IV (A-27, 66; C. 1. 3-8,12, 16, 20; C.2.2-77; C. 3-59; D. 4-7, 8, 9; D. 5-30, 52, 64, 67; D.C-17i21,22, 23,27, 30); V (B-71)-,..•• .-.-.... Simonet G. IV (C. 2. 1-33,44, 46) Sinev M.N. I (219) Singleton J.H. IV(C.1.2-14) Sivetz N. • i •• . •'-•• V (C-2) SkarreO.K. I (70)'' :; ,:>.:: Skrinnikova H. P. • :; ::IV (C. 3-33) SlackC.M. ;;:;. IV.(C 3-49; .p. 6-7) SUn'ko M. G.,. IV (C.l. 3-46) Slutskaya N. M. Ill (10, 11, 16); IV (C. 3-12, 40) 364

Small P.A. IV (C, 1.1-13) Smirnov B.I. Ill (15.1) Smith D.M. IV (C.'2.2-18) Smith E.R. Ill (C); IV (C. 2. 2-2, 3; C. 3-5) Smith F.A. IV (C.'3-20) . Smith H.A. IV (0.2.2-51,60, 65) Smith N. A. IV (F.'1.'G.2-1) Smith S.R. IV (D. 5-11) Smythc II. D. I (112) Snyder J. A. IV (C.1.1-12) SokolovE. Y. IV(F.2.ö-3) Solli R. IV (C. 3-68) Sollich-Baumgartner W. A. IV (F. 1. 2. 1-5; F. 1. 3, 1-1, 2) Solomon E. IV (C. 2. 2-34) Solomon J. 111(105) Sonderhoff R. Ill (15) Sonoda S. V (C-26) Soudors Jr. M. IV (C. 2. 2-38) Souza-Reis F. de - 1(71) Spacilll.S. IV (C.3-85) Spaepcn J. Ill (82). SperandioA. IV (D. 5-65) SpevackJ.S. IV (A-14,16; B. 1-4,18; C. 1.1-1, 3,4, 5, 53) Spraklcn S. B. Ill (63) Spray P. H. G. IV (D. 2-26,28) Stacey I. IV (F. 1. 2. 2-2) Starke K. IV (C.2.1-15) 365

Staschcwski D. 111(203) StasovLch B. M. - 111(71) StodmanD.C. IV (F. 2. 4-1) Stcdman D. F. IV (C. 1. 2-22; C. 2. 1-5) Steinberg M. I (229) Steiner I-I. IV (C. 3-31) SteLnert B. I (76) Steinert C. V (B-42, 52) Storming A. H. IV (C. 2. 2-53) Stephan M. J. IV (F. 1.1-3) Stephan W.J. IV (D. 6.-15) Stephens W. E. 1(124) Stern F. IV (C.2.2-58) Stevens CM. 111(21) Stevens W.U. 111(60,104,118,138,149,163) Stevenson D. P. IV (F.1.3.2-2) Steward D.W. I (98) •Stiehl G. IV(A-147) Stockmaycr W. II. IV (A-13,15) Stoeckl K. I(59) Stoicovici L. IV (D. 4-17) Stouls L. IV (A-83, 86; C. 2. 1-44,46; D. 5-44) StrauleaR.S. IV (D. 4-18) Street E. E. . IV (F. 2. 8-2) Striganov A. It. ', 111(93) Strugaru D. IV (C.1. 3-55) Stumper R. IV (C. 2. 2-11) Stutheit J.S. Ill (208) ' Stziganov A. R. 111(78) 366

Subranianian G.S. IV (C. 3-G4) Suda N. V (B-GG) Sucss II. I (G8, 107); IV (C. 1. 3-G) Sulima L. V. IV (C. 1.2-12) SunC. IV (F.1.11-1) Surowicc A.J. IV (D. 5-48) SuslovB.N. 1(156) Suzdaltseva S. F. Ill (94, 97) Svendsas P. V (C-18) Svenke E. IV (A-150) Swain C.G. IV (C. 1. 3-.19) Swaroop J. IV (A-170) Swiatowski W. IV (C. 2. 2-70) Swislochi M. HI (37) SychevV.V. 1(188) Symons W.J. 111(196) SzeM.C. IV (C. 2.1-45) Szentgyorgyi P. 11 (59); IV (C. 1.3-25,30,41,48,61) 367

- T -

Tai Y.K. IV (D.G-31) Takamatsu T. IV (A-94); V (C-2G) Tamaru K. IV (C. 1. 2-56) Tanaka K. IV (C.1.2-56) Tashiro T. IV (C. 2. 1-30) Taylor E.H. IV (A-35)

TaylorH.S. I (14, 94); IV (A-35; C.3-8, 34; F.2.2-1) Taylor J.K. Ill (198) Taylor T.I. I (201); IV (A-129; F. 1. 2. 2-5) Tatevskii V. M. IV (C. 1. 1-8) TealG.K. II (3) Temkin M. I (38); IV (C. 1. 3-33) TerrillJ.B. IV (F. 1. 6. 1-2) Terry E. A. 111(136)

Thayer V.R. IV (A-41, 42, 90, 115; C. 1.1-.17, 35; C. 2. 2-62; D. 2-11, 12, 13; E-22, 25, 32)

Thiel S- IV (A-147; C.2. 2-74) Thiele E.W. IV (C. 2. 1-6, 7) ThodeH.G. IV (D. 5-11) Thomas B.W. Ijj (35)

Thomas C.O. IV (A-78; C. 2. 2-65) Thomas H.. II (15) Thomas H. C. IV (F. 1. 7.1-2) Thomas J. R. 11(39), 3C>8

Thomas M.H, V (C-25) Thompson S. O. IV (P. 1.1-G) Thompson T.J. Thompson \V.I. IV (C. 1.2-17) Thornton V. HI (39) Thucrkauf M. HI (112); IV (C. 2. 2-G3; D. 5-G3) Thurston W. M. ni '(GO, 163) TiaS.Y. V (C-22) Tillol A. IV (C. 1.1.-22; D. 3-7) Timmerhaus K.D. IV (C.2.1-24,28; C.2.2-G1; D. 5-37) Timrot D.L. i (188) Tipton Jr. C.R. I (1G5); V (B-18) Titani T. Ill (12); IV (C. 2. 2-7) Tohmfor G. IV (C. 2. 2-13) ,v Tomaskova L. Ill (200) Tomkins F.S. Ill (25) Topley B. IV (C.3-4,17,23) Traurouder It. , IV (A-171) Trenner N.R. Ill (4G) Tretyakova N.N. IV (A-59) Trilling C.A. 1(234) Trcwistand L. ni (18); IV (B. 10-0; C. 3-32; D. 6-3) Trubitsyn B. A. IV (C. 1. 2-55) Tuchòlski T. IV (C. 2. 2-5) Tuck R. IV (C.2.1-13) Tung T. C. V (C-22) •Turchia V.F. m (151) Türkin V.K.. I (144) Tuxworth R. H. IV (P. 1. 3. 2-4) 369

U -

Uclovichcnko P.M. I(219) Ucda T. IV (F. 1.2. 1-1,3,4,7) Ugajin II. IV (C. 1.3-28) Uhlmarm W. •IV (C. 3-24) Updike O. L. Jr. IV (C.2.2-39) Urey'.H.C. I (2, 15, 16, 42, 46, 77, 78, 79, 95, 96, 125, 127); II (3, 6); III (3, 5); IV (A-10, 20, 53; C. 1.2-4, 5; C.l.3-3,4; C.2. 1-1,2; C. 2, 2-10; C.3-1, 10, 25, 54; D. 5-1, 2, 3; F. 2.6-3) ,.Ursu D. II (59) Uruguchi Y. IV (B.6-3) Ussing II. III (13) 370

- V -

Vaccaro G. IV (D. 3-15) Vagncr J. 111(211) Vaisberg S. E. I (138)- IV (A-45, 9G, 128; C. 1. 3-13, 35; F. 1. 3. 3-2; F. 1. 8. 1-3: F. 1. 8. 3-2) Valant P. V (B-48) Vancler-Aroncl P. C. IV (C. 2. 1-47; D. 5-25) Vaniscotte C. IV (C. 1. 2-33, 34) Varbcrg T. IV (C. 3-G3,68,69) Varshnvskii Ya. M. I (138,148); II (84, 96); IV (A-45, 96,128; C. 1. 3-13, 35; F. 1, 3. 2-6; F. 1. 3. 3-2; F. 1. 8. 1-1,3; F. 1.8.2-3; F. 1. 8. 3-1,2, 3,4) Vasaru G. I (186,191, 227); II (56, 57, 59, 60); IV (A-140, 144, 155; C. 1. 2-68; C. 3-86; F.2. 7-4) Vasatkova J. Ill (184) Vasilcscu A. IV (F. 1. 2.4-1,3) Vasiliev A. M. I (37) Vasiliev G. Ya. IV (F. 1. 3. 2-6) Vasilyev D.I. Ill (102) Veil S. I (31) Venditti P. V (B-30,49) Versino B. Ill (131) Verterssian K.A. IV (C. 2. 2-15) Viallaid R. Ill (34,40) Vic R. Jit (133) Vielstich W. IV (B. 10-19) 371

Villani S. I (176); IV (A-74; C. 1. 1-20;.C. 1.3-8, IG; D. 2-10; D. 4-G, 7; D. 5-30, 52; D. ß-23, 25; E-2G); V (B-71) Villard R. V (C-34) Viratolle J. IV (A-171) Vladimirskii K. V. 111(71) Vlasov N. A. I (189) Voevodski V. V. Ili (62); IV (F. 1. 3. 2-1, 3, 5, 7) Volpi G.G. IV (F. 1.1-5) VoskuylR. J. 111(24,27,29) Voyer R. D. I (215) VromenB. H. IV (C. 2. 2-47; D. 5-19) 372

W

Wagomann K, V (B-53) Wagencr K. IV (C. 3-83) Wagner CD. IV (F. 1.3. 2-2) Wagner II. G. IV (C. 2. 2-83) Wahl M. II. IV (C. 2. 2-10; C. 3-10,25) Waincrdi E. II. III (210) Walchcr W. 1(75,105) Wald AI. 1(52) Waiden G. IV (C.3-54) Wald mann L. 1(90) Walen R. I (130); IV (D.G-19) Walker P. T. IV (A-114; D.2-8; E-27) .. ,- Walker II. W. III (4G) Walker W. IV (A-116) Wallung F. O. IV (D. 5-11) Walter A. I (169) Walter S. IV (C. 1.2-48, 53; D. 3-2,12; D.4-13) Walton U.F. IV (G.3-41,43,46, 52) Wanick R.W. IV (D. 6-16) Wansbrough-Jones O. H. 1(17) Ward D.E. IV (C.2.1-26) .Warren J. IV (C. 1.1-12) Wartenweiler M. V (C-3G) Washburn E.W. III (6); IV (A-1; C.2.2-2, 3; C. 3-1, 5, 20) Washburn [I.W. III (52); IV (C. 2. 2-2,3)- Watson U.E. -ß'' IV (C. 2. 2-49) 373

Watson L.C. V (C-25) Watson-Munro C.N. V (B-2) Wattenberg A. I (92); IV (F. 2. 5-2) WebbG.M. IV (A-19) Webb J. IV (F.3-1) WebbR.J. 111(120) Webb W. A. IV (A-2; B. 10-2; C.2.2-17; C.3-14) Wei C.W. Ili (160) Weight M.M. IV (D. 4-1) Weinberg A.M. 1(221) WelngaertnerE. I (183); III (76, 113) Weise G. IV (A-147) Weiss G. IV (C. 1.1-14, 18) Weisser R. IT. IV (D. 5-40) Weissman Y. IV (D. 5-41) Weitzel D.H." 111(69); IV(C.2.1r28; C.2.2-61; D. 5-37) Welch L.M. IV (C. 2. 2-31) Wender I. IH (30) WenworthT.O. IV (C. 2. 2-19, 23) Weston R. E. jr.. IV (F; 1; 7. 2-1, 2, 3, 4) Wetzel K. I (210); IV (A-lll, 147; B. G-14; C. 2. 2-64, G6,G9; C.3-74; F. 2.5-4) Whateley T.'L. HI (189) Wheat J.'A. . Ili (176) Whcts.ol H.B. II (10) Whitaker II, III (7) White A,S. IV (A-85) White D. IV (F. 2. 2-5, 7, 8, 9, 15) 374

White D.W. IV (C. 3-85) White L.E. 111(69) White R. R. IV (C..2.2-37) Whittem R. N. III (189) Whytlawgray R. III (7) Wicke E. IV (B. 10-25) WidigerA. H. IV (F. 2. 5.-1) Wilmarth W. K. IV (C. 1. 2-26; F. 1. 5. 2-1) Wilson C.L. IV (A-26; C.2.2-6) Wilson R, L. IV (C. 1. 1-36)

Wilson T. IL V (C-l) ; ; Winnaker K. 1(232) WinsGl A. IV (C.3-81) Winter E.R. S. IV (C. 1.2-14) Wirtz K. 1(62); IV (C. 1.3-1) WohlK. IV (C. 2.2-41) Wolczek O. IV (A-3 0) Wolfenclen J. H. IV (C. 3-22, 41,43, 52) Wood J. I. IV (A-163) Woodhead L. W. : V (C-25) Wooley H.W. '.-.'; I (110) ; Wright C.R. 111(197) Wright G. E. IV (F. 1.2. 4-2) Wright M. M. IV (D. 6-12) Wroblenska M. III (143) Wullum T. IV (A-1G3) 375

Yagi S.' IV (B. G-3) Yak: nonlco L. M. IV (A-7 7) Yakovleva E. A. I (148); III (77, 97) Yamada M." IV (F. 1.2.4-4) Ya mat ora I-I. III (168) Yoneda Y. IV (C. 1.3-21) Yoshida A. IV (A-94) Yoshilcawa Y. IV (C.3-66) Yoshioka Y. IV (F. 1.2. 4-4) Young A. R. 11(2) Young J. R. IV (C. 2.2-82,84) 376

a

Zabcc A.W, IV (F.1.3, 1-6) Zanantoiii C, V (B-45, 55) ZavattarclH .fl. IV (D.4-9) Zeldovirch A, G, IV (C. 2,1-32, 40) Zeiger P. V (ß-73) Zellmann E. IV (IM. 7, 3-1) Zelvenskii Ya. D. IV (A-137; C, 1, 2-61; D. 5-21) Zemyan E.M. V (B-5) Zevos N. tV (F 1.2.2-7) Zhavoronkov N.M. I (187); IV(A-05,103, 107,122; C. 1. 1-15; 17.5-21) Zinn W. H. 1(92,100) Zinovyeva N. P. III (C8) Zlotowski ,T, III (143) Zmasek R. IV (D. 5-74); V (C-37) Znamirovsclii V. IV (C. 3-07) Zoch O. IV (A-173; ' 12-37) Zvyagintseva 13. N. 1(148); III (08) 377

Societies Index

A. E.C. Ltd IV (R.2-4G; B. 10-35)

Air Liquido IV (B. 1-10; B. 2-9, 27,31,32,40,41, 42,45; B. 3-23; B.5-12)

Air Products & Chemicals IV (B. 5-21)

Allmanna Svcnska Eloktriska A. B. IV (B. 1-14, IG)

American Security & Trust Co. IV (B. 10-1)

A.M. F. IV (B.11-32)

Asahi Kasci Kogyo K. K. IV (B. 10-33, 34)

Atlantic Refining Co. IV (B. 11-25)

Atomic Fuel Corp. IV (B. 10-33)

Badisdio Anilin & Soda Fabrik A.G. IV (B. 2-23)

British American Oil Cy Ltd IV (B.8-1)

Canadian General Electric Co. IV (B. 1-22, 31)

Cas sella Farbwerke IV (B.11-9,13) '

C.E.A. IV (B. 1-7, 8, 9, 11, 23,24;' B. 2-13, IG, 17;18, 19, 20, 27, 31, 32, 34, 37,38,40,41,42,43,44,45; B. 5-22,23; B.10-27; B. 11-5, 30, 38) ! 378

C.F. T.H. IV (B. 10-30)

Cie de Construction Mecanique IV (B. 2-27, 31, 32,40,41, 42, 45)

C.I.S.E. IV (B. 3-11)

Constructors John Brown Ltd IV (B. 1-15; B.2-10; B. 7-3) & N.W. Roberts

Costain John Brown Ltd IV (B.2-4; B.7-1)

Degussa IV (B. 3-26, 30, 32; B. 5-17; B. 1.1-4,11)

Dow Chemical Co. IV (B.1-21)

Esso Research &. Eng. Co. IV ÜB.1-25)

Fertilizers &. Chemicals Ltd IV (B. 11-28) ^'••P"

Fluor Corp. IV (B. 11-24)' '

F. Uhde GmbH IV (B. 2-5, 8, 12, 25, 26, 28, 30, 33, 35; B. 3-17, 27, 34, 35, 38; B.10-16)

General Electric Co. IV (B. 11-31)

Gesellschaft für Kernforschung mbH IV (B.2-33; B.3-38; B. 11-29)

Gesellschaft 'fUr Lindc's Eis machinen A. G. IV (B. 5-15,18,19,20)

Gulf General Atomic Inc. '-._: IV (B.11-37) &:

Hoechst IV (ß.'5-10)

Houdry Process Corp. IV (B. 3-15)

Ilouilleros du Bassin du Nord et du Pas-dc-Calais IV (B. 2-14,17, 18, 27, 31, 32, 40, 41, 42,45; B. 10-27) 379

I. G. -Farbonindustric A. G. IV (B. 10-3)

Johnson, Matthey & Cy Ltd IV (B. 10-32)

Junta de Energia Nuclear IV (B.10-15)

Lonza IV (B.5-8)

Lummus Co. IV (B.'1-26)

Metalgescllschaft A. G. IV(B.'3-31)

Norsk Hydro-Elektrisk Kvaelstofaktiesclskab IV (B.l-17; B. 2-21; B.3-14; .

B." 10-6, 17,23)

Oerlikon IV (B.5-4,5,6; B.10-11,12,13)

Office National Industriel del'Azote IV (B.3-33)

Osterreichische-Stickstoffwerke A.G.IV (B.2-11)

Pactide Corp. IV(B.C-18)

Pintsch-Bamag A. G. . IV (B. 1-13)

Quartz &Silice i IV (B. 9-3)

Rensselaer Polytechnic Institute IV (B. 1-5, G)

Iluhrchemie A. G. IV (B. 3-20, 29; B. 10-18, 24, 2C;

B. 11-15, 17)

SiemcnsA.G. /. IV (B.'10-31; B. 11-7, 26)

S.N. P. A. • IV (B.' 11-30)

Société de Produits Azoté ' • IV (B. 7-2)

Société d'Etudes pour l'Obtention du Deuterium IV (B. 1-12) 380

Sociótó Industrielle & Commerciale de la Cie des Salines du Midi IV (B.6-9,15,17; B.11-18)

Socony Mobil Oil IV (B. 3^37)

South American Coal Oil and Gas Corp. Ltd IV (B.11-10)

S. R.T.I. IV (B. 11-34,35)

Stamicarbon N. V. IV (B.5-1,2,3,7,11)

Stcinkolilun Elektrizitaet A.C. IV (B. 3-20; B. G-20; B. 10-18, 2G)

Sulzer IV (B. 2-15, 27, 31, 32, 40, 41, 42, 45, 47; B.4-3,4, 5, 6,7, 8, 9, 11, 1.2, B.5-16; B.G-10,11,12,13,19)

U.K.A.E.A. IV (B. 2-6, 7, 22) 24,-36, 39; B. 3-18, 19, 21, 24,25; B.5-9,14; B.6-6; B. 10-7,8; B. 11-6, 8)

Union Carbide Corp. IV (B.4-10)

Union Oil Co. IV (B.11-2)

U.S. A.E.C. IV (B. 1-1,2, 3,27, 28, 29,30; B. 2-l,2;>3; B. 3-3, 4, 5, G, 7, 8, 9, 10;"B. 4-1,2; B. 5-13; B. 6-5; B. 10-10; B.11-12)

Varta A. G. IV (B. .10-31)

Veb Vakutronik •IV (B.3-36)

Western Electric Co. IV (B.11-19)

Zaidan Ilojin Iloguchi Kcnkyu Jo IV (B.10-21) ANNEX

FLOW DIAGRAMS OF HEAVY WATER PRODUCTION PLANTS

Figures in parenthesis show plant number in Table IV. D. 1; FIRST STAGE SECOND STAGE THIRD STAGE (3 IN PARALLELI

A, 8 & C HOT TOWER COLD TOWER

HYDROGEN SULPHIDE DEPLETED IN DEUTERIUM

FEED WATER

COLD SECTION 90°F

DEUTERIUM ENRICHED WATER ID20)

HYDROGEN SULPHIDE ENRICHED IN DEUTERIUM

HOT SECTION 26J°F

DEPLETED WATER

HYDROGEN SULPHIDE ENRICHED WATER GAS FLOW r T0 FINISHING SECTION WATER FLOW

CANADA: Simplified process diagram (2,3) *\trJ*Ó**ì-àì3~?Wve*iw»fi J^T*Hf?trtCt ,&a^ a*^igfa;g'-lfihc**—• W^r^^»*iS. i.'V^ai»'

r~~> Supplementary compressor -On

t

A

1 1 1 1

r"> 1 1 1 ! 1 --I i J Feet) lank d pump Production tonk

FRANCE: Block diagx-am of Lacq facility (4)

araaiafjfiaaag Ill

a % D,o

GERMANY'R. F.rFlowshcet of-German H2S - I-IDO pilot plant (6) IV

Wa, 4 Ml- I

Closed

Open water cycle SWEDEN : Kvarntorp pilot plant. (13) r* ""I r-i n V Feed

CT-I .1/

n , :r t. Product

\ J I-egend Qj •Liquid - (Jail and Vnp<>r Meat llecovcf.i Flow diagram of a SRP GS Unit

Tmic.l WJJ.II- Uiv-r Tr A'.ilcr Ujtiv 0 O'.V. V «feg flslit

V/////////'/////'/_\

Trjln A ^ ! il Train H ^——L*-—T-l—J—, h'astc 4. SI

I'tolaled (n? Rework April IPCÜ » .1 — : mv PLANT Irir.lr.IL'ri (p.- Rrwnrk I < ! t— . (vacuum Dis'.ilt&tion) Occcn.bcr lüS? ||S.v:e4 | n:

F l'LANT I (Electrolytic)

Currently Oneratine j j Dote Shut Pt.wn P%$)

% Indicatali moie % U00 "

History of Operation of SRP GS Plant

• USA : r Savannah River Plant (17)

^WrWlClWMiWIjT - é >r*»*f*wö'"»Äa)stMiM*ei^^ ^t^^ttZF?. r^»[^ »

FIRST STAGE DRIER ANO EXCHANGER SECCNO STAGE FINAL STAGE DjO FORMATION NHJ-MJ NKJ-HJ EXCHANGE NH, OISTILLATION NH , SYNTHESIS GAS „ B0BBm/1) EXCHANGE .EFFLUENT -_-|-||-.|-^--. 21447 Mj 2697 NH,

m__j

HEAVY WATER SOS NH, G.8 NH, O.907 0,0

(73G00) (53.8%1 T I 1 1 i Li r IT

SYNTHESIS, BQ86 m/h Hl | GAS FEEO r 11230) I f Y {45001 ' I 0.605 «hjl 199.8%)

1 NOfE:" 1 f 1 . FÌ.0WSHE ET I spm) IN PARENTHESIS

IS8° NK j- Hz EXCHANGE

70 TONS 0?0/ vr L SYNTHESIS GAS FEED *| L. t 1

CANADA : Chalk River planned pilot plant (20) jj^^Sl^^^sm-s^^ms^^sss^s^^s VII

DjpKUgwalawr colotìfug«

Arrfvfl* d% g

Hxv> -DXJ—, • r-0 I Séparottur

V

Capaci >• Sépoiataur BollitiliBoutfill«« •chaftlillonH,

Mil« a l'air u CZÌ

:FRANCE: Small pilot plant UCMa (21) To SfnlM*li

JJÜ T H c'^)—

T( ,?,K.r ,.„,., „ni M

.1, it..... >V !

plow diagram

Gos mixture (N2+3HZ) . far ommonia synthesis Ammonio ••«»•/production

Final concentration: distinction ot fijmmonia

Heavy woter

Cracking v PURIFICATION ISOTOPE RECOVERY AND FINAL EXCHANGE TREATMENT OF ' PROCESS CATALYST

Schematic arrangement

FRANCE: Mazingarbe heavy water plart ^ ?&a—\ ..-»™ ff* 4 <§ Syntticsegn -,

-4* „XI K- a Amrroniok-Kreislauf é* Sytilhtseyos-Kreistouf c j£~ J7 £M fràte^ Dampfhcitung

ajmxi

a,, a,, un Flussigki-ilvibsitii'iriiT, 1) SilioifN.'l/Aklivkuhlc-Filtcr, cGasri'iriiyuii(|skulniiii,., «MiHllc Kolnnn», r,/bilie Kolonnen, fli» 9i' 5» GiKkflliloi, n, his /i. Fliissigkuilspiitnppii, i Gaskom- : prc-isor. ft,,• fcä V»rrdl!>l>p|iji|ii>r für <|en'ini(|l'" Ammoniak und Amld-I.fiMini|Ph, / Aininniiiiik-Vpriliiitipfrr, "i IPPII» KH- loniicn&tü

GERMANY R. F. .:' Flow diagram of semiindustrial plant ui for the system H2/li

AMMONIA

Sil r

Nl-Ig - HD exchange section

H

33- a~Q- }

-&~

1 TJ u-rj- -fr-

Nllg distillation section

U. K. : Construction John Brown Ltd. Project (29) lo Chemical Plani /"rei/ Waler XI

\ üi/ii/r Cap Plolos Catalyst (ledi.

inox?/;?!1,

jlj•_. I J.\.> GosSupcrheoler

I

Electrolytic Celti .. J-, .Humidifier i • 0, \-l —H //, V-^;i ^Condenser ( lo Higher Stages

Schematic diagram of Trail exchange plant, based on the hydrogen/water system with gas-phase catalysis

Watir tlrluiRI'i I'rtiniry rianl nun»- "" "1 -, 1 J*™, |

Carter n*fiftf p—* »>cJ ilfttr I ™ l I rill r+u>r f'rtiniry 5*l»ni L_J r CT fen.

1 I'ju.rr »--, ! ...I. —riirr t- *—!••) Ci j'Jn*i.-ttj: 1 r r#*.or -•L L ! I„^J T^

Iljnrr I I KIT linai F(f- KvopTfcHim «ml II •Vaniti ni U ? r.i'.tticiim; 0"il f.-..iJlnr IMpr. Rili T/I.k f*;or t rilff , -J" £ ill 1 H. I 0...

CANADA :; Diagram of the Secondary Plant at Trail for Concentrat­ ing D20 by a Cascade of Electrolytic Cells. Trail Plant XII

Cold Columns Cooler

\ UppvrHeal Hydrogen Exchanger N Hoi \y Column

Electric j. Healer •• Calalysl Suspension'' ~ J Lower Heal ^JJ Exchanger

GERMANY It. F. : Diagram of pilot plant, lor the system hydro­ gen/aqueous, catalyst suspension, built by .;.' t Fi-iccli-ich Uhclc G. m. b. II (34)

S " 5 2

+ O I Mixtur« of Nj + 3Hj Mixturo with o.ooisr; D

Compressor

X E FRANCE: 2, 5 t/y pilot plant Toulouse"- Semplified diagram (35) XIV

rifu, \ -i [[ILMI; a Pirni.i*r»riti.il n

1 Ciili'lJlj.-fliiljtf 7 0llMlilicnilUr IrJ Ditl:!i!:«r. intintili Vr.-L'lTifc' £15.' PtlitA T- nrr TT r i Ì -l_i- 1 i i ~tr dittiti. I I' i i

1 te-'iitua •i I '' H

IL.cb'.ldung W.tii j.ii'iNtm

IV- L Vull. -cs-

,t: :, •: '" rh_. KjlJjtilH Cjlj'fiei CJPS.MSW I J—*

c «,»lil'3, a S|r,|.htiE}JI C.iJc g ii GERMANY 11. F. : Block diagram of the Farbwerke Hoechst 4 t/y heavy-water plant based on IT, distillation (38)

?5O0O Nm'Hj/h 5000 Nm'Depleted H:/h to the Arnn ionia Pioni HO Conen 20 ppm "T" I I I 12500Nm'lt?/h [ 7500Hm'HJh, 1 5000 Nm'HJh Hydrogen . HO Cone. 032 N• ' HO Cone. 05ÌN] HOCoiK._3Jj Distillation I Plani I Electrolytic Cels f-,, ", 1 iv,-"-?! r—1 Sfogo 2 •]—•-[ Slago J | reed V/aler !. ... Slag f I Produci HD Conen IN(-300rpm)

INDIA :Combin.ition or walor electrolysis and low-tempera-

ture II2 distillation in Nangal plant. (39) XV

^1 ©T0

P , j£r® ®> rrrj-_'-.rr.' i ?j* L- nirmirr rjj URSS : Side and Top Views of USSR Hydrogen Distillation Pilot Plant A Low Temperature Block, Including Distillation Column and Heat Exchangers operated at temperatures below 80°K 13 Block- containing Heat Exchangers and Filters operat­ ed at temperatures above 80°K (43)

CM

flu«.

r^T""^'^

URSS : Flowsheet of the cycle of the USSR industrial plant (44) £ h® I o J5 ni

to. {3D JP "3

+-> . s = s: C 0» s IID ! o - *> "! "» "! c a O

0) N i—i 1 Zt r *— II in

P -®- 5 ill

'li »! .-"' - Vide U C-f

Rejet

C, c Alimentatici Ci :

r —1 i.—

cìtniil liijiiWf B, a circuii ru/icur 3 C„ : enntlens:ur C. : columi' Il : tmuiltcìir

FRANCE: Soiilom pilot plant

NEW ZEALAND : Flowsheet of the px-ojected plant ir. Warakei XVIII

CONDENSER i 1

STRI PP KD WAT fit 0.0130-. D m.ocoLn/im TO WE» 1 A PRODUCT WATEK SI AT % D 0. 85 LB/IIH

mPUMI

nKllülI-EU 0 FEED STEAM 150 P.ÌIG 0.0113 AT % n WASTE CONDENSATE 202.75')Ln/IIR (S> O.OII.V; i) as.7so L3/im

USA ;l;'low Diagram of Water Distillation Unit of tlie MOW Primary Plant (53)

<"•> f'eod t'/ater «,» / rx 0,-Scrubber H,-Scrubbor

Electrolytic Ccls e -E3- Stage I Conrfenspr Catalyst ^-T

-.ra­ 5/ogrpi ? TT

r— \~5lage 3 V- li CS3-; {TstogTT}—^-?--——--

S/oges 5.....S r I / T 1 Burnerflu; lo Stage 6 \ '-IS-- -J^eWf^St^. ^ I

L /o HigherSlages

NORWAY : The Norsk Plant for Producing D2O by a Combination of Electrolysis of Water and UD- 1120 Catalytic Exchange XX

!.. i,,_.,,,.• .,.,„.. ,,i^,i..Jr.M«..j..i|iju;..--ii-LiuuuJBPaj XXI

*-/o Chom.Plant

Reflux Compressor

Expansion Turbines

Product

SWITZERLAND':' Flow-sheet of hydrogen distillation plant built by the firm Gebrüder Sulzer (41) XXX

0, »l cantiti'*

Ä(Q«i(p'rc OjO)

• — • Idrsgtn« .

— "— • -» —— - Otti^cfla

— •-*— »—.— AMU* 4i »j||»»d«l*m»»U o rtttittfimcnl*

ITALY : Electrolytic .plant at Nera Montoro (Soc. Terni) Lay-out of the fourth stage of an isotopie ex­ (58) change unit

.^t ««-*•*«(»» ''»i _r«, A«KJO "•*• »Am*!*»' 'S***'